Optical modeling of volcanic ash particles using ellipsoids

NASA Astrophysics Data System (ADS)

Merikallio, Sini; Muñoz, Olga; Sundström, Anu-Maija; Virtanen, Timo H.; Horttanainen, Matti; de Leeuw, Gerrit; Nousiainen, Timo

2015-05-01

The single-scattering properties of volcanic ash particles are modeled here by using ellipsoidal shapes. Ellipsoids are expected to improve the accuracy of the retrieval of aerosol properties using remote sensing techniques, which are currently often based on oversimplified assumptions of spherical ash particles. Measurements of the single-scattering optical properties of ash particles from several volcanoes across the globe, including previously unpublished measurements from the Eyjafjallajökull and Puyehue volcanoes, are used to assess the performance of the ellipsoidal particle models. These comparisons between the measurements and the ellipsoidal particle model include consideration of the whole scattering matrix, as well as sensitivity studies on the point of view of the Advanced Along Track Scanning Radiometer (AATSR) instrument. AATSR, which flew on the ENVISAT satellite, offers two viewing directions but no information on polarization, so usually only the phase function is relevant for interpreting its measurements. As expected, ensembles of ellipsoids are able to reproduce the observed scattering matrix more faithfully than spheres. Performance of ellipsoid ensembles depends on the distribution of particle shapes, which we tried to optimize. No single specific shape distribution could be found that would perform superiorly in all situations, but all of the best-fit ellipsoidal distributions, as well as the additionally tested equiprobable distribution, improved greatly over the performance of spheres. We conclude that an equiprobable shape distribution of ellipsoidal model particles is a relatively good, yet enticingly simple, approach for modeling volcanic ash single-scattering optical properties.

Chemistry and Artists' Colors: Part III. Preparation and Properties of Artists' Pigments.

ERIC Educational Resources Information Center

Orna, Mary Virginia

1980-01-01

Describes laboratory methods for synthesizing chrome yellow, prussian blue, and phthalalocyanine blue; reviews chemical properties of artists' pigments including chemical structure and light-scattering properties; and explains how pigments are classified. (CS)

Tip-Enhanced Raman Scattering Microscopy: A Step toward Nanoscale Control of Intrinsic Molecular Properties

NASA Astrophysics Data System (ADS)

Yano, Taka-aki; Hara, Masahiko

2018-06-01

Tip-enhanced Raman scattering microscopy, a family of scanning probe microscopy techniques, has been recognized as a powerful surface analytical technique with both single-molecule sensitivity and angstrom-scale spatial resolution. This review covers the current status of tip-enhanced Raman scattering microscopy in surface and material nanosciences, including a brief history, the basic principles, and applications for the nanoscale characterization of a variety of nanomaterials. The focus is on the recent trend of combining tip-enhanced Raman scattering microscopy with various external stimuli such as pressure, voltage, light, and temperature, which enables the local control of the molecular properties and functions and also enables chemical reactions to be induced on a nanometer scale.

Spectrum of an electromagnetic light wave on scattering from an anisotropic semisoft boundary medium.

PubMed

Wang, Tao; Jiang, Zhenfei; Ji, Xiaoling; Zhao, Daomu

2016-04-01

Spectral shifts and spectral switches of a polychromatic electromagnetic light wave on scattering from an anisotropic semisoft boundary medium are discussed. It is shown that both the property of the incident field and the character of the scattering medium play roles in the change of the spectrum of the far-zone scattered field. It is also shown that the distribution of the far-zone scattered spectrum, including the magnitude of the spectral shift and the direction at which the spectral switch occurs, is rotationally nonsymmetric.

Time-varying phononic crystals

NASA Astrophysics Data System (ADS)

Wright, Derek Warren

The primary objective of this thesis was to gain a deeper understanding of acoustic wave propagation in phononic crystals, particularly those that include materials whose properties can be varied periodically in time. This research was accomplished in three ways. First, a 2D phononic crystal was designed, created, and characterized. Its properties closely matched those determined through simulation. The crystal demonstrated band gaps, dispersion, and negative refraction. It served as a means of elucidating the practicalities of phononic crystal design and construction and as a physical verification of their more interesting properties. Next, the transmission matrix method for analyzing 1D phononic crystals was extended to include the effects of time-varying material parameters. The method was then used to provide a closed-form solution for the case of periodically time-varying material parameters. Some intriguing results from the use of the extended method include dramatically altered transmission properties and parametric amplification. New insights can be gained from the governing equations and have helped to identify the conditions that lead to parametric amplification in these structures. Finally, 2D multiple scattering theory was modified to analyze scatterers with time-varying material parameters. It is shown to be highly compatible with existing multiple scattering theories. It allows the total scattered field from a 2D time-varying phononic crystal to be determined. It was shown that time-varying material parameters significantly affect the phononic crystal transmission spectrum, and this was used to switch an incident monochromatic wave. Parametric amplification can occur under certain circumstances, and this effect was investigated using the closed-form solutions provided by the new 1D method. The complexity of the extended methods grows logarithmically as opposed linearly with existing methods, resulting in superior computational complexity for large numbers of scatterers. Also, since both extended methods provide analytic solutions, they may give further insights into the factors that govern the behaviour of time-varying phononic crystals. These extended methods may now be used to design an active phononic crystal that could demonstrate new or enhanced properties.

Effects of mixing states on the multiple-scattering properties of soot aerosols.

PubMed

Cheng, Tianhai; Wu, Yu; Gu, Xingfa; Chen, Hao

2015-04-20

The radiative properties of soot aerosols are highly sensitive to the mixing states of black carbon particles and other aerosol components. Light absorption properties are enhanced by the mixing state of soot aerosols. Quantification of the effects of mixing states on the scattering properties of soot aerosol are still not completely resolved, especially for multiple-scattering properties. This study focuses on the effects of the mixing state on the multiple scattering of soot aerosols using the vector radiative transfer model. Two types of soot aerosols with different mixing states such as external mixture soot aerosols and internal mixture soot aerosols are studied. Upward radiance/polarization and hemispheric flux are studied with variable soot aerosol loadings for clear and haze scenarios. Our study showed dramatic changes in upward radiance/polarization due to the effects of the mixing state on the multiple scattering of soot aerosols. The relative difference in upward radiance due to the different mixing states can reach 16%, whereas the relative difference of upward polarization can reach 200%. The effects of the mixing state on the multiple-scattering properties of soot aerosols increase with increasing soot aerosol loading. The effects of the soot aerosol mixing state on upwelling hemispheric flux are much smaller than in upward radiance/polarization, which increase with increasing solar zenith angle. The relative difference in upwelling hemispheric flux due to the different soot aerosol mixing states can reach 18% when the solar zenith angle is 75°. The findings should improve our understanding of the effects of mixing states on the optical properties of soot aerosols and their effects on climate. The mixing mechanism of soot aerosols is of critical importance in evaluating the climate effects of soot aerosols, which should be explicitly included in radiative forcing models and aerosol remote sensing.

Modeling ultrasonic transient scattering from biological tissues including their dispersive properties directly in the time domain.

PubMed

Norton, G V; Novarini, J C

2007-06-01

Ultrasonic imaging in medical applications involves propagation and scattering of acoustic waves within and by biological tissues that are intrinsically dispersive. Analytical approaches for modeling propagation and scattering in inhomogeneous media are difficult and often require extremely simplifying approximations in order to achieve a solution. To avoid such approximations, the direct numerical solution of the wave equation via the method of finite differences offers the most direct tool, which takes into account diffraction and refraction. It also allows for detailed modeling of the real anatomic structure and combination/layering of tissues. In all cases the correct inclusion of the dispersive properties of the tissues can make the difference in the interpretation of the results. However, the inclusion of dispersion directly in the time domain proved until recently to be an elusive problem. In order to model the transient signal a convolution operator that takes into account the dispersive characteristics of the medium is introduced to the linear wave equation. To test the ability of this operator to handle scattering from localized scatterers, in this work, two-dimensional numerical modeling of scattering from an infinite cylinder with physical properties associated with biological tissue is calculated. The numerical solutions are compared with the exact solution synthesized from the frequency domain for a variety of tissues having distinct dispersive properties. It is shown that in all cases, the use of the convolutional propagation operator leads to the correct solution for the scattered field.

Long-term variability of aerosol optical properties and radiative effects in Northern Finland

NASA Astrophysics Data System (ADS)

Lihavainen, Heikki; Hyvärinen, Antti; Asmi, Eija; Hatakka, Juha; Viisanen, Yrjö

2017-04-01

We introduce long term dataset of aerosol scattering and absorption properties and combined aerosol optical properties measured in Pallas Atmosphere-Ecosystem Supersite in Norhern Finland. The station is located 170 km north of the Arctic Circle. The station is affected by both pristine Arctic air masses as well as long transported air pollution from northern Europe. We studied the optical properties of aerosols and their radiative effects in continental and marine air masses, including seasonal cycles and long-term trends. The average (median) scattering coefficient, backscattering fraction, absorption coefficient and single scattering albedo at the wavelength of 550 nm were 7.9 (4.4) 1/Mm, 0.13 (0.12), 0.74 (0.35) 1/Mm and 0.92 (0.93), respectively. We observed clear seasonal cycles in these variables, the scattering coefficient having high values during summer and low in fall, and absorption coefficient having high values during winter and low in fall. We found that the high values of the absorption coefficient and low values of the single scattering albedo were related to continental air masses from lower latitudes. These aerosols can induce an additional effect on the surface albedo and melting of snow. We observed the signal of the Arctic haze in marine (northern) air masses during March and April. The haze increased the value of the absorption coefficient by almost 80% and that of the scattering coefficient by about 50% compared with the annual-average values. We did not observe any long-term trend in the scattering coefficient, while our analysis showed a clear decreasing trend in the backscattering fraction and scattering Ångström exponent during winter. We also observed clear relationship with temperature and aerosol scattering coefficient. We will present also how these different features affects to aerosol direct radiative forcing.

Investigating the Spectral Dependence of Biomass Burning Aerosol Optical Properties

NASA Astrophysics Data System (ADS)

Odwuor, A.; Corr, C.; Pusede, S.

2016-12-01

Aerosol optical properties, such as light absorption and scattering, are important for understanding how aerosols affect the global radiation budget and for comparison with data gathered from remote sensing. It has been established that the optical properties of aerosols are wavelength dependent, although some remote sensing measurements do not consider this. Airborne measurements of these optical properties were used to calculate the absorption Angstrom exponent, a parameter that characterizes the wavelength dependence of light absorption by aerosols, and single scattering albedo, which measures the relative magnitude of light scattering to total extinction (scattering and absorption combined). Aerosols produced by biomass burning in Saskatchewan, Canada in July 2008 and a forest fire in Southern California, U.S. in June 2016 were included in this analysis. These wildfires were sampled by the NASA DC-8 aircraft during the Arctic Research of the Composition of the Troposphere from Aircraft and Satellites (ARCTAS) and NASA Student Airborne Research Program (SARP) missions, respectively. Aerosol absorption was measured using a particle soot photometer (PSAP) at 470, 532 and 660 nm. Scattering was measured using a 3-wavelength (450, 550 and 700 nm) nephelometer. Absorption Angstrom exponents were calculated at 470 and 660 nm and single scattering albedos were calculated at 450 and 550 nm. Results of this study indicate that disregarding the wavelength dependence of organic aerosol can understate the positive radiative forcing (warming) associated with aerosol absorption.

Application of conditional simulation of heterogeneous rock properties to seismic scattering and attenuation analysis in gas hydrate reservoirs

NASA Astrophysics Data System (ADS)

Huang, Jun-Wei; Bellefleur, Gilles; Milkereit, Bernd

2012-02-01

We present a conditional simulation algorithm to parameterize three-dimensional heterogeneities and construct heterogeneous petrophysical reservoir models. The models match the data at borehole locations, simulate heterogeneities at the same resolution as borehole logging data elsewhere in the model space, and simultaneously honor the correlations among multiple rock properties. The model provides a heterogeneous environment in which a variety of geophysical experiments can be simulated. This includes the estimation of petrophysical properties and the study of geophysical response to the heterogeneities. As an example, we model the elastic properties of a gas hydrate accumulation located at Mallik, Northwest Territories, Canada. The modeled properties include compressional and shear-wave velocities that primarily depend on the saturation of hydrate in the pore space of the subsurface lithologies. We introduce the conditional heterogeneous petrophysical models into a finite difference modeling program to study seismic scattering and attenuation due to multi-scale heterogeneity. Similarities between resonance scattering analysis of synthetic and field Vertical Seismic Profile data reveal heterogeneity with a horizontal-scale of approximately 50 m in the shallow part of the gas hydrate interval. A cross-borehole numerical experiment demonstrates that apparent seismic energy loss can occur in a pure elastic medium without any intrinsic attenuation of hydrate-bearing sediments. This apparent attenuation is largely attributed to attenuative leaky mode propagation of seismic waves through large-scale gas hydrate occurrence as well as scattering from patchy distribution of gas hydrate.

Quantum Monte Carlo calculation of neutral-current ν -12C inclusive quasielastic scattering

NASA Astrophysics Data System (ADS)

Lovato, A.; Gandolfi, S.; Carlson, J.; Lusk, Ewing; Pieper, Steven C.; Schiavilla, R.

2018-02-01

Quasielastic neutrino scattering is an important aspect of the experimental program to study fundamental neutrino properties including neutrino masses, mixing angles, mass hierarchy, and charge-conjugation parity (CP)- violating phase. Proper interpretation of the experiments requires reliable theoretical calculations of neutrino-nucleus scattering. In this paper we present calculations of response functions and cross sections by neutral-current scattering of neutrinos off 12C. These calculations are based on realistic treatments of nuclear interactions and currents, the latter including the axial, vector, and vector-axial interference terms crucial for determining the difference between neutrino and antineutrino scattering and the CP-violating phase. We find that the strength and energy dependence of two-nucleon processes induced by correlation effects and interaction currents are crucial in providing the most accurate description of neutrino-nucleus scattering in the quasielastic regime.

Optical Sensors Using Stimulated Brillouin Scattering

NASA Technical Reports Server (NTRS)

Christensen, Caleb A (Inventor); Zavriyev, Anton (Inventor)

2017-01-01

A method for enhancing a sensitivity of an optical sensor having an optical cavity counter-propagates beams of pump light within the optical cavity to produce scattered light based on Stimulated Brillouin Scattering (SBS). The properties of the pump light are selected to generate fast-light conditions for the scattered light, such that the scattered light includes counter-propagating beams of fast light. The method prevents the pump light from resonating within the optical cavity, while allowing the scattered light to resonate within the optical cavity. At least portions of the scattered light are interfered outside of the optical cavity to produce a beat note for a measurement of the optical sensor. The disclosed method is particularly applicable to optical gyroscopes.

X-ray data booklet. Revision

DOE Office of Scientific and Technical Information (OSTI.GOV)

Vaughan, D.

A compilation of data is presented. Included are properties of the elements, electron binding energies, characteristic x-ray energies, fluorescence yields for K and L shells, Auger energies, energy levels for hydrogen-, helium-, and neonlike ions, scattering factors and mass absorption coefficients, and transmission bands of selected filters. Also included are selected reprints on scattering processes, x-ray sources, optics, x-ray detectors, and synchrotron radiation facilities. (WRF)

Comprehensive Understanding for Vegetated Scene Radiance Relationships

NASA Technical Reports Server (NTRS)

Kimes, D. S.; Deering, D. W.

1984-01-01

The improvement of our fundamental understanding of the dynamics of directional scattering properties of vegetation canopies through analysis of field data and model simulation data is discussed. Directional reflectance distributions spanning the entire existance hemisphere were measured in two field studies; one using a Mark III 3-band radiometer and one using rapid scanning bidirectional field instrument called PARABOLA. Surfaces measured included corn, soybeans, bare soils, grass lawn, orchard grass, alfalfa, cotton row crops, plowed field, annual grassland, stipa grass, hard wheat, salt plain shrubland, and irrigated wheat. Some structural and optical measurements were taken. Field data show unique reflectance distributions ranging from bare soil to complete vegetation canopies. Physical mechanisms causing these trends are proposed based on scattering properties of soil and vegetation. Soil exhibited a strong backscattering peak toward the Sun. Complete vegetation exhibited a bowl distribution with the minimum reflectance near nadir. Incomplete vegetation canopies show shifting of the minimum reflectance off of nadir in the forward scattering direction because both the scattering properties or the vegetation and soil are observed.

Method and apparatus for determining the physical properties of materials using dynamic light scattering techniques

NASA Technical Reports Server (NTRS)

Dhadwal, Harbans S. (Inventor)

1992-01-01

A system for determining the physical properties of materials through the use of dynamic light scattering is disclosed. The system includes a probe, a laser source for directing a laser beam into the probe, and a photodetector for converting scattered light detected by the probe into electrical signals. The probe includes at least one optical fiber connected to the laser source and a second optical fiber connected to the photodetector. Each of the fibers may adjoin a gradient index microlens which is capable of providing a collimated laser beam into a scattering medium. The position of the second optical fiber with respect to the optical axis of the probe determines whether homodyne or self-beating detection is provided. Self-beating detection may be provided without a gradient index microlens. This allows a very small probe to be constructed which is insertable through a hypodermic needle or the like into a droplet extending from such a needle. A method of detecting scattered light through the use of a collimated, Gaussian laser beam is also provided. A method for controlling the waist and divergence of the optical field emanating from the free end of an optical fiber is also provided.

Quantum Monte Carlo calculation of neutral-current ν - C 12 inclusive quasielastic scattering

DOE PAGES

Lovato, A.; Gandolfi, S.; Carlson, J.; ...

2018-02-28

Quasielastic neutrino scattering is an important aspect of the experimental program to study fundamental neutrino properties including neutrino masses, mixing angles, the mass hierarchy and CP-violating phase. Proper interpretation of the experiments requires reliable theoretical calculations of neutrino-nucleus scattering. In this paper we present calculations of response functions and cross sections by neutral-current scattering of neutrinos offmore » $$^{12}$$C. These calculations are based on realistic treatments of nuclear interactions and currents, the latter including the axial, vector, and vector-axial interference terms crucial for determining the difference between neutrino and anti-neutrino scattering and the CP-violating phase. Here in this paper, we find that the strength and energy-dependence of two-nucleon processes induced by correlation effects and interaction currents are crucial in providing the most accurate description of neutrino-nucleus scattering in the quasielastic regime.« less

Quantum Monte Carlo calculation of neutral-current ν - C 12 inclusive quasielastic scattering

DOE Office of Scientific and Technical Information (OSTI.GOV)

Lovato, A.; Gandolfi, S.; Carlson, J.

Quasielastic neutrino scattering is an important aspect of the experimental program to study fundamental neutrino properties including neutrino masses, mixing angles, the mass hierarchy and CP-violating phase. Proper interpretation of the experiments requires reliable theoretical calculations of neutrino-nucleus scattering. In this paper we present calculations of response functions and cross sections by neutral-current scattering of neutrinos offmore » $$^{12}$$C. These calculations are based on realistic treatments of nuclear interactions and currents, the latter including the axial, vector, and vector-axial interference terms crucial for determining the difference between neutrino and anti-neutrino scattering and the CP-violating phase. Here in this paper, we find that the strength and energy-dependence of two-nucleon processes induced by correlation effects and interaction currents are crucial in providing the most accurate description of neutrino-nucleus scattering in the quasielastic regime.« less

Calculation of optical properties of dental composites as a basis for determining color impression and penetration depth of laser light

NASA Astrophysics Data System (ADS)

Weniger, Kirsten K.; Muller, Gerhard J.

2005-03-01

In order to achieve esthetic dental restorations, there should be no visible difference between restorative material and treated teeth. This requires a match of the optical properties of both restorative material and natural teeth. These optical properties are determined by absorption and scattering of light emerging not only on the surface but also inside the material. Investigating different dental composites in several shades, a method has been developed to calculate the optical parameters absorption coefficient μa, scattering coefficient μs, anisotropy factor g and reduced scattering coefficient μs'. The method includes sample preparation and measurements of transmittance and reflectance in an integrating sphere spectrometer, followed by inverse Monte Carlo simulations. Determination of optical properties is more precise and comprehensive than with the previously used Kubelka Munk theory because scattering can be looked at separated into pure scattering with the scattering coefficient μs and its direction with the anisotropy factor g. Moreover the use of the inverse Monte Carlo simulation not only minimizes systematic errors and considers the scattering phase function, but also takes into account the measuring geometry. The compilation of a data pool of optical parameters now enables the application of further calculation models as a basis for optimization of the composition of new materials. For example, a prediction of the general color impression for multiple layers can be carried out as well as the calculation of the wavelength dependent penetration depths of light with regard to photo polymerization. Further applications are possible in the area of laser ablation.

MODELING POROUS DUST GRAINS WITH BALLISTIC AGGREGATES. II. LIGHT SCATTERING PROPERTIES

DOE Office of Scientific and Technical Information (OSTI.GOV)

Shen Yue; Draine, B. T.; Johnson, Eric T.

2009-05-10

We study the light scattering properties of random ballistic aggregates constructed in Shen et al. Using the discrete-dipole approximation, we compute the scattering phase function and linear polarization for random aggregates with various sizes and porosities, and with two different compositions: 100% silicate and 50% silicate +50% graphite. We investigate the dependence of light scattering properties on wavelength, cluster size, and porosity using these aggregate models. We find that while the shape of the phase function depends mainly on the size parameter of the aggregates, the linear polarization depends on both the size parameter and the porosity of the aggregates,more » with increasing degree of polarization as the porosity increases. Contrary to previous studies, we argue that the monomer size has negligible effects on the light scattering properties of ballistic aggregates, as long as the constituent monomer is smaller than the incident wavelength up to 2{pi}a {sub 0}/{lambda} {approx} 1.6 where a {sub 0} is the monomer radius. Previous claims for such monomer size effects are in fact the combined effects of size parameter and porosity. Finally, we present aggregate models that can reproduce the phase function and polarization of scattered light from the AU Mic debris disk and from cometary dust, including the negative polarization observed for comets at scattering angles 160 deg. {approx}< {theta} < 180 deg. These aggregates have moderate porosities, P{approx}0.6, and are of sub-{mu}m size for the debris disk case, or {mu}m size for the comet case.« less

Abstracts of papers presented at the Eleventh International Laser Radar Conference

NASA Technical Reports Server (NTRS)

1982-01-01

Abstracts of 39 papers discuss measurements of properties from the Earth's ocean surface to the mesosphere, made with techniques ranging from elastic and inelastic scattering to Doppler shifts and differential absorption. Topics covered include: (1) middle atmospheric measurements; (2) meteorological parameters: temperature, density, humidity; (3) trace gases by Raman and DIAL techniques; (4) techniques and technology; (5) plume dispersion; (6) boundary layer dynamics; (7) wind measurements; visibility and aerosol properties; and (9) multiple scattering, clouds, and hydrometers.

The extraordinary radar echoes from Europa, Ganymede, and Callisto: A geological perspective

USGS Publications Warehouse

Ostro, S.J.; Shoemaker, E.M.

1990-01-01

This outline of plausible geologic explanations for the icy Galilean satellites' radar properties takes into consideration electromagnetic scattering models for the echoes, available empirical and theoretical information about regolith formation, and ice physics. The strange radar signatures arise because (1) ice is electrically different from silicates and/or (2) icy regoliths contain bulk-density (and hence refractive-index) structures absent within silicate regoliths. Ice's relatively high radar-frequency transparency compared with that of silicates permits longer photon path lengths, deeper radar sounding, and a greater number of scattering events. Consequently, scattering mechanisms that cannot contribute significantly to lunar echoes can dominate icy-satellite echoes. Possible phenomena unique to icy regoliths include (1) smoothing out of discontinuities between solid ejecta fragments and more porous surroundings under the action of thermal annealing to form refraction-scattering (RS) "lenses" and (2) formation of density enhancements in the shape of crater floors that result in RS and/or total internal reflection (TIR). In either case, high-order multiple scattering is more likely to be responsible for the echoes than low-order scattering. Radar/radio observations can constrain the order of the scattering and the scale of the structures responsible for the echoes but might not determine whether TIR or RS dominates the scattering. Multiwavelength investigations of the degree of correlation between radar properties and geologic terrain type should prove most useful, because inter- and intrasatellite variations in radar properties probably correspond to variations in ice purity, regolith thickness, and regolith thermal history and age. ?? 1990.

Optical characterization of fritted glass for architectural applications

NASA Astrophysics Data System (ADS)

Jonsson, Jacob C.; Rubin, Michael D.; Nilsson, Annica M.; Jonsson, Andreas; Roos, Arne

2009-04-01

Fritted glass is commonly used as a light diffusing element in modern buildings. Traditionally it has been used for aesthetic purposes but it can also be used for energy savings by incorporating it in novel daylighting systems? To answer such questions the light scattering properties must be properly characterized. This paper contains measurements of different varieties of fritted glass, ranging from the simplest direct-hemispherical measurements to angle-resolved goniometer measurements. Modeling the light scattering to obtain the full bidirectional scattering distribution function (BSDF) extends the measured data, making it useful in simulation programs such as Window 6 and Radiance. Surface profilometry results and SEM micrographs are included to demonstrate the surface properties of the samples studied.

Quasiparticle Properties of a Mobile Impurity in a Bose-Einstein Condensate.

PubMed

Christensen, Rasmus Søgaard; Levinsen, Jesper; Bruun, Georg M

2015-10-16

We develop a systematic perturbation theory for the quasiparticle properties of a single impurity immersed in a Bose-Einstein condensate. Analytical results are derived for the impurity energy, effective mass, and residue to third order in the impurity-boson scattering length. The energy is shown to depend logarithmically on the scattering length to third order, whereas the residue and the effective mass are given by analytical power series. When the boson-boson scattering length equals the boson-impurity scattering length, the energy has the same structure as that of a weakly interacting Bose gas, including terms of the Lee-Huang-Yang and fourth order logarithmic form. Our results, which cannot be obtained within the canonical Fröhlich model of an impurity interacting with phonons, provide valuable benchmarks for many-body theories and for experiments.

Equivalence of internal and external mixture schemes of single scattering properties in vector radiative transfer

PubMed Central

Mukherjee, Lipi; Zhai, Peng-Wang; Hu, Yongxiang; Winker, David M.

2018-01-01

Polarized radiation fields in a turbid medium are influenced by single-scattering properties of scatterers. It is common that media contain two or more types of scatterers, which makes it essential to properly mix single-scattering properties of different types of scatterers in the vector radiative transfer theory. The vector radiative transfer solvers can be divided into two basic categories: the stochastic and deterministic methods. The stochastic method is basically the Monte Carlo method, which can handle scatterers with different scattering properties explicitly. This mixture scheme is called the external mixture scheme in this paper. The deterministic methods, however, can only deal with a single set of scattering properties in the smallest discretized spatial volume. The single-scattering properties of different types of scatterers have to be averaged before they are input to deterministic solvers. This second scheme is called the internal mixture scheme. The equivalence of these two different mixture schemes of scattering properties has not been demonstrated so far. In this paper, polarized radiation fields for several scattering media are solved using the Monte Carlo and successive order of scattering (SOS) methods and scattering media contain two types of scatterers: Rayleigh scatterers (molecules) and Mie scatterers (aerosols). The Monte Carlo and SOS methods employ external and internal mixture schemes of scatterers, respectively. It is found that the percentage differences between radiances solved by these two methods with different mixture schemes are of the order of 0.1%. The differences of Q/I, U/I, and V/I are of the order of 10−5 ~ 10−4, where I, Q, U, and V are the Stokes parameters. Therefore, the equivalence between these two mixture schemes is confirmed to the accuracy level of the radiative transfer numerical benchmarks. This result provides important guidelines for many radiative transfer applications that involve the mixture of different scattering and absorptive particles. PMID:29047543

Parametric amplification and bidirectional invisibility in PT -symmetric time-Floquet systems

NASA Astrophysics Data System (ADS)

Koutserimpas, Theodoros T.; Alù, Andrea; Fleury, Romain

2018-01-01

Parity-time (PT )-symmetric wave devices, which exploit balanced interactions between material gain and loss, exhibit extraordinary properties, including lasing and flux-conserving scattering processes. In a seemingly different research field, periodically driven systems, also known as time-Floquet systems, have been widely studied as a relevant platform for reconfigurable active wave control and manipulation. In this article, we explore the connection between PT -symmetry and parametric time-Floquet systems. Instead of relying on material gain, we use parametric amplification by considering a time-periodic modulation of the refractive index at a frequency equal to twice the incident signal frequency. We show that the scattering from a simple parametric slab, whose dynamics follows the Mathieu equation, can be described by a PT -symmetric scattering matrix, whose PT -breaking threshold corresponds to the Mathieu instability threshold. By combining different parametric slabs modulated out of phase, we create PT -symmetric time-Floquet systems that feature exceptional scattering properties, such as coherent perfect absorption (CPA)-laser operation and bidirectional invisibility. These bidirectional properties, rare for regular PT -symmetric systems, are related to a compensation of parametric amplification due to multiple scattering between two parametric systems modulated with a phase difference.

Scattering properties of normal and cancerous tissues from human stomach based on phase-contrast microscope

NASA Astrophysics Data System (ADS)

Zhang, Hui; Li, Zhifang; Li, Hui

2012-12-01

In order to study scattering properties of normal and cancerous tissues from human stomach, we collect images for human gastric specimens by using phase-contrast microscope. The images were processed by the way of mathematics morphology. The equivalent particle size distribution of tissues can be obtained. Combining with Mie scattering theory, the scattering properties of tissues can be calculated. Assume scattering of light in biological tissue can be seen as separate scattering events by different particles, total scattering properties can be equivalent to as scattering sum of particles with different diameters. The results suggest that scattering coefficient of the cancerous tissue is significantly higher than that of normal tissue. The scattering phase function is different especially in the backscattering area. Those are significant clinical benefits to diagnosis cancerous tissue

PHIPS-HALO: the airborne Particle Habit Imaging and Polar Scattering probe - Part 1: Design and operation

NASA Astrophysics Data System (ADS)

Abdelmonem, Ahmed; Järvinen, Emma; Duft, Denis; Hirst, Edwin; Vogt, Steffen; Leisner, Thomas; Schnaiter, Martin

2016-07-01

The number and shape of ice crystals present in mixed-phase and ice clouds influence the radiation properties, precipitation occurrence and lifetime of these clouds. Since clouds play a major role in the climate system, influencing the energy budget by scattering sunlight and absorbing heat radiation from the earth, it is necessary to investigate the optical and microphysical properties of cloud particles particularly in situ. The relationship between the microphysics and the single scattering properties of cloud particles is usually obtained by modelling the optical scattering properties from in situ measurements of ice crystal size distributions. The measured size distribution and the assumed particle shape might be erroneous in case of non-spherical ice particles. There is a demand to obtain both information correspondently and simultaneously for individual cloud particles in their natural environment. For evaluating the average scattering phase function as a function of ice particle habit and crystal complexity, in situ measurements are required. To this end we have developed a novel airborne optical sensor (PHIPS-HALO) to measure the optical properties and the corresponding microphysical parameters of individual cloud particles simultaneously. PHIPS-HALO has been tested in the AIDA cloud simulation chamber and deployed in mountain stations as well as research aircraft (HALO and Polar 6). It is a successive version of the laboratory prototype instrument PHIPS-AIDA. In this paper we present the detailed design of PHIPS-HALO, including the detection mechanism, optical design, mechanical construction and aerodynamic characterization.

Bio-physical modeling of time-resolved forward scattering by Listeria colonies

NASA Astrophysics Data System (ADS)

Bae, Euiwon; Banada, Padmapriya P.; Bhunia, Arun K.; Hirleman, E. Daniel

2006-10-01

We have developed a detection system and associated protocol based on optical forward scattering where the bacterial colonies of various species and strains growing on solid nutrient surfaces produced unique scatter signatures. The aim of the present investigation was to develop a bio-physical model for the relevant phenomena. In particular, we considered time-varying macroscopic morphological properties of the growing colonies and modeled the scattering using scalar diffraction theory. For the present work we performed detailed studies with three species of Listeria; L. innocua, L. monocytogenes, and L. ivanovii. The baseline experiments involved cultures grown on brain heart infusion (BHI) agar and the scatter images were captured every six hours for an incubation period of 42 hours. The morphologies of the colonies were studied by phase contrast microscopy, including measurement of the diameter of the colony. Growth curves, represented by colony diameter as a function of time, were compared with the time-evolution of scattering signatures. Similar studies were carried out with L. monocytogenes grown on different substrates. Non-dimensionalizing incubation time in terms of the time to reach stationary phase was effective in reducing the dimensionality of the model. Bio-physical properties of the colony such as diameter, bacteria density variation, surface curvature/profile, and transmission coefficient are important parameters in predicting the features of the forward scattering signatures. These parameters are included in a baseline model that treats the colony as a concentric structure with radial variations in phase modulation. In some cases azimuthal variations and random phase inclusions were included as well. The end result is a protocol (growth media, incubation time and conditions) that produces reproducible and distinguishable scatter patterns for a variety of harmful food borne pathogens in a short period of time. Further, the bio-physical model we developed is very effective in predicting the dominant features of the scattering signatures required by the identification process and will be effective for informing further improvements in the instrumentation.

Spin-scattering rates in metallic thin films measured by ferromagnetic resonance damping enhanced by spin-pumping

DOE Office of Scientific and Technical Information (OSTI.GOV)

Boone, C. T.; Shaw, J. M.; Nembach, H. T.

2015-06-14

We determined the spin-transport properties of Pd and Pt thin films by measuring the increase in ferromagnetic resonance damping due to spin-pumping in ferromagnetic (FM)-nonferromagnetic metal (NM) multilayers with varying NM thicknesses. The increase in damping with NM thickness depends strongly on both the spin- and charge-transport properties of the NM, as modeled by diffusion equations that include both momentum- and spin-scattering parameters. We use the analytical solution to the spin-diffusion equations to obtain spin-diffusion lengths for Pt and Pd. By measuring the dependence of conductivity on NM thickness, we correlate the charge- and spin-transport parameters, and validate the applicabilitymore » of various models for momentum-scattering and spin-scattering rates in these systems: constant, inverse-proportional (Dyakanov-Perel), and linear-proportional (Elliot-Yafet). We confirm previous reports that the spin-scattering time appears to be shorter than the momentum scattering time in Pt, and the Dyakanov-Perel-like model is the best fit to the data.« less

Spin-orbit scattering visualized in quasiparticle interference

NASA Astrophysics Data System (ADS)

Kohsaka, Y.; Machida, T.; Iwaya, K.; Kanou, M.; Hanaguri, T.; Sasagawa, T.

2017-03-01

In the presence of spin-orbit coupling, electron scattering off impurities depends on both spin and orbital angular momentum of electrons—spin-orbit scattering. Although some transport properties are subject to spin-orbit scattering, experimental techniques directly accessible to this effect are limited. Here we show that a signature of spin-orbit scattering manifests itself in quasiparticle interference (QPI) imaged by spectroscopic-imaging scanning tunneling microscopy. The experimental data of a polar semiconductor BiTeI are well reproduced by numerical simulations with the T -matrix formalism that include not only scalar scattering normally adopted but also spin-orbit scattering stronger than scalar scattering. To accelerate the simulations, we extend the standard efficient method of QPI calculation for momentum-independent scattering to be applicable even for spin-orbit scattering. We further identify a selection rule that makes spin-orbit scattering visible in the QPI pattern. These results demonstrate that spin-orbit scattering can exert predominant influence on QPI patterns and thus suggest that QPI measurement is available to detect spin-orbit scattering.

Closed-loop multiple-scattering imaging with sparse seismic measurements

NASA Astrophysics Data System (ADS)

Berkhout, A. J. Guus

2018-03-01

In the theoretical situation of noise-free, complete data volumes (`perfect data'), seismic data matrices are fully filled and multiple-scattering operators have the minimum-phase property. Perfect data allow direct inversion methods to be successful in removing surface and internal multiple scattering. Moreover, under these perfect data conditions direct source wavefields realize complete illumination (no irrecoverable shadow zones) and, therefore, primary reflections (first-order response) can provide us with the complete seismic image. However, in practice seismic measurements always contain noise and we never have complete data volumes at our disposal. We actually deal with sparse data matrices that cannot be directly inverted. The message of this paper is that in practice multiple scattering (including source ghosting) must not be removed but must be utilized. It is explained that in the real world we badly need multiple scattering to fill the illumination gaps in the subsurface. It is also explained that the proposed multiple-scattering imaging algorithm gives us the opportunity to decompose both the image and the wavefields into order-based constituents, making the multiple scattering extension easy to apply. Last but not least, the algorithm allows us to use the minimum-phase property to validate and improve images in an objective way.

On the performance of infrared sensors in earth observations

NASA Technical Reports Server (NTRS)

Johnson, L. F.

1972-01-01

The performance of infrared sensing systems is dependent upon the radiative properties of targets in addition to constraints imposed by system components. The unclassified state-of-the-art of infrared system performance figures is reviewed to indicate the relevance to system performance of target radiative properties. A theory of rough surface scattering is developed which allows the formulation of the reflective characteristics of extended targets. The thermal radiation emission from extended targets is formulated on the basis of internal radiation characteristics of natural materials and the transmissive scattering effects at the surface. Finally, the total radiative characteristics may be expressed as functions of material properties and incident and received directions, although the expressions are extremely complex functions and do not account for the effects of shadowing or multiple scattering. It is believed that the theory may be extended to include these effects and to incorporate the local radii of curvature of the surface.

Feasibility of interstitial diffuse optical tomography using cylindrical diffusing fiber for prostate PDT

PubMed Central

Liang, Xing; Wang, Ken Kang-Hsin; Zhu, Timothy C.

2013-01-01

Interstitial diffuse optical tomography (DOT) has been used to characterize spatial distribution of optical properties for prostate photodynamic therapy (PDT) dosimetry. We have developed an interstitial DOT method using cylindrical diffuse fibers (CDFs) as light sources, so that the same light sources can be used for both DOT measurement and PDT treatment. In this novel interstitial CDF-DOT method, absolute light fluence per source strength (in unit of 1/cm2) is used to separate absorption and scattering coefficients. A mathematical phantom and a solid prostate phantom including anomalies with known optical properties were used, respectively, to test the feasibility of reconstructing optical properties using interstitial CDF-DOT. Three dimension spatial distributions of the optical properties were reconstructed for both scenarios. Our studies show that absorption coefficient can be reliably extrapolated while there are some cross talks between absorption and scattering properties. Even with the suboptimal reduced scattering coefficients, the reconstructed light fluence rate agreed with the measured values to within ±10%, thus the proposed CDF-DOT allows greatly improved light dosimetry calculation for interstitial PDT. PMID:23629149

Diffuse Surface Scattering in the Plasmonic Resonances of Ultralow Electron Density Nanospheres.

PubMed

Monreal, R Carmina; Antosiewicz, Tomasz J; Apell, S Peter

2015-05-21

Localized surface plasmon resonances (LSPRs) have recently been identified in extremely diluted electron systems obtained by doping semiconductor quantum dots. Here, we investigate the role that different surface effects, namely, electronic spill-out and diffuse surface scattering, play in the optical properties of these ultralow electron density nanosystems. Diffuse scattering originates from imperfections or roughness at a microscopic scale on the surface. Using an electromagnetic theory that describes this mechanism in conjunction with a dielectric function including the quantum size effect, we find that the LSPRs show an oscillatory behavior in both position and width for large particles and a strong blue shift in energy and an increased width for smaller radii, consistent with recent experimental results for photodoped ZnO nanocrystals. We thus show that the commonly ignored process of diffuse surface scattering is a more important mechanism affecting the plasmonic properties of ultralow electron density nanoparticles than the spill-out effect.

A New Way to Measure Cirrus Ice Water Content by Using Ice Raman Scatter with Raman Lidar

NASA Technical Reports Server (NTRS)

Wang, Zhien; Whiteman, David N.; Demoz, Belay; Veselovskii, Igor

2004-01-01

High and cold cirrus clouds mainly contain irregular ice crystals, such as, columns, hexagonal plates, bullet rosettes, and dendrites, and have different impacts on the climate system than low-level clouds, such as stratus, stratocumulus, and cumulus. The radiative effects of cirrus clouds on the current and future climate depend strongly on cirrus cloud microphysical properties including ice water content (IWC) and ice crystal sizes, which are mostly an unknown aspect of cinus clouds. Because of the natural complexity of cirrus clouds and their high locations, it is a challenging task to get them accurately by both remote sensing and in situ sampling. This study presents a new method to remotely sense cirrus microphysical properties by using ice Raman scatter with a Raman lidar. The intensity of Raman scattering is fundamentally proportional to the number of molecules involved. Therefore, ice Raman scattering signal provides a more direct way to measure IWC than other remote sensing methods. Case studies show that this method has the potential to provide essential information of cirrus microphysical properties to study cloud physical processes in cirrus clouds.

The single scattering properties of the aerosol particles as aggregated spheres

NASA Astrophysics Data System (ADS)

Wu, Y.; Gu, X.; Cheng, T.; Xie, D.; Yu, T.; Chen, H.; Guo, J.

2012-08-01

The light scattering and absorption properties of anthropogenic aerosol particles such as soot aggregates are complicated in the temporal and spatial distribution, which introduce uncertainty of radiative forcing on global climate change. In order to study the single scattering properties of anthorpogenic aerosol particles, the structures of these aerosols such as soot paticles and soot-containing mixtures with the sulfate or organic matter, are simulated using the parallel diffusion limited aggregation algorithm (DLA) based on the transmission electron microscope images (TEM). Then, the single scattering properties of randomly oriented aerosols, such as scattering matrix, single scattering albedo (SSA), and asymmetry parameter (AP), are computed using the superposition T-matrix method. The comparisons of the single scattering properties of these specific types of clusters with different morphological and chemical factors such as fractal parameters, aspect ratio, monomer radius, mixture mode and refractive index, indicate that these different impact factors can respectively generate the significant influences on the single scattering properties of these aerosols. The results show that aspect ratio of circumscribed shape has relatively small effect on single scattering properties, for both differences of SSA and AP are less than 0.1. However, mixture modes of soot clusters with larger sulfate particles have remarkably important effects on the scattering and absorption properties of aggregated spheres, and SSA of those soot-containing mixtures are increased in proportion to the ratio of larger weakly absorbing attachments. Therefore, these complex aerosols come from man made pollution cannot be neglected in the aerosol retrievals. The study of the single scattering properties on these kinds of aggregated spheres is important and helpful in remote sensing observations and atmospheric radiation balance computations.

Inversion of scattered radiance horizon profiles for gaseous concentrations and aerosol parameters

NASA Technical Reports Server (NTRS)

Malchow, H. L.; Whitney, C. K.

1977-01-01

Techniques have been developed and used to invert limb scan measurements for vertical profiles of atmospheric state parameters. The parameters which can be found are concentrations of Rayleigh scatters, ozone, NO2, and aerosols, and aerosol physical properties including a Junge-size distribution parameter and real and imaginary parts of the index of refraction.

Optical properties of selected components of mineral dust aerosol processed with organic acids and humic material

NASA Astrophysics Data System (ADS)

Alexander, Jennifer M.; Grassian, V. H.; Young, M. A.; Kleiber, P. D.

2015-03-01

Visible light scattering phase function and linear polarization profiles of mineral dust components processed with organic acids and humic material are measured, and results are compared to T-matrix simulations of the scattering properties. Processed samples include quartz mixed with humic material, and calcite reacted with acetic and oxalic acids. Clear differences in light scattering properties are observed for all three processed samples when compared to the unprocessed dust or organic salt products. Results for quartz processed with humic acid sodium salt (NaHA) indicate the presence of both internally mixed quartz-NaHA particles and externally mixed NaHA aerosol. Simulations of light scattering suggest that the processed quartz particles become more moderate in shape due to the formation of a coating of humic material over the mineral core. Experimental results for calcite reacted with acetic acid are consistent with an external mixture of calcite and the reaction product, calcium acetate. Modeling of the light scattering properties does not require any significant change to the calcite particle shape distribution although morphology changes cannot be ruled out by our data. It is expected that calcite reacted with oxalic acid will produce internally mixed particles of calcite and calcium oxalate due to the low solubility of the product salt. However, simulations of the scattering for the calcite-oxalic acid system result in rather poor fits to the data when compared to the other samples. The poor fit provides a less accurate picture of the impact of processing in the calcite-oxalic acid system.

Hybrid Theory of Electron-Hydrogenic Systems Elastic Scattering

NASA Technical Reports Server (NTRS)

Bhatia, A. K.

2007-01-01

Accurate electron-hydrogen and electron-hydrogenic cross sections are required to interpret fusion experiments, laboratory plasma physics and properties of the solar and astrophysical plasmas. We have developed a method in which the short-range and long-range correlations can be included at the same time in the scattering equations. The phase shifts have rigorous lower bounds and the scattering lengths have rigorous upper bounds. The phase shifts in the resonance region can be used to calculate very accurately the resonance parameters.

Comparison and validation of point spread models for imaging in natural waters.

PubMed

Hou, Weilin; Gray, Deric J; Weidemann, Alan D; Arnone, Robert A

2008-06-23

It is known that scattering by particulates within natural waters is the main cause of the blur in underwater images. Underwater images can be better restored or enhanced with knowledge of the point spread function (PSF) of the water. This will extend the performance range as well as the information retrieval from underwater electro-optical systems, which is critical in many civilian and military applications, including target and especially mine detection, search and rescue, and diver visibility. A better understanding of the physical process involved also helps to predict system performance and simulate it accurately on demand. The presented effort first reviews several PSF models, including the introduction of a semi-analytical PSF given optical properties of the medium, including scattering albedo, mean scattering angles and the optical range. The models under comparison include the empirical model of Duntley, a modified PSF model by Dolin et al, as well as the numerical integration of analytical forms from Wells, as a benchmark of theoretical results. For experimental results, in addition to that of Duntley, we validate the above models with measured point spread functions by applying field measured scattering properties with Monte Carlo simulations. Results from these comparisons suggest it is sufficient but necessary to have the three parameters listed above to model PSFs. The simplified approach introduced also provides adequate accuracy and flexibility for imaging applications, as shown by examples of restored underwater images.

Polarized optical scattering by inhomogeneities and surface roughness in an anisotropic thin film

DOE PAGES

Germer, Thomas A.; Sharma, Katelynn A.; Brown, Thomas G.; ...

2017-10-18

We extend the theory for scattering by oblique columnar structure thin films to include the induced form birefringence and the propagation of radiation in those films. We generalize the 4 × 4 matrix theory to include arbitrary sources in the layer, which are necessary to determine the Green function for the inhomogeneous wave equation. We further extend first-order vector perturbation theory for scattering by roughness in the smooth surface limit, when the layer is anisotropic. Scattering by an inhomogeneous medium is approximated by a distorted Born approximation, where effective medium theory is used to determine the effective properties of themore » medium and strong fluctuation theory is used to determine the inhomogeneous sources. In this manner, we develop a model for scattering by inhomogeneous films, with anisotropic correlation functions. Here, the results are compared to Mueller matrix bidirectional scattering distribution function measurements for a glancing-angle deposition (GLAD) film. While the results are applied to the GLAD film example, the development of the theory is general enough that it can guide simulations for scattering in other anisotropic thin films.« less

Monte Carlo evaluation of accuracy and noise properties of two scatter correction methods for /sup 201/Tl cardiac SPECT

NASA Astrophysics Data System (ADS)

Narita, Y.; Iida, H.; Ebert, S.; Nakamura, T.

1997-12-01

Two independent scatter correction techniques, transmission dependent convolution subtraction (TDCS) and triple-energy window (TEW) method, were evaluated in terms of quantitative accuracy and noise properties using Monte Carlo simulation (EGS4). Emission projections (primary, scatter and scatter plus primary) were simulated for three numerical phantoms for /sup 201/Tl. Data were reconstructed with ordered-subset EM algorithm including noise-less transmission data based attenuation correction. Accuracy of TDCS and TEW scatter corrections were assessed by comparison with simulated true primary data. The uniform cylindrical phantom simulation demonstrated better quantitative accuracy with TDCS than with TEW (-2.0% vs. 16.7%) and better S/N (6.48 vs. 5.05). A uniform ring myocardial phantom simulation demonstrated better homogeneity with TDCS than TEW in the myocardium; i.e., anterior-to-posterior wall count ratios were 0.99 and 0.76 with TDCS and TEW, respectively. For the MCAT phantom, TDCS provided good visual and quantitative agreement with simulated true primary image without noticeably increasing the noise after scatter correction. Overall TDCS proved to be more accurate and less noisy than TEW, facilitating quantitative assessment of physiological functions with SPECT.

Light Scattering Analysis of Irregularly Shaped Dust Particles: A Study Using 3-Dimensional Reconstructions from Focused Ion-Beam (FIB) Tomography and Q-Space Analysis

NASA Astrophysics Data System (ADS)

Ortiz-Montalvo, D. L.; Conny, J. M.

2017-12-01

We study the scattering properties of irregularly shaped ambient dust particles. The way in which they scatter and absorb light has implications for aerosol optical remote sensing and aerosol radiative forcing applications. However, understanding light scattering and absorption by non-spherical particles can be very challenging. We used focused ion-beam scanning electron microscopy and energy-dispersive x-ray spectroscopy (FIB-SEM-EDS) to reconstruct three-dimensional (3-D) configurations of dust particles collected from urban and Asian sources. The 3-D reconstructions were then used in a discrete dipole approximation method (DDA) to determine their scattering properties for a range of shapes, sizes, and refractive indices. Scattering properties where obtained using actual-shapes of the particles, as well as, (theoretical) equivalently-sized geometrical shapes like spheres, ellipsoids, cubes, rectangular prisms, and tetrahedrons. We use Q-space analysis to interpret the angular distribution of the scattered light obtained for each particle. Q-space analysis has been recently used to distinguish scattering by particles of different shapes, and it involves plotting the scattered intensity versus the scattering wave vector (q or qR) on a log-log scale, where q = 2ksin(θ/2), k = 2π/λ, and R = particle effective radius. Results from a limited number of particles show that when Q-space analysis is applied, common patterns appear that agree with previous Q-space studies done on ice crystals and other irregularly shaped particles. More specifically, we found similar Q-space regimes including a forward scattering regime of constant intensity when qR < 1, followed by the Guinier regime when qR ≈ 1, which is then followed by a complex power law regime with a -3 slope regime, a transition regime, and then a -4 slope regime. Currently, Q-space comparisons between actual- and geometric shapes are underway with the objective of determining which geometric shape best represents the angular distribution and magnitude of the scattered light. Current work also focuses on the effects of the imaginary part of the refractive index on the light scattering of our dust particles.

Atmospheric aerosols: Their Optical Properties and Effects (supplement)

NASA Technical Reports Server (NTRS)

1976-01-01

A digest of technical papers is presented. Topics include aerosol size distribution from spectral attenuation with scattering measurements; comparison of extinction and backscattering coefficients for measured and analytic stratospheric aerosol size distributions; using hybrid methods to solve problems in radiative transfer and in multiple scattering; blue moon phenomena; absorption refractive index of aerosols in the Denver pollution cloud; a two dimensional stratospheric model of the dispersion of aerosols from the Fuego volcanic eruption; the variation of the aerosol volume to light scattering coefficient; spectrophone in situ measurements of the absorption of visible light by aerosols; a reassessment of the Krakatoa volcanic turbidity, and multiple scattering in the sky radiance.

Weak scattering of scalar and electromagnetic random fields

NASA Astrophysics Data System (ADS)

Tong, Zhisong

This dissertation encompasses several studies relating to the theory of weak potential scattering of scalar and electromagnetic random, wide-sense statistically stationary fields from various types of deterministic or random linear media. The proposed theory is largely based on the first Born approximation for potential scattering and on the angular spectrum representation of fields. The main focus of the scalar counterpart of the theory is made on calculation of the second-order statistics of scattered light fields in cases when the scattering medium consists of several types of discrete particles with deterministic or random potentials. It is shown that the knowledge of the correlation properties for the particles of the same and different types, described with the newly introduced pair-scattering matrix, is crucial for determining the spectral and coherence states of the scattered radiation. The approach based on the pair-scattering matrix is then used for solving an inverse problem of determining the location of an "alien" particle within the scattering collection of "normal" particles, from several measurements of the spectral density of scattered light. Weak scalar scattering of light from a particulate medium in the presence of optical turbulence existing between the scattering centers is then approached using the combination of the Born's theory for treating the light interaction with discrete particles and the Rytov's theory for light propagation in extended turbulent medium. It is demonstrated how the statistics of scattered radiation depend on scattering potentials of particles and the power spectra of the refractive index fluctuations of turbulence. This theory is of utmost importance for applications involving atmospheric and oceanic light transmission. The second part of the dissertation includes the theoretical procedure developed for predicting the second-order statistics of the electromagnetic random fields, such as polarization and linear momentum, scattered from static media. The spatial distribution of these properties of scattered fields is shown to be substantially dependent on the correlation and polarization properties of incident fields and on the statistics of the refractive index distribution within the scatterers. Further, an example is considered which illustrates the usefulness of the electromagnetic scattering theory of random fields in the case when the scattering medium is a thin bio-tissue layer with the prescribed power spectrum of the refractive index fluctuations. The polarization state of the scattered light is shown to be influenced by correlation and polarization states of the illumination as well as by the particle size distribution of the tissue slice.

Spatial distribution of mineral dust single scattering albedo based on DREAM model

NASA Astrophysics Data System (ADS)

Kuzmanoski, Maja; Ničković, Slobodan; Ilić, Luka

2016-04-01

Mineral dust comprises a significant part of global aerosol burden. There is a large uncertainty in estimating role of dust in Earth's climate system, partly due to poor characterization of its optical properties. Single scattering albedo is one of key optical properties determining radiative effects of dust particles. While it depends on dust particle sizes, it is also strongly influenced by dust mineral composition, particularly the content of light-absorbing iron oxides and the mixing state (external or internal). However, an assumption of uniform dust composition is typically used in models. To better represent single scattering albedo in dust atmospheric models, required to increase accuracy of dust radiative effect estimates, it is necessary to include information on particle mineral content. In this study, we present the spatial distribution of dust single scattering albedo based on the Dust Regional Atmospheric Model (DREAM) with incorporated particle mineral composition. The domain of the model covers Northern Africa, Middle East and the European continent, with horizontal resolution set to 1/5°. It uses eight particle size bins within the 0.1-10 μm radius range. Focusing on dust episode of June 2010, we analyze dust single scattering albedo spatial distribution over the model domain, based on particle sizes and mineral composition from model output; we discuss changes in this optical property after long-range transport. Furthermore, we examine how the AERONET-derived aerosol properties respond to dust mineralogy. Finally we use AERONET data to evaluate model-based single scattering albedo. Acknowledgement We would like to thank the AERONET network and the principal investigators, as well as their staff, for establishing and maintaining the AERONET sites used in this work.

Liquid Dynamics in high melting materials studied by inelastic X-ray scattering

NASA Astrophysics Data System (ADS)

Sinn, Harald; Alatas, Ahmet; Said, Ayman; Alp, Esen E.; Price, David L.; Saboungi, Marie Louis; Scheunemann, Richard

2004-03-01

The transport properties of high melting materials are of interest for a variety of applications, including geo-sciences, nuclear waste confinement and aerospace technology. While traditional methods of measuring transport properties are often extremely difficult due to the high reactivity of the melts, the combination of containerless levitation and inelastic X-ray scattering offers new insights in the microscopic dynamics of these liquids. Data on the dynamic structure factor of liquid aluminum oxide and liquid boron between 2000-2800 degree Celsius are discussed and related to several macroscopic quantities like sound velocity, viscosity and diffusion.

Active and Passive Radiative Transfer Modeling with Preferentially-Aligned Particles

NASA Technical Reports Server (NTRS)

Adams, Ian Stuart

2017-01-01

The fluid dynamics of falling hydrometeors often results in preferential orientations that can affect both the intensity and polarization of electromagnetic radiation. In order to properly interpret remote sensing observations of ice and snow, such alignments should be considered when constructing databases of scattering particles; however, the inclusion of aligned particles increases the complexity of the scattering data. To demonstrate the use of scattering properties of preferentially-aligned particles, millimeter-wave brightness temperatures and radar observables, including reflectivity and linear depolarization ratio, are modeled using the Atmospheric Radiative Transfer Simulator (ARTS). The necessary scattering parameters for vector radiative transfer, particularly with respect to ARTS, are reviewed, and the exploitation of particle symmetries, as well as scattering reciprocity relationships, are detailed.

Characteristics of aerosol light scattering and absorption properties observed at Gosan, Korea, during GOPOEX 2014

NASA Astrophysics Data System (ADS)

Cho, C.; Kim, S. W.; Sheridan, P. J.; Gustafsson, O.; Lee, M.; Yoon, S. C.

2016-12-01

Anthropogenic fine pollution and wind-blown mineral dust aerosols have a significant effect on the regional radiation budget by scattering or absorbing the solar radiation reaching the Earth's surface. We investigate the optical and physical properties of dust and pollution aerosols at Gosan Climate Observatory (GCO), Korea during Gosan Pollution Experiment 2014 (GOPOEX 2014; January 2014).Mean values of aerosol scattering coefficient and absorption coefficient during GOPOEX 2014 were 72 ± 86 Mm-1 and 6 ± 5 Mm-1 at 550 nm, respectively. Aerosol scattering coefficient and absorption coefficient during dust episodes were 245 ± 171 Mm-1 and 22 ± 13 Mm-1 at 550 nm, which were approximately 3.5 times greater than mean values during GOPOEX 2014. Values for scattering and absorption coefficient of pollution episodes were recorded as 153 ± 95 Mm-1 and 12 ± 7 Mm-1 at 550 nm. Therefore, single scattering albedo of pollution episodes (0.92 ± 0.02) was slightly higher than those of dust episodes (0.90 ± 0.03). This is because that pollutant aerosols include more scattering fraction such as SO42-, and NO3- in fine particulate matter emitted from industrial areas in the eastern coastal region of China while dust aerosols are transported from North China to Gosan.Aerosol optical properties are influenced by where the air mass is transported from, either South China or North China. The mean values of aerosol scattering coefficient and absorption coefficient when air mass was transported from South China were 136 ± 132 Mm-1 and 15 ± 14 Mm-1 at 550 nm whereas those from North China were 108 ± 112 Mm-1 and 8 ± 7 Mm-1 at 550 nm. Single scattering albedo are almost identical as 0.9 ± 0.03 for both air masses.Carbonaceous composition of aerosols, which occupy a considerable fraction of fine particulate matter, also depends on the origin of the air mass. Radiocarbon (14C) is a good indicator for distinguishing between fossil combustion and biomass combustion. Detailed source contribution based on radiocarbon measurements and its relationship to aerosol optical properties at GCO will be presented.

Mixing Single Scattering Properties in Vector Radiative Transfer for Deterministic and Stochastic Solutions

NASA Astrophysics Data System (ADS)

Mukherjee, L.; Zhai, P.; Hu, Y.; Winker, D. M.

2016-12-01

Among the primary factors, which determine the polarized radiation, field of a turbid medium are the single scattering properties of the medium. When multiple types of scatterers are present, the single scattering properties of the scatterers need to be properly mixed in order to find the solutions to the vector radiative transfer theory (VRT). The VRT solvers can be divided into two types: deterministic and stochastic. The deterministic solver can only accept one set of single scattering property in its smallest discretized spatial volume. When the medium contains more than one kind of scatterer, their single scattering properties are averaged, and then used as input for the deterministic solver. The stochastic solver, can work with different kinds of scatterers explicitly. In this work, two different mixing schemes are studied using the Successive Order of Scattering (SOS) method and Monte Carlo (MC) methods. One scheme is used for deterministic and the other is used for the stochastic Monte Carlo method. It is found that the solutions from the two VRT solvers using two different mixing schemes agree with each other extremely well. This confirms the equivalence to the two mixing schemes and also provides a benchmark for the VRT solution for the medium studied.

Transport properties of the two-dimensional electron gas in AlxGa1-xN/GaN heterostructures

NASA Astrophysics Data System (ADS)

Han, Xiuxun; Honda, Yoshio; Narita, Tetsuo; Yamaguchi, Masahito; Sawaki, Nobuhiko

2007-01-01

Magnetotransport measurements were performed on a series of AlxGa1-xN/GaN heterostructures with different Al compositions (x = 0.15, 0.20 and 0.30) at 4.2 K. Adopting a fast Fourier transform method, we analysed the Shubnikov-de Hass oscillations due to the two-dimensional electron gas to derive the quantum scattering time (τq). It was found that the quantum scattering time in the ground subband decreases with increasing Al composition: 0.194 ps (x = 0.15), 0.174 ps (x = 0.20) and 0.123 ps (x = 0.30), respectively. To discern the predominant scattering process, the scattering time limited by interface roughness, the residual impurity and the alloy disorder were investigated numerically by including inter-subband scattering. We found that enhanced interface roughness scattering dominates both the transport and quantum scattering time in the ground subband.

Multiparametric, Longitudinal Optical Coherence Tomography Imaging Reveals Acute Injury and Chronic Recovery in Experimental Ischemic Stroke

PubMed Central

Srinivasan, Vivek J.; Mandeville, Emiri T.; Can, Anil; Blasi, Francesco; Climov, Mihail; Daneshmand, Ali; Lee, Jeong Hyun; Yu, Esther; Radhakrishnan, Harsha; Lo, Eng H.; Sakadžić, Sava; Eikermann-Haerter, Katharina; Ayata, Cenk

2013-01-01

Progress in experimental stroke and translational medicine could be accelerated by high-resolution in vivo imaging of disease progression in the mouse cortex. Here, we introduce optical microscopic methods that monitor brain injury progression using intrinsic optical scattering properties of cortical tissue. A multi-parametric Optical Coherence Tomography (OCT) platform for longitudinal imaging of ischemic stroke in mice, through thinned-skull, reinforced cranial window surgical preparations, is described. In the acute stages, the spatiotemporal interplay between hemodynamics and cell viability, a key determinant of pathogenesis, was imaged. In acute stroke, microscopic biomarkers for eventual infarction, including capillary non-perfusion, cerebral blood flow deficiency, altered cellular scattering, and impaired autoregulation of cerebral blood flow, were quantified and correlated with histology. Additionally, longitudinal microscopy revealed remodeling and flow recovery after one week of chronic stroke. Intrinsic scattering properties serve as reporters of acute cellular and vascular injury and recovery in experimental stroke. Multi-parametric OCT represents a robust in vivo imaging platform to comprehensively investigate these properties. PMID:23940761

The impact of defect scattering on the quasi-ballistic transport of nanoscale conductors

DOE Office of Scientific and Technical Information (OSTI.GOV)

Esqueda, I. S., E-mail: isanchez@isi.edu; Fritze, M.; Cress, C. D.

2015-02-28

Using the Landauer approach for carrier transport, we analyze the impact of defects induced by ion irradiation on the transport properties of nanoscale conductors that operate in the quasi-ballistic regime. Degradation of conductance results from a reduction of carrier mean free path due to the introduction of defects in the conducting channel. We incorporate scattering mechanisms from radiation-induced defects into calculations of the transmission coefficient and present a technique for extracting modeling parameters from near-equilibrium transport measurements. These parameters are used to describe degradation in the transport properties of nanoscale devices using a formalism that is valid under quasi-ballistic operation.more » The analysis includes the effects of bandstructure and dimensionality on the impact of defect scattering and discusses transport properties of nanoscale devices from the diffusive to the ballistic limit. We compare calculations with recently published measurements of irradiated nanoscale devices such as single-walled carbon nanotubes, graphene, and deep-submicron Si metal-oxide-semiconductor field-effect transistors.« less

On the shape of martian dust and water ice aerosols

NASA Astrophysics Data System (ADS)

Pitman, K. M.; Wolff, M. J.; Clancy, R. T.; Clayton, G. C.

2000-10-01

Researchers have often calculated radiative properties of Martian aerosols using either Mie theory for homogeneous spheres or semi-empirical theories. Given that these atmospheric particles are randomly oriented, this approach seems fairly reasonable. However, the idea that randomly oriented nonspherical particles have scattering properties equivalent to even a select subset of spheres is demonstratably false} (Bohren and Huffman 1983; Bohren and Koh 1985, Appl. Optics, 24, 1023). Fortunately, recent computational developments now enable us to directly compute scattering properties for nonspherical particles. We have combined a numerical approach for axisymmetric particle shapes, i.e., cylinders, disks, spheroids (Waterman's T-Matrix approach as improved by Mishchenko and collaborators; cf., Mishchenko et al. 1997, JGR, 102, D14, 16,831), with a multiple-scattering radiative transfer algorithm to constrain the shape of water ice and dust aerosols. We utilize a two-stage iterative process. First, we empirically derive a scattering phase function for each aerosol component (starting with some ``guess'') from radiative transfer models of MGS Thermal Emission Spectrometer Emission Phase Function (EPF) sequences (for details on this step, see Clancy et al., DPS 2000). Next, we perform a series of scattering calculations, adjusting our parameters to arrive at a ``best-fit'' theoretical phase function. In this presentation, we provide details on the second step in our analysis, including the derived phase functions (for several characteristic EPF sequences) as well as the particle properties of the best-fit theoretical models. We provide a sensitivity analysis for the EPF model-data comparisons in terms of perturbations in the particle properties (i.e., range of axial ratios, sizes, refractive indices, etc). This work is supported through NASA grant NAGS-9820 (MJW) and JPL contract no. 961471 (RTC).

Surface-enhanced Raman scattering (SERS) dosimeter and probe

DOEpatents

Vo-Dinh, Tuan

1995-01-01

A dosimeter and probe for measuring exposure to chemical and biological compounds is disclosed. The dosimeter or probe includes a collector which may be analyzed by surface-enhanced Raman spectroscopy. The collector comprises a surface-enhanced Raman scattering-active material having a coating applied thereto to improve the adsorption properties of the collector. The collector may also be used in automated sequential devises, in probe array devices.

Scattering properties of alumina particle clusters with different radius of monomers in aerocraft plume

NASA Astrophysics Data System (ADS)

Li, Jingying; Bai, Lu; Wu, Zhensen; Guo, Lixin; Gong, Yanjun

2017-11-01

In this paper, diffusion limited aggregation (DLA) algorithm is improved to generate the alumina particle cluster with different radius of monomers in the plume. Scattering properties of these alumina clusters are solved by the multiple sphere T matrix method (MSTM). The effect of the number and radius of monomers on the scattering properties of clusters of alumina particles is discussed. The scattering properties of two types of alumina particle clusters are compared, one has different radius of monomers that follows lognormal probability distribution, another has the same radius of monomers that equals the mean of lognormal probability distribution. The result show that the scattering phase functions and linear polarization degrees of these two types of alumina particle clusters are of great differences. For the alumina clusters with different radius of monomers, the forward scatterings are bigger and the linear polarization degree has multiple peaks. Moreover, the vary of their scattering properties do not have strong correlative with the change of number of monomers. For larger booster motors, 25-38% of the plume being condensed alumina. The alumina can scatter radiation from other sources present in the plume and effect on radiation transfer characteristics of plume. In addition, the shape, size distribution and refractive index of the particles in the plume are estimated by linear polarization degree. Therefore, accurate scattering properties calculation is very important to decrease the deviation in the related research.

Numerical Studies of Scattering Properties of Leaves and Leaf Moisture Influences on the Scattering at Microwave Wavelengths

NASA Technical Reports Server (NTRS)

Lin, Bing; Hu, Yongxiang; Sun, Wenbo; Min, Qilong

2008-01-01

This study uses 3-dimensional finite difference time domain method to accurately calculate single-scattering properties of randomly orientated leaves and evaluate the influences of vegetation water content (VWC) on these properties at 19 and 37 GHz frequencies. The studied leaves are assumed to be thin elliptic disks with two different sizes and have various VWC values. Although the leaf moisture produces considerable absorption during scattering processes, the effective efficiencies of extinction and scattering of leaves still near-linearly increase with VWC. Calculated asymmetry factors and phase functions indicate that there are significant amounts of scattering at large scattering angles in microwave wavelengths, which provides good opportunities for off-nadir microwave remote sensing of forests. This study lays a basic foundation in future quantifications of the relations between satellite measurements and physical properties of vegetation canopies.

Painting galaxies into dark matter halos using machine learning

NASA Astrophysics Data System (ADS)

Agarwal, Shankar; Davé, Romeel; Bassett, Bruce A.

2018-05-01

We develop a machine learning (ML) framework to populate large dark matter-only simulations with baryonic galaxies. Our ML framework takes input halo properties including halo mass, environment, spin, and recent growth history, and outputs central galaxy and halo baryonic properties including stellar mass (M*), star formation rate (SFR), metallicity (Z), neutral (H I) and molecular (H_2) hydrogen mass. We apply this to the MUFASA cosmological hydrodynamic simulation, and show that it recovers the mean trends of output quantities with halo mass highly accurately, including following the sharp drop in SFR and gas in quenched massive galaxies. However, the scatter around the mean relations is under-predicted. Examining galaxies individually, at z = 0 the stellar mass and metallicity are accurately recovered (σ ≲ 0.2 dex), but SFR and H I show larger scatter (σ ≳ 0.3 dex); these values improve somewhat at z = 1, 2. Remarkably, ML quantitatively recovers second parameter trends in galaxy properties, e.g. that galaxies with higher gas content and lower metallicity have higher SFR at a given M*. Testing various ML algorithms, we find that none perform significantly better than the others, nor does ensembling improve performance, likely because none of the algorithms reproduce the large observed scatter around the mean properties. For the random forest algorithm, we find that halo mass and nearby (˜200 kpc) environment are the most important predictive variables followed by growth history, while halo spin and ˜Mpc scale environment are not important. Finally we study the impact of additionally inputting key baryonic properties M*, SFR, and Z, as would be available e.g. from an equilibrium model, and show that particularly providing the SFR enables H I to be recovered substantially more accurately.

Effects of ice crystal surface roughness and air bubble inclusions on cirrus cloud radiative properties from remote sensing perspective

NASA Astrophysics Data System (ADS)

Tang, Guanglin; Panetta, R. Lee; Yang, Ping; Kattawar, George W.; Zhai, Peng-Wang

2017-07-01

We study the combined effects of surface roughness and inhomogeneity on the optical scattering properties of ice crystals and explore the consequent implications to remote sensing of cirrus cloud properties. Specifically, surface roughness and inhomogeneity are added to the Moderate Resolution Imaging Spectroradiometer (MODIS) collection 6 (MC6) cirrus cloud particle habit model. Light scattering properties of the new habit model are simulated using a modified version of the Improved Geometric Optics Method (IGOM). Both inhomogeneity and surface roughness affect the single scattering properties significantly. In visible bands, inhomogeneity and surface roughness both tend to smooth the phase function and eliminate halos and the backscattering peak. The asymmetry parameter varies with the degree of surface roughness following a U shape - decreases and then increases - with a minimum at around 0.15, whereas it decreases monotonically with the air bubble volume fraction. Air bubble inclusions significantly increase phase matrix element -P12 for scattering angles between 20°-120°, whereas surface roughness has a much weaker effect, increasing -P12 slightly from 60°-120°. Radiative transfer simulations and cirrus cloud property retrievals are conducted by including both the factors. In terms of surface roughness and air bubble volume fraction, retrievals of cirrus cloud optical thickness or the asymmetry parameter using solar bands show similar patterns of variation. Polarimetric simulations using the MC6 cirrus cloud particle habit model are shown to be more consistent with observations when both surface roughness and inhomogeneity are simultaneously considered.

Aerosol Optical Properties Measured Onboard the Ronald H. Brown During ACE Asia as a Function of Aerosol Chemical Composition and Source Region

NASA Technical Reports Server (NTRS)

Quinn, P. K.; Coffman, D. J.; Bates, T. S.; Welton, E. J.; Covert, D. S.; Miller, T. L.; Johnson, J. E.; Maria, S.; Russell, L.; Arimoto, R.

2004-01-01

During the ACE Asia intensive field campaign conducted in the spring of 2001 aerosol properties were measured onboard the R/V Ronald H. Brown to study the effects of the Asian aerosol on atmospheric chemistry and climate in downwind regions. Aerosol properties measured in the marine boundary layer included chemical composition; number size distribution; and light scattering, hemispheric backscattering, and absorption coefficients. In addition, optical depth and vertical profiles of aerosol 180 deg backscatter were measured. Aerosol within the ACE Asia study region was found to be a complex mixture resulting from marine, pollution, volcanic, and dust sources. Presented here as a function of air mass source region are the mass fractions of the dominant aerosol chemical components, the fraction of the scattering measured at the surface due to each component, mass scattering efficiencies of the individual components, aerosol scattering and absorption coefficients, single scattering albedo, Angstrom exponents, optical depth, and vertical profiles of aerosol extinction. All results except aerosol optical depth and the vertical profiles of aerosol extinction are reported at a relative humidity of 55 +/- 5%. An over-determined data set was collected so that measured and calculated aerosol properties could be compared, internal consistency in the data set could be assessed, and sources of uncertainty could be identified. By taking into account non-sphericity of the dust aerosol, calculated and measured aerosol mass and scattering coefficients agreed within overall experimental uncertainties. Differences between measured and calculated aerosol absorption coefficients were not within reasonable uncertainty limits, however, and may indicate the inability of Mie theory and the assumption of internally mixed homogeneous spheres to predict absorption by the ACE Asia aerosol. Mass scattering efficiencies of non-sea salt sulfate aerosol, sea salt, submicron particulate organic matter, and dust found for the ACE Asia aerosol are comparable to values estimated for ACE 1, Aerosols99, and INDOEX. Unique to the ACE Asia aerosol was the large mass fractions of dust, the dominance of dust in controlling the aerosol optical properties, and the interaction of dust with soot aerosol.

Subsurface polarimetric migration imaging for full polarimetric ground-penetrating radar

NASA Astrophysics Data System (ADS)

Feng, Xuan; Yu, Yue; Liu, Cai; Fehler, Michael

2015-08-01

Polarization is a property of electromagnetic wave that generally refers to the locus of the electric field vector, which can be used to characterize surface properties by polarimetric radar. However, its use has been less common in the ground-penetrating radar (GPR) community. Full polarimetric GPR data include scattering matrices, by which the polarization properties can be extracted, at each survey point. Different components of the measured scattering matrix are sensitive to different types of subsurface objects, which offers a potential improvement in the detection ability of GPR. This paper develops a polarimetric migration imaging method. By merging the Pauli polarimetric decomposition technique with the Krichhoff migration equation, we develop a polarimetric migration algorithm, which can extract three migrated coefficients that are sensitive to different types of objects. Then fusing the three migrated coefficients, we can obtain subsurface colour-coded reconstructed object images, which can be employed to interpret both the geometrical information and the scattering mechanism of the subsurface objects. A 3-D full polarimetric GPR data set was acquired in a laboratory experiment and was used to test the method. In the laboratory experiment, four objects-a scatterer, a ball, a plate and a dihedral target-were buried in homogeneous dry sand under a flat ground surface. By merging the reconstructed image with polarization properties, we enhanced the subsurface image and improved the classification ability of GPR.

Incoherent Diffractive Imaging via Intensity Correlations of Hard X Rays

NASA Astrophysics Data System (ADS)

Classen, Anton; Ayyer, Kartik; Chapman, Henry N.; Röhlsberger, Ralf; von Zanthier, Joachim

2017-08-01

Established x-ray diffraction methods allow for high-resolution structure determination of crystals, crystallized protein structures, or even single molecules. While these techniques rely on coherent scattering, incoherent processes like fluorescence emission—often the predominant scattering mechanism—are generally considered detrimental for imaging applications. Here, we show that intensity correlations of incoherently scattered x-ray radiation can be used to image the full 3D arrangement of the scattering atoms with significantly higher resolution compared to conventional coherent diffraction imaging and crystallography, including additional three-dimensional information in Fourier space for a single sample orientation. We present a number of properties of incoherent diffractive imaging that are conceptually superior to those of coherent methods.

The Dubna-Mainz-Taipei Dynamical Model for πN Scattering and π Electromagnetic Production

NASA Astrophysics Data System (ADS)

Yang, Shin Nan

Some of the featured results of the Dubna-Mainz-Taipei (DMT) dynamical model for πN scattering and π0 electromagnetic production are summarized. These include results for threshold π0 production, deformation of Δ(1232),and the extracted properties of higher resonances below 2 GeV. The excellent agreement of DMT model's predictions with threshold π0 production data, including the recent precision measurements from MAMI establishes results of DMT model as a benchmark for experimentalists and theorists in dealing with threshold pion production.

Optical properties of mineral dust aerosol including analysis of particle size, composition, and shape effects, and the impact of physical and chemical processing

NASA Astrophysics Data System (ADS)

Alexander, Jennifer Mary

Atmospheric mineral dust has a large impact on the earth's radiation balance and climate. The radiative effects of mineral dust depend on factors including, particle size, shape, and composition which can all be extremely complex. Mineral dust particles are typically irregular in shape and can include sharp edges, voids, and fine scale surface roughness. Particle shape can also depend on the type of mineral and can vary as a function of particle size. In addition, atmospheric mineral dust is a complex mixture of different minerals as well as other, possibly organic, components that have been mixed in while these particles are suspended in the atmosphere. Aerosol optical properties are investigated in this work, including studies of the effect of particle size, shape, and composition on the infrared (IR) extinction and visible scattering properties in order to achieve more accurate modeling methods. Studies of particle shape effects on dust optical properties for single component mineral samples of silicate clay and diatomaceous earth are carried out here first. Experimental measurements are modeled using T-matrix theory in a uniform spheroid approximation. Previous efforts to simulate the measured optical properties of silicate clay, using models that assumed particle shape was independent of particle size, have achieved only limited success. However, a model which accounts for a correlation between particle size and shape for the silicate clays offers a large improvement over earlier modeling approaches. Diatomaceous earth is also studied as an example of a single component mineral dust aerosol with extreme particle shapes. A particle shape distribution, determined by fitting the experimental IR extinction data, used as a basis for modeling the visible light scattering properties. While the visible simulations show only modestly good agreement with the scattering data, the fits are generally better than those obtained using more commonly invoked particle shape distributions. The next goal of this work is to investigate if modeling methods developed in the studies of single mineral components can be generalized to predict the optical properties of more authentic aerosol samples which are complex mixtures of different minerals. Samples of Saharan sand, Iowa loess, and Arizona road dust are used here as test cases. T-matrix based simulations of the authentic samples, using measured particle size distributions, empirical mineralogies, and a priori particle shape models for each mineral component are directly compared with the measured IR extinction spectra and visible scattering profiles. This modeling approach offers a significant improvement over more commonly applied models that ignore variations in particle shape with size or mineralogy and include only a moderate range of shape parameters. Mineral dust samples processed with organic acids and humic material are also studied in order to explore how the optical properties of dust can change after being aged in the atmosphere. Processed samples include quartz mixed with humic material, and calcite reacted with acetic and oxalic acid. Clear differences in the light scattering properties are observed for all three processed mineral dust samples when compared to the unprocessed mineral dust or organic salt products. These interactions result in both internal and external mixtures depending on the sample. In addition, the presence of these organic materials can alter the mineral dust particle shape. Overall, however, these results demonstrate the need to account for the effects of atmospheric aging of mineral dust on aerosol optical properties. Particle shape can also affect the aerodynamic properties of mineral dust aerosol. In order to account for these effects, the dynamic shape factor is used to give a measure of particle asphericity. Dynamic shape factors of quartz are measured by mass and mobility selecting particles and measuring their vacuum aerodynamic diameter. From this, dynamic shape factors in both the transition and vacuum regime can be derived. The measured dynamic shape factors of quartz agree quite well with the spheroidal shape distributions derived through studies of the optical properties.

Airborne characterization of aerosols over the contiguous United States during the SEAC4RS and DC3 campaigns: an in situ light scattering perspective

NASA Astrophysics Data System (ADS)

Espinosa, R.; Remer, L.; Puthukkudy, A.; Orozco, D.; Dubovik, O.; Martins, J. V.

2017-12-01

Models used to estimate climate change and interpret remote sensing observations must make assumptions regarding aerosol radiation interactions. This presentation will summarize aerosol light scattering measurements made by the Polarized Imaging Nephelometer (PI-Neph) during the Studies of Emissions and Atmospheric Composition, Clouds and Climate Coupling by Regional Surveys (SEAC4RS) and Deep Convective Clouds and Chemistry (DC3) experiments. The data presented includes direct measurements of phase function (P11) and polarized phase function (-P12/P11) as well as retrievals of size distribution, sphericity and complex refractive index made using the Generalized Retrieval of Aerosol and Surface Properties (GRASP). An aerosol classification scheme is developed to identify different aerosol types measured during the deployments, making use of ancillary data that includes gas tracers, chemical composition, aerodynamic particle size and geographic location. Principal component analysis (PCA) is then used to reduce the dimensionality of the multi-angle PI-Neph scattering data and a strong link between the PCA scores and the ancillary classification results is observed. The scattering differences that reliable distinguish the different aerosol types are found to be quite subtle and often rely on the relationships between many scattering angles simultaneously. This fact emphasis the value of multi-angle scattering measurements, as well as principal component analysis's ability to reveal the underlying patterns in these datasets. The parameters retrieved from the DC3 scattering data suggest the presence of a significant amount of dust in aerosols influenced by convective systems, with the quantity of dust correlating strongly with sampling location and the underlying surface features. All fine mode dominated aerosol types from SEAC4RS had remarkably similar retrieved properties, except for the real refractive index of the biomass burning cases, which was consistently elevated (n532=1.54) when compared to the other types (n532=1.50). This result suggests that climate and remote sensing models may often be able to capture the differences in optical properties between biomass burning and other fine mode aerosols by only adjusting the real refractive index of the particles.

Surface-enhanced Raman scattering (SERS) dosimeter and probe

DOEpatents

Vo-Dinh, T.

1995-03-21

A dosimeter and probe for measuring exposure to chemical and biological compounds is disclosed. The dosimeter or probe includes a collector which may be analyzed by surface-enhanced Raman spectroscopy. The collector comprises a surface-enhanced Raman scattering-active material having a coating applied thereto to improve the adsorption properties of the collector. The collector may also be used in automated sequential devices, in probe array devices. 10 figures.

Scattering properties of soot-containing particles and their impact by humidity in 1.6 μm

NASA Astrophysics Data System (ADS)

Fan, M.; Chen, L.; Xiong, X.; Li, S.; Tao, J.; Su, L.; Zou, M.; Zhang, Y.

2014-02-01

Short-wave infrared (SWIR) band in wavelength near 1.6 μm is one of the key bands used for satellite observation of Carbon Dioxide (CO2). However, one major uncertainty to use this band for the CO2 retrieval is the scattering by cloud and aerosol particles. To better understand the scattering properties of soot-containing particles in this band, this paper studied the scattering properties for three typical types of soot-containing particles in China: (I) internal mixture, (II) pure soot aggregate, and (III) semi-external mixture. Assumed as single non-spherical particle for type I, its scattering property is computed using the T-matrix method combined with the Maxwell-Garnett effective medium theory and the hygroscopic growth theory. For types II and III, a particle-cluster aggregation algorithm is employed to generate fractal-like aggregates, and their scattering properties are computed using the Core-Mantle Generalized Multi-sphere Mie-solution method combined with the hygroscopic growth theory of both monomers and aggregated particles. The simulated results demonstrate that their scattering properties are quite different and strongly impacted by the levels of relative humidity (RH). For type I, the RH plays a much more important role than the morphology in impacting the scattering properties, and the scattering phase functions among different shaped particles have a larger difference for larger particles and higher RH. For type II, both the RH and morphology significantly affect its scattering properties. The single scattering albedo (ω) can be underestimated up to ~50% without considering the effects of RH and morphological changes. For type III, its scattering properties mainly depend on the RH and the size of the large water-soluble particle. Although the enlarged soot aggregate, which is attached to a water-soluble particle, almost does not change the light direction, it can result in a significant reduction in ω (~0.15) at low RH for small particles. By comparing the scattering parameters of wet particles at a certain RH level with the dry ones, the impact by the heterogeneity of aerosols generally becomes larger with the increase of RH, but becomes smaller with the increase of particle size. These results suggest that, although the water vapor absorption itself is small in 1.6 μm CO2 band, it can significantly impact the scattering properties of these particles through its effect on the hygroscopic growth of the non-spherical and heterogeneous aerosols. This impact should be taken into account in the retrieval of CO2 using 1.6 μm as well as other related remote sensing applications.

Southeast Asian Summer Burning: A Micro Pulse Lidar Network Study of Aerosol Particle Physical Properties near Fires in Borneo and Sumatra

NASA Astrophysics Data System (ADS)

Lolli, S.; Welton, E. J.; Holben, B. N.; Campbell, J. R.

2013-12-01

In August and September 2012, as part of the continuing Seven South East Asian Studies (7-SEAS) project, three autonomous elastic-scattering 355 nm lidars were deployed by the NASA Micro Pulse Lidar Network (MPLNET) to Sumatra and Borneo, measuring the vertical profile of aerosol particle scattering during peak burning season. In coordination with the Aerosol Robotic Network (AERONET), a regional characterization of aerosol particle physical properties and distribution was performed. In addition to a permanent regional network site at Singapore, the three temporary sites established for this research include Jambi (Sumatra, Indonesia), Kuching (northwest Borneo, Malaysia) and Palangkaraya (south-central Borneo, Indonesia). In this paper, we discuss the mission and instruments, and introduce data products available to the community through the MPLNET online website. We further describe initial results of the study, including a contrast of mean vertical scattering profiles versus those observed near active fire sources at Jambi and Palangkaraya, and resolve longer-range particle evolution at receptor sites, like Kuching, that are most commonly 1-2 days downwind of larger fire complexes.

Gold coatings for cube-corner retro-reflectors

NASA Technical Reports Server (NTRS)

Dligatch, Svetlana; Gross, Mark; Netterfield, Roger P.; Pereira, Nathan; Platt, Benjamin C.; Nemati, Bijan

2005-01-01

We report on a comparative study of optical performance of gold films deposited by resistive and e-beam evaporation, including measurements of the scattering from the coated surfaces. The effects of oxygen bombardment and titanium under-layer on optical properties and adhesion were evaluated. The influence of surface preparation on the optical properties was examined also.

Numerical analysis of dysplasia-associated changes in depth-dependent light scattering profile of cervical epithelium

NASA Astrophysics Data System (ADS)

Arifler, Dizem; MacAulay, Calum; Follen, Michele; Guillaud, Martial

2013-06-01

Dysplastic progression is known to be associated with changes in morphology and internal structure of cells. A detailed assessment of the influence of these changes on cellular scattering response is needed to develop and optimize optical diagnostic techniques. In this study, we first analyzed a set of quantitative histopathologic images from cervical biopsies and we obtained detailed information on morphometric and photometric features of segmented epithelial cell nuclei. Morphometric parameters included average size and eccentricity of the best-fit ellipse. Photometric parameters included optical density measures that can be related to dielectric properties and texture characteristics of the nuclei. These features enabled us to construct realistic three-dimensional computational models of basal, parabasal, intermediate, and superficial cell nuclei that were representative of four diagnostic categories, namely normal (or negative for dysplasia), mild dysplasia, moderate dysplasia, and severe dysplasia or carcinoma in situ. We then employed the finite-difference time-domain method, a popular numerical tool in electromagnetics, to compute the angle-resolved light scattering properties of these representative models. Results indicated that a high degree of variability can characterize a given diagnostic category, but scattering from moderately and severely dysplastic or cancerous nuclei was generally observed to be stronger compared to scattering from normal and mildly dysplastic nuclei. Simulation results also pointed to significant intensity level variations among different epithelial depths. This suggests that intensity changes associated with dysplastic progression need to be analyzed in a depth-dependent manner.

The role of scattering and absorption on the optical properties of birefringent polycrystalline ceramics: Modeling and experiments on ruby (Cr:Al2O3)

NASA Astrophysics Data System (ADS)

Penilla, E. H.; Hardin, C. L.; Kodera, Y.; Basun, S. A.; Evans, D. R.; Garay, J. E.

2016-01-01

Light scattering due to birefringence has prevented the use of polycrystalline ceramics with anisotropic optical properties in applications such as laser gain media. However, continued development of processing technology has allowed for very low porosity and fine grains, significantly improving transparency and is paving the way for polycrystalline ceramics to be used in demanding optical applications. We present a method for producing highly transparent Cr3+ doped Al2O3 (ruby) using current activated pressure assisted densification. The one-step doping/densification process produces fine grained ceramics with well integrated (doped) Cr, resulting in good absorption and emission. In order to explain the light transmission properties, we extend the analytical model based on the Rayleigh-Gans-Debye approximation that has been previously used for undoped alumina to include absorption. The model presented captures reflection, scattering, and absorption phenomena in the ceramics. Comparison with measured transmission confirms that the model adequately describes the properties of polycrystalline ruby. In addition the measured emission spectra and emission lifetime are found to be similar to single crystals, confirming the high optical quality of the ceramics.

Size-dependent longitudinal plasmon resonance wavelength and extraordinary scattering properties of Au nanobipyramids.

PubMed

Wang, Wenhao; Yu, Peng; Zhong, Zhiqin; Tong, Xin; Liu, Tianji; Li, Yanbo; Ashalley, Eric; Chen, Huanyang; Wu, Jiang; Wang, Zhiming

2018-08-31

Au nanobipyramids (NBPs) with sharp tips and narrow plasmon linewidths are ideal candidates for plasmonic applications. In this paper, we investigated the influencing factors of longitudinal plasmon resonance wavelength (LPRW) and scattering properties of single Au NBP by simulation. Compared with the volume, we establish the aspect ratio (length/width) as the dominant factor that affects the LPRW of Au NBPs. Plasmonic nanoparticles have been widely used for light-trapping enhancement in photovoltaics. To give a profound understanding of the superior light harvesting properties of Au NBPs, the near-field localization effect and far-field scattering mechanism of Au NBPs were investigated. Under the light injection at LPRW, the tip area shows near-field enhancement and the maximum scattering intensity appears on the side area of the waist owing to the remarkable optical absorption near the tips. Additionally, we confirm the fraction of light scattered into the substrate and angular distribution of the light scattered by the Au NBPs. The fraction of light scattered into the substrate reaches up to 97% from 400-1100 nm and preserves a broadband spectrum. This suggests that the NBP has a predominant forward scattering and reduced backward scattering. The excellent plasmonic scattering properties of Au NBPs are promising in photovoltaic devices and photothermal therapy.

Study of ZnO nanoparticles: Antibacterial property and light depolarization property using light scattering tool

NASA Astrophysics Data System (ADS)

Roy, Sanchita; Barua, Nilakshi; Buragohain, Alak K.; Ahmed, Gazi A.

2013-03-01

Investigations on treatment of ZnO nanoparticles on Staphylococcus aureus MTCC 737 strain was essentially made by using standard biochemical method. The anti-microbial assay against S. aureus, and time kill assay revealed the anti-bacterial activity of ZnO nanoparticles. We have substantiated this property of ZnO nanoparticles and light depolarization property by using light scattering tool. Light scattering measurements were carried out for ZnO, S. aureus, and ZnO treated S. aureus as a function of scattering angle at 543.5 and 632.8 nm wavelengths. This was done in order to find the scattering profile of the consequent product after the action of ZnO nanoparticles on bacteria by means of light scattering tool. S. aureus treated with ZnO nanoparticles showed closer agreement of the scattering profiles at both the wavelengths, however, the scattering profiles of ZnO nanoparticles and untreated S. aureus significantly varied for the two different laser wavelengths. It was also observed that there was higher intensity of scattering from all S. aureus treated with ZnO particles compared to the untreated ones. In our work, we have studied ZnO nanoparticles and the possibility of observing its anti-bacterial activity by using light scattering tool.

Unravelling Doping Effects on PEDOT at the Molecular Level: From Geometry to Thermoelectric Transport Properties.

PubMed

Shi, Wen; Zhao, Tianqi; Xi, Jinyang; Wang, Dong; Shuai, Zhigang

2015-10-14

Tuning carrier concentration via chemical doping is the most successful strategy to optimize the thermoelectric figure of merit. Nevertheless, how the dopants affect charge transport is not completely understood. Here we unravel the doping effects by explicitly including the scattering of charge carriers with dopants on thermoelectric properties of poly(3,4-ethylenedioxythiophene), PEDOT, which is a p-type thermoelectric material with the highest figure of merit reported. We corroborate that the PEDOT exhibits a distinct transition from the aromatic to quinoid-like structure of backbone, and a semiconductor-to-metal transition with an increase in the level of doping. We identify a close-to-unity charge transfer from PEDOT to the dopant, and find that the ionized impurity scattering dominates over the acoustic phonon scattering in the doped PEDOT. By incorporating both scattering mechanisms, the doped PEDOT exhibits mobility, Seebeck coefficient and power factors in very good agreement with the experimental data, and the lightly doped PEDOT exhibits thermoelectric properties superior to the heavily doped one. We reveal that the thermoelectric transport is highly anisotropic in ordered crystals, and suggest to utilize large power factors in the direction of polymer backbone and low lattice thermal conductivity in the stacking and lamellar directions, which is viable in chain-oriented amorphous nanofibers.

Structural and magnetic properties of multi-core nanoparticles analysed using a generalised numerical inversion method

PubMed Central

Bender, P.; Bogart, L. K.; Posth, O.; Szczerba, W.; Rogers, S. E.; Castro, A.; Nilsson, L.; Zeng, L. J.; Sugunan, A.; Sommertune, J.; Fornara, A.; González-Alonso, D.; Barquín, L. Fernández; Johansson, C.

2017-01-01

The structural and magnetic properties of magnetic multi-core particles were determined by numerical inversion of small angle scattering and isothermal magnetisation data. The investigated particles consist of iron oxide nanoparticle cores (9 nm) embedded in poly(styrene) spheres (160 nm). A thorough physical characterisation of the particles included transmission electron microscopy, X-ray diffraction and asymmetrical flow field-flow fractionation. Their structure was ultimately disclosed by an indirect Fourier transform of static light scattering, small angle X-ray scattering and small angle neutron scattering data of the colloidal dispersion. The extracted pair distance distribution functions clearly indicated that the cores were mostly accumulated in the outer surface layers of the poly(styrene) spheres. To investigate the magnetic properties, the isothermal magnetisation curves of the multi-core particles (immobilised and dispersed in water) were analysed. The study stands out by applying the same numerical approach to extract the apparent moment distributions of the particles as for the indirect Fourier transform. It could be shown that the main peak of the apparent moment distributions correlated to the expected intrinsic moment distribution of the cores. Additional peaks were observed which signaled deviations of the isothermal magnetisation behavior from the non-interacting case, indicating weak dipolar interactions. PMID:28397851

Purcell effect for active tuning of light scattering from semiconductor optical antennas.

PubMed

Holsteen, Aaron L; Raza, Søren; Fan, Pengyu; Kik, Pieter G; Brongersma, Mark L

2017-12-15

Subwavelength, high-refractive index semiconductor nanostructures support optical resonances that endow them with valuable antenna functions. Control over the intrinsic properties, including their complex refractive index, size, and geometry, has been used to manipulate fundamental light absorption, scattering, and emission processes in nanostructured optoelectronic devices. In this study, we harness the electric and magnetic resonances of such antennas to achieve a very strong dependence of the optical properties on the external environment. Specifically, we illustrate how the resonant scattering wavelength of single silicon nanowires is tunable across the entire visible spectrum by simply moving the height of the nanowires above a metallic mirror. We apply this concept by using a nanoelectromechanical platform to demonstrate active tuning. Copyright © 2017 The Authors, some rights reserved; exclusive licensee American Association for the Advancement of Science. No claim to original U.S. Government Works.

Optimizing laser crater enhanced Raman scattering spectroscopy

NASA Astrophysics Data System (ADS)

Lednev, V. N.; Sdvizhenskii, P. A.; Grishin, M. Ya.; Fedorov, A. N.; Khokhlova, O. V.; Oshurko, V. B.; Pershin, S. M.

2018-05-01

The laser crater enhanced Raman scattering (LCERS) spectroscopy technique has been systematically studied for chosen sampling strategy and influence of powder material properties on spectra intensity enhancement. The same nanosecond pulsed solid state Nd:YAG laser (532 nm, 10 ns, 0.1-1.5 mJ/pulse) was used for laser crater production and Raman scattering experiments for L-aspartic acid powder. Increased sampling area inside crater cavity is the key factor for Raman signal improvement for the LCERS technique, thus Raman signal enhancement was studied as a function of numerous experimental parameters including lens-to-sample distance, wavelength (532 and 1064 nm) and laser pulse energy utilized for crater production. Combining laser pulses of 1064 and 532 nm wavelengths for crater ablation was shown to be an effective way for additional LCERS signal improvement. Powder material properties (particle size distribution, powder compactness) were demonstrated to affect LCERS measurements with better results achieved for smaller particles and lower compactness.

Effect of surface roughness of trench sidewalls on electrical properties in 4H-SiC trench MOSFETs

NASA Astrophysics Data System (ADS)

Kutsuki, Katsuhiro; Murakami, Yuki; Watanabe, Yukihiko; Onishi, Toru; Yamamoto, Kensaku; Fujiwara, Hirokazu; Ito, Takahiro

2018-04-01

The effects of the surface roughness of trench sidewalls on electrical properties have been investigated in 4H-SiC trench MOSFETs. The surface roughness of trench sidewalls was well controlled and evaluated by atomic force microscopy. The effective channel mobility at each measurement temperature was analyzed on the basis of the mobility model including optical phonon scattering. The results revealed that surface roughness scattering had a small contribution to channel mobility, and at the arithmetic average roughness in the range of 0.4-1.4 nm, there was no correlation between the experimental surface roughness and the surface roughness scattering mobility. On the other hand, the characteristics of the gate leakage current and constant current stress time-dependent dielectric breakdown tests demonstrated that surface morphology had great impact on the long-term reliability of gate oxides.

Symmetry in polarimetric remote sensing

NASA Technical Reports Server (NTRS)

Nghiem, S. V.; Yueh, S. H.; Kwok, R.

1993-01-01

Relationships among polarimetric backscattering coefficients are derived from the viewpoint of symmetry groups. For both reciprocal and non-reciprocal media, symmetry encountered in remote sensing due to reflection, rotation, azimuthal, and centrical symmetry groups is considered. The derived properties are general and valid to all scattering mechanisms, including volume and surface scatterings and their interactions, in a given symmetrical configuration. The scattering coefficients calculated from theoretical models for layer random media and rough surfaces are shown to obey the symmetry relations. Use of symmetry properties in remote sensing of structural and environmental responses of scattering media is also discussed. Orientations of spheroidal scatterers described by spherical, uniform, planophile, plagiothile, erectophile, and extremophile distributions are considered to derive their polarimetric backscattering characteristics. These distributions can be identified from the observed scattering coefficients by comparison with theoretical symmetry calculations. A new parameter is then defined to study scattering structures in geophysical media. Observations from polarimetric data acquired by the Jet Propulsion Laboratory airborne synthetic aperture radar over forests, sea ice, and sea surface are presented. Experimental evidences of the symmetry relationships are shown and their use in polarimetric remote sensing is illustrated. For forests, the coniferous forest in Mt. Shasta area (California) and mixed forest near Presque Isle (Maine) exhibit characteristics of the centrical symmetry at C-band. For sea ice in the Beaufort Sea, multi-year sea ice has a cross-polarized ratio e close to e(sub 0), calculated from symmetry, due to the randomness in the scattering structure. First-year sea ice has e much smaller than e(sub 0) due to the preferential alignment of the columnar structure of the ice. From polarimetric data of a sea surface in the Bering Sea, it is observed that e and e(sub 0) are increasing with incident angle and e is greater than e(sub 0) at L-band because of the directional feature of sea surface waves. Symmetry properties of geophysical media can also be used to calibrate polarimetric radars.

Shear-mediated contributions to the effective properties of soft acoustic metamaterials including negative index

PubMed Central

Forrester, Derek Michael; Pinfield, Valerie J.

2015-01-01

Here we show that, for sub-wavelength particles in a fluid, viscous losses due to shear waves and their influence on neighbouring particles significantly modify the effective acoustic properties, and thereby the conditions at which negative acoustic refraction occurs. Building upon earlier single particle scattering work, we adopt a multiple scattering approach to derive the effective properties (density, bulk modulus, wavenumber). We show,through theoretical prediction, the implications for the design of “soft” (ultrasonic) metamaterials based on locally-resonant sub-wavelength porous rubber particles, through selection of particle size and concentration, and demonstrate tunability of the negative speed zones by modifying the viscosity of the suspending medium. For these lossy materials with complex effective properties, we confirm the use of phase angles to define the backward propagation condition in preference to “single-” and “double-negative” designations. PMID:26686414

Multilayered phantoms with tunable optical properties for a better understanding of light/tissue interactions

NASA Astrophysics Data System (ADS)

Roig, Blandine; Koenig, Anne; Perraut, François; Piot, Olivier; Vignoud, Séverine; Lavaud, Jonathan; Manfait, Michel; Dinten, Jean-Marc

2015-03-01

Light/tissue interactions, like diffuse reflectance, endogenous fluorescence and Raman scattering, are a powerful means for providing skin diagnosis. Instrument calibration is an important step. We thus developed multilayered phantoms for calibration of optical systems. These phantoms mimic the optical properties of biological tissues such as skin. Our final objective is to better understand light/tissue interactions especially in the case of confocal Raman spectroscopy. The phantom preparation procedure is described, including the employed method to obtain a stratified object. PDMS was chosen as the bulk material. TiO2 was used as light scattering agent. Dye and ink were adopted to mimic, respectively, oxy-hemoglobin and melanin absorption spectra. By varying the amount of the incorporated components, we created a material with tunable optical properties. Monolayer and multilayered phantoms were designed to allow several characterization methods. Among them, we can name: X-ray tomography for structural information; Diffuse Reflectance Spectroscopy (DRS) with a homemade fibered bundle system for optical characterization; and Raman depth profiling with a commercial confocal Raman microscope for structural information and for our final objective. For each technique, the obtained results are presented and correlated when possible. A few words are said on our final objective. Raman depth profiles of the multilayered phantoms are distorted by elastic scattering. The signal attenuation through each single layer is directly dependent on its own scattering property. Therefore, determining the optical properties, obtained here with DRS, is crucial to properly correct Raman depth profiles. Thus, it would be permitted to consider quantitative studies on skin for drug permeation follow-up or hydration assessment, for instance.

Colors of the Sky.

ERIC Educational Resources Information Center

Bohren, Craig F.; Fraser, Alistair B.

1985-01-01

Explains the physical principles which result in various colors of the sky. Topics addressed include: blueness, mystical properties of water vapor, ozone, fluctuation theory of scattering, variation of purity and brightness, and red sunsets and sunrises. (DH)

Supercritical Fuel Measurements

DTIC Science & Technology

2012-09-01

TERMS Fuels, supercritical fluids , stimulated scattering, Brillouin scattering, Rayleigh scattering, elastic properties, thermal properties 16...10 Supercritical Cell and Fluid Handling ....................................................................................... 11...motion in supercritical fluids . Thus, the method can perform diagnostics on the heat transfer of high-temperature and high-pressure fuels, measuring

A preview of a modular surface light scattering instrument with autotracking optics

NASA Technical Reports Server (NTRS)

Meyer, William V.; Tin, Padetha; Mann, J. Adin, Jr.; Cheung, H. Michael; Rogers, Richard B.; Lading, Lars

1994-01-01

NASA's Advanced Technology Development (ATD) program is sponsoring the development of a new generation of surface light scattering hardware. This instrument is designed to non-invasively measure the surface response function of liquids over a wide range of operating conditions while automatically compensating for a sloshing surface. The surface response function can be used to compute surface tension, properties of monolayers present, viscosity, surface tension gradient and surface temperature. The instrument uses optical and electronic building blocks developed for the laser light scattering program at NASA Lewis along with several unique surface light scattering components. The emphasis of this paper is the compensation for bulk surface motion (slosh). Some data processing background information is also included.

Vertical distribution of aerosol optical properties based on aircraft measurements over the Loess Plateau in China.

PubMed

Li, Junxia; Liu, Xingang; Yuan, Liang; Yin, Yan; Li, Zhanqing; Li, Peiren; Ren, Gang; Jin, Lijun; Li, Runjun; Dong, Zipeng; Li, Yiyu; Yang, Junmei

2015-08-01

Vertical distributions of aerosol optical properties based on aircraft measurements over the Loess Plateau were measured for the first time during a summertime aircraft campaign, 2013 in Shanxi, China. Data from four flights were analyzed. The vertical distributions of aerosol optical properties including aerosol scattering coefficients (σsc), absorption coefficients (σab), Angström exponent (α), single scattering albedo (ω), backscattering ratio (βsc), aerosol mass scattering proficiency (Qsc) and aerosol surface scattering proficiency (Qsc(')) were obtained. The mean statistical values of σsc were 77.45 Mm(-1) (at 450 nm), 50.72 Mm(-1) (at 550n m), and 32.02 Mm(-1) (at 700 nm). The mean value of σab was 7.62 Mm(-1) (at 550 nm). The mean values of α, βsc and ω were 1.93, 0.15, and 0.91, respectively. Aerosol concentration decreased with altitude. Most effective diameters (ED) of aerosols were less than 0.8 μm. The vertical profiles of σsc,, α, βsc, Qsc and Qsc(') showed that the aerosol scattering properties at lower levels contributed the most to the total aerosol radiative forcing. Both α and βsc had relatively large values, suggesting that most aerosols in the observational region were small particles. The mean values of σsc, α, βsc, Qsc, Qsc('), σab and ω at different height ranges showed that most of the parameters decreased with altitude. The forty-eight hour backward trajectories of air masses during the observation days indicated that the majority of aerosols in the lower level contributed the most to the total aerosol loading, and most of these particles originated from local or regional pollution emissions. Copyright © 2015. Published by Elsevier B.V.

Impressed sources and fields in the volume-integral-equation formulation of electromagnetic scattering by a finite object: A tutorial

NASA Astrophysics Data System (ADS)

Mishchenko, Michael I.; Yurkin, Maxim A.

2018-07-01

Although free space cannot generate electromagnetic waves, the majority of existing accounts of frequency-domain electromagnetic scattering by particles and particle groups are based on the postulate of existence of an impressed incident field, usually in the form of a plane wave. In this tutorial we discuss how to account for the actual existence of impressed source currents rather than impressed incident fields. Specifically, we outline a self-consistent theoretical formalism describing electromagnetic scattering by an arbitrary finite object in the presence of arbitrarily distributed impressed currents, some of which can be far removed from the object and some can reside in its vicinity, including inside the object. To make the resulting formalism applicable to a wide range of scattering-object morphologies, we use the framework of the volume integral equation formulation of electromagnetic scattering, couple it with the notion of the transition operator, and exploit the fundamental symmetry property of this operator. Among novel results, this tutorial includes a streamlined proof of fundamental symmetry (reciprocity) relations, a simplified derivation of the Foldy equations, and an explicit analytical expression for the transition operator of a multi-component scattering object.

Dissipative quantum hydrodynamics model of x-ray Thomson scattering in dense plasmas

NASA Astrophysics Data System (ADS)

Diaw, Abdourahmane; Murillo, Michael

2017-10-01

X-ray Thomson scattering (XRTS) provides detailed diagnostic information about dense plasma experiments. The inferences made rely on an accurate model for the form factor, which is typically expressed in terms of a well-known response function. Here, we develop an alternate approach based on quantum hydrodynamics using a viscous form of dynamical density functional theory. This approach is shown to include the equation of state self-consistently, including sum rules, as well as irreversibility arising from collisions. This framework is used to generate a model for the scattering spectrum, and it offers an avenue for measuring hydrodynamic properties, such as transport coefficients, using XRTS. This work was supported by the Air Force Office of Scientific Research (Grant No. FA9550-12-1-0344).

The forward rainbow scattering of low energy protons by a graphene sheet

NASA Astrophysics Data System (ADS)

Ćosić, M.; Petrović, S.; Nešković, N.

2018-05-01

This article studies the rainbow scattering of 5-keV protons by the single sheet of free-standing graphene and its possible use as a tool for investigation of the ion-graphene interaction. The proton-graphene interaction potential was constructed by using the Doyle-Turner, ZBL, and Molière proton-carbon interaction potentials. The thermal motion of carbon atoms was included by averaging the potentials according to the Debye model. Proton trajectories were obtained by numerical solution of the corresponding Newton equations of motion. They were used to obtain the mapping of the proton initial positions to their scattering angles. Morphological properties of the introduced mapping including its multiplicity and the rainbow singularities were used to explain important features of the obtained angular distributions of transmitted protons.

Electronic structure of alloys

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ehrenreich, H.; Schwartz, L.M.

1976-01-01

The description of electronic properties of binary substitutional alloys within the single particle approximation is reviewed. Emphasis is placed on a didactic exposition of the equilibrium properties of the transport and magnetic properties of such alloys. Topics covered include: multiple scattering theory; the single band alloy; formal extensions of the theory; the alloy potential; realistic model state densities; the s-d model; and the muffin tin model. 43 figures, 3 tables, 151 references. (GHT)

Polarized optical scattering by inhomogeneities and surface roughness in an anisotropic thin film.

PubMed

Germer, Thomas A; Sharma, Katelynn A; Brown, Thomas G; Oliver, James B

2017-11-01

We extend the theory of Kassam et al. [J. Opt. Soc. Am. A12, 2009 (1995)JOAOD60740-323210.1364/JOSAA.12.002009] for scattering by oblique columnar structure thin films to include the induced form birefringence and the propagation of radiation in those films. We generalize the 4×4 matrix theory of Berreman [J. Opt. Soc. Am.62, 502 (1972)JOSAAH0030-394110.1364/JOSA.62.000502] to include arbitrary sources in the layer, which are necessary to determine the Green function for the inhomogeneous wave equation. We further extend first-order vector perturbation theory for scattering by roughness in the smooth surface limit, when the layer is anisotropic. Scattering by an inhomogeneous medium is approximated by a distorted Born approximation, where effective medium theory is used to determine the effective properties of the medium, and strong fluctuation theory is used to determine the inhomogeneous sources. In this manner, we develop a model for scattering by inhomogeneous films, with anisotropic correlation functions. The results are compared with Mueller matrix bidirectional scattering distribution function measurements for a glancing-angle deposition (GLAD) film. While the results are applied to the GLAD film example, the development of the theory is general enough that it can guide simulations for scattering in other anisotropic thin films.

Preliminary investigation of Faraday rotation effects and description of polarization measurements on the AFGL high latitude meteor scatter test bed

NASA Astrophysics Data System (ADS)

Ostergaard, Jens C.

1989-01-01

The background, methodology and preliminary results of an investigation of Faraday rotation effects on the Meteor Scatter High Latitude Test Bed in Greenland are presented. A short review of polarization theory for radio waves, presenting basic properties and changes when reflected from the surface of the earth or propagated through the ionosphere is included. Material published by other workers is presented to give the background for the current interest in Faraday rotation on meteor scatter links. Propagation losses for meteor scatter paths originate from spatial spreading of RF energy, scattering losses at the meteor trail, ionospheric absorption and polarization mismatch at the receiving antenna. That part of the polarization mismatch generated by the ionosphere, the Faraday rotation, is described and evaluated. A method to compute the Faraday rotation is presented and results obtained for the AFGL MSHL Test Bed are given. An experiment, including the measurement of signal strength and polarization throughout the lifetime of the individual meteor scatter return is needed to fully assess the combined affects of absorption and depolarization during both quiet and disturbed ionospheric conditions. The measurement accuracy to be expected from a proposed experiment is evaluated. A few examples of meteor scatter returns obtained with a prototype experiment in Greenland are shown and discussed.

On the interpolation of light-scattering responses from irregularly shaped particles

NASA Astrophysics Data System (ADS)

Videen, Gorden; Zubko, Evgenij; Arnold, Jessica A.; MacCall, Benjamin; Weinberger, Alycia J.; Shkuratov, Yuriy; Muñoz, Olga

2018-05-01

Common particle characteristics needed for many applications may include size, eccentricity, porosity and refractive index. Determining such characteristics from scattered light is a primary goal of remote sensing. For other applications, like differentiating a hazardous particle from the natural background, information about higher fidelity particle characteristics may be required, including specific shape or chemical composition. While a complete characterization of a particle system from its scattered light through the inversion process remains unachievable, great strides have been made in providing information in the form of constraints on particle characteristics. Recent advances have been made in quantifying the characteristics of polydispersions of irregularly shaped particles by making comparisons of the light-scattering signals from model simulant particles. We show that when the refractive index is changed, the light-scattering characteristics from polydispersions of such particles behave monotonically over relatively large parameter ranges compared with those of monodisperse distributions of particles having regular shapes, like spheres, spheroids, etc. This allows for their properties to be interpolated, which results in a significant reduction of the computational load when performing inversions.

Static and dynamic light scattering by red blood cells: A numerical study.

PubMed

Mauer, Johannes; Peltomäki, Matti; Poblete, Simón; Gompper, Gerhard; Fedosov, Dmitry A

2017-01-01

Light scattering is a well-established experimental technique, which gains more and more popularity in the biological field because it offers the means for non-invasive imaging and detection. However, the interpretation of light-scattering signals remains challenging due to the complexity of most biological systems. Here, we investigate static and dynamic scattering properties of red blood cells (RBCs) using two mesoscopic hydrodynamics simulation methods-multi-particle collision dynamics and dissipative particle dynamics. Light scattering is studied for various membrane shear elasticities, bending rigidities, and RBC shapes (e.g., biconcave and stomatocyte). Simulation results from the two simulation methods show good agreement, and demonstrate that the static light scattering of a diffusing RBC is not very sensitive to the changes in membrane properties and moderate alterations in cell shapes. We also compute dynamic light scattering of a diffusing RBC, from which dynamic properties of RBCs such as diffusion coefficients can be accessed. In contrast to static light scattering, the dynamic measurements can be employed to differentiate between the biconcave and stomatocytic RBC shapes and generally allow the differentiation based on the membrane properties. Our simulation results can be used for better understanding of light scattering by RBCs and the development of new non-invasive methods for blood-flow monitoring.

Static and dynamic light scattering by red blood cells: A numerical study

PubMed Central

Mauer, Johannes; Peltomäki, Matti; Poblete, Simón; Gompper, Gerhard

2017-01-01

Light scattering is a well-established experimental technique, which gains more and more popularity in the biological field because it offers the means for non-invasive imaging and detection. However, the interpretation of light-scattering signals remains challenging due to the complexity of most biological systems. Here, we investigate static and dynamic scattering properties of red blood cells (RBCs) using two mesoscopic hydrodynamics simulation methods—multi-particle collision dynamics and dissipative particle dynamics. Light scattering is studied for various membrane shear elasticities, bending rigidities, and RBC shapes (e.g., biconcave and stomatocyte). Simulation results from the two simulation methods show good agreement, and demonstrate that the static light scattering of a diffusing RBC is not very sensitive to the changes in membrane properties and moderate alterations in cell shapes. We also compute dynamic light scattering of a diffusing RBC, from which dynamic properties of RBCs such as diffusion coefficients can be accessed. In contrast to static light scattering, the dynamic measurements can be employed to differentiate between the biconcave and stomatocytic RBC shapes and generally allow the differentiation based on the membrane properties. Our simulation results can be used for better understanding of light scattering by RBCs and the development of new non-invasive methods for blood-flow monitoring. PMID:28472125

Microwave model prediction and verifications for vegetated terrain

NASA Technical Reports Server (NTRS)

Fung, A. K.

1985-01-01

To understand the scattering properties of a deciduous and a coniferous type vegetation scattering models were developed assuming either a disc type leaf or a needle type leaf. The major effort is to calculate the corresponding scattering phase functions and then each of the functions is used in a radiative transfer formulation to compute the scattering intensity and consequently the scattering coefficient. The radiative transfer formulation takes into account the irregular ground surface by including the rough soil surface in the boundary condition. Thus, the scattering model accounts for volume scattering inside the vegetation layer, the surface scattering from the ground and the interaction between scattering from the soil surface and the vegetation volume. The contribution to backscattering by each of the three scattering mechanisms is illustrated along with the effects of each layer or surface parameter. The major difference between the two types of vegetation is that when the incident wavelength is comparable to the size of the leaf there is a peak appearing in the mid angular region of the backscattering curve for the disc type leaf whereas it is a dip in the same region for a needle type leaf.

High Spectral Resolution Lidar Measurements of Multiple Scattering

NASA Technical Reports Server (NTRS)

Eloranta, E. W.; Piironen, P.

1996-01-01

The University of Wisconsin High Spectral Resolution Lidar (HSRL) provides unambiguous measurements of backscatter cross section, backscatter phase function, depolarization, and optical depth. This is accomplished by dividing the lidar return into separate particulate and molecular contributions. The molecular return is then used as a calibration target. We have modified the HSRL to use an I2 molecular absorption filter to separate aerosol and molecular signals. This allows measurement in dense clouds. Useful profiles extend above the cloud base until the two way optical depth reaches values between 5 and 6; beyond this, photon counting errors become large. In order to observe multiple scattering, the HSRL includes a channel which records the combined aerosol and molecular lidar return simultaneously with the spectrometer channel measurements of optical properties. This paper describes HSRL multiple scattering measurements from both water and ice clouds. These include signal strengths and depolarizations as a function of receiver field of view. All observations include profiles of extinction and backscatter cross sections. Measurements are also compared to predictions of a multiple scattering model based on small angle approximations.

Impact of Snow Grain Shape and Internal Mixing with Black Carbon Aerosol on Snow Optical Properties for use in Climate Models

NASA Astrophysics Data System (ADS)

He, C.; Liou, K. N.; Takano, Y.; Yang, P.; Li, Q.; Chen, F.

2017-12-01

A set of parameterizations is developed for spectral single-scattering properties of clean and black carbon (BC)-contaminated snow based on geometric-optic surface-wave (GOS) computations, which explicitly resolves BC-snow internal mixing and various snow grain shapes. GOS calculations show that, compared with nonspherical grains, volume-equivalent snow spheres show up to 20% larger asymmetry factors and hence stronger forward scattering, particularly at wavelengths <1 mm. In contrast, snow grain sizes have a rather small impact on the asymmetry factor at wavelengths <1 mm, whereas size effects are important at longer wavelengths. The snow asymmetry factor is parameterized as a function of effective size, aspect ratio, and shape factor, and shows excellent agreement with GOS calculations. According to GOS calculations, the single-scattering coalbedo of pure snow is predominantly affected by grain sizes, rather than grain shapes, with higher values for larger grains. The snow single-scattering coalbedo is parameterized in terms of the effective size that combines shape and size effects, with an accuracy of >99%. Based on GOS calculations, BC-snow internal mixing enhances the snow single-scattering coalbedo at wavelengths <1 mm, but it does not alter the snow asymmetry factor. The BC-induced enhancement ratio of snow single-scattering coalbedo, independent of snow grain size and shape, is parameterized as a function of BC concentration with an accuracy of >99%. Overall, in addition to snow grain size, both BC-snow internal mixing and snow grain shape play critical roles in quantifying BC effects on snow optical properties. The present parameterizations can be conveniently applied to snow, land surface, and climate models including snowpack radiative transfer processes.

Absorption Filter Based Optical Diagnostics in High Speed Flows

NASA Technical Reports Server (NTRS)

Samimy, Mo; Elliott, Gregory; Arnette, Stephen

1996-01-01

Two major regimes where laser light scattered by molecules or particles in a flow contains significant information about the flow are Mie scattering and Rayleigh scattering. Mie scattering is used to obtain only velocity information, while Rayleigh scattering can be used to measure both the velocity and the thermodynamic properties of the flow. Now, recently introduced (1990, 1991) absorption filter based diagnostic techniques have started a new era in flow visualization, simultaneous velocity and thermodynamic measurements, and planar velocity measurements. Using a filtered planar velocimetry (FPV) technique, we have modified the optically thick iodine filter profile of Miles, et al., and used it in the pressure-broaden regime which accommodates measurements in a wide range of velocity applications. Measuring velocity and thermodynamic properties simultaneously, using absorption filtered based Rayleigh scattering, involves not only the measurement of the Doppler shift, but also the spectral profile of the Rayleigh scattering signal. Using multiple observation angles, simultaneous measurement of one component velocity and thermodynamic properties in a supersonic jet were measured. Presently, the technique is being extended for simultaneous measurements of all three components of velocity and thermodynamic properties.

Are Planetary Regolith Particles Back Scattering? Response to a Paper by M. Mishchenko

NASA Technical Reports Server (NTRS)

Hapke, Bruce

1996-01-01

In a recent paper Mishchenko asserts that soil particles are strongly forward scattering, whereas particles on the surfaces of objects in the solar system have been inferred to be back scattering. Mishchenko suggests that this apparent discrepancy is an artifact caused by using an approximate light scattering model to analyse the data, and that planetary regolith particles are actually strong forward scatterers. The purpose of the present paper is to point out the errors in Mishchenko's paper and to show from both theoretical arguments and experimental data that inhomogencous composite particles which are large compared to the wavelength of visible light, such as rock fragments and agglutinates, can be strongly back scattering and are the fundamental scatterers in media composed of them. Such particles appear to be abundant in planetary regoliths and can account for the back scattering character of the surfaces of many bodies in the solar system. If the range of phase angles covered by a data set is insufficient, serious errors in retrieving the particle scattering properties can result whether an exact or approximate scattering model is used. However, if the data set includes both large and small phase angles, approximate regolith scattering models can correctly retrieve the sign of the particle scattering asymmetry.

Influence of diffuse reflectance measurement accuracy on the scattering coefficient in determination of optical properties with integrating sphere optics (a secondary publication).

PubMed

Horibe, Takuro; Ishii, Katsunori; Fukutomi, Daichi; Awazu, Kunio

2015-12-30

An estimation error of the scattering coefficient of hemoglobin in the high absorption wavelength range has been observed in optical property calculations of blood-rich tissues. In this study, the relationship between the accuracy of diffuse reflectance measurement in the integrating sphere and calculated scattering coefficient was evaluated with a system to calculate optical properties combined with an integrating sphere setup and the inverse Monte Carlo simulation. Diffuse reflectance was measured with the integrating sphere using a small incident port diameter and optical properties were calculated. As a result, the estimation error of the scattering coefficient was improved by accurate measurement of diffuse reflectance. In the high absorption wavelength range, the accuracy of diffuse reflectance measurement has an effect on the calculated scattering coefficient.

Generic Detection of Register Realignment

NASA Astrophysics Data System (ADS)

Ďurfina, Lukáš; Kolář, Dušan

2011-09-01

The register realignment is a method of binary obfuscation and it is used by malware writers. The paper introduces the method how register realignment can be recognized by analysis based on the scattered context grammars. Such an analysis includes exploration of bytes affected by realignment, finding new valid values for them, building the scattered context grammar and parse an obfuscated code by this grammar. The created grammar has LL property--an ability for parsing by this type of grammar.

Relationship between the Kubelka-Munk scattering and radiative transfer coefficients.

PubMed

Thennadil, Suresh N

2008-07-01

The relationship between the Kubelka-Munk (K-M) and the transport scattering coefficient is obtained through a semi-empirical approach. This approach gives the same result as that given by Gate [Appl. Opt.13, 236 (1974)] when the incident beam is diffuse. This result and those given by Star et al. [Phys. Med. Biol.33, 437 (1988)] and Brinkworth [Appl. Opt.11, 1434 (1972)] are compared with the exact solution of the radiative transfer equation over a large range of optical properties. It is found that the latter expressions, which include an absorption component, do not give accurate results over the range considered. Using the semi-empirical approach, the relationship between the K-M and the transport scattering coefficient is derived for the case where the incident light is collimated. It is shown that although the K-M equation is derived based on diffuse incident light, it can also represent very well the reflectance from a slab of infinite thickness when the incident light is collimated. However, in this case the relationship between the coefficients has to include a function that is dependent on the anisotropy factor. Analysis indicates that the K-M transform achieves the objective of obtaining a measure that gives the ratio of absorption to scattering effects for both diffuse and collimated incident beams over a large range of optical properties.

Aerosol analysis with the Coastal Zone Color Scanner - A simple method for including multiple scattering effects

NASA Technical Reports Server (NTRS)

Gordon, Howard R.; Castano, Diego J.

1989-01-01

A method for studying aerosols over the ocean using Nimbus-7 CZCS data is proposed which circumvents having to perform radiative transfer computations involving the aerosol properties. The method is applied to the CZCS band 4 at 670 nm, and yields the total radiance (L sub t) backscattered from the top of a stratified atmosphere containing both stratospheric and tropospheric aerosols and the the Rayleigh scattered radiance (L sub r). The radiance which the aerosol would produce in the single scattering approximation is retrieved from (L sub t) - (L sub r) with an error of not greater than 5-7 percent.

Particle size analysis in a turbid media with a single-fiber, optical probe while using a visible spectrometer

DOEpatents

Canpolat, Murat; Mourant, Judith R.

2003-12-09

Apparatus and method for measuring scatterer size in a dense media with only a single fiber for both light delivery and collection are disclosed. White light is used as a source and oscillations of the detected light intensities are measured as a function of wavelength. The maximum and minimum of the oscillations can be used to determine scatterer size for monodisperse distributions of spheres when the refractive indices are known. In addition several properties of the probe relevant to tissue diagnosis are disclosed including the effects of absorption, a broad distribution of scatterers, and the depth probed.

POlarized Light Angle Reflectance Instrument I Polarized Incidence (POLAR:I)

NASA Technical Reports Server (NTRS)

Sarto, Anthony W.; Woldemar, Christopher M.; Vanderbilt, V. C.

1989-01-01

The light scattering properties of leaves are used as input data for models which mathematically describe the transport of photons within plant canopies. Polarization measurements may aid in the investigation of these properties. This paper describes an instrument for rapidly determining the bidirectional light scattering properties of leaves illuminated by linearly polarized light. Results for one species, magnolia, show large differences in the bidirectional light scattering properties depending whether or not the electric vector E is parallel to the foliage surface.

Light scattering properties of self-organized nanostructured substrates for thin-film solar cells.

PubMed

Mennucci, C; Del Sorbo, S; Pirotta, S; Galli, M; Andreani, L C; Martella, C; Giordano, M C; Buatier de Mongeot, F

2018-06-01

We investigate the scattering properties of novel kinds of nano-textured substrates, fabricated in a self-organized fashion by defocused ion beam sputtering. These substrates provide strong and broadband scattering of light and can be useful for applications in thin-film solar cells. In particular, we characterize the transmitted light in terms of haze and angle-resolved scattering, and we compare our results with those obtained for the commonly employed Asahi-U texture. The results indicate that the novel substrate has better scattering properties compared to reference Asahi-U substrates. We observe super-Lambertian light scattering behavior in selected spectral and angular regions due to the peculiar morphology of the nano-textured interface, which combines high aspect ratio pseudo random structures with a one-dimensional periodic pattern. The enhancement of light absorption observed in a prototype thin film semiconductor absorber grown on nano-textured glass with respect to an Asahi-U substrate further confirms the superior light trapping properties of the novel substrate.

Light scattering properties of spheroidal particles

NASA Technical Reports Server (NTRS)

Asano, S.

1979-01-01

In the present paper, the light scattering characteristics of spheroidal particles are evaluated within the framework of a scattering theory developed for a homogeneous isotropic spheroid. This approach is shown to be well suited for computing the scattering quantities of spheroidal particles of fairly large sizes (up to a size parameter of 30). The effects of particle size, shape, index of refraction, and orientation on the scattering efficiency factors and the scattering intensity functions are studied and interpreted physically. It is shown that, in the case of oblique incidence, the scattering properties of a long slender prolate spheroid resemble those of an infinitely long circular cylinder.

Metallic Iron and Iron Oxide as an Explanation for the Dark Material Observed on Saturn's Icy Satellites and Rings with Cassini VIMS

NASA Astrophysics Data System (ADS)

Clark, Roger Nelson; Cruikshank, D. P.; Jaumann, R.; Brown, R. H.; Dalle Ore, C.; Stephan, K.; Hoefen, T. M.; Curchin, J. M.; Buratti, B. J.; Filacchione, G.; Baines, K. H.; Nicholson, P. D.

2010-10-01

The Visual and Infrared Mapping Spectrometer (VIMS) on Cassini has obtained spatially resolved spectra on satellites of Saturn. The Cassini Rev 49 Iapetus fly-by on September 10, 2007, provided data on both the dark material and the transition zone between the dark material and the visually bright ice. The dark material has low albedo with a linear increase in reflectance with wavelength, 3-micron water, and CO2 absorptions. The transition between bright and dark regions shows mixing with unusual optical properties including increased blue scattering and increasing strength of a UV absorber in areas with stronger ice absorptions. Similar spectral effects are observed on other Saturnian satellites and in the rings. We have been unable to match these spectral properties and trends using tholins and carbon compounds. However, the dark material is spectrally matched by fine-grained metallic iron plus nano-phase hematite and adsorbed water which contribute UV and 3-micron absorption, respectively. The blue scattering peak and UV absorption can be explained by Rayleigh scattering from sub-micron particles with a UV absorption, or a combination of Rayleigh scattering and Rayleigh absorption as has been attributed to spectral properties of the Moon. A new radiative transfer model that includes Rayleigh scattering and Rayleigh absorption has been constructed. Models of ice, sub-micron metallic iron, hydrated iron oxide, and trace CO2 explain the observed spectra. Rayleigh absorption requires high absorption coefficient nano-sized particles, which is also consistent with metallic iron. The UV absorber appears to have increased strength on satellite surfaces close to Saturn, with a corresponding decrease in metallic iron signature. A possible explanation is that the iron is oxidized closer to Saturn by oxygen in the extended atmosphere of Saturn's rings, or the dark material is simply covered by clean fine-grained ice particles, for example, from the E-ring.

Scattering and Absorption Properties of Biomaterials for Dental Restorative Applications

NASA Astrophysics Data System (ADS)

Fernandez-Oliveras, A.; Rubiño, M.; Pérez, M. M.

2013-08-01

The physical understanding of the optical properties of dental biomaterials is mandatory for their final success in restorative applications.Light propagation in biological media is characterized by the absorption coefficient, the scattering coefficient, the scattering phase function,the refractive index, and the surface conditions (roughness). We have employed the inverse adding-doubling (IAD) method to combine transmittance and reflectance measurements performed using an integrating-sphere setup with the results of the previous scattering-anisotropygoniometric measurements. This has led to the determination of the absorption and the scattering coefficients. The aim was to optically characterize two different dental-resin composites (nanocomposite and hybrid) and one type of zirconia ceramic, and comparatively study them. The experimental procedure was conducted under repeatability conditions of measurement in order to determine the uncertainty associated to the optical properties of the biomaterials. Spectral variations of the refraction index and the scattering anisotropy factor were also considered. The whole experimental procedure fulfilled all the necessary requirements to provide optical-property values with lower associated uncertainties. The effective transport coefficient presented a similar spectral behavior for the two composites but completely different for the zirconia ceramic. The results demonstrated that the scattering anisotropy exerted a clearly distinct impact on the optical properties of the zirconia ceramic compared with those of the dental-resin composites.

Apparatus for measuring particle properties

DOEpatents

Rader, Daniel J.; Castaneda, Jaime N.; Grasser, Thomas W.; Brockmann, John E.

1998-01-01

An apparatus for determining particle properties from detected light scattered by the particles. The apparatus uses a light beam with novel intensity characteristics to discriminate between particles that pass through the beam and those that pass through an edge of the beam. The apparatus can also discriminate between light scattered by one particle and light scattered by multiple particles. The particle's size can be determined from the intensity of the light scattered. The particle's velocity can be determined from the elapsed time between various intensities of the light scattered.

Cotton fiber quality characterization with light scattering and fourier transform infrared techniques.

PubMed

Thomasson, J A; Manickavasagam, S; Mengüç, M P

2009-03-01

Fiber quality measurement is critical to assessing the value of a bale of cotton for various textile purposes. An instrument that could measure numerous cotton quality properties by optical means could be made simpler and faster than current fiber quality measurement instruments, and it might be more amenable to on-line measurement at processing facilities. To that end, a laser system was used to investigate cotton fiber samples with respect to electromagnetic scattering at various wavelengths, polarization angles, and scattering angles. A Fourier transform infrared (FT-IR) instrument was also used to investigate the transmission of electromagnetic energy at various mid-infrared wavelengths. Cotton samples were selected to represent a wide range of micronaire values. Varying the wavelength of the laser at a fixed polarization resulted in little variation in scattered light among the cotton samples. However, varying the polarization at a fixed wavelength produced notable variation, indicating that polarization might be used to differentiate among cotton samples with respect to certain fiber properties. The FT-IR data in the 12 to 22 microm range produced relatively large differences in the amount of scattered light among all samples, and FT-IR data at certain combinations of fixed wavelengths were highly linearly related to certain measures of cotton quality including micronaire.

On the radiative properties of soot aggregates part 1: Necking and overlapping

NASA Astrophysics Data System (ADS)

Yon, J.; Bescond, A.; Liu, F.

2015-09-01

There is a strong interest in accurately modelling the radiative properties of soot aggregates (also known as black carbon particles) emitted from combustion systems and fires to gain improved understanding of the role of black carbon to global warming. This study conducted a systematic investigation of the effects of overlapping and necking between neighbouring primary particles on the radiative properties of soot aggregates using the discrete dipole approximation. The degrees of overlapping and necking are quantified by the overlapping and necking parameters. Realistic soot aggregates were generated numerically by constructing overlapping and necking to fractal aggregates formed by point-touch primary particles simulated using a diffusion-limited cluster aggregation algorithm. Radiative properties (differential scattering, absorption, total scattering, specific extinction, asymmetry factor and single scattering albedo) were calculated using the experimentally measured soot refractive index over the spectral range of 266-1064 nm for 9 combinations of the overlapping and necking parameters. Overlapping and necking affect significantly the absorption and scattering properties of soot aggregates, especially in the near UV spectrum due to the enhanced multiple scattering effects within an aggregate. By using correctly modified aggregate properties (fractal dimension, prefactor, primary particle radius, and the number of primary particle) and by accounting for the effects of multiple scattering, the simple Rayleigh-Debye-Gans theory for fractal aggregates can reproduce reasonably accurate radiative properties of realistic soot aggregates.

Evaluation of light scattering properties and chromophore concentrations in skin tissue based on diffuse reflectance signals at isosbestic wavelengths of hemoglobin

NASA Astrophysics Data System (ADS)

Yokokawa, Takumi; Nishidate, Izumi

2016-04-01

We investigate a method to evaluate light-scattering properties and chromophore concentrations in human skin tissue through diffuse reflectance spectroscopy using the reflectance signals acquired at isosbestic wavelengths of hemoglobin (420, 450, 500, and 585 nm). In the proposed method, Monte Carlo simulation-based empirical formulas are used to specify the scattering parameters of skin tissue, such as the scattering amplitude a and the scattering power b, as well as the concentration of melanin C m and the total blood concentration C tb. The use of isosbestic wavelengths of hemoglobin enables the values of C m, C tb, a, and b to be estimated independently of the oxygenation of hemoglobin. The spectrum of the reduced scattering coefficient is reconstructed from the scattering parameters. Experiments using in vivo human skin tissues were performed to confirm the feasibility of the proposed method for evaluating the changes in scattering properties and chromophore concentrations in skin tissue. The experimental results revealed that light scattering is significantly reduced by the application of a glycerol solution, which indicates an optical clearing effect due to osmotic dehydration and the matching of the refractive indices of scatterers in the epidermis.

Refractive indices at visible wavelengths of soot emitted from buoyant turbulent diffusion flames

DOE Office of Scientific and Technical Information (OSTI.GOV)

Wu, J.S.; Krishnan, S.K.; Faeth, G.M.

1996-11-01

Measurements of the optical properties of soot, emphasizing refractive indices, are reported for visible wavelengths. The experiments considered soot in the fuel-lean (overfire) region of buoyant turbulent diffusion flames in the long residence time regime where soot properties are independent of position in the overfire region and residence time. Flames fueled with acetylene, propylene, ethylene and propane burning in still air provided a range of soot physical and structure properties. Measurements included soot composition, density, structure, gravimetric volume fraction, scattering properties and absorption properties. These data were analyzed to find soot fractal dimensions, refractive indices and dimensionless extinction coefficients, assumingmore » Rayleigh-Debye-Gans scattering for polydisperse mass fractal aggregates (RDG-PFA theory). RDG-PFA theory was successfully evaluated, based on measured scattering patterns. Soot fractal dimensions were independent of both fuel type and wavelength, yielding a mean value of 1.77 with a standard deviation of 0.04. Refractive indices were independent of fuel type within experimental uncertainties and were in reasonably good agreement with earlier measurements for soot in the fuel-lean region of diffusion flames due to Dalzell and Sarofim (1969). Dimensionless extinction coefficients were independent of both fuel type and wavelength, yielding a mean value of 5.1 with a standard deviation of 0.5, which is lower than earlier measurements for reasons that still must be explained.« less

Phonon Lifetime Observation in Epitaxial ScN Film with Inelastic X-Ray Scattering Spectroscopy.

PubMed

Uchiyama, H; Oshima, Y; Patterson, R; Iwamoto, S; Shiomi, J; Shimamura, K

2018-06-08

Phonon-phonon scattering dominates the thermal properties in nonmetallic materials, and it directly influences device performance in applications. The understanding of the scattering has been progressing using computational approaches, and the direct and systematic observation of phonon modes that include momentum dependences is desirable. We report experimental data on the phonon dispersion curves and lifetimes in an epitaxially grown ScN film using inelastic x-ray scattering measurements. The momentum dependence of the optical phonon lifetimes is estimated from the spectral width, and the highest-energy phonon mode around the zone center is found to possess a short lifetime of 0.21 ps. A comparison with first-principles calculations shows that our observed phonon lifetimes are quantitatively explained by three-body phonon-phonon interactions.

Reflection and extinction of light by self-assembled monolayers of a quinque-thiophene derivative: A coherent scattering approach

DOE Office of Scientific and Technical Information (OSTI.GOV)

Gholamrezaie, Fatemeh; Meskers, Stefan C. J., E-mail: s.c.j.meskers@tue.nl; Leeuw, Dago M. de

Scattering matrix theory is used to describe resonant optical properties of molecular monolayers. Three types of coupling are included: exciton-exciton, exciton-photon, and exciton-phonon coupling. We use the K-matrix formalism, developed originally to describe neutron scattering spectra in nuclear physics to compute the scattering of polaritons by phonons. This perturbation approach takes into account the three couplings and allows one to go beyond molecular exciton theory without the need of introducing additional boundary conditions for the polariton. We demonstrate that reflection, absorption, and extinction of light by 2D self-assembled monolayers of molecules containing quinque-thiophene chromophoric groups can be calculated. The extractedmore » coherence length of the Frenkel exciton is discussed.« less

Phonon Lifetime Observation in Epitaxial ScN Film with Inelastic X-Ray Scattering Spectroscopy

NASA Astrophysics Data System (ADS)

Uchiyama, H.; Oshima, Y.; Patterson, R.; Iwamoto, S.; Shiomi, J.; Shimamura, K.

2018-06-01

Phonon-phonon scattering dominates the thermal properties in nonmetallic materials, and it directly influences device performance in applications. The understanding of the scattering has been progressing using computational approaches, and the direct and systematic observation of phonon modes that include momentum dependences is desirable. We report experimental data on the phonon dispersion curves and lifetimes in an epitaxially grown ScN film using inelastic x-ray scattering measurements. The momentum dependence of the optical phonon lifetimes is estimated from the spectral width, and the highest-energy phonon mode around the zone center is found to possess a short lifetime of 0.21 ps. A comparison with first-principles calculations shows that our observed phonon lifetimes are quantitatively explained by three-body phonon-phonon interactions.

Experimental Phase Functions of Millimeter-sized Cosmic Dust Grains

NASA Astrophysics Data System (ADS)

Muñoz, O.; Moreno, F.; Vargas-Martín, F.; Guirado, D.; Escobar-Cerezo, J.; Min, M.; Hovenier, J. W.

2017-09-01

We present the experimental phase functions of three types of millimeter-sized dust grains consisting of enstatite, quartz, and volcanic material from Mount Etna, respectively. The three grains present similar sizes but different absorbing properties. The measurements are performed at 527 nm covering the scattering angle range from 3° to 170°. The measured phase functions show two well-defined regions: (I) soft forward peaks and (II) a continuous increase with the scattering angle at side- and back-scattering regions. This behavior at side- and back-scattering regions is in agreement with the observed phase functions of the Fomalhaut and HR 4796A dust rings. Further computations and measurements (including polarization) for millimeter-sized grains are needed to draw some conclusions about the fluffy or compact structure of the dust grains.

The Momentum Distribution of Liquid ⁴He

DOE PAGES

Prisk, T. R.; Bryan, M. S.; Sokol, P. E.; ...

2017-07-24

We report a high-resolution neutron Compton scattering study of liquid ⁴He under milli-Kelvin temperature control. To interpret the scattering data, we performed Quantum Monte Carlo calculations of the atomic momentum distribution and final state effects for the conditions of temperature and density considered in the experiment. There is excellent agreement between the observed scattering and ab initio calculations of its lineshape at all temperatures. We also used model fit functions to obtain from the scattering data empirical estimates of the average atomic kinetic energy and Bose condensate fraction. These quantities are also in excellent agreement with ab initio calculations. Wemore » conclude that contemporary Quantum Monte Carlo methods can furnish accurate predictions for the properties of Bose liquids, including the condensate fraction, close to the superfluid transition temperature.« less

TRUST. I. A 3D externally illuminated slab benchmark for dust radiative transfer

NASA Astrophysics Data System (ADS)

Gordon, K. D.; Baes, M.; Bianchi, S.; Camps, P.; Juvela, M.; Kuiper, R.; Lunttila, T.; Misselt, K. A.; Natale, G.; Robitaille, T.; Steinacker, J.

2017-07-01

Context. The radiative transport of photons through arbitrary three-dimensional (3D) structures of dust is a challenging problem due to the anisotropic scattering of dust grains and strong coupling between different spatial regions. The radiative transfer problem in 3D is solved using Monte Carlo or Ray Tracing techniques as no full analytic solution exists for the true 3D structures. Aims: We provide the first 3D dust radiative transfer benchmark composed of a slab of dust with uniform density externally illuminated by a star. This simple 3D benchmark is explicitly formulated to provide tests of the different components of the radiative transfer problem including dust absorption, scattering, and emission. Methods: The details of the external star, the slab itself, and the dust properties are provided. This benchmark includes models with a range of dust optical depths fully probing cases that are optically thin at all wavelengths to optically thick at most wavelengths. The dust properties adopted are characteristic of the diffuse Milky Way interstellar medium. This benchmark includes solutions for the full dust emission including single photon (stochastic) heating as well as two simplifying approximations: One where all grains are considered in equilibrium with the radiation field and one where the emission is from a single effective grain with size-distribution-averaged properties. A total of six Monte Carlo codes and one Ray Tracing code provide solutions to this benchmark. Results: The solution to this benchmark is given as global spectral energy distributions (SEDs) and images at select diagnostic wavelengths from the ultraviolet through the infrared. Comparison of the results revealed that the global SEDs are consistent on average to a few percent for all but the scattered stellar flux at very high optical depths. The image results are consistent within 10%, again except for the stellar scattered flux at very high optical depths. The lack of agreement between different codes of the scattered flux at high optical depths is quantified for the first time. Convergence tests using one of the Monte Carlo codes illustrate the sensitivity of the solutions to various model parameters. Conclusions: We provide the first 3D dust radiative transfer benchmark and validate the accuracy of this benchmark through comparisons between multiple independent codes and detailed convergence tests.

Remote sensing of Earth terrain

NASA Technical Reports Server (NTRS)

Kong, Jin AU; Yueh, Herng-Aung

1990-01-01

The layered random medium model is used to investigate the fully polarimetric scattering of electromagnetic waves from vegetation. The vegetation canopy is modeled as an anisotropic random medium containing nonspherical scatterers with preferred alignment. The underlying medium is considered as a homogeneous half space. The scattering effect of the vegetation canopy are characterized by 3-D correlation functions with variances and correlation lengths respectively corresponding to the fluctuation strengths and the physical geometries of the scatterers. The strong fluctuation theory is used to calculate the anisotropic effective permittivity tensor of the random medium and the distorted Born approximation is then applied to obtain the covariance matrix which describes the fully polarimetric scattering properties of the vegetation field. This model accounts for all the interaction processes between the boundaries and the scatterers and includes all the coherent effects due to wave propagation in different directions such as the constructive and destructive interferences. For a vegetation canopy with low attenuation, the boundary between the vegetation and the underlying medium can give rise to significant coherent effects.

Fast radiative transfer models for retrieval of cloud properties in the back-scattering region: application to DSCOVR-EPIC sensor

NASA Astrophysics Data System (ADS)

Molina Garcia, Victor; Sasi, Sruthy; Efremenko, Dmitry; Doicu, Adrian; Loyola, Diego

2017-04-01

In this work, the requirements for the retrieval of cloud properties in the back-scattering region are described, and their application to the measurements taken by the Earth Polychromatic Imaging Camera (EPIC) on board the Deep Space Climate Observatory (DSCOVR) is shown. Various radiative transfer models and their linearizations are implemented, and their advantages and issues are analyzed. As radiative transfer calculations in the back-scattering region are computationally time-consuming, several acceleration techniques are also studied. The radiative transfer models analyzed include the exact Discrete Ordinate method with Matrix Exponential (DOME), the Matrix Operator method with Matrix Exponential (MOME), and the approximate asymptotic and equivalent Lambertian cloud models. To reduce the computational cost of the line-by-line (LBL) calculations, the k-distribution method, the Principal Component Analysis (PCA) and a combination of the k-distribution method plus PCA are used. The linearized radiative transfer models for retrieval of cloud properties include the Linearized Discrete Ordinate method with Matrix Exponential (LDOME), the Linearized Matrix Operator method with Matrix Exponential (LMOME) and the Forward-Adjoint Discrete Ordinate method with Matrix Exponential (FADOME). These models were applied to the EPIC oxygen-A band absorption channel at 764 nm. It is shown that the approximate asymptotic and equivalent Lambertian cloud models give inaccurate results, so an offline processor for the retrieval of cloud properties in the back-scattering region requires the use of exact models such as DOME and MOME, which behave similarly. The combination of the k-distribution method plus PCA presents similar accuracy to the LBL calculations, but it is up to 360 times faster, and the relative errors for the computed radiances are less than 1.5% compared to the results when the exact phase function is used. Finally, the linearized models studied show similar behavior, with relative errors less than 1% for the radiance derivatives, but FADOME is 2 times faster than LDOME and 2.5 times faster than LMOME.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Datta, Kaustuv; Neder, Reinhard B.; Chen, Jun

Revelation of unequivocal structural information at the atomic level for complex systems is uniquely important for deeper and generic understanding of the structure property connections and a key challenge in materials science. Here in this paper we report an experimental study of the local structure by applying total elastic scattering and Raman scattering analyses to an important non-relaxor ferroelectric solid solution exhibiting the so-called composition-induced morphotropic phase boundary (MPB), where concomitant enhancement of physical properties have been detected. The powerful combination of static and dynamic structural probes enabled us to derive direct correspondence between the atomic-level structural correlations and reportedmore » properties. The atomic pair distribution functions obtained from the neutron total scattering experiments were analysed through big-box atom-modelling implementing reverse Monte Carlo method, from which distributions of magnitudes and directions of off-centred cationic displacements were extracted. We found that an enhanced randomness of the displacement-directions for all ferroelectrically active cations combined with a strong dynamical coupling between the A- and B-site cations of the perovskite structure, can explain the abrupt amplification of piezoelectric response of the system near MPB. Finally, altogether this provides a more fundamental basis in inferring structure-property connections in similar systems including important implications in designing novel and bespoke materials.« less

Frequency-domain method for measuring spectral properties in multiple-scattering media: methemoglobin absorption spectrum in a tissuelike phantom

NASA Astrophysics Data System (ADS)

Fishkin, Joshua B.; So, Peter T. C.; Cerussi, Albert E.; Gratton, Enrico; Fantini, Sergio; Franceschini, Maria Angela

1995-03-01

We have measured the optical absorption and scattering coefficient spectra of a multiple-scattering medium (i.e., a biological tissue-simulating phantom comprising a lipid colloid) containing methemoglobin by using frequency-domain techniques. The methemoglobin absorption spectrum determined in the multiple-scattering medium is in excellent agreement with a corrected methemoglobin absorption spectrum obtained from a steady-state spectrophotometer measurement of the optical density of a minimally scattering medium. The determination of the corrected methemoglobin absorption spectrum takes into account the scattering from impurities in the methemoglobin solution containing no lipid colloid. Frequency-domain techniques allow for the separation of the absorbing from the scattering properties of multiple-scattering media, and these techniques thus provide an absolute

Radiative properties of flame-generated soot

DOE Office of Scientific and Technical Information (OSTI.GOV)

Koeylue, U.O.; Faeth, G.M.

1993-05-01

Approximate methods for estimating the optical properties of flame-generated soot aggregates were evaluated using existing computer simulations and measurements in the visible and near-infrared portions of the spectrum. The following approximate methods were evaluated for both individual aggregates and polydisperse aggregate populations: the Rayleigh scattering approximation, Mie scattering for an equivalent sphere, and Rayleigh-Debye-Gans (R-D-G) scattering for both given and fractal aggregates. Results of computer simulations involved both prescribed aggregate geometry and numerically generated aggregates by cluster-cluster aggregation; multiple scattering was considered exactly using the mean-field approximation, and ignored using the R-D-G approximation. Measurements involved the angular scattering properties ofmore » soot in the postflame regions of both premixed and nonpremixed flames. The results show that available computer simulations and measurements of soot aggregate optical properties are not adequate to provide a definitive evaluation of the approximate prediction methods. 40 refs., 7 figs., 1 tab.« less

The Measurement of Aerosol Optical Properties using Continuous Wave Cavity Ring-Down Techniques

NASA Technical Reports Server (NTRS)

Strawa, Anthony W.; Castaneda, Rene; Owano, Thomas; Baer, Douglas S.; Paldus, Barbara A.; Gore, Warren J. (Technical Monitor)

2002-01-01

Large uncertainties in the effects that aerosols have on climate require improved in situ measurements of extinction coefficient and single-scattering albedo. This paper describes the use of continuous wave cavity ring-down (CW-CRD) technology to address this problem. The innovations in this instrument are the use of CW-CRD to measure aerosol extinction coefficient, the simultaneous measurement of scattering coefficient, and small size suitable for a wide range of aircraft applications. Our prototype instrument measures extinction and scattering coefficient at 690 nm and extinction coefficient at 1550 nm. The instrument itself is small (60 x 48 x 15 cm) and relatively insensitive to vibrations. The prototype instrument has been tested in our lab and used in the field. While improvements in performance are needed, the prototype has been shown to make accurate and sensitive measurements of extinction and scattering coefficients. Combining these two parameters, one can obtain the single-scattering albedo and absorption coefficient, both important aerosol properties. The use of two wavelengths also allows us to obtain a quantitative idea of the size of the aerosol through the Angstrom exponent. Minimum sensitivity of the prototype instrument is 1.5 x 10(exp -6)/m (1.5 M/m). Validation of the measurement of extinction coefficient has been accomplished by comparing the measurement of calibration spheres with Mie calculations. This instrument and its successors have potential to help reduce uncertainty currently associated with aerosol optical properties and their spatial and temporal variation. Possible applications include studies of visibility, climate forcing by aerosol, and the validation of aerosol retrieval schemes from satellite data.

The Measurement of Aerosol Optical Properties Using Continuous Wave Cavity Ring-Down Techniques

NASA Technical Reports Server (NTRS)

Strawa, A. W.; Owano, T.; Castaneda, R.; Baer, D. S.; Paldus, B. A.; Gore, Warren J. (Technical Monitor)

2002-01-01

Large uncertainties in the effects that aerosols have on climate require improved in-situ measurements of extinction coefficient and single-scattering albedo. This abstract describes the use of continuous wave cavity ring-down (CW-CRD) technology to address this problem. The innovations in this instrument are the use of CW-CRD to measure aerosol extinction coefficient, the simultaneous measurement of scattering coefficient, and small size suitable for a wide range of aircraft applications. Our prototype instrument measures extinction and scattering coefficient at 690 nm and extinction coefficient at 1550 nm. The instrument itself is small (60 x 48 x 15 cm) and relatively insensitive to vibrations. The prototype instrument has been tested in our lab and used in the field. While improvements in performance are needed, the prototype has been shown to make accurate and sensitive measurements of extinction and scattering coefficients. Combining these two parameters, one can obtain the single-scattering albedo and absorption coefficient, both important aerosol properties. The use of two wavelengths also allows us to obtain a quantitative idea of the size of the aerosol through the Angstrom exponent. Minimum sensitivity of the prototype instrument is 1.5 x 10(exp -6)/m (1.5/Mm). Validation of the measurement of extinction coefficient has been accomplished by comparing the measurement of calibration spheres with Mie calculations. This instrument and its successors have potential to help reduce uncertainty currently associated with aerosol optical properties and their spatial and temporal variation. Possible applications include studies of visibility, climate forcing by aerosol, and the validation of aerosol retrieval schemes from satellite data.

Derivation of Physical and Optical Properties of Midlatitude Cirrus Ice Crystals for a Size-Resolved Cloud Microphysics Model

NASA Technical Reports Server (NTRS)

Fridlind, Ann M.; Atlas, Rachel; Van Diedenhoven, Bastiaan; Um, Junshik; McFarquhar, Greg M.; Ackerman, Andrew S.; Moyer, Elisabeth J.; Lawson, R. Paul

2016-01-01

Single-crystal images collected in mid-latitude cirrus are analyzed to provide internally consistent ice physical and optical properties for a size-resolved cloud microphysics model, including single-particle mass, projected area, fall speed, capacitance, single-scattering albedo, and asymmetry parameter. Using measurements gathered during two flights through a widespread synoptic cirrus shield, bullet rosettes are found to be the dominant identifiable habit among ice crystals with maximum dimension (Dmax) greater than 100µm. Properties are therefore first derived for bullet rosettes based on measurements of arm lengths and widths, then for aggregates of bullet rosettes and for unclassified (irregular) crystals. Derived bullet rosette masses are substantially greater than reported in existing literature, whereas measured projected areas are similar or lesser, resulting in factors of 1.5-2 greater fall speeds, and, in the limit of large Dmax, near-infrared single-scattering albedo and asymmetry parameter (g) greater by approx. 0.2 and 0.05, respectively. A model that includes commonly imaged side plane growth on bullet rosettes exhibits relatively little difference in microphysical and optical properties aside from approx. 0:05 increase in mid-visible g primarily attributable to plate aspect ratio. In parcel simulations, ice size distribution, and g are sensitive to assumed ice properties.

Scattering property based contextual PolSAR speckle filter

NASA Astrophysics Data System (ADS)

Mullissa, Adugna G.; Tolpekin, Valentyn; Stein, Alfred

2017-12-01

Reliability of the scattering model based polarimetric SAR (PolSAR) speckle filter depends upon the accurate decomposition and classification of the scattering mechanisms. This paper presents an improved scattering property based contextual speckle filter based upon an iterative classification of the scattering mechanisms. It applies a Cloude-Pottier eigenvalue-eigenvector decomposition and a fuzzy H/α classification to determine the scattering mechanisms on a pre-estimate of the coherency matrix. The H/α classification identifies pixels with homogeneous scattering properties. A coarse pixel selection rule groups pixels that are either single bounce, double bounce or volume scatterers. A fine pixel selection rule is applied to pixels within each canonical scattering mechanism. We filter the PolSAR data and depending on the type of image scene (urban or rural) use either the coarse or fine pixel selection rule. Iterative refinement of the Wishart H/α classification reduces the speckle in the PolSAR data. Effectiveness of this new filter is demonstrated by using both simulated and real PolSAR data. It is compared with the refined Lee filter, the scattering model based filter and the non-local means filter. The study concludes that the proposed filter compares favorably with other polarimetric speckle filters in preserving polarimetric information, point scatterers and subtle features in PolSAR data.

Light Scattering by Ice Crystals Containing Air Bubbles

NASA Astrophysics Data System (ADS)

Zhang, J.; Panetta, R. L.; Yang, P.; Bi, L.

2014-12-01

The radiative effects of ice clouds are often difficult to estimate accurately, but are very important for interpretation of observations and for climate modeling. Our understanding of these effects is primarily based on scattering calculations, but due to the variability in ice habit it is computationally difficult to determine the required scattering and absorption properties, and the difficulties are only compounded by the need to include consideration of air and carbon inclusions of the sort frequently observed in collected samples. Much of the previous work on effects of inclusions in ice particles on scattering properties has been conducted with variants of geometric optics methods. We report on simulations of scattering by ice crystals with enclosed air bubbles using the pseudo-spectral time domain method (PSTD) and improved geometric optics method (IGOM). A Bouncing Ball Model (BBM) is proposed as a parametrization of air bubbles, and the results are compared with Monte Carlo radiative transfer calculations. Consistent with earlier studies, we find that air inclusions lead to a smoothing of variations in the phase function, weakening of halos, and a reduction of backscattering. We extend these studies by examining the effects of the particular arrangement of a fixed number of bubbles, as well as the effects of splitting a given number of bubbles into a greater number of smaller bubbles with the same total volume fraction. The result shows that the phase function will not change much for stochastic distributed air bubbles. It also shows that local maxima of phase functions are smoothed out for backward directions, when we break bubbles into small ones, single big bubble scatter favors more forward scattering than multi small internal scatters.

Optical diagnostics based on elastic scattering: An update of clinical demonstrations with the Optical Biopsy System

DOE Office of Scientific and Technical Information (OSTI.GOV)

Bigio, I.J.; Boyer, J.; Johnson, T.M.

1994-10-01

The Los Alamos National Laboratory has continued the development of the Optical Biopsy System (OBS) for noninvasive, real-time in situ diagnosis of tissue pathologies. Our clinical studies have expanded since the last Biomedical Optics Europe conference (Budapest, September 1993), and we report here on the latest results of clinical tests in gastrointestinal tract. The OBS invokes a unique approach to optical diagnosis of tissue pathologies based on the elastic scattering properties, over a wide range of wavelengths, of the tissue. The use of elastic scattering as the key to optical tissue diagnostics in the OBS is based on the factmore » that many tissue pathologies, including a majority of cancer forms, manifest significant architectural changes at the cellular and sub-cellular level. Since the cellular components that cause elastic scattering have dimensions typically on the order of visible to near-IR wavelengths, the elastic (Mie) scattering properties will be wavelength dependent. Thus, morphology and size changes can be expected to cause significant changes in an optical signature that is derived from the wavelength-dependence of elastic scattering. The OBS employs a small fiberoptic probe that is amenable to use with any endoscope or catheter, or to direct surface examination. The probe is designed to be used in optical contact with the tissue under examination and has separate illuminating and collecting fibers. Thus, the light that is collected and transmitted to the analyzing spectrometer must first scatter through a small volume of the tissue before entering the collection fiber(s). Consequently, the system is also sensitive to the optical absorption spectrum of the tissue, over an effective operating range of <300 to 950 nm, and such absorption adds valuable complexity to the scattering spectral signature.« less

Controlling the scattering properties of thin, particle-doped coatings

NASA Astrophysics Data System (ADS)

Rogers, William; Corbett, Madeleine; Manoharan, Vinothan

2013-03-01

Coatings and thin films of small particles suspended in a matrix possess optical properties that are important in several industries from cosmetics and paints to polymer composites. Many of the most interesting applications require coatings that produce several bulk effects simultaneously, but it is often difficult to rationally formulate materials with these desired optical properties. Here, we focus on the specific challenge of designing a thin colloidal film that maximizes both diffuse and total hemispherical transmission. We demonstrate that these bulk optical properties follow a simple scaling with two microscopic length scales: the scattering and transport mean free paths. Using these length scales and Mie scattering calculations, we generate basic design rules that relate scattering at the single particle level to the film's bulk optical properties. These ideas will be useful in the rational design of future optically active coatings.

Measurement and Modeling of the Optical Scattering Properties of Crop Canopies

NASA Technical Reports Server (NTRS)

Vanderbilt, V. C.; Grant, L.

1984-01-01

Efforts in measuring, analyzing, and mathematically modeling the specular, polarized, and diffuse light scattering properties of several plant canopies and their component parts (leaves, stems, fruit, soil) as a function of view angle and illumination angle are reported. Specific objectives were: (1) to demonstrate a technique for determining the specular and diffuse components of the reflectance factor of plant canopies; (2) to acquire the measurements and begin assembling a data set for developing and testing canopy reflectance models; (3) to design and build a new optical instrument to measure the light scattering properties of individual leaves; and (4) to use this instrument to survey and investigate the information in the light scattering properties of individual leaves of crops, forests, weeds, and horticulture.

Retrieval of haze properties and HCN concentrations from the three-micron spectrum of Titan

NASA Astrophysics Data System (ADS)

Kim, Sang J.; Lee, D. W.; Sim, C. K.; Seon, K. I.; Courtin, R.; Geballe, T. R.

2018-05-01

The 3 μm spectrum of Titan contains line emission and absorption as well as a significant haze continuum. The line emission has been previously analyzed in the literature, but that analysis has not properly included the influence of haze on the line emission. We report a new analysis of the 3 μm HCN emission spectrum using radiative transfer equations that include scattering and absorption by molecules and haze particles at altitudes lower than 500 km, where the influence of haze on the emergent spectrum becomes significant. Taking advantage of the dominance of resonant single scattering in the HCN ν3 fundamental and of the moderate haze optical thickness of the atmosphere around 3 μm, we adopt single dust and molecular scattering and present a formulation for the radiative transfer process. We evaluate the quantitative influence of haze scattering on the emission line intensities, and derive vertically-resolved single scattering albedos of the haze from model fits. We also present the resulting concentrations of HCN for altitudes below 500 km, where we find that the haze scattering significantly influences the retrieval of the concentrations of HCN. We conclude that the formulation we present is useful for the analysis of the HCN line emission from Titan and other similar hazy planetary or celestial objects.

Extended ecosystem signatures with application to Eos synergism requirements

NASA Technical Reports Server (NTRS)

Ulaby, Fawwaz T.; Dobson, M. Craig; Sarabandi, Kamal

1993-01-01

The primary objective is to define the advantages of synergistically combining optical and microwave remote sensing measurements for the determination of biophysical properties important in ecosystem modeling. This objective was approached in a stepwise fashion starting with ground-based observations of controlled agricultural and orchard canopies and progressing to airborne observations of more natural forest ecosystems. This observational program is complemented by a parallel effort to model the visible reflectance and microwave scattering properties of composite vegetation canopies. The goals of the modeling studies are to verify our basic understanding of the sensor-scene interaction physics and to provide the basis for development of inverse models optimized for retrieval of key biophysical properties. These retrieval algorithms can then be used to simulate the expected performance of various aspects of Eos including the need for simultaneous SAR and HIRIS observations or justification for other (non-synchronous) relative timing constraints and the frequency, polarization, and angle of incidence requirements for accurate biophysical parameter extractions. This program completed a very successful series of truck-mounted experiments, made remarkable progress in development and validation of optical reflectance and microwave scattering models for vegetation, extended the scattering models to accommodate discontinuous and periodic canopies, developed inversion approaches for surface and canopy properties, and disseminated these results widely through symposia and journal publications. In addition, the third generation of the computer code for the microwave scattering models was provided to a number of other US, Canadian, Australian, and European investigators who are currently presenting and publishing results using the MIMICS research code.

Differentiation of oral precancerous stages with optical coherence tomography based on the evaluation of optical scattering properties of oral mucosae

NASA Astrophysics Data System (ADS)

Tsai, M. T.; Lee, J. D.; Lee, Y. J.; Lee, C. K.; Jin, H. L.; Chang, F. Y.; Hu, K. Y.; Wu, C. P.; Chiang, C. P.; Yang, C. C.

2013-04-01

Optical coherence tomography (OCT) has been demonstrated to be a powerful tool for noninvasive, real-time oral cancer diagnosis. However, in previous reports, OCT has still been found to be difficult to use in the diagnosis of oral precancerous stages, including mild dysplasia and moderate dysplasia. In clinical applications, early diagnosis and treatment of oral cancer can greatly improve the survival rate. Therefore, in this study, we propose a new approach to differentiate the oral precancerous stages based on the evaluation of the optical scattering properties of the epithelial layer, which is where the dysplastic cells start to develop in the precancerous stages. Instead of using exponential decay fitting to evaluate the scattering properties of mucosal tissues based on the Beer-Lambert law, linear fitting of the OCT depth intensity is used to evaluate the scattering properties of normal and dysplastic cells. From the statistical results of the linear fitting, the slope, a, can be an effective indicator to discriminate healthy mucosa and moderate dysplasia when an a value equal to zero is the threshold value, and the intercept, b, can be used to differentiate healthy and dysplastic mucosae, as well as mild and moderate dysplasia, when b values of 0.15 and 0.18 are used as the threshold values, respectively. Furthermore, this approach is also applied to the determination of the safe margin between normal and abnormal mucosae, making it possible to provide real-time, in vivo inspection during oral maxillofacial surgery.

Apparatus for measuring particle properties

DOEpatents

Rader, D.J.; Castaneda, J.N.; Grasser, T.W.; Brockmann, J.E.

1998-08-11

An apparatus is described for determining particle properties from detected light scattered by the particles. The apparatus uses a light beam with novel intensity characteristics to discriminate between particles that pass through the beam and those that pass through an edge of the beam. The apparatus can also discriminate between light scattered by one particle and light scattered by multiple particles. The particle`s size can be determined from the intensity of the light scattered. The particle`s velocity can be determined from the elapsed time between various intensities of the light scattered. 11 figs.

Scattering Properties of Ground-State 23Na Vapor Using Generalized Scattering Theory

NASA Astrophysics Data System (ADS)

Al-Harazneh, A. A.; Sandouqa, A. S.; Joudeh, B. R.; Ghassib, H. B.

2018-04-01

The scattering properties of ground-state 23Na vapor are investigated within the framework of the Galitskii-Migdal-Feynman formalism. Viewed as a generalized scattering theory, this formalism is used to calculate the medium phase shifts. The scattering properties of the system—the total, viscosity, spin-exchange, and average cross sections—are then computed using these phase shifts according to standard recipes. The total cross section is found to exhibit the Ramsauer-Townsend effect as well as resonance peaks. These peaks are caused by the large difference between the potentials for electronic spin-singlet and spin-triplet states. They represent quasi-bound states in the system. The results obtained for the complex spin-exchange cross sections are particularly highlighted because of their importance in the spectroscopy of the Na2 dimer. So are the results for the scattering lengths pertaining to both singlet and triplet states. Wherever possible, comparison is made with other published results.

Physical-geometric optics method for large size faceted particles.

PubMed

Sun, Bingqiang; Yang, Ping; Kattawar, George W; Zhang, Xiaodong

2017-10-02

A new physical-geometric optics method is developed to compute the single-scattering properties of faceted particles. It incorporates a general absorption vector to accurately account for inhomogeneous wave effects, and subsequently yields the relevant analytical formulas effective and computationally efficient for absorptive scattering particles. A bundle of rays incident on a certain facet can be traced as a single beam. For a beam incident on multiple facets, a systematic beam-splitting technique based on computer graphics is used to split the original beam into several sub-beams so that each sub-beam is incident only on an individual facet. The new beam-splitting technique significantly reduces the computational burden. The present physical-geometric optics method can be generalized to arbitrary faceted particles with either convex or concave shapes and with a homogeneous or an inhomogeneous (e.g., a particle with a core) composition. The single-scattering properties of irregular convex homogeneous and inhomogeneous hexahedra are simulated and compared to their counterparts from two other methods including a numerically rigorous method.

The observed properties of Fast Radio Bursts

NASA Astrophysics Data System (ADS)

Ravi, Vikram

2018-06-01

I present an empirical study of the properties of fast radio bursts (FRBs): Gigahertz-frequency, dispersed pulses of extragalactic origin. I focus my investigation on a sample of seventeen FRBs detected at the Parkes radio telescope with largely self-consistent instrumentation. Of this sample, six are temporally unresolved, eight exhibit evidence for scattering in inhomogeneous plasma, and five display potentially intrinsic temporal structure. The characteristic scattering timescales at a frequency of 1 GHz range between 0.005 ms and 32 ms; moderate evidence exists for a relation between FRB scattering timescales and dispersion measures. Additionally, I present constraints on the fluences of Parkes FRBs, accounting for their uncertain sky-positions, and use the multiple-beam detection of FRB 010724 (the Lorimer burst) to measure its fluence to be 800 ± 400 Jy ms. FRBs, including the repeating FRB 121102, appear to manifest with a plethora of characteristics, and it is uncertain at present whether they share a common class of progenitor object, or arise from a selection of independent progenitors.

The artefacts of radiochromic film dosimetry with flatbed scanners and their causation by light scattering from radiation-induced polymers.

PubMed

Schoenfeld, Andreas A; Poppinga, Daniela; Harder, Dietrich; Doerner, Karl-Joachim; Poppe, Bjoern

2014-07-07

Optical experiments and theoretical considerations have been undertaken in order to understand the causes of the 'orientation effect' and the 'parabola effect', the artefacts impairing the desired light absorption measurement on radiochromic EBT3 films with flatbed scanners. EBT3 films exposed to doses up to 20.9 Gy were scanned with an Epson Expression 10000XL flatbed scanner in landscape and portrait orientation. The horizontally and vertically polarized light components of the scanner were determined, and another Epson Expression 10000XL flatbed scanner was disassembled to examine its optical components. The optical properties of exposed and unexposed EBT3 films were studied with incident polarized and unpolarized white light, and the transmitted red light was investigated for its polarization and scattering properties including the distribution of the scattering angles. Neutral density filters were studied for comparison. Guidance was sought from the theory of light scattering from rod-like macromolecular structures. The drastic dose-dependent variation of the transmitted total light current as function of the orientation of front and rear polarizers, interpreted by light scattering theory, shows that the radiation-induced polymerization of the monomers of EBT3 films produces light scattering oscillators preferably polarized at right angles with the coating direction of the film. The directional distribution of the scattered light is partly anisotropic, with a preferred scattering plane at right angles with the coating direction, indicating light scattering from stacks of coherently vibrating oscillators piled up along the monomer crystals. The polyester carrier film also participates in these effects. The 'orientation' and 'parabola' artefacts due to flatbed scanning of radiochromic films can be explained by the interaction of the polarization-dependent and anisotropic light scattering from exposed and unexposed EBT3 films with the quantitative difference between the scanner's horizontally and vertically polarized light supply and with the limited directional acceptance of the scanner's light recording system.

Study of the mesosphere using wide-field twilight polarization measurements: Early results beyond the polar circle

NASA Astrophysics Data System (ADS)

Ugolnikov, O. S.; Kozelov, B. V.

2016-07-01

This paper discusses the results of early measurements of temperature and dust in the mesosphere on the basis of wide-field twilight sky polarimetry, which began in 2015 in Apatity (North of Russia, 67.6° N, 33.4° E) using the original entire-sky camera. These measurements have been performed for the first time beyond the Polar Circle in the winter and early spring period. The general polarization properties of the twilight sky and the procedure for identifying single scattering are described. The key results of the study include the Boltzmann temperature values at altitudes higher than 70 km and the conclusion on a weak effect of dust on scattering properties of the mesosphere during this period.

Surface-enhanced Raman scattering from silver nanostructures with different morphologies

NASA Astrophysics Data System (ADS)

Zhang, W. C.; Wu, X. L.; Kan, C. X.; Pan, F. M.; Chen, H. T.; Zhu, J.; Chu, Paul K.

2010-07-01

Scanning electron microscopy and X-ray diffraction reveal that four different types of crystalline silver nanostructures including nanoparticles, nanowires, nanocubes, and bipyramids are synthesized by a solvothermal method by reducing silver nitrate with ethylene glycol using poly(vinylpyrrolidone) as an adsorption agent and adding different quantities of sodium chloride to the solution. These nanostructures which exhibit different surface plasma resonance properties in the ultraviolet-visible region are shown to be good surface-enhanced Raman scattering (SERS) substrates using rhodamine 6G molecules. Our results demonstrate that the silver nanocubes, bipyramids with sharp corners and edges, and aggregated silver nanoparticles possess better SERS properties than the silver nanowires, indicating that they can serve as high-sensitivity substrates in SERS-based measurements.

Synthesis of gold nanoflowers using deep eutectic solvent with high surface enhanced Raman scattering properties

NASA Astrophysics Data System (ADS)

Aghakhani Mahyari, Farzaneh; Tohidi, Maryam; Safavi, Afsaneh

2016-09-01

A facile, seed-less and one-pot method was developed for synthesis of gold nanoflowers with multiple tips through reduction of HAuCl4 with deep eutectic solvent at room temperature. This solvent is eco-friendly, low-cost, non-toxic and biodegradable and can act as both reducing and shape-controlling agent. In this protocol, highly branched and stable gold nanoflowers were obtained without using any capping agent. The obtained products were characterized by different techniques including, field emission scanning electron microscopy, transmission electron microscopy, x-ray diffraction and UV-vis spectroscopy. The as-prepared gold nanoflowers exhibit efficient surface-enhanced Raman scattering (SERS) properties which can be used as excellent substrates for SERS.

Atmospheric Multiple Scattering Effects on GLAS Altimetry. Part 2; Analysis of Expected Errors in Antarctic Altitude Measurements

NASA Technical Reports Server (NTRS)

Mahesh, Ashwin; Spinhirne, James D.; Duda, David P.; Eloranta, Edwin W.; Starr, David O'C (Technical Monitor)

2001-01-01

The altimetry bias in GLAS (Geoscience Laser Altimeter System) or other laser altimeters resulting from atmospheric multiple scattering is studied in relationship to current knowledge of cloud properties over the Antarctic Plateau. Estimates of seasonal and interannual changes in the bias are presented. Results show the bias in altitude from multiple scattering in clouds would be a significant error source without correction. The selective use of low optical depth clouds or cloudfree observations, as well as improved analysis of the return pulse such as by the Gaussian method used here, are necessary to minimize the surface altitude errors. The magnitude of the bias is affected by variations in cloud height, cloud effective particle size and optical depth. Interannual variations in these properties as well as in cloud cover fraction could lead to significant year-to-year variations in the altitude bias. Although cloud-free observations reduce biases in surface elevation measurements from space, over Antarctica these may often include near-surface blowing snow, also a source of scattering-induced delay. With careful selection and analysis of data, laser altimetry specifications can be met.

Effective and Accurate Morphology Models for Asian and Saharan Mineral Dust Scattering Properties

NASA Astrophysics Data System (ADS)

Stegmann, P.; Yang, P.

2017-12-01

It is well known that mineral dust particles from desert sources can have a significant influence on the planetary radiation balance. In order to determine the sign and magnitude of the dust radiative forcing effect, complex models have been and continue to be developed. Key factors which influence the single-scattering properties of mineral dust are dust source regions and thus mineralogical composition, and its mixture with water, sea salt, and products of human activity, such as soot. The ensemble of mineral dust scattering particles may then be modeled either as a simple placeholder shape, often ellipsoidal, through the utilization of an appropriate effective medium refractive index scheme. On the other hand, the scattering particles may be represented in a more rigorous manner, such as Voronoi-tessellated aggregates including fractal soot chains. The consequences and differences of either choice are investigated in the project at hand. It will be shown that the effective medium model indicates a drastic dependence of the mineral dust particle composition on the particle size. Thus the refractive index of a dust particle is in fact a function of its size, amongst other factors. Regional differences between African and Asian mineral dust are also of significance.

Detection of gastrointestinal cancer by elastic scattering and absorption spectroscopies with the Los Alamos Optical Biopsy System

DOE Office of Scientific and Technical Information (OSTI.GOV)

Mourant, J.R.; Boyer, J.; Johnson, T.M.

1995-03-01

The Los Alamos National Laboratory has continued the development of the Optical Biopsy System (OBS) for noninvasive, real-time in situ diagnosis of tissue pathologies. In proceedings of earlier SPIE conferences we reported on clinical measurements in the bladder, and we report here on recent results of clinical tests in the gastrointestinal tract. With the OBS, tissue pathologies are detected/diagnosed using spectral measurements of the elastic optical transport properties (scattering and absorption) of the tissue over a wide range of wavelengths. The use of elastic scattering as the key to optical tissue diagnostics in the OBS is based on the factmore » that many tissue pathologies, including a majority of cancer forms, exhibit significant architectural changes at the cellular and sub-cellular level. Since the cellular components that cause elastic scattering have dimensions typically on the order of visible to near-IR wavelengths, the elastic (Mie) scattering properties will be wavelength dependent. Thus, morphology and size changes can be expected to cause significant changes m an optical signature that is derived from the wavelength-dependence of elastic scattering. Additionally, the optical geometry of the OBS beneficially enhances its sensitivity for measuring absorption bands. The OBS employs a small fiber-optic probe that is amenable to use with any endoscope or catheter, or to direct surface examination, as well as interstitial needle insertion. Data acquistion/display time is <1 second.« less

Multi-Parameter Aerosol Scattering Sensor

NASA Technical Reports Server (NTRS)

Greenberg, Paul S.; Fischer, David G.

2011-01-01

This work relates to the development of sensors that measure specific aerosol properties. These properties are in the form of integrated moment distributions, i.e., total surface area, total mass, etc., or mathematical combinations of these moment distributions. Specifically, the innovation involves two fundamental features: a computational tool to design and optimize such sensors and the embodiment of these sensors in actual practice. The measurement of aerosol properties is a problem of general interest. Applications include, but are not limited to, environmental monitoring, assessment of human respiratory health, fire detection, emission characterization and control, and pollutant monitoring. The objectives for sensor development include increased accuracy and/or dynamic range, the inclusion in a single sensor of the ability to measure multiple aerosol properties, and developing an overall physical package that is rugged, compact, and low in power consumption, so as to enable deployment in harsh or confined field applications, and as distributed sensor networks. Existing instruments for this purpose include scattering photometers, direct-reading mass instruments, Beta absorption devices, differential mobility analyzers, and gravitational samplers. The family of sensors reported here is predicated on the interaction of light and matter; specifically, the scattering of light from distributions of aerosol particles. The particular arrangement of the sensor, e.g. the wavelength(s) of incident radiation, the number and location of optical detectors, etc., can be derived so as to optimize the sensor response to aerosol properties of practical interest. A key feature of the design is the potential embodiment as an extremely compact, integrated microsensor package. This is of fundamental importance, as it enables numerous previously inaccessible applications. The embodiment of these sensors is inherently low maintenance and high reliability by design. The novel and unique features include the underlying computational underpinning that allows the optimization for specific applications, and the physical embodiment that affords the construction of a compact, durable, and reliable integrated package. The advantage appears in the form of increased accuracy relative to existing instruments, and the applications enabled by the physical attributes of the resulting configuration

Grassmannians for scattering amplitudes in 4d $$\\mathcal{N}=4 $$ SYM and 3d ABJM

DOE PAGES

Elvang, Henriette; Huang, Yu-tin; Keeler, Cynthia; ...

2014-12-31

Scattering amplitudes in 4d N=4 super Yang-Mills theory (SYM) can be described by Grassmannian contour integrals whose form depends on whether the external data is encoded in momentum space, twistor space, or momentum twistor space. Here, after a pedagogical review, we present a new, streamlined proof of the equivalence of the three integral formulations. A similar strategy allows us to derive a new Grassmannian integral for 3d N = 6 ABJM theory amplitudes in momentum twistor space: it is a contour integral in an orthogonal Grassmannian with the novel property that the internal metric depends on the external data. Themore » result can be viewed as a central step towards developing an amplituhedron formulation for ABJM amplitudes. Various properties of Grassmannian integrals are examined, including boundary properties, pole structure, and a homological interpretation of the global residue theorems for N = 4 SYM.« less

System and technique for ultrasonic characterization of settling suspensions

DOEpatents

Greenwood, Margaret S [Richland, WA; Panetta, Paul D [Richland, WA; Bamberger, Judith A [Richland, WA; Pappas, Richard A [Richland, WA

2006-11-28

A system for determining properties of settling suspensions includes a settling container, a mixer, and devices for ultrasonic interrogation transverse to the settling direction. A computer system controls operation of the mixer and the interrogation devices and records the response to the interrogating as a function of settling time, which is then used to determine suspension properties. Attenuation versus settling time for dilute suspensions, such as dilute wood pulp suspension, exhibits a peak at different settling times for suspensions having different properties, and the location of this peak is used as one mechanism for characterizing suspensions. Alternatively or in addition, a plurality of ultrasound receivers are arranged at different angles to a common transmitter to receive scattering responses at a variety of angles during particle settling. Angular differences in scattering as a function of settling time are also used to characterize the suspension.

The application of contraction theory to an iterative formulation of electromagnetic scattering

NASA Technical Reports Server (NTRS)

Brand, J. C.; Kauffman, J. F.

1985-01-01

Contraction theory is applied to an iterative formulation of electromagnetic scattering from periodic structures and a computational method for insuring convergence is developed. A short history of spectral (or k-space) formulation is presented with an emphasis on application to periodic surfaces. To insure a convergent solution of the iterative equation, a process called the contraction corrector method is developed. Convergence properties of previously presented iterative solutions to one-dimensional problems are examined utilizing contraction theory and the general conditions for achieving a convergent solution are explored. The contraction corrector method is then applied to several scattering problems including an infinite grating of thin wires with the solution data compared to previous works.

Analysis of dependent scattering mechanism in hard-sphere Yukawa random media

NASA Astrophysics Data System (ADS)

Wang, B. X.; Zhao, C. Y.

2018-06-01

The structural correlations in the microscopic structures of random media can induce the dependent scattering mechanism and thus influence the optical scattering properties. Based on our recent theory on the dependent scattering mechanism in random media composed of discrete dipolar scatterers [B. X. Wang and C. Y. Zhao, Phys. Rev. A 97, 023836 (2018)], in this paper, we study the hard-sphere Yukawa random media, in order to further elucidate the role of structural correlations in the dependent scattering mechanism and hence optical scattering properties. Here, we consider charged colloidal suspensions, whose effective pair interaction between colloids is described by a screened Coulomb (Yukawa) potential. By means of adding salt ions, the pair interaction between the charged particles can be flexibly tailored and therefore the structural correlations are modified. It is shown that this strategy can affect the optical properties significantly. For colloidal TiO2 suspensions, the modification of electric and magnetic dipole excitations induced by the structural correlations can substantially influence the optical scattering properties, in addition to the far-field interference effect described by the structure factor. However, this modification is only slightly altered by different salt concentrations and is mainly because of the packing-density-dependent screening effect. On the other hand, for low refractive index colloidal polystyrene suspensions, the dependent scattering mechanism mainly involves the far-field interference effect, and the effective exciting field amplitude for the electric dipole almost remains unchanged under different structural correlations. The present study has profound implications for understanding the role of structural correlations in the dependent scattering mechanism.

Light transport in turbid media with non-scattering, low-scattering and high absorption heterogeneities based on hybrid simplified spherical harmonics with radiosity model

PubMed Central

Yang, Defu; Chen, Xueli; Peng, Zhen; Wang, Xiaorui; Ripoll, Jorge; Wang, Jing; Liang, Jimin

2013-01-01

Modeling light propagation in the whole body is essential and necessary for optical imaging. However, non-scattering, low-scattering and high absorption regions commonly exist in biological tissues, which lead to inaccuracy of the existing light transport models. In this paper, a novel hybrid light transport model that couples the simplified spherical harmonics approximation (SPN) with the radiosity theory (HSRM) was presented, to accurately describe light transport in turbid media with non-scattering, low-scattering and high absorption heterogeneities. In the model, the radiosity theory was used to characterize the light transport in non-scattering regions and the SPN was employed to handle the scattering problems, including subsets of low-scattering and high absorption. A Neumann source constructed by the light transport in the non-scattering region and formed at the interface between the non-scattering and scattering regions was superposed into the original light source, to couple the SPN with the radiosity theory. The accuracy and effectiveness of the HSRM was first verified with both regular and digital mouse model based simulations and a physical phantom based experiment. The feasibility and applicability of the HSRM was then investigated by a broad range of optical properties. Lastly, the influence of depth of the light source on the model was also discussed. Primary results showed that the proposed model provided high performance for light transport in turbid media with non-scattering, low-scattering and high absorption heterogeneities. PMID:24156077

Light transport in turbid media with non-scattering, low-scattering and high absorption heterogeneities based on hybrid simplified spherical harmonics with radiosity model.

PubMed

Yang, Defu; Chen, Xueli; Peng, Zhen; Wang, Xiaorui; Ripoll, Jorge; Wang, Jing; Liang, Jimin

2013-01-01

Modeling light propagation in the whole body is essential and necessary for optical imaging. However, non-scattering, low-scattering and high absorption regions commonly exist in biological tissues, which lead to inaccuracy of the existing light transport models. In this paper, a novel hybrid light transport model that couples the simplified spherical harmonics approximation (SPN) with the radiosity theory (HSRM) was presented, to accurately describe light transport in turbid media with non-scattering, low-scattering and high absorption heterogeneities. In the model, the radiosity theory was used to characterize the light transport in non-scattering regions and the SPN was employed to handle the scattering problems, including subsets of low-scattering and high absorption. A Neumann source constructed by the light transport in the non-scattering region and formed at the interface between the non-scattering and scattering regions was superposed into the original light source, to couple the SPN with the radiosity theory. The accuracy and effectiveness of the HSRM was first verified with both regular and digital mouse model based simulations and a physical phantom based experiment. The feasibility and applicability of the HSRM was then investigated by a broad range of optical properties. Lastly, the influence of depth of the light source on the model was also discussed. Primary results showed that the proposed model provided high performance for light transport in turbid media with non-scattering, low-scattering and high absorption heterogeneities.

Experimental Phase Functions of Millimeter-sized Cosmic Dust Grains

DOE Office of Scientific and Technical Information (OSTI.GOV)

Muñoz, O.; Moreno, F.; Guirado, D.

We present the experimental phase functions of three types of millimeter-sized dust grains consisting of enstatite, quartz, and volcanic material from Mount Etna, respectively. The three grains present similar sizes but different absorbing properties. The measurements are performed at 527 nm covering the scattering angle range from 3° to 170°. The measured phase functions show two well-defined regions: (i) soft forward peaks and (ii) a continuous increase with the scattering angle at side- and back-scattering regions. This behavior at side- and back-scattering regions is in agreement with the observed phase functions of the Fomalhaut and HR 4796A dust rings. Furthermore » computations and measurements (including polarization) for millimeter-sized grains are needed to draw some conclusions about the fluffy or compact structure of the dust grains.« less

On the convergence of an iterative formulation of the electromagnetic scattering from an infinite grating of thin wires

NASA Technical Reports Server (NTRS)

Brand, J. C.

1985-01-01

Contraction theory is applied to an iterative formulation of electromagnetic scattering from periodic structures and a computational method for insuring convergence is developed. A short history of spectral (or k-space) formulation is presented with an emphasis on application to periodic surfaces. The mathematical background for formulating an iterative equation is covered using straightforward single variable examples including an extension to vector spaces. To insure a convergent solution of the iterative equation, a process called the contraction corrector method is developed. Convergence properties of previously presented iterative solutions to one-dimensional problems are examined utilizing contraction theory and the general conditions for achieving a convergent solution are explored. The contraction corrector method is then applied to several scattering problems including an infinite grating of thin wires with the solution data compared to previous works.

Dynamic mineral clouds on HD 189733b. II. Monte Carlo radiative transfer for 3D cloudy exoplanet atmospheres: combining scattering and emission spectra

NASA Astrophysics Data System (ADS)

Lee, G. K. H.; Wood, K.; Dobbs-Dixon, I.; Rice, A.; Helling, Ch.

2017-05-01

Context. As the 3D spatial properties of exoplanet atmospheres are being observed in increasing detail by current and new generations of telescopes, the modelling of the 3D scattering effects of cloud forming atmospheres with inhomogeneous opacity structures becomes increasingly important to interpret observational data. Aims: We model the scattering and emission properties of a simulated cloud forming, inhomogeneous opacity, hot Jupiter atmosphere of HD 189733b. We compare our results to available Hubble Space Telescope (HST) and Spitzer data and quantify the effects of 3D multiple scattering on observable properties of the atmosphere. We discuss potential observational properties of HD 189733b for the upcoming Transiting Exoplanet Survey Satellite (TESS) and CHaracterising ExOPlanet Satellite (CHEOPS) missions. Methods: We developed a Monte Carlo radiative transfer code and applied it to post-process output of our 3D radiative-hydrodynamic, cloud formation simulation of HD 189733b. We employed three variance reduction techniques, I.e. next event estimation, survival biasing, and composite emission biasing, to improve signal to noise of the output. For cloud particle scattering events, we constructed a log-normal area distribution from the 3D cloud formation radiative-hydrodynamic results, which is stochastically sampled in order to model the Rayleigh and Mie scattering behaviour of a mixture of grain sizes. Results: Stellar photon packets incident on the eastern dayside hemisphere show predominantly Rayleigh, single-scattering behaviour, while multiple scattering occurs on the western hemisphere. Combined scattered and thermal emitted light predictions are consistent with published HST and Spitzer secondary transit observations. Our model predictions are also consistent with geometric albedo constraints from optical wavelength ground-based polarimetry and HST B band measurements. We predict an apparent geometric albedo for HD 189733b of 0.205 and 0.229, in the TESS and CHEOPS photometric bands respectively. Conclusions: Modelling the 3D geometric scattering effects of clouds on observables of exoplanet atmospheres provides an important contribution to the attempt to determine the cloud properties of these objects. Comparisons between TESS and CHEOPS photometry may provide qualitative information on the cloud properties of nearby hot Jupiter exoplanets.

Investigation of ice particle habits to be used for ice cloud remote sensing for the GCOM-C satellite mission

NASA Astrophysics Data System (ADS)

Letu, Husi; Ishimoto, Hiroshi; Riedi, Jerome; Nakajima, Takashi Y.; -Labonnote, Laurent C.; Baran, Anthony J.; Nagao, Takashi M.; Sekiguchi, Miho

2016-09-01

In this study, various ice particle habits are investigated in conjunction with inferring the optical properties of ice clouds for use in the Global Change Observation Mission-Climate (GCOM-C) satellite programme. We develop a database of the single-scattering properties of five ice habit models: plates, columns, droxtals, bullet rosettes, and Voronoi. The database is based on the specification of the Second Generation Global Imager (SGLI) sensor on board the GCOM-C satellite, which is scheduled to be launched in 2017 by the Japan Aerospace Exploration Agency. A combination of the finite-difference time-domain method, the geometric optics integral equation technique, and the geometric optics method is applied to compute the single-scattering properties of the selected ice particle habits at 36 wavelengths, from the visible to the infrared spectral regions. This covers the SGLI channels for the size parameter, which is defined as a single-particle radius of an equivalent volume sphere, ranging between 6 and 9000 µm. The database includes the extinction efficiency, absorption efficiency, average geometrical cross section, single-scattering albedo, asymmetry factor, size parameter of a volume-equivalent sphere, maximum distance from the centre of mass, particle volume, and six nonzero elements of the scattering phase matrix. The characteristics of calculated extinction efficiency, single-scattering albedo, and asymmetry factor of the five ice particle habits are compared. Furthermore, size-integrated bulk scattering properties for the five ice particle habit models are calculated from the single-scattering database and microphysical data. Using the five ice particle habit models, the optical thickness and spherical albedo of ice clouds are retrieved from the Polarization and Directionality of the Earth's Reflectances-3 (POLDER-3) measurements, recorded on board the Polarization and Anisotropy of Reflectances for Atmospheric Sciences coupled with Observations from a Lidar (PARASOL) satellite. The optimal ice particle habit for retrieving the SGLI ice cloud properties is investigated by adopting the spherical albedo difference (SAD) method. It is found that the SAD is distributed stably due to the scattering angle increases for bullet rosettes with an effective diameter (Deff) of 10 µm and Voronoi particles with Deff values of 10, 60, and 100 µm. It is confirmed that the SAD of small bullet-rosette particles and all sizes of Voronoi particles has a low angular dependence, indicating that a combination of the bullet-rosette and Voronoi models is sufficient for retrieval of the ice cloud's spherical albedo and optical thickness as effective habit models for the SGLI sensor. Finally, SAD analysis based on the Voronoi habit model with moderate particle size (Deff = 60 µm) is compared with the conventional general habit mixture model, inhomogeneous hexagonal monocrystal model, five-plate aggregate model, and ensemble ice particle model. The Voronoi habit model is found to have an effect similar to that found in some conventional models for the retrieval of ice cloud properties from space-borne radiometric observations.

Theory of lasing in a multiple-scattering medium

NASA Astrophysics Data System (ADS)

John, Sajeev; Pang, Gendi

1996-10-01

In several recent experiments, isotropic lasing action was observed in paints that contain rhodamine 640 dye molecules in methanol solution as gain media and titania particles as optical scatterers. These so-called paint-on laser systems are extraordinary because they are highly disordered systems. The microscopic mechanism for laser activity and the coherence properties of light emission in this multiple-light-scattering medium have not yet been elucidated. In this paper we derive the emission intensity properties of a model dye system with excited singlet and triplet electronic energy levels, which is immersed in a multiple-scattering medium with transport mean free path l*. Using physically reasonable estimates for the absorption and emission cross section for the singlet and triplet manifolds, and the singlet-triplet intersystem crossing rate, we solve the nonlinear laser rate equations for the dye molecules. This leads to a diffusion equation for the light intensity in the medium with a nonlinear intensity-dependent gain coefficient. Using this model we are able to account for nearly all of the experimentally observed properties of laser paint reported so far when l*>>λ0, the emission wavelength. This includes the dependence of the peak intensity of amplified emission on the mean free path l*, the dye concentration ρ, and the pump intensity characteristics. Our model recaptures the collapse of the emission linewidth at a specific threshold pump intensity and describes how this threshold intensity varies with l*. In addition, our model predicts a dramatic increase in the peak intensity and a further lowering of the lasing threshold for the strong scattering limit l*-->λ0. This suggests a striking enhancement of the characteristics of laser paint near the photon localization threshold in a disordered medium.

Analysis on the electromagnetic scattering properties of crops at multi-band

NASA Astrophysics Data System (ADS)

Wu, Tao; Wu, Zhensen; Liu, Xiaoyi

2014-12-01

The vector radiative transfer (VRT) theory for active microwave remote sensing and Rayleigh-Gans approximation (GRG) are applied in the study, and an iterative algorithm is used to solve the RT equations, thus we obtain the zeroorder and first-order equation for numerical results. The Michigan Microwave Canopy Scattering (MIMICS) model is simplified to adapt to the crop model, by analyzing body-surface bistatic scattering and backscattering properties between a layer of soybean or wheat consisting of stems and leaves and different underlying soil surface at multi-band (i.e. P, L, S, X, Ku-band), we obtain microwave scattering mechanisms of crop components and the effect of underlying ground on total crop scattering. Stem and leaf are regard as a needle and a circular disk, respectively. The final results are compared with some literature data to verify our calculating method, numerical results show multi-band crop microwave scattering properties differ from scattering angle, azimuth angle and moisture of vegetation and soil, which offer the part needed information for the design of future bistatic radar systems for crop sensing applications.

Retrieval of Macro- and Micro-Physical Properties of Oceanic Hydrosols from Polarimetric Observations

NASA Technical Reports Server (NTRS)

Ibrahim, Amir; Gilerson, Alexander; Chowdhary, Jacek; Ahmed, Samir

2016-01-01

Remote sensing has mainly relied on measurements of scalar radiance and its spectral and angular features to retrieve micro- and macro-physical properties of aerosols/hydrosols. However, it is recognized that measurements that include the polarimetric characteristics of light provide more intrinsic information about particulate scattering. To take advantage of this, we used vector radiative transfer (VRT) simulations and developed an analytical relationship to retrieve the macro and micro-physical properties of the oceanic hydrosols. Specifically, we investigated the relationship between the observed degree of linear polarization (DoLP) and the ratio of attenuation-to- absorption coefficients (c/a) in water, from which the scattering coefficient can be readily computed (b equals c minus a), after retrieving a. This relationship was parameterized for various scattering geometries, including sensor zenith/azimuth angles relative to the Sun's principal plane, and for varying Sun zenith angles. An inversion method was also developed for the retrieval of the microphysical properties of hydrosols, such as the bulk refractive index and the particle size distribution. The DoLP vs c/a relationship was tested and validated against in-situ measurements of underwater light polarization obtained by a custom-built polarimeter and measurements of the coefficients a and c, obtained using an in-water WET (Western Environmental Technologies) Labs ac-s (attenuation coefficients In-Situ Spectrophotometer) instrument package. These measurements confirmed the validity of the approach, with retrievals of attenuation coefficients showing a high coefficient of determination depending on the wavelength. We also performed a sensitivity analysis of the DoLP at the Top of Atmosphere (TOA) over coastal waters showing the possibility of polarimetric remote sensing application for ocean color.

First correlated measurements of the shape and light scattering properties of cloud particles using the new Particle Habit Imaging and Polar Scattering (PHIPS) probe

NASA Astrophysics Data System (ADS)

Abdelmonem, A.; Schnaiter, M.; Amsler, P.; Hesse, E.; Meyer, J.; Leisner, T.

2011-10-01

Studying the radiative impact of cirrus clouds requires knowledge of the relationship between their microphysics and the single scattering properties of cloud particles. Usually, this relationship is obtained by modeling the optical scattering properties from in situ measurements of ice crystal size distributions. The measured size distribution and the assumed particle shape might be erroneous in case of non-spherical ice particles. We present here a novel optical sensor (the Particle Habit Imaging and Polar Scattering probe, PHIPS) designed to measure simultaneously the 3-D morphology and the corresponding optical and microphysical parameters of individual cloud particles. Clouds containing particles ranging from a few micrometers to about 800 μm diameter in size can be characterized systematically with an optical resolution power of 2 μm and polar scattering resolution of 1° for forward scattering directions (from 1° to 10°) and 8° for side and backscattering directions (from 18° to 170°). The maximum acquisition rates for scattering phase functions and images are 262 KHz and 10 Hz, respectively. Some preliminary results collected in two ice cloud campaigns conducted in the AIDA cloud simulation chamber are presented. PHIPS showed reliability in operation and produced size distributions and images comparable to those given by other certified cloud particles instruments. A 3-D model of a hexagonal ice plate is constructed and the corresponding scattering phase function is compared to that modeled using the Ray Tracing with Diffraction on Facets (RTDF) program. PHIPS is a highly promising novel airborne optical sensor for studying the radiative impact of cirrus clouds and correlating the particle habit-scattering properties which will serve as a reference for other single, or multi-independent, measurement instruments.

Estimates of oceanic surface wind speed and direction using orthogonal beam scatterometer measurements and comparison of recent sea scattering theories

NASA Technical Reports Server (NTRS)

Moore, R. K.; Fung, A. K.; Dome, G. J.; Birrer, I. J.

1978-01-01

The wind direction properties of radar backscatter from the sea were empirically modelled using a cosine Fourier series through the 4th harmonic in wind direction (referenced to upwind). A comparison with 1975 JONSWAP (Joint North Sea Wave Project) scatterometer data, at incidence angles of 40 and 65, indicates that effects to third and fourth harmonics are negligible. Another important result is that the Fourier coefficients through the second harmonic are related to wind speed by a power law expression. A technique is also proposed to estimate the wind speed and direction over the ocean from two orthogonal scattering measurements. A comparison between two different types of sea scatter theories, one type presented by the work of Wright and the other by that of Chan and Fung, was made with recent scatterometer measurements. It demonstrates that a complete scattering model must include some provisions for the anisotropic characteristics of the sea scatter, and use a sea spectrum which depends upon wind speed.

A Small Angle Scattering Sensor System for the Characterization of Combustion Generated Particulate

NASA Technical Reports Server (NTRS)

Feikema, Douglas A.; Kim, W.; Sivathanu, Yudaya

2007-01-01

One of the critical issues for the US space program is fire safety of the space station and future launch vehicles. A detailed understanding of the scattering signatures of particulate is essential for the development of a false alarm free fire detection system. This paper describes advanced optical instrumentation developed and applied for fire detection. The system is being designed to determine four important physical properties of disperse fractal aggregates and particulates including size distribution, number density, refractive indices, and fractal dimension. Combustion generated particulate are the primary detection target; however, in order to discriminate from other particulate, non-combustion generated particles should also be characterized. The angular scattering signature is measured and analyzed using two photon optical laser scattering. The Rayleigh-Debye-Gans (R-D-G) scattering theory for disperse fractal aggregates is utilized. The system consists of a pulsed laser module, detection module and data acquisition system and software to analyze the signals. The theory and applications are described.

Linking Aerosol Optical Properties Between Laboratory, Field, and Model Studies

NASA Astrophysics Data System (ADS)

Murphy, S. M.; Pokhrel, R. P.; Foster, K. A.; Brown, H.; Liu, X.

2017-12-01

The optical properties of aerosol emissions from biomass burning have a significant impact on the Earth's radiative balance. Based on measurements made during the Fourth Fire Lab in Missoula Experiment, our group published a series of parameterizations that related optical properties (single scattering albedo and absorption due to brown carbon at multiple wavelengths) to the elemental to total carbon ratio of aerosols emitted from biomass burning. In this presentation, the ability of these parameterizations to simulate the optical properties of ambient aerosol is assessed using observations collected in 2017 from our mobile laboratory chasing wildfires in the Western United States. The ambient data includes measurements of multi-wavelength absorption, scattering, and extinction, size distribution, chemical composition, and volatility. In addition to testing the laboratory parameterizations, this combination of measurements allows us to assess the ability of core-shell Mie Theory to replicate observations and to assess the impact of brown carbon and mixing state on optical properties. Finally, both laboratory and ambient data are compared to the optical properties generated by a prominent climate model (Community Earth System Model (CESM) coupled with the Community Atmosphere Model (CAM 5)). The discrepancies between lab observations, ambient observations and model output will be discussed.

Extinction and Scattering Properties of Soot Emitted from Buoyant Turbulent Diffusion Flames. Appendix F

NASA Technical Reports Server (NTRS)

Krishnan, S. S.; Lin, K.-C.; Faeth, G. M.; Yuan, Z.-G. (Technical Monitor); Urban, D. L. (Technical Monitor); Yuan, Z.-G. (Technical Monitor)

2001-01-01

Extinction and scattering properties at wavelengths of 250-5200 nm were studied for soot emitted from buoyant turbulent diffusion flames in the long residence time regime where soot properties are independent of position in the overfire region and characteristic flame residence times. Flames burning in still air and fueled with gas (acetylene, ethylene, propane, and propylene) and liquid (benzene, toluene, cyclohexane, and n-heptane) hydrocarbon fuels were considered. Measured scattering patterns and ratios of total scattering/absorption cross sections were in good agreement with predictions based on the Rayleigh-Debye-Gans (RDG) scattering approximation in the visible. Measured depolarization ratios were roughly correlated by primary particle size parameter, suggesting potential for completing RDG methodology needed to make soot scattering predictions as well as providing a nonintrusive way to measure primary soot particle diameters. Measurements of dimensionless extinction coefficients were in good agreement with earlier measurements for similar soot populations and were independent of fuel type and wavelength except for reduced values as the near ultraviolet was approached. The ratios of the scattering/absorption refractive index functions were independent of fuel type within experimental uncertainties and were in good agreement with earlier measurements. The refractive index junction for absorption was similarly independent of fuel type but was larger than earlier reflectometry measurements in the infrared. Ratios of total scattering/absorption cross sections were relatively large in the visible and near infrared, with maximum values as large as 0.9 and with values as large as 0.2 at 2000 nm, suggesting greater potential for scattering from soot particles to affect flame radiation properties than previously thought.

Extinction and Scattering Properties of Soot Emitted from Buoyant Turbulent Diffusion Flames. Appendix D

NASA Technical Reports Server (NTRS)

Krishnan, S. S.; Lin, K.-C.; Faeth, G. M.; Urban, D. L. (Technical Monitor); Yuan, Z.-G. (Technical Monitor)

2001-01-01

Extinction and scattering properties at wavelengths of 250-5200 nm were studied for soot emitted from buoyant turbulent diffusion flames in the long residence time regime where soot properties are independent of position in the overfire region and characteristic flame residence times. Flames burning in still air and fueled with gas (acetylene, ethylene, propane, and propylene) and liquid (benzene, toluene, cyclohexane, and n-heptane) hydrocarbon fuels were considered Measured scattering patterns and ratios of total scattering/absorption cross sections were in good agreement with predictions based on the Rayleigh-Debye-Gans (RDG) scattering approximation in the visible. Measured depolarization ratios were roughly correlated by primary particle size parameter, suggesting potential for completing RDG methodology needed to make soot scattering predictions as well as providing a nonintrusive way to measure primary soot particle diameters. Measurements of dimensionless extinction coefficients were in good agreement with earlier measurements for similar soot populations and were independent of fuel type and wavelength except for reduced values as the near ultraviolet was approached. The ratios of the scattering/absorption refractive index functions were independent of fuel type within experimental uncertainties and were in good agreement with earlier measurements. The refractive index function for absorption was similarly independent of fuel type but was larger than earlier reflectometry measurements in the infrared. Ratios of total scattering/absorption cross sections were relatively large in the visible and near infrared, with maximum values as large as 0.9 and with values as large as 0.2 at 2000 nm, suggesting greater potential for scattering from soot particles to affect flame radiation properties than previously thought.

Solid State Division progress report for period ending September 30, 1984

DOE Office of Scientific and Technical Information (OSTI.GOV)

Green, P.H.; Watson, D.M.

1985-03-01

During the reporting period, relatively minor changes have occurred in the research areas of interest to the Division. Nearly all the research of the Division can be classified broadly as mission-oriented basic research. Topics covered include: theoretical solid state physics; surface and near-surface properties of solids; defects in solids; transport properties of solids; neutron scattering; and preparation and characterization of research materials. (GHT)

Derivation of physical and optical properties of mid-latitude cirrus ice crystals for a size-resolved cloud microphysics model

DOE PAGES

Fridlind, Ann M.; Atlas, Rachel; van Diedenhoven, Bastiaan; ...

2016-06-10

Single-crystal images collected in mid-latitude cirrus are analyzed to provide internally consistent ice physical and optical properties for a size-resolved cloud microphysics model, including single-particle mass, projected area, fall speed, capacitance, single-scattering albedo, and asymmetry parameter. Using measurements gathered during two flights through a widespread synoptic cirrus shield, bullet rosettes are found to be the dominant identifiable habit among ice crystals with maximum dimension ( D max) greater than 100 µm. Properties are therefore first derived for bullet rosettes based on measurements of arm lengths and widths, then for aggregates of bullet rosettes and for unclassified (irregular) crystals. Derived bulletmore » rosette masses are substantially greater than reported in existing literature, whereas measured projected areas are similar or lesser, resulting in factors of 1.5–2 greater fall speeds, and, in the limit of large D max, near-infrared single-scattering albedo and asymmetry parameter ( g) greater by ~0.2 and 0.05, respectively. Furthermore, a model that includes commonly imaged side plane growth on bullet rosettes exhibits relatively little difference in microphysical and optical properties aside from ~0.05 increase in mid-visible g primarily attributable to plate aspect ratio. In parcel simulations, ice size distribution, and g are sensitive to assumed ice properties.« less

Scattering and extinction properties of overfire soot in large buoyant turbulent diffusion flames

DOE Office of Scientific and Technical Information (OSTI.GOV)

Krishnan, S.S.; Lin, K.C.; Faeth, G.M.

1999-07-01

Measurements of the scattering and extinction properties of soot at visible wavelengths (351.2--632.8 nm) were completed for soot in the overfire region of large buoyant turbulent diffusion flames burning in still air where soot properties are independent of position and characteristic flame residence time for a particular fuel. Flames fueled with both gas (acetylene, ethylene, propylene and butadiene) and liquid (benzene, toluene, cyclohexane and n-heptane) hydrocarbon fuels were considered during the experiments. The measurements were considered during the experiments. The measurements were used to evaluate Rayleigh-Debye-Gans/polydisperse-fractal-aggregate theory for the absorption and scattering properties of soot, finding good performance for themore » present test range which included primary particle size parameters as large as 0.46; in addition, effects of fuel type over the test range were comparable to experimental uncertainties. Fractal dimensions were properly independent of wavelength and yielded a mean value of 1.79 with a standard deviation of 0.05, which is in excellent agreement with earlier work. Dimensionless extinction coefficients were relatively independent of wavelength and yielded a mean value of 8.4 with a standard deviation of 1.5. Present refractive indices did not exhibit a resonance condition, seen for graphite, as the uv was approached. Values of the refractive index function for absorption, E(m), increased as wavelength increased and were comparable to most earlier measurements for wavelengths greater than 400 nm. Values of the refractive index function for scattering, F(m), agreed with earlier measurements at wavelengths of 450--550 nm but otherwise increased with increasing wavelength more rapidly than seen before.« less

Nuclei and the Unitary Limit

NASA Astrophysics Data System (ADS)

Hammer, H.-W.

2018-07-01

Few-body systems with large scattering length display universal properties which are independent of the details of short-distance dynamics. These features include universal correlations between few-body observables and a geometric spectrum of three- and higher-body bound states. They can be observed in a wide range of systems from ultracold atoms to hadrons and nuclei. In this contribution, we review universality in nuclei dominated by few-body physics. In particular, we discuss halo nuclei and the description of light nuclei in a strict expansion around the unitary limit of infinite scattering length.

Simulating propagation of coherent light in random media using the Fredholm type integral equation

NASA Astrophysics Data System (ADS)

Kraszewski, Maciej; Pluciński, Jerzy

2017-06-01

Studying propagation of light in random scattering materials is important for both basic and applied research. Such studies often require usage of numerical method for simulating behavior of light beams in random media. However, if such simulations require consideration of coherence properties of light, they may become a complex numerical problems. There are well established methods for simulating multiple scattering of light (e.g. Radiative Transfer Theory and Monte Carlo methods) but they do not treat coherence properties of light directly. Some variations of these methods allows to predict behavior of coherent light but only for an averaged realization of the scattering medium. This limits their application in studying many physical phenomena connected to a specific distribution of scattering particles (e.g. laser speckle). In general, numerical simulation of coherent light propagation in a specific realization of random medium is a time- and memory-consuming problem. The goal of the presented research was to develop new efficient method for solving this problem. The method, presented in our earlier works, is based on solving the Fredholm type integral equation, which describes multiple light scattering process. This equation can be discretized and solved numerically using various algorithms e.g. by direct solving the corresponding linear equations system, as well as by using iterative or Monte Carlo solvers. Here we present recent development of this method including its comparison with well-known analytical results and a finite-difference type simulations. We also present extension of the method for problems of multiple scattering of a polarized light on large spherical particles that joins presented mathematical formalism with Mie theory.

Polarization of Light from Leaves Measured from 0.5 - 1.6 mm

NASA Technical Reports Server (NTRS)

Vanderbilt, V. C.; Ustin, S. L.; Daughtry, C. S. T.; Walthal, C. L.; Greenberg, J. A.

2006-01-01

The light scattered by plant canopies depends in part on the light scattering/absorbing properties of the leaves. Insights into these properties gained at the leaf scale are necessary ultimately to accomplish the region and global scale environmental goals of the EOS era. While this scattered light may be described by the four components of the Stokes vector, (intensity, magnitude of line= polarization, angle of plane of linear polarization, and magnitude of circular polarization), significant progress has been achieved toward understanding only the first component, the intensity of the scattered light. Recent research shows that the magnitude of the linearly polarized light may be a significant part of the light scattered by some canopies. Thus, consideration of the second component may be necessary to obtain an unambiguous understanding of the canopy processes. We measured the intensity and the linear polarization of the light scattered by single leaves, testing the hypothesis that the polarization of the light scattered by each leaf was attributable to properties of the surfaces of the leaf and specifically did not depend upon the properties of the interior of the leaf. This research extends previous investigations limited to the single leaves of approximately 20 species typically found in the area of Lafayette, Indiana, to the leaves of 30 species representing monocots, dicots and ferns from six continents.

North Atlantic Aerosol Single Scattering Albedos: TARFOX and ACE-2 Results and Their Relation to Radiative Effects Derived from Satellite Optical Depths

NASA Technical Reports Server (NTRS)

Russell, P. B.; Bergstrom, R. W.; Schmid, B.; Livingston, J. M.; Redemann, J.; Quinn, P. K.; Carrico, C. M.; Rood, M. J.

2000-01-01

Bergstrom and Russell estimated direct solar radiative flux changes caused by atmospheric aerosols over the mid-latitude North Atlantic Ocean under cloud-free and cloudy conditions. They excluded African dust aerosols, primarily by restricting calculations to latitudes 25-60 N. As inputs they used midvisible aerosol optical depth (AOD) maps derived from AVHRR satellite measurements and aerosol intensive properties determined primarily in the 1996 IGAC Troposheric Aerosol Radiative Forcing Observational Experiment (TARFOX). Those aerosol intensive properties, which included optical depth wavelength dependence and spectra of single scattering albedo (SSA) and scattering asymmetry parameter, were also checked against initial properties from the 1997 North Atlantic Aerosol Characterization Experiment (ACE 2). Bergstrom and Russell investigated the sensitivity of their derived flux changes to assumed input parameters, including midvisible AOD, SSA, and scattering asymmetry parameter. Although the sensitivity of net flux change at the tropopause to SSA was moderate over the ocean (e.g., a SSA uncertainty of 0.07 produced a flux-change uncertainty of 21%), the sensitivity over common land surfaces can be much larger. Also, flux changes within and below the aerosol layer, which affect atmospheric stability, heating rates, and cloud formation and persistence, are quite sensitive to aerosol SSA. Therefore, this paper focuses on the question: "What have we learned from TARFOX and ACE 2 regarding aerosol single scattering albedo?" Three techniques were used in TARFOX to determine midvisible SSA. One of these derived SSA as a best-fit parameter in comparing radiative flux changes measured by airborne pyranometer to those computed from aerosol properties. Another technique combined airborne measurements of aerosol scattering and absorption by nephelometer and absorption photometer. A third technique obtained SSA from best-fit complex refractive indices derived by comparing vertical profiles of lidar backscatter, sunphotometer extinction, and relative size distribution. In ACE 2 midvisible SSA was determined both as a best-fit parameter in comparing measured and calculated flux changes at the surface and by combining nephelometer and absorption photometer measurements. The nephelometer/absorption-photometer results were obtained on the ACE 2 ship (10 m asl), at the Sagres, Portugal site at 50 m asl, and also on the Pelican aircraft. This paper presents and compares the TARFOX and ACE 2 SSA results from the above techniques for different situations (e.g., marine vs continental flows, "clean" vs polluted conditions). It also discusses the strengths and limitations of the techniques, including whether they describe the aerosol in its ambient state or as perturbed by sampling processes; whether they describe the aerosol at the surface, as a function of altitude, or integrated over a column; the ease of acquiring representative data sets; results obtained in tests of consistency with radiative flux changes, and the likelihood of various artifacts and errors.

Visible and near-infrared bulk optical properties of raw milk.

PubMed

Aernouts, B; Van Beers, R; Watté, R; Huybrechts, T; Lammertyn, J; Saeys, W

2015-10-01

The implementation of optical sensor technology to monitor the milk quality on dairy farms and milk processing plants would support the early detection of altering production processes. Basic visible and near-infrared spectroscopy is already widely used to measure the composition of agricultural and food products. However, to obtain maximal performance, the design of such optical sensors should be optimized with regard to the optical properties of the samples to be measured. Therefore, the aim of this study was to determine the visible and near-infrared bulk absorption coefficient, bulk scattering coefficient, and scattering anisotropy spectra for a diverse set of raw milk samples originating from individual cow milkings, representing the milk variability present on dairy farms. Accordingly, this database of bulk optical properties can be used in future simulation studies to efficiently optimize and validate the design of an optical milk quality sensor. In a next step of the current study, the relation between the obtained bulk optical properties and milk quality properties was analyzed in detail. The bulk absorption coefficient spectra were found to mainly contain information on the water, fat, and casein content, whereas the bulk scattering coefficient spectra were found to be primarily influenced by the quantity and the size of the fat globules. Moreover, a strong positive correlation (r ≥ 0.975) was found between the fat content in raw milk and the measured bulk scattering coefficients in the 1,300 to 1,400 nm wavelength range. Relative to the bulk scattering coefficient, the variability on the scattering anisotropy factor was found to be limited. This is because the milk scattering anisotropy is nearly independent of the fat globule and casein micelle quantity, while it is mainly determined by the size of the fat globules. As this study shows high correlations between the sample's bulk optical properties and the milk composition and fat globule size, a sensor that allows for robust separation between the absorption and scattering properties would enable accurate prediction of the raw milk quality parameters. Copyright © 2015 American Dairy Science Association. Published by Elsevier Inc. All rights reserved.

Optical properties of cells with melanin

NASA Astrophysics Data System (ADS)

Rohde, Barukh; Coats, Israel; Krueger, James; Gareau, Dan

2014-02-01

The optical properties of pigmented lesions have been studied using diffuse reflectance spectroscopy in a noninvasive configuration on optically thick samples such as skin in vivo. However, it is difficult to un-mix the effects of absorption and scattering with diffuse reflectance spectroscopy techniques due to the complex anatomical distributions of absorbing and scattering biomolecules. We present a device and technique that enables absorption and scattering measurements of tissue volumes much smaller than the optical mean-free path. Because these measurements are taken on fresh-frozen sections, they are direct measurements of the optical properties of tissue, albeit in a different hydration state than in vivo tissue. Our results on lesions from 20 patients including melanomas and nevi show the absorption spectrum of melanin in melanocytes and basal keratinocytes. Our samples consisted of fresh frozen sections that were unstained. Fitting the spectrum as an exponential decay between 500 and 1100 nm [mua = A*exp(-B*(lambda-C)) + D], we report on the fit parameters of and their variation due to biological heterogeneity as A = 4.20e4 +/- 1.57e5 [1/cm], B = 4.57e-3 +/- 1.62e-3 [1/nm], C = 210 +/- 510 [nm] , D = 613 +/- 534 [1/cm]. The variability in these results is likely due to highly heterogeneous distributions of eumelanin and pheomelanin.

A scattering database of marine particles and its application in optical analysis

NASA Astrophysics Data System (ADS)

Xu, G.; Yang, P.; Kattawar, G.; Zhang, X.

2016-12-01

In modeling the scattering properties of marine particles (e.g. phytoplankton), the laboratory studies imply a need to properly account for the influence of particle morphology, in addition to size and composition. In this study, a marine particle scattering database is constructed using a collection of distorted hexahedral shapes. Specifically, the scattering properties of each size bin and refractive index are obtained by the ensemble average associated with distorted hexahedra with randomly tilted facets and selected aspect ratios (from elongated to flattened). The randomness degree in shape-generation process defines the geometric irregularity of the particles in the group. The geometric irregularity and particle aspect ratios constitute a set of "shape factors" to be accounted for (e.g. in best-fit analysis). To cover most of the marine particle size range, we combine the Invariant Imbedding T-matrix (II-TM) method and the Physical-Geometric Optics Hybrid (PGOH) method in the calculations. The simulated optical properties are shown and compared with those obtained from Lorenz-Mie Theory. Using the scattering database, we present a preliminary optical analysis of laboratory-measured optical properties of marine particles.

Aerosol optical properties at the Lulin Atmospheric Background Station in Taiwan and the influences of long-range transport of air pollutants

NASA Astrophysics Data System (ADS)

Hsiao, Ta-Chih; Chen, Wei-Nai; Ye, Wei-Cheng; Lin, Neng-Huei; Tsay, Si-Chee; Lin, Tang-Huang; Lee, Chung-Te; Chuang, Ming-Tung; Pantina, Peter; Wang, Sheng-Hsiang

2017-02-01

The Lulin Atmospheric Background Station (LABS, 23.47°N 120.87°E, 2862 m ASL) in Central Taiwan was constructed in 2006 and is the only high-altitude background station in the western Pacific region for studying the influence of continental outflow. In this study, extensive optical properties of aerosols, including the aerosol light scattering coefficient (σs) and light absorption coefficient (σa), were collected from 2013 to 2014. The intensive optical properties, including mass scattering efficiency (αs), mass absorption efficiency (αa), single scattering albedo (ω), scattering Ångstrӧm exponent (Å), and backscattering fraction (b), were determined and investigated, and the distinct seasonal cycle was observed. The value of αs began to increase in January and reached a maximum in April; the mean in spring was 5.89 m2 g-1 with a standard deviation (SD) of 4.54 m2 g-1 and a 4.48 m2 g-1 interquartile range (IQR: 2.95-7.43 m2 g-1). The trend was similar in αa, with a maximum in March and a monthly mean of 0.84 m2 g-1. The peak values of ω (Mean = 0.92, SD = 0.03, IQR: 0.90-0.93) and Å (Mean = 2.22, SD = 0.61, IQR: 2.12-2.47) occurred in autumn. These annual patterns of optical properties were associated with different long-range transport patterns of air pollutants such as biomass burning (BB) aerosol in spring and potential anthropogenic emissions in autumn. The optical measurements performed at LABS during spring in 2013 were compared with those simultaneously performed at the Doi Ang Kang Meteorology Station, Chiang Mai Province, Thailand (DAK, 19.93°N, 99.05°E, 1536 m a.s.l.), which is located in the Southeast Asia BB source region. Furthermore, the relationships among αs, αa, and b were used to characterize the potential aerosol types transported to LABS during different seasons, and the data were inspected according to the HYSPLIT 5-day backward trajectories, which differentiate between different regions of air mass origin.

A database of microwave and sub-millimetre ice particle single scattering properties

NASA Astrophysics Data System (ADS)

Ekelund, Robin; Eriksson, Patrick

2016-04-01

Ice crystal particles are today a large contributing factor as to why cold-type clouds such as cirrus remain a large uncertainty in global climate models and measurements. The reason for this is the complex and varied morphology in which ice particles appear, as compared to liquid droplets with an in general spheroidal shape, thus making the description of electromagnetic properties of ice particles more complicated. Single scattering properties of frozen hydrometers have traditionally been approximated by representing the particles as spheres using Mie theory. While such practices may work well in radio applications, where the size parameter of the particles is generally low, comparisons with measurements and simulations show that this assumption is insufficient when observing tropospheric cloud ice in the microwave or sub-millimetre regions. In order to assist the radiative transfer and remote sensing communities, a database of single scattering properties of semi-realistic particles is being produced. The data is being produced using DDA (Discrete Dipole Approximation) code which can treat arbitrarily shaped particles, and Tmatrix code for simpler shapes when found sufficiently accurate. The aim has been to mainly cover frequencies used by the upcoming ICI (Ice Cloud Imager) mission with launch in 2022. Examples of particles to be included are columns, plates, bullet rosettes, sector snowflakes and aggregates. The idea is to treat particles with good average optical properties with respect to the multitude of particles and aggregate types appearing in nature. The database will initially only cover macroscopically isotropic orientation, but will eventually also include horizontally aligned particles. Databases of DDA particles do already exist with varying accessibility. The goal of this database is to complement existing data. Regarding the distribution of the data, the plan is that the database shall be available in conjunction with the ARTS (Atmospheric Radiative Transfer Simulator) project.

Light Scattering by Fractal Dust Aggregates. I. Angular Dependence of Scattering

NASA Astrophysics Data System (ADS)

Tazaki, Ryo; Tanaka, Hidekazu; Okuzumi, Satoshi; Kataoka, Akimasa; Nomura, Hideko

2016-06-01

In protoplanetary disks, micron-sized dust grains coagulate to form highly porous dust aggregates. Because the optical properties of these aggregates are not completely understood, it is important to investigate how porous dust aggregates scatter light. In this study, the light scattering properties of porous dust aggregates were calculated using a rigorous method, the T-matrix method, and the results were then compared with those obtained using the Rayleigh-Gans-Debye (RGD) theory and Mie theory with the effective medium approximation (EMT). The RGD theory is applicable to moderately large aggregates made of nearly transparent monomers. This study considered two types of porous dust aggregates—ballistic cluster-cluster agglomerates (BCCAs) and ballistic particle-cluster agglomerates. First, the angular dependence of the scattered intensity was shown to reflect the hierarchical structure of dust aggregates; the large-scale structure of the aggregates is responsible for the intensity at small scattering angles, and their small-scale structure determines the intensity at large scattering angles. Second, it was determined that the EMT underestimates the backward scattering intensity by multiple orders of magnitude, especially in BCCAs, because the EMT averages the structure within the size of the aggregates. It was concluded that the RGD theory is a very useful method for calculating the optical properties of BCCAs.

LIGHT SCATTERING BY FRACTAL DUST AGGREGATES. I. ANGULAR DEPENDENCE OF SCATTERING

DOE Office of Scientific and Technical Information (OSTI.GOV)

Tazaki, Ryo; Tanaka, Hidekazu; Okuzumi, Satoshi

2016-06-01

In protoplanetary disks, micron-sized dust grains coagulate to form highly porous dust aggregates. Because the optical properties of these aggregates are not completely understood, it is important to investigate how porous dust aggregates scatter light. In this study, the light scattering properties of porous dust aggregates were calculated using a rigorous method, the T -matrix method, and the results were then compared with those obtained using the Rayleigh–Gans–Debye (RGD) theory and Mie theory with the effective medium approximation (EMT). The RGD theory is applicable to moderately large aggregates made of nearly transparent monomers. This study considered two types of porousmore » dust aggregates—ballistic cluster–cluster agglomerates (BCCAs) and ballistic particle–cluster agglomerates. First, the angular dependence of the scattered intensity was shown to reflect the hierarchical structure of dust aggregates; the large-scale structure of the aggregates is responsible for the intensity at small scattering angles, and their small-scale structure determines the intensity at large scattering angles. Second, it was determined that the EMT underestimates the backward scattering intensity by multiple orders of magnitude, especially in BCCAs, because the EMT averages the structure within the size of the aggregates. It was concluded that the RGD theory is a very useful method for calculating the optical properties of BCCAs.« less

Numerical simulation of raindrop scattering for C-band dual-polarization Doppler weather radar parameters

NASA Astrophysics Data System (ADS)

Teng, Shiwen; Hu, Hanfeng; Liu, Chao; Hu, Fangchao; Wang, Zhenhui; Yin, Yan

2018-07-01

The dual-polarization Doppler weather radar plays an important role in precipitation estimation and weather monitoring. For radar applications, the retrieval of precipitation microphysical characteristics is of great importance, and requires assumed scattering properties of raindrops. This study numerically investigates the scattering properties of raindrops and considers the capability of numerical models for raindrop scattering simulations. Besides the widely used spherical and oblate spheroid models, a non-spheroidal model based on realistic raindrop geometries with a flattened base and a smoothly rounded top is also considered. To study the effects of scattering simulations on radar applications, the polarization radar parameters are modeled based on the scattering properties calculated by different scattering models (i.e. the extended boundary condition T-matrix (EBCM) method and discretize dipole approximation (DDA)) and given size distributions, and compared with observations of a C-band dual-polarization radar. Note that, when the spatial resolution of the DDA simulation is large enough, the DDA results can be very close to those of the EBCM. Most simulated radar variables, except copolar correlation coefficient, match closely with radar observations, and the results based on different non-spheroidal models considered in this study show little differences. The comparison indicates that, even for the C-band radar, the effects of raindrop shape and canting angle on scattering properties are relatively minor due to relatively small size parameters. However, although more realistic particle geometry model may provide better representation on raindrop shape, considering the relatively time-consuming and complex scattering simulations for those particles, the oblate spheroid model with appropriate axis ratio variation is suggested for polarization radar applications.

Optical extinction dependence on wavelength and size distribution of airborne dust

NASA Astrophysics Data System (ADS)

Pangle, Garrett E.; Hook, D. A.; Long, Brandon J. N.; Philbrick, C. R.; Hallen, Hans D.

2013-05-01

The optical scattering from laser beams propagating through atmospheric aerosols has been shown to be very useful in describing air pollution aerosol properties. This research explores and extends that capability to particulate matter. The optical properties of Arizona Road Dust (ARD) samples are measured in a chamber that simulates the particle dispersal of dust aerosols in the atmospheric environment. Visible, near infrared, and long wave infrared lasers are used. Optical scattering measurements show the expected dependence of laser wavelength and particle size on the extinction of laser beams. The extinction at long wavelengths demonstrates reduced scattering, but chemical absorption of dust species must be considered. The extinction and depolarization of laser wavelengths interacting with several size cuts of ARD are examined. The measurements include studies of different size distributions, and their evolution over time is recorded by an Aerodynamic Particle Sizer. We analyze the size-dependent extinction and depolarization of ARD. We present a method of predicting extinction for an arbitrary ARD size distribution. These studies provide new insights for understanding the optical propagation of laser beams through airborne particulate matter.

Assessment of laser tracking and data transfer for underwater optical communications

NASA Astrophysics Data System (ADS)

Watson, Malcolm A.; Blanchard, Paul M.; Stace, Chris; Bhogul, Priya K.; White, Henry J.; Kelly, Anthony E.; Watson, Scott; Valyrakis, Manousos; Najda, Stephen P.; Marona, Lucja; Perlin, Piotr

2014-10-01

We report on an investigation into optical alignment and tracking for high bandwidth, laser-based underwater optical communication links. Link acquisition approaches (including scanning of narrow laser beams versus a wide-angle `beacon' approach) for different underwater laser-based communications scenarios are discussed. An underwater laserbased tracking system was tested in a large water flume facility using water whose scattering properties resembled that of a turbid coastal or harbour region. The lasers used were state-of-the-art, temperature-controlled, high modulation bandwidth gallium nitride (GaN) devices. These operate at blue wavelengths and can achieve powers up to ~100 mW. The tracking performance and characteristics of the system were studied as the light-scattering properties of the water were increased using commercial antacid (Maalox) solution, and the results are reported here. Optical tracking is expected to be possible even in high scattering water environments, assuming better components are developed commercially; in particular, more sensitive detector arrays. High speed data transmission using underwater optical links, based on blue light sources, is also reported.

Crucial Experiments in Quantum Physics.

ERIC Educational Resources Information Center

Trigg, George L.

The six experiments included in this monography are titled Blackbody Radiation, Collision of Electrons with Atoms, The Photoelectric Effect, Magnetic Properties of Atoms, The Scattering of X-Rays, and Diffraction of Electrons by a Crystal Lattice. The discussion provides historical background by giving description of the original experiments and…

Electronic Holography with a Broad Spectrum Laser for Time Gated Imaging Through Highly Scattering Media.

NASA Astrophysics Data System (ADS)

Shih, Marian Pei-Ling

The problem of optical imaging through a highly scattering volume diffuser, in particular, biological tissue, has received renewed interest in recent years because of a search for alternative imaging diagnostics in the optical wavelengths for the early detection of human breast cancer. This dissertation discusses the optical imaging of objects obscured by diffusers that contribute an otherwise overwhelming degree of multiple scatter. Many optical imaging techniques are based on the first-arriving light principle. These methods usually combine a transilluminating optical short pulse with a time windowing gate in order to form a flat shadowgraph image of absorbing objects either embedded within or hidden behind a scattering medium. The gate selectively records an image of the first-arriving light, while simultaneously rejecting the later-arriving scattered light. One set of the many implementations of the first -arriving light principle relies on the gating property of holography. This thesis presents several holographic optical gating experiments that demonstrate the role that the temporal coherence function of the illumination source plays in the imaging of all objects with short coherence length holography, with special emphasis on the application to image through diffusers and its resolution capabilities. Previous researchers have already successfully combined electronic holography, holography in which the recording medium is a two dimensional detector array instead of photographic film, with light-in-flight holography into a short coherence length holography method that images through various types of multiply scattering random media, including chicken breast tissue and wax. This thesis reports further experimental exploration of the short coherence holography method for imaging through severely scattering diffusers. There is a study on the effectiveness of spatial filtering of the first-arriving light, as well as a report of the imaging, by means of the short coherence holographic method, of an absorber through a living human hand. This thesis also includes both theoretical analyses and experimental results of a spectral dispersion holography system which, instead of optically synthesizing the broad spectrum illumination source that is used for the short coherence holography method, digitally synthesizes a broad spectrum hologram from a collection of single frequency component holograms. This system has the time gating properties of short coherence length holography, as well as experimentally demonstrated applications for imaging through multiply scattering media.

Derivation of Mars Surface Scattering Properties from OMEGA Spot Pointing Observations

NASA Astrophysics Data System (ADS)

Pinet, P. C.; Daydou, Y.; Cord, A.; Chevrel, S. C.; Poulet, F.; Erard, S.; Bibring, J.-P.; Langevin, Y.; Melchiorri, R.; Bellucci, G.; Altieri, F.; Arvidson, R. E.; OMEGA Co-Investigator Team

2005-03-01

OMEGA emission phase function (EPF) observation shows that one may access from orbit to geology-driven surface scattering properties such as surface roughness. It has implications for spectroscopic interpretation and for CRISM observations to come.

Geometrical-optics code for computing the optical properties of large dielectric spheres.

PubMed

Zhou, Xiaobing; Li, Shusun; Stamnes, Knut

2003-07-20

Absorption of electromagnetic radiation by absorptive dielectric spheres such as snow grains in the near-infrared part of the solar spectrum cannot be neglected when radiative properties of snow are computed. Thus a new, to our knowledge, geometrical-optics code is developed to compute scattering and absorption cross sections of large dielectric particles of arbitrary complex refractive index. The number of internal reflections and transmissions are truncated on the basis of the ratio of the irradiance incident at the nth interface to the irradiance incident at the first interface for a specific optical ray. Thus the truncation number is a function of the angle of incidence. Phase functions for both near- and far-field absorption and scattering of electromagnetic radiation are calculated directly at any desired scattering angle by using a hybrid algorithm based on the bisection and Newton-Raphson methods. With these methods a large sphere's absorption and scattering properties of light can be calculated for any wavelength from the ultraviolet to the microwave regions. Assuming that large snow meltclusters (1-cm order), observed ubiquitously in the snow cover during summer, can be characterized as spheres, one may compute absorption and scattering efficiencies and the scattering phase function on the basis of this geometrical-optics method. A geometrical-optics method for sphere (GOMsphere) code is developed and tested against Wiscombe's Mie scattering code (MIE0) and a Monte Carlo code for a range of size parameters. GOMsphere can be combined with MIE0 to calculate the single-scattering properties of dielectric spheres of any size.

Design of liquid crystals with 'de Vries-like' properties: structural variants of carbosilane-terminated 5-phenylpyrimidine mesogens.

PubMed

Schubert, Christopher P J; Müller, Carsten; Bogner, Andreas; Giesselmann, Frank; Lemieux, Robert P

2017-05-14

Structural variants of the 'de Vries-like' mesogen 5-[4-(12,12,14,14,16,16-hexamethyl-12,14,16-trisilaheptadecyloxy)phenyl]-2-hexyloxypyrimidine (QL16-6), including two isomers with branched iso-tricarbosilane end-groups, were synthesized and their mesomorphic and 'de Vries-like' properties were characterized by polarized optical microscopy, differential scanning calorimetry, small angle and 2D X-ray scattering techniques. A comparative analysis of isomers with linear and branched tricarbosilane end-groups shows that they exhibit comparable mesomorphic and 'de Vries-like' properties. Furthermore, the difference in effective molecular length L eff between the linear and branched isomers in the SmA and SmC phases (ca. 4-5 Å), which was derived from 2D X-ray scattering experiments, suggests that the linear tricarbosilane end-group is hemispherical in shape on the time-average, as predicted by a DFT conformational analysis at the B3LYP/6-31G* level.

In vivo light scattering for the detection of cancerous and precancerous lesions of the cervix

PubMed Central

Mourant, Judith R.; Powers, Tamara M.; Bocklage, Thérese J.; Greene, Heather M.; Dorin, Maxine H.; Waxman, Alan G.; Zsemlye, Meggan M.; Smith, Harriet O.

2009-01-01

A non-invasive optical diagnostic system for detection of cancerous and precancerous lesions of the cervix was evaluated, in vivo. The optical system included a fiber optic probe designed to measure polarized and unpolarized light transport properties of a small volume of tissue. An algorithm for diagnosing tissue based on the optical measurements was developed which used four optical properties, three of which were related to light scattering properties and the fourth of which was related to hemoglobin concentration. A sensitivity of ∼77% and specificities in the mid 60's were obtained for separating high grade squamous intraepithelial lesions and cancer from other pathologies and normal tissue. The use of different cross-validation methods in algorithm development is analyzed and the relative difficulties of diagnosing certain pathologies is assessed. Furthermore, the robustness of the optical system for use by different doctors and to changes in fiber optic probe were also assessed and potential improvements in the optical system are discussed. PMID:19340117

Relative influence upon microwave emissivity of fine-scale stratigraphy, internal scattering, and dielectric properties

USGS Publications Warehouse

England, A.W.

1976-01-01

The microwave emissivity of relatively low-loss media such as snow, ice, frozen ground, and lunar soil is strongly influenced by fine-scale layering and by internal scattering. Radiometric data, however, are commonly interpreted using a model of emission from a homogeneous, dielectric halfspace whose emissivity derives exclusively from dielectric properties. Conclusions based upon these simple interpretations can be erroneous. Examples are presented showing that the emission from fresh or hardpacked snow over either frozen or moist soil is governed dominantly by the size distribution of ice grains in the snowpack. Similarly, the thickness of seasonally frozen soil and the concentration of rock clasts in lunar soil noticeably affect, respectively, the emissivities of northern latitude soils in winter and of the lunar regolith. Petrophysical data accumulated in support of the geophysical interpretation of microwave data must include measurements of not only dielectric properties, but also of geometric factors such as finescale layering and size distributions of grains, inclusions, and voids. ?? 1976 Birkha??user Verlag.

Press forging and optical properties of lithium fluoride

NASA Astrophysics Data System (ADS)

Ready, J. F.; Vora, H.

1980-07-01

Lithium fluoride is an important candidate material for windows on high power, short-pulse ultraviolet and visible lasers. Lithium fluoride crystals were press forged in one step over the temperature range 300 to 600 C to obtain fine grained polycrystalline material with improved mechanical properties. The deformation that can be given to a lithium fluoride crystal during forging is limited by the formation of internal cloudiness (veiling) with the deformation limit increasing with increasing forging temperature from about 40 percent at 400 C to 65 percent at 600 C. To suppress veiling, lithium fluoride crystals were forged in two steps over the temperature range 300 to 600 C, to total deformations of 69 to 76 percent, with intermediate annealing at 700 C. This technique yields a material which has lower scattering with more homogeneous microstructure than that obtained in one step forging. The results of characterization of various optical and mechanical properties of single crystal and forged lithium fluoride, including scattering, optical homogeneity, residual absorption, damage thresholds, environmental stability, and thresholds for microyield are described.

Realizing total reciprocity violation in the phase for photon scattering

PubMed Central

Deák, László; Bottyán, László; Fülöp, Tamás; Merkel, Dániel Géza; Nagy, Dénes Lajos; Sajti, Szilárd; Schulze, Kai Sven; Spiering, Hartmut; Uschmann, Ingo; Wille, Hans-Christian

2017-01-01

Reciprocity is when wave or quantum scattering satisfies a symmetry property, connecting a scattering process with the reversed one. While reciprocity involves the interchange of source and detector, it is fundamentally different from rotational invariance, and is a generalization of time reversal invariance, occurring in absorptive media as well. Due to its presence at diverse areas of physics, it admits a wide variety of applications. For polarization dependent scatterings, reciprocity is often violated, but violation in the phase of the scattering amplitude is much harder to experimentally observe than violation in magnitude. Enabled by the advantageous properties of nuclear resonance scattering of synchrotron radiation, we have measured maximal, i.e., 180-degree, reciprocity violation in the phase. For accessing phase information, we introduced a new version of stroboscopic detection. The scattering setting was devised based on a generalized reciprocity theorem that opens the way to construct new types of reciprocity related devices. PMID:28225031

Realizing total reciprocity violation in the phase for photon scattering.

PubMed

Deák, László; Bottyán, László; Fülöp, Tamás; Merkel, Dániel Géza; Nagy, Dénes Lajos; Sajti, Szilárd; Schulze, Kai Sven; Spiering, Hartmut; Uschmann, Ingo; Wille, Hans-Christian

2017-02-22

Reciprocity is when wave or quantum scattering satisfies a symmetry property, connecting a scattering process with the reversed one. While reciprocity involves the interchange of source and detector, it is fundamentally different from rotational invariance, and is a generalization of time reversal invariance, occurring in absorptive media as well. Due to its presence at diverse areas of physics, it admits a wide variety of applications. For polarization dependent scatterings, reciprocity is often violated, but violation in the phase of the scattering amplitude is much harder to experimentally observe than violation in magnitude. Enabled by the advantageous properties of nuclear resonance scattering of synchrotron radiation, we have measured maximal, i.e., 180-degree, reciprocity violation in the phase. For accessing phase information, we introduced a new version of stroboscopic detection. The scattering setting was devised based on a generalized reciprocity theorem that opens the way to construct new types of reciprocity related devices.

Accurately Measuring the Color of the Ocean on Earth and from Space: Uncertainties Revisited and A Report from the Community-Led Spectral Absorption Workshop to Update and Revise the NASA Inherent Optical Properties Protocol

NASA Technical Reports Server (NTRS)

Neeley, Aimee Renee

2014-01-01

The color of the ocean (apparent optical properties or AOPs) is determined by the spectral scattering and absorption of light by its dissolved and particulate constituents.The absorption and scattering properties of the water column are the so-called inherent optical properties.

Electron transport in erbium arsenide:indium gallium(aluminum)arsenide metal/semiconductor nanocomposites for thermoelectric power generation

NASA Astrophysics Data System (ADS)

Bahk, Je-Hyeong

Electron transport in thin film ErAs:InGa(Al)As metal/semiconductor nanocomposite materials grown by molecular beam epitaxy is investigated experimentally and theoretically for efficient thermoelectric power generation. Thermoelectric properties such as the Seebeck coefficient, the electrical conductivity, and the thermal conductivity are measured for the various compositions of the material up to 840 K. A special sample preparation method is proposed to protect the thin films from damage and/or decomposition, and prevent the parasitic substrate conduction effect during the high temperature measurements. The sample preparation method includes surface passivation, high temperature metallization with a diffusion barrier, and the covalent oxide bonding technique for substrate removal. The experimental results for the nanocomposite materials are analyzed using the Boltzmann transport equation under the relaxation time approximation. The scattering characteristics of free electrons in the InGa(Al)As is defined by four major scattering mechanisms such as the polar optical phonon scattering, the ionized impurity scattering, the alloy scattering, and the acoustic phonon deformation potential scattering. Combining these scattering mechanisms, the electron transport model successfully fits the temperature-dependent thermoelectric properties of Si-doped InGaAlAs materials, and predicts the figure of merits at various doping levels in various Al compositions. The nanoparticle-electron interaction is modeled as a momentum scattering for free electrons caused by the electrostatic potential perturbation around nanoparticles and the band offset at the interface. The ErAs nanoparticles are assumed to be semi-metals that can donate electrons to the matrix, and positively charged after the charge transfer to build up the screened coulomb potential outside them. The nanoparticle scattering rate is calculated for this potential profile using the partial wave method, and used to analyze the enhancement of the Seebeck coefficient. Finally, the experimental results for the various compositions of the ErAs:InGa(Al)As nanocomposites are fit using the electron transport model and the nanoparticle scattering. It is shown that nanoparticle scattering can enhance the power factor via energy-dependent electron scattering in ErAs:InGaAs system. The figure of merit for the 0.6% ErAs:(InGaAs)0.8(InAlAs) 0.2 lattice matched to InP is measured to be 1.3 at 800 K, and the theory predicts that it can reach 1.9 at 1000 K.

Long term measurements of optical properties and their hygroscopic enhancement

NASA Astrophysics Data System (ADS)

Hervo, M.; Sellegri, K.; Pichon, J. M.; Roger, J. C.; Laj, P.

2014-11-01

Optical properties of aerosols were measured from the GAW Puy de Dôme station (1465 m) over a seven year period (2006-2012). The impact of hygroscopicity on aerosol optical properties was calculated over a two year period (2010-2011). The analysis of the spatial and temporal variability of the optical properties showed that while no long term trend was found, a clear seasonal and diurnal variation was observed on the extensive parameters (scattering, absorption). Scattering and absorption coefficients were highest during the warm season and daytime, in concordance with the seasonality and diurnal variation of the PBL height reaching the site. Intensive parameters (single scattering albedo, asymmetry factor, refractive index) did not show such a strong diurnal variability, but still indicated different values depending on the season. Both extensive and intensive optical parameters were sensitive to the air mass origin. A strong impact of hygroscopicity on aerosol optical properties was calculated, mainly on aerosol scattering, with a dependence on the aerosol type. At 90% humidity, the scattering factor enhancement (fσsca) was more than 4.4 for oceanic aerosol that have mixed with a pollution plume. Consequently, the aerosol radiative forcing was estimated to be 2.8 times higher at RH = 90% and 1.75 times higher at ambient RH when hygroscopic growth of the aerosol was considered. The hygroscopicity enhancement factor of the scattering coefficient was parameterized as a function of humidity and air mass type.

Solid harmonic wavelet scattering for predictions of molecule properties

NASA Astrophysics Data System (ADS)

Eickenberg, Michael; Exarchakis, Georgios; Hirn, Matthew; Mallat, Stéphane; Thiry, Louis

2018-06-01

We present a machine learning algorithm for the prediction of molecule properties inspired by ideas from density functional theory (DFT). Using Gaussian-type orbital functions, we create surrogate electronic densities of the molecule from which we compute invariant "solid harmonic scattering coefficients" that account for different types of interactions at different scales. Multilinear regressions of various physical properties of molecules are computed from these invariant coefficients. Numerical experiments show that these regressions have near state-of-the-art performance, even with relatively few training examples. Predictions over small sets of scattering coefficients can reach a DFT precision while being interpretable.

Matter scattering in quadratic gravity and unitarity

NASA Astrophysics Data System (ADS)

Abe, Yugo; Inami, Takeo; Izumi, Keisuke; Kitamura, Tomotaka

2018-03-01

We investigate the ultraviolet (UV) behavior of two-scalar elastic scattering with graviton exchanges in higher-curvature gravity theory. In Einstein gravity, matter scattering is shown not to satisfy the unitarity bound at tree level at high energy. Among some of the possible directions for the UV completion of Einstein gravity, such as string theory, modified gravity, and inclusion of high-mass/high-spin states, we take R_{μν}^2 gravity coupled to matter. We show that matter scattering with graviton interactions satisfies the unitarity bound at high energy, even with negative norm states due to the higher-order derivatives of metric components. The difference in the unitarity property of these two gravity theories is probably connected to that in another UV property, namely, the renormalizability property of the two.

Spectral scattering characteristics of space target in near-UV to visible bands.

PubMed

Bai, Lu; Wu, Zhensen; Cao, Yunhua; Huang, Xun

2014-04-07

In this study, the spectral scattering characteristics of a space target are calculated in the near-UV to visible bands on the basis of measured data of spectral hemispheric reflectivity in the upper half space. Further, the bidirectional reflection distribution function (BRDF) model proposed by Davies is modified to describe the light scattering properties of a target surface. This modification aims to improve the characteristics identifying ability for different space targets. By using this modified Davies spectrum BRDF model, the spectral scattering characteristics of each subsurface can be obtained. A mathematical model of spectral scattering properties of the space target is built by summing all the contributing surface grid reflection scattering components, considering the impact of surface shadow effect.Moreover, the spectral scattering characteristics of the space target calculated with both the traditional and modified Davies BRDF models are compared. The results show that in the fixed and modified cases, the hemispheric reflectivity significantly affects the spectral scattering irradiance of the target.

Completeness of the Coulomb Wave Functions in Quantum Mechanics

ERIC Educational Resources Information Center

Mukunda, N.

1978-01-01

Gives an explicit and elementary proof that the radial energy eigenfunctions for the hydrogen atom in quantum mechanics, bound and scattering states included, form a complete set. The proof uses some properties of the confluent hypergeometric functions and the Cauchy residue theorem from analytic function theory. (Author/GA)

Full-wave Nonlinear Inverse Scattering for Acoustic and Electromagnetic Breast Imaging

NASA Astrophysics Data System (ADS)

Haynes, Mark Spencer

Acoustic and electromagnetic full-wave nonlinear inverse scattering techniques are explored in both theory and experiment with the ultimate aim of noninvasively mapping the material properties of the breast. There is evidence that benign and malignant breast tissue have different acoustic and electrical properties and imaging these properties directly could provide higher quality images with better diagnostic certainty. In this dissertation, acoustic and electromagnetic inverse scattering algorithms are first developed and validated in simulation. The forward solvers and optimization cost functions are modified from traditional forms in order to handle the large or lossy imaging scenes present in ultrasonic and microwave breast imaging. An antenna model is then presented, modified, and experimentally validated for microwave S-parameter measurements. Using the antenna model, a new electromagnetic volume integral equation is derived in order to link the material properties of the inverse scattering algorithms to microwave S-parameters measurements allowing direct comparison of model predictions and measurements in the imaging algorithms. This volume integral equation is validated with several experiments and used as the basis of a free-space inverse scattering experiment, where images of the dielectric properties of plastic objects are formed without the use of calibration targets. These efforts are used as the foundation of a solution and formulation for the numerical characterization of a microwave near-field cavity-based breast imaging system. The system is constructed and imaging results of simple targets are given. Finally, the same techniques are used to explore a new self-characterization method for commercial ultrasound probes. The method is used to calibrate an ultrasound inverse scattering experiment and imaging results of simple targets are presented. This work has demonstrated the feasibility of quantitative microwave inverse scattering by way of a self-consistent characterization formalism, and has made headway in the same area for ultrasound.

Atomic-level structural correlations across the morphotropic phase boundary of a ferroelectric solid solution: xBiMg 1/2Ti 1/2O 3-(1$-$x)PbTiO 3

DOE PAGES

Datta, Kaustuv; Neder, Reinhard B.; Chen, Jun; ...

2017-03-28

Revelation of unequivocal structural information at the atomic level for complex systems is uniquely important for deeper and generic understanding of the structure property connections and a key challenge in materials science. Here in this paper we report an experimental study of the local structure by applying total elastic scattering and Raman scattering analyses to an important non-relaxor ferroelectric solid solution exhibiting the so-called composition-induced morphotropic phase boundary (MPB), where concomitant enhancement of physical properties have been detected. The powerful combination of static and dynamic structural probes enabled us to derive direct correspondence between the atomic-level structural correlations and reportedmore » properties. The atomic pair distribution functions obtained from the neutron total scattering experiments were analysed through big-box atom-modelling implementing reverse Monte Carlo method, from which distributions of magnitudes and directions of off-centred cationic displacements were extracted. We found that an enhanced randomness of the displacement-directions for all ferroelectrically active cations combined with a strong dynamical coupling between the A- and B-site cations of the perovskite structure, can explain the abrupt amplification of piezoelectric response of the system near MPB. Finally, altogether this provides a more fundamental basis in inferring structure-property connections in similar systems including important implications in designing novel and bespoke materials.« less

First correlated measurements of the shape and scattering properties of cloud particles using the new Particle Habit Imaging and Polar Scattering (PHIPS) probe

NASA Astrophysics Data System (ADS)

Abdelmonem, A.; Schnaiter, M.; Amsler, P.; Hesse, E.; Meyer, J.; Leisner, T.

2011-05-01

Studying the radiative impact of cirrus clouds requires the knowledge of the link between their microphysics and the single scattering properties of the cloud particles. Usually, this link is created by modeling the optical scattering properties from in situ measurements of ice crystal size distributions. The measured size distribution and the assumed particle shape might be erroneous in case of non-spherical ice particles. We present here a novel optical sensor (the Particle Habit Imaging and Polar Scattering probe, PHIPS) designed to measure the 3-D morphology and the corresponding optical and microphysical parameters of individual cloud particles, simultaneously. Clouds containing particles ranging in size from a few micrometers to about 800 μm diameter can be systematically characterized with an optical resolution power of 2 μm and polar scattering resolution of 1° for forward scattering directions (from 1° to 10°) and 8° for side and backscattering directions (from 18° to 170°). The maximum acquisition rates for scattering phase functions and images are 262 KHz and 10 Hz, respectively. Some preliminary results collected in two ice cloud campaigns which were conducted in the AIDA cloud simulation chamber are presented. PHIPS showed reliability in operation and produced comparable size distributions and images to those given by other certified cloud particles instruments. A 3-D model of a hexagonal ice plate is constructed and the corresponding scattering phase function is compared to that modeled using the Ray Tracing with Diffraction on Facets (RTDF) program. PHIPS is candidate to be a novel air borne optical sensor for studying the radiative impact of cirrus clouds and correlating the particle habit-scattering properties which will serve as a reference for other single, or multi-independent, measurements instruments.

A stochastic model for density-dependent microwave Snow- and Graupel scattering coefficients of the NOAA JCSDA community radiative transfer model

NASA Astrophysics Data System (ADS)

Stegmann, Patrick G.; Tang, Guanglin; Yang, Ping; Johnson, Benjamin T.

2018-05-01

A structural model is developed for the single-scattering properties of snow and graupel particles with a strongly heterogeneous morphology and an arbitrary variable mass density. This effort is aimed to provide a mechanism to consider particle mass density variation in the microwave scattering coefficients implemented in the Community Radiative Transfer Model (CRTM). The stochastic model applies a bicontinuous random medium algorithm to a simple base shape and uses the Finite-Difference-Time-Domain (FDTD) method to compute the single-scattering properties of the resulting complex morphology.

Single scattering from nonspherical Chebyshev particles: A compendium of calculations

NASA Technical Reports Server (NTRS)

Wiscombe, W. J.; Mugnai, A.

1986-01-01

A large set of exact calculations of the scattering from a class of nonspherical particles known as Chebyshev particles' has been performed. Phase function and degree of polarization in random orientation, and parallel and perpendicular intensities in fixed orientations, are plotted for a variety of particles shapes and sizes. The intention is to furnish a data base against which both experimental data, and the predictions of approximate methods, can be tested. The calculations are performed with the widely-used Extended Boundary Condition Method. An extensive discussion of this method is given, including much material that is not easily available elsewhere (especially the analysis of its convergence properties). An extensive review is also given of all extant methods for nonspherical scattering calculations, as well as of the available pool of experimental data.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Dudek, Jozef

Highlights of the research include: the determination of the form of the lowest energy gluonic excitation within QCD and the spectrum of hybrid hadrons which follows; the first calculation of the spectrum of hybrid baryons within a first-principles approach to QCD; a detailed mapping out of the phase-shift of elastic ππ scattering featuring the ρ resonance at two values of the light quark mass within lattice QCD; the first (and to date, only) determinations of coupled-channel meson-meson scattering within first-principles QCD; the first (and to date, only) determinations of the radiative coupling of a resonant state, the ρ appearing inmore » πγ→ππ; the first (and to date, only) determination of the properties of the broad σ resonance in elastic ππ scattering within QCD without unjustified approximations.« less

Systematic approach to thermal leptogenesis

NASA Astrophysics Data System (ADS)

Frossard, T.; Garny, M.; Hohenegger, A.; Kartavtsev, A.; Mitrouskas, D.

2013-04-01

In this work we study thermal leptogenesis using nonequilibrium quantum field theory. Starting from fundamental equations for correlators of the quantum fields we describe the steps necessary to obtain quantum-kinetic equations for quasiparticles. These can easily be compared to conventional results and overcome conceptional problems inherent in the canonical approach. Beyond CP-violating decays we include also those scattering processes which are tightly related to the decays in a consistent approximation of fourth order in the Yukawa couplings. It is demonstrated explicitly how the S-matrix elements for the scattering processes in the conventional approach are related to two- and three-loop contributions to the effective action. We derive effective decay and scattering amplitudes taking medium corrections and thermal masses into account. In this context we also investigate CP-violating Higgs decay within the same formalism. From the kinetic equations we derive rate equations for the lepton asymmetry improved in that they include quantum-statistical effects and medium corrections to the quasiparticle properties.

Light scattering by nonspherical particles: Remote sensing and climatic implications

NASA Astrophysics Data System (ADS)

Liou, K. N.; Takano, Y.

Calculations of the scattering and adsorption properties of ice crystals and aerosols, which are usually nonspherical, require specific methodologies. There is no unique theoretical solution for the scattering by nonspherical particles. Practically, all the numerical solutions for the scattering of nonspherical particles, including the exact wave equation approach, integral equation method, and discrete-dipole approximation, are applicable only to size parameters less than about 20. Thus, these methods are useful for the study of radiation problems involving nonspherical aerosols and small ice crystals in the thermal infrared wavelengths. The geometric optics approximation has been used to evaluate the scattering, absorption and polarization properties of hexagonal ice crystals whose sizes are much larger than the incident wavelength. This approximation is generally valid for hexagonal ice crystals with size parameters larger than about 30. From existing laboratory data and theoretical results, we illustrate that nonspherical particles absorb less and have a smaller asymmetry factor than the equal-projected area/volume spherical counterparts. In particular, we show that hexagonal ice crystals exhibit numerous halo and arc features that cannot be obtained from spherical particles; and that ice crystals scatter more light in the 60° to 140° scattering angle regions than the spherical counterparts. Satellite remote sensing of the optical depth and height of cirrus clouds using visible and IR channels must use appropriate phase functions for ice crystals. Use of an equivalent sphere model would lead to a significant overestimation and underestimation of the cirrus optical depth and height, respectively. Interpretation of the measurements for polarization reflected from sunlight involving cirrus clouds cannot be made without an appropriate ice crystal model. Large deviations exist for the polarization patterns between spheres and hexagonal ice crystals. Interpretation of lidar backscattering and depolarization signals must also utilize the scattering characteristics of hexagonal ice crystals. Equivalent spherical models substantially underestimate the broadband solar albedos of ice crystal clouds because of stronger forward scattering and larger absorption by spherical particles than hexagonal ice crystals. We illustrate that the net cloud radiative forcing at the top of the atmosphere involving most cirrus clouds is positive, implying that the IR greenhouse effect outweighs the solar albedo effect. If the radiative properties of equivalent spheres are used, a significant increase in cloud radiative forcing occurs. Using a one-dimensional cloud and climate model, we further demonstrate that there is sufficient model sensitivity, in terms of temperature increase, to the use of ice crystal models in radiation calculations.

Method for using polarization gating to measure a scattering sample

DOEpatents

Baba, Justin S.

2015-08-04

Described herein are systems, devices, and methods facilitating optical characterization of scattering samples. A polarized optical beam can be directed to pass through a sample to be tested. The optical beam exiting the sample can then be analyzed to determine its degree of polarization, from which other properties of the sample can be determined. In some cases, an apparatus can include a source of an optical beam, an input polarizer, a sample, an output polarizer, and a photodetector. In some cases, a signal from a photodetector can be processed through attenuation, variable offset, and variable gain.

Optical diagnostics based on elastic scattering: Recent clinical demonstrations with the Los Alamos Optical Biopsy System

DOE Office of Scientific and Technical Information (OSTI.GOV)

Bigio, I.J.; Loree, T.R.; Mourant, J.

1993-08-01

A non-invasive diagnostic tool that could identify malignancy in situ and in real time would have a major impact on the detection and treatment of cancer. We have developed and are testing early prototypes of an optical biopsy system (OBS) for detection of cancer and other tissue pathologies. The OBS invokes a unique approach to optical diagnosis of tissue pathologies based on the elastic scattering properties, over a wide range of wavelengths, of the microscopic structure of the tissue. The use of elastic scattering as the key to optical tissue diagnostics in the OBS is based on the fact thatmore » many tissue pathologies, including a majority of cancer forms, manifest significant architectural changes at the cellular and sub-cellular level. Since the cellular components that cause elastic scattering have dimensions typically on the order of visible to near-IR wavelengths, the elastic (Mie) scattering properties will be strongly wavelength dependent. Thus, morphology and size changes can be expected to cause significant changes in an optical signature that is derived from the wavelength dependence of elastic scattering. The data acquisition and storage/display time with the OBS instrument is {approximately}1 second. Thus, in addition to the reduced invasiveness of this technique compared with current state-of-the-art methods (surgical biopsy and pathology analysis), the OBS offers the possibility of impressively faster diagnostic assessment. The OBS employs a small fiber-optic probe that is amenable to use with any endoscope, catheter or hypodermic, or to direct surface examination (e.g. as in skin cancer or cervical cancer). It has been tested in vitro on animal and human tissue samples, and clinical testing in vivo is currently in progress.« less

Effect of Diffuse Backscatter in Cassini Datasets on the Inferred Properties of Titan's surface

NASA Astrophysics Data System (ADS)

Sultan-Salem, A. K.; Tyler, G. L.

2006-12-01

Microwave (2.18 cm-λ) backscatter data for the surface of Titan obtained with the Cassini Radar instrument exhibit a significant diffuse scattering component. An empirical scattering law of the form Acos^{n}θ, with free parameters A and n, is often employed to model diffuse scattering, which may involve one or more unidentified mechanisms and processes, such as volume scattering and scattering from surface structure that is much smaller than the electromagnetic wavelength used to probe the surface. The cosine law in general is not explicit in its dependence on either the surface structure or electromagnetic parameters. Further, the cosine law often is only a poor representation of the observed diffuse scattering, as can be inferred from computation of standard goodness-of-fit measures such as the statistical significance. We fit four Cassini datasets (TA Inbound and Outbound, T3 Outbound, and T8 Inbound) with a linear combination of a cosine law and a generalized fractal-based quasi-specular scattering law (A. K. Sultan- Salem and G. L. Tyler, J. Geophys. Res., 111, E06S08, doi:10.1029/2005JE002540, 2006), in order to demonstrate how the presence of diffuse scattering increases considerably the uncertainty in surface parameters inferred from the quasi-specular component, typically the dielectric constant of the surface material and the surface root-mean-square slope. This uncertainty impacts inferences concerning the physical properties of the surfaces that display mixed scattering properties.

Inherent and Apparent Scattering Properties of Coated or Uncoated Spheres Embedded in an Absorbing Host Medium

NASA Technical Reports Server (NTRS)

Yang, P.; Gao, B.-C.; Wiscombe, W. J.; Mishchenko, M. I.; Platnick, S.; Huang, H.-L.; Baum, B. A.; Hu, Y. X.; Winkler, D,; Tsay, S.-C.;

Operational properties of fluctuation X-ray scattering data

DOE PAGES

Malmerberg, Erik; Kerfeld, Cheryl A.; Zwart, Petrus H.

2015-03-20

X-ray scattering images collected on timescales shorter than rotation diffusion times using a (partially) coherent beam result in a significant increase in information content in the scattered data. These measurements, named fluctuation X-ray scattering (FXS), are typically performed on an X-ray free-electron laser (XFEL) and can provide fundamental insights into the structure of biological molecules, engineered nanoparticles or energy-related mesoscopic materials beyond what can be obtained with standard X-ray scattering techniques. In order to understand, use and validate experimental FXS data, the availability of basic data characteristics and operational properties is essential, but has been absent up to this point.more » In this communication, an intuitive view of the nature of FXS data and their properties is provided, the effect of FXS data on the derived structural models is highlighted, and generalizations of the Guinier and Porod laws that can ultimately be used to plan experiments and assess the quality of experimental data are presented.« less

Light Scattering by Lunar Exospheric Dust: What could be Learned from LRO LAMP and LADEE UVS?

NASA Astrophysics Data System (ADS)

Glenar, D. A.; Stubbs, T. J.; Richard, D. T.; Stern, S. A.; Retherford, K. D.; Gladstone, R.; Feldman, P. D.; Colaprete, A.; Delory, G. T.

2011-12-01

Two complementary spectrometers, namely the Lunar Reconnaissance Orbiter, Lyman Alpha Mapping Project (LAMP) and the planned Lunar Atmosphere and Dust Environment Explorer (LADEE) Ultraviolet Explorer (UVS) will carry out sensitive searches for high altitude exospheric dust, via detection of scattered sunlight. The combined spectral coverage of these instruments extends from far-UV to near-IR wavelengths. Over this wavelength range, grain size parameter (X=2πr/λ, with r the grain radius and λ the wavelength) changes dramatically, which makes broad wavelength coverage a good diagnostic of grain size. Utilizing different pointing geometries, both LAMP and UVS are able to observe dust over a range of scattering angles, as well as measure the dust vertical profile via limb measurements at multiple tangent heights. We summarize several categories of information that can be inferred from the data sets, using broadband simulations of horizon glow as observed at the limb. Grain scattering properties used in these simulations were computed for multiple grain shapes using Discrete-Dipole theory. Some cautionary remarks are included regarding the use of Mie theory to interpret scattering measurements.

Scattering Properties of Needle-Like and plate-like Ice Spheroids with Moderate Size Parameters

NASA Technical Reports Server (NTRS)

Zakharova, Nadia T.; Mishchenko, Michael I.; Hansen, James E. (Technical Monitor)

2000-01-01

We use the current advanced version of the T-matrix method to compute the optical cross sections, the asymmetry parameter of the phase function, and the scattering matrix elements of ice spheroids with aspect ratios up to 20 and surface-equivalent-sphere size parameters up to 12. We demonstrate that plate-like and needle-like particles with moderate size parameters possess unique scattering properties: their asymmetry parameters and phase functions are similar to those of surface-equivalent spheres, whereas all other elements of the scattering matrix are typical of particles much smaller than the wavelength (Rayleigh scatterers). This result may have important implications for optical particle sizing and remote sensing of the terrestrial and planetary atmospheres.

Optical property retrievals of subvisual cirrus clouds from OSIRIS limb-scatter measurements

NASA Astrophysics Data System (ADS)

Wiensz, J. T.; Degenstein, D. A.; Lloyd, N. D.; Bourassa, A. E.

2012-08-01

We present a technique for retrieving the optical properties of subvisual cirrus clouds detected by OSIRIS, a limb-viewing satellite instrument that measures scattered radiances from the UV to the near-IR. The measurement set is composed of a ratio of limb radiance profiles at two wavelengths that indicates the presence of cloud-scattering regions. Optical properties from an in-situ database are used to simulate scattering by cloud-particles. With appropriate configurations discussed in this paper, the SASKTRAN successive-orders of scatter radiative transfer model is able to simulate accurately the in-cloud radiances from OSIRIS. Configured in this way, the model is used with a multiplicative algebraic reconstruction technique (MART) to retrieve the cloud extinction profile for an assumed effective cloud particle size. The sensitivity of these retrievals to key auxiliary model parameters is shown, and it is demonstrated that the retrieved extinction profile models accurately the measured in-cloud radiances from OSIRIS. Since OSIRIS has an 11-yr record of subvisual cirrus cloud detections, the work described in this manuscript provides a very useful method for providing a long-term global record of the properties of these clouds.

Instantaneous influence of dust storms on the optical scattering property of the ocean: a case study in the Yellow Sea, China.

PubMed

Chen, Shuguo; Zhang, Tinglu; Chen, Wenzhong; Shi, Jinhui; Hu, Lianbo; Song, Qingjun

2016-12-12

Asian dust storms originating from arid or semi-arid regions of China or her adjacent regions have important impact on the atmosphere and water composition, and ecological environment of the Eastern China Seas. This research used data collected in the middle of the South Yellow Sea, China, during a dust storm event from 23 April to 24 April 2006 to analyze the instantaneous influence of dust storms on optical scattering properties, which are closely related to particle characteristics. The analysis results showed that the dust storm had a remarkable influence on the optical scattering property in the upper mixed layer of water, and dust particles drily deposited from the dust storm with an aerosol optical depth of nearly 2.5 into the water could induce a 0.14 m^-1 change in the water optical scattering coefficient at 532 nm at the depth of 4 m. The duration of the instantaneous influence of the dust storm on the water optical scattering properties was short, and this influence disappeared rapidly within approximately 3 hours after the end of the dust storm.

Z-pinch Plasma Temperature and Implosion Velocity from Laboratory Plasma Jets using Thomson Scattering

NASA Astrophysics Data System (ADS)

Banasek, Jacob; Byvank, Tom; Kusse, Bruce; Hammer, David

2016-10-01

We discuss the use of collective Thomson scattering to determine the implosion velocity and other properties of laboratory plasma jets. The plasma jet is created using a 1 MA pulsed power machine with a 15 μm Al radial foil load. The Thomson scattering laser has a maximum energy of 10 J at 526.5 nm with a pulse duration of 3 ns. Using a time gated ICCD camera and spectrometer system we are able to record the scattered spectrum from 9 or 18 regions along the laser path with sub-mm spatial resolution. Collecting scattered radiation from the same area at two different angles simultaneously enables determination of both the radial and azimuthal velocities. The scattered spectrum for non-magnetized jets indicates a radial implosion velocity of 27 km/s into the jets. A determination of ion and electron temperatures from the scattered spectrum is in progress. Comparing results using a laser energy of 10 J and 1 J shows noticeable effects on plasma jet properties when using 10 J. Therefore the lower laser energy must be used to determine the plasma properties. This research is supported by the NNSA Stewardship Sciences Academic Programs under DOE Cooperative Agreement DE-NA0001836.

Diagnostics of Unseeded Air and Nitrogen Flows by Molecular Tagging

DTIC Science & Technology

2015-07-21

the polarization components across the FLEET line and the computed molecular density and dissociation fraction. Rayleigh Scattering Polarimetry V...Pol H Pol BPF HP CCM FLEET Emission Imaging Planar Rayleigh Scattering Rayleigh Scattering Polarimetry Density of molecules (normalized...the flow transport properties. This has been studied using Rayleigh scattering and Rayleigh scattering polarimetry . Figure 8 shows the evolution of

Impact of Interfacial Roughness on the Sorption Properties of Nanocast Polymers

DOE PAGES

Sridhar, Manasa; Gunugunuri, Krishna R.; Hu, Naiping; ...

2016-03-16

Nanocasting is an emerging method to prepare organic polymers with regular, nanometer pores using inorganic templates. This report assesses the impact of imperfect template replication on the sorption properties of such polymer castings. Existing X-ray diffraction data show that substantial diffuse scattering exists in the small-angle region even though TEM images show near perfect lattices of uniform pores. To assess the origin of the diffuse scattering, the morphology of the phenol - formaldehyde foams (PFF) was investigated by small-angle X-ray scattering (SAXS). The observed diffuse scattering is attributed to interfacial roughness due to fractal structures. Such roughness has a profoundmore » impact on the sorption properties. Conventional pore- filling models, for example, overestimate protein sorption capacity. A mathematical framework is presented to calculate sorption properties based on observed morphological parameters. The formalism uses the surface fractal dimension determined by SAXS in conjunction with nitrogen adsorption isotherms to predict lysozyme sorption. The results are consistent with measured lysozyme loading.« less

Optical properties (bidirectional reflectance distribution function) of shot fabric.

PubMed

Lu, R; Koenderink, J J; Kappers, A M

2000-11-01

To study the optical properties of materials, one needs a complete set of the angular distribution functions of surface scattering from the materials. Here we present a convenient method for collecting a large set of bidirectional reflectance distribution function (BRDF) samples in the hemispherical scattering space. Material samples are wrapped around a right-circular cylinder and irradiated by a parallel light source, and the scattered radiance is collected by a digital camera. We tilted the cylinder around its center to collect the BRDF samples outside the plane of incidence. This method can be used with materials that have isotropic and anisotropic scattering properties. We demonstrate this method in a detailed investigation of shot fabrics. The warps and the fillings of shot fabrics are dyed different colors so that the fabric appears to change color at different viewing angles. These color-changing characteristics are found to be related to the physical and geometrical structure of shot fabric. Our study reveals that the color-changing property of shot fabrics is due mainly to an occlusion effect.

Effect of void shape in Czochralski-Si wafers on the intensity of laser-scattering

NASA Astrophysics Data System (ADS)

Takahashi, J.; Kawakami, K.; Nakai, K.

2001-06-01

The shape effect of anisotropic-shaped microvoid defects in Czochralski-grown silicon wafers on the intensity of laser scattering has been investigated. The size and shape of the defects were examined by means of transmission electron microscopy. Octahedral voids in conventional (nitrogen-undoped) wafers showed an almost isotropic scattering property under the incident condition of a p-polarization beam. On the other hand, parallelepiped-plate-shaped voids in nitrogen-doped wafers showed an anisotropic scattering property on both p- and s-polarized components of scattered light, depending strongly on the incident laser direction. The measured results were explained not by scattering calculation using Born approximation but by calculation based on Rayleigh scattering. It was found that the s component is explained by an inclination of a dipole moment induced on a defect from the scattering plane. Furthermore, using numerical electromagnetic analysis it was shown that the asymmetric behavior of the s component on the parallelepiped-plate voids is ascribed to the parallelepiped shape effect. These results suggest that correction of the scattering intensity is necessary to evaluate the size and volume of anisotropic-shaped defects from the scattered intensity.

Retrieval of Snow Properties for Ku- and Ka-band Dual-Frequency Radar

NASA Technical Reports Server (NTRS)

Liao, Liang; Meneghini, Robert; Tokay, Ali; Bliven, Larry F.

2016-01-01

The focus of this study is on the estimation of snow microphysical properties and the associated bulk parameters such as snow water content and water equivalent snowfall rate for Ku- and Ka-band dual-frequency radar. This is done by exploring a suitable scattering model and the proper particle size distribution (PSD) assumption that accurately represent, in the electromagnetic domain, the micro/macro-physical properties of snow. The scattering databases computed from simulated aggregates for small-to-moderate particle sizes are combined with a simple scattering model for large particle sizes to characterize snow scattering properties over the full range of particle sizes. With use of the single-scattering results, the snow retrieval lookup tables can be formed in a way that directly links the Ku- and Ka-band radar reflectivities to snow water content and equivalent snowfall rate without use of the derived PSD parameters. A sensitivity study of the retrieval results to the PSD and scattering models is performed to better understand the dual-wavelength retrieval uncertainties. To aid in the development of the Ku- and Ka-band dual-wavelength radar technique and to further evaluate its performance, self-consistency tests are conducted using measurements of the snow PSD and fall velocity acquired from the Snow Video Imager Particle Image Probe (SVIPIP) duringthe winter of 2014 at the NASA Wallops Flight Facility site in Wallops Island, Virginia.

Retrieval of Snow Properties for Ku- and Ka-Band Dual-Frequency Radar

NASA Technical Reports Server (NTRS)

Liao, Liang; Meneghini, Robert; Tokay, Ali; Bliven, Larry F.

2016-01-01

The focus of this study is on the estimation of snow microphysical properties and the associated bulk parameters such as snow water content and water equivalent snowfall rate for Ku- and Ka-band dual-frequency radar. This is done by exploring a suitable scattering model and the proper particle size distribution (PSD) assumption that accurately represent, in the electromagnetic domain, the micro-macrophysical properties of snow. The scattering databases computed from simulated aggregates for small-to-moderate particle sizes are combined with a simple scattering model for large particle sizes to characterize snow-scattering properties over the full range of particle sizes. With use of the single-scattering results, the snow retrieval lookup tables can be formed in a way that directly links the Ku- and Ka-band radar reflectivities to snow water content and equivalent snowfall rate without use of the derived PSD parameters. A sensitivity study of the retrieval results to the PSD and scattering models is performed to better understand the dual-wavelength retrieval uncertainties. To aid in the development of the Ku- and Ka-band dual-wavelength radar technique and to further evaluate its performance, self-consistency tests are conducted using measurements of the snow PSD and fall velocity acquired from the Snow Video Imager Particle Image Probe (SVIPIP) during the winter of 2014 at the NASA Wallops Flight Facility site in Wallops Island, Virginia.

Local scattering property scales flow speed estimation in laser speckle contrast imaging

NASA Astrophysics Data System (ADS)

Miao, Peng; Chao, Zhen; Feng, Shihan; Yu, Hang; Ji, Yuanyuan; Li, Nan; Thakor, Nitish V.

2015-07-01

Laser speckle contrast imaging (LSCI) has been widely used in in vivo blood flow imaging. However, the effect of local scattering property (scattering coefficient µ s ) on blood flow speed estimation has not been well investigated. In this study, such an effect was quantified and involved in relation between speckle autocorrelation time τ c and flow speed v based on simulation flow experiments. For in vivo blood flow imaging, an improved estimation strategy was developed to eliminate the estimation bias due to the inhomogeneous distribution of the scattering property. Compared to traditional LSCI, a new estimation method significantly suppressed the imaging noise and improves the imaging contrast of vasculatures. Furthermore, the new method successfully captured the blood flow changes and vascular constriction patterns in rats’ cerebral cortex from normothermia to mild and moderate hypothermia.

Scattering properties of electromagnetic waves from metal object in the lower terahertz region

NASA Astrophysics Data System (ADS)

Chen, Gang; Dang, H. X.; Hu, T. Y.; Su, Xiang; Lv, R. C.; Li, Hao; Tan, X. M.; Cui, T. J.

2018-01-01

An efficient hybrid algorithm is proposed to analyze the electromagnetic scattering properties of metal objects in the lower terahertz (THz) frequency. The metal object can be viewed as perfectly electrical conducting object with a slightly rough surface in the lower THz region. Hence the THz scattered field from metal object can be divided into coherent and incoherent parts. The physical optics and truncated-wedge incremental-length diffraction coefficients methods are combined to compute the coherent part; while the small perturbation method is used for the incoherent part. With the MonteCarlo method, the radar cross section of the rough metal surface is computed by the multilevel fast multipole algorithm and the proposed hybrid algorithm, respectively. The numerical results show that the proposed algorithm has good accuracy to simulate the scattering properties rapidly in the lower THz region.

Effects of energy conservation on equilibrium properties of hot asymmetric nuclear matter

NASA Astrophysics Data System (ADS)

Zhang, Zhen; Ko, Che Ming

2018-01-01

Based on the relativistic Vlasov-Uehling-Uhlenbeck transport model, which includes relativistic scalar and vector potentials on baryons, we consider an N -Δ -π system in a box with periodic boundary conditions to study the effects of energy conservation in particle production and absorption processes on the equilibrium properties of the system. The density and temperature of the matter in the box are taken to be similar to the hot dense matter formed in heavy ion collisions at intermediate energies. We find that to maintain the equilibrium numbers of N ,Δ , and π , which depend on the mean-field potentials of N and Δ , we must include these potentials in the energy conservation condition that determines the momenta of outgoing particles after a scattering or decay process. We further find that the baryon scalar potentials mainly affect the Δ and pion equilibrium numbers, while the baryon vector potentials have considerable effect on the effective charged pion ratio at equilibrium. Our results thus indicate that it is essential to include in the transport model the effect of potentials in the energy conservation of a scattering or decay process, which is ignored in most transport models, for studying pion production in heavy ion collisions.

Polarimetry of Solar System Objects: Observations vs. Models

NASA Astrophysics Data System (ADS)

Yanamandra-Fisher, P. A.

2014-04-01

The overarching goals for the remote sensing and robotic exploration of planetary systems are: (1) understanding the formation of planetary systems and their diversity; and (2) search for habitability. Since all objects have unique polarimetric signatures inclusion of spectrophotopolarimetry as a complementary approach to standard techniques of imaging and spectroscopy, provides insight into the scattering properties of the planetary media. Specifically, linear and circular polarimetric signatures of the object arise from different physical processes and their study proves essential to the characterization of the object. Linear polarization of reflected light by various solar system objects provides insight into the scattering characteristics of atmospheric aerosols and hazes? and surficial properties of atmosphereless bodies. Many optically active materials are anisotropic and so their scattering properties differ with the object's principal axes (such as dichroic or birefringent materials) and are crystalline in structure instead of amorphous, (eg., the presence of olivines and silicates in cometary dust and circumstellar disks? Titan, etc.). Ices (water and other species) are abundant in the system indicated in their near - infrared spectra. Gas giants form outside the frost line (where ices condense), and their satellites and ring systems exhibit signature of water ice? clathrates, nonices (Si, C, Fe) in their NIR spectra and spectral dependence of linear polarization. Additionally, spectral dependence of polarization is important to separate the macroscopic (bulk) properties of the scattering medium from the microscopic (particulate) properties of the scattering medium. Circular polarization, on the other hand, is indicative of magnetic fields and biologically active molecules, necessary for habitability. These applications suffer from lack of detailed observations, instrumentation, dedicated missions and numericalretrieval methods. With recent discoveries and results of main belt comets, asteroids with ring system, lunar studies, planned exploration of planetary satellites that may harbour sub-surface oceans, there is increasing need to include polarimetric (linear, circular and differential) as an integral observing mode of instruments and facilities. For laboratory measurements, there is a need to identify simulants that mimic the polarimetric behaviour of solar system small bodies and measure their polarimetric behavior as function of various physical process they are subject to and have undergone radiation changes of their surfaces. Therefore, inclusion of polarimetric remote sensing and development of spectropolarimeters for groundbased facilities and instruments on space missions is needed, with similar maturation of vector radiative transfer models and related laboratory measurements.

Laboratory Measurements of Single-Particle Polarimetric Spectrum

NASA Astrophysics Data System (ADS)

Gritsevich, M.; Penttila, A.; Maconi, G.; Kassamakov, I.; Helander, P.; Puranen, T.; Salmi, A.; Hæggström, E.; Muinonen, K.

2017-12-01

Measuring scattering properties of different targets is important for material characterization, remote sensing applications, and for verifying theoretical results. Furthermore, there are usually simplifications made when we model targets and compute the scattering properties, e.g., ideal shape or constant optical parameters throughout the target material. Experimental studies help in understanding the link between the observed properties and computed results. Experimentally derived Mueller matrices of studied particles can be used as input for larger-scale scattering simulations, e.g., radiative transfer computations. This method allows to bypass the problem of using an idealized model for single-particle optical properties. While existing approaches offer ensemble- and orientation-averaged particle properties, our aim is to measure individual particles with controlled or known orientation. With the newly developed scatterometer, we aim to offer novel possibility to measure single, small (down to μm-scale) targets and their polarimetric spectra. This work presents an experimental setup that measures light scattered by a fixed small particle with dimensions ranging between micrometer and millimeter sizes. The goal of our setup is nondestructive characterization of such particles by measuring light of multiple wavelengths scattered in 360° in a horizontal plane by an ultrasonically levitating sample, whilst simultaneously controlling its 3D position and orientation. We describe the principles and design of our instrument and its calibration. We also present example measurements of real samples. This study was conducted under the support from the European Research Council, in the frame of the Advanced Grant project No. 320773 `Scattering and Absorption of Electromagnetic Waves in Particulate Media' (SAEMPL).

Biophotonics of skin: method for correction of deep Raman spectra distorted by elastic scattering

NASA Astrophysics Data System (ADS)

Roig, Blandine; Koenig, Anne; Perraut, François; Piot, Olivier; Gobinet, Cyril; Manfait, Michel; Dinten, Jean-Marc

2015-03-01

Confocal Raman microspectroscopy allows in-depth molecular and conformational characterization of biological tissues non-invasively. Unfortunately, spectral distortions occur due to elastic scattering. Our objective is to correct the attenuation of in-depth Raman peaks intensity by considering this phenomenon, enabling thus quantitative diagnosis. In this purpose, we developed PDMS phantoms mimicking skin optical properties used as tools for instrument calibration and data processing method validation. An optical system based on a fibers bundle has been previously developed for in vivo skin characterization with Diffuse Reflectance Spectroscopy (DRS). Used on our phantoms, this technique allows checking their optical properties: the targeted ones were retrieved. Raman microspectroscopy was performed using a commercial confocal microscope. Depth profiles were constructed from integrated intensity of some specific PDMS Raman vibrations. Acquired on monolayer phantoms, they display a decline which is increasing with the scattering coefficient. Furthermore, when acquiring Raman spectra on multilayered phantoms, the signal attenuation through each single layer is directly dependent on its own scattering property. Therefore, determining the optical properties of any biological sample, obtained with DRS for example, is crucial to correct properly Raman depth profiles. A model, inspired from S.L. Jacques's expression for Confocal Reflectance Microscopy and modified at some points, is proposed and tested to fit the depth profiles obtained on the phantoms as function of the reduced scattering coefficient. Consequently, once the optical properties of a biological sample are known, the intensity of deep Raman spectra distorted by elastic scattering can be corrected with our reliable model, permitting thus to consider quantitative studies for purposes of characterization or diagnosis.

Sequential weighted Wiener estimation for extraction of key tissue parameters in color imaging: a phantom study

NASA Astrophysics Data System (ADS)

Chen, Shuo; Lin, Xiaoqian; Zhu, Caigang; Liu, Quan

2014-12-01

Key tissue parameters, e.g., total hemoglobin concentration and tissue oxygenation, are important biomarkers in clinical diagnosis for various diseases. Although point measurement techniques based on diffuse reflectance spectroscopy can accurately recover these tissue parameters, they are not suitable for the examination of a large tissue region due to slow data acquisition. The previous imaging studies have shown that hemoglobin concentration and oxygenation can be estimated from color measurements with the assumption of known scattering properties, which is impractical in clinical applications. To overcome this limitation and speed-up image processing, we propose a method of sequential weighted Wiener estimation (WE) to quickly extract key tissue parameters, including total hemoglobin concentration (CtHb), hemoglobin oxygenation (StO2), scatterer density (α), and scattering power (β), from wide-band color measurements. This method takes advantage of the fact that each parameter is sensitive to the color measurements in a different way and attempts to maximize the contribution of those color measurements likely to generate correct results in WE. The method was evaluated on skin phantoms with varying CtHb, StO2, and scattering properties. The results demonstrate excellent agreement between the estimated tissue parameters and the corresponding reference values. Compared with traditional WE, the sequential weighted WE shows significant improvement in the estimation accuracy. This method could be used to monitor tissue parameters in an imaging setup in real time.

Analysis of derived optical parameters of atmospheric particles during a biomass burning event. Comparison with fossil fuel burning

NASA Astrophysics Data System (ADS)

Costa, A.; Mogo, S.; Cachorro, V.; de Frutos, A.; Medeiros, M.; Martins, R.; López, J. F.; Marcos, A.; Marcos, N.; Bizarro, S.; Mano, F.

2015-12-01

During the day November 26, 2014, a scheduled cleanup of the woods took place around the GOA-UVa aerosol measurement station located at the campus of the University of Beira Interior (40° 16’30”N, 7°30’35”W, 704m a.s.l.), Covilhã, Portugal. This cleanup included excessive vegetation removal during the morning, using fossil fuel-burning machinery, and burning of the vegetation during the afternoon. In situ measurements of aerosol optical properties were made and this study aims the characterization of the evolution of aerosol properties during the day. The optical parameters were monitored using a 3-wavelength nephelometer and a 3-wavelength particle soot absorption photometer. Selective sampling/exclusion of the coarse particles was done each 5 minutes. The scattering and absorption Ångström exponents as well as the single scattering albedo were derived and fully analyzed. The scattering and absorption coefficients increased dramatically during the event, reaching values as high as 720.3 Mm-1 and 181.9 Mm-1, respectively, for the green wavelength and PM10 size fraction. The spectral behavior of these parameters also changed wildly along the day and an inversion of the slope from positive to negative in the case of the single scattering albedo was observed.

Aerosol Optical Properties and Chemical Composition Measured on the Ronald H. Brown During ACE-Asia

NASA Astrophysics Data System (ADS)

Quinn, P. K.; Bates, T. S.; Miller, T. L.; Coffman, D.

2001-12-01

Measurements of aerosol chemical, physical, and optical properties were made onboard the NOAA R/V Ronald H. Brown during the ACE-Asia Intensive Field Program to characterize Asian aerosol as it was transported across the Pacific Ocean. The ship traveled across the Pacific from Hawaii to Japan and into the East China Sea and the Sea of Japan. Trajectories indicate that remote marine air masses were sampled on the transit to Japan. In the ACE-Asia study region air masses from Japan, China, Mongolia, and the Korea Peninsula were sampled. A variety of aerosol types were encountered including those of marine, volcanic, crustal, and industrial origin. Presented here, for the different air masses encountered, are aerosol optical properties (scattering and absorption coefficients, single scattering albedo, Angstrom Exponent, and aerosol optical depth) and chemical composition (major ions, total organic and black carbon, and trace elements). Scattering by submicron aerosol (55 % RH and 550 nm) was less than 20 1/Mm during the transit from Hawaii to Japan. In continental air masses, values ranged from 60 to 320 1/Mm with the highest submicron scattering coefficients occurring during prefrontal conditions with a low marine boundary layer height and trajectories from Japan. For the continental air masses, the ratio of scattering by submicron to sub-10 micron aerosol during polluted conditions averaged 0.8 and during a dust event 0.41. Aerosol optical depth (500 nm) ranged from 0.08 during the Pacific transit to 1.3 in the prefrontal conditions described above. Optical depths during dust events ranged from 0.2 to 0.6. Submicron non-sea salt (nss) sulfate concentrations ranged from 0.5 ug/m-3 during the Pacific transit to near 30 ug/m-3 during the prefrontal conditions described above. Black carbon to total carbon mass ratios in air masses from Asia averaged 0.18 with highest values (0.32) corresponding to trajectories crossing the Yangtze River valley.

Subsurface Scattered Photons: Friend or Foe? Improving visible light laser altimeter elevation estimates, and measuring surface properties using subsurface scattered photons

NASA Astrophysics Data System (ADS)

Greeley, A.; Kurtz, N. T.; Neumann, T.; Cook, W. B.; Markus, T.

2016-12-01

Photon counting laser altimeters such as MABEL (Multiple Altimeter Beam Experimental Lidar) - a single photon counting simulator for ATLAS (Advanced Topographical Laser Altimeter System) - use individual photons with visible wavelengths to measure their range to target surfaces. ATLAS, the sole instrument on NASA's upcoming ICESat-2 mission, will provide scientists a view of Earth's ice sheets, glaciers, and sea ice with unprecedented detail. Precise calibration of these instruments is needed to understand rapidly changing parameters such as sea ice freeboard, and to measure optical properties of surfaces like snow covered ice sheets using subsurface scattered photons. Photons that travel through snow, ice, or water before scattering back to an altimeter receiving system travel farther than photons taking the shortest path between the observatory and the target of interest. These delayed photons produce a negative elevation bias relative to photons scattered directly off these surfaces. We use laboratory measurements of snow surfaces using a flight-tested laser altimeter (MABEL), and Monte Carlo simulations of backscattered photons from snow to estimate elevation biases from subsurface scattered photons. We also use these techniques to demonstrate the ability to retrieve snow surface properties like snow grain size.

Flow cytometry of sputum: assessing inflammation and immune response elements in the bronchial airways

PubMed Central

Lay, John C.; Peden, David B.; Alexis, Neil E.

2012-01-01

Background The evaluation of sputum leukocytes by flow cytometry is an opportunity to assess characteristics of cells residing in the central airways, yet it is hampered by certain inherent properties of sputum including mucus and large amounts of contaminating cells and debris. Objective To develop a gating strategy based on specific antibody panels in combination with light scatter properties for flow cytometric evaluation of sputum cells. Methods Healthy and mild asthmatic volunteers underwent sputum induction. Manually selected mucus “plug” material was treated with dithiothrietol, filtered and total leukocytes acquired. Multicolor flow cytometry was performed using specific gating strategies based on light scatter properties, differential expression of CD45 and cell lineage markers to discriminate leukocytes from squamous epithelial cells and debris. Results The combination of forward scatter and CD45 expression reliably segregated sputum leukocytes from contaminating squamous epithelial cells and debris. Overlap of major leukocyte populations (neutrophils, macrophages/monocytes) required the use of specific antibodies (e.g. CD16, CD64, CD14, HLA-DR) that differentiated granulocytes from monocytes and macrophages. These gating strategies allowed identification of small populations of eosinophils, CD11c+ myeloid dendritic cells, B cells and NK cells. Conclusions Multicolor flow cytometry can be successfully applied to sputum samples to identify and characterize leukocyte populations residing on the surfaces of the central airways. PMID:21639708

RT DDA: A hybrid method for predicting the scattering properties by densely packed media

NASA Astrophysics Data System (ADS)

Ramezan Pour, B.; Mackowski, D.

2017-12-01

The most accurate approaches to predicting the scattering properties of particulate media are based on exact solutions of the Maxwell's equations (MEs), such as the T-matrix and discrete dipole methods. Applying these techniques for optically thick targets is challenging problem due to the large-scale computations and are usually substituted by phenomenological radiative transfer (RT) methods. On the other hand, the RT technique is of questionable validity in media with large particle packing densities. In recent works, we used numerically exact ME solvers to examine the effects of particle concentration on the polarized reflection properties of plane parallel random media. The simulations were performed for plane parallel layers of wavelength-sized spherical particles, and results were compared with RT predictions. We have shown that RTE results monotonically converge to the exact solution as the particle volume fraction becomes smaller and one can observe a nearly perfect fit for packing densities of 2%-5%. This study describes the hybrid technique composed of exact and numerical scalar RT methods. The exact methodology in this work is the plane parallel discrete dipole approximation whereas the numerical method is based on the adding and doubling method. This approach not only decreases the computational time owing to the RT method but also includes the interference and multiple scattering effects, so it may be applicable to large particle density conditions.

Thermodynamic properties of superfluid helium-3 and measurements of the specific heat of helium-3 in confined geometries as a probe for effects of impurity scattering

NASA Astrophysics Data System (ADS)

Choi, Hyoungsoon

Since its emergence, the Ginzburg-Landau theory has had a tremendous success in describing thermodynamic properties of superconductivity. In the case of superfluid 3He, not all five fourth-order parameters in the theory are known. Only four combinations of the five parameters have been experimentally established and theoretical attempts to calculate the parameters have had limited success as well. We present in this thesis a method to identify the five parameters independent of one another through a close inspection of the experiments and the theoretical calculation of Sauls and Serene. In an attempt to extend our understanding of the thermodynamic properties of 3He, we have also measured the specific heat of superfluid 3He. The measurements were performed on 3He confined in a high porosity silica aerogel and they served as a probe for the effects of impurity scattering. 3He in aerogel clearly shows behavior different from that of pure 3He: including suppression of the transition temperature and the order parameter. We have also looked at 3He in silver sinter. The difference in structures between the silver sinter and the aerogel are manifested in differences in the specific heat. In both cases, however, the impurity scattering creates Andreev bound states and we present evidence for them with our measurements.

Universal dimer–dimer scattering in lattice effective field theory

DOE Office of Scientific and Technical Information (OSTI.GOV)

Elhatisari, Serdar; Katterjohn, Kris; Lee, Dean

We consider two-component fermions with short-range interactions and large scattering length. This system has universal properties that are realized in several different fields of physics. In the limit of large fermion–fermion scattering length a ff and zero-range interaction, all properties of the system scale proportionally with a ff. For the case with shallow bound dimers, we calculate the dimer–dimer scattering phase shifts using lattice effective field theory. We extract the universal dimer–dimer scattering length a dd/a ff=0.618(30) and effective range r dd/a ff=-0.431(48). This result for the effective range is the first calculation with quantified and controlled systematic errors. Wemore » also benchmark our methods by computing the fermion–dimer scattering parameters and testing some predictions of conformal scaling of irrelevant operators near the unitarity limit.« less

Solar system applications of Mie theory and of radiative transfer of polarized light

NASA Technical Reports Server (NTRS)

Whitehill, L. P.

1972-01-01

A theory of the multiple scattering of polarized light is discussed using the doubling method of van de Hulst. The concept of the Stokes parameters is derived and used to develop the form of the scattering phase matrix of a single particle. The diffuse reflection and transmission matrices of a single scattering plane parallel atmosphere are expressed as a function of the phase matrix, and the symmetry properties of these matrices are examined. Four matrices are required to describe scattering and transmission. The scattering matrix that results from the addition of two identical layers is derived. Using the doubling method, the scattering and transmission matrices of layers of arbitrary optical thickness can be derived. The doubling equations are then rewritten in terms of their Fourier components. Computation time is reduced since each Fourier component doubles independently. Computation time is also reduced through the use of symmetry properties.

Universal dimer–dimer scattering in lattice effective field theory

DOE PAGES

Elhatisari, Serdar; Katterjohn, Kris; Lee, Dean; ...

2017-03-14

We consider two-component fermions with short-range interactions and large scattering length. This system has universal properties that are realized in several different fields of physics. In the limit of large fermion–fermion scattering length a ff and zero-range interaction, all properties of the system scale proportionally with a ff. For the case with shallow bound dimers, we calculate the dimer–dimer scattering phase shifts using lattice effective field theory. We extract the universal dimer–dimer scattering length a dd/a ff=0.618(30) and effective range r dd/a ff=-0.431(48). This result for the effective range is the first calculation with quantified and controlled systematic errors. Wemore » also benchmark our methods by computing the fermion–dimer scattering parameters and testing some predictions of conformal scaling of irrelevant operators near the unitarity limit.« less

Light Scattering by Gaussian Particles: A Solution with Finite-Difference Time Domain Technique

NASA Technical Reports Server (NTRS)

Sun, W.; Nousiainen, T.; Fu, Q.; Loeb, N. G.; Videen, G.; Muinonen, K.

2003-01-01

The understanding of single-scattering properties of complex ice crystals has significance in atmospheric radiative transfer and remote-sensing applications. In this work, light scattering by irregularly shaped Gaussian ice crystals is studied with the finite-difference time-domain (FDTD) technique. For given sample particle shapes and size parameters in the resonance region, the scattering phase matrices and asymmetry factors are calculated. It is found that the deformation of the particle surface can significantly smooth the scattering phase functions and slightly reduce the asymmetry factors. The polarization properties of irregular ice crystals are also significantly different from those of spherical cloud particles. These FDTD results could provide a reference for approximate light-scattering models developed for irregular particle shapes and can have potential applications in developing a much simpler practical light scattering model for ice clouds angular-distribution models and for remote sensing of ice clouds and aerosols using polarized light. (copyright) 2003 Elsevier Science Ltd. All rights reserved.

Light scattering properties of kidney epithelial cells and nuclei

NASA Astrophysics Data System (ADS)

Vitol, Elina A.; Kurzweg, Timothy P.; Nabet, Bahram

2006-02-01

Enlargement of mammalian cells nuclei due to the cancerous inflammation can be detected early through noninvasive optical techniques. We report on the results of cellular experiments, aimed towards the development of a fiber optic endoscopic probe used for precancerous detection of Barrett's esophagus. We previously presented white light scattering results from tissue phantoms (polystyrene polybead microspheres). In this paper, we discuss light scattering properties of epithelial MDCK (Madine-Darby Canine Kidney) cells and cell nuclei suspensions. A bifurcated optical fiber is used for experimental illumination and signal detection. The resulting scattering spectra from the cells do not exhibit the predicted Mie theory oscillatory behavior inherent to ideally spherical scatterers, such as polystyrene microspheres. However, we are able to demonstrate that the Fourier transform spectra of the cell suspensions are well correlated with the Fourier transform spectra of cell nuclei, concluding that the dominate scatterer in the backscattering region is the nucleus. This correlation experimentally illustrates that in the backscattering region, the cell nuclei are the main scatterer in the cells of the incident light.

Impact of wavefront distortion and scattering on 2-photon microscopy in mammalian brain tissue

PubMed Central

Chaigneau, Emmanuelle; Wright, Amanda J.; Poland, Simon P.; Girkin, John M.; Silver, R. Angus

2011-01-01

Two-photon (2P) microscopy is widely used in neuroscience, but the optical properties of brain tissue are poorly understood. We have investigated the effect of brain tissue on the 2P point spread function (PSF2P) by imaging fluorescent beads through living cortical slices. By combining this with measurements of the mean free path of the excitation light, adaptive optics and vector-based modeling that includes phase modulation and scattering, we show that tissue-induced wavefront distortions are the main determinant of enlargement and distortion of the PSF2P at intermediate imaging depths. Furthermore, they generate surrounding lobes that contain more than half of the 2P excitation. These effects reduce the resolution of fine structures and contrast and they, together with scattering, limit 2P excitation. Our results disentangle the contributions of scattering and wavefront distortion in shaping the cortical PSF2P, thereby providing a basis for improved 2P microscopy. PMID:22109156

Scatter from optical components; Proceedings of the Meeting, San Diego, CA, Aug. 8-10, 1989

NASA Astrophysics Data System (ADS)

Stover, John C.

Various papers on scatter from optical components are presented. Individual topics addressed include: BRDF of SiC and Al foam compared to black paint at 3.39 microns, characterization of optical baffle materials, bidirectional transmittance distribution function of several IR materials at 3.39 microns, thermal cycling effects on the BRDF of beryllium mirrors, BTDV of ZnSe with multilayer coatings at 3.39 microns, scattering from contaminated surfaces, cleanliness correlation by BRDF and PFO instruments, contamination effects on optical surfaces, means of eliminating the effects of particulate contamination on scatter measurements of superfine optical surfaces, vacuum BRDF measurement of cryogenic optical surfaces, Monte Carlo simulation of contaminant transport to and deposition on complex spacecraft surfaces, surface particle observation and BRDF predictions, satellite material contaminant optical properties, dark field photographic techniques for documenting optical surface contamination, design of a laboratory study of contaminant film darkening in space, contamination monitoring approaches for EUV space optics.

Quasielastic small-angle neutron scattering from heavy water solutions of cyclodextrins

NASA Astrophysics Data System (ADS)

Kusmin, André; Lechner, Ruep E.; Saenger, Wolfram

2011-01-01

We present a model for quasielastic neutron scattering (QENS) by an aqueous solution of compact and inflexible molecules. This model accounts for time-dependent spatial pair correlations between the atoms of the same as well as of distinct molecules and includes all coherent and incoherent neutron scattering contributions. The extension of the static theory of the excluded volume effect [A. K. Soper, J. Phys.: Condens. Matter 9, 2399 (1997)] to the time-dependent (dynamic) case allows us to obtain simplified model expressions for QENS spectra in the low Q region in the uniform fluid approximation. The resulting expressions describe the quasielastic small-angle neutron scattering (QESANS) spectra of D _2O solutions of native and methylated cyclodextrins well, yielding in particular translational and rotational diffusion coefficients of these compounds in aqueous solution. Finally, we discuss the full potential of the QESANS analysis (that is, beyond the uniform fluid approximation), in particular, the information on solute-solvent interactions (e.g., hydration shell properties) that such an analysis can provide, in principle.

Quantum Monte Carlo methods for nuclear physics

DOE PAGES

Carlson, J.; Gandolfi, S.; Pederiva, F.; ...

2015-09-09

Quantum Monte Carlo methods have proved valuable to study the structure and reactions of light nuclei and nucleonic matter starting from realistic nuclear interactions and currents. These ab-initio calculations reproduce many low-lying states, moments, and transitions in light nuclei, and simultaneously predict many properties of light nuclei and neutron matter over a rather wide range of energy and momenta. The nuclear interactions and currents are reviewed along with a description of the continuum quantum Monte Carlo methods used in nuclear physics. These methods are similar to those used in condensed matter and electronic structure but naturally include spin-isospin, tensor, spin-orbit,more » and three-body interactions. A variety of results are presented, including the low-lying spectra of light nuclei, nuclear form factors, and transition matrix elements. Low-energy scattering techniques, studies of the electroweak response of nuclei relevant in electron and neutrino scattering, and the properties of dense nucleonic matter as found in neutron stars are also described. Furthermore, a coherent picture of nuclear structure and dynamics emerges based upon rather simple but realistic interactions and currents.« less

Quantum Monte Carlo methods for nuclear physics

DOE PAGES

Carlson, Joseph A.; Gandolfi, Stefano; Pederiva, Francesco; ...

2014-10-19

Quantum Monte Carlo methods have proved very valuable to study the structure and reactions of light nuclei and nucleonic matter starting from realistic nuclear interactions and currents. These ab-initio calculations reproduce many low-lying states, moments and transitions in light nuclei, and simultaneously predict many properties of light nuclei and neutron matter over a rather wide range of energy and momenta. We review the nuclear interactions and currents, and describe the continuum Quantum Monte Carlo methods used in nuclear physics. These methods are similar to those used in condensed matter and electronic structure but naturally include spin-isospin, tensor, spin-orbit, and three-bodymore » interactions. We present a variety of results including the low-lying spectra of light nuclei, nuclear form factors, and transition matrix elements. We also describe low-energy scattering techniques, studies of the electroweak response of nuclei relevant in electron and neutrino scattering, and the properties of dense nucleonic matter as found in neutron stars. A coherent picture of nuclear structure and dynamics emerges based upon rather simple but realistic interactions and currents.« less

Effective Albedo of Vegetated Terrain at L-Band

NASA Technical Reports Server (NTRS)

Kurum, Mehmet; O'Neill, Peggy E.; Lang, Roger H.

2011-01-01

This paper derives an explicit expression for an effective albedo of vegetated terrain from the zero- and multiple- order radiative transfer (RT) model comparison. The formulation establishes a direct physical link between the effective vegetation parameterization and the theoretical description of absorption and scattering within the canopy. The paper will present an evaluation of the derived albedo for corn canopies with data taken during an experiment at Alabama A&M Winfield A. Thomas Agricultural Research Station near Huntsville, Alabama in June, 1998. The test site consisted of two 50-m x 60-m plots - one with a bare surface and the other with grass cover - and four 30-m x 50-m plots of corn at different planting densities. One corn field was planted at a full density of 9.5 plants/sq m while the others were planted at 1/3, 1/2 and 2/3 of the full density. The fields were observed with a truck-mounted L-band radiometer at incident angle of 15 degree for the period of two weeks. Soil moisture (SM) changed daily due to irrigation and natural rainfall. Variations in gravimetric SM from 18 % to 34 % were seen during this period. Ground truth data, including careful characterization of the corn size and orientation statistics, and its dielectric, was also collected and used to simulate the effective albedo for the vegetation. The single-scattering albedo is defined as the fractional power scattered from individual vegetation constituents with respect to canopy extinction. It represents single-scattering properties of vegetation elements only, and is independent of ground properties. The values of the albedo get higher when there is dense vegetation (i.e. forest, mature corn, etc.) with scatterers, such as branches and trunks (or stalks in the case of corn), which are large with respect to the wavelength. This large albedo leads to a reduction in brightness temperature in the zero-order RT solution (known as tau-omega model). Higher-order multiple-scattering RT solutions are required for proper representation of scattering within vegetation. In this paper, an expression for an effective albedo for the whole canopy including the ground is derived for use in the zero-order RT model-based SM retrieval. This effective albedo takes into account of all the processes taking place within the canopy, including multiple-scattering. This new formulation will be presented and its importance for microwave SM retrieval will be evaluated for corn canopies in conjunction with the detailed ground truth data obtained during the experiment at Alabama in 1998. Emphasis will be placed on examining how the radiometer response to SM is modified by the corn canopy scattering under different field conditions. A semi-empirical parameterization of the effective albedo will be investigated through analysis of SM and vegetation water content effects on the effective albedo.

Application of CaCO3, CaF2, SiO2, and TiO2 particles to silicone lens for enhancing angular color uniformity of white LED lamp

NASA Astrophysics Data System (ADS)

Nguyen, Anh Q. D.; Nguyen, Vinh H.

2017-08-01

In this study, we present an insightful investigation on optimal selection of scattering enhancement particles (SEP) to satisfy each specific optical property of white LEDs (WLEDs). The interested contenders include CaCO3, CaF2, SiO2, and TiO2, each of them is added with YAG:Ce phosphor compounding. The quality improvement on each considered property is demonstrated convincingly by applying Mie-scattering theory together with Monte Carlo simulation on a particular WLEDs which has the color temperature of 8500K. It is observed by simulation results that TiO2 particles provide the highest color uniformity among the SEP, as increasing TiO2 concentration. These results of this work can serve as a practical guideline for manufacturing high-quality WLEDs.

Analyzing asteroid reflectance spectra with numerical tools based on scattering simulations

NASA Astrophysics Data System (ADS)

Penttilä, Antti; Väisänen, Timo; Markkanen, Johannes; Martikainen, Julia; Gritsevich, Maria; Muinonen, Karri

2017-04-01

We are developing a set of numerical tools that can be used in analyzing the reflectance spectra of granular materials such as the regolith surface of atmosphereless Solar system objects. Our goal is to be able to explain, with realistic numerical scattering models, the spectral features arising when materials are intimately mixed together. We include the space-weathering -type effects in our simulations, i.e., mixing host mineral locally with small inclusions of another material in small proportions. Our motivation for this study comes from the present lack of such tools. The current common practice is to apply a semi-physical approximate model such as some variation of Hapke models [e.g., 1] or the Shkuratov model [2]. These models are expressed in a closed form so that they are relatively fast to apply. They are based on simplifications on the radiative transfer theory. The problem is that the validity of the model is not always guaranteed, and the derived physical properties related to particle scattering properties can be unrealistic [3]. We base our numerical tool into a chain of scattering simulations. Scattering properties of small inclusions inside an absorbing host matrix can be derived using exact methods solving the Maxwell equations of the system. The next step, scattering by a single regolith grain, is solved using a geometrical optics method accounting for surface reflections, internal absorption, and possibly the internal diffuse scattering. The third step involves the radiative transfer simulations of these regolith grains in a macroscopic planar element. The chain can be continued next with shadowing simulation over the target surface elements, and finally by integrating the bidirectional reflectance distribution function over the object's shape. Most of the tools in the proposed chain already exist, and one practical task for us is to tie these together into an easy-to-use toolchain that can be publicly distributed. We plan to open the abovementioned toolchain as a web-based open service. Acknowledgments: The research is funded by the ERC Advanced Grant No. 320773 (SAEMPL) References: [1] B. Hapke, Icarus 195, 918-926, 2008. [2] Yu. Shkuratov et al, Icarus 137, 235-246, 1999. [3] Yu. Shkuratov et al, JQSRT 113, 2431-2456, 2012. [4] K. Muinonen et al, JQSRT 110, 1628-1639, 2009.

Self-association of analgesics in aqueous solution: micellar properties of dextropropoxyphene hydrochloride and methadone hydrochloride.

PubMed

Attwood, D; Tolley, J A

1980-08-01

The solution properties of several analgesics including dextropropoxyphene hydrochloride, methadone hydrochloride, dextromoramide acid tartrate and dipipanone hydrochloride have been examined using light scattering, conductivity, vapour pressure osmometry and surface tension techniques. A micellar pattern of association was established for dextropropoxyphene hydrochloride and methadone hydrochloride and critical micelle concentrations and aggregation numbers are reported. The hydrophobic contribution to the free energy of micellization of dextropropoxyphene was determined from measurement of the critical micelle concentration in the presence of added electrolyte.

Aerosol physical properties in the stratosphere (APPS) radiometer design

NASA Technical Reports Server (NTRS)

Gray, C. R.; Woodin, E. A.; Anderson, T. J.; Magee, R. J.; Karthas, G. W.

1977-01-01

The measurement concepts and radiometer design developed to obtain earth-limb spectral radiance measurements for the Aerosol Physical Properties in the Stratosphere (APPS) measurement program are presented. The measurements made by a radiometer of this design can be inverted to yield vertical profiles of Rayleigh scatterers, ozone, nitrogen dioxide, aerosol extinction, and aerosol physical properties, including a Junge size-distribution parameter, and a real and imaginary index of refraction. The radiometer design provides the capacity for remote sensing of stratospheric constituents from space on platforms such as the space shuttle and satellites, and therefore provides for global measurements on a daily basis.

Integrated ray tracing simulation of annual variation of spectral bio-signatures from cloud free 3D optical Earth model

NASA Astrophysics Data System (ADS)

Ryu, Dongok; Kim, Sug-Whan; Kim, Dae Wook; Lee, Jae-Min; Lee, Hanshin; Park, Won Hyun; Seong, Sehyun; Ham, Sun-Jeong

2010-09-01

Understanding the Earth spectral bio-signatures provides an important reference datum for accurate de-convolution of collapsed spectral signals from potential earth-like planets of other star systems. This study presents a new ray tracing computation method including an improved 3D optical earth model constructed with the coastal line and vegetation distribution data from the Global Ecological Zone (GEZ) map. Using non-Lambertian bidirectional scattering distribution function (BSDF) models, the input earth surface model is characterized with three different scattering properties and their annual variations depending on monthly changes in vegetation distribution, sea ice coverage and illumination angle. The input atmosphere model consists of one layer with Rayleigh scattering model from the sea level to 100 km in altitude and its radiative transfer characteristics is computed for four seasons using the SMART codes. The ocean scattering model is a combination of sun-glint scattering and Lambertian scattering models. The land surface scattering is defined with the semi empirical parametric kernel method used for MODIS and POLDER missions. These three component models were integrated into the final Earth model that was then incorporated into the in-house built integrated ray tracing (IRT) model capable of computing both spectral imaging and radiative transfer performance of a hypothetical space instrument as it observes the Earth from its designated orbit. The IRT model simulation inputs include variation in earth orientation, illuminated phases, and seasonal sea ice and vegetation distribution. The trial simulation runs result in the annual variations in phase dependent disk averaged spectra (DAS) and its associated bio-signatures such as NDVI. The full computational details are presented together with the resulting annual variation in DAS and its associated bio-signatures.

Inverse Scattering and Local Observable Algebras in Integrable Quantum Field Theories

NASA Astrophysics Data System (ADS)

Alazzawi, Sabina; Lechner, Gandalf

2017-09-01

We present a solution method for the inverse scattering problem for integrable two-dimensional relativistic quantum field theories, specified in terms of a given massive single particle spectrum and a factorizing S-matrix. An arbitrary number of massive particles transforming under an arbitrary compact global gauge group is allowed, thereby generalizing previous constructions of scalar theories. The two-particle S-matrix S is assumed to be an analytic solution of the Yang-Baxter equation with standard properties, including unitarity, TCP invariance, and crossing symmetry. Using methods from operator algebras and complex analysis, we identify sufficient criteria on S that imply the solution of the inverse scattering problem. These conditions are shown to be satisfied in particular by so-called diagonal S-matrices, but presumably also in other cases such as the O( N)-invariant nonlinear {σ}-models.

Asymptotic neutron scattering laws for anomalously diffusing quantum particles

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kneller, Gerald R.; Université d’Orléans, Chateau de la Source-Ave. du Parc Floral, 45067 Orléans; Synchrotron-SOLEIL, L’Orme de Merisiers, 91192 Gif-sur-Yvette

2016-07-28

The paper deals with a model-free approach to the analysis of quasielastic neutron scattering intensities from anomalously diffusing quantum particles. All quantities are inferred from the asymptotic form of their time-dependent mean square displacements which grow ∝t{sup α}, with 0 ≤ α < 2. Confined diffusion (α = 0) is here explicitly included. We discuss in particular the intermediate scattering function for long times and the Fourier spectrum of the velocity autocorrelation function for small frequencies. Quantum effects enter in both cases through the general symmetry properties of quantum time correlation functions. It is shown that the fractional diffusion constantmore » can be expressed by a Green-Kubo type relation involving the real part of the velocity autocorrelation function. The theory is exact in the diffusive regime and at moderate momentum transfers.« less

Phantom Preparation and Optical Property Determination

NASA Astrophysics Data System (ADS)

He, Di; He, Jie; Mao, Heng

2018-12-01

Tissue-like optical phantoms are important in testing new imaging algorithms. Homogeneous optical phantoms with determined optical properties are the first step of making a proper heterogeneous phantom for multi-modality imaging. Typical recipes for such phantoms consist of epoxy resin, hardener, India ink and titanium oxide. By altering the concentration of India ink and titanium oxide, we are able to get multiple homogeneous phantoms with different absorption and scattering coefficients by carefully mixing all the ingredients. After fabricating the phantoms, we need to find their individual optical properties including the absorption and scattering coefficients. This is achieved by solving diffusion equation of each phantom as a homogeneous slab under canonical illumination. We solve the diffusion equation of homogeneous slab in frequency domain and get the formula for theoretical measurements. Under our steady-state diffused optical tomography (DOT) imaging system, we are able to obtain the real distribution of the incident light produced by a laser. With this source distribution we got and the formula we derived, numerical experiments show how measurements change while varying the value of absorption and scattering coefficients. Then we notice that the measurements alone will not be enough for us to get unique optical properties for steady-state DOT problem. Thus in order to determine the optical properties of a homogeneous slab we want to fix one of the coefficients first and use optimization methods to find another one. Then by assemble multiple homogeneous slab phantoms with different optical properties, we are able to obtain a heterogeneous phantom suitable for testing multi-modality imaging algorithms. In this paper, we describe how to make phantoms, derive a formula to solve the diffusion equation, demonstrate the non-uniqueness of steady-state DOT problem by analysing some numerical results of our formula, and finally propose a possible way to determine optical properties for homogeneous slab for our future work.

Influence of Ice Particle Surface Roughening on the Global Cloud Radiative Effect

NASA Technical Reports Server (NTRS)

Yi, Bingqi; Yang, Ping; Baum, Bryan A.; LEcuyer, Tristan; Oreopoulos, Lazaros; Mlawer, Eli J.; Heymsfield, Andrew J.; Liou, Kuo-Nan

2013-01-01

Ice clouds influence the climate system by changing the radiation budget and large-scale circulation. Therefore, climate models need to have an accurate representation of ice clouds and their radiative effects. In this paper, new broadband parameterizations for ice cloud bulk scattering properties are developed for severely roughened ice particles. The parameterizations are based on a general habit mixture that includes nine habits (droxtals, hollow/solid columns, plates, solid/hollow bullet rosettes, aggregate of solid columns, and small/large aggregates of plates). The scattering properties for these individual habits incorporate recent advances in light-scattering computations. The influence of ice particle surface roughness on the ice cloud radiative effect is determined through simulations with the Fu-Liou and the GCM version of the Rapid Radiative Transfer Model (RRTMG) codes and the National Center for Atmospheric Research Community Atmosphere Model (CAM, version 5.1). The differences in shortwave (SW) and longwave (LW) radiative effect at both the top of the atmosphere and the surface are determined for smooth and severely roughened ice particles. While the influence of particle roughening on the single-scattering properties is negligible in the LW, the results indicate that ice crystal roughness can change the SW forcing locally by more than 10 W m(exp -2) over a range of effective diameters. The global-averaged SW cloud radiative effect due to ice particle surface roughness is estimated to be roughly 1-2 W m(exp -2). The CAM results indicate that ice particle roughening can result in a large regional SW radiative effect and a small but nonnegligible increase in the global LW cloud radiative effect.

Millimeter wave propagation modeling of inhomogeneous rain media for satellite communications systems

NASA Technical Reports Server (NTRS)

Persinger, R. R.; Stutzman, W. L.

1978-01-01

A theoretical propagation model that represents the scattering properties of an inhomogeneous rain often found on a satellite communications link is presented. The model includes the scattering effects of an arbitrary distribution of particle type (rain or ice), particle shape, particle size, and particle orientation within a given rain cell. An associated rain propagation prediction program predicts attenuation, isolation and phase shift as a function of ground rain rate. A frequency independent synthetic storm algorithm is presented that models nonuniform rain rates present on a satellite link. Antenna effects are included along with a discussion of rain reciprocity. The model is verified using the latest available multiple frequency data from the CTS and COMSTAR satellites. The data covers a wide range of frequencies, elevation angles, and ground site locations.

Three-dimensional surface profile intensity correction for spatially modulated imaging

NASA Astrophysics Data System (ADS)

Gioux, Sylvain; Mazhar, Amaan; Cuccia, David J.; Durkin, Anthony J.; Tromberg, Bruce J.; Frangioni, John V.

2009-05-01

We describe a noncontact profile correction technique for quantitative, wide-field optical measurement of tissue absorption (μa) and reduced scattering (μs') coefficients, based on geometric correction of the sample's Lambertian (diffuse) reflectance intensity. Because the projection of structured light onto an object is the basis for both phase-shifting profilometry and modulated imaging, we were able to develop a single instrument capable of performing both techniques. In so doing, the surface of the three-dimensional object could be acquired and used to extract the object's optical properties. The optical properties of flat polydimethylsiloxane (silicone) phantoms with homogenous tissue-like optical properties were extracted, with and without profilometry correction, after vertical translation and tilting of the phantoms at various angles. Objects having a complex shape, including a hemispheric silicone phantom and human fingers, were acquired and similarly processed, with vascular constriction of a finger being readily detectable through changes in its optical properties. Using profilometry correction, the accuracy of extracted absorption and reduced scattering coefficients improved from two- to ten-fold for surfaces having height variations as much as 3 cm and tilt angles as high as 40 deg. These data lay the foundation for employing structured light for quantitative imaging during surgery.

Size effect on thermoelectric properties of Bi2Te3 nanoparticles

NASA Astrophysics Data System (ADS)

Choudhary, K. K.; Sharma, Uttam; Lodhi, Pavitra Devi; Kaurav, Netram

2018-05-01

Bi2Te3 nanoparticles exhibit size dependent thermoelectric properties which gives an opportunity to tune the size for optimization of the thermoelectric figure of merit (ZT). We have quantitatively analyzed the thermoelectric properties of Bi2Te3 using phonon scattering mechanism by incorporating the scattering of phonons with defects, grain boundaries, electrons and Umklapp phonon scatterings. The maximum value of ZT = 0.92 is obtained at T = 400 K for 30 nm Bi2Te3 nanoparticles in comparison to ZT = 0.45 for 150 nm nanoparticles at the same temperature. With decrease in size of nanoparticles interface volume ratio increases which increase the phonon scatterings with grain boundaries and point defects, results in decrease in thermal conductivity due to reduction in mean free path of phonons. As a result of decrease in thermal conductivity (κ), Seeback coefficient (S) and ZT increases.

Application of symmetry properties to polarimetric remote sensing with JPL AIRSAR data

NASA Technical Reports Server (NTRS)

Nghiem, S. V.; Yueh, Simon H.; Kwok, R.; Li, F. K.

1992-01-01

Based on symmetry properties, polarimetric remote sensing of geophysical media is studied. From the viewpoint of symmetry groups, media with reflection, rotation, azimuthal, and centrical symmetries are considered. The symmetries impose relations among polarimetric scattering coefficients, which are valid to all scattering mechanisms in the symmetrical configurations. Various orientation distributions of non-spherical scatterers can be identified from the scattering coefficients by a comparison with the symmetry calculations. Experimental observations are then analyzed for many geophysical scenes acquired with the Jet Propulsion Laboratory (JPL) airborne polarimetric SAR at microwave frequencies over sea ice and vegetation. Polarimetric characteristics of different ice types are compared with symmetry behaviors. The polarimetric response of a tropical rain forest reveals characteristics close to the centrical symmetry properties, which can be used as a distributed target to relatively calibrate polarimetric radars without any deployment of manmade calibration targets.

Optical Properties of Ice Particles in Young Contrails

NASA Technical Reports Server (NTRS)

Hong, Gang; Feng, Qian; Yang, Ping; Kattawar, George; Minnis, Patrick; Hu, Yong X.

2008-01-01

The single-scattering properties of four types of ice crystals (pure ice crystals, ice crystals with an internal mixture of ice and black carbon, ice crystals coated with black carbon, and soot coated with ice) in young contrails are investigated at wavelengths 0.65 and 2.13 micrometers using Mie codes from coated spheres. The four types of ice crystals have distinct differences in their single-scattering properties because of the embedded black carbon. The bulk scattering properties of young contrails consisting of the four types of ice crystals are further investigated by averaging their single-scattering properties over a typical ice particle size distribution found in young contrails. The effect of the radiative properties of the four types of ice particles on the Stokes parameters I, Q, U, and V is also investigated for different viewing zenith angles and relative azimuth angles with a solar zenith angle of 30 degrees using a vector radiative transfer model based on the adding-doubling technique. The Stokes parameters at a wavelength of 0.65 micrometers show pronounced differences for the four types of ice crystals. Those at a wavelength of 2.13 micrometers show similar variations with the viewing zenith angle and relative azimuth angle, but their values are noticeably different.

Investigation on the properties of the formation and coherence of intense fringe near nonlinear medium slab

NASA Astrophysics Data System (ADS)

Hu, Yonghua; Qiu, Yaqiong; Li, Yang; Shi, Lin

2018-03-01

Near medium intense (NMI) fringe is a kind of intense fringe which can be formed near Kerr medium in high-power laser beam propagation. The formation properties of NMI fringe and the relations between NMI fringe and related important parameters are systematically investigated. It is found that it is the co-existence of two wirelike phase-typed scatterers in the incident beam spot which is mainly responsible for the high intensity of NMI fringe. From the viewpoint of coherent superposition, the formation process of NMI fringe is analyzed, and the mechanism that NMI fringe is formed by the coherent superposition of the localized bright fringes in the exit field of Kerr medium slab is demonstrated. The fluctuations of NMI fringe properties with beam wavelength, scatterer spacing and object distance are studied, the coherence of NMI fringe are revealed, and the approximate periodicity of the appearance of remarkable NMI fringe for these parameters are obtained. Especially, it is found that the intensity of NMI fringe is very sensitive to scatterer spacing. Besides, the laws about how NMI fringe properties will be changed by the modulation properties of scatterers and the medium thickness are demonstrated.

Performance of a lookup table-based approach for measuring tissue optical properties with diffuse optical spectroscopy

NASA Astrophysics Data System (ADS)

Nichols, Brandon S.; Rajaram, Narasimhan; Tunnell, James W.

2012-05-01

Diffuse optical spectroscopy (DOS) provides a powerful tool for fast and noninvasive disease diagnosis. The ability to leverage DOS to accurately quantify tissue optical parameters hinges on the model used to estimate light-tissue interaction. We describe the accuracy of a lookup table (LUT)-based inverse model for measuring optical properties under different conditions relevant to biological tissue. The LUT is a matrix of reflectance values acquired experimentally from calibration standards of varying scattering and absorption properties. Because it is based on experimental values, the LUT inherently accounts for system response and probe geometry. We tested our approach in tissue phantoms containing multiple absorbers, different sizes of scatterers, and varying oxygen saturation of hemoglobin. The LUT-based model was able to extract scattering and absorption properties under most conditions with errors of less than 5 percent. We demonstrate the validity of the lookup table over a range of source-detector separations from 0.25 to 1.48 mm. Finally, we describe the rapid fabrication of a lookup table using only six calibration standards. This optimized LUT was able to extract scattering and absorption properties with average RMS errors of 2.5 and 4 percent, respectively.

Modeling Optical Properties of Mineral Aerosol Particles by Using Nonsymmetric Hexahedra

NASA Technical Reports Server (NTRS)

Bi, Lei; Yang, Ping; Kattawar, George W.; Kahn, Ralph

2010-01-01

We explore the use of nonsymmetric geometries to simulate the single-scattering properties of airborne dust particles with complicated morphologies. Specifically, the shapes of irregular dust particles are assumed to be nonsymmetric hexahedra defined by using the Monte Carlo method. A combination of the discrete dipole approximation method and an improved geometric optics method is employed to compute the single-scattering properties of dust particles for size parameters ranging from 0.5 to 3000. The primary optical effect of eliminating the geometric symmetry of regular hexahedra is to smooth the scattering features in the phase function and to decrease the backscatter. The optical properties of the nonsymmetric hexahedra are used to mimic the laboratory measurements. It is demonstrated that a relatively close agreement can be achieved by using only one shape of nonsymmetric hexahedra. The agreement between the theoretical results and their measurement counterparts can be further improved by using a mixture of nonsymmetric hexahedra. It is also shown that the hexahedron model is much more appropriate than the "equivalent sphere" model for simulating the optical properties of dust particles, particularly, in the case of the elements of the phase matrix that associated with the polarization state of scattered light.

A model study of aggregates composed of spherical soot monomers with an acentric carbon shell

NASA Astrophysics Data System (ADS)

Luo, Jie; Zhang, Yongming; Zhang, Qixing

2018-01-01

Influences of morphology on the optical properties of soot particles have gained increasing attentions. However, studies on the effect of the way primary particles are coated on the optical properties is few. Aimed to understand how the primary particles are coated affect the optical properties of soot particles, the coated soot particle was simulated using the acentric core-shell monomers model (ACM), which was generated by randomly moving the cores of concentric core-shell monomers (CCM) model. Single scattering properties of the CCM model with identical fractal parameters were calculated 50 times at first to evaluate the optical diversities of different realizations of fractal aggregates with identical parameters. The results show that optical diversities of different realizations for fractal aggregates with identical parameters cannot be eliminated by averaging over ten random realizations. To preserve the fractal characteristics, 10 realizations of each model were generated based on the identical 10 parent fractal aggregates, and then the results were averaged over each 10 realizations, respectively. The single scattering properties of all models were calculated using the numerically exact multiple-sphere T-matrix (MSTM) method. It is found that the single scattering properties of randomly coated soot particles calculated using the ACM model are extremely close to those using CCM model and homogeneous aggregate (HA) model using Maxwell-Garnett effective medium theory. Our results are different from previous studies. The reason may be that the differences in previous studies were caused by fractal characteristics but not models. Our findings indicate that how the individual primary particles are coated has little effect on the single scattering properties of soot particles with acentric core-shell monomers. This work provides a suggestion for scattering model simplification and model selection.

Method for accurate quantitation of background tissue optical properties in the presence of emission from a strong fluorescence marker

NASA Astrophysics Data System (ADS)

Bravo, Jaime; Davis, Scott C.; Roberts, David W.; Paulsen, Keith D.; Kanick, Stephen C.

2015-03-01

Quantification of targeted fluorescence markers during neurosurgery has the potential to improve and standardize surgical distinction between normal and cancerous tissues. However, quantitative analysis of marker fluorescence is complicated by tissue background absorption and scattering properties. Correction algorithms that transform raw fluorescence intensity into quantitative units, independent of absorption and scattering, require a paired measurement of localized white light reflectance to provide estimates of the optical properties. This study focuses on the unique problem of developing a spectral analysis algorithm to extract tissue absorption and scattering properties from white light spectra that contain contributions from both elastically scattered photons and fluorescence emission from a strong fluorophore (i.e. fluorescein). A fiber-optic reflectance device was used to perform measurements in a small set of optical phantoms, constructed with Intralipid (1% lipid), whole blood (1% volume fraction) and fluorescein (0.16-10 μg/mL). Results show that the novel spectral analysis algorithm yields accurate estimates of tissue parameters independent of fluorescein concentration, with relative errors of blood volume fraction, blood oxygenation fraction (BOF), and the reduced scattering coefficient (at 521 nm) of <7%, <1%, and <22%, respectively. These data represent a first step towards quantification of fluorescein in tissue in vivo.

Improved scatter correction using adaptive scatter kernel superposition

NASA Astrophysics Data System (ADS)

Sun, M.; Star-Lack, J. M.

2010-11-01

Accurate scatter correction is required to produce high-quality reconstructions of x-ray cone-beam computed tomography (CBCT) scans. This paper describes new scatter kernel superposition (SKS) algorithms for deconvolving scatter from projection data. The algorithms are designed to improve upon the conventional approach whose accuracy is limited by the use of symmetric kernels that characterize the scatter properties of uniform slabs. To model scatter transport in more realistic objects, nonstationary kernels, whose shapes adapt to local thickness variations in the projection data, are proposed. Two methods are introduced: (1) adaptive scatter kernel superposition (ASKS) requiring spatial domain convolutions and (2) fast adaptive scatter kernel superposition (fASKS) where, through a linearity approximation, convolution is efficiently performed in Fourier space. The conventional SKS algorithm, ASKS, and fASKS, were tested with Monte Carlo simulations and with phantom data acquired on a table-top CBCT system matching the Varian On-Board Imager (OBI). All three models accounted for scatter point-spread broadening due to object thickening, object edge effects, detector scatter properties and an anti-scatter grid. Hounsfield unit (HU) errors in reconstructions of a large pelvis phantom with a measured maximum scatter-to-primary ratio over 200% were reduced from -90 ± 58 HU (mean ± standard deviation) with no scatter correction to 53 ± 82 HU with SKS, to 19 ± 25 HU with fASKS and to 13 ± 21 HU with ASKS. HU accuracies and measured contrast were similarly improved in reconstructions of a body-sized elliptical Catphan phantom. The results show that the adaptive SKS methods offer significant advantages over the conventional scatter deconvolution technique.

Characterizing optical properties and spatial heterogeneity of human ovarian tissue using spatial frequency domain imaging

NASA Astrophysics Data System (ADS)

Nandy, Sreyankar; Mostafa, Atahar; Kumavor, Patrick D.; Sanders, Melinda; Brewer, Molly; Zhu, Quing

2016-10-01

A spatial frequency domain imaging (SFDI) system was developed for characterizing ex vivo human ovarian tissue using wide-field absorption and scattering properties and their spatial heterogeneities. Based on the observed differences between absorption and scattering images of different ovarian tissue groups, six parameters were quantitatively extracted. These are the mean absorption and scattering, spatial heterogeneities of both absorption and scattering maps measured by a standard deviation, and a fitting error of a Gaussian model fitted to normalized mean Radon transform of the absorption and scattering maps. A logistic regression model was used for classification of malignant and normal ovarian tissues. A sensitivity of 95%, specificity of 100%, and area under the curve of 0.98 were obtained using six parameters extracted from the SFDI images. The preliminary results demonstrate the diagnostic potential of the SFDI method for quantitative characterization of wide-field optical properties and the spatial distribution heterogeneity of human ovarian tissue. SFDI could be an extremely robust and valuable tool for evaluation of the ovary and detection of neoplastic changes of ovarian cancer.

Structural Significance of Lipid Diversity as Studied by Small Angle Neutron and X-ray Scattering

DOE PAGES

Kučerka, Norbert; Heberle, Frederick A.; Pan, Jianjun; ...

2015-09-21

In this paper, we review recent developments in the rapidly growing field of membrane biophysics, with a focus on the structural properties of single lipid bilayers determined by different scattering techniques, namely neutron and X-ray scattering. The need for accurate lipid structural properties is emphasized by the sometimes conflicting results found in the literature, even in the case of the most studied lipid bilayers. Increasingly, accurate and detailed structural models require more experimental data, such as those from contrast varied neutron scattering and X-ray scattering experiments that are jointly refined with molecular dynamics simulations. This experimental and computational approach producesmore » robust bilayer structural parameters that enable insights, for example, into the interplay between collective membrane properties and its components (e.g., hydrocarbon chain length and unsaturation, and lipid headgroup composition). Finally, from model studies such as these, one is better able to appreciate how a real biological membrane can be tuned by balancing the contributions from the lipid’s different moieties (e.g., acyl chains, headgroups, backbones, etc.).« less

Relating Cirrus Cloud Properties to Observed Fluxes: A Critical Assessment.

NASA Astrophysics Data System (ADS)

Vogelmann, A. M.; Ackerman, T. P.

1995-12-01

The accuracy needed in cirrus cloud scattering and microphysical properties is quantified such that the radiative effect on climate can he determined. Our ability to compute and observe these properties to within needed accuracies is assessed, with the greatest attention given to those properties that most affect the fluxes.Model calculations indicate that computing net longwave fluxes at the surface to within ±5% requires that cloud temperature be known to within as little as ±3 K in cold climates for extinction optical depths greater than two. Such accuracy could be more difficult to obtain than that needed in the values of scattering parameters. For a baseline case (defined in text), computing net shortwave fluxes at the surface to within ±5% requires accuracies in cloud ice water content that, when the optical depth is greater than 1.25, are beyond the accuracies of current measurements. Similarly, surface shortwave flux computations require accuracies in the asymmetry parameter that are beyond our current abilities when the optical depth is greater than four. Unless simplifications are discovered, the scattering properties needed to compute cirrus cloud fluxes cannot be obtained explicitly with existing scattering algorithms because the range of crystal sizes is too great and crystal shapes are too varied to be treated computationally. Thus, bulk cirrus scattering properties might be better obtained by inverting cirrus cloud fluxes and radiances. Finally, typical aircraft broadband flux measurements are not sufficiently accurate to provide a convincing validation of calculations. In light of these findings we recommend a reexamination of the methodology used in field programs such as FIRE and suggest a complementary approach.

Calculation of Transverse-Momentum-Dependent Evolution for Sivers Transverse Single Spin Asymmetry Measurements

NASA Astrophysics Data System (ADS)

Aybat, S. Mert; Prokudin, Alexei; Rogers, Ted C.

2012-06-01

The Sivers transverse single spin asymmetry (TSSA) is calculated and compared at different scales using the transverse-momentum-dependent (TMD) evolution equations applied to previously existing extractions. We apply the Collins-Soper-Sterman (CSS) formalism, using the version recently developed by Collins. Our calculations rely on the universality properties of TMD functions that follow from the TMD-factorization theorem. Accordingly, the nonperturbative input is fixed by earlier experimental measurements, including both polarized semi-inclusive deep inelastic scattering (SIDIS) and unpolarized Drell-Yan (DY) scattering. It is shown that recent preliminary COMPASS measurements are consistent with the suppression prescribed by TMD evolution.

A 'range test' for determining scatterers with unknown physical properties

NASA Astrophysics Data System (ADS)

Potthast, Roland; Sylvester, John; Kusiak, Steven

2003-06-01

We describe a new scheme for determining the convex scattering support of an unknown scatterer when the physical properties of the scatterers are not known. The convex scattering support is a subset of the scatterer and provides information about its location and estimates for its shape. For convex polygonal scatterers the scattering support coincides with the scatterer and we obtain full shape reconstructions. The method will be formulated for the reconstruction of the scatterers from the far field pattern for one or a few incident waves. The method is non-iterative in nature and belongs to the type of recently derived generalized sampling schemes such as the 'no response test' of Luke-Potthast. The range test operates by testing whether it is possible to analytically continue a far field to the exterior of any test domain Omegatest. By intersecting the convex hulls of various test domains we can produce a minimal convex set, the convex scattering support of which must be contained in the convex hull of the support of any scatterer which produces that far field. The convex scattering support is calculated by testing the range of special integral operators for a sampling set of test domains. The numerical results can be used as an approximation for the support of the unknown scatterer. We prove convergence and regularity of the scheme and show numerical examples for sound-soft, sound-hard and medium scatterers. We can apply the range test to non-convex scatterers as well. We can conclude that an Omegatest which passes the range test has a non-empty intersection with the infinity-support (the complement of the unbounded component of the complement of the support) of the true scatterer, but cannot find a minimal set which must be contained therein.

Aerosol Optical Properties at the Lulin Atmospheric Background Station in Taiwan and the Influences of Long-Range Transport of Air Pollutants

NASA Technical Reports Server (NTRS)

Hsiao, Ta-Chih; Chen, Wei-Nai; Ye, Wei-Cheng; Lin, Neng-Huei; Tsay, Si-Chee; Lin, Tang-Huang; Lee, Chung-Te; Chuang, Ming-Tung; Pantina, Peter; Wang, Sheng-Hsiang

2016-01-01

The Lulin Atmospheric Background Station (LABS, 23.47 deg. N 120.87 deg. E, 2862 m ASL) in Central Taiwan was constructed in 2006 and is the only high-altitude background station in the western Pacific region for studying the influence of continental outflow. In this study, extensive optical properties of aerosols, including the aerosol light scattering coefficient [Sigma(sub s)] and light absorption coefficient [Sigma(sub a)], were collected from 2013 to 2014. The intensive optical properties, including mass scattering efficiency [Sigma(sub s)], mass absorption efficiency [Sigma(sub a)] single scattering albedo (Omega), scattering Angstrom exponent (A), and backscattering fraction (b), were determined and investigated, and the distinct seasonal cycle was observed. The value of [Alpha(sub a)] began to increase in January and reached a maximum in April; the mean in spring was 5.89 m(exp. 2) g(exp. -1) with a standard deviation (SD) of 4.54 m(exp. 2) g(exp. -1) and a 4.48 m(exp. 2) g(exp. -1) interquartile range (IQR: 2.95-7.43 m(exp. 2) g(exp. -1). The trend was similar in [Sigma(sub a)], with a maximum in March and a monthly mean of 0.84 m(exp. 2) g(exp. -1). The peak values of Omega (Mean = 0.92, SD = 0.03, IQR: 0.90 - 0.93) and A (Mean = 2.22, SD = 0.61, IQR: 2.12 = 2.47) occurred in autumn. These annual patterns of optical properties were associated with different long-range transport patterns of air pollutants such as biomass burning (BB) aerosol in spring and potential anthropogenic emissions in autumn. The optical measurements performed at LABS during spring in 2013 were compared with those simultaneously performed at the Doi Ang Kang Meteorology Station, Chiang Mai Province, Thailand (DAK, 19.93 deg. N, 99.05 deg. E, 1536 m a.s.l.), which is located in the Southeast Asia BB source region. Furthermore, the relationships among [Sigma(sub s)], [Sigma(sub a)], and (b) were used to characterize the potential aerosol types transported to LABS during different seasons, and the data were inspected according to the HYSPLIT 5-day backward trajectories, which differentiate between different regions of air mass origin.

The applicability of physical optics in the millimetre and sub-millimetre spectral region. Part II: Application to a three-component model of ice cloud and its evaluation against the bulk single-scattering properties of various other aggregate models

NASA Astrophysics Data System (ADS)

Baran, Anthony J.; Ishimoto, Hiroshi; Sourdeval, Odran; Hesse, Evelyn; Harlow, Chawn

2018-02-01

The bulk single-scattering properties of various randomly oriented aggregate ice crystal models are compared and contrasted at a number of frequencies between 89 and 874 GHz. The model ice particles consist of the ten-branched plate aggregate, five-branched plate aggregate, eight-branched hexagonal aggregate, Voronoi ice aggregate, six-branched hollow bullet rosette, hexagonal column of aspect ratio unity, and the ten-branched hexagonal aggregate. The bulk single-scattering properties of the latter two ice particle models have been calculated using the light scattering methods described in Part I, which represent the two most extreme members of an ensemble model of cirrus ice crystals. In Part I, it was shown that the method of physical optics could be combined with the T-matrix at a size parameter of about 18 to compute the bulk integral ice optical properties and the phase function in the microwave to sufficient accuracy to be of practical value. Here, the bulk single-scattering properties predicted by the two ensemble model members and the Voronoi model are shown to generally bound those of all other models at frequencies between 89 and 874 GHz, thus representing a three-component model of ice cloud that can be generally applied to the microwave, rather than using many differing ice particle models. Moreover, the Voronoi model and hollow bullet rosette scatter similarly to each other in the microwave. Furthermore, from the various comparisons, the importance of assumed shapes of the particle size distribution as well as cm-sized ice aggregates is demonstrated.

An investigation of the forward scattering theorem

NASA Technical Reports Server (NTRS)

Karam, M. A.; Fung, A. K.

1987-01-01

The calculation of an EM wave's extinction loss during propagation within an inhomogeneous medium, as in active and passive remote sensing modeling, can be undertaken either through the summation of the scattering and absorption losses or through the use of the forward scattering theorem. Attention is presently given to the similarities and differences of these two approaches as a function of dielectric properties of a spherical scatterer and the incident frequency. Scattering loss is obtainable by integrating the magnitude-squared of the scattered field over a spherical surface surrounding the scatterer; the scattered field and the field within the scatterer are computed according to Mie theory.

Sound scattering by several zooplankton groups. I. Experimental determination of dominant scattering mechanisms.

PubMed

Stanton, T K; Chu, D; Wiebe, P H; Martin, L V; Eastwood, R L

1998-01-01

The acoustic scattering properties of live individual zooplankton from several gross anatomical groups have been investigated. The groups involve (1) euphausiids (Meganyctiphanes norvegica) whose bodies behave acoustically as a fluid material, (2) gastropods (Limacina retroversa) whose bodies include a hard elastic shell, and (3) siphonophores (Agalma okeni or elegans and Nanomia cara) whose bodies contain a gas inclusion (pneumatophore). The animals were collected from ocean waters off New England (Slope Water, Georges Bank, and the Gulf of Maine). The scattering properties were measured over parts or all of the frequency range 50 kHz to 1 MHz in a laboratory-style pulse-echo setup in a large tank at sea using live fresh specimens. Individual echoes as well as averages and ping-to-ping fluctuations of repeated echoes were studied. The material type of each group is shown to strongly affect both the overall echo level and pattern of the target strength versus frequency plots. In this first article of a two-part series, the dominant scattering mechanisms of the three animal types are determined principally by examining the structure of both the frequency spectra of individual broadband echoes and the compressed pulse (time series) output. Other information is also used involving the effect on overall levels due to (1) animal orientation and (2) tissue in animals having a gas inclusion (siphonophores). The results of this first paper show that (1) the euphausiids behave as weakly scattering fluid bodies and there are major contributions from at least two parts of the body to the echo (the number of contributions depends upon angle of orientation and shape), (2) the gastropods produce echoes from the front interface and possibly from a slow-traveling circumferential (Lamb) wave, and (3) the gas inclusion of the siphonophore dominates the echoes, but the tissue plays a role in the scattering and is especially important when analyzing echoes from individual animals on a ping-by-ping basis. The results of this paper serve as the basis for the development of acoustic scattering models in the companion paper [Stanton et al., J. Acoust. Soc. Am. 103, 236-253 (1998)].

Multi-property isotropic intermolecular potentials and predicted spectral lineshapes of collision-induced absorption (CIA), collision-induced light scattering (CILS) and collision-induced hyper-Rayleigh scattering (CIHR) for H2sbnd Ne, -Kr and -Xe

NASA Astrophysics Data System (ADS)

El-Kader, M. S. A.; Godet, J.-L.; Gustafsson, M.; Maroulis, G.

2018-04-01

Quantum mechanical lineshapes of collision-induced absorption (CIA), collision-induced light scattering (CILS) and collision-induced hyper-Rayleigh scattering (CIHR) at room temperature (295 K) are computed for gaseous mixtures of molecular hydrogen with neon, krypton and xenon. The induced spectra are detected using theoretical values for induced dipole moment, pair-polarizability trace and anisotropy, hyper-polarizability and updated intermolecular potentials. Good agreement is observed for all spectra when the literature and the present potentials which are constructed from the transport and thermo-physical properties are used.

A high definition Mueller polarimetric endoscope for tissue characterisation (Conference Presentation)

NASA Astrophysics Data System (ADS)

Qi, Ji; Elson, Daniel

2016-03-01

The mechanism of most medical endoscopes is based on the interaction between light and biological tissue, inclusive of absorption, elastic scattering and fluorescence. In essence, the metrics of those interactions are obtained from the fundamental properties of light as an electro-magnetic waves, namely, the radiation intensity and wavelength. As another fundamental property of light, polarisation can not only reveal tissue scattering and absorption information from a different perspective, but is also able to provide a fresh insight into directional tissue birefringence properties induced by birefringent compositions and anisotropic fibrous structures, such as collagen, elastin, muscle fibre, etc at the same time. Here we demonstrate a low cost high definition Muller polarimetric endoscope with minimal alteration of a rigid endoscope. By imaging birefringent tissue mimicking phantoms and a porcine bladder, we show that this novel endoscopic imaging modality is able to provide different information of interest from unpolarised endoscopic imaging, including linear depolarization, circular depolarization, birefringence, optic axis orientation and dichroism. This endoscope can potentially be employed for better tissue visualisation and benefit endoscopic investigations and intra-operative guidance.

Exact quantum scattering calculation of transport properties for free radicals: OH(X2Π)-helium.

PubMed

Dagdigian, Paul J; Alexander, Millard H

2012-09-07

Transport properties for OH-He are computed through quantum scattering calculations using the ab initio potential energy surfaces determined by Lee et al. [J. Chem. Phys. 113, 5736 (2000)]. To gauge the importance of the open-shell character of OH and the anisotropy of the potential on the transport properties, including the collision integrals Ω((1,1)) and Ω((2,2)), as well as the diffusion coefficient, calculations were performed with the full potential, with the difference potential V(dif) set to zero, and with only the spherical average of the potential. Slight differences (3%-5%) in the computed diffusion coefficient were found between the values obtained using the full potential and the truncated potentials. The computed diffusion coefficients were compared to recent experimental measurements and those computed with a Lennard-Jones (LJ) 12-6 potential. The values obtained with the full potential were slightly higher than the experimental values. The LJ 12-6 potential was found to underestimate the variation in temperature as compared to that obtained using the full OH-He ab initio potential.

Magnetic properties of tapiolite (FeTa2O6); a quasi two-dimensional (2D) antiferromagnet

NASA Astrophysics Data System (ADS)

Chung, E. M. L.; Lees, M. R.; McIntyre, G. J.; Wilkinson, C.; Balakrishnan, G.; Hague, J. P.; Visser, D.; McK Paul, D.

2004-11-01

The possibilities of two-dimensional (2D) short-range magnetic correlations and frustration effects in the mineral tapiolite are investigated using bulk-property measurements and neutron Laue diffraction. In this study of the magnetic properties of synthetic single-crystals of tapiolite, we find that single crystals of FeTa2O6 order antiferromagnetically at TN = 7.95 ± 0.05 K, with extensive two-dimensional correlations existing up to at least 40 K. Although we find no evidence that FeTa2O6 is magnetically frustrated, hallmarks of two-dimensional magnetism observed in our single-crystal data include: (i) broadening of the susceptibility maximum due to short-range correlations, (ii) a spin-flop transition and (iii) lambda anomalies in the heat capacity and d(χT)/dT. Complementary neutron Laue diffraction measurements reveal 1D magnetic diffuse scattering extending along the c* direction perpendicular to the magnetic planes. This magnetic diffuse scattering, observed for the first time using the neutron Laue technique by VIVALDI, arises directly as a result of 2D short-range spin correlations.

Temporal and vertical variability in optical properties of New England shelf waters during late summer and spring

NASA Astrophysics Data System (ADS)

Sosik, Heidi M.; Green, Rebecca E.; Pegau, W. Scott; Roesler, Collin S.

2001-05-01

Relationships between optical and physical properties were examined on the basis of intensive sampling at a site on the New England continental shelf during late summer 1996 and spring 1997. During both seasons, particles were found to be the primary source of temporal and vertical variability in optical properties since light absorption by dissolved material, though significant in magnitude, was relatively constant. Within the particle pool, changes in phytoplankton were responsible for much of the observed optical variability. Physical processes associated with characteristic seasonal patterns in stratification and mixing contributed to optical variability mostly through effects on phytoplankton. An exception to this generalization occurred during summer as the passage of a hurricane led to a breakdown in stratification and substantial resuspension of nonphytoplankton particulate material. Prior to the hurricane, conditions in summer were highly stratified with subsurface maxima in absorption and scattering coefficients. In spring, stratification was much weaker but increased over the sampling period, and a modest phytoplankton bloom caused surface layer maxima in absorption and scattering coefficients. These seasonal differences in the vertical distribution of inherent optical properties were evident in surface reflectance spectra, which were elevated and shifted toward blue wavelengths in the summer. Some seasonal differences in optical properties, including reflectance spectra, suggest that a significant shift toward a smaller particle size distribution occurred in summer. Shorter timescale optical variability was consistent with a variety of influences including episodic events such as the hurricane, physical processes associated with shelfbreak frontal dynamics, biological processes such as phytoplankton growth, and horizontal patchiness combined with water mass advection.

High-resolution Earth-based lunar radar studies: Applications to lunar resource assessment

NASA Technical Reports Server (NTRS)

Stacy, N. J. S.; Campbell, D. B.

1992-01-01

The lunar regolith will most likely be a primary raw material for lunar base construction and resource extraction. High-resolution radar observations of the Moon provide maps of radar backscatter that have intensity variations generally controlled by the local slope, material, and structural properties of the regolith. The properties that can be measured by the radar system include the dielectric constant, density, loss tangent, and wavelength scale roughness. The radar systems currently in operation at several astronomical observatories provide the ability to image the lunar surface at spatial resolutions approaching 30 m at 3.8 cm and 12.6 cm wavelengths and approximately 500 m at 70 cm wavelength. The radar signal penetrates the lunar regolith to a depth of 10-20 wavelengths so the measured backscatter contains contributions from the vacuum-regolith interface and from wavelength-scale heterogeneities in the electrical properties of the subsurface material. The three wavelengths, which are sensitive to different scale structures and scattering volumes, provide complementary information on the regolith properties. Aims of the previous and future observations include (1) analysis of the scattering properties associated with fresh impact craters, impact crater rays, and mantled deposits; (2) analysis of high-incidence-angle observations of the lunar mare to investigate measurement of the regolith dielectric constant and hence porosity; (3) investigation of interferometric techniques using two time-delayed observations of the same site, observations that require a difference in viewing geometry less than 0.05 deg and, hence, fortuitous alignment of the Earth-Moon system when visible from Arecibo Observatory.

Diurnal Evolution of Aerosol Optical Properties and Morphology at Pico Tres Padres: A Phenomenological Analysis

NASA Astrophysics Data System (ADS)

Mazzoleni, C.; Chakrabarty, R.; Dubey, M. K.; Moosmuller, H.; Chylek, P.; Onasch, T. B.; Herndon, S.; Zavala, M.; Kolb, C.

2007-05-01

Aerosol optical properties affect planetary radiative balance and therefore climate. The optical properties are related to chemical composition, size distribution, and morphology, which also have implications for human health and environmental degradation. During the MILAGRO field campaign, we measured ensemble aerosol absorption and angle-integrated scattering in Mexico City. These measurements were performed using the Los Alamos aerosol photoacoustic instrument with an integrated nephelometer (LAPA) operating at 781 nm. The LAPA was mounted on-board the Aerodyne Inc. mobile laboratory, which hosted a wide variety of gaseous and aerosol instruments. During the campaign, the Aerodyne mobile laboratory was moved to different sites, capturing the influence of spatial and temporal parameters including location, aging, elevation, and sources on ambient air pollution. The LAPA operated almost continuously between the 3rd and the 28th of March 2006. During the same period we collected ambient aerosols on more than 100 Nuclepore filters for scanning electron microscopy (SEM) analysis. Filter samples were collected during specific pollution events and different times of the day. Subsequently, SEM images of selected filters were taken to study particle morphology. The elemental composition of a few individual particles was also qualitatively assessed by energy dispersive X-ray spectroscopy. Between March 7th and 19th the laboratory was sampling air close to the top of the Pico Tres Padres, a ~3000 m high mountain on the north side of the Mexico City. Daily changes of aerosol loading and pollutant concentrations followed the expected diurnal variations of the boundary layer height. Here we report a preliminary analysis of aerosol absorption, scattering, and morphology at Pico Tres Padres for three specific days (9th, 11th and 12th of March 2006). The single scattering albedo (ratio of scattering to total extinction) during these three days showed a characteristic drop in the tens-of-minutes-to-hour time frame immediately following the growth of the boundary layer above the sampling site. Later in the day the single scattering albedo grew steadily to reach a maximum in the late afternoon. The SEM images show a wide variety of aerosol shapes including fractal-like chain aggregates (possibly soot), spherical particles (possibly tar balls), cylinders, and irregular non-fractal shapes. The increased afternoon single scattering albedo in the hottest part of the day qualitatively correlated with a relative increase in spherical particles that typically are not strongly light absorbing relative to fractal-like chain aggregates that are typically strongly light absorbing. These changes in optical properties and/or morphology can be explained by multiple mechanisms such as the collapse of fractal-like chain aggregates due to thermal effects and/or condensation of volatile compounds, coating by organic compounds, and photochemical secondary organic particle formation. Elemental analysis of a few individual particles yielded a relative large carbon abundance combined with smaller fractions of oxygen, silicon, metals, and other elements.

Character of the opposition effect and negative polarization

NASA Technical Reports Server (NTRS)

Pieters, Carle M.; Shkuratov, Yu. G.; Stankevich, D. G.

1991-01-01

Photometric and polarimetric properties at small phase angles were measured for silicates with controlled surface properties in order to distinguish properties that are associated with surface reflection from those that are associated with multiple scattering from internal grain boundaries. These data provide insight into the causes and conditions of photometric properties observed at small phase angles for dark bodies of the solar system. Obsidian was chosen to represent a silicate dielectric with no internal scattering boundaries. Because obsidian is free of internal scatterers, light reflected from both the rough and smooth obsidian samples is almost entirely single and multiple Fresnel reflections form surface facets with no body component. Surface structure alone cannot produce an opposition effect. Comparison of the obsidian and basalt results indicates that for an opposition effect to occur, surface texture must be both rough and contain internal scattering interfaces. Although the negative polarization observed for the obsidian samples indicates single and multiple reflections are part of negative polarization, the longer inversion angle of the multigrain inversion samples implies that internal reflections must also contribute a significant negative polarization component.

Geometries and focal properties of two electron-lens systems useful in low-energy electron or ion scattering

NASA Technical Reports Server (NTRS)

Chutjian, A.

1979-01-01

Geometries and focal properties are given for two types of electron-lens system commonly needed in electron scattering. One is an electron gun that focuses electrons from a thermionic emitter onto a fixed point (target) over a wide range of final energies. The other is an electron analyzer system that focuses scattered electrons of variable energy onto a fixed position (e.g., the entrance plane of an analyzer) at fixed energy with a zero final beam angle. Analyzer-system focusing properties are given for superelastically, elastically, and inelastically scattered electrons. Computer calculations incorporating recent accurate tube-lens focal properties are used to compute lens voltages, locations and diameters of all pupils and windows, filling factors, and asymptotic rays throughout each lens system. Focus voltages as a function of electron energy and energy change are given, and limits of operation of each system discussed. Both lens systems have been in routine use for several years, and good agreement has been consistently found between calculated and operating lens voltages.

Retrieval of aerosol properties and water leaving radiance from multi-angle spectro-polarimetric measurement over coastal waters

NASA Astrophysics Data System (ADS)

Gao, M.; Zhai, P.; Franz, B. A.; Hu, Y.; Knobelspiesse, K. D.; Xu, F.; Ibrahim, A.

2017-12-01

Ocean color remote sensing in coastal waters remains a challenging task due to the complex optical properties of aerosols and ocean water properties. It is highly desirable to develop an advanced ocean color and aerosol retrieval algorithm for coastal waters, to advance our capabilities in monitoring water quality, improve our understanding of coastal carbon cycle dynamics, and allow for the development of more accurate circulation models. However, distinguishing the dissolved and suspended material from absorbing aerosols over coastal waters is challenging as they share similar absorption spectrum within the deep blue to UV range. In this paper we report a research algorithm on aerosol and ocean color retrieval with emphasis on coastal waters. The main features of our algorithm include: 1) combining co-located measurements from a hyperspectral ocean color instrument (OCI) and a multi-angle polarimeter (MAP); 2) using the radiative transfer model for coupled atmosphere and ocean system (CAOS), which is based on the highly accurate and efficient successive order of scattering method; and 3) incorporating a generalized bio-optical model with direct accounting of the total absorption of phytoplankton, CDOM and non-algal particles(NAP), and the total scattering of phytoplankton and NAP for improved description of ocean light scattering. The non-linear least square fitting algorithm is used to optimize the bio-optical model parameters and the aerosol optical and microphysical properties including refractive indices and size distributions for both fine and coarse modes. The retrieved aerosol information is used to calculate the atmospheric path radiance, which is then subtracted from the OCI observations to obtain the water leaving radiance contribution. Our work aims to maximize the use of available information from the co-located dataset and conduct the atmospheric correction with minimal assumptions. The algorithm will contribute to the success of current MAP instruments, such as the Research Scanning Polarimeter (RSP), and future ocean color missions, such as the Plankton, Aerosol, Cloud, and ocean Ecosystem (PACE) mission, by enabling retrieval of ocean biogeochemical properties under optically-complex atmospheric and oceanic conditions.

Biomembranes research using thermal and cold neutrons

DOE PAGES

Heberle, Frederick A.; Myles, Dean A. A.; Katsaras, John

2015-08-01

In 1932 James Chadwick discovered the neutron using a polonium source and a beryllium target (Chadwick, 1932). In a letter to Niels Bohr dated February 24, 1932, Chadwick wrote: “whatever the radiation from Be may be, it has most remarkable properties.” Where it concerns hydrogen-rich biological materials, the “most remarkable” property is the neutron’s differential sensitivity for hydrogen and its isotope deuterium. Such differential sensitivity is unique to neutron scattering, which unlike X-ray scattering, arises from nuclear forces. Consequently, the coherent neutron scattering length can experience a dramatic change in magnitude and phase as a result of resonance scattering, impartingmore » sensitivity to both light and heavy atoms, and in favorable cases to their isotopic variants. Furthermore, this article describes recent biomembranes research using a variety of neutron scattering techniques.« less

A new theory for X-ray diffraction.

PubMed

Fewster, Paul F

2014-05-01

This article proposes a new theory of X-ray scattering that has particular relevance to powder diffraction. The underlying concept of this theory is that the scattering from a crystal or crystallite is distributed throughout space: this leads to the effect that enhanced scatter can be observed at the `Bragg position' even if the `Bragg condition' is not satisfied. The scatter from a single crystal or crystallite, in any fixed orientation, has the fascinating property of contributing simultaneously to many `Bragg positions'. It also explains why diffraction peaks are obtained from samples with very few crystallites, which cannot be explained with the conventional theory. The intensity ratios for an Si powder sample are predicted with greater accuracy and the temperature factors are more realistic. Another consequence is that this new theory predicts a reliability in the intensity measurements which agrees much more closely with experimental observations compared to conventional theory that is based on `Bragg-type' scatter. The role of dynamical effects (extinction etc.) is discussed and how they are suppressed with diffuse scattering. An alternative explanation for the Lorentz factor is presented that is more general and based on the capture volume in diffraction space. This theory, when applied to the scattering from powders, will evaluate the full scattering profile, including peak widths and the `background'. The theory should provide an increased understanding of the reliability of powder diffraction measurements, and may also have wider implications for the analysis of powder diffraction data, by increasing the accuracy of intensities predicted from structural models.

Scattering and Diffraction of Electromagnetic Radiation: An Effective Probe to Material Structure

NASA Technical Reports Server (NTRS)

Xu, Yu-Lin

2016-01-01

Scattered electromagnetic waves from material bodies of different forms contain, in an intricate way, precise information on the intrinsic, geometrical and physical properties of the objects. Scattering theories, ever deepening, aim to provide dependable interpretation and prediction to the complicated interaction of electromagnetic radiation with matter. There are well-established multiple-scattering formulations based on classical electromagnetic theories. An example is the Generalized Multi-particle Mie-solution (GMM), which has recently been extended to a special version ? the GMM-PA approach, applicable to finite periodic arrays consisting of a huge number (e.g., >>106) of identical scattering centers [1]. The framework of the GMM-PA is nearly complete. When the size of the constituent unit scatterers becomes considerably small in comparison with incident wavelength, an appropriate array of such small element volumes may well be a satisfactory representation of a material entity having an arbitrary structure. X-ray diffraction is a powerful characterization tool used in a variety of scientific and technical fields, including material science. A diffraction pattern is nothing more than the spatial distribution of scattered intensity, determined by the distribution of scattering matter by way of its Fourier transform [1]. Since all linear dimensions entered into Maxwell's equations are normalized by wavelength, an analogy exists between optical and X-ray diffraction patterns. A large set of optical diffraction patterns experimentally obtained can be found in the literature [e.g., 2,3]. Theoretical results from the GMM-PA have been scrutinized using a large collection of publically accessible, experimentally obtained Fraunhofer diffraction patterns. As far as characteristic structures of the patterns are concerned, theoretical and experimental results are in uniform agreement; no exception has been found so far. Closely connected with the spatial distribution of scattered intensities are cross sections, such as for extinction, scattering, absorption, and radiation pressure, as a critical type of key quantity addressed in most theoretical and experimental studies of radiative scattering. Cross sections predicted from different scattering theories are supposed to be in general agreement. For objects of irregular shape, the GMM-PA solutions can be compared with the highly flexible Discrete Dipole Approximation (DDA) [4,5] when dividing a target to no more than 106 unit cells. Also, there are different ways to calculate the cross sections in the GMM-PA, providing an additional means to examine the accuracy of the numerical solutions and to unveil potential issues concerning the theoretical formulations and numerical aspects. To solve multiple scattering by an assembly of material volumes through classical theories such as the GMM-PA, the radiative properties of the component scatterers, the complex refractive index in particular, must be provided as input parameters. When using a PA to characterize a material body, this involves the use of an adequate theoretical tool, an effective medium theory, to connect Maxwell's phenomenogical theory with the atomistic theory of matter. In the atomic theory, one regards matter as composed of interacting particles (atoms and molecules) embedded in the vacuum [6]. However, the radiative properties of atomic-scaled particles are known to be substantially different from bulk materials. Intensive research efforts in the fields of cluster science and nanoscience attempt to bridge the gap between bulk and atom and to understand the transition from classical to quantum physics. The GMM-PA calculations, which place virtually no restriction on the component-particle size, might help to gain certain insight into the transition.

Worldwide Ocean Optics Database (WOOD)

DTIC Science & Technology

2002-09-30

attenuation estimated from diffuse attenuation and backscatter data). Error estimates will also be provided for the computed results. Extensive algorithm...empirical algorithms (e.g., beam attenuation estimated from diffuse attenuation and backscatter data). Error estimates will also be provided for the...properties, including diffuse attenuation, beam attenuation, and scattering. Data from ONR-funded bio-optical cruises will be given priority for loading

Worldwide Ocean Optics Database (WOOD)

DTIC Science & Technology

2001-09-30

user can obtain values computed from empirical algorithms (e.g., beam attenuation estimated from diffuse attenuation and backscatter data). Error ...from empirical algorithms (e.g., beam attenuation estimated from diffuse attenuation and backscatter data). Error estimates will also be provided for...properties, including diffuse attenuation, beam attenuation, and scattering. The database shall be easy to use, Internet accessible, and frequently updated

Electrically Reconfigurable Liquid Crystalline Mirrors (Postprint)

DTIC Science & Technology

2018-04-24

preparation of a structurally chiral polymer stabilizing network that enforces anchoring of a low-molar- mass liquid crystalline media with positive...crystals (LCs). The distinctive responses detailed here are enabled by the preparation of a structurally chiral polymer stabilizing network that enforces ...aerospace systems . Dynamic changes to optical material properties including absorption, diffraction, reflection, and scatter have been the subject to

Photopolarimetric properties of leaf and vegetation covers over a wide range of measurement directions

NASA Astrophysics Data System (ADS)

Sun, Zhongqiu; Peng, Zhiyan; Wu, Di; Lv, Yunfeng

2018-02-01

The optical scattering property of the target is the essential signal for passive remote sensing applications. To deepen our understanding of the light reflected from vegetation, we present results of photopolarimetric laboratory measurements from single leaf and two vegetation covers (planophile and erectophile) over a wide range of viewing directions. The bidirectional polarized reflectance factor (BPRF) was used to characterize the polarization property of our samples. We observed positive and negative polarization (-BPRFQ) of all samples in the forward scattering and backward scattering directions, respectively. Based on the comparison of the BPRF among single leaf, planophile vegetation and erectophile vegetation, our measurements demonstrate that the orientation of the leaf is a key factor in describing the amount of polarization in the forward scattering direction. Our measurements also validated certain model results stating that (1) specular reflection generates a portion of polarization in the forward scattering direction and diffuses scattering of polarized light in all hemisphere directions, (2) BPRFU is anti-symmetric in the principal plane from a recent study in which the authors simulated the polarized reflectance of vegetation cover using the vector radiative transfer theory. These photopolarimetric measurement results, which can be completely explained by the theoretical results, are useful in remote sensing applications to vegetation.

Modeling silica aerogel optical performance by determining its radiative properties

NASA Astrophysics Data System (ADS)

Zhao, Lin; Yang, Sungwoo; Bhatia, Bikram; Strobach, Elise; Wang, Evelyn N.

2016-02-01

Silica aerogel has been known as a promising candidate for high performance transparent insulation material (TIM). Optical transparency is a crucial metric for silica aerogels in many solar related applications. Both scattering and absorption can reduce the amount of light transmitted through an aerogel slab. Due to multiple scattering, the transmittance deviates from the Beer-Lambert law (exponential attenuation). To better understand its optical performance, we decoupled and quantified the extinction contributions of absorption and scattering separately by identifying two sets of radiative properties. The radiative properties are deduced from the measured total transmittance and reflectance spectra (from 250 nm to 2500 nm) of synthesized aerogel samples by solving the inverse problem of the 1-D Radiative Transfer Equation (RTE). The obtained radiative properties are found to be independent of the sample geometry and can be considered intrinsic material properties, which originate from the aerogel's microstructure. This finding allows for these properties to be directly compared between different samples. We also demonstrate that by using the obtained radiative properties, we can model the photon transport in aerogels of arbitrary shapes, where an analytical solution is difficult to obtain.

Probabilistic micromechanics for metal matrix composites

NASA Astrophysics Data System (ADS)

Engelstad, S. P.; Reddy, J. N.; Hopkins, Dale A.

A probabilistic micromechanics-based nonlinear analysis procedure is developed to predict and quantify the variability in the properties of high temperature metal matrix composites. Monte Carlo simulation is used to model the probabilistic distributions of the constituent level properties including fiber, matrix, and interphase properties, volume and void ratios, strengths, fiber misalignment, and nonlinear empirical parameters. The procedure predicts the resultant ply properties and quantifies their statistical scatter. Graphite copper and Silicon Carbide Titanlum Aluminide (SCS-6 TI15) unidirectional plies are considered to demonstrate the predictive capabilities. The procedure is believed to have a high potential for use in material characterization and selection to precede and assist in experimental studies of new high temperature metal matrix composites.

In Situ Microphysical and Scattering Properties of Falling Snow in GPM-GCPEx

NASA Astrophysics Data System (ADS)

Duffy, G.; Nesbitt, S. W.; McFarquhar, G. M.; Poellot, M.; Chandrasekar, C. V.; Hudak, D. R.

2013-12-01

The Global Precipitation Measurement Cold-season Precipitation Experiment (GPM-GCPEx) field campaign was conducted near Egbert, Ontario, Canada in January-February 2012 to study the physical characteristics and microwave radiative properties of the column of hydrometeors in cold season precipitation events. Extensive in situ aircraft profiling was conducted with the University of North Dakota (UND) Citation aircraft within the volume of several remote sensing instruments within a wide variety of precipitation events, from snow to freezing drizzle. Several of the primary goals of GCPEx include improving our understanding of the microphysical characteristics of falling snow and how those characteristics relate to the multi-wavelength radiative characteristics In this study, particle size distribution parameters, effective particle densities, and habit distributions are determined using in-situ cloud measurements obtained on the UND citation using the High Volume Precipitation Spectrometer, the Cloud Particle Imager, and the Cloud Imaging Probe. These quantities are matched compared to multi-frequency radar measurements from the Environment Canada King City C-Band and NASA D3R Ku-Ka Band dual polarization radars. These analysis composites provide the basis for direct evaluation of particle size distributions and observed multi-wavelength and multi-polarization radar observations, including radar reflectivity, differential reflectivity, and dual wavelength ratio) in falling snow at weather radar and GPM radar frequencies. Theoretical predictions from Mie, Rayleigh-Gans, and more complex snowflake aggregate scattering model predictions using observed particle size distributions are compared with observed radar scattering characteristics along the Citation flight track.

Coupling of the microphysical and optical properties of an Arctic nimbostratus cloud during the ASTAR 2004 experiment: Implications for light-scattering modeling

NASA Astrophysics Data System (ADS)

Jourdan, Olivier; Mioche, Guillaume; Garrett, Timothy J.; SchwarzenböCk, Alfons; Vidot, JéRôMe; Xie, Yu; Shcherbakov, Valery; Yang, Ping; Gayet, Jean-FrançOis

2010-12-01

Airborne measurements in an Arctic mixed-phase nimbostratus cloud were conducted in Spitsbergen on 21 May 2004 during the international Arctic Study of Tropospheric Aerosol, Clouds and Radiation (ASTAR) campaign. The in situ instrument suite aboard the Alfred Wegener Institute Polar 2 aircraft included a polar nephelometer (PN), a cloud particle imager (CPI), a Nevzorov probe, and a standard PMS 2DC probe to measure the cloud particle single-scattering properties (at a wavelength of 0.8 μm), and the particle morphology and size, as well as the in-cloud partitioning of ice/water content. The main objective of this work is to present a technique based on principal component analysis and light-scattering modeling to link the microphysical properties of cloud particles to their optical characteristics. The technique is applied to the data collected during the 21 May case study where a wide variety of ice crystal shapes and liquid water fractions were observed at temperatures ranging from -1°C to -12°C. CPI measurements highlight the presence of large supercooled water droplets with diameters close to 500 μm. Although the majority of ice particles were found to have irregular shapes, columns and needles were the prevailing regular habits between -3°C and -6°C while stellars and plates were observed at temperatures below -8°C. The implementation of the principal component analysis of the PN scattering phase function measurements revealed representative optical patterns that were consistent with the particle habit classification derived from the CPI. This indicates that the synergy between the CPI and the PN can be exploited to link the microphysical and shape properties of cloud particles to their single-scattering characteristics. Using light-scattering modeling, we have established equivalent microphysical models based on a limited set of free parameters (roughness, mixture of idealized particle habits, and aspect ratio of ice crystals) that reproduce the main optical features assessed for cloud regions with different particle geometries and liquid water fractions. However, the retrieved bulk microphysical parameters can substantially differ from the measurements (by several times for the effective size and up to 3 orders of magnitude for the number concentration). Several possible explanations for these discrepancies are discussed. The retrievals show that the optical contribution of small particles with sizes lower than 50 μm (droplets and ice crystals) is significant, always exceeding 50% of the total scattering signal, and thus needs to be more accurately quantified. The shattering of large ice crystals on the shrouded inlet of the PN could also strongly affect the retrieved microphysical parameters.

Multiple Light Scattering Probes of Soft Materials

NASA Astrophysics Data System (ADS)

Scheffold, Frank

2007-02-01

I will discuss both static and dynamic properties of diffuse waves. In practical applications the optical properties of colloidal systems play an important role, for example in commercial products such as sunscreen lotions, food (drinks), coatings but also in medicine for example in cataract formation (eye lens turbidity). It is thus of importance to know the key parameters governing optical turbidity from the single to the multiple scattering regime. Temporal fluctuations of multiply scattered light are studied with photon correlation spectroscopy (Diffusing Wave Spectroscopy). This DWS method and its various implementations will be treated.

A model for the scattering of high-frequency electromagnetic fields from dielectrics exhibiting thermally-activated electrical losses

NASA Technical Reports Server (NTRS)

Hann, Raiford E.

1991-01-01

An equivalent circuit model (ECM) approach is used to predict the scattering behavior of temperature-activated, electrically lossy dielectric layers. The total electrical response of the dielectric (relaxation + conductive) is given by the ECM and used in combination with transmission line theory to compute reflectance spectra for a Dallenbach layer configuration. The effects of thermally-activated relaxation processes on the scattering properties is discussed. Also, the effect of relaxation and conduction activation energy on the electrical properties of the dielectric is described.

Properties of dust and clouds in the Mars atmosphere: Analysis of Viking IRTM emission phase function sequences

NASA Technical Reports Server (NTRS)

Clancy, R. T.; Lee, S. W.

1991-01-01

An analysis of emission-phase-function (EPF) observations from the Viking Orbiter Infrared Thermal Mapper (IRTM) yields a wide variety of results regarding dust and cloud scattering in the Mars atmosphere and atmospheric-corrected albedos for the surface of Mars. A multiple scattering radiative transfer model incorporating a bidirectional phase function for the surface and atmospheric scattering by dust and clouds is used to derive surface albedos and dust and ice optical properties and optical depths for these various conditions on Mars.

Small-angle scattering from 3D Sierpinski tetrahedron generated using chaos game

NASA Astrophysics Data System (ADS)

Slyamov, Azat

2017-12-01

We approximate a three dimensional version of deterministic Sierpinski gasket (SG), also known as Sierpinski tetrahedron (ST), by using the chaos game representation (CGR). Structural properties of the fractal, generated by both deterministic and CGR algorithms are determined using small-angle scattering (SAS) technique. We calculate the corresponding monodisperse structure factor of ST, using an optimized Debye formula. We show that scattering from CGR of ST recovers basic fractal properties, such as fractal dimension, iteration number, scaling factor, overall size of the system and the number of units composing the fractal.

Temperature-Dependent Second Shell Interference in the First Shell Analysis of Crystalline InP X-ray Absorption Spectroscopy Data

NASA Astrophysics Data System (ADS)

Schnohr, Claudia S.; Araujo, Leandro L.; Ridgway, Mark C.

2014-09-01

Analysing only the first nearest neighbour (NN) scattering signal is a commonly used and often successful way to treat extended X-ray absorption fine structure data. However, using temperature-dependent measurements of InP as an example, we demonstrate how this approach can lead to erroneous first NN structural parameters in systems with a weak first but strong second NN scatterer. In such cases, particularly low temperature data may suffer from an overlap of first and second NN scattering signals caused by the Fourier transformation (FT) even if the dominant peaks appear to be well separated. The first NN structural parameters then vary as a function of the FT settings if only the first NN scattering contribution is considered in the analysis. Although this variation is small, it can also lead to significant differences in other calculated properties such as the Einstein temperature. We demonstrate that these variations can be avoided either by choosing an appropriate FT window or by including the scattering contributions of higher shells in the analysis. The latter is achieved by a path fitting approach and yields structural parameters independent of the FT settings used.

Scattering of electromagnetic plane wave from a perfect electric conducting strip placed at interface of topological insulator-chiral medium

NASA Astrophysics Data System (ADS)

Shoukat, Sobia; Naqvi, Qaisar A.

2016-12-01

In this manuscript, scattering from a perfect electric conducting strip located at planar interface of topological insulator (TI)-chiral medium is investigated using the Kobayashi Potential method. Longitudinal components of electric and magnetic vector potential in terms of unknown weighting function are considered. Use of related set of boundary conditions yields two algebraic equations and four dual integral equations (DIEs). Integrand of two DIEs are expanded in terms of the characteristic functions with expansion coefficients which must satisfy, simultaneously, the discontinuous property of the Weber-Schafheitlin integrals, required edge and boundary conditions. The resulting expressions are then combined with algebraic equations to express the weighting function in terms of expansion coefficients, these expansion coefficients are then substituted in remaining DIEs. The projection is applied using the Jacobi polynomials. This treatment yields matrix equation for expansion coefficients which is solved numerically. These unknown expansion coefficients are used to find the scattered field. The far zone scattering width is investigated with respect to different parameters of the geometry, i.e, chirality of chiral medium, angle of incidence, size of the strip. Significant effects of different parameters including TI parameter on the scattering width are noted.

Solar glint suppression in compact planetary ultraviolet spectrographs

NASA Astrophysics Data System (ADS)

Davis, Michael W.; Cook, Jason C.; Grava, Cesare; Greathouse, Thomas K.; Gladstone, G. Randall; Retherford, Kurt D.

2015-08-01

Solar glint suppression is an important consideration in the design of compact photon-counting ultraviolet spectrographs. Southwest Research Institute developed the Lyman Alpha Mapping Project for the Lunar Reconnaissance Orbiter (launch in 2009), and the Ultraviolet Spectrograph on Juno (Juno-UVS, launch in 2011). Both of these compact spectrographs revealed minor solar glints in flight that did not appear in pre-launch analyses. These glints only appeared when their respective spacecraft were operating outside primary science mission parameters. Post-facto scattered light analysis verifies the geometries at which these glints occurred and why they were not caught during ground testing or nominal mission operations. The limitations of standard baffle design at near-grazing angles are discussed, as well as the importance of including surface scatter properties in standard stray light analyses when determining solar keep-out efficiency. In particular, the scattered light analysis of these two instruments shows that standard "one bounce" assumptions in baffle design are not always enough to prevent scattered sunlight from reaching the instrument focal plane. Future builds, such as JUICE-UVS, will implement improved scattered and stray light modeling early in the design phase to enhance capabilities in extended mission science phases, as well as optimize solar keep out volume.

Light scattering by dust and anthropogenic aerosol at a remote site in the Negev desert, Israel

NASA Astrophysics Data System (ADS)

Andreae, Tracey W.; Andreae, Meinrat O.; Ichoku, Charles; Maenhaut, Willy; Cafmeyer, Jan; Karnieli, Arnon; Orlovsky, Leah

2002-01-01

We investigated aerosol optical properties, mass concentration, and chemical composition over a 2 year period at a remote site in the Negev desert, Israel (Sde Boker, 30° 51'N, 34° 47'E, 470 m above sea level). Light-scattering measurements were made at three wavelengths (450, 550, and 700 nm), using an integrating nephelometer, and included the separate determination of the backscatter fraction. Aerosol coarse and fine fractions were collected with stacked filter units; mass concentrations were determined by weighing, and the chemical composition by proton-induced X-ray emission and instrumental neutron activation analysis. The total scattering coefficient at 550 nm showed a median of 66.7 Mm-1(mean value 75.2 Mm-1, standard deviation 41.7 Mm-1) typical of moderately polluted continental air masses. Values of 1000 Mm-1and higher were encountered during severe dust storm events. During the study period, 31 such dust events were detected. In addition to high scattering levels, they were characterized by a sharp drop in the Ångström coefficient (i.e., the spectral dispersion of the light scattering) to values near zero. Mass-scattering efficiencies were obtained by a multivariate regression of the scattering coefficients on dust, sulfate, and residual components. An analysis of the contributions of these components to the total scattering observed showed that anthropogenic aerosol accounted for about 70% of scattering. The rest was dominated by the effect of the large dust events mentioned above and of small dust episodes typically occurring during midafternoon.

Vibrational properties of nanocrystals from the Debye Scattering Equation

DOE PAGES

Scardi, P.; Gelisio, L.

2016-02-26

One hundred years after the original formulation by Petrus J.W. Debije (aka Peter Debye), the Debye Scattering Equation (DSE) is still the most accurate expression to model the diffraction pattern from nanoparticle systems. A major limitation in the original form of the DSE is that it refers to a static domain, so that including thermal disorder usually requires rescaling the equation by a Debye-Waller thermal factor. The last is taken from the traditional diffraction theory developed in Reciprocal Space (RS), which is opposed to the atomistic paradigm of the DSE, usually referred to as Direct Space (DS) approach. Besides beingmore » a hybrid of DS and RS expressions, rescaling the DSE by the Debye-Waller factor is an approximation which completely misses the contribution of Temperature Diffuse Scattering (TDS). The present work proposes a solution to include thermal effects coherently with the atomistic approach of the DSE. Here, a deeper insight into the vibrational dynamics of nanostructured materials can be obtained with few changes with respect to the standard formulation of the DSE, providing information on the correlated displacement of vibrating atoms.« less

Microstructural effect on radiative scattering coefficient and asymmetry factor of anisotropic thermal barrier coatings

NASA Astrophysics Data System (ADS)

Chen, X. W.; Zhao, C. Y.; Wang, B. X.

2018-05-01

Thermal barrier coatings are common porous materials coated on the surface of devices operating under high temperatures and designed for heat insulation. This study presents a comprehensive investigation on the microstructural effect on radiative scattering coefficient and asymmetry factor of anisotropic thermal barrier coatings. Based on the quartet structure generation set algorithm, the finite-difference-time-domain method is applied to calculate angular scattering intensity distribution of complicated random microstructure, which takes wave nature into account. Combining Monte Carlo method with Particle Swarm Optimization, asymmetry factor, scattering coefficient and absorption coefficient are retrieved simultaneously. The retrieved radiative properties are identified with the angular scattering intensity distribution under different pore shapes, which takes dependent scattering and anisotropic pore shape into account implicitly. It has been found that microstructure significantly affects the radiative properties in thermal barrier coatings. Compared with spherical shape, irregular anisotropic pore shape reduces the forward scattering peak. The method used in this paper can also be applied to other porous media, which designs a frame work for further quantitative study on porous media.

A high rigor temperature, not sarcomere length, determines light scattering properties and muscle colour in beef M. sternomandibularis meat and muscle fibres.

PubMed

Hughes, J; Clarke, F; Purslow, P; Warner, R

2018-05-18

Beef meat colour is impacted by both myoglobin status and the light scattering properties of the muscle, and the specific causative scattering elements of the latter are still unknown. We hypothesize that stretching muscles during rigor will generate a structure which favours light scattering, by increasing the length of the I-band (longer sarcomeres) and that a high rigor temperature will cause protein reconfiguration, changing the muscle structure and promoting light scattering. Muscle fibre fragments were isolated from four beef M. sternomandibularis and subjected to stretching (plus, minus) and three incubation temperatures (5, 15, 35 °C). Reflectance confocal laser scanning microscopy (rCLSM) revealed sarcomere stretching alone was not solely responsible for light scattering development. A high rigor temperature (35 °C) was more favourable for light scattering. Stretching and taking muscle into rigor at 35 °C promoted transverse shrinkage of muscle fibres and increased light scattering and could be applied post-mortem (PM) to reduce the occurrence of problematic dark meat. Crown Copyright © 2018. Published by Elsevier Ltd. All rights reserved.

Laser scattering method applied to determine the concentration of alfa 1-antitrypsin

NASA Astrophysics Data System (ADS)

Riquelme, Bibiana D.; Foresto, Patricia; Valverde, Juana R.; Rasia, Rodolfo J.

2000-04-01

An optical method has been developed to find (alpha) 1- antitrypsin unknown concentrations in human serum samples. This method applies light scattering properties exhibited by initially formed enzyme-inhibitor complexes and uses the curves of aggregation kinetics. It is independent of molecular hydrodynamics. Theoretical approaches showed that scattering properties of transient complexes obey the Rayleigh-Debie conditions. Experiments were performed on the Trypsin/(alpha) 1-antitrypsin system. Measurements were performed in newborn, adult and pregnant sera containing (alpha) 1-antitrypsin in the Trypsin excess region. The solution was excite by a He-Ne laser beam. SO, the particles formed during the reaction are scattering centers for the interacting light. The intensity of the scattered light at 90 degrees from incident beam depends on the nature of those scattering centers. Th rate of increase in scattered intensity depends on the variation in size and shape of the scatterers, being independent of its original size. Peak values of the first derivative linearly correlate with the concentration of (alpha) 1-antitrypsin originally present in the sample. Results are displayed 5 minutes after the initiation of the experimental process. Such speed is of great importance in the immuno-biochemistry determinations.

Computation of scattering matrix elements of large and complex shaped absorbing particles with multilevel fast multipole algorithm

NASA Astrophysics Data System (ADS)

Wu, Yueqian; Yang, Minglin; Sheng, Xinqing; Ren, Kuan Fang

2015-05-01

Light scattering properties of absorbing particles, such as the mineral dusts, attract a wide attention due to its importance in geophysical and environment researches. Due to the absorbing effect, light scattering properties of particles with absorption differ from those without absorption. Simple shaped absorbing particles such as spheres and spheroids have been well studied with different methods but little work on large complex shaped particles has been reported. In this paper, the surface Integral Equation (SIE) with Multilevel Fast Multipole Algorithm (MLFMA) is applied to study scattering properties of large non-spherical absorbing particles. SIEs are carefully discretized with piecewise linear basis functions on triangle patches to model whole surface of the particle, hence computation resource needs increase much more slowly with the particle size parameter than the volume discretized methods. To improve further its capability, MLFMA is well parallelized with Message Passing Interface (MPI) on distributed memory computer platform. Without loss of generality, we choose the computation of scattering matrix elements of absorbing dust particles as an example. The comparison of the scattering matrix elements computed by our method and the discrete dipole approximation method (DDA) for an ellipsoid dust particle shows that the precision of our method is very good. The scattering matrix elements of large ellipsoid dusts with different aspect ratios and size parameters are computed. To show the capability of the presented algorithm for complex shaped particles, scattering by asymmetry Chebyshev particle with size parameter larger than 600 of complex refractive index m = 1.555 + 0.004 i and different orientations are studied.

Controlling Nanoantenna Polarizability through Backaction via a Single Cavity Mode

NASA Astrophysics Data System (ADS)

Ruesink, Freek; Doeleman, Hugo M.; Verhagen, Ewold; Koenderink, A. Femius

2018-05-01

The polarizability α determines the absorption, extinction, and scattering by small particles. Beyond being purely set by scatterer size and material, in fact polarizability can be affected by backaction: the influence of the photonic environment on the scatterer. As such, controlling the strength of backaction provides a tool to tailor the (radiative) properties of nanoparticles. Here, we control the backaction between broadband scatterers and a single mode of a high-quality cavity. We demonstrate that backaction from a microtoroid ring resonator significantly alters the polarizability of an array of nanorods: the polarizability is renormalized as fields scattered from—and returning to—the nanorods via the ring resonator depolarize the rods. Moreover, we show that it is possible to control the strength of the backaction by exploiting the diffractive properties of the array. This perturbation of a strong scatterer by a nearby cavity has important implications for hybrid plasmonic-photonic resonators and the understanding of coupled optical resonators in general.

Modified Monte Carlo method for study of electron transport in degenerate electron gas in the presence of electron-electron interactions, application to graphene

NASA Astrophysics Data System (ADS)

Borowik, Piotr; Thobel, Jean-Luc; Adamowicz, Leszek

2017-07-01

Standard computational methods used to take account of the Pauli Exclusion Principle into Monte Carlo (MC) simulations of electron transport in semiconductors may give unphysical results in low field regime, where obtained electron distribution function takes values exceeding unity. Modified algorithms were already proposed and allow to correctly account for electron scattering on phonons or impurities. Present paper extends this approach and proposes improved simulation scheme allowing including Pauli exclusion principle for electron-electron (e-e) scattering into MC simulations. Simulations with significantly reduced computational cost recreate correct values of the electron distribution function. Proposed algorithm is applied to study transport properties of degenerate electrons in graphene with e-e interactions. This required adapting the treatment of e-e scattering in the case of linear band dispersion relation. Hence, this part of the simulation algorithm is described in details.

The scatter and evolution of the global hot gas properties of simulated galaxy cluster populations

NASA Astrophysics Data System (ADS)

Le Brun, Amandine M. C.; McCarthy, Ian G.; Schaye, Joop; Ponman, Trevor J.

2017-04-01

We use the cosmo-OverWhelmingly Large Simulation (cosmo-OWLS) suite of cosmological hydrodynamical simulations to investigate the scatter and evolution of the global hot gas properties of large simulated populations of galaxy groups and clusters. Our aim is to compare the predictions of different physical models and to explore the extent to which commonly adopted assumptions in observational analyses (e.g. self-similar evolution) are violated. We examine the relations between (true) halo mass and the X-ray temperature, X-ray luminosity, gas mass, Sunyaev-Zel'dovich (SZ) flux, the X-ray analogue of the SZ flux (YX) and the hydrostatic mass. For the most realistic models, which include active galactic nuclei (AGN) feedback, the slopes of the various mass-observable relations deviate substantially from the self-similar ones, particularly at late times and for low-mass clusters. The amplitude of the mass-temperature relation shows negative evolution with respect to the self-similar prediction (I.e. slower than the prediction) for all models, driven by an increase in non-thermal pressure support at higher redshifts. The AGN models predict strong positive evolution of the gas mass fractions at low halo masses. The SZ flux and YX show positive evolution with respect to self-similarity at low mass but negative evolution at high mass. The scatter about the relations is well approximated by log-normal distributions, with widths that depend mildly on halo mass. The scatter decreases significantly with increasing redshift. The exception is the hydrostatic mass-halo mass relation, for which the scatter increases with redshift. Finally, we discuss the relative merits of various hot gas-based mass proxies.

Noninvasive identification of bladder cancer with sub-surface backscattered light

DOE Office of Scientific and Technical Information (OSTI.GOV)

Bigio, I.J.; Mourant, J.R.; Boyer, J.

1994-02-01

A non-invasive diagnostic tool that could identify malignancy in situ and in real time would have a major impact on the detection and treatment of cancer. We have developed and are testing early prototypes of an optical biopsy system (OBS) for detection of cancer and other tissue pathologies. The OBS invokes a unique approach to optical diagnosis of tissue pathologies based on the elastic scattering properties, over a wide range of wavelengths, of the microscopic structure of the tissue. Absorption bands in the tissue also add useful complexity to the spectral data collected. The use of elastic scattering as themore » key to optical tissue diagnostics in the OBS is based on the fact that many tissue pathologies, including a majority of cancer forms, manifest significant architectural changes at the cellular and sub-cellular level. Since the cellular components that cause elastic scattering have dimensions typically on the order of visible to near-IR wavelengths, the elastic (Mie) scattering properties will be strongly wavelength dependent. Thus, morphology and size changes can be expected to cause significant changes in an optical signature that is derived from the wavelength-dependence of elastic scattering as well as absorption. The data acquisition and storage/display time with the OBS instrument is {approximately}1 second. Thus, in addition to the reduced invasiveness of this technique compared with current state-of-the-art methods (surgical biopsy and pathology analysis), the OBS offers the possibility of impressively faster diagnostic assessment. The OBS employs a small fiber-optic probe that is amenable to use with any endoscope, catheter or hypodermic, or to direct surface examination (e.g., as in skin cancer or cervical cancer). We report here specifically on its potential application in the detection of bladder cancer.« less

Impact of calcification state on the inherent optical properties of Emiliania huxleyi coccoliths and coccolithophores

NASA Astrophysics Data System (ADS)

Bi, Lei; Yang, Ping

2015-04-01

Understanding the inherent optical properties (IOPs) of coccoliths and coccolithophores is important in oceanic radiative transfer simulations and remote sensing implementations. In this study, the invariant imbedding T-matrix method (II-TM) is employed to investigate the IOPs of coccoliths and coccolithophores. The Emiliania huxleyi (Ehux) coccolith and coccolithophore models are built based on observed biometric parameters including the eccentricity, the number of slits, and the rim width of detached coccoliths. The calcification state that specifies the amount of calcium of a single coccolith is critical in the determination of the size-volume/mass relationship (note, the volume/mass of coccoltihs at different calcification states are different although the diameters are the same). The present results show that the calcification state, namely, under-calcification, normal-calcification, or over-calcification, significantly influences the backscattering cross section and the phase matrix. Furthermore, the linear depolarization ratio of the light scattered by coccoliths is sensitive to the degree of calcification, and provides a potentially valuable parameter for interpreting oceanic remote sensing data. The phase function of an ensemble of randomly oriented coccolithophores has a similar pattern to that of individual coccoliths, but the forward scattering is dominant in the coccolithophores due to the large geometric cross sections. The linear depolarization ratio associated with coccolithophores is found to be larger than that for coccoliths as polarization is more sensitive to multiple scattering than the phase function. The simulated coccolithophore phase matrix numerical results are compared with laboratory measurements. For scattering angles larger than 100°, an increase of the phase function with respect to the scattering angle is confirmed based on the present coccolithophore model while the spherical approximation fails.

Replacing backscattering with reduced scattering. A better formulation of reflectance function?

NASA Astrophysics Data System (ADS)

Piskozub, Jacek; McKee, David; Freda, Wlodzimierz

2014-05-01

Modern reflectance formulas all involve backscattering coefficient divided by absorption coefficient (bb/a). The backscattering (or backward scattering) coefficient describes how much of the incident radiation is scattered at angles between 90 and 180 deg. However, water leaving photons are not necessarily backscattered because it is possible for a variable fraction to exit after multiple forward scattering events. Therefore the whole angular function of scattering probability (phase function) influences the reflectance signal. This is the reason why phase functions of identical backscattering ratio may result in different reflectance values, contrary to the universally used formula. This creates the question whether there may exist a better formula using a parameter better describing phase function shape than backscattering ratio. The asymmetry parameter g (the average scattering cosine) is commonly used to parametrize phase functions. A replacement for backscattering should decrease with increasing g. Therefore, the simplest candidate to replace backscattering has the form of b(1-g), where b is the scattering coefficient. Such a parameter is well known in biomedical optics under the name of reduced scattering (sometimes transport scattering). It has even been used in parametrizing reflectance in (highly turbid) human tissues. However no attempt has been made to check its usefulness in marine optics. We perform Monte Carlo radiative transfer calculations of reflectance for multiple combinations of inherent optical properties, including different phase functions. The results are used to create a new reflectance formula as a function of reduced scattering and absorption and test its robustness to changes in phase function shape compared to the traditional bb/a formula. We discuss its usefulness as well as advantages and disadvantages compared to the traditional formulation.

Light Scattering by Coated Sphere Immersed in Absorbing Medium: A Comparison between the FDTD and Analytic Solutions

NASA Technical Reports Server (NTRS)

Sun, W.; Loeb, N. G.; Fu, Q.

2004-01-01

A recently developed finite-difference time domain scheme is examined using the exact analytic solutions for light scattering by a coated sphere immersed in an absorbing medium. The relative differences are less than 1% in the extinction, scattering, and absorption efficiencies and less than 5% in the scattering phase functions. The definition of apparent single-scattering properties is also discussed. (C) 2003 Elsevier Ltd. All rights reserved.

Quantifying the risks of solid aerosol geoengineering: the role of fundamental material properties

NASA Astrophysics Data System (ADS)

Dykema, J. A.; Keutsch, F. N.; Keith, D.

2017-12-01

Solid aerosols have been considered as an alternative to sulfate aerosols for solar geoengineering due to their optical and chemical properties, which lead to different and possibly more attractive risk profiles. Solid aerosols can achieve higher solar scattering efficiency due to their higher refractive index, and in some cases may also be less effective absorbers of thermal infrared radiation. The optical properties of solid aerosols are however sensitive functions of the detailed physical properties of solid materials in question. The relevant details include the exact crystalline structure of the aerosols, the physical size of the particles, and interactions with background stratospheric molecular and particulate constituents. In this work, we examine the impact of these detailed physical properties on the radiative properties of calcite (CaCO3) solid aerosols. We examine how crystal morphology, size, chemical reactions, and interaction with background stratospheric aerosol may alter the scattering and absorption properties of calcite aerosols for solar and thermal infrared radiation. For example, in small particles, crystal lattice vibrations associated with the particle surface may lead to substantially different infrared absorption properties than bulk materials. We examine the wavelength dependence of absorption by the particles, which may lead to altered patterns of stratospheric radiative heating and equilibrium temperatures. Such temperature changes can lead to dynamical changes, with consequences for both stratospheric composition and tropospheric climate. We identify important uncertainties in the current state of understanding, investigate risks associated with these uncertainties, and survey potential approaches to quantitatively improving our knowledge of the relevant material properties.

Radiative Effects of Aerosol in the Marine Environment: Tales from the Two-Column Aerosol Project

NASA Astrophysics Data System (ADS)

Berg, L. K.; Fast, J. D.; Barnard, J.; Chand, D.; Chapman, E. G.; Comstock, J. M.; Ferrare, R. A.; Flynn, C. J.; Hair, J. W.; Hostetler, C. A.; Hubbe, J.; Johnson, R.; Kassianov, E.; Kluzek, C.; Laskin, A.; Lee, Y.; Mei, F.; Michalsky, J. J.; Redemann, J.; Rogers, R. R.; Russell, P. B.; Sedlacek, A. J.; Schmid, B.; Shilling, J. E.; Shinozuka, Y.; Springston, S. R.; Tomlinson, J. M.; Wilson, J. M.; Zelenyuk, A.; Berkowitz, C. M.

2013-12-01

There is still uncertainty associated with the direct radiative forcing by atmospheric aerosol and its representation in atmospheric models. This is particularly true in marine environments near the coast where the aerosol loading is a function of both naturally occurring and anthropogenic aerosol. These regions are also subject to variable synoptic and thermally driven flows (land-sea breezes) that transport aerosol between the continental and marine environments. The situation is made more complicated due to seasonal changes in aerosol emissions. Given these differences in emissions, we expect significant differences in the aerosol intensive and extensive properties between summer and winter and data is needed to evaluate models over the wide range of conditions. To address this issue, the recently completed Two Column Aerosol Project (TCAP) was designed to measure the key aerosol parameters in two atmospheric columns, one located over Cape Cod, Massachusetts and another approximately 200 km from the coast over the Atlantic Ocean. Measurements included aerosol size distribution, chemical composition, optical properties and vertical distribution. Several aspects make TCAP unique, including the year-long deployment of a suite of surface-based instruments by the US Department of Energy's Atmospheric Radiation Measurement (ARM) Climate Research Facility and two aircraft intensive operations periods supported by the ARM Airborne Facility, one conducted in July 2012 and a second in February 2013. The presentation will include a discussion of the impact of the aerosol optical properties and their uncertainty on simulations of the radiation budget within the TCAP domain in the context of both single column and regional scale models. Data from TCAP will be used to highlight a number of important factors, including diurnal variation in aerosol optical depth measured at the surface site, systematic changes in aerosol optical properties (including scattering, absorption, and single scattering albedo) as a function of height, and changes in aerosol loading, chemical composition, and mixing state with height and distance from the coast.

Non-perturbative Approach to Equation of State and Collective Modes of the QGP

NASA Astrophysics Data System (ADS)

Liu, Y. F. Shuai; Rappxs, Ralf

2018-01-01

We discuss a non-perturbative T-matrix approach to investigate the microscopic structure of the quark-gluon plasma (QGP). Utilizing an effective Hamiltonian which includes both light- and heavy-parton degrees of freedoms. The basic two-body interaction includes color-Coulomb and confining contributions in all available color channels, and is constrained by lattice-QCD data for the heavy-quark free energy. The in-medium T-matrices and parton spectral functions are computed selfconsistently with full account of off-shell properties encoded in large scattering widths. We apply the T-matrices to calculate the equation of state (EoS) for the QGP, including a ladder resummation of the Luttinger-Ward functional using a matrix-log technique to account for the dynamical formation of bound states. It turns out that the latter become the dominant degrees of freedom in the EoS at low QGP temperatures indicating a transition from parton to hadron degrees of freedom. The calculated spectral properties of one- and two-body states confirm this picture, where large parton scattering rates dissolve the parton quasiparticle structures while broad resonances start to form as the pseudocritical temperature is approached from above. Further calculations of transport coefficients reveal a small viscosity and heavy-quark diffusion coefficient.

Alternative Measurement Configurations for Extracting Bulk Optical Properties Using an Integrating Sphere Setup.

PubMed

Thennadil, Suresh N; Chen, Yi-Chieh

2017-02-01

The usual approach for estimating bulk optical properties using an integrating sphere measurement setup is by acquiring spectra from three measurement modes namely collimated transmittance (T c ), total transmittance (T d ), and total diffuse reflectance (R d ), followed by the inversion of these measurements using the adding-doubling method. At high scattering levels, accurate acquisition of T c becomes problematic due to the presence of significant amounts of forward-scattered light in this measurement which is supposed to contain only unscattered light. In this paper, we propose and investigate the effectiveness of using alternative sets of integrating sphere measurements that avoid the use of T c and could potentially increase the upper limit of concentrations of suspensions at which bulk optical property measurements can be obtained in the visible-near-infrared (Vis-NIR) region of the spectrum. We examine the possibility of replacing T c with one or more reflectance measurements at different sample thicknesses. We also examine the possibility of replacing both the collimated (T c ) and total transmittance (T d ) measurements with reflectance measurements taken from different sample thicknesses. The analysis presented here indicates that replacing T c with a reflectance measurement can reduce the errors in the bulk scattering properties when scattering levels are high. When only multiple reflectance measurements are used, good estimates of the bulk optical properties can be obtained when the absorption levels are low. In addition, we examine whether there is any advantage in using three measurements instead of two to obtain the reduced bulk scattering coefficient and the bulk absorption coefficient. This investigation is made in the context of chemical and biological suspensions which have a much larger range of optical properties compared to those encountered with tissue.

Optical properties of phosphor-in-glass through modification of pore properties for LED packaging

NASA Astrophysics Data System (ADS)

Kim, Sunil; Kim, Hyungsun

2018-01-01

The volume and size of the voids present between the frit and the phosphor particles used before sintering determine the pore properties of the resulting phosphor-in-glass (PIG). The pores formed from the voids influence the path of the incident light, thus changing the optical properties of the PIG. Therefore, the trends observed for the shrinkage and the green and sintered densities of the PIG were investigated using SiO2-B2O3-ZnO-K2O glass frit of four sizes to understand the tendency for the pore size, porosity, and optical properties of PIG. It has been demonstrated that variation in the pore properties according to the particle size influences parameters defining the light scattering phenomenon, such as the scattering angle of the light and the scattering coefficient, as well as the color rendering index, correlated color temperature, and package efficacy. The results obtained for the variation in the optical properties with the frit size can be used as a reference to select the appropriate glass frit size to achieve the required optical properties for a light-emitting diode (LED) package.

THERMOS. 30-Group ENDF/B Scattered Kernels

DOE Office of Scientific and Technical Information (OSTI.GOV)

McCrosson, F.J.; Finch, D.R.

1973-12-01

These data are 30-group THERMOS thermal scattering kernels for P0 to P5 Legendre orders for every temperature of every material from s(alpha,beta) data stored in the ENDF/B library. These scattering kernels were generated using the FLANGE2 computer code. To test the kernels, the integral properties of each set of kernels were determined by a precision integration of the diffusion length equation and compared to experimental measurements of these properties. In general, the agreement was very good. Details of the methods used and results obtained are contained in the reference. The scattering kernels are organized into a two volume magnetic tapemore » library from which they may be retrieved easily for use in any 30-group THERMOS library.« less

THE EFFECT OF TWO-MAGNON SCATTERING ON PARALLEL-PUMP INSTABILITY THRESHOLDS.

DTIC Science & Technology

Following a general description of the important properties and symmetries of the parallel-pump coupling and of two- magnon scattering, several...theoretical approaches to the problem of the effect of two- magnon scattering on the parallel-pump instability threshold are explored. A successful approach

Light Scattering by Marine Particles: Modeling with Non-spherical Shapes

DTIC Science & Technology

2008-01-01

Emiliania huxleyi, Limnology and Oceanography, 46, 1438−1454. Gordon, H.R., 2004, Inverse Radiative Transfer, Coccolith Backscattering, and Light Scattering...16430. Voss, K.J., W.M. Balch, and K.A. Kilpatrick, 1998, Scattering and attenuation properties of Emiliania huxleyi cells and their detached

Size-dependent Measurements of the Scattering Properties of Planetary Regolith Analogs: A Challenge to Theory

NASA Technical Reports Server (NTRS)

Piatek, J. L.; Hapke, B. W.; Nelson, R. M.; Hale, A. S.; Smythe, W. D.

2003-01-01

The nature of the scattering of light is thought to be well understood when the medium is made up of independent scatterers that are much larger than the wavelength of that light. This is not the case when the size of the scattering objects is similar to or smaller than the wavelength or the scatterers are not independent. In an attempt to examine the applicability of independent particle scattering models, to planetary regoliths, a dataset of experimental results were compared with theoretical predictions.

Mars dust and cloud opacities and scattering properties

NASA Technical Reports Server (NTRS)

Clancy, R. T.; Lee, S. W.

1992-01-01

We have recently completed an analysis of the visible emission-phase function (EPF) sequences obtained with the solar-band channel of the Infrared Thermal Mapping (IRTM) instrument onboard the two Viking Orbiters. Roughly 100 of these EPF sequences were gathered during the 1977-1980 period, in which the total broadband (.3-3.0 microns) reflectances of the atmosphere/surface above specific locations on Mars were measured versus emission angle as the spacecraft passed overhead. A multiple scattering radiative transfer program was employed to model the EPF observations in terms of the optical depths of dust/clouds, their single scattering albedos and phase functions, and the Lambert albedos and phase coefficient of the underlying surfaces. Due to the predominance of atmospheric scattering at large atmospheric pathlengths and/or large dust opacities, we were able to obtain strong constraints on the scattering properties of dust/clouds and their opacities for a wide range of latitudes, longitudes, and seasons on Mars.

Scattering Effects of Solar Panels on Space Station Antenna Performance

NASA Technical Reports Server (NTRS)

Panneton, Robert J.; Ngo, John C.; Hwu, Shian U.; Johnson, Larry A.; Elmore, James D.; Lu, Ba P.; Kelley, James S.

1994-01-01

Characterizing the scattering properties of the solar array panels is important in predicting Space Station antenna performance. A series of far-field, near-field, and radar cross section (RCS) scattering measurements were performed at S-Band and Ku-Band microwave frequencies on Space Station solar array panels. Based on investigation of the measured scattering patterns, the solar array panels exhibit similar scattering properties to that of the same size aluminum or copper panel mockup. As a first order approximation, and for worse case interference simulation, the solar array panels may be modeled using perfect reflecting plates. Numerical results obtained using the Geometrical Theory of Diffraction (GTD) modeling technique are presented for Space Station antenna pattern degradation due to solar panel interference. The computational and experimental techniques presented in this paper are applicable for antennas mounted on other platforms such as ship, aircraft, satellite, and space or land vehicle.

Assessment and validation of the community radiative transfer model for ice cloud conditions

NASA Astrophysics Data System (ADS)

Yi, Bingqi; Yang, Ping; Weng, Fuzhong; Liu, Quanhua

2014-11-01

The performance of the Community Radiative Transfer Model (CRTM) under ice cloud conditions is evaluated and improved with the implementation of MODIS collection 6 ice cloud optical property model based on the use of severely roughened solid column aggregates and a modified Gamma particle size distribution. New ice cloud bulk scattering properties (namely, the extinction efficiency, single-scattering albedo, asymmetry factor, and scattering phase function) suitable for application to the CRTM are calculated by using the most up-to-date ice particle optical property library. CRTM-based simulations illustrate reasonable accuracy in comparison with the counterparts derived from a combination of the Discrete Ordinate Radiative Transfer (DISORT) model and the Line-by-line Radiative Transfer Model (LBLRTM). Furthermore, simulations of the top of the atmosphere brightness temperature with CRTM for the Crosstrack Infrared Sounder (CrIS) are carried out to further evaluate the updated CRTM ice cloud optical property look-up table.

Solid State Research.

DTIC Science & Technology

1982-11-15

Optics Y-Junction and Mach-Zehnder Interferometric Modulator Using Four -Port Scattering Matrix 7 1.3 Heterodyne and Direct Detection at 10 om with High...and of the Mach-Zehnder interferometric modulator have been analyzed using the four -port scattering i- matrix. The interferometric properties of the Y...USING FOUR -PORT SCATTERING MATRIX The scattering matrix formalism for a lossless four -port device has been used to describe the performance of the

The scattering variety

NASA Astrophysics Data System (ADS)

He, Yang-Hui; Matti, Cyril; Sun, Chuang

2014-10-01

The so-called Scattering Equations which govern the kinematics of the scattering of massless particles in arbitrary dimensions have recently been cast into a system of homogeneous polynomials. We study these as affine and projective geometries which we call Scattering Varieties by analyzing such properties as Hilbert series, Euler characteristic and singularities. Interestingly, we find structures such as affine Calabi-Yau threefolds as well as singular K3 and Fano varieties.

Nucleon-deuteron scattering with the JISP16 potential

NASA Astrophysics Data System (ADS)

Skibiński, R.; Golak, J.; Topolnicki, K.; Witała, H.; Volkotrub, Yu.; Kamada, H.; Shirokov, A. M.; Okamoto, R.; Suzuki, K.; Vary, J. P.

2018-01-01

The nucleon-nucleon J -matrix inverse scattering potential JISP16 is applied to elastic nucleon-deuteron scattering and the deuteron breakup process at the laboratory nucleon energies up to 135 MeV. The formalism of the Faddeev equations is used to obtain three-nucleon scattering states. We compare predictions based on the JISP16 force with data and with results based on various two-body interactions, including the CD Bonn, the Argonne AV18, the chiral force with the semilocal regularization at the fifth order of the chiral expansion and with low-momentum interactions obtained from the CD Bonn force as well as with the predictions from the combination of the AV18 NN interaction and the Urbana IX 3 N force. JISP16 provides a satisfactory description of some observables at low energies but strong deviations from data as well as from standard and chiral potential predictions with increasing energy. However, there are also polarization observables at low energies for which the JISP16 predictions differ from those based on the other forces by a factor of two. The reason for such a behavior can be traced back to the P -wave components of the JISP16 force. At higher energies the deviations can be enhanced by an interference with higher partial waves and by the properties of the JISP16 deuteron wave function. In addition, we compare the energy and angular dependence of predictions based on the JISP16 force with the results of the low-momentum interactions obtained with different values of the momentum cutoff parameter. We found that such low-momentum forces can be employed to interpret the nucleon-deuteron elastic scattering data only below some specific energy which depends on the cutoff parameter. Since JISP16 is defined in a finite oscillator basis, it has properties similar to low momentum interactions and its application to the description of nucleon-deuteron scattering data is limited to a low momentum transfer region.

Active and Passive 3D Vector Radiative Transfer with Preferentially-Aligned Ice Particles

NASA Astrophysics Data System (ADS)

Adams, I. S.; Munchak, S. J.; Pelissier, C.; Kuo, K. S.; Heymsfield, G. M.

2017-12-01

To support the observation of clouds and precipitation using combinations of radars and radiometers, a forward model capable of representing diverse sensing geometries for active and passive instruments is necessary for correctly interpreting and consistently combining multi-sensor measurements from ground-based, airborne, and spaceborne platforms. As such, the Atmospheric Radiative Transfer Simulator (ARTS) uses Monte Carlo integration to produce radar reflectivities and radiometric brightness temperatures for three-dimensional cloud and precipitation input fields. This radiative transfer framework is capable of efficiently sampling Gaussian antenna beams and fully accounting for multiple scattering. By relying on common ray-tracing tools, gaseous absorption models, and scattering properties, the model reproduces accurate and consistent radar and radiometer observables. While such a framework is an important component for simulating remote sensing observables, the key driver for self-consistent radiative transfer calculations of clouds and precipitation is scattering data. Research over the past decade has demonstrated that spheroidal models of frozen hydrometeors cannot accurately reproduce all necessary scattering properties at all desired frequencies. The discrete dipole approximation offers flexibility in calculating scattering for arbitrary particle geometries, but at great computational expense. When considering scattering for certain pristine ice particles, the Extended Boundary Condition Method, or T-Matrix, is much more computationally efficient; however, convergence for T-Matrix calculations fails at large size parameters and high aspect ratios. To address these deficiencies, we implemented the Invariant Imbedding T-Matrix Method (IITM). A brief overview of ARTS and IITM will be given, including details for handling preferentially-aligned hydrometeors. Examples highlighting the performance of the model for simulating space-based and airborne measurements will be offered, and some case studies showing the response to particle type and orientation will be presented. Simulations of polarized radar (Z, LDR, ZDR) and radiometer (Stokes I and Q) quantities will be used to demonstrate the capabilities of the model.

Estimation of Scatterer Diameter by Normalized Power Spectrum of High-Frequency Ultrasonic RF Echo for Assessment of Red Blood Cell Aggregation

NASA Astrophysics Data System (ADS)

Fukushima, Taku; Hasegawa, Hideyuki; Kanai, Hiroshi

2011-07-01

Red blood cell (RBC) aggregation, as one of the determinants of blood viscosity, plays an important role in blood rheology, including the condition of blood. RBC aggregation is induced by the adhesion of RBCs when the electrostatic repulsion between RBCs weakens owing to increases in protein and saturated fatty acid levels in blood, excessive RBC aggregation leads to various circulatory diseases. This study was conducted to establish a noninvasive quantitative method for assessment of RBC aggregation. The power spectrum of ultrasonic RF echoes from nonaggregating RBCs, which shows the frequency property of scattering, exhibits Rayleigh behavior. On the other hand, ultrasonic RF echoes from aggregating RBCs contain the components of reflection, which have no frequency dependence. By dividing the measured power spectrum of echoes from RBCs in the lumen by that of echoes from a posterior wall of the vein in the dorsum manus, the attenuation property of the propagating medium and the frequency responses of transmitting and receiving transducers are removed from the former spectrum. RBC aggregation was assessed by the diameter of a scatterer, which was estimated by minimizing the square difference between the measured normalized power spectrum and the theoretical power spectrum. In this study, spherical scatterers with diameters of 5, 11, 15, and 30 µm were measured in basic experiments. The estimated scatterer diameters were close to the actual diameters. Furthermore, the transient change of the scatterer diameters were measured in an in vivo experiment with respect to a 24-year-old healthy male during the avascularization using a cuff. The estimated diameters (12-22 µm) of RBCs during avascularization were larger than the diameters (4-8 µm) at rest and after recirculation. These results show the possibility of the use of the proposed method for noninvasive assessment of RBC aggregation.

Diffuse reflectance relations based on diffusion dipole theory for large absorption and reduced scattering

NASA Astrophysics Data System (ADS)

Bremmer, Rolf H.; van Gemert, Martin J. C.; Faber, Dirk J.; van Leeuwen, Ton G.; Aalders, Maurice C. G.

2013-08-01

Diffuse reflectance spectra are used to determine the optical properties of biological samples. In medicine and forensic science, the turbid objects under study often possess large absorption and/or scattering properties. However, data analysis is frequently based on the diffusion approximation to the radiative transfer equation, implying that it is limited to tissues where the reduced scattering coefficient dominates over the absorption coefficient. Nevertheless, up to absorption coefficients of 20 m at reduced scattering coefficients of 1 and 11.5 mm-1, we observed excellent agreement (r2=0.994) between reflectance measurements of phantoms and the diffuse reflectance equation proposed by Zonios et al. [Appl. Opt. 38, 6628-6637 (1999)], derived as an approximation to one of the diffusion dipole equations of Farrell et al. [Med. Phys. 19, 879-888 (1992)]. However, two parameters were fitted to all phantom experiments, including strongly absorbing samples, implying that the reflectance equation differs from diffusion theory. Yet, the exact diffusion dipole approximation at high reduced scattering and absorption also showed agreement with the phantom measurements. The mathematical structure of the diffuse reflectance relation used, derived by Zonios et al. [Appl. Opt. 38, 6628-6637 (1999)], explains this observation. In conclusion, diffuse reflectance relations derived as an approximation to the diffusion dipole theory of Farrell et al. can analyze reflectance ratios accurately, even for much larger absorption than reduced scattering coefficients. This allows calibration of fiber-probe set-ups so that the object's diffuse reflectance can be related to its absorption even when large. These findings will greatly expand the application of diffuse reflection spectroscopy. In medicine, it may allow the use of blue/green wavelengths and measurements on whole blood, and in forensic science, it may allow inclusion of objects such as blood stains and cloth at crime scenes.

Aerosol optical properties at rural background area in Western Saudi Arabia

NASA Astrophysics Data System (ADS)

Lihavainen, H.; Alghamdi, M. A.; Hyvärinen, A.; Hussein, T.; Neitola, K.; Khoder, M.; Abdelmaksoud, A. S.; Al-Jeelani, H.; Shabbaj, I. I.; Almehmadi, F. M.

2017-11-01

To derive the comprehensive aerosol in situ characteristics at a rural background area in Saudi Arabia, an aerosol measurements station was established to Hada Al Sham, 60 km east from the Red Sea and the city of Jeddah. The present sturdy describes the observational data from February 2013 to February 2015 of scattering and absorption coefficients, Ångström exponents and single scattering albedo over the measurement period. The average scattering and absorption coefficients at wavelength 525 nm were 109 ± 71 Mm- 1 (mean ± SD, at STP conditions) and 15 ± 17 Mm- 1 (at STP conditions), respectively. As expected, the scattering coefficient was dominated by large desert dust particles with low Ångström scattering exponent, 0.49 ± 0.62. Especially from February to June the Ångström scattering exponent was clearly lower (0.23) and scattering coefficients higher (124 Mm- 1) than total averages because of the dust outbreak season. Aerosol optical properties had clear diurnal cycle. The lowest scattering and absorption coefficients and aerosol optical depths were observed around noon. The observed diurnal variation is caused by wind direction and speed, during night time very calm easterly winds are dominating whereas during daytime the stronger westerly winds are dominating (sea breeze). Positive Matrix Factorization mathematical tool was applied to the scattering and absorption coefficients and PM2.5 and coarse mode (PM10-PM2.5) mass concentrations to identify source characteristics. Three different factors with clearly different properties were found; anthropogenic, BC source and desert dust. Mass absorption efficiencies for BC source and desert dust factors were, 6.0 m2 g- 1 and 0.4 m2 g- 1, respectively, and mass scattering efficiencies for anthropogenic (sulphate) and desert dust, 2.5 m2 g- 1 and 0.8 m2 g- 1, respectively.

Group theoretic approach to the perturbative string S-matrix

NASA Astrophysics Data System (ADS)

Neveu, A.; West, P.

1987-07-01

A new approach to the computation of string scattering is given. From duality, unitarity and a generic overlap property, we determine entirely the N-string amplitude, including the integration measure, and its gauge properties. The techniques do not use any oscillator algebra, but the computation is reduced to a straightforward exercise in conformal group theory. This can be applied to fermionic trees and multiloop diagrams, but in this paper it is demonstrated on the open bosonic tree. Permanent address: Mathematics Department, King's College, Strand, London WC2R 2LS, UK.

Phase Contrast Microscopy Analysis of Breast Tissue

PubMed Central

Wells, Wendy A.; Wang, Xin; Daghlian, Charles P.; Paulsen, Keith D.; Pogue, Brian W.

2010-01-01

OBJECTIVE To assess how optical scatter properties in breast tissue, as measured by phase contrast microscopy and interpreted pathophysiologically, might be exploited as a diagnostic tool to differentiate cancer from benign tissue. STUDY DESIGN We evaluated frozen human breast tissue sections of adipose tissue, normal breast parenchyma, benign fibroadenoma tumors and noninvasive and invasive malignant cancers by phase contrast microscopy through quantification of grayscale values, using multiple regions of interest (ROI). Student’s t tests were performed on phase contrast measures across diagnostic categories testing data from individual cases; all ROI data were used as separate measures. RESULTS Stroma demonstrated significantly higher scatter intensity than did epithelium, with lower scattering in tumor-associated stroma as compared with normal or benign-associated stroma. Measures were comparable for invasive and noninvasive malignant tumors but were higher than those found in benign tumors and were lowest in adipose tissue. CONCLUSION Significant differences were found in scatter coefficient properties of epithelium and stroma across diagnostic categories of breast tissue, particularly between benign and malignant-associated stroma. Improved understanding of how scatter properties correlate with morphologic criteria used in routine pathologic diagnoses could have a significant clinical impact as developing optical technology allows macroscopic in situ phase contrast imaging. PMID:19736867

Easy Volcanic Aerosol (EVA v1.0): an idealized forcing generator for climate simulations

NASA Astrophysics Data System (ADS)

Toohey, Matthew; Stevens, Bjorn; Schmidt, Hauke; Timmreck, Claudia

2016-11-01

Stratospheric sulfate aerosols from volcanic eruptions have a significant impact on the Earth's climate. To include the effects of volcanic eruptions in climate model simulations, the Easy Volcanic Aerosol (EVA) forcing generator provides stratospheric aerosol optical properties as a function of time, latitude, height, and wavelength for a given input list of volcanic eruption attributes. EVA is based on a parameterized three-box model of stratospheric transport and simple scaling relationships used to derive mid-visible (550 nm) aerosol optical depth and aerosol effective radius from stratospheric sulfate mass. Precalculated look-up tables computed from Mie theory are used to produce wavelength-dependent aerosol extinction, single scattering albedo, and scattering asymmetry factor values. The structural form of EVA and the tuning of its parameters are chosen to produce best agreement with the satellite-based reconstruction of stratospheric aerosol properties following the 1991 Pinatubo eruption, and with prior millennial-timescale forcing reconstructions, including the 1815 eruption of Tambora. EVA can be used to produce volcanic forcing for climate models which is based on recent observations and physical understanding but internally self-consistent over any timescale of choice. In addition, EVA is constructed so as to allow for easy modification of different aspects of aerosol properties, in order to be used in model experiments to help advance understanding of what aspects of the volcanic aerosol are important for the climate system.

Time-dependent photon migration imaging

NASA Astrophysics Data System (ADS)

Sevick, Eva M.; Wang, NaiGuang; Chance, Britton

1992-02-01

Recently, the application of both time- and frequency-resolved fluorescence techniques for the determination of photon migration characteristics in strongly scattering media has been used to characterize the optical properties in strongly scattering media. Specifically, Chance and coworkers have utilized measurement of photon migration characteristics to determine tissue hemoglobin absorbance and ultimately oxygenation status in homogeneous tissues. In this study, we present simulation results and experimental measurements for both techniques to show the capacity of time-dependent photon migration characteristics to image optically obscure absorbers located in strongly scattering media. The applications of time-dependent photon imaging in the biomedical community include imaging of light absorbing hematomas, tumors, hypoxic tissue volumes, and other tissue abnormalities. Herein, we show that the time-resolved parameter of mean photon path length, , and the frequency- resolved parameter of phase-shift, (theta) , can be used similarly to obtain three dimensional information of absorber position from two-dimensional measurements. Finally, we show that unlike imaging techniques that monitor the intensity of light without regard to the migration characteristics, the resolution of time-dependent photon migration measurements is enhanced by tissue scattering, further potentiating their use for biomedical imaging.

RCS of fundamental scatterers in the HF band by wire-grid modelling

NASA Astrophysics Data System (ADS)

Trueman, C. W.; Kubina, S. J.

To extract the maximum information from the return of a radar target such as an aircraft, the target's scattering properties must be well known. Wire grid modeling allows a detailed representation of the surface of a complex scatterer such as an aircraft, in the frequency range where the aircraft size is comparable to a wavelength. A moment method analysis determines the currents on the wires of the grid including the interactions between all parts of the structure. Wire grid models of fundamental scatterers (plates, strips, cubes, and spheres) of sizes comparable to the wavelength in the 2-30 MHz range are analyzed. The study of the radar cross section (RCS) of wire grids in comparison with measured RCS data helps to establish guidelines for building wire grid models, specifying such parameters as where to locate wires, how short the segments must be, and what radius to use. The guidelines so developed can then be applied to build wire grid models of much more complex bodies such as aircraft with much greater confidence.

Using Radars in Place of Magnetometers: Detection and Properties of Pc3-5 Wave Fields in HF Radar Data

NASA Astrophysics Data System (ADS)

Ponomarenko, P.; Menk, F. W.; Waters, C. L.

2004-12-01

SuperDARN HF radars are usually used to examine HF echoes from field-aligned ionospheric irregularity structures. However, ground scatter is also often recorded. Because the ground scatter signal is reflected from the ionosphere its Doppler shift is a sensitive indicator of ionospheric motions. We have used the TIGER radar, which operates at relatively low latitudes, to examine ground scatter returns with high time resolution. Ground scatter returns are present virtually every day and wave-like Doppler shift features are evident almost each time. Comparison with ground magnetometer data shows that these are the ionospheric signature of downgoing ULF waves. Several different types of wave features have been observed, including very large scale Pc5, harmonics of field line resonances in the Pc3-4 range, and bandlimited Pc4 at night. This paper presents examples and discusses the wave generation and propagation mechanisms. Furthermore, estimates of the ionospheric transfer function over the 10-110 mHz range are compared with results of numerical and analytical modelling.

Polymer encapsulated inorganic black pigment nanoparticles and their electrophoretic characteristics.

PubMed

Sim, H H; Kim, Y J; Choi, H J

2012-12-01

Black inorganic pigment modified with poly(styrene-co-acrylonitrile) was fabricated via dispersion polymerization, and then the synthesized hybrid nanoparticles were examined by SEM to confirm their morphology, while their density and size were studied using a gas pycnometer and electrophoretic light scattering apparatus, respectively. We also confirmed their chemical structure and coated state via FT-IR and TGA. Electrophoretic characteristics including the zeta potential were examined via an electrophoretic light scattering apparatus, while the movement of particles was directly observed by an optical microscopy under an electric field applied. The hybrid nanoparticles were confirmed to possess an electrophoretic property as a potential candidate for the microcapsule-type electrophoretic display.

Precision measurements of linear scattering density using muon tomography

NASA Astrophysics Data System (ADS)

Åström, E.; Bonomi, G.; Calliari, I.; Calvini, P.; Checchia, P.; Donzella, A.; Faraci, E.; Forsberg, F.; Gonella, F.; Hu, X.; Klinger, J.; Sundqvist Ökvist, L.; Pagano, D.; Rigoni, A.; Ramous, E.; Urbani, M.; Vanini, S.; Zenoni, A.; Zumerle, G.

2016-07-01

We demonstrate that muon tomography can be used to precisely measure the properties of various materials. The materials which have been considered have been extracted from an experimental blast furnace, including carbon (coke) and iron oxides, for which measurements of the linear scattering density relative to the mass density have been performed with an absolute precision of 10%. We report the procedures that are used in order to obtain such precision, and a discussion is presented to address the expected performance of the technique when applied to heavier materials. The results we obtain do not depend on the specific type of material considered and therefore they can be extended to any application.

Photoconductivity in Dirac materials

NASA Astrophysics Data System (ADS)

Shao, J. M.; Yang, G. W.

2015-11-01

Two-dimensional (2D) Dirac materials including graphene and the surface of a three-dimensional (3D) topological insulator, and 3D Dirac materials including 3D Dirac semimetal and Weyl semimetal have attracted great attention due to their linear Dirac nodes and exotic properties. Here, we use the Fermi's golden rule and Boltzmann equation within the relaxation time approximation to study and compare the photoconductivity of Dirac materials under different far- or mid-infrared irradiation. Theoretical results show that the photoconductivity exhibits the anisotropic property under the polarized irradiation, but the anisotropic strength is different between 2D and 3D Dirac materials. The photoconductivity depends strongly on the relaxation time for different scattering mechanism, just like the dark conductivity.

Spoof surface plasmon based planar antennas for the realization of Terahertz hotspots

PubMed Central

Zhang, Yusheng; Han, Zhanghua

2015-01-01

Novel spoof surface plasmon based terahertz (THz) antennas are realized using a few number of rectangular grooves perforated in ultrathin metal stripes and the properties of them, including both scattering cross sections and field enhancement, are numerically analyzed. The dependence of these properties on the incident angle and groove number is discussed and the results show that sharp resonances in scattering cross section spectra associated with strong local field enhancement can be achieved. These resonances are due to the formation of Fabry-Perot resonances of the spoof surface plasmon mode and it is found that the order of resonance exhibiting strongest field enhancements is found to coincide with the number of grooves at normal incidence, due to hybridization of the antenna resonance with the individual groove resonance. The terahertz hotspots within the grooves at resonances due to the local field enhancement may open up new possibilities for the investigation of terahertz-matter interactions and boost a variety of THz applications including novel sensing and THz detections. The planar stripe antennas with sharper resonances than dipolar-like resonances, together with their ease of fabrication may also promise new design methodology for metamaterials. PMID:26691003

Electromagnetic properties of material coated surfaces

NASA Technical Reports Server (NTRS)

Beard, L.; Berrie, J.; Burkholder, R.; Dominek, A.; Walton, E.; Wang, N.

1989-01-01

The electromagnetic properties of material coated conducting surfaces were investigated. The coating geometries consist of uniform layers over a planar surface, irregularly shaped formations near edges and randomly positioned, electrically small, irregularly shaped formations over a surface. Techniques to measure the scattered field and constitutive parameters from these geometries were studied. The significance of the scattered field from these geometries warrants further study.

Application of spatially modulated near-infrared structured light to study changes in optical properties of mouse brain tissue during heatstress.

PubMed

Shaul, Oren; Fanrazi-Kahana, Michal; Meitav, Omri; Pinhasi, Gad A; Abookasis, David

2017-11-10

Heat stress (HS) is a medical emergency defined by abnormally elevated body temperature that causes biochemical, physiological, and hematological changes. The goal of the present research was to detect variations in optical properties (absorption, reduced scattering, and refractive index coefficients) of mouse brain tissue during HS by using near-infrared (NIR) spatial light modulation. NIR spatial patterns with different spatial phases were used to differentiate the effects of tissue scattering from those of absorption. Decoupling optical scattering from absorption enabled the quantification of a tissue's chemical constituents (related to light absorption) and structural properties (related to light scattering). Technically, structured light patterns at low and high spatial frequencies of six wavelengths ranging between 690 and 970 nm were projected onto the mouse scalp surface while diffuse reflected light was recorded by a CCD camera positioned perpendicular to the mouse scalp. Concurrently to pattern projection, brain temperature was measured with a thermal camera positioned slightly off angle from the mouse head while core body temperature was monitored by thermocouple probe. Data analysis demonstrated variations from baseline measurements in a battery of intrinsic brain properties following HS.

Monitoring of tissue optical properties using OCT: application for blood glucose analysis

NASA Astrophysics Data System (ADS)

Larin, Kirill V.; Eledrisi, Mohsen S.; Ashitkov, Taras V.; Motamedi, Massoud; Esenaliev, Rinat O.

2002-07-01

Noninvasive monitoring of tissue optical properties in real time could significantly improve diagnostics and management of various diseases. Recently we proposed to use high- resolution Optical Coherence Tomography (OCT) technique for measurement of tissue scattering coefficient at the depth of up to 1mm. Our pilot studies performed in vitro and in vivo demonstrated that measurement of tissue scattering with this technique can potentially be applied for noninvasive monitoring of blood glucose concentration. High resolution and coherent photon detection of the OCT technique allowed detection of glucose-induced changes in the scattering coefficient. In this paper we report results of in vivo studies performed in dog, New Zealand rabbits, and first human subjects. OCT system with the wavelength of 1300 nm was used in our experiments. OCT signal slope was measured and compared with actual blood glucose concentration. Bolus glucose injections and glucose clamping administrations were used in animal studies. OCT signals were recorded form human subjects during oral glucose tolerance test. Results obtained form both animal and human studies show good correlation between slope of the OCT signals and actual blood glucose concentration measured using standard glucometesr. Sensitivity and accuracy of blood glucose concentrations monitoring with the OCT is discussed. Obtained result suggest that OCT is a promising technique for noninvasive monitoring of tissue analytes including glucose.

Dynamics of hard sphere colloidal dispersions

NASA Technical Reports Server (NTRS)

Zhu, J. X.; Chaikin, Paul M.; Phan, S.-E.; Russel, W. B.

1994-01-01

Our objective is to perform on homogeneous, fully equilibrated dispersions the full set of experiments characterizing the transition from fluid to solid and the properties of the crystalline and glassy solid. These include measurements quantifying the nucleation and growth of crystallites, the structure of the initial fluid and the fully crystalline solid, and Brownian motion of particles within the crystal, and the elasticity of the crystal and the glass. Experiments are being built and tested for ideal microgravity environment. Here we describe the ground based effort, which exploits a fluidized bed to create a homogeneous, steady dispersion for the studies. The differences between the microgravity environment and the fluidized bed is gauged by the Peclet number Pe, which measures the rate of convection/sedimentation relative to Brownian motion. We have designed our experiment to accomplish three types of measurements on hard sphere suspensions in a fluidized bed: the static scattering intensity as a function of angle to determine the structure factor, the temporal autocorrelation function at all scattering angles to probe the dynamics, and the amplitude of the response to an oscillatory forcing to deduce the low frequency viscoelasticity. Thus the scattering instrument and the colloidal dispersion were chosen such as that the important features of each physical property lie within the detectable range for each measurement.

Short-Range Order and Collective Dynamics of DMPC Bilayers: A Comparison between Molecular Dynamics Simulations, X-Ray, and Neutron Scattering Experiments

PubMed Central

Hub, Jochen S.; Salditt, Tim; Rheinstädter, Maikel C.; de Groot, Bert L.

2007-01-01

We present an extensive comparison of short-range order and short wavelength dynamics of a hydrated phospholipid bilayer derived by molecular dynamics simulations, elastic x-ray, and inelastic neutron scattering experiments. The quantities that are compared between simulation and experiment include static and dynamic structure factors, reciprocal space mappings, and electron density profiles. We show that the simultaneous use of molecular dynamics and diffraction data can help to extract real space properties like the area per lipid and the lipid chain ordering from experimental data. In addition, we assert that the interchain distance can be computed to high accuracy from the interchain correlation peak of the structure factor. Moreover, it is found that the position of the interchain correlation peak is not affected by the area per lipid, while its correlation length decreases linearly with the area per lipid. This finding allows us to relate a property of the structure factor quantitatively to the area per lipid. Finally, the short wavelength dynamics obtained from the simulations and from inelastic neutron scattering are analyzed and compared. The conventional interpretation in terms of the three-effective-eigenmode model is found to be only partly suitable to describe the complex fluid dynamics of lipid chains. PMID:17631531

Behavior of optical properties of coagulated blood sample at 633 nm wavelength

NASA Astrophysics Data System (ADS)

Morales Cruzado, Beatriz; Vázquez y Montiel, Sergio; Delgado Atencio, José Alberto

2011-03-01

Determination of tissue optical parameters is fundamental for application of light in either diagnostics or therapeutical procedures. However, in samples of biological tissue in vitro, the optical properties are modified by cellular death or cellular agglomeration that can not be avoided. This phenomena change the propagation of light within the biological sample. Optical properties of human blood tissue were investigated in vitro at 633 nm using an optical setup that includes a double integrating sphere system. We measure the diffuse transmittance and diffuse reflectance of the blood sample and compare these physical properties with those obtained by Monte Carlo Multi-Layered (MCML). The extraction of the optical parameters: absorption coefficient μa, scattering coefficient μs and anisotropic factor g from the measurements were carried out using a Genetic Algorithm, in which the search procedure is based in the evolution of a population due to selection of the best individual, evaluated by a function that compares the diffuse transmittance and diffuse reflectance of those individuals with the experimental ones. The algorithm converges rapidly to the best individual, extracting the optical parameters of the sample. We compare our results with those obtained by using other retrieve procedures. We found that the scattering coefficient and the anisotropic factor change dramatically due to the formation of clusters.

Low angle light scattering analysis: a novel quantitative method for functional characterization of human and murine platelet receptors.

PubMed

Mindukshev, Igor; Gambaryan, Stepan; Kehrer, Linda; Schuetz, Claudia; Kobsar, Anna; Rukoyatkina, Natalia; Nikolaev, Viacheslav O; Krivchenko, Alexander; Watson, Steve P; Walter, Ulrich; Geiger, Joerg

2012-07-01

Determinations of platelet receptor functions are indispensable diagnostic indicators of cardiovascular and hemostatic diseases including hereditary and acquired receptor defects and receptor responses to drugs. However, presently available techniques for assessing platelet function have some disadvantages, such as low sensitivity and the requirement of large sample sizes and unphysiologically high agonist concentrations. Our goal was to develop and initially characterize a new technique designed to quantitatively analyze platelet receptor activation and platelet function on the basis of measuring changes in low angle light scattering. We developed a novel technique based on low angle light scattering registering changes in light scattering at a range of different angles in platelet suspensions during activation. The method proved to be highly sensitive for simultaneous real time detection of changes in size and shape of platelets during activation. Unlike commonly-used methods, the light scattering method could detect platelet shape change and aggregation in response to nanomolar concentrations of extracellular nucleotides. Furthermore, our results demonstrate that the advantages of the light scattering method make it a choice method for platelet receptor monitoring and for investigation of both murine and human platelets in disease models. Our data demonstrate the suitability and superiority of this new low angle light scattering method for comprehensive analyses of platelet receptors and functions. This highly sensitive, quantitative, and online detection of essential physiological, pathophysiological and pharmacological-response properties of human and mouse platelets is a significant improvement over conventional techniques.

A new theory for X-ray diffraction

PubMed Central

Fewster, Paul F.

2014-01-01

This article proposes a new theory of X-ray scattering that has particular relevance to powder diffraction. The underlying concept of this theory is that the scattering from a crystal or crystallite is distributed throughout space: this leads to the effect that enhanced scatter can be observed at the ‘Bragg position’ even if the ‘Bragg condition’ is not satisfied. The scatter from a single crystal or crystallite, in any fixed orientation, has the fascinating property of contributing simultaneously to many ‘Bragg positions’. It also explains why diffraction peaks are obtained from samples with very few crystallites, which cannot be explained with the conventional theory. The intensity ratios for an Si powder sample are predicted with greater accuracy and the temperature factors are more realistic. Another consequence is that this new theory predicts a reliability in the intensity measurements which agrees much more closely with experimental observations compared to conventional theory that is based on ‘Bragg-type’ scatter. The role of dynamical effects (extinction etc.) is discussed and how they are suppressed with diffuse scattering. An alternative explanation for the Lorentz factor is presented that is more general and based on the capture volume in diffraction space. This theory, when applied to the scattering from powders, will evaluate the full scattering profile, including peak widths and the ‘background’. The theory should provide an increased understanding of the reliability of powder diffraction measurements, and may also have wider implications for the analysis of powder diffraction data, by increasing the accuracy of intensities predicted from structural models. PMID:24815975

Synchrotron x-ray thermal diffuse scattering probes for phonons in Si/SiGe/Si trilayer nanomembranes

DOE PAGES

McElhinny, Kyle M.; Gopalakrishnan, Gokul; Savage, Donald E.; ...

2016-05-17

Nanostructures offer the opportunity to control the vibrational properties of via the scattering of phonons due to boundaries and mass disorder as well as through changes in the phonon dispersion due to spatial confinement. Advances in understanding these effects have the potential to lead to thermoelectrics with an improved figure of merit by lowering the thermal conductivity and to provide insight into electron-phonon scattering rates in nanoelectronics. However, characterizing the phonon population in nanomaterials has been challenging because of their small volume and because optical techniques probe only a small fraction of reciprocal space. Recent developments in x-ray scattering nowmore » allow the phonon population to be evaluated across all of reciprocal space in samples with volumes as small as several cubic micrometers. We apply this approach, synchrotron x-ray thermal diffuse scattering (TDS), to probe the population of phonons within a Si/SiGe/Si trilayer nanomembrane. The distributions of scattered intensity from Si/SiGe/Si trilayer nanomembranes and Si nanomembranes with uniform composition are qualitatively similar, with features arising from the elastic anisotropy of the diamond structure. The TDS signal for the Si/SiGe/Si nanomembrane, however, has higher intensity than the Si membrane of the same total thickness by approximately 3.75%. Possible origins of the enhancement in scattering from SiGe in comparison with Si include the larger atomic scattering factor of Ge atoms within the SiGe layer or reduced phonon frequencies due to alloying.« less

Static and dynamic light scattering of healthy and malaria-parasite invaded red blood cells

NASA Astrophysics Data System (ADS)

Park, Yongkeun; Diez-Silva, Monica; Fu, Dan; Popescu, Gabriel; Choi, Wonshik; Barman, Ishan; Suresh, Subra; Feld, Michael S.

2010-03-01

We present the light scattering of individual Plasmodium falciparum-parasitized human red blood cells (Pf-RBCs), and demonstrate progressive alterations to the scattering signal arising from the development of malaria-inducing parasites. By selectively imaging the electric fields using quantitative phase microscopy and a Fourier transform light scattering technique, we calculate the light scattering maps of individual Pf-RBCs. We show that the onset and progression of pathological states of the Pf-RBCs can be clearly identified by the static scattering maps. Progressive changes to the biophysical properties of the Pf-RBC membrane are captured from dynamic light scattering.

Solid-State Division progress report for period ending March 31, 1983

DOE Office of Scientific and Technical Information (OSTI.GOV)

Green, P.H.; Watson, D.M.

1983-09-01

Progress and activities are reported on: theoretical solid-state physics (surfaces; electronic, vibrational, and magnetic properties; particle-solid interactions; laser annealing), surface and near-surface properties of solids (surface, plasma-material interactions, ion implantation and ion-beam mixing, pulsed-laser and thermal processing), defects in solids (radiation effects, fracture, impurities and defects, semiconductor physics and photovoltaic conversion), transport properties of solids (fast-ion conductors, superconductivity, mass and charge transport in materials), neutron scattering (small-angle scattering, lattice dynamics, magnetic properties, structure and instrumentation), and preparation and characterization of research materials (growth and preparative methods, nuclear waste forms, special materials). (DLC)

An effective field theory for forward scattering and factorization violation

DOE PAGES

Rothstein, Ira Z.; Stewart, Iain W.

2016-08-03

Starting with QCD, we derive an effective field theory description for forward scattering and factorization violation as part of the soft-collinear effective field theory (SCET) for high energy scattering. These phenomena are mediated by long distance Glauber gluon exchanges, which are static in time, localized in the longitudinal distance, and act as a kernel for forward scattering where |t| << s. In hard scattering, Glauber gluons can induce corrections which invalidate factorization. With SCET, Glauber exchange graphs can be calculated explicitly, and are distinct from graphs involving soft, collinear, or ultrasoft gluons. We derive a complete basis of operators whichmore » describe the leading power effects of Glauber exchange. Key ingredients include regulating light-cone rapidity singularities and subtractions which prevent double counting. Our results include a novel all orders gauge invariant pure glue soft operator which appears between two collinear rapidity sectors. The 1-gluon Feynman rule for the soft operator coincides with the Lipatov vertex, but it also contributes to emissions with ≥ 2 soft gluons. Our Glauber operator basis is derived using tree level and one-loop matching calculations from full QCD to both SCET II and SCET I. The one-loop amplitude’s rapidity renormalization involves mixing of color octet operators and yields gluon Reggeization at the amplitude level. The rapidity renormalization group equation for the leading soft and collinear functions in the forward scattering cross section are each given by the BFKL equation. Various properties of Glauber gluon exchange in the context of both forward scattering and hard scattering factorization are described. For example, we derive an explicit rule for when eikonalization is valid, and provide a direct connection to the picture of multiple Wilson lines crossing a shockwave. In hard scattering operators Glauber subtractions for soft and collinear loop diagrams ensure that we are not sensitive to the directions for soft and collinear Wilson lines. Conversely, certain Glauber interactions can be absorbed into these soft and collinear Wilson lines by taking them to be in specific directions. Finally, we also discuss criteria for factorization violation.« less

The Western Hemisphere of Venus: 3.5 CM Dual Circular-Polarization Radar Images

NASA Astrophysics Data System (ADS)

Haldemann, Albert F. C.; Muhleman, Duane O.; Butler, Bryan J.; Slade, Martin A.

1997-08-01

We present new dual circular-polarization radar maps of the western hemisphere of Venus. The results are from a 1993 experiment imaging Venus with 3.5 cm radar. Continuous-wave right circularly polarized flux was transmitted toward Venus from the 70 m Deep Space Network antenna in Goldstone, California. The echo was received in both the same sense (SS) and the opposite sense (OS) of circular polarization at the Very Large Array in New Mexico. By spatially reconstructing the echo with the interferometer, maps of Venusian radar albedo were made for each of two days of observation in both OS (echo principally due to specular reflection) and SS (diffuse echo) channels. On both days, the sub-earth longitude was near 300 E. The SS maps are dominated by a significant component of diffuse backscatter from the 285 E longitude highlands: Beta, Phoebe, and Themis Regiones. Beta Regio includes radar-anomalous regions with high reflectivity and low emissivity. The nature of these altitude-related electrical properties on Venus is one of the outstanding surface process questions that remain after Magellan. Our experiment adds the first full-disk polarization ratio (μc) maps to the discussion. The data show that different geology determines different radar scattering properties within Beta. Diffuse scattering is very important in Beta, and may be due to either surface or volume scattering. We find a strong correlation of the SS albedo σSSwith altitudeRp(km) in Beta, σSS∝ 0.3Rp. Also, σOS∝ 0.7Rp. The onset of this relationship is at theRp∼ 6054 km planetary radius contour. The nature and morphology of the highland radar anomalies in Beta is consistent with a diffuse scattering mechanism. In Beta Regio we find μc> 0.5 in general, with μcas high as 0.8 between Rhea and Theia Montes, to the west of Devana Chasma. These values are compatible with measurements of blocky terrestrial lava flows if surface scattering dominates. If volume scattering is important, the high RCP cross-sections may indicate an important decrease in embedded scatterer size with altitude, which could be related to enhanced weathering.

Initial characterization of mudstone nanoporosity with small angle neutron scattering using caprocks from carbon sequestration sites.

DOE Office of Scientific and Technical Information (OSTI.GOV)

McCray, John; Navarre-Sitchler, Alexis; Mouzakis, Katherine

Geological carbon sequestration relies on the principle that CO{sub 2} injected deep into the subsurface is unable to leak to the atmosphere. Structural trapping by a relatively impermeable caprock (often mudstone such as a shale) is the main trapping mechanism that is currently relied on for the first hundreds of years. Many of the pores of the caprock are of micrometer to nanometer scale. However, the distribution, geometry and volume of porosity at these scales are poorly characterized. Differences in pore shape and size can cause variation in capillary properties and fluid transport resulting in fluid pathways with different capillarymore » entry pressures in the same sample. Prediction of pore network properties for distinct geologic environments would result in significant advancement in our ability to model subsurface fluid flow. Specifically, prediction of fluid flow through caprocks of geologic CO{sub 2} sequestration reservoirs is a critical step in evaluating the risk of leakage to overlying aquifers. The micro- and nanoporosity was analyzed in four mudstones using small angle neutron scattering (SANS). These mudstones are caprocks of formations that are currently under study or being used for carbon sequestration projects and include the Marine Tuscaloosa Group, the Lower Tuscaloosa Group, the upper and lower shale members of the Kirtland Formation, and the Pennsylvanian Gothic shale. Total organic carbon varies from <0.3% to 4% by weight. Expandable clay contents range from 10% to {approx}40% in the Gothic shale and Kirtland Formation, respectively. Neutrons effectively scatter from interfaces between materials with differing scattering length density (i.e. minerals and pores). The intensity of scattered neutrons, I(Q), where Q is the scattering vector, gives information about the volume of pores and their arrangement in the sample. The slope of the scattering data when plotted as log I(Q) vs. log Q provides information about the fractality or geometry of the pore network. Results from this study, combined with high-resolution TEM imaging, provide insight into the differences in volume and geometry of porosity between these various mudstones.« less

The Effect of Sub-Aperture in DRIA Framework Applied on Multi-Aspect PolSAR Data

NASA Astrophysics Data System (ADS)

Xue, Feiteng; Yin, Qiang; Lin, Yun; Hong, Wen

2016-08-01

Multi-aspect SAR is a new remote sensing technology, achieves consecutive data in large look angle as platform moves. Multi- aspect observation brings higher resolution and SNR to SAR picture. Multi-aspect PolSAR data can increase the accuracy of target identify and classification because it contains the 3-D polarimetric scattering properties.DRIA(detecting-removing-incoherent-adding)framework is a multi-aspect PolSAR data processing method. In this method, the anisotropic and isotropic scattering is separated by maximum- likelihood ratio test. The anisotropic scattering is removed to gain a removal series. The isotropic scattering is incoherent added to gain a high resolution picture. The removal series describes the anisotropic scattering property and is used in features extraction and classification.This article focuses on the effect brought by difference of sub-aperture numbers in anisotropic scattering detection and removal. The more sub-apertures are, the less look angle is. Artificial target has anisotropic scattering because of Bragg resonances. The increase of sub-aperture number brings more accurate observation in azimuth though the quality of each single image may loss. The accuracy of classification in agricultural fields is affected by the anisotropic scattering brought by Bragg resonances. The size of the sub-aperture has a significant effect in the removal result of Bragg resonances.

Characterization of the Optical Properties of Turbid Media by Supervised Learning of Scattering Patterns.

PubMed

Hassaninia, Iman; Bostanabad, Ramin; Chen, Wei; Mohseni, Hooman

2017-11-10

Fabricated tissue phantoms are instrumental in optical in-vitro investigations concerning cancer diagnosis, therapeutic applications, and drug efficacy tests. We present a simple non-invasive computational technique that, when coupled with experiments, has the potential for characterization of a wide range of biological tissues. The fundamental idea of our approach is to find a supervised learner that links the scattering pattern of a turbid sample to its thickness and scattering parameters. Once found, this supervised learner is employed in an inverse optimization problem for estimating the scattering parameters of a sample given its thickness and scattering pattern. Multi-response Gaussian processes are used for the supervised learning task and a simple setup is introduced to obtain the scattering pattern of a tissue sample. To increase the predictive power of the supervised learner, the scattering patterns are filtered, enriched by a regressor, and finally characterized with two parameters, namely, transmitted power and scaled Gaussian width. We computationally illustrate that our approach achieves errors of roughly 5% in predicting the scattering properties of many biological tissues. Our method has the potential to facilitate the characterization of tissues and fabrication of phantoms used for diagnostic and therapeutic purposes over a wide range of optical spectrum.

Elastic scattering spectroscopy of coagulated brain tissues

NASA Astrophysics Data System (ADS)

Ateş, Filiz; Tabakoğlu, Haşim Özgür; Bozkulak, Özgüncem; Canpolat, Murat; Gülsoy, Murat

2006-02-01

The goal of this study was to differentiate the parts of lamb brain according to elastic scattering spectroscopy and detect the optical alterations due to coagulation. Cells and tissues are not uniform and have complex structures and shapes. They can be referred to as scattering particles. The process of scattering depends on the light wavelength and on the scattering medium properties; especially on the size and the density of the medium. When elastic scattering spectroscopy (ESS) is employed, the morphological alterations of tissues can be detected using spectral measurements of the elastic scattered light over a wide range of wavelengths. In this study firstly, the slopes of ESS spectra were used to differentiate the parts of lamb brains (brainstem, cerebellum, gray matter, white matter) in vitro in the range of 450 - 750 nm. Secondly, tissues were coagulated at different temperatures (45, 60, and 80 °C) and ESS spectra were taken from native and coagulated tissues. It was observed that as the coagulation temperature increased, the slope of the elastic scattering spectra decreased. Thus, optical properties of tissues were changed with respect to the change in nuclear to cytoplasmic ratio due to the water loss. Results showed that the slopes of ESS spectra in the visible range revealed valuable information about the morphological changes caused by coagulation.

Diurnal Cycles of Aerosol Optical Properties at Pico Tres Padres, Mexico City: Evidences for Changes in Particle Morphology and Secondary Aerosol Formation

NASA Astrophysics Data System (ADS)

Mazzoleni, C.; Dubey, M.; Chakrabarty, R.; Moosmuller, H.; Onasch, T.; Zavala, M.; Herndon, S.; Kolb, C.

2007-12-01

Aerosol optical properties affect planetary radiative balance and depend on chemical composition, size distribution, and morphology. During the MILAGRO field campaign, we measured aerosol absorption and scattering in Mexico City using the Los Alamos aerosol photoacoustic (LAPA) instrument operating at 781 nm. The LAPA was mounted on-board the Aerodyne Research Inc. mobile laboratory, which hosted a variety of gaseous and aerosol instruments. During the campaign, the laboratory was moved to different sites, capturing spatial and temporal variability. Additionally, we collected ambient aerosols on Nuclepore filters for scanning electron microscopy (SEM) analysis. SEM images of selected filters were taken to study particle morphology. Between March 7th and 19th air was sampled at the top of Pico Tres Padres, a mountain on the north side of Mexico City. Aerosol absorption and scattering followed diurnal patterns related to boundary layer height and solar insulation. We report an analysis of aerosol absorption, scattering, and morphology for three days (9th, 11th and 12th of March 2006). The single scattering albedo (SSA, ratio of scattering to total extinction) showed a drop in the tens-of-minutes-to-hour time frame after the boundary layer grew above the sampling site. Later in the day the SSA rose steadily reaching a maximum in the afternoon. The SEM images showed a variety of aerosol shapes including fractal-like aggregates, spherical particles, and other shapes. The absorption correlated with the CO2 signal and qualitatively with the fraction of fractal-like particles to the total particle count. In the afternoon the SSA qualitatively correlated with a relative increase in spherical particles and total particle count. These observed changes in optical properties and morphology can be explained by the dominant contribution of freshly emitted particles in the morning and by secondary particle formation in the afternoon. SSA hourly averaged values ranged from ~0.63 in the morning to ~0.83 in the afternoon/night, indicating light absorbing aerosols, which have a large impact on radiative forcing.

Radiative Properties of Cirrus Clouds in the Infrared (8-13 microns) Spectral Region

NASA Technical Reports Server (NTRS)

Yang, Ping; Gao, Bo-Cai; Baum, Bryan A.; Hu, Yong X.; Wiscombe, Warren J.; Tsay, Si-Chee; Winker, Dave M.; Einaudi, Franco (Technical Monitor)

2000-01-01

Atmospheric radiation in the infrared (IR) 8-13 microns spectral region contains a wealth of information that is very useful for the retrieval of ice cloud properties from aircraft or space-borne measurements. To provide the scattering and absorption properties of nonspherical ice crystals that are fundamental to the IR retrieval implementation, we use the finite-difference time domain (FDTD) method to solve for the extinction efficiency, single-scattering albedo, and the asymmetry parameter of the phase function for ice crystals smaller than 40 microns. For particles larger than this size, the improved geometric optics method (IGOM) can be employed to calculate the asymmetry parameter with an acceptable accuracy, provided that we properly account for the inhomogeneity of the refracted wave due to strong absorption inside the ice particle. A combination of the results computed from the two methods provides the asymmetry parameter for the entire practical range of particle sizes between 1 micron and 10000 microns over wavelengths ranging from 8 microns to 13 microns. For the extinction and absorption efficiency calculations, several methods including the IGOM, Mie solution for equivalent spheres (MSFES), and the anomalous diffraction theory (ADT) can lead to a substantial discontinuity in comparison with the FDTD solutions for particle sizes on the order of 40 microns. To overcome this difficulty, we have developed a novel approach called the stretched scattering potential method (SSPM). For the IR 8-13 microns spectral region, we show that SSPM is a more accurate approximation than ADT, MSFES, and IGOM. The SSPM solution can be further refined numerically. Through a combination of the FDTD and SSPM, we have computed the extinction and absorption efficiency for hexagonal ice crystals with sizes ranging from 1 to 10000 microns at 12 wavelengths between 8 and 13 microns Calculations of the cirrus bulk scattering and absorption properties are performed for 30 size distributions obtained from various field campaigns for midlatitude and tropical cirrus cloud systems. Parameterization of these bulk scattering properties is carried out by using second-order polynomial functions for the extinction efficiency and the single-scattering albedo and the power law expression for the asymmetry parameter. We note that the volume-normalized extinction coefficient can be separated into two parts: one is inversely proportional to effective size and is independent of wavelength, and the other is the wavelength-dependent effective extinction efficiency. Unlike conventional parameterization efforts, the present parameterization scheme is more accurate because only the latter part of the volume-normalized extinction coefficient is approximated in terms of an analytical expression. After averaging over size distribution, the single-scattering albedo is shown to decrease with an increase in effective size for wavelengths shorter than 10.0 microns whereas the opposite behavior is observed for longer wavelengths. The variation of the asymmetry parameter as a function of effective size is substantial when the effective size is smaller than 50 microns. For effective sizes larger than 100 microns, the asymmetry parameter approaches its asymptotic value. The results derived in this study can be useful to remote sensing applications involving IR window bands under cirrus cloud conditions.

Characterization of target camouflage structures by means of different microwave imaging procedures

NASA Astrophysics Data System (ADS)

Inaebnit, Christian; John, Marc-Andre; Aulenbacher, Uwe; Akyol, Zeynrep; Hueppi, Rudolf; Wellig, Peter

2009-05-01

This paper presents two different test methods for camouflage layers (CL) like nets or foam based structures. The effectiveness of CL in preventing radar detection and recognition of targets depends on the interaction of CL properties as absorption and diffuse scattering with target specific scattering properties. This fact is taken into account by representing target backscattering as interference of different types of GTD contributions and evaluating the impact of CL onto these individual contributions separately. The first method investigates how a CL under test alters these individual scattering contributions and which "new" contributions are produced by "self-scattering" at the CL. This information is gained by applying ISAR imaging technique to a test structure with different types of scattering contributions. The second test method aims for separating the effects of absorption and "diffuse scattering" in case of a planar metallic plate covered by CL. For this, the equivalent source distribution in the plane of the CL is reconstructed from bistatic scattering data. Both test methods were verified by experimental results obtained from X-band measurements at different CL and proved to be well suited for an application specific evaluation of camouflage structures from different manufacturers.

LiquidLib: A comprehensive toolbox for analyzing classical and ab initio molecular dynamics simulations of liquids and liquid-like matter with applications to neutron scattering experiments

NASA Astrophysics Data System (ADS)

Walter, Nathan P.; Jaiswal, Abhishek; Cai, Zhikun; Zhang, Yang

2018-07-01

Neutron scattering is a powerful experimental technique for characterizing the structure and dynamics of materials on the atomic or molecular scale. However, the interpretation of experimental data from neutron scattering is oftentimes not trivial, partly because scattering methods probe ensemble-averaged information in the reciprocal space. Therefore, computer simulations, such as classical and ab initio molecular dynamics, are frequently used to unravel the time-dependent atomistic configurations that can reproduce the scattering patterns and thus assist in the understanding of the microscopic origin of certain properties of materials. LiquidLib is a post-processing package for analyzing the trajectory of atomistic simulations of liquids and liquid-like matter with application to neutron scattering experiments. From an atomistic simulation, LiquidLib provides the computation of various statistical quantities including the pair distribution function, the weighted and unweighted structure factors, the mean squared displacement, the non-Gaussian parameter, the four-point correlation function, the velocity auto correlation function, the self and collective van Hove correlation functions, the self and collective intermediate scattering functions, and the bond orientational order parameter. LiquidLib analyzes atomistic trajectories generated from packages such as LAMMPS, GROMACS, and VASP. It also offers an extendable platform to conveniently integrate new quantities into the library and integrate simulation trajectories of other file formats for analysis. Weighting the quantities by element-specific neutron-scattering lengths provides results directly comparable to neutron scattering measurements. Lastly, LiquidLib is independent of dimensionality, which allows analysis of trajectories in two, three, and higher dimensions. The code is beginning to find worldwide use.

Temperature Distribution in a Composite of Opaque and Semitransparent Spectral Layers

NASA Technical Reports Server (NTRS)

Siegel, Robert

1997-01-01

The analysis of radiative transfer becomes computationally complex for a composite when there are multiple layers and multiple spectral bands. A convenient analytical method is developed for combined radiation and conduction in a composite of alternating semitransparent and opaque layers. The semi- transparent layers absorb, scatter, and emit radiation, and spectral properties with large scattering are included. The two-flux method is used, and its applicability is verified by comparison with a basic solution in the literature. The differential equation in the two-flux method Is solved by deriving a Green's function. The solution technique is applied to analyze radiation effects in a multilayer zirconia thermal barrier coating with internal radiation shields for conditions in an aircraft engine combustor. The zirconia radiative properties are modeled by two spectral bands. Thin opaque layers within the coating are used to decrease radiant transmission that can degrade the zirconia insulating ability. With radiation shields, the temperature distributions more closely approach the opaque limit that provides the lowest metal wall temperatures.

Applications of the similarity relations in radiative transfer to remote sensing implementation and flux simulation

NASA Astrophysics Data System (ADS)

Yang, P.; Ding, J.; Tang, G.; King, M. D.; Platnick, S. E.; Meyer, K.; Mlawer, E. J.

2017-12-01

Van de Hulst (1974) showed several quasi-invariant quantities in radiative transfer concerning multiple scattering. Recently, we illustrated that the aforesaid quasi-invariant quantities are useful in remote sensing of ice cloud properties from spaceborne radiometric observations (Ding et al. 2017). Specifically, the overall performance of an ice cloud optical property model can be estimated without carrying out detailed retrieval implementation. In this presentation, we will review the radiative transfer similarity relations and some recent results including the study by Ding et al. (2017). Furthermore, we will illustrate an application of the similarity relations to improvement of broadband radiative flux computation. For example, the Rapid Radiative Transfer Model (RRTM, Mlawer et al, 1999) does not consider multiple scattering in the longwave spectral regime (RRTMG-LW) ("G" indicates a version suitable for GCM applications). We show that the similarity relations can be used to effectively improve the accuracy of RRTMG-LW without increasing computational effort.

Transport properties of random media: A new effective medium theory

DOE Office of Scientific and Technical Information (OSTI.GOV)

Busch, K.; Soukoulis, C.M.

We present a new method for efficient, accurate calculations of transport properties of random media. It is based on the principle that the wave energy density should be uniform when averaged over length scales larger than the size of the scatterers. This scheme captures the effects of resonant scattering of the individual scatterer exactly, as well as the multiple scattering in a mean-field sense. It has been successfully applied to both ``scalar`` and ``vector`` classical wave calculations. Results for the energy transport velocity are in agreement with experiment. This approach is of general use and can be easily extended tomore » treat different types of wave propagation in random media. {copyright} {ital 1995} {ital The} {ital American} {ital Physical} {ital Society}.« less

Scattering analysis of LOFAR pulsar observations

NASA Astrophysics Data System (ADS)

Geyer, M.; Karastergiou, A.; Kondratiev, V. I.; Zagkouris, K.; Kramer, M.; Stappers, B. W.; Grießmeier, J.-M.; Hessels, J. W. T.; Michilli, D.; Pilia, M.; Sobey, C.

2017-09-01

We measure the effects of interstellar scattering on average pulse profiles from 13 radio pulsars with simple pulse shapes. We use data from the LOFAR High Band Antennas, at frequencies between 110 and 190 MHz. We apply a forward fitting technique, and simultaneously determine the intrinsic pulse shape, assuming single Gaussian component profiles. We find that the constant τ, associated with scattering by a single thin screen, has a power-law dependence on frequency τ ∝ ν-α, with indices ranging from α = 1.50 to 4.0, despite simplest theoretical models predicting α = 4.0 or 4.4. Modelling the screen as an isotropic or extremely anisotropic scatterer, we find anisotropic scattering fits lead to larger power-law indices, often in better agreement with theoretically expected values. We compare the scattering models based on the inferred, frequency-dependent parameters of the intrinsic pulse, and the resulting correction to the dispersion measure (DM). We highlight the cases in which fits of extreme anisotropic scattering are appealing, while stressing that the data do not strictly favour either model for any of the 13 pulsars. The pulsars show anomalous scattering properties that are consistent with finite scattering screens and/or anisotropy, but these data alone do not provide the means for an unambiguous characterization of the screens. We revisit the empirical τ versus DM relation and consider how our results support a frequency dependence of α. Very long baseline interferometry, and observations of the scattering and scintillation properties of these sources at higher frequencies, will provide further evidence.

EXTINCTION LAWS TOWARD STELLAR SOURCES WITHIN A DUSTY CIRCUMSTELLAR MEDIUM AND IMPLICATIONS FOR TYPE IA SUPERNOVAE

DOE Office of Scientific and Technical Information (OSTI.GOV)

Nagao, Takashi; Maeda, Keiichi; Nozawa, Takaya, E-mail: nagao@kusastro.kyoto-u.ac.jp

Many astronomical objects are surrounded by dusty environments. In such dusty objects, multiple scattering processes of photons by circumstellar (CS) dust grains can effectively alter extinction properties. In this paper, we systematically investigate the effects of multiple scattering on extinction laws for steady-emission sources surrounded by the dusty CS medium using a radiation transfer simulation based on the Monte Carlo technique. In particular, we focus on whether and how the extinction properties are affected by properties of CS dust grains by adopting various dust grain models. We confirm that behaviors of the (effective) extinction laws are highly dependent on themore » properties of CS grains, especially the total-to-selective extinction ratio R{sub V}, which characterizes the extinction law and can be either increased or decreased and compared with the case without multiple scattering. We find that the criterion for this behavior is given by a ratio of albedos in the B and V bands. We also find that either small silicate grains or polycyclic aromatic hydrocarbons are necessary for realizing a low value of R{sub V} as often measured toward SNe Ia if the multiple scattering by CS dust is responsible for their non-standard extinction laws. Using the derived relations between the properties of dust grains and the resulting effective extinction laws, we propose that the extinction laws toward dusty objects could be used to constrain the properties of dust grains in CS environments.« less

Study the effects of varying interference upon the optical properties of turbid samples using NIR spatial light modulation

NASA Astrophysics Data System (ADS)

Shaul, Oren; Fanrazi-Kahana, Michal; Meitav, Omri; Pinhasi, Gad A.; Abookasis, David

2018-03-01

Optical properties of biological tissues are valuable diagnostic parameters which can provide necessary information regarding tissue state during disease pathogenesis and therapy. However, different sources of interference, such as temperature changes may modify these properties, introducing confounding factors and artifacts to data, consequently skewing their interpretation and misinforming clinical decision-making. In the current study, we apply spatial light modulation, a type of diffuse reflectance hyperspectral imaging technique, to monitor the variation in optical properties of highly scattering turbid media in the presence varying levels of the following sources of interference: scattering concentration, temperature, and pressure. Spatial near-infrared (NIR) light modulation is a wide-field, non-contact emerging optical imaging platform capable of separating the effects of tissue scattering from those of absorption, thereby accurately estimating both parameters. With this technique, periodic NIR illumination patterns at alternately low and high spatial frequencies, at six discrete wavelengths between 690 to 970 nm, were sequentially projected upon the medium while a CCD camera collects the diffusely reflected light. Data analysis based assumptions is then performed off-line to recover the medium's optical properties. We conducted a series of experiments demonstrating the changes in absorption and reduced scattering coefficients of commercially available fresh milk and chicken breast tissue under different interference conditions. In addition, information on the refractive index was study under increased pressure. This work demonstrates the utility of NIR spatial light modulation to detect varying sources of interference upon the optical properties of biological samples.

Study of light scattering using C-Quant® in patients with Fuchs' endothelial dystrophy: A pilot study.

PubMed

Castaño-Martín, B; Gros-Otero, J; Martínez, J; Teus, M

2017-11-01

The purpose of this study was to determine the light scattering in patients with Fuchs' endothelial dystrophy without clinically significant corneal oedema, and evaluate its relationship with endothelial cell count, corneal thickness, and corneal biomechanical parameters. The values of light scattering were measured by C-Quant ® (Oculus Optikgeräte GmbH, Germany) in 32 eyes of 17 patients diagnosed with Fuchs' endothelial dystrophy without clinically significant corneal oedema. Corneal biomechanical properties were determined using ORA (ocular response) and Corvis ST ® (tonometry). A light scattering value outside the normal range was observed in 93.8% of eyes studied. No statistically significant association (P>.05) was found between the values of the measured light scattering by C-Quant ® and endothelial count, pachymetry, or corneal biomechanical properties. In this study, changes were found in the values of light scattering values of patients with corneal Fuchs' endothelial dystrophy. This change does not appear to correlate significantly with disease severity. Copyright © 2017 Sociedad Española de Oftalmología. Publicado por Elsevier España, S.L.U. All rights reserved.

Particle Scattering in the Resonance Regime: Full-Wave Solution for Axisymmetric Particles with Large Aspect Ratios

NASA Technical Reports Server (NTRS)

Zuffada, Cinzia; Crisp, David

1997-01-01

Reliable descriptions of the optical properties of clouds and aerosols are essential for studies of radiative transfer in planetary atmospheres. The scattering algorithms provide accurate estimates of these properties for spherical particles with a wide range of sizes and refractive indices, but these methods are not valid for non-spherical particles (e.g., ice crystals, mineral dust, and smoke). Even though a host of methods exist for deriving the optical properties of nonspherical particles that are very small or very large compared with the wavelength, only a few methods are valid in the resonance regime, where the particle dimensions are comparable with the wavelength. Most such methods are not ideal for particles with sharp edges or large axial ratios. We explore the utility of an integral equation approach for deriving the single-scattering optical properties of axisymmetric particles with large axial ratios. The accuracy of this technique is shown for spheres of increasing size parameters and an ensemble of randomly oriented prolate spheroids of size parameter equal to 10.079368. In this last case our results are compared with published results obtained with the T-matrix approach. Next we derive cross sections, single-scattering albedos, and phase functions for cylinders, disks, and spheroids of ice with dimensions extending from the Rayleigh to the geometric optics regime. Compared with those for a standard surface integral equation method, the storage requirement and the computer time needed by this method are reduced, thus making it attractive for generating databases to be used in multiple-scattering calculations. Our results show that water ice disks and cylinders are more strongly absorbing than equivalent volume spheres at most infrared wavelengths. The geometry of these particles also affects the angular dependence of the scattering. Disks and columns with maximum linear dimensions larger than the wavelength scatter much more radiation in the forward and backward directions and much less radiation at intermediate phase angles than equivalent volume spheres.

Multispectral imaging of absorption and scattering properties of in vivo exposed rat brain using a digital red-green-blue camera.

PubMed

Yoshida, Keiichiro; Nishidate, Izumi; Ishizuka, Tomohiro; Kawauchi, Satoko; Sato, Shunichi; Sato, Manabu

2015-05-01

In order to estimate multispectral images of the absorption and scattering properties in the cerebral cortex of in vivo rat brain, we investigated spectral reflectance images estimated by the Wiener estimation method using a digital RGB camera. A Monte Carlo simulation-based multiple regression analysis for the corresponding spectral absorbance images at nine wavelengths (500, 520, 540, 560, 570, 580, 600, 730, and 760 nm) was then used to specify the absorption and scattering parameters of brain tissue. In this analysis, the concentrations of oxygenated hemoglobin and that of deoxygenated hemoglobin were estimated as the absorption parameters, whereas the coefficient a and the exponent b of the reduced scattering coefficient spectrum approximated by a power law function were estimated as the scattering parameters. The spectra of absorption and reduced scattering coefficients were reconstructed from the absorption and scattering parameters, and the spectral images of absorption and reduced scattering coefficients were then estimated. In order to confirm the feasibility of this method, we performed in vivo experiments on exposed rat brain. The estimated images of the absorption coefficients were dominated by the spectral characteristics of hemoglobin. The estimated spectral images of the reduced scattering coefficients had a broad scattering spectrum, exhibiting a larger magnitude at shorter wavelengths, corresponding to the typical spectrum of brain tissue published in the literature. The changes in the estimated absorption and scattering parameters during normoxia, hyperoxia, and anoxia indicate the potential applicability of the method by which to evaluate the pathophysiological conditions of in vivo brain due to the loss of tissue viability.

Photoacoustic-fluorescence in vitro flow cytometry for quantification of absorption, scattering and fluorescence properties of the cells

NASA Astrophysics Data System (ADS)

Nedosekin, D. A.; Sarimollaoglu, M.; Foster, S.; Galanzha, E. I.; Zharov, V. P.

2013-03-01

Fluorescence flow cytometry is a well-established analytical tool that provides quantification of multiple biological parameters of cells at molecular levels, including their functional states, morphology, composition, proliferation, and protein expression. However, only the fluorescence and scattering parameters of the cells or labels are available for detection. Cell pigmentation, presence of non-fluorescent dyes or nanoparticles cannot be reliably quantified. Herewith, we present a novel photoacoustic (PA) flow cytometry design for simple integration of absorbance measurements into schematics of conventional in vitro flow cytometers. The integrated system allow simultaneous measurements of light absorbance, scattering and of multicolor fluorescence from single cells in the flow at rates up to 2 m/s. We compared various combinations of excitation laser sources for multicolor detection, including simultaneous excitation of PA and fluorescence using a single 500 kHz pulsed nanosecond laser. Multichannel detection scheme allows simultaneous detection of up to 8 labels, including 4 fluorescent tags and 4 PA colors. In vitro PA-fluorescence flow cytometer was used for studies of nanoparticles uptake and for the analysis of cell line pigmentation, including genetically encoded melanin expression in breast cancer cell line. We demonstrate that this system can be used for direct nanotoxicity studies with simultaneous quantification of nanoparticles content and assessment of cell viability using a conventional fluorescent apoptosis assays.

Light Scattering by Fractal Dust Aggregates. II. Opacity and Asymmetry Parameter

NASA Astrophysics Data System (ADS)

Tazaki, Ryo; Tanaka, Hidekazu

2018-06-01

Optical properties of dust aggregates are important at various astrophysical environments. To find a reliable approximation method for optical properties of dust aggregates, we calculate the opacity and the asymmetry parameter of dust aggregates by using a rigorous numerical method, the T-Matrix Method, and then the results are compared to those obtained by approximate methods: the Rayleigh–Gans–Debye (RGD) theory, the effective medium theory (EMT), and the distribution of hollow spheres method (DHS). First of all, we confirm that the RGD theory breaks down when multiple scattering is important. In addition, we find that both EMT and DHS fail to reproduce the optical properties of dust aggregates with fractal dimensions of 2 when the incident wavelength is shorter than the aggregate radius. In order to solve these problems, we test the mean field theory (MFT), where multiple scattering can be taken into account. We show that the extinction opacity of dust aggregates can be well reproduced by MFT. However, it is also shown that MFT is not able to reproduce the scattering and absorption opacities when multiple scattering is important. We successfully resolve this weak point of MFT, by newly developing a modified mean field theory (MMF). Hence, we conclude that MMF can be a useful tool to investigate radiative transfer properties of various astrophysical environments. We also point out an enhancement of the absorption opacity of dust aggregates in the Rayleigh domain, which would be important to explain the large millimeter-wave opacity inferred from observations of protoplanetary disks.

Influence of aerosols, clouds, and sunglint on polarization spectra of Earthshine

NASA Astrophysics Data System (ADS)

Emde, Claudia; Buras-Schnell, Robert; Sterzik, Michael; Bagnulo, Stefano

2017-08-01

Context. Ground-based observations of the Earthshine, I.e., the light scattered by Earth to the Moon, and then reflected back to Earth, simulate space observations of our planet and represent a powerful benchmark for the studies of Earth-like planets. Earthshine spectra are strongly linearly polarized, owing to scattering by molecules and small particles in the atmosphere of the Earth and surface reflection, and may allow us to measure global atmospheric and surface properties of planet Earth. Aims: We aim to interpret already published spectropolarimetric observations of the Earthshine by comparing them with new radiative transfer model simulations including a fully realistic three-dimensional (3D) surface-atmosphere model for planet Earth. Methods: We used the highly advanced Monte Carlo radiative transfer model MYSTIC to simulate polarized radiative transfer in the atmosphere of the Earth without approximations regarding the geometry, taking into account the polarization from surface reflection and multiple scattering by molecules, aerosol particles, cloud droplets, and ice crystals. Results: We have shown that Earth spectropolarimetry is highly sensitive to all these input parameters, and we have presented simulations of a fully realistic Earth atmosphere-surface model including 3D cloud fields and two-dimensional (2D) surface property maps. Our modeling results show that scattering in high ice water clouds and reflection from the ocean surface are crucial to explain the continuum polarization at longer wavelengths as has been reported in Earthshine observations taken at the Very Large Telescope in 2011 (3.8% and 6.6% at 800 nm, depending on which part of Earth was visible from the Moon at the time of the observations). We found that the relatively high degree of polarization of 6.6% can be attributed to light reflected by the ocean surface in the sunglint region. High ice-water clouds reduce the amount of absorption in the O2A band and thus explain the weak O2A band feature in the observations.

Multiphonon: Phonon Density of States tools for Inelastic Neutron Scattering Powder Data

DOE Office of Scientific and Technical Information (OSTI.GOV)

Y. Y. Lin, Jiao; Islam, Fahima; Kresh, Max

The multiphonon python package calculates phonon density of states, a reduced representation of vibrational property of condensed matter (see, for example, Section “Density of Normal Modes” in Chapter 23 “Quantum Theory of the Harmonic Crystal” of (Ashcroft and Mermin 2011)), from inelastic neutron scattering (see, for example (B. Fultz et al. 2006–2016)) spectrum from a powder sample. Inelastic neutron spectroscopy (INS) is a probe of excitations in solids of vibrational or magnetic origins. In INS, neutrons can lose(gain) energy to(from) the solid in the form of quantized lattice vibrations – phonons. Measuring phonon density of states is usually the firstmore » step in determining the phonon properties of a material experimentally. Phonons play a very important role in understanding the physical properties of a solid, including thermal conductivity and electrical conductivity. Hence, INS is an important tool for studying thermoelectric materials (Budai et al. 2014, Li et al. (2015)), where low thermal conductivity and high electrical conductivity are desired. Study of phonon entropy also made important contributions to the research of thermal dynamics and phase stability of materials (B. Fultz 2010, bogdanoff2002phonon, swan2006vibrational).« less

Chain length effects of p-oligophenyls with comparison of benzene by Raman scattering

NASA Astrophysics Data System (ADS)

Zhang, Kai; Chen, Xiao-Jia

2018-02-01

Raman scattering measurements are performed on benzene and a number of p-oligophenyls including biphenyl, p-terphenyl, p-quaterphenyl, p-quinquephenyl, and p-sexiphenyl at ambient conditions. The vibrational modes of the intra- and intermolecular terms in these materials are analyzed and compared. Chain length effects on the vibrational properties are examined for the C-H in-plane bending mode and the inter-ring C-C stretching mode at around 1200 cm-1 and 1280 cm-1, respectively, and the C-C stretching modes at around 1600 cm-1. The complex and fluctuating properties of these modes result in an imprecise estimation of the chain length of these molecules. Meanwhile, the obtained ratio of the intensities of the 1200 cm-1 mode and 1280 cm-1 mode is sensitive to the applied lasers. A librational motion mode with the lowest energy is found to have a monotonous change with the increase in the chain length. This mode is simply relevant to the c axis of the unit cell. Such an obvious trend makes it a better indicator for determining the chain length effects on the physical and chemical properties in these molecules.

Multiphonon: Phonon Density of States tools for Inelastic Neutron Scattering Powder Data

DOE PAGES

Y. Y. Lin, Jiao; Islam, Fahima; Kresh, Max

2018-01-29

The multiphonon python package calculates phonon density of states, a reduced representation of vibrational property of condensed matter (see, for example, Section “Density of Normal Modes” in Chapter 23 “Quantum Theory of the Harmonic Crystal” of (Ashcroft and Mermin 2011)), from inelastic neutron scattering (see, for example (B. Fultz et al. 2006–2016)) spectrum from a powder sample. Inelastic neutron spectroscopy (INS) is a probe of excitations in solids of vibrational or magnetic origins. In INS, neutrons can lose(gain) energy to(from) the solid in the form of quantized lattice vibrations – phonons. Measuring phonon density of states is usually the firstmore » step in determining the phonon properties of a material experimentally. Phonons play a very important role in understanding the physical properties of a solid, including thermal conductivity and electrical conductivity. Hence, INS is an important tool for studying thermoelectric materials (Budai et al. 2014, Li et al. (2015)), where low thermal conductivity and high electrical conductivity are desired. Study of phonon entropy also made important contributions to the research of thermal dynamics and phase stability of materials (B. Fultz 2010, bogdanoff2002phonon, swan2006vibrational).« less

Tunable plasmonic properties of Ag-Fe nanoparticles

NASA Astrophysics Data System (ADS)

Bhatia, Pradeep; Verma, S. S.; Sinha, M. M.

2018-05-01

Compatibility problems with electronic processes, limited availability and the high cost of noble metals motivate towards the search of alternative materials to enhance the suitability and efficiency of plasmonic based devices. Alloy or coated bimetallic material configuration is an attractive way to engineer a system possessing tuneable plasmonic properties. Magneto-plasmonic nanoparticles (MPNPs) present the possibility to exhibit their tuneable magnetic and optical properties with extensive applications. We studied the optical properties of Ag-Fe alloy for different compositions. The Localised Surface Plasmon Resonance (LSPR) tunability of Agx-Fe1-x (x = 0.25, 0.50 and 0.75) alloy for nanospheres has been calculated by using Discrete Dipole Approximation (DDA) simulation technique. It is found that absorption and scattering efficiencies of Ag-Fe alloy are found in near ultra violet and visible region of electromagnetic spectrum. Large LSPR shift has been observed in absorption and scattering efficiencies peak for 40 nm and 80 nm size of nanospheres alloys. It is concluded that the LSPR can be tuned by changing nanoparticle size and the alloy composition. Results of the plasmonics properties for Ag-Fe alloy at wavelength 330-545nm (absorption) and 331-507nm (scattering) will open the avenues for new applications in optical imaging, biomedical fields particularly in (calorimetric)-DNA, pentose's, proteins (absorption) and plasmonic-enhanced spectroscopies/spectrometer devices (scattering) for determination of optical densities of cell cultures.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Akerib, DS; Alsum, S; Araújo, HM

The LUX experiment has performed searches for dark matter particles scattering elastically on xenon nuclei, leading to stringent upper limits on the nuclear scattering cross sections for dark matter. Here, for results derived frommore » $${1.4}\\times 10^{4}\\;\\mathrm{kg\\,days}$$ of target exposure in 2013, details of the calibration, event-reconstruction, modeling, and statistical tests that underlie the results are presented. Detector performance is characterized, including measured efficiencies, stability of response, position resolution, and discrimination between electron- and nuclear-recoil populations. Models are developed for the drift field, optical properties, background populations, the electron- and nuclear-recoil responses, and the absolute rate of low-energy background events. Innovations in the analysis include in situ measurement of the photomultipliers' response to xenon scintillation photons, verification of fiducial mass with a low-energy internal calibration source, and new empirical models for low-energy signal yield based on large-sample, in situ calibrations.« less

Perspectives: Nanofibers and nanowires for disordered photonics

NASA Astrophysics Data System (ADS)

Pisignano, Dario; Persano, Luana; Camposeo, Andrea

2017-03-01

As building blocks of microscopically non-homogeneous materials, semiconductor nanowires and polymer nanofibers are emerging component materials for disordered photonics, with unique properties of light emission and scattering. Effects found in assemblies of nanowires and nanofibers include broadband reflection, significant localization of light, strong and collective multiple scattering, enhanced absorption of incident photons, synergistic effects with plasmonic particles, and random lasing. We highlight recent related discoveries, with a focus on material aspects. The control of spatial correlations in complex assemblies during deposition, the coupling of modes with efficient transmission channels provided by nanofiber waveguides, and the embedment of random architectures into individually coded nanowires will allow the potential of these photonic materials to be fully exploited, unconventional physics to be highlighted, and next-generation optical devices to be achieved. The prospects opened by this technology include enhanced random lasing and mode-locking, multi-directionally guided coupling to sensors and receivers, and low-cost encrypting miniatures for encoders and labels.

Calibration, event reconstruction, data analysis, and limit calculation for the LUX dark matter experiment

NASA Astrophysics Data System (ADS)

Akerib, D. S.; Alsum, S.; Araújo, H. M.; Bai, X.; Bailey, A. J.; Balajthy, J.; Beltrame, P.; Bernard, E. P.; Bernstein, A.; Biesiadzinski, T. P.; Boulton, E. M.; Brás, P.; Byram, D.; Cahn, S. B.; Carmona-Benitez, M. C.; Chan, C.; Currie, A.; Cutter, J. E.; Davison, T. J. R.; Dobi, A.; Dobson, J. E. Y.; Druszkiewicz, E.; Edwards, B. N.; Faham, C. H.; Fallon, S. R.; Fan, A.; Fiorucci, S.; Gaitskell, R. J.; Gehman, V. M.; Genovesi, J.; Ghag, C.; Gilchriese, M. G. D.; Hall, C. R.; Hanhardt, M.; Haselschwardt, S. J.; Hertel, S. A.; Hogan, D. P.; Horn, M.; Huang, D. Q.; Ignarra, C. M.; Jacobsen, R. G.; Ji, W.; Kamdin, K.; Kazkaz, K.; Khaitan, D.; Knoche, R.; Larsen, N. A.; Lee, C.; Lenardo, B. G.; Lesko, K. T.; Lindote, A.; Lopes, M. I.; Manalaysay, A.; Mannino, R. L.; Marzioni, M. F.; McKinsey, D. N.; Mei, D.-M.; Mock, J.; Moongweluwan, M.; Morad, J. A.; Murphy, A. St. J.; Nehrkorn, C.; Nelson, H. N.; Neves, F.; O'Sullivan, K.; Oliver-Mallory, K. C.; Palladino, K. J.; Pease, E. K.; Reichhart, L.; Rhyne, C.; Shaw, S.; Shutt, T. A.; Silva, C.; Solmaz, M.; Solovov, V. N.; Sorensen, P.; Sumner, T. J.; Szydagis, M.; Taylor, D. J.; Taylor, W. C.; Tennyson, B. P.; Terman, P. A.; Tiedt, D. R.; To, W. H.; Tripathi, M.; Tvrznikova, L.; Uvarov, S.; Velan, V.; Verbus, J. R.; Webb, R. C.; White, J. T.; Whitis, T. J.; Witherell, M. S.; Wolfs, F. L. H.; Xu, J.; Yazdani, K.; Young, S. K.; Zhang, C.; LUX Collaboration

2018-05-01

The LUX experiment has performed searches for dark-matter particles scattering elastically on xenon nuclei, leading to stringent upper limits on the nuclear scattering cross sections for dark matter. Here, for results derived from 1.4 ×104 kg days of target exposure in 2013, details of the calibration, event-reconstruction, modeling, and statistical tests that underlie the results are presented. Detector performance is characterized, including measured efficiencies, stability of response, position resolution, and discrimination between electron- and nuclear-recoil populations. Models are developed for the drift field, optical properties, background populations, the electron- and nuclear-recoil responses, and the absolute rate of low-energy background events. Innovations in the analysis include in situ measurement of the photomultipliers' response to xenon scintillation photons, verification of fiducial mass with a low-energy internal calibration source, and new empirical models for low-energy signal yield based on large-sample, in situ calibrations.

Compact quasi-monoenergetic photon sources from laser-plasma accelerators for nuclear detection and characterization

NASA Astrophysics Data System (ADS)

Geddes, Cameron G. R.; Rykovanov, Sergey; Matlis, Nicholas H.; Steinke, Sven; Vay, Jean-Luc; Esarey, Eric H.; Ludewigt, Bernhard; Nakamura, Kei; Quiter, Brian J.; Schroeder, Carl B.; Toth, Csaba; Leemans, Wim P.

2015-05-01

Near-monoenergetic photon sources at MeV energies offer improved sensitivity at greatly reduced dose for active interrogation, and new capabilities in treaty verification, nondestructive assay of spent nuclear fuel and emergency response. Thomson (also referred to as Compton) scattering sources are an established method to produce appropriate photon beams. Applications are however restricted by the size of the required high-energy electron linac, scattering (photon production) system, and shielding for disposal of the high energy electron beam. Laser-plasma accelerators (LPAs) produce GeV electron beams in centimeters, using the plasma wave driven by the radiation pressure of an intense laser. Recent LPA experiments are presented which have greatly improved beam quality and efficiency, rendering them appropriate for compact high-quality photon sources based on Thomson scattering. Designs for MeV photon sources utilizing the unique properties of LPAs are presented. It is shown that control of the scattering laser, including plasma guiding, can increase photon production efficiency. This reduces scattering laser size and/or electron beam current requirements to scale compatible with the LPA. Lastly, the plasma structure can decelerate the electron beam after photon production, reducing the size of shielding required for beam disposal. Together, these techniques provide a path to a compact photon source system.

Multiple scattering modeling pipeline for spectroscopy and photometry of airless Solar System objects

NASA Astrophysics Data System (ADS)

Penttilä, Antti; Väisänen, Timo; Markkanen, Johannes; Martikainen, Julia; Gritsevich, Maria; Muinonen, Karri

2017-10-01

We combine numerical tools to analyze the reflectance spectra of granular materials. Our motivation comes from the lack of tools when it comes to intimate mixing of materials and modeling space-weathering effects with nano- or micron-sized inclusions. The current practice is to apply a semi-physical models such as the Hapke models (e.g., Icarus 195, 2008). These are expressed in a closed form so that they are fast to apply. The problem is that the validity of the model is not guaranteed, and the derived properties related to particle scattering can be unrealistic (JQSRT 113, 2012).Our pipeline consists of individual scattering simulation codes and a main program that chains them together. The chain for analyzing a macroscopic target with space-weathered mineral would go as: (1) Scattering properties of small inclusions inside a host matrix are derived using exact Maxwell equation solvers. From the scattering properties, we use the so-called incoherent fields and Mueller matrices as input for the next step; (2) Scattering by a regolith grain is solved using a geometrical optics method with surface reflections, internal absorption, and internal diffuse scattering; (3) The radiative transfer simulation is executed inputting the regolith grains from the previous step as the scatterers in a macroscopic planar volume element.For the most realistic asteroid reflectance model, the chain would produce the properties of a planar surface element. Then, a shadowing simulation over the surface elements would be considered, and finally the asteroid phase function would be solved by integrating the bidirectional reflectance distribution function of the planar element over the object's realistic shape model.The tools in the proposed chain already exist, and practical task for us is to tie these together into an easy-to-use public pipeline. We plan to open the pipeline as a web-based open service a dedicated server, using Django application server and Python environment for the main functionality. The individual programs to be ran under the chain can still be programmed with Fortran, C, or other.We acknowledge the ERC AdG No. 320773 ‘SAEMPL’ and the computational resources provided by CSC — IT Center for Science Ltd., Finland.

Microphysical and optical properties of aerosol particles in urban zone during ESCOMPTE

NASA Astrophysics Data System (ADS)

Mallet, M.; Roger, J. C.; Despiau, S.; Dubovik, O.; Putaud, J. P.

2003-10-01

Microphysical and optical properties of the main aerosol species on a peri-urban site have been investigated during the ESCOMPTE experiment. Ammonium sulfate (AS), nitrate (N), black carbon (BC), particulate organic matter (POM), sea salt (SS) and mineral aerosol (D) size distributions have been used, associated with their refractive index, to compute, from the Mie theory, the key radiative aerosol properties as the extinction coefficient Kext, the mass extinction efficiencies σext, the single scattering albedo ω0 and the asymmetry parameter g at the wavelength of 550 nm. Optical computations show that 90% of the light extinction is due to anthropogenic aerosol and only 10% is due to natural aerosol (SS and D). 44±6% of the extinction is due to (AS) and 40±6% to carbonaceous particles (20±4% to BC and 21±4% to POM). Nitrate aerosol has a weak contribution of 5±2%. Computations of the mass extinction efficiencies σext, single scattering albedo ω0 and asymmetry parameter g indicate that the optical properties of the anthropogenic aerosol are often quite different from those yet published and generally used in global models. For example, the (AS) mean specific mass extinction presents a large difference with the value classically adopted at low relative humidity ( h<60%) (2.6±0.5 instead of 6 m 2 g -1 at 550 nm). The optical properties of the total aerosol layer, including all the aerosol species, indicate a mean observed single-scattering albedo ω0=0.85±0.05, leading to an important absorption of the solar radiation and an asymmetry parameter g=0.59±0.05 which are in a reasonably good agreements with the AERONET retrieval of ω0 (=0.86±0.05) and g (=0.64±0.05) at this wavelength.

How do the optical properties of Asian aerosols change when they cross the Pacific?

NASA Astrophysics Data System (ADS)

Fischer, E. V.; Jaffe, D. A.

2009-12-01

Primary and secondary aerosols from Asia may have important climate implications. These aerosols are emitted locally, but can then be lofted into the free troposphere and advected across the Pacific. In this analysis we used observations from the Mount Bachelor Observatory (MBO) in conjunction with satellite data to identify the dominant aerosol types in specific Asian plumes that crossed the Pacific. In situ data from MBO is used to understand the observed changes in radiative properties. A suite of gas phase and aerosol measurements were made during spring 2008 and spring 2009 at MBO (2763 masl), located in central Oregon. Here we focus on observations of dry sub-μm aerosol scattering (σsp) and absorption (σap), made with an integrating nephelometer and a particle soot absorption photometer (PSAP). Using a combination of backward trajectory calculations and satellite observations, we identified 7 well defined plumes of Asian origin. These plumes included the highest σsp (34.8 Mm-1 hourly average) and σap (4.8 Mm-1 hourly average) observed at MBO over the 2008 and 2009 spring campaigns. Of interest in this analysis is 1) whether the intensive optical properties differ between these 7 Asian events, 2) whether these differences can be linked to differences in composition, and 3) whether the intensive optical properties differ from those observed closer to the Asian source region. Preliminary results show that the plumes clustered in terms of their optical properties; plumes hypothesized to contain a large fraction of mineral dust were the most distinct. We also observed larger variability in the average scattering Ångstrom exponent of the plumes and a higher average single scatter albedo than observations closer to the Asian coast. This work will be extended to compare observations at MBO with the most recent observations from Asia as they become available.

Longwave radiative effects of Saharan dust during the ICE-D campaign

NASA Astrophysics Data System (ADS)

Brooke, Jennifer; Havemann, Stephan; Ryder, Claire; O'Sullivan, Debbie

2017-04-01

The Havemann-Taylor Fast Radiative Transfer Code (HT-FRTC) is a fast radiative transfer model based on Principal Components. Scattering has been incorporated into HT-FRTC which allows simulations of aerosol as well as clear-sky atmospheres. This work evaluates the scattering scheme in HT-FRTC and investigates dust-affected brightness temperatures using in-situ observations from Ice in Clouds Experiment - Dust (ICE-D) campaign. The ICE-D campaign occurred during August 2015 and was based from Cape Verde. The ICE-D campaign is a multidisciplinary project which achieved measurements of in-situ mineral dust properties of the dust advected from the Sahara, and on the aerosol-cloud interactions using the FAAM BAe-146 research aircraft. ICE-D encountered a range of low (0.3), intermediate (0.8) and high (1.3) aerosol optical depths, AODs, and therefore provides a range of atmospheric dust loadings in the assessment of dust scattering in HT-FRTC. Spectral radiances in the thermal infrared window region (800 - 1200 cm-1) are sensitive to the presence of mineral dust; mineral dust acts to reduce the upwelling infrared radiation caused by the absorption and re-emission of radiation by the dust layer. ARIES (Airborne Research Interferometer Evaluation System) is a nadir-facing interferometer, measuring infrared radiances between 550 and 3000 cm-1. The ARIES spectral radiances are converted to brightness temperatures by inversion of the Planck function. The mineral dust size distribution is important for radiative transfer applications as it provides a measure of aerosol scattering. The longwave spectral mineral dust optical properties including the mass extinction coefficients, single scattering albedos and the asymmetry parameter have been derived from the mean ICE-D size distribution. HT-FRTC scattering simulations are initialised with vertical mass fractions which can be derived from extinction profiles from the lidar along with the specific extinction coefficient, kext (m2/g) at 355 nm. In general the comparison between the lidar retrieval of aerosol extinction coefficients and in-situ measurements show a good agreement. The root mean square of the brightness temperature residuals in the window region for observations (ARIES) minus model simulations for i) clear-sky, ii) HT-FRTC 'line-by-line' scattering and, iii) HT-FRTC fast scattering are calculated. For the ICE-D case studies mineral dust impacts on the brightness temperature of the background on the order of 1 - 1.5 K.

Optical properties of the Martian aerosols as derived from Imager for Mars Pathfinder midday sky brightness data

NASA Astrophysics Data System (ADS)

Shalygina, O. S.; Markiewicz, W. J.; Hviid, S. F.

2012-09-01

It is well known that the aerosol play a major role in the energy budget of the Martian atmosphere. The importance of the aerosols for the radiative loading of the atmosphere has hence, direct impact on the Martian present weather and its seasonal cycle as well as consequences for its long term climate. Very accurate models of the sky brightness are required to separate the atmospheric illumination from the spectrum of the Martian surface, and hence to understand the mineralogy of the surface rocks and soil. Such accurate models are only possible if the optical properties of the Martian aerosols are known. In this work we analyze the images of the brightness of the Martian sky at midday acquired from the surface of the Mars during the Mars Pathfinder mission. The Imager for Mars Pathfinder (IMP) obtained data in filters centered at 443.6, 481.0, 670.8, 896.1 and 965.3 nm. Useful data sets were returned on sols 27, 40, 56, 65, 68, 74 and 82. Although the coverage in scattering angles of this sequence is limited to about 100°, having the Sun near zenith minimizes multiple scattering. This property should help in accuracy of constraining the size distribution and material properties. The shape of the particles can be expected to be less well constrained, as scattering events at angles around 150° are only present through multiple scattering. Data from sol 56 (Figure 1) were fitted with multiple scattering radiative transfer calculations to extract the size distribution, optical properties, and shape of the aerosols suspended in the atmosphere [1].

Radar cross section studies

NASA Technical Reports Server (NTRS)

Burnside, W. D.; Dominek, A. K.; Gupta, I. J.; Newman, E. H.; Pathak, P. H.; Peters, L., Jr.

1987-01-01

The ultimate goal is to generate experimental techniques and computer codes of rather general capability that would enable the aerospace industry to evaluate the scattering properties of aerodynamic shapes. Another goal involves developing an understanding of scattering mechanisms so that modification of the vehicular structure could be introduced within constraints set by aerodynamics. The development of indoor scattering measurement systems with special attention given to the compact range is another goal. There has been considerable progress in advancing state-of-the-art scattering measurements and control and analysis of the electromagnetic scattering from general targets.

Designer Disordered Complex Media: Hyperuniform Photonic and Phononic Band Gap Materials

NASA Astrophysics Data System (ADS)

Amoah, Timothy

In this thesis we investigate designer disordered complex media for photonics and phononics applications. Initially we focus on the photonic properties and we analyse hyperuniform disordered structures (HUDS) using numerical simulations. Photonic HUDS are a new class of photonic solids, which display large, isotropic photonic band gaps (PBG) comparable in size to the ones found in photonic crystals (PC). We review their complex interference properties, including the origin of PBGs and potential applications. HUDS combine advantages of both isotropy due to disorder (absence of long-range order) and controlled scattering properties from uniform local topology due to hyperuniformity (constrained disorder). The existence of large band gaps in HUDS contradicts the longstanding intuition that Bragg scattering and long-range translational order is required in PBG formation, and demonstrates that interactions between Mie-like local resonances and multiple scattering can induce on their own PBGs. The discussion is extended to finite height effects of planar architectures such as pseudo-band-gaps in photonic slabs as well as the vertical confinement in the presence of disorder. The particular case of a silicon-on-insulator compatible hyperuniform disordered network structure is considered for TE polarised light. We address technologically realisable designs of HUDS including localisation of light in point-defect-like optical cavities and the guiding of light in freeform PC waveguide analogues. Using finite-difference time domain and band structure computer simulations, we show that it is possible to construct optical cavities in planar hyperuniform disordered solids with isotropic band gaps that effciently confine TE polarised radiation. We thus demonstrate that HUDS are a promising general-purpose design platform for integrated optical micro-circuitry. After analysing HUDS for photonic applications we investigate them in the context of elastic waves towards phononics applications. We demonstrate the first phononic band gaps (PnBG) for HUDS. We find that PnBGs in phononic HUDS can confine and guide elastic waves similar to photonic HUDS for EM radiation.

Lunar single-scattering, porosity, and surface-roughness properties with SMART-1/AMIE

NASA Astrophysics Data System (ADS)

Parviainen, H.; Muinonen, K.; Näränen, J.; Josset, J.-L.; Beauvivre, S.; Pinet, P.; Chevrel, S.; Koschny, D.; Grieger, B.; Foing, B.

2009-04-01

We analyze the single-scattering albedo and phase function, local surface roughness and regolith porosity, and the coherent backscattering, single scattering, and shadowing contributions to the opposition effect for specific lunar mare regions imaged by the SMART-1/AMIE camera. We account for shadowing due to surface roughness and mutual shadowing among the regolith particles with ray-tracing computations for densely-packed particulate media with a fractional-Brownian-motion interface with free space. The shadowing modeling allows us to derive the hundred-micron-scale volume-element scattering phase function for the lunar mare regolith. We explain the volume-element phase function by a coherent-backscattering model, where the single scatterers are the submicron-to-micron-scale particle inhomogeneities and/or the smallest particles on the lunar surface. We express the single-scatterer phase function as a sum of three Henyey-Greenstein terms, accounting for increased backward scattering in both narrow and wide angular ranges. The Moon exhibits an opposition effect, that is, a nonlinear increase of disk-integrated brightness with decreasing solar phase angle, the angle between the Sun and the observer as seen from the object. Recently, the coherent-backscattering mechanism (CBM) has been introduced to explain the opposition effect. CBM is a multiple-scattering interference mechanism, where reciprocal waves propagating through the same scatterers in opposite directions always interfere constructively in the backward-scattering direction but with varying interference characteristics in other directions. In addition to CBM, mutual shadowing among regolith particles (SMp) and rough-surface shadowing (SMr) have their effect on the behavior of the observed lunar surface brightness. In order to accrue knowledge on the volume-element and, ultimately, single-scattering properties of the lunar regolith, both SMp and SMr need to be accurately accounted for. We included four different lunar mare regions in our study. Each of these regions covers several hundreds of square kilometers of lunar surface. When selecting the regions, we have required that they have been imaged by AMIE across a wide range of phase angles, including the opposition geometry. The phase-angle range covered is 0-109 °, with incidence and emergence angles (ι and ε) ranging within 7-87 ° and 0-53 °, respectively. The pixel scale varies from 288m down to 29m. Biases and dark currents were subtracted from the images in the usual way, followed by a flat-field correction. New dark-current reduction procedures have recently been derived from in-flight measurements to replace the ground-calibration images . The clear filter was chosen for the present study as it provides the largest field of view and is currently the best-calibrated channel. Off-nadir-pointing observations allowed for the extensive phase-angle coverage. In total, 220 images are used for the present study. The photometric data points were extracted as follows. First, on average, 50 sample areas of 10 Ã- 10 pixels were chosen by hand from each image. Second, the surface normal, ι, ε, °, and α were computed for each pixel in each sample area using the NASA/NAIF SPICE software toolkit with the latest and corrected SMART-1/AMIE SPICE kernels. Finally, the illumination angles and the observed intensity were averaged over each sample area. In total, the images used in the study resulted in approximately 11000 photometric sample points for the four mare regions. We make use of fractional-Brownian-motion surfaces in modeling the interface between free space and regolith and a size distribution of spherical particles in modeling the particulate medium. We extract the effects of the stochastic geometry from the lunar photometry and, simultaneously, obtain the volume-element scattering phase function of the lunar regolith locations studied. The volume-element phase function allows us to constrain the physical properties of the regolith particles. Based on the present theoretical modeling of the lunar photometry from SMART-1/AMIE, we conclude that most of the lunar mare opposition effect is caused by coherent backscattering and single scattering within volume elements comparable to lunar particle sizes, with only a small contribution from shadowing effects. We thus suggest that the lunar single scatterers exhibit intensity enhancement towards the backward scattering direction in resemblance to the scattering characteristics experimentally measured and theoretically computed for realistic small particles. Further interpretations of the lunar volume-element phase function will be the subject of future research.

Hyperspectral diffuse reflectance for determination of the optical properties of milk and fruit and vegetable juices

NASA Astrophysics Data System (ADS)

Qin, Jianwei; Lu, Renfu

2005-11-01

Absorption and reduced scattering coefficients are two fundamental optical properties for turbid biological materials. This paper presents the technique and method of using hyperspectral diffuse reflectance for fast determination of the optical properties of fruit and vegetable juices and milks. A hyperspectral imaging system was used to acquire spatially resolved steady-state diffuse reflectance over the spectral region between 530 and 900 nm from a variety of fruit and vegetable juices (citrus, grapefruit, orange, and vegetable) and milks with different fat levels (full, skim and mixed). The system collected diffuse reflectance in the source-detector separation range from 1.1 to 10.0 mm. The hyperspectral reflectance data were analyzed by using a diffusion theory model for semi-infinite homogeneous media. The absorption and reduced scattering coefficients of the fruit and vegetable juices and milks were extracted by inverse algorithms from the scattering profiles for wavelengths of 530-900 nm. Values of the absorption and reduced scattering coefficient at 650 nm were highly correlated to the fat content of the milk samples with the correlation coefficient of 0.990 and 0.989, respectively. The hyperspectral imaging technique can be extended to the measurement of other liquid and solid foods in which light scattering is dominant.

Measuring the light scattering and orientation of a spheroidal particle using in-line holography.

PubMed

Seo, Kyung Won; Byeon, Hyeok Jun; Lee, Sang Joon

2014-07-01

The light scattering properties of a horizontally and vertically oriented spheroidal particle under laser illumination are experimentally investigated using digital in-line holography. The reconstructed wave field shows the bright singular points as a result of the condensed beam formed by a transparent spheroidal particle acting as a lens. The in-plane (θ) and out-of-plane (ϕ) rotating angles of an arbitrarily oriented spheroidal particle are measured by using these scattering properties. As a feasibility test, the 3D orientation of a transparent spheroidal particle suspended in a microscale pipe flow is successfully reconstructed by adapting the proposed method.

Physics and applications of atmospheric nonlinear optics and filamentation.

PubMed

Kasparian, Jérôme; Wolf, Jean-Pierre

2008-01-07

We review the properties and applications of ultrashort laser pulses in the atmosphere, with a particular focus on filamentation. Filamentation is a non-linear propagation regime specific of ultrashort and ultraintense laser pulses in the atmosphere. Typical applications include remote sensing of atmospheric gases and aerosols, lightning control, laser-induced spectroscopy, coherent anti-stokes Raman scattering, and the generation of sub-THz radiation.

Impact of nongray multiphase radiation in pulverized coal combustion

NASA Astrophysics Data System (ADS)

Roy, Somesh; Wu, Bifen; Modest, Michael; Zhao, Xinyu

2016-11-01

Detailed modeling of radiation is important for accurate modeling of pulverized coal combustion. Because of high temperature and optical properties, radiative heat transfer from coal particles is often more dominant than convective heat transfer. In this work a multiphase photon Monte Carlo radiation solver is used to investigate and to quantify the effect of nongray radiation in a laboratory-scale pulverized coal flame. The nongray radiative properties of carrier phase (gas) is modeled using HITEMP database. Three major species - CO, CO2, and H2O - are treated as participating gases. Two optical models are used to evaluate radiative properties of coal particles: a formulation based on the large particle limit and a size-dependent correlation. Effect of scattering due to coal particle is also investigated using both isotropic scattering and anisotropic scattering using a Henyey-Greenstein function. Lastly, since the optical properties of ash is very different from that of coal, the effect of ash content on the radiative properties of coal particle is examined. This work used Extreme Science and Engineering Discovery Environment (XSEDE), which is supported by National Science Foundation Grant Number ACI-1053575.

Free–free experiments: the search for dressed atom effects

NASA Astrophysics Data System (ADS)

Martin, N. L. S.; Weaver, C. M.; Kim, B. N.; deHarak, B. A.

2018-07-01

Experiments on free–free electron scattering, specifically the absorption or emission of 1.17 eV photons from a Nd:YAG laser field by an unbound electron when it is scattered by an atom or molecule, are reviewed. For large scattering angles such experiments are well described by a simple analytical theory that is independent of the properties of the target. At small scattering angles this theory breaks down for targets with a high dipole polarizability α, and an additional term needs to be incorporated in the scattering amplitude. This term is proportional to the dipole polarizability, and hence introduces the properties of the target into the free–free cross section—i.e., the laser field ‘dresses’ the atom. A progress report is given of free–free experiments designed to look for such ‘dressed atom’ effects during the electron-impact excitation of argon in the presence of a laser field; the lowest excited states of argon have α ≈ 300 atomic units.

Charge ordering and scattering pre-peaks in ionic liquids and alcohols.

PubMed

Perera, Aurélien

2017-01-04

The structural properties of ionic liquids and alcohols are viewed under the charge ordering process as a common basis to explain the peculiarity of their radiation scattering properties, namely the presence, or absence, of a scattering pre-peak. Through the analysis of models, it is shown that the presence, or absence, of a radiation scattering pre-peak is principally related to the symmetry breaking, or not, of the global charge order, induced by the peculiarities of the molecular shapes. This symmetry breaking is achieved, in practice, by the emergence of specific types of clusters, which manifests how the global charge order has changed into a local form. Various atom-atom correlations witness the symmetry breaking induced by this re organization, and this is manifested into a pre-peak in the structure factor. This approach explains why associated liquids such as water do not show a scattering pre-peak. It also explains under which conditions core-soft models can mimic associating liquids.

Implementation of an Analytical Raman Scattering Correction for Satellite Ocean-Color Processing

NASA Technical Reports Server (NTRS)

McKinna, Lachlan I. W.; Werdell, P. Jeremy; Proctor, Christopher W.

2016-01-01

Raman scattering of photons by seawater molecules is an inelastic scattering process. This effect can contribute significantly to the water-leaving radiance signal observed by space-borne ocean-color spectroradiometers. If not accounted for during ocean-color processing, Raman scattering can cause biases in derived inherent optical properties (IOPs). Here we describe a Raman scattering correction (RSC) algorithm that has been integrated within NASA's standard ocean-color processing software. We tested the RSC with NASA's Generalized Inherent Optical Properties algorithm (GIOP). A comparison between derived IOPs and in situ data revealed that the magnitude of the derived backscattering coefficient and the phytoplankton absorption coefficient were reduced when the RSC was applied, whilst the absorption coefficient of colored dissolved and detrital matter remained unchanged. Importantly, our results show that the RSC did not degrade the retrieval skill of the GIOP. In addition, a timeseries study of oligotrophic waters near Bermuda showed that the RSC did not introduce unwanted temporal trends or artifacts into derived IOPs.

Study of resonance light scattering for remote optical probing

NASA Technical Reports Server (NTRS)

Penney, C. M.; Morey, W. W.; St. Peters, R. L.; Silverstein, S. D.; Lapp, M.; White, D. R.

1973-01-01

Enhanced scattering and fluorescence processes in the visible and UV were investigated which will enable improved remote measurements of gas properties. The theoretical relationship between scattering and fluorescence from an isolated molecule in the approach to resonance is examined through analysis of the time dependence of re-emitted light following excitation of pulsed incident light. Quantitative estimates are developed for the relative and absolute intensities of fluorescence and resonance scattering. New results are obtained for depolarization of scattering excited by light at wavelengths within a dissociative continuum. The experimental work was performed in two separate facilities. One of these utilizes argon and krypton lasers, single moded by a tilted etalon, and a 3/4 meter double monochromator. This facility was used to determine properties of the re-emission from NO2, I2 and O3 excited by visible light. The second facility involves a narrow-line dye laser, and a 3/4 meter single monochromator. The dye laser produces pulsed light with 5 nsec pulse duration and 0.005 nm spectral width.

Applications of Neutron Scattering in the Chemical Industry: Proton Dynamics of Highly Dispersed Materials, Characterization of Fuel Cell Catalysts, and Catalysts from Large-Scale Chemical Processes

NASA Astrophysics Data System (ADS)

Albers, Peter W.; Parker, Stewart F.

The attractiveness of neutron scattering techniques for the detailed characterization of materials of high degrees of dispersity and structural complexity as encountered in the chemical industry is discussed. Neutron scattering picks up where other analytical methods leave off because of the physico-chemical properties of finely divided products and materials whose absorption behavior toward electromagnetic radiation and electrical conductivity causes serious problems. This is demonstrated by presenting typical applications from large-scale production technology and industrial catalysis. These include the determination of the proton-related surface chemistry of advanced materials that are used as reinforcing fillers in the manufacture of tires, where interrelations between surface chemistry, rheological properties, improved safety, and significant reduction of fuel consumption are the focus of recent developments. Neutron scattering allows surface science studies of the dissociative adsorption of hydrogen on nanodispersed, supported precious metal particles of fuel cell catalysts under in situ loading at realistic gas pressures of about 1 bar. Insight into the occupation of catalytically relevant surface sites provides valuable information about the catalyst in the working state and supplies essential scientific input for tailoring better catalysts by technologists. The impact of deactivation phenomena on industrial catalysts by coke deposition, chemical transformation of carbonaceous deposits, and other processes in catalytic hydrogenation processes that result in significant shortening of the time of useful operation in large-scale plants can often be traced back in detail to surface or bulk properties of catalysts or materials of catalytic relevance. A better understanding of avoidable or unavoidable aspects of catalyst deactivation phenomena under certain in-process conditions and the development of effective means for reducing deactivation leads to more energy-efficient and, therefore, environmentally friendly processes and helps to save valuable resources. Even small or gradual improvements in all these fields are of considerable economic impact.

Cobalt coordination and clustering in alpha-Co(OH)(2) revealed by synchrotron X-ray total scattering.

PubMed

Neilson, James R; Kurzman, Joshua A; Seshadri, Ram; Morse, Daniel E

2010-09-03

Structures of layered metal hydroxides are not well described by traditional crystallography. Total scattering from a synthesis-controlled subset of these materials, as described here, reveals that different cobalt coordination polyhedra cluster within each layer on short length scales, offering new insights and approaches for understanding the properties of these and related layered materials. Structures related to that of brucite [Mg(OH)(2)] are ubiquitous in the mineral world and offer a variety of useful functions ranging from catalysis and ion-exchange to sequestration and energy transduction, including applications in batteries. However, it has been difficult to resolve the atomic structure of these layered compounds because interlayer disorder disrupts the long-range periodicity necessary for diffraction-based structure determination. For this reason, traditional unit-cell-based descriptions have remained inaccurate. Here we apply, for the first time to such layered hydroxides, synchrotron X-ray total scattering methods-analyzing both the Bragg and diffuse components-to resolve the intralayer structure of three different alpha-cobalt hydroxides, revealing the nature and distribution of metal site coordination. The different compounds with incorporated chloride ions have been prepared with kinetic control of hydrolysis to yield different ratios of octahedrally and tetrahedrally coordinated cobalt ions within the layers, as confirmed by total scattering. Real-space analyses indicate local clustering of polyhedra within the layers, manifested in the weighted average of different ordered phases with fixed fractions of tetrahedrally coordinated cobalt sites. These results, hidden from an averaged unit-cell description, reveal new structural characteristics that are essential to understanding the origin of fundamental material properties such as color, anion exchange capacity, and magnetic behavior. Our results also provide further insights into the detailed mechanisms of aqueous hydrolysis chemistry of hydrated metal salts. We emphasize the power of the methods used here for establishing structure-property correlations in functional materials with related layered structures.

Ultrasonic characterization of solid liquid suspensions

DOEpatents

Panetta, Paul D.

2010-06-22

Using an ultrasonic field, properties of a solid liquid suspension such as through-transmission attenuation, backscattering, and diffuse field are measured. These properties are converted to quantities indicating the strength of different loss mechanisms (such as absorption, single scattering and multiple scattering) among particles in the suspension. Such separation of the loss mechanisms can allow for direct comparison of the attenuating effects of the mechanisms. These comparisons can also indicate a model most likely to accurately characterize the suspension and can aid in determination of properties such as particle size, concentration, and density of the suspension.

Long term measurements of the estimated hygroscopic enhancement of aerosol optical properties

NASA Astrophysics Data System (ADS)

Hervo, Maxime; Sellegri, Karine; Pichon, Jean Marc; Roger, Jean Claude; Laj, Paolo

2015-04-01

Water vapour has a major impact on aerosol optical properties, thus on the Radiative Forcing for aerosol-radiation interaction (RFari). However there is few studies measuring this impact over a large period. Optical properties of aerosols were measured at the GAW Puy de Dôme station (1465m) over a seven year period (2006-2012). The impact of hygroscopicity on aerosol optical properties was calculated over a two year period (2010-2011). The analysis of the spatial and temporal variability of the dry optical properties showed that while no long term trend was found, a clear seasonal and diurnal variation was observed on the extensive parameters (scattering, absorption). Scattering and absorption coefficients were highest during the warm season and daytime, in concordance with the seasonality and diurnal variation of the planetary boundary layer height reaching the site. Intensive parameters (single scattering albedo, asymmetry factor, refractive index) did not show such a strong diurnal variability, but still indicated different values depending on the season. Both extensive and intensive optical parameters were sensitive to the air mass origin. A strong impact of hygroscopicity on aerosol optical properties was calculated, mainly on aerosol scattering, with a dependence on the aerosol type and the season. At 90% humidity, the scattering factor enhancement (fsca) was more than 4.4 for oceanic aerosol that have mixed with a pollution plume. Consequently, the aerosol radiative forcing was estimated to be 2.8 times higher at RH= 90% and 1.75 times higher at ambient RH when hygroscopic growth of the aerosol was considered. The hygroscopicity enhancement factor of the scattering coefficient was parameterized as a function of humidity and air mass type. To our knowledge, these results are one of the first presenting the impact of water vapour on the aerosol optical properties for a long period, and the first for a site at the border between the planetary boundary layer and the free troposphere. Acknowledgements. The authors would like to acknowledge the OPGC and its staff and INSU/CNRS for their contribution to establishing and maintaining the PdD measurement site. This work was performed in the frame of the european EUSAAR (R113-CT-2006-026140) and EUCAARI (0136833-2) and the french ORAURE SOERE.

Electronic and magnetic properties of manganite thin films with different compositions and its correlation with transport properties: An X-ray resonant magnetic scattering study

DOE PAGES

Singh, Surendra; Freeland, J. W.; Fitzsimmons, M. R.; ...

2014-12-08

Here, we present x-ray resonant magnetic dichroism and x-ray resonant magnetic scattering measurements of the temperature dependence of magnetism in Pr-doped La-Ca-Mn-O films grown on (110) NdGaO3 substrates. We observed thermal hysteresis of the ferromagnetism in one film that also showed large thermal hysteresis of ~18K in transport measurements. While in a second film of a different nominal chemistry, which showed very small thermal hysteresis ~3K in transport measurements, no thermal hysteresis of the ferromagnetism was observed. As a result, these macroscopic properties are correlated with evolution of surface magnetization across metal insulator transition for these films as observed bymore » soft x-ray resonant magnetic scattering measurements.« less

Dynamical properties of water in living cells

NASA Astrophysics Data System (ADS)

Piazza, Irina; Cupane, Antonio; Barbier, Emmanuel L.; Rome, Claire; Collomb, Nora; Ollivier, Jacques; Gonzalez, Miguel A.; Natali, Francesca

2018-02-01

With the aim of studying the effect of water dynamics on the properties of biological systems, in this paper, we present a quasi-elastic neutron scattering study on three different types of living cells, differing both in their morphological and tumor properties. The measured scattering signal, which essentially originates from hydrogen atoms present in the investigated systems, has been analyzed using a global fitting strategy using an optimized theoretical model that considers various classes of hydrogen atoms and allows disentangling diffusive and rotational motions. The approach has been carefully validated by checking the reliability of the calculation of parameters and their 99% confidence intervals. We demonstrate that quasi-elastic neutron scattering is a suitable experimental technique to characterize the dynamics of intracellular water in the angstrom/picosecond space/time scale and to investigate the effect of water dynamics on cellular biodiversity.

A model for pion-pion scattering in large- N QCD

NASA Astrophysics Data System (ADS)

Veneziano, G.; Yankielowicz, S.; Onofri, E.

2017-04-01

Following up on recent work by Caron-Huot et al. we consider a generalization of the old Lovelace-Shapiro model as a toy model for ππ scattering satisfying (most of) the properties expected to hold in ('t Hooft's) large- N limit of massless QCD. In particular, the model has asymptotically linear and parallel Regge trajectories at positive t, a positive leading Regge intercept α 0 < 1, and an effective bending of the trajectories in the negative- t region producing a fixed branch point at J = 0 for t < t 0 < 0. Fixed (physical) angle scattering can be tuned to match the power-like behavior (including logarithmic corrections) predicted by perturbative QCD: A( s, t) ˜ s - β log( s)-γ F ( θ). Tree-level unitarity (i.e. positivity of residues for all values of s and J ) imposes strong constraints on the allowed region in the α0- β-γ parameter space, which nicely includes a physically interesting region around α 0 = 0 .5, β = 2 and γ = 3. The full consistency of the model would require an extension to multi-pion processes, a program we do not undertake in this paper.

Light-scattering properties of a Venetian blind slat used for daylighting applications

DOE Office of Scientific and Technical Information (OSTI.GOV)

Nilsson, Annica M.; Jonsson, Jacob C.

2010-12-15

The low cost, simplicity, and aesthetic appearance of external and internal shading devices, make them commonly used for daylighting and glare-control applications. Shading devices, such as Venetian blinds, screens, and roller shades, generally exhibit light scattering and/or light redirecting properties. This requires the bi-directional scattering distribution function (BSDF) of the material to be known in order to accurately predict the daylight distribution and energy flow through the fenestration system. Acquiring the complete BSDF is not a straightforward task, and to complete the process it is often required that a model is used to complement the measured data. In this project,more » a Venetian blind slat with a white top surface and a brushed aluminum bottom surface was optically characterized. A goniophotometer and an integrating sphere spectrophotometer were used to determine the angle resolved and hemispherical reflectance of the sample, respectively. The acquired data were fitted to a scattering model providing one Lambertian and one angle dependent description of the surface properties. These were used in combination with raytracing to obtain the complete BSDFs of the Venetian blind system. (author)« less

Physical characteristics of cometary dust from optical studies

NASA Technical Reports Server (NTRS)

Hanner, M. S.

1980-01-01

Observations of the sunlight scattered and thermal emission from cometary dust, which may be used to infer the physical properties of the dust grains, are reviewed. Consideration is given to the observed wavelength dependence of the scattered light from cometary coma and tails, the average scattering function of the dust grains, the average grain Bond albedo, the polarization of the scattered light, and grain temperatures deduced from thermal infrared emission. The thermal properties of dust grains are illustrated for models based on magnetite or olivine grain materials, with consideration given to the variation of thermal properties with particle radius and heliocentric distance. Comparison of the models with observations indicates that a disordered or amorphous olivine composition can give a reasonable fit to the data for appropriate grain sizes and temperatures. The observations acquired are noted to indicate an optically important particle size of 1 micron, with silicate particles not larger than a few microns usually present although pure silicate grains can not be responsible for the thermal emission, and the cometary dust grains are most likely not spherical. Further observations needed in the infrared are indicated.

Acoustic vibrations contribute to the diffuse scatter produced by ribosome crystals

DOE Office of Scientific and Technical Information (OSTI.GOV)

Polikanov, Yury S.; Moore, Peter B.

2015-09-26

The diffuse scattering pattern produced by frozen crystals of the 70S ribosome fromThermus thermophilusis as highly structured as it would be if it resulted entirely from domain-scale motions within these particles. However, the qualitative properties of the scattering pattern suggest that acoustic displacements of the crystal lattice make a major contribution to it.

Rupture Dynamics and Ground Motion from Earthquakes on Rough Faults in Heterogeneous Media

NASA Astrophysics Data System (ADS)

Bydlon, S. A.; Kozdon, J. E.; Duru, K.; Dunham, E. M.

2013-12-01

Heterogeneities in the material properties of Earth's crust scatter propagating seismic waves. The effects of scattered waves are reflected in the seismic coda and depend on the amplitude of the heterogeneities, spatial arrangement, and distance from source to receiver. In the vicinity of the fault, scattered waves influence the rupture process by introducing fluctuations in the stresses driving propagating ruptures. Further variability in the rupture process is introduced by naturally occurring geometric complexity of fault surfaces, and the stress changes that accompany slip on rough surfaces. Our goal is to better understand the origin of complexity in the earthquake source process, and to quantify the relative importance of source complexity and scattering along the propagation path in causing incoherence of high frequency ground motion. Using a 2D high order finite difference rupture dynamics code, we nucleate ruptures on either flat or rough faults that obey strongly rate-weakening friction laws. These faults are embedded in domains with spatially varying material properties characterized by Von Karman autocorrelation functions and their associated power spectral density functions, with variations in wave speed of approximately 5 to 10%. Flat fault simulations demonstrate that off-fault material heterogeneity, at least with this particular form and amplitude, has only a minor influence on the rupture process (i.e., fluctuations in slip and rupture velocity). In contrast, ruptures histories on rough faults in both homogeneous and heterogeneous media include much larger short-wavelength fluctuations in slip and rupture velocity. We therefore conclude that source complexity is dominantly influenced by fault geometric complexity. To examine contributions of scattering versus fault geometry on ground motions, we compute spatially averaged root-mean-square (RMS) acceleration values as a function of fault perpendicular distance for a homogeneous medium and several heterogeneous media characterized by different statistical properties. We find that at distances less than ~6 km from the fault, RMS acceleration values from simulations with homogeneous and heterogeneous media are similar, but at greater distances the RMS values associated with heterogeneous media are larger than those associated with homogeneous media. The magnitude of this divergence increases with the amplitude of the heterogeneities. For instance, for a heterogeneous medium with a 10% standard deviation in material property values relative to mean values, RMS accelerations are ~50% larger than for a homogeneous medium at distances greater than 6 km. This finding is attributed to the scattering of coherent pulses into multiple pulses of decreased amplitude that subsequently arrive at later times. In order to understand the robustness of these results, an extension of our dynamic rupture and wave propagation code to 3D is underway.

The extinction properties of forest components

NASA Technical Reports Server (NTRS)

Karam, M. A.; Fung, A. K.; Blanchard, A. J.; Nance, C. E.

1988-01-01

The effect of each forest component on the extinction of electromagnetic waves is investigated by modeling the branches with finite cylinders, deciduous leaves with elliptic disks, and coniferous leaves with needles. The inner field is estimated by the field inside an infinitely long cylinder of similar properties for the branches, and by the Shifrin approximation for the leaves. For each forest component analytic expressions were derived for the extinction cross section via the forward scattering theorem and for ohmic and scattered losses. For branches, the variation of the extinction cross section obtained via the forward scattering theorem is illustrated numerically as a function of the branch radius and the imaginery part of its dielectric constant. It is compared with the measurements from a single branch. For the leaves, the forward scattering theorem gives value for the extinction cross section equal to the ohmic cross section.

Impact of finite temperatures on the transport properties of Gd from first principles

NASA Astrophysics Data System (ADS)

Chadova, K.; Mankovsky, S.; Minár, J.; Ebert, H.

2017-03-01

Finite-temperature effects have a pronounced impact on the transport properties of solids. In magnetic systems, besides the scattering of conduction electrons by impurities and phonons, an additional scattering source coming from the magnetic degrees of freedom must be taken into account. A first-principle scheme which treats all these scattering effects on equal footing was recently suggested within the framework of the multiple scattering formalism. Employing the alloy analogy model treated by means of the CPA, thermal lattice vibrations and spin fluctuations are effectively taken into account. In the present work the temperature dependence of the longitudinal resistivity and the anomalous Hall effect in the strongly correlated metal Gd is considered. The comparison with experiments demonstrates that the proposed numerical scheme does provide an adequate description of the electronic transport at finite temperatures.

Retrieval of ice cloud properties from Himawari-8 satellite measurements by Voronoi ice particle model

NASA Astrophysics Data System (ADS)

Letu, H.; Nagao, T. M.; Nakajima, T. Y.; Ishimoto, H.; Riedi, J.; Shang, H.

2017-12-01

Ice cloud property product from satellite measurements is applicable in climate change study, numerical weather prediction, as well as atmospheric study. Ishimoto et al., (2010) and Letu et al., (2016) developed a single scattering property of the highly irregular ice particle model, called the Voronoi model for developing ice cloud product of the GCOM-C satellite program. It is investigated that Voronoi model has a good performance on retrieval of the ice cloud properties by comparing it with other well-known scattering models. Cloud property algorithm (Nakajima et al., 1995, Ishida and Nakajima., 2009, Ishimoto et al., 2009, Letu et al., 2012, 2014, 2016) of the GCOM-C satellite program is improved to produce the Himawari-8/AHI cloud products based on the variation of the solar zenith angle. Himawari-8 is the new-generational geostationary meteorological satellite, which is successfully launched by the Japan Meteorological Agency (JMA) on 7 October 2014. In this study, ice cloud optical and microphysical properties are simulated from RSTAR radiative transfer code by using various model. Scattering property of the Voronoi model is investigated for developing the AHI ice cloud products. Furthermore, optical and microphysical properties of the ice clouds are retrieved from Himawari-8/AHI satellite measurements. Finally, retrieval results from Himawari-8/AHI are compared to MODIS-C6 cloud property products for validation of the AHI cloud products.

Label-free hyperspectral dark-field microscopy for quantitative scatter imaging

NASA Astrophysics Data System (ADS)

Cheney, Philip; McClatchy, David; Kanick, Stephen; Lemaillet, Paul; Allen, David; Samarov, Daniel; Pogue, Brian; Hwang, Jeeseong

2017-03-01

A hyperspectral dark-field microscope has been developed for imaging spatially distributed diffuse reflectance spectra from light-scattering samples. In this report, quantitative scatter spectroscopy is demonstrated with a uniform scattering phantom, namely a solution of polystyrene microspheres. A Monte Carlo-based inverse model was used to calculate the reduced scattering coefficients of samples of different microsphere concentrations from wavelength-dependent backscattered signal measured by the dark-field microscope. The results are compared to the measurement results from a NIST double-integrating sphere system for validation. Ongoing efforts involve quantitative mapping of scattering and absorption coefficients in samples with spatially heterogeneous optical properties.

LIGHT SCATTERING PROPERTIES OF GLIADIN AFTER X-RAY IRRADIATION

DOE Office of Scientific and Technical Information (OSTI.GOV)

Wu, J.

1962-01-01

The gliadin portion of wheat gluten prepared in 60% ethanol solution was investigated for its light scattering properties after x irradiation. Results show that the effect of irradiation depends on the quality of the sample, such as dry or wet. The average molecular weight of liadin decreased in accordance with the time of irradiation. The longer the irradiated time, the more SH groups were setfree. (P.C.H.)

Seamless Integration of Detection and Therapy for Breast Cancer using Targeted Engineered Nanoparticles

DTIC Science & Technology

2007-06-01

and exhibit strong scattering and ab- sorption effects due to the strong plasmon resonance of the metallic-dielectric concentric spherical...neglecting its ab- sorption properties. Thus, the studies will be further separated into two sets, one considering only the scattering properties of the... sorption from the gold nanoshells, the reflectance is more de- pendent on the volume-normalized absorption cross section than the combination of

Quantitative analysis of optical properties of flowing blood using a photon-cell interactive Monte Carlo code: effects of red blood cells' orientation on light scattering.

PubMed

Sakota, Daisuke; Takatani, Setsuo

2012-05-01

Optical properties of flowing blood were analyzed using a photon-cell interactive Monte Carlo (pciMC) model with the physical properties of the flowing red blood cells (RBCs) such as cell size, shape, refractive index, distribution, and orientation as the parameters. The scattering of light by flowing blood at the He-Ne laser wavelength of 632.8 nm was significantly affected by the shear rate. The light was scattered more in the direction of flow as the flow rate increased. Therefore, the light intensity transmitted forward in the direction perpendicular to flow axis decreased. The pciMC model can duplicate the changes in the photon propagation due to moving RBCs with various orientations. The resulting RBC's orientation that best simulated the experimental results was with their long axis perpendicular to the direction of blood flow. Moreover, the scattering probability was dependent on the orientation of the RBCs. Finally, the pciMC code was used to predict the hematocrit of flowing blood with accuracy of approximately 1.0 HCT%. The photon-cell interactive Monte Carlo (pciMC) model can provide optical properties of flowing blood and will facilitate the development of the non-invasive monitoring of blood in extra corporeal circulatory systems.

Root-cause estimation of ultrasonic scattering signatures within a complex textured titanium

NASA Astrophysics Data System (ADS)

Blackshire, James L.; Na, Jeong K.; Freed, Shaun

2016-02-01

The nondestructive evaluation of polycrystalline materials has been an active area of research for many decades, and continues to be an area of growth in recent years. Titanium alloys in particular have become a critical material system used in modern turbine engine applications, where an evaluation of the local microstructure properties of engine disk/blade components is desired for performance and remaining life assessments. Current NDE methods are often limited to estimating ensemble material properties or detecting localized voids, inclusions, or damage features within a material. Recent advances in computational NDE and material science characterization methods are providing new and unprecedented access to heterogeneous material properties, which permits microstructure-sensing interactions to be studied in detail. In the present research, Integrated Computational Materials Engineering (ICME) methods and tools are being leveraged to gain a comprehensive understanding of root-cause ultrasonic scattering processes occurring within a textured titanium aerospace material. A combination of destructive, nondestructive, and computational methods are combined within the ICME framework to collect, holistically integrate, and study complex ultrasound scattering using realistic 2-dimensional representations of the microstructure properties. Progress towards validating the computational sensing methods are discussed, along with insight into the key scattering processes occurring within the bulk microstructure, and how they manifest in pulse-echo immersion ultrasound measurements.

Polarization simulations of stellar wind bow-shock nebulae - I. The case of electron scattering

NASA Astrophysics Data System (ADS)

Shrestha, Manisha; Neilson, Hilding R.; Hoffman, Jennifer L.; Ignace, Richard

2018-06-01

Bow shocks and related density enhancements produced by the winds of massive stars moving through the interstellar medium provide important information regarding the motions of the stars, the properties of their stellar winds, and the characteristics of the local medium. Since bow-shock nebulae are aspherical structures, light scattering within them produces a net polarization signal even if the region is spatially unresolved. Scattering opacity arising from free electrons and dust leads to a distribution of polarized intensity across the bow-shock structure. That polarization encodes information about the shape, composition, opacity, density, and ionization state of the material within the structure. In this paper, we use the Monte Carlo radiative transfer code SLIP to investigate the polarization created when photons scatter in a bow-shock-shaped region of enhanced density surrounding a stellar source. We present results for electron scattering, and investigate the polarization behaviour as a function of optical depth, temperature, and source of photons for two different cases: pure scattering and scattering with absorption. In both regimes, we consider resolved and unresolved cases. We discuss the implications of these results as well as their possible use along with observational data to constrain the properties of observed bow-shock systems. In different situations and under certain assumptions, our simulations can constrain viewing angle, optical depth and temperature of the scattering region, and the relative luminosities of the star and shock.

Influence of size and shape of sub-micrometer light scattering centers in ZnO-assisted TiO2 photoanode for dye-sensitized solar cells

NASA Astrophysics Data System (ADS)

Pham, Trang T. T.; Mathews, Nripan; Lam, Yeng-Ming; Mhaisalkar, Subodh

2018-03-01

Sub-micrometer cavities have been incorporated in the TiO2 photoanode of dye-sensitized solar cell to enhance its optical property with light scattering effect. These are large pores of several hundred nanometers in size and scatter incident light due to the difference refraction index between the scattering center and the surrounding materials, according to Mie theory. The pores are created using polystyrene (PS) or zinc oxide (ZnO) templates reported previously which resulted in ellipsoidal and spherical shapes, respectively. The effect of size and shape of scattering center was modeled using a numerical analysis finite-difference time-domain (FDTD). The scattering cross-section was not affected significantly with different shapes if the total displacement volume of the scattering center is comparable. Experiments were carried out to evaluate the optical property with varying size of ZnO templates. Photovoltaic effect of dye-sensitized solar cells made from these ZnO-assisted films were investigated with incident-photon-to-current efficiency to understand the effect of scattering center size on the enhancement of absorption. With 380 nm macropores incorporated, the power conversion efficiency has increased by 11% mostly thanks to the improved current density, while 170 nm and 500 nm macropores samples did not have increment in sufficiently wide range of absorbing wavelengths.

Evolution of a beam dynamics model for the transport line in a proton therapy facility

NASA Astrophysics Data System (ADS)

Rizzoglio, V.; Adelmann, A.; Baumgarten, C.; Frey, M.; Gerbershagen, A.; Meer, D.; Schippers, J. M.

2017-12-01

During the conceptual design of an accelerator or beamline, first-order beam dynamics models are essential for studying beam properties. However, they can only produce approximate results. During commissioning, these approximate results are compared to measurements, which will rarely coincide if the model does not include the relevant physics. It is therefore essential that this linear model is extended to include higher-order effects. In this paper, the effects of particle-matter interaction have been included in the model of the transport lines in the proton therapy facility at the Paul Scherrer Institut (PSI) in Switzerland. The first-order models of these beamlines provide an approximated estimation of beam size, energy loss and transmission. To improve the performance of the facility, a more precise model was required and has been developed with opal (Object Oriented Parallel Accelerator Library), a multiparticle open source beam dynamics code. In opal, the Monte Carlo simulations of Coulomb scattering and energy loss are performed seamless with the particle tracking. Beside the linear optics, the influence of the passive elements (e.g., degrader, collimators, scattering foils, and air gaps) on the beam emittance and energy spread can be analyzed in the new model. This allows for a significantly improved precision in the prediction of beam transmission and beam properties. The accuracy of the opal model has been confirmed by numerous measurements.

The application of laser pointers for demonstration experiments in nanotechnology lessons at secondary school level

NASA Astrophysics Data System (ADS)

Markin, Alexey V.; Markina, Natalia E.; Eilks, Ingo

2017-03-01

The article contains description of several demonstration experiments connected with application of light scattering (LS) for investigation of optical properties of nanoparticles solutions. The demonstrations are based on the usage of laser pointers with different wavelengths (405, 532, and 650 nm) for observing of light scattering and absorbance by various nanoparticles (silver, gold, sulfur, and cadmium selenide). These experiments were used during short course for secondary school students ("Introduction to Nanotechnology") and applied as hands-on activities in order to introduce students to methods of investigation of nanostructures. The demonstrations (included to the course) were tested during summer-camp school (in 2015 and 2016) and in club in chemistry (2016) for secondary school students (15-17 years old).

Investigation of Aggregates as a Model for Titan's Aerosols Using Microwave Analog Experiments and Radiative Transfer Theory

NASA Astrophysics Data System (ADS)

Thomas-Osip, J. E.; Gustafson, B. Å. S.

1996-09-01

It has been suggested that the aerosols in the atmosphere of Titan have an aggregate morphology (Bar-Nun et al., 1988: West and Smith, 1991). Previous studies were based on formulations of the Discrete Dipole Approximation to calculate the single scattering properties of such aggregates. These studies were limited in the size of the individual spheres and total size of the aggregate. We present microwave to light analog scattering measurements and radiative transfer calculations for aggregates of 250-500 individual spheres near the Raleigh size limit in a plane parallel atmosphere. The advantages of using microwave analog experiments include the possibility of investigating a broad range of particle sizes and morphologies.

Ultrasound scatter in heterogeneous 3D microstructures: Parameters affecting multiple scattering

NASA Astrophysics Data System (ADS)

Engle, B. J.; Roberts, R. A.; Grandin, R. J.

2018-04-01

This paper reports on a computational study of ultrasound propagation in heterogeneous metal microstructures. Random spatial fluctuations in elastic properties over a range of length scales relative to ultrasound wavelength can give rise to scatter-induced attenuation, backscatter noise, and phase front aberration. It is of interest to quantify the dependence of these phenomena on the microstructure parameters, for the purpose of quantifying deleterious consequences on flaw detectability, and for the purpose of material characterization. Valuable tools for estimation of microstructure parameters (e.g. grain size) through analysis of ultrasound backscatter have been developed based on approximate weak-scattering models. While useful, it is understood that these tools display inherent inaccuracy when multiple scattering phenomena significantly contribute to the measurement. It is the goal of this work to supplement weak scattering model predictions with corrections derived through application of an exact computational scattering model to explicitly prescribed microstructures. The scattering problem is formulated as a volume integral equation (VIE) displaying a convolutional Green-function-derived kernel. The VIE is solved iteratively employing FFT-based con-volution. Realizations of random microstructures are specified on the micron scale using statistical property descriptions (e.g. grain size and orientation distributions), which are then spatially filtered to provide rigorously equivalent scattering media on a length scale relevant to ultrasound propagation. Scattering responses from ensembles of media representations are averaged to obtain mean and variance of quantities such as attenuation and backscatter noise levels, as a function of microstructure descriptors. The computational approach will be summarized, and examples of application will be presented.

Characterization of aerosol scattering and spectral absorption by unique methods: a polar/imaging nephelometer and spectral reflectance measurements of aerosol samples collected on filters

NASA Astrophysics Data System (ADS)

Dolgos, Gergely; Martins, J. Vanderlei; Remer, Lorraine A.; Correia, Alexandre L.; Tabacniks, Manfredo; Lima, Adriana R.

2010-02-01

Characterization of aerosol scattering and absorption properties is essential to accurate radiative transfer calculations in the atmosphere. Applications of this work include remote sensing of aerosols, corrections for aerosol distortions in satellite imagery of the surface, global climate models, and atmospheric beam propagation. Here we demonstrate successful instrument development at the Laboratory for Aerosols, Clouds and Optics at UMBC that better characterizes aerosol scattering phase matrix using an imaging polar nephelometer (LACO-I-Neph) and enables measurement of spectral aerosol absorption from 200 nm to 2500 nm. The LACO-I-Neph measures the scattering phase function from 1.5° to 178.5° scattering angle with sufficient sensitivity to match theoretical expectations of Rayleigh scattering of various gases. Previous measurements either lack a sufficiently wide range of measured scattering angles or their sensitivity is too low and therefore the required sample amount is prohibitively high for in situ measurements. The LACO-I-Neph also returns expected characterization of the linear polarization signal of Rayleigh scattering. Previous work demonstrated the ability of measuring spectral absorption of aerosol particles using a reflectance technique characterization of aerosol samples collected on Nuclepore filters. This first generation methodology yielded absorption measurements from 350 nm to 2500 nm. Here we demonstrate the possibility of extending this wavelength range into the deep UV, to 200 nm. This extended UV region holds much promise in identifying and characterizing aerosol types and species. The second generation, deep UV, procedure requires careful choice of filter substrates. Here the choice of substrates is explored and preliminary results are provided.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Rothstein, Ira Z.; Stewart, Iain W.

Starting with QCD, we derive an effective field theory description for forward scattering and factorization violation as part of the soft-collinear effective field theory (SCET) for high energy scattering. These phenomena are mediated by long distance Glauber gluon exchanges, which are static in time, localized in the longitudinal distance, and act as a kernel for forward scattering where |t| << s. In hard scattering, Glauber gluons can induce corrections which invalidate factorization. With SCET, Glauber exchange graphs can be calculated explicitly, and are distinct from graphs involving soft, collinear, or ultrasoft gluons. We derive a complete basis of operators whichmore » describe the leading power effects of Glauber exchange. Key ingredients include regulating light-cone rapidity singularities and subtractions which prevent double counting. Our results include a novel all orders gauge invariant pure glue soft operator which appears between two collinear rapidity sectors. The 1-gluon Feynman rule for the soft operator coincides with the Lipatov vertex, but it also contributes to emissions with ≥ 2 soft gluons. Our Glauber operator basis is derived using tree level and one-loop matching calculations from full QCD to both SCET II and SCET I. The one-loop amplitude’s rapidity renormalization involves mixing of color octet operators and yields gluon Reggeization at the amplitude level. The rapidity renormalization group equation for the leading soft and collinear functions in the forward scattering cross section are each given by the BFKL equation. Various properties of Glauber gluon exchange in the context of both forward scattering and hard scattering factorization are described. For example, we derive an explicit rule for when eikonalization is valid, and provide a direct connection to the picture of multiple Wilson lines crossing a shockwave. In hard scattering operators Glauber subtractions for soft and collinear loop diagrams ensure that we are not sensitive to the directions for soft and collinear Wilson lines. Conversely, certain Glauber interactions can be absorbed into these soft and collinear Wilson lines by taking them to be in specific directions. Finally, we also discuss criteria for factorization violation.« less

Electromagnetic Model Reliably Predicts Radar Scattering Characteristics of Airborne Organisms

NASA Astrophysics Data System (ADS)

Mirkovic, Djordje; Stepanian, Phillip M.; Kelly, Jeffrey F.; Chilson, Phillip B.

2016-10-01

The radar scattering characteristics of aerial animals are typically obtained from controlled laboratory measurements of a freshly harvested specimen. These measurements are tedious to perform, difficult to replicate, and typically yield only a small subset of the full azimuthal, elevational, and polarimetric radio scattering data. As an alternative, biological applications of radar often assume that the radar cross sections of flying animals are isotropic, since sophisticated computer models are required to estimate the 3D scattering properties of objects having complex shapes. Using the method of moments implemented in the WIPL-D software package, we show for the first time that such electromagnetic modeling techniques (typically applied to man-made objects) can accurately predict organismal radio scattering characteristics from an anatomical model: here the Brazilian free-tailed bat (Tadarida brasiliensis). The simulated scattering properties of the bat agree with controlled measurements and radar observations made during a field study of bats in flight. This numerical technique can produce the full angular set of quantitative polarimetric scattering characteristics, while eliminating many practical difficulties associated with physical measurements. Such a modeling framework can be applied for bird, bat, and insect species, and will help drive a shift in radar biology from a largely qualitative and phenomenological science toward quantitative estimation of animal densities and taxonomic identification.

Electromagnetic Model Reliably Predicts Radar Scattering Characteristics of Airborne Organisms

PubMed Central

Mirkovic, Djordje; Stepanian, Phillip M.; Kelly, Jeffrey F.; Chilson, Phillip B.

2016-01-01

The radar scattering characteristics of aerial animals are typically obtained from controlled laboratory measurements of a freshly harvested specimen. These measurements are tedious to perform, difficult to replicate, and typically yield only a small subset of the full azimuthal, elevational, and polarimetric radio scattering data. As an alternative, biological applications of radar often assume that the radar cross sections of flying animals are isotropic, since sophisticated computer models are required to estimate the 3D scattering properties of objects having complex shapes. Using the method of moments implemented in the WIPL-D software package, we show for the first time that such electromagnetic modeling techniques (typically applied to man-made objects) can accurately predict organismal radio scattering characteristics from an anatomical model: here the Brazilian free-tailed bat (Tadarida brasiliensis). The simulated scattering properties of the bat agree with controlled measurements and radar observations made during a field study of bats in flight. This numerical technique can produce the full angular set of quantitative polarimetric scattering characteristics, while eliminating many practical difficulties associated with physical measurements. Such a modeling framework can be applied for bird, bat, and insect species, and will help drive a shift in radar biology from a largely qualitative and phenomenological science toward quantitative estimation of animal densities and taxonomic identification. PMID:27762292

Electromagnetic Model Reliably Predicts Radar Scattering Characteristics of Airborne Organisms.

PubMed

Mirkovic, Djordje; Stepanian, Phillip M; Kelly, Jeffrey F; Chilson, Phillip B

2016-10-20

The radar scattering characteristics of aerial animals are typically obtained from controlled laboratory measurements of a freshly harvested specimen. These measurements are tedious to perform, difficult to replicate, and typically yield only a small subset of the full azimuthal, elevational, and polarimetric radio scattering data. As an alternative, biological applications of radar often assume that the radar cross sections of flying animals are isotropic, since sophisticated computer models are required to estimate the 3D scattering properties of objects having complex shapes. Using the method of moments implemented in the WIPL-D software package, we show for the first time that such electromagnetic modeling techniques (typically applied to man-made objects) can accurately predict organismal radio scattering characteristics from an anatomical model: here the Brazilian free-tailed bat (Tadarida brasiliensis). The simulated scattering properties of the bat agree with controlled measurements and radar observations made during a field study of bats in flight. This numerical technique can produce the full angular set of quantitative polarimetric scattering characteristics, while eliminating many practical difficulties associated with physical measurements. Such a modeling framework can be applied for bird, bat, and insect species, and will help drive a shift in radar biology from a largely qualitative and phenomenological science toward quantitative estimation of animal densities and taxonomic identification.

Quasiparticle interference in ZrSiS: Strongly band-selective scattering depending on impurity lattice site

NASA Astrophysics Data System (ADS)

Butler, Christopher J.; Wu, Yu-Mi; Hsing, Cheng-Rong; Tseng, Yi; Sankar, Raman; Wei, Ching-Ming; Chou, Fang-Cheng; Lin, Minn-Tsong

2017-11-01

Scanning tunneling microscopy visualizations of quasiparticle interference (QPI) enable powerful insights into the k -space properties of superconducting, topological, Rashba, and other exotic electronic phases, but their reliance on impurities acting as scattering centers is rarely scrutinized. Here, we investigate QPI at the vacuum-cleaved (001) surface of the Dirac semimetal ZrSiS. We find that interference patterns around impurities located on the Zr and S lattice sites appear very different, and can be ascribed to selective scattering of different subsets of the predominantly Zr 4 d -derived band structure, namely, the m =0 and ±1 components. We show that the selectivity of scattering channels requires an explanation beyond the different bands' orbital characteristics and their respective charge density distributions over Zr and S lattice sites. Importantly, this result shows that the usual assumption of generic scattering centers allowing observations of quasiparticle interference to shed light indiscriminately and isotropically upon the q space of scattering events does not hold, and that the scope and interpretation of QPI observations can therefore be be strongly contingent on the material defect chemistry. This finding promises to spur new investigations into the quasiparticle scattering process itself, to inform future interpretations of quasiparticle interference observations, and ultimately to aid the understanding and engineering of quantum electronic transport properties.

Thermophysical properties of liquid UO2, ZrO2 and corium by molecular dynamics and predictive models

NASA Astrophysics Data System (ADS)

Kim, Woong Kee; Shim, Ji Hoon; Kaviany, Massoud

2017-08-01

Predicting the fate of accident-melted nuclear fuel-cladding requires the understanding of the thermophysical properties which are lacking or have large scatter due to high-temperature experimental challenges. Using equilibrium classical molecular dynamics (MD), we predict the properties of melted UO2 and ZrO2 and compare them with the available experimental data and the predictive models. The existing interatomic potential models have been developed mainly for the polymorphic solid phases of these oxides, so they cannot be used to predict all the properties accurately. We compare and decipher the distinctions of those MD predictions using the specific property-related autocorrelation decays. The predicted properties are density, specific heat, heat of fusion, compressibility, viscosity, surface tension, and the molecular and electronic thermal conductivities. After the comparisons, we provide readily usable temperature-dependent correlations (including UO2-ZrO2 compounds, i.e. corium melt).

A New Observation Technique Applied to Early/Fast VLF Scattering Events

NASA Astrophysics Data System (ADS)

Kotovsky, D. A.; Moore, R. C.

2012-12-01

Early/fast very low frequency (VLF, 3-30 kHz) events are understood to result from ionospheric conductivity changes associated with lightning. Early/fast amplitude and phase perturbations have been observed coincidentally with various optical observations of transient luminous events (TLEs), including elves, sprites, and sprite halos, each of which can have temporal characteristics consistent with those of early/fast VLF events. It is yet unresolved, however, whether a specific type of TLE is directly related to the ionospheric conductivity changes responsible for the typical early/fast event. In this paper, we present spread spectrum VLF scattering observations of early/fast events. The spread spectrum analysis technique determines the amplitude and phase of a subionospherically propagating VLF signal as a function of time during the early/fast event and as a function of frequency across the 200 Hz bandwidth of the VLF transmission. VLF scattering observations, each identified with causative lightning logged by the National Lightning Detection Network (NLDN), are compared with the predictions of the Long-Wave Propagation Capability (LWPC) code, a three-dimensional earth-ionosphere waveguide propagation and scattering model. Theoretical predictions for VLF scattering from ionization changes associated with elves are compared with those associated with sprite halos, and each are compared with experimental observations. Results indicate that the observed frequency dependence of VLF scattering during early/fast events results from the combination of scattering source properties and Earth-ionosphere waveguide propagation effects. Observations are more consistent with the modeled amplitude perturbations associated with sprite halos than those with elves.

Interpretation of light scattering and turbidity measurements in aggregated systems: effect of intra-cluster multiple-light scattering.

PubMed

Soos, Miroslav; Lattuada, Marco; Sefcik, Jan

2009-11-12

In this work we studied the effect of intracluster multiple-light scattering on the scattering properties of a population of fractal aggregates. To do so, experimental data of diffusion-limited aggregation for three polystyrene latexes with similar surface properties but different primary particle diameters (equal to 118, 420, and 810 nm) were obtained by static light scattering and by means of a spectrophotometer. In parallel, a population balance equation (PBE) model, which takes into account the effect of intracluster multiple-light scattering by solving the T-matrix and the mean-field version of T-matrix, was formulated and validated against time evolution of the root mean radius of gyration, , of the zero angle intensity of scattered light, I(0), and of the turbidity, tau. It was found that the mean-field version of the T-matrix theory is able to correctly predict the time evolution of all measured light scattering quantities for all sizes of primary particles without any adjustable parameter. The structure of the aggregates, characterized by fractal dimension, d(f), was independent of the primary particle size and equal to 1.7, which is in agreement with values found in literature. Since the mean-field version of the T-matrix theory used is rather complicated and requires advanced knowledge of cluster structure (i.e., the particle-particle correlation function), a simplified version of the light scattering model was proposed and tested. It was found that within the range of operating conditions investigated, the simplified version of the light scattering model was able to describe with reasonable accuracy the time evolution of all measured light scattering quantities of the cluster mass distribution (CMD) for all three sizes of primary particles and two values of the laser wavelength.

Statistical parameters of random heterogeneity estimated by analysing coda waves based on finite difference method

NASA Astrophysics Data System (ADS)

Emoto, K.; Saito, T.; Shiomi, K.

2017-12-01

Short-period (<1 s) seismograms are strongly affected by small-scale (<10 km) heterogeneities in the lithosphere. In general, short-period seismograms are analysed based on the statistical method by considering the interaction between seismic waves and randomly distributed small-scale heterogeneities. Statistical properties of the random heterogeneities have been estimated by analysing short-period seismograms. However, generally, the small-scale random heterogeneity is not taken into account for the modelling of long-period (>2 s) seismograms. We found that the energy of the coda of long-period seismograms shows a spatially flat distribution. This phenomenon is well known in short-period seismograms and results from the scattering by small-scale heterogeneities. We estimate the statistical parameters that characterize the small-scale random heterogeneity by modelling the spatiotemporal energy distribution of long-period seismograms. We analyse three moderate-size earthquakes that occurred in southwest Japan. We calculate the spatial distribution of the energy density recorded by a dense seismograph network in Japan at the period bands of 8-16 s, 4-8 s and 2-4 s and model them by using 3-D finite difference (FD) simulations. Compared to conventional methods based on statistical theories, we can calculate more realistic synthetics by using the FD simulation. It is not necessary to assume a uniform background velocity, body or surface waves and scattering properties considered in general scattering theories. By taking the ratio of the energy of the coda area to that of the entire area, we can separately estimate the scattering and the intrinsic absorption effects. Our result reveals the spectrum of the random inhomogeneity in a wide wavenumber range including the intensity around the corner wavenumber as P(m) = 8πε2a3/(1 + a2m2)2, where ε = 0.05 and a = 3.1 km, even though past studies analysing higher-frequency records could not detect the corner. Finally, we estimate the intrinsic attenuation by modelling the decay rate of the energy. The method proposed in this study is suitable for quantifying the statistical properties of long-wavelength subsurface random inhomogeneity, which leads the way to characterizing a wider wavenumber range of spectra, including the corner wavenumber.

Review of Quantitative Ultrasound: Envelope Statistics and Backscatter Coefficient Imaging and Contributions to Diagnostic Ultrasound.

PubMed

Oelze, Michael L; Mamou, Jonathan

2016-02-01

Conventional medical imaging technologies, including ultrasound, have continued to improve over the years. For example, in oncology, medical imaging is characterized by high sensitivity, i.e., the ability to detect anomalous tissue features, but the ability to classify these tissue features from images often lacks specificity. As a result, a large number of biopsies of tissues with suspicious image findings are performed each year with a vast majority of these biopsies resulting in a negative finding. To improve specificity of cancer imaging, quantitative imaging techniques can play an important role. Conventional ultrasound B-mode imaging is mainly qualitative in nature. However, quantitative ultrasound (QUS) imaging can provide specific numbers related to tissue features that can increase the specificity of image findings leading to improvements in diagnostic ultrasound. QUS imaging can encompass a wide variety of techniques including spectral-based parameterization, elastography, shear wave imaging, flow estimation, and envelope statistics. Currently, spectral-based parameterization and envelope statistics are not available on most conventional clinical ultrasound machines. However, in recent years, QUS techniques involving spectral-based parameterization and envelope statistics have demonstrated success in many applications, providing additional diagnostic capabilities. Spectral-based techniques include the estimation of the backscatter coefficient (BSC), estimation of attenuation, and estimation of scatterer properties such as the correlation length associated with an effective scatterer diameter (ESD) and the effective acoustic concentration (EAC) of scatterers. Envelope statistics include the estimation of the number density of scatterers and quantification of coherent to incoherent signals produced from the tissue. Challenges for clinical application include correctly accounting for attenuation effects and transmission losses and implementation of QUS on clinical devices. Successful clinical and preclinical applications demonstrating the ability of QUS to improve medical diagnostics include characterization of the myocardium during the cardiac cycle, cancer detection, classification of solid tumors and lymph nodes, detection and quantification of fatty liver disease, and monitoring and assessment of therapy.

Review of quantitative ultrasound: envelope statistics and backscatter coefficient imaging and contributions to diagnostic ultrasound

PubMed Central

Oelze, Michael L.; Mamou, Jonathan

2017-01-01

Conventional medical imaging technologies, including ultrasound, have continued to improve over the years. For example, in oncology, medical imaging is characterized by high sensitivity, i.e., the ability to detect anomalous tissue features, but the ability to classify these tissue features from images often lacks specificity. As a result, a large number of biopsies of tissues with suspicious image findings are performed each year with a vast majority of these biopsies resulting in a negative finding. To improve specificity of cancer imaging, quantitative imaging techniques can play an important role. Conventional ultrasound B-mode imaging is mainly qualitative in nature. However, quantitative ultrasound (QUS) imaging can provide specific numbers related to tissue features that can increase the specificity of image findings leading to improvements in diagnostic ultrasound. QUS imaging techniques can encompass a wide variety of techniques including spectral-based parameterization, elastography, shear wave imaging, flow estimation and envelope statistics. Currently, spectral-based parameterization and envelope statistics are not available on most conventional clinical ultrasound machines. However, in recent years QUS techniques involving spectral-based parameterization and envelope statistics have demonstrated success in many applications, providing additional diagnostic capabilities. Spectral-based techniques include the estimation of the backscatter coefficient, estimation of attenuation, and estimation of scatterer properties such as the correlation length associated with an effective scatterer diameter and the effective acoustic concentration of scatterers. Envelope statistics include the estimation of the number density of scatterers and quantification of coherent to incoherent signals produced from the tissue. Challenges for clinical application include correctly accounting for attenuation effects and transmission losses and implementation of QUS on clinical devices. Successful clinical and pre-clinical applications demonstrating the ability of QUS to improve medical diagnostics include characterization of the myocardium during the cardiac cycle, cancer detection, classification of solid tumors and lymph nodes, detection and quantification of fatty liver disease, and monitoring and assessment of therapy. PMID:26761606

Observations of strong ion-ion correlations in dense plasmas

DOE PAGES

Ma, T.; Fletcher, L.; Pak, A.; ...

2014-04-24

Using simultaneous spectrally, angularly, and temporally resolved x-ray scattering, we measure the pronounced ion-ion correlation peak in a strongly coupled plasma. Laser-driven shock-compressed aluminum at ~3× solid density is probed with high-energy photons at 17.9 keV created by molybdenum He-α emission in a laser-driven plasma source. The measured elastic scattering feature shows a well-pronounced correlation peak at a wave vector of k=4Å –1. The magnitude of this correlation peak cannot be described by standard plasma theories employing a linear screened Coulomb potential. Advanced models, including a strong short-range repulsion due to the inner structure of the aluminum ions are howevermore » in good agreement with the scattering data. These studies have demonstrated a new highly accurate diagnostic technique to directly measure the state of compression and the ion-ion correlations. Furthermore, we have since applied this new method in single-shot wave-number resolved S(k) measurements to characterize the physical properties of dense plasmas.« less

On the failure load and mechanism of polycrystalline graphene by nanoindentation

PubMed Central

Sha, Z. D.; Wan, Q.; Pei, Q. X.; Quek, S. S.; Liu, Z. S.; Zhang, Y. W.; Shenoy, V. B.

2014-01-01

Nanoindentation has been recently used to measure the mechanical properties of polycrystalline graphene. However, the measured failure loads are found to be scattered widely and vary from lab to lab. We perform molecular dynamics simulations of nanoindentation on polycrystalline graphene at different sites including grain center, grain boundary (GB), GB triple junction, and holes. Depending on the relative position between the indenter tip and defects, significant scattering in failure load is observed. This scattering is found to arise from a combination of the non-uniform stress state, varied and weakened strengths of different defects, and the relative location between the indenter tip and the defects in polycrystalline graphene. Consequently, the failure behavior of polycrystalline graphene by nanoindentation is critically dependent on the indentation site, and is thus distinct from uniaxial tensile loading. Our work highlights the importance of the interaction between the indentation tip and defects, and the need to explicitly consider the defect characteristics at and near the indentation site in polycrystalline graphene during nanoindentation. PMID:25500732

Solid State Division progress report, September 30, 1981

DOE Office of Scientific and Technical Information (OSTI.GOV)

Not Available

1982-04-01

Progress made during the 19 months from March 1, 1980, through September 30, 1981, is reported in the following areas: theoretical solid state physics (surfaces, electronic and magnetic properties, particle-solid interactions, and laser annealing); surface and near-surface properties of solids (plasma materials interactions, ion-solid interactions, pulsed laser annealing, and semiconductor physics and photovoltaic conversion); defects in solids (radiation effects, fracture, and defects and impurities in insulating crystals); transport properties of solids (fast-ion conductors, superconductivity, and physical properties of insulating materials); neutron scattering (small-angle scattering, lattice dynamics, and magnetic properties); crystal growth and characterization (nuclear waste forms, ferroelectric mateirals, high-temperature materials,more » and special materials); and isotope research materials. Publications and papers are listed. (WHK)« less

Effects of nanoscale aggregation on mechanical properties and local dynamics of precise acid- and ion-containing polymers

NASA Astrophysics Data System (ADS)

Middleton, Luri Robert

Acid- and ion-containing polymers have interchain interactions that alter polymer behavior at the nano, micro, and bulk length scales. Strong secondary-bonds act as thermo-reversible physical crosslinks between chains which drive self-assembly. Tuning theses interactions can modify bulk polymer properties including stiffness, toughness, melt viscosity, resilience, clarity, abrasion resistance and puncture resistance. Furthermore, understanding and improving the relevant factors that control transport properties would have vast implications on developing solid polymer electrolytes (SPEs) for technologically important applications including water desalination, ion exchange membranes and microelectronics. This thesis explores the structure - processing - morphology - property relationships of acid and ionic functionalized polymers. Improvements in synthetic techniques and advancements in characterization methods have enabled new studies of associating polymer systems. Synthesis of entangled, high molecular weight, linear polyethylene (PE) chains functionalized with interacting pendant groups (acidic or ionic) placed periodically along the polymer backbone represent a new class of associating polymers. These polymers with periodic distributions of acid groups are much more homogenous than the commercially available polymers. Previous studies of these polymers with greater structural homogeneity revealed great variety in morphologies of the nano-aggregated polar groups within the non-polar polymer matrix. This thesis correlated the morphologies with bulk properties through real-time X-ray scattering and tensile deformation at a range of temperatures and sample compositions. New, transient morphologies and hierarchical morphologies were observed which coincided with unusual tensile strain hardening. These results indicate that improvements in synthetic control of polymers can enhance physical properties such as tensile strain-hardening, through cooperative bonding between chains. The structural regularity of precise polyethylenes also enables robust comparisons between experiments and computer simulations. At pico- to nano-seconds time scales and length scales of polymer and aggregate dynamics, neutron scattering and molecular dynamics simulations were combined to extend the knowledge of the molecular-level aggregated polymer dynamics. These experiments provide a baseline for future studies of ion-conduction in associating polymer melts.

Single Crystal Diffuse Neutron Scattering

DOE PAGES

Welberry, Richard; Whitfield, Ross

2018-01-11

Diffuse neutron scattering has become a valuable tool for investigating local structure in materials ranging from organic molecular crystals containing only light atoms to piezo-ceramics that frequently contain heavy elements. Although neutron sources will never be able to compete with X-rays in terms of the available flux the special properties of neutrons, viz. the ability to explore inelastic scattering events, the fact that scattering lengths do not vary systematically with atomic number and their ability to scatter from magnetic moments, provides strong motivation for developing neutron diffuse scattering methods. Here, we compare three different instruments that have been used bymore » us to collect neutron diffuse scattering data. Two of these are on a spallation source and one on a reactor source.« less

Single Crystal Diffuse Neutron Scattering

DOE Office of Scientific and Technical Information (OSTI.GOV)

Welberry, Richard; Whitfield, Ross

Diffuse neutron scattering has become a valuable tool for investigating local structure in materials ranging from organic molecular crystals containing only light atoms to piezo-ceramics that frequently contain heavy elements. Although neutron sources will never be able to compete with X-rays in terms of the available flux the special properties of neutrons, viz. the ability to explore inelastic scattering events, the fact that scattering lengths do not vary systematically with atomic number and their ability to scatter from magnetic moments, provides strong motivation for developing neutron diffuse scattering methods. Here, we compare three different instruments that have been used bymore » us to collect neutron diffuse scattering data. Two of these are on a spallation source and one on a reactor source.« less

Mie and debye scattering in dusty plasmas

PubMed

Guerra; Mendonca

2000-07-01

We calculate the total field scattered by a charged sphere immersed in a plasma using a unified treatment that includes the usual Mie scattering and the scattering by the Debye cloud around the particle. This is accomplished by use of the Dyadic Green function to determine the field radiated by the electrons of the Debye cloud, which is then obtained as a series of spherical vector wave functions similar to that of the Mie field. Thus we treat the Debye-Mie field as a whole and study its properties. The main results of this study are (1) the Mie (Debye) field dominates at small (large) wavelengths and in the Rayleigh limit the Debye field is constant; (2) the total cross section has an interference term between the Debye and Mie fields, important in some regimes; (3) this term is negative for negative charge of the grain, implying a total cross section smaller than previously thought; (4) a method is proposed to determine the charge of the grain (divided by a certain suppression factor) and the Debye length of the plasma; (5) a correction to the dispersion relation of an electromagnetic wave propagating in a plasma is derived.

A programmable metasurface with dynamic polarization, scattering and focusing control

NASA Astrophysics Data System (ADS)

Yang, Huanhuan; Cao, Xiangyu; Yang, Fan; Gao, Jun; Xu, Shenheng; Li, Maokun; Chen, Xibi; Zhao, Yi; Zheng, Yuejun; Li, Sijia

2016-10-01

Diverse electromagnetic (EM) responses of a programmable metasurface with a relatively large scale have been investigated, where multiple functionalities are obtained on the same surface. The unit cell in the metasurface is integrated with one PIN diode, and thus a binary coded phase is realized for a single polarization. Exploiting this anisotropic characteristic, reconfigurable polarization conversion is presented first. Then the dynamic scattering performance for two kinds of sources, i.e. a plane wave and a point source, is carefully elaborated. To tailor the scattering properties, genetic algorithm, normally based on binary coding, is coupled with the scattering pattern analysis to optimize the coding matrix. Besides, inverse fast Fourier transform (IFFT) technique is also introduced to expedite the optimization process of a large metasurface. Since the coding control of each unit cell allows a local and direct modulation of EM wave, various EM phenomena including anomalous reflection, diffusion, beam steering and beam forming are successfully demonstrated by both simulations and experiments. It is worthwhile to point out that a real-time switch among these functionalities is also achieved by using a field-programmable gate array (FPGA). All the results suggest that the proposed programmable metasurface has great potentials for future applications.

A programmable metasurface with dynamic polarization, scattering and focusing control

PubMed Central

Yang, Huanhuan; Cao, Xiangyu; Yang, Fan; Gao, Jun; Xu, Shenheng; Li, Maokun; Chen, Xibi; Zhao, Yi; Zheng, Yuejun; Li, Sijia

2016-01-01

Diverse electromagnetic (EM) responses of a programmable metasurface with a relatively large scale have been investigated, where multiple functionalities are obtained on the same surface. The unit cell in the metasurface is integrated with one PIN diode, and thus a binary coded phase is realized for a single polarization. Exploiting this anisotropic characteristic, reconfigurable polarization conversion is presented first. Then the dynamic scattering performance for two kinds of sources, i.e. a plane wave and a point source, is carefully elaborated. To tailor the scattering properties, genetic algorithm, normally based on binary coding, is coupled with the scattering pattern analysis to optimize the coding matrix. Besides, inverse fast Fourier transform (IFFT) technique is also introduced to expedite the optimization process of a large metasurface. Since the coding control of each unit cell allows a local and direct modulation of EM wave, various EM phenomena including anomalous reflection, diffusion, beam steering and beam forming are successfully demonstrated by both simulations and experiments. It is worthwhile to point out that a real-time switch among these functionalities is also achieved by using a field-programmable gate array (FPGA). All the results suggest that the proposed programmable metasurface has great potentials for future applications. PMID:27774997

A programmable metasurface with dynamic polarization, scattering and focusing control.

PubMed

Yang, Huanhuan; Cao, Xiangyu; Yang, Fan; Gao, Jun; Xu, Shenheng; Li, Maokun; Chen, Xibi; Zhao, Yi; Zheng, Yuejun; Li, Sijia

2016-10-24

Diverse electromagnetic (EM) responses of a programmable metasurface with a relatively large scale have been investigated, where multiple functionalities are obtained on the same surface. The unit cell in the metasurface is integrated with one PIN diode, and thus a binary coded phase is realized for a single polarization. Exploiting this anisotropic characteristic, reconfigurable polarization conversion is presented first. Then the dynamic scattering performance for two kinds of sources, i.e. a plane wave and a point source, is carefully elaborated. To tailor the scattering properties, genetic algorithm, normally based on binary coding, is coupled with the scattering pattern analysis to optimize the coding matrix. Besides, inverse fast Fourier transform (IFFT) technique is also introduced to expedite the optimization process of a large metasurface. Since the coding control of each unit cell allows a local and direct modulation of EM wave, various EM phenomena including anomalous reflection, diffusion, beam steering and beam forming are successfully demonstrated by both simulations and experiments. It is worthwhile to point out that a real-time switch among these functionalities is also achieved by using a field-programmable gate array (FPGA). All the results suggest that the proposed programmable metasurface has great potentials for future applications.

Scattering and radiative properties of complex soot and soot-containing particles

NASA Astrophysics Data System (ADS)

Liu, L.; Mishchenko, M. I.; Mackowski, D. W.; Dlugach, J.

2012-12-01

Tropospheric soot and soot containing aerosols often exhibit nonspherical overall shapes and complex morphologies. They can externally, semi-externally, and internally mix with other aerosol species. This poses a tremendous challenge in particle characterization, remote sensing, and global climate modeling studies. To address these challenges, we used the new numerically exact public-domain Fortran-90 code based on the superposition T-matrix method (STMM) and other theoretical models to analyze the potential effects of aggregation and heterogeneity on light scattering and absorption by morphologically complex soot containing particles. The parameters we computed include the whole scattering matrix elements, linear depolarization ratios, optical cross-sections, asymmetry parameters, and single scattering albedos. It is shown that the optical characteristics of soot and soot containing aerosols very much depend on particle sizes, compositions, and aerosol overall shapes. The soot particle configurations and heterogeneities can have a substantial effect that can result in a significant enhancement of extinction and absorption relative to those computed from the Lorenz-Mie theory. Meanwhile the model calculated information combined with in-situ and remote sensed data can be used to constrain soot particle shapes and sizes which are much needed in climate models.

Measurements of Ocean Surface Scattering Using an Airborne 94-GHz Cloud Radar: Implication for Calibration of Airborne and Spaceborne W-band Radars

NASA Technical Reports Server (NTRS)

Li, Li-Hua; Heymsfield, Gerald M.; Tian, Lin; Racette, Paul E.

2004-01-01

Scattering properties of the Ocean surface have been widely used as a calibration reference for airborne and spaceborne microwave sensors. However, at millimeter-wave frequencies, the ocean surface backscattering mechanism is still not well understood, in part, due to the lack of experimental measurements. During the Cirrus Regional Study of Tropical Anvils and Cirrus Layers-Florida Area Cirrus Experiment (CRYSTAL-FACE), measurements of ocean surface backscattering were made using a 94-GHz (W-band) cloud radar onboard a NASA ER-2 high-altitude aircraft. The measurement set includes the normalized Ocean surface cross section over a range of the incidence angles under a variety of wind conditions. Analysis of the radar measurements shows good agreement with a quasi-specular scattering model. This unprecedented dataset enhances our knowledge about the Ocean surface scattering mechanism at 94 GHz. The results of this work support the proposition of using the Ocean surface as a calibration reference for airborne millimeter-wave cloud radars and for the ongoing NASA CloudSat mission, which will use a 94-GHz spaceborne cloud radar for global cloud measurements.

SS-HORSE method for studying resonances

DOE Office of Scientific and Technical Information (OSTI.GOV)

Blokhintsev, L. D.; Mazur, A. I.; Mazur, I. A., E-mail: 008043@pnu.edu.ru

A new method for analyzing resonance states based on the Harmonic-Oscillator Representation of Scattering Equations (HORSE) formalism and analytic properties of partial-wave scattering amplitudes is proposed. The method is tested by applying it to the model problem of neutral-particle scattering and can be used to study resonance states on the basis of microscopic calculations performed within various versions of the shell model.

The Toda lattice as a forced integrable system

NASA Technical Reports Server (NTRS)

Hansen, P. J.; Kaup, D. J.

1985-01-01

The analytic properties of the Jost functions for the inverse scattering transform associated with the forced Toda lattice are shown to determine the time evolution of this particular boundary value problem. It is suggested that inverse scattering methods may be used generally to analyze forced integrable systems. Thus an extension of the applicability of the inverse scattering transform is indicated.

Scattering of aerosol particles by a Hermite-Gaussian beam in marine atmosphere.

PubMed

Huang, Qingqing; Cheng, Mingjian; Guo, Lixin; Li, Jiangting; Yan, Xu; Liu, Songhua

2017-07-01

Based on the complex-source-point method and the generalized Lorenz-Mie theory, the scattering properties and polarization of aerosol particles by a Hermite-Gaussian (HG) beam in marine atmosphere is investigated. The influences of beam mode, beam width, and humidity on the scattered field are analyzed numerically. Results indicate that when the number of HG beam modes u (v) increase, the radar cross section of aerosol particles alternating appears at maximum and minimum values in the forward and backward scattering, respectively, because of the special petal-shaped distribution of the HG beam. The forward and backward scattering of aerosol particles decreases with the increase in beam waist. When beam waist is less than the radius of the aerosol particle, a minimum value is observed in the forward direction. The scattering properties of aerosol particles by the HG beam are more sensitive to the change in relative humidity compared with those by the plane wave and the Gaussian beam (GB). The HG beam shows superiority over the plane wave and the GB in detecting changes in the relative humidity of marine atmosphere aerosol. The effects of relative humidity on the polarization of the HG beam have been numerically analyzed in detail.

Scattering of elastic waves by a spheroidal inclusion

NASA Astrophysics Data System (ADS)

Johnson, Lane R.

2018-03-01

An analytical solution is presented for scattering of elastic waves by prolate and oblate spheroidal inclusions. The problem is solved in the frequency domain where separation of variables leads to a solution involving spheroidal wave functions of the angular and radial kind. Unlike the spherical problem, the boundary equations remain coupled with respect to one of the separation indices. Expanding the angular spheroidal wave functions in terms of associated Legendre functions and using their orthogonality properties leads to a set of linear equations that can be solved to simultaneously obtain solutions for all coupled modes of both scattered and interior fields. To illustrate some of the properties of the spheroidal solution, total scattering cross-sections for P, SV and SH plane waves incident at an oblique angle on a prolate spheroid, an oblate spheroid and a sphere are compared. The waveforms of the scattered field exterior to the inclusion are calculated for these same incident waves. The waveforms scattered by a spheroid are strongly dependent upon the angle of incidence, are different for incident SV and SH waves and are asymmetrical about the centre of the spheroid with the asymmetry different for prolate and oblate spheroids.

A multiwave range test for obstacle reconstructions with unknown physical properties

NASA Astrophysics Data System (ADS)

Potthast, Roland; Schulz, Jochen

2007-08-01

We develop a new multiwave version of the range test for shape reconstruction in inverse scattering theory. The range test [R. Potthast, et al., A `range test' for determining scatterers with unknown physical properties, Inverse Problems 19(3) (2003) 533-547] has originally been proposed to obtain knowledge about an unknown scatterer when the far field pattern for only one plane wave is given. Here, we extend the method to the case of multiple waves and show that the full shape of the unknown scatterer can be reconstructed. We further will clarify the relation between the range test methods, the potential method [A. Kirsch, R. Kress, On an integral equation of the first kind in inverse acoustic scattering, in: Inverse Problems (Oberwolfach, 1986), Internationale Schriftenreihe zur Numerischen Mathematik, vol. 77, Birkhauser, Basel, 1986, pp. 93-102] and the singular sources method [R. Potthast, Point sources and multipoles in inverse scattering theory, Habilitation Thesis, Gottingen, 1999]. In particular, we propose a new version of the Kirsch-Kress method using the range test and a new approach to the singular sources method based on the range test and potential method. Numerical examples of reconstructions for all four methods are provided.

Directly Characterizing the Relative Strength and Momentum Dependence of Electron-Phonon Coupling Using Resonant Inelastic X-Ray Scattering

DOE Office of Scientific and Technical Information (OSTI.GOV)

Devereaux, T. P.; Shvaika, A. M.; Wu, K.

The coupling between lattice and charge degrees of freedom in condensed matter materials is ubiquitous and can often result in interesting properties and ordered phases, including conventional superconductivity, charge-density wave order, and metal-insulator transitions. Angle-resolved photoemission spectroscopy and both neutron and nonresonant x-ray scattering serve as effective probes for determining the behavior of appropriate, individual degrees of freedom—the electronic structure and lattice excitation, or phonon dispersion, respectively. However, each provides less direct information about the mutual coupling between the degrees of freedom, usually through self-energy effects, which tend to renormalize and broaden spectral features precisely where the coupling is strong,more » impacting one’s ability to quantitatively characterize the coupling. Here, we demonstrate that resonant inelastic x-ray scattering, or RIXS, can be an effective tool to directly determine the relative strength and momentum dependence of the electron-phonon coupling in condensed matter systems. Using a diagrammatic approach for an eight-band model of copper oxides, we study the contributions from the lowest-order diagrams to the full RIXS intensity for a realistic scattering geometry, accounting for matrix element effects in the scattering cross section, as well as the momentum dependence of the electron-phonon coupling vertex. A detailed examination of these maps offers a unique perspective into the characteristics of electron-phonon coupling, which complements both neutron and nonresonant x-ray scattering, as well as Raman and infrared conductivity.« less

Directly Characterizing the Relative Strength and Momentum Dependence of Electron-Phonon Coupling Using Resonant Inelastic X-Ray Scattering

DOE PAGES

Devereaux, T. P.; Shvaika, A. M.; Wu, K.; ...

2016-10-25

The coupling between lattice and charge degrees of freedom in condensed matter materials is ubiquitous and can often result in interesting properties and ordered phases, including conventional superconductivity, charge-density wave order, and metal-insulator transitions. Angle-resolved photoemission spectroscopy and both neutron and nonresonant x-ray scattering serve as effective probes for determining the behavior of appropriate, individual degrees of freedom—the electronic structure and lattice excitation, or phonon dispersion, respectively. However, each provides less direct information about the mutual coupling between the degrees of freedom, usually through self-energy effects, which tend to renormalize and broaden spectral features precisely where the coupling is strong,more » impacting one’s ability to quantitatively characterize the coupling. Here, we demonstrate that resonant inelastic x-ray scattering, or RIXS, can be an effective tool to directly determine the relative strength and momentum dependence of the electron-phonon coupling in condensed matter systems. Using a diagrammatic approach for an eight-band model of copper oxides, we study the contributions from the lowest-order diagrams to the full RIXS intensity for a realistic scattering geometry, accounting for matrix element effects in the scattering cross section, as well as the momentum dependence of the electron-phonon coupling vertex. A detailed examination of these maps offers a unique perspective into the characteristics of electron-phonon coupling, which complements both neutron and nonresonant x-ray scattering, as well as Raman and infrared conductivity.« less

SECULAR BEHAVIOR OF EXOPLANETS: SELF-CONSISTENCY AND COMPARISONS WITH THE PLANET-PLANET SCATTERING HYPOTHESIS

DOE Office of Scientific and Technical Information (OSTI.GOV)

Timpe, Miles; Barnes, Rory; Kopparapu, Ravikumar

2013-09-15

If mutual gravitational scattering among exoplanets occurs, then it may produce unique orbital properties. For example, two-planet systems that lie near the boundary between circulation and libration of their periapses could result if planet-planet scattering ejected a former third planet quickly, leaving one planet on an eccentric orbit and the other on a circular orbit. We first improve upon previous work that examined the apsidal behavior of known multiplanet systems by doubling the sample size and including observational uncertainties. This analysis recovers previous results that demonstrated that many systems lay on the apsidal boundary between libration and circulation. We thenmore » performed over 12,000 three-dimensional N-body simulations of hypothetical three-body systems that are unstable, but stabilize to two-body systems after an ejection. Using these synthetic two-planet systems, we test the planet-planet scattering hypothesis by comparing their apsidal behavior, over a range of viewing angles, to that of the observed systems and find that they are statistically consistent regardless of the multiplicity of the observed systems. Finally, we combine our results with previous studies to show that, from the sampled cases, the most likely planetary mass function prior to planet-planet scattering follows a power law with index -1.1. We find that this pre-scattering mass function predicts a mutual inclination frequency distribution that follows an exponential function with an index between -0.06 and -0.1.« less

Photometric Properties of Network and faculae derived by HMI data compensated for scattered-light

NASA Astrophysics Data System (ADS)

Criscuoli, Serena; Norton, Aimee Ann; Whitney, Taylor

2017-08-01

We report on the photometric properties of faculae and network as observed in full-disk,scattered-light corrected images from the Helioseismic Magnetic Imager (HMI). We usea Lucy-Richardson deconvolution routine that corrects a full-disk intensity image in lessthan one second. Faculae are distinguished from network through proximity to activeregions in addition to continuum intensity and magnetogram thresholds. This is the firstreport that full-disk image data, including center-to-limb variations, reproduce the photometric properties of faculae and network observed previously only in sub-arcsecond resolution, small field-of-view studies, i.e. that network exhibit in general higher photometric contrasts. More specifically, for magnetic flux values larger than approximately 300 G, the network is always brighter than faculae and the contrast differences increases toward the limb, where the network contrast is about twice the facular one. For lower magnetic flux values, pixels in network regions appear always darker than facular ones. Contrary to reports from previous full-disk observations, we also found that network exhibits a higher center-to-limb variation. Our results are in agreement with reports from simulations that indicate magnetic flux alone is a poor proxy of the photometric properties of magnetic features. We estimate that the facular and network contribution to irradiance variability of the current Cycle 24 is overestimated by at least 11% due to the photometric properties of network and faculae not being recognized as distinctly different.

Radiation Transfer in the Atmosphere: Scattering

NASA Technical Reports Server (NTRS)

Mishchenko, M.; Travis, L.; Lacis, Andrew A.

2014-01-01

Sunlight illuminating the Earth's atmosphere is scattered by gas molecules and suspended particles, giving rise to blue skies, white clouds, and optical displays such as rainbows and halos. By scattering and absorbing the shortwave solar radiation and the longwave radiation emitted by the underlying surface, cloud and aerosol particles strongly affect the radiation budget of the terrestrial climate system. As a consequence of the dependence of scattering characteristics on particle size, morphology, and composition, scattered light can be remarkably rich in information on particle properties and thus provides a sensitive tool for remote retrievals of macro- and microphysical parameters of clouds and aerosols.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Alekseev, A E; Potapov, V T; Gorshkov, B G

We report the results of studying statistical properties of the intensity of partially polarised coherent light backscattered by a single mode optical fibre. An expression is derived for the deviation of the backscattered light intensity depending on the scattering region length, the degree of the light source coherence and the degree of scattered light polarisation. It is shown that the backscattered light in a fibre scattered-light interferometer is partially polarised with the polarisation degree P = 1/3 in the case of external perturbations of the interferometer fibre. (scattering of light)

Three-body unitarity with isobars revisited

DOE Office of Scientific and Technical Information (OSTI.GOV)

Mai, M.; Hu, B.; Döring, M.

The particle exchange model of hadron interactions can be used to describe three-body scattering under the isobar assumption. Here, we start from the 3->3 scattering amplitude for spinless particles, which contains an isobar-spectator scattering amplitude. Using a Bethe-Salpeter Ansatz for the latter, we derive a relativistic three-dimensional scattering equation that manifestly fulfills three-body unitarity and two-body unitarity for the sub-amplitudes. Furthermore, this property holds for energies above breakup and also in the presence of resonances in the sub-amplitudes.

Three-body unitarity with isobars revisited

DOE PAGES

Mai, M.; Hu, B.; Döring, M.; ...

2017-09-08

The particle exchange model of hadron interactions can be used to describe three-body scattering under the isobar assumption. Here, we start from the 3->3 scattering amplitude for spinless particles, which contains an isobar-spectator scattering amplitude. Using a Bethe-Salpeter Ansatz for the latter, we derive a relativistic three-dimensional scattering equation that manifestly fulfills three-body unitarity and two-body unitarity for the sub-amplitudes. Furthermore, this property holds for energies above breakup and also in the presence of resonances in the sub-amplitudes.

On the size dependence of the scattering greenhouse effect of CO2 ice particles

NASA Astrophysics Data System (ADS)

Kitzmann, D.; Patzer, A. B. C.; Rauer, H.

2011-10-01

In this contribution we study the potential greenhouse effect due to scattering of CO2 ice clouds for atmospheric conditions of terrestrial extrasolar planets. Therefore, we calculate the scattering and absorption properties of CO2 ice particles using Mie theory for assumed particle size distributions with different effective radii and particle densities to determine the scattering and absorption characteristics of such clouds. Implications especially in view of a potential greenhouse warming of the planetary surface are discussed.

Computation of the intensities of parametric holographic scattering patterns in photorefractive crystals.

PubMed

Schwalenberg, Simon

2005-06-01

The present work represents a first attempt to perform computations of output intensity distributions for different parametric holographic scattering patterns. Based on the model for parametric four-wave mixing processes in photorefractive crystals and taking into account realistic material properties, we present computed images of selected scattering patterns. We compare these calculated light distributions to the corresponding experimental observations. Our analysis is especially devoted to dark scattering patterns as they make high demands on the underlying model.

Properties of cutoff corrugated surfaces for corrugated horn design. [corrugation shape and density effects on scattering

NASA Technical Reports Server (NTRS)

Mentzer, C. A.; Peters, L., Jr.

1974-01-01

Corrugated horns involve a junction between the corrugated surface and a conducting ground plane. Proper horn design requires an understanding of the electromagnetic properties of the corrugated surface and this junction. An integral equation solution has been used to study the influence of corrugation density and tooth thickness on the power loss, surface current, and the scattering from a ground plane/corrugated surface junction.

Defect Chemistry and Plasmon Physics of Colloidal Metal Oxide Nanocrystals.

PubMed

Lounis, Sebastien D; Runnerstrom, Evan L; Llordés, Anna; Milliron, Delia J

2014-05-01

Plasmonic nanocrystals of highly doped metal oxides have seen rapid development in the past decade and represent a class of materials with unique optoelectronic properties. In this Perspective, we discuss doping mechanisms in metal oxides and the accompanying physics of free carrier scattering, both of which have implications in determining the properties of localized surface plasmon resonances (LSPRs) in these nanocrystals. The balance between activation and compensation of dopants limits the free carrier concentration of the most common metal oxides, placing a ceiling on the LSPR frequency. Furthermore, because of ionized impurity scattering of the oscillating plasma by dopant ions, scattering must be treated in a fundamentally different way in semiconductor metal oxide materials when compared with conventional metals. Though these effects are well-understood in bulk metal oxides, further study is needed to understand their manifestation in nanocrystals and corresponding impact on plasmonic properties, and to develop materials that surpass current limitations in free carrier concentration.

Scattering Properties of Lunar Dust Analogs

NASA Technical Reports Server (NTRS)

Davis, S.; Marshall, J.; Richard, D.; Adler, D.; Adler, B.

2013-01-01

A number of space missions are planned to explore the lunar exosphere which may contain a small population of dust particles. The objective of this paper is to present preliminary results from scattering experiments on a suspension of lunar simulants to support one such mission. The intensity of the light scattered from a lunar simulant is measured with a commercial version of the spectrometer used in the forthcoming LADEE mission. Physical properties of the lunar simulant are described along with two similarly-sized reference microspheres. We confirm that micron-sized particles tend to form agglomerates rather than remaining isolated entities and that certain general characteristic of the target particles can be predicted from intensity measurements alone. These results can be used directly to assess general features of the lunar exosphere from LADEE instrument data. Further analysis of particle properties from such remote sensing data will require measurements of polarization signatures.

TIMING AND INTERSTELLAR SCATTERING OF 35 DISTANT PULSARS DISCOVERED IN THE PALFA SURVEY

DOE Office of Scientific and Technical Information (OSTI.GOV)

Nice, D. J.; Altiere, E.; Farrington, D.

2013-07-20

We have made extensive observations of 35 distant slow (non-recycled) pulsars discovered in the ongoing Arecibo PALFA pulsar survey. Timing observations of these pulsars over several years at Arecibo Observatory and Jodrell Bank Observatory have yielded high-precision positions and measurements of rotation properties. Despite being a relatively distant population, these pulsars have properties that mirror those of the previously known pulsar population. Many of the sources exhibit timing noise, and one underwent a small glitch. We have used multifrequency data to measure the interstellar scattering properties of these pulsars. We find scattering to be higher than predicted along some linesmore » of sight, particularly in the Cygnus region. Finally, we present XMM-Newton and Chandra observations of the youngest and most energetic of the pulsars, J1856+0245, which has previously been associated with the GeV-TeV pulsar wind nebula HESS J1857+026.« less

An Accurate Analytic Approximation for Light Scattering by Non-absorbing Spherical Aerosol Particles

NASA Astrophysics Data System (ADS)

Lewis, E. R.

2017-12-01

The scattering of light by particles in the atmosphere is a ubiquitous and important phenomenon, with applications to numerous fields of science and technology. The problem of scattering of electromagnetic radiation by a uniform spherical particle can be solved by the method of Mie and Debye as a series of terms depending on the size parameter, x=2πr/λ, and the complex index of refraction, m. However, this solution does not provide insight into the dependence of the scattering on the radius of the particle, the wavelength, or the index of refraction, or how the scattering varies with relative humidity. Van de Hulst demonstrated that the scattering efficiency (the scattering cross section divided by the geometric cross section) of a non-absorbing sphere, over a wide range of particle sizes of atmospheric importance, depends not on x and m separately, but on the quantity 2x(m-1); this is the basis for the anomalous diffraction approximation. Here an analytic approximation for the scattering efficiency of a non-absorbing spherical particle is presented in terms of this new quantity that is accurate over a wide range of particle sizes of atmospheric importance and which readily displays the dependences of the scattering efficiency on particle radius, index of refraction, and wavelength. For an aerosol for which the particle size distribution is parameterized as a gamma function, this approximation also yields analytical results for the scattering coefficient and for the Ångström exponent, with the dependences of scattering properties on wavelength and index of refraction clearly displayed. This approximation provides insight into the dependence of light scattering properties on factors such as relative humidity, readily enables conversion of scattering from one index of refraction to another, and demonstrates the conditions under which the aerosol index (the product of the aerosol optical depth and the Ångström exponent) is a useful proxy for the number of cloud condensation nuclei.

Gold Nanoparticle Labels Amplify Ellipsometric Signals

NASA Technical Reports Server (NTRS)

Venkatasubbarao, Srivatsa

2008-01-01

The ellipsometric method reported in the immediately preceding article was developed in conjunction with a method of using gold nanoparticles as labels on biomolecules that one seeks to detect. The purpose of the labeling is to exploit the optical properties of the gold nanoparticles in order to amplify the measurable ellipsometric effects and thereby to enable ultrasensitive detection of the labeled biomolecules without need to develop more-complex ellipsometric instrumentation. The colorimetric, polarization, light-scattering, and other optical properties of nanoparticles depend on their sizes and shapes. In the present method, these size-and-shape-dependent properties are used to magnify the polarization of scattered light and the diattenuation and retardance of signals derived from ellipsometry. The size-and-shape-dependent optical properties of the nanoparticles make it possible to interrogate the nanoparticles by use of light of various wavelengths, as appropriate, to optimally detect particles of a specific type at high sensitivity. Hence, by incorporating gold nanoparticles bound to biomolecules as primary or secondary labels, the performance of ellipsometry as a means of detecting the biomolecules can be improved. The use of gold nanoparticles as labels in ellipsometry has been found to afford sensitivity that equals or exceeds the sensitivity achieved by use of fluorescence-based methods. Potential applications for ellipsometric detection of gold nanoparticle-labeled biomolecules include monitoring molecules of interest in biological samples, in-vitro diagnostics, process monitoring, general environmental monitoring, and detection of biohazards.

Ab initio study of several static and dynamic properties of bulk liquid Ni near melting

NASA Astrophysics Data System (ADS)

del Rio, B. G.; González, L. E.; González, D. J.

2017-01-01

Several static and dynamic properties of bulk liquid Ni at a thermodynamic state near its triple point have been evaluated by ab initio molecular dynamics simulations. The calculated static structure shows very good agreement with the available experimental data, including an asymmetric second peak in the static structure factor, which underlines a marked local icosahedral short-range order in the liquid. The dynamical structure reveals propagating density fluctuations, and the calculated dynamic structure factors, S (q ,ω ) , show a good agreement with the inelastic x-ray scattering measurements. The obtained dispersion relation closely follows that obtained from the inelastic x-ray scattering measurements; moreover we analyze the possible reasons behind its discrepancy with respect to the dispersion relation derived from the inelastic neutron scattering data. The dynamical processes behind the S (q ,ω ) have been analyzed by using a model with two decay channels (a fast and a slow) associated with the relaxations of the collective excitations. We have found that the transverse current spectral functions exhibit some features which, so far, had previously been shown by high pressure liquid metals only. Furthermore, the calculated S (q ,ω ) show, within some q-range, the appearance of transverse-like excitation modes, similar to those recently found in other liquid metals. Finally, results are also reported for several transport coefficients.

Characterizing the weathering induced changes in optical performance and properties of poly(ethylene-terephthalate) via MaPd:RTS spectroscopy

NASA Astrophysics Data System (ADS)

Gordon, Devin A.; DeNoyer, Lin; Meyer, Corey W.; Sweet, Noah W.; Burns, David M.; Bruckman, Laura S.; French, Roger H.

2017-08-01

Poly(ethylene-terephthalate) (PET) film is widely used in photovoltaic module backsheets for its dielectric break- down strength, and in applications requiring high optical clarity for its high transmission in the visible region. However, PET degrades and loses optical clarity under exposure to ultraviolet (UV) irradiance, heat, and moisture. Stabilizers are often included in PET formulation to increase its longevity; however, even these are subject to degradation and further reduce optical clarity. To study the weathering induced changes in the optical properties in PET films, samples of a UV-stabilized grade of PET were exposed to heat, moisture, and UV irradiance as prescribed by ASTM-G154 Cycle 4 for 168 hour time intervals. UV-Vis reflection and transmission spectra were collected via Multi-Angle, Polarization-Dependent, Reflection, Transmission, and Scattering (MaPd:RTS) spectroscopy after each exposure interval. The resulting spectra were used to calculate the complex index of refraction throughout the UV-Vis spectral region via an iterative optimization process based upon the Fresnel equations. The index of refraction and extinction coefficient were found to vary throughout the UV-Vis region with time under exposure. The spectra were also used to investigate changes in light scattering behavior with increasing exposure time. The intensity of scattered light was found to increase at higher angles with time under exposure.

Fluctuating volume-current formulation of electromagnetic fluctuations in inhomogeneous media: Incandescence and luminescence in arbitrary geometries

NASA Astrophysics Data System (ADS)

Polimeridis, Athanasios G.; Reid, M. T. H.; Jin, Weiliang; Johnson, Steven G.; White, Jacob K.; Rodriguez, Alejandro W.

2015-10-01

We describe a fluctuating volume-current formulation of electromagnetic fluctuations that extends our recent work on heat exchange and Casimir interactions between arbitrarily shaped homogeneous bodies [A. W. Rodriguez, M. T. H. Reid, and S. G. Johnson, Phys. Rev. B 88, 054305 (2013), 10.1103/PhysRevB.88.054305] to situations involving incandescence and luminescence problems, including thermal radiation, heat transfer, Casimir forces, spontaneous emission, fluorescence, and Raman scattering, in inhomogeneous media. Unlike previous scattering formulations based on field and/or surface unknowns, our work exploits powerful techniques from the volume-integral equation (VIE) method, in which electromagnetic scattering is described in terms of volumetric, current unknowns throughout the bodies. The resulting trace formulas (boxed equations) involve products of well-studied VIE matrices and describe power and momentum transfer between objects with spatially varying material properties and fluctuation characteristics. We demonstrate that thanks to the low-rank properties of the associated matrices, these formulas are susceptible to fast-trace computations based on iterative methods, making practical calculations tractable. We apply our techniques to study thermal radiation, heat transfer, and fluorescence in complicated geometries, checking our method against established techniques best suited for homogeneous bodies as well as applying it to obtain predictions of radiation from complex bodies with spatially varying permittivities and/or temperature profiles.

Thickness and microstructure effects in the optical and electrical properties of silver thin films

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ding, Guowen, E-mail: gding@intermolecular.com; Clavero, César; Schweigert, Daniel

The optical and electrical response of metal thin films approaching thicknesses in the range of the electron mean free path is highly affected by electronic scattering with the interfaces and defects. Here, we present a theoretical and experimental study on how thickness and microstructure affect the properties of Ag thin films. We are able to successfully model the electrical resistivity and IR optical response using a thickness dependent electronic scattering time. Remarkably, the product of electronic scattering time and resistivity remains constant regardless of the thickness (τx ρ = C), with a value of 59 ± 2 μΩ cm ⋅more » fs for Ag films in the investigated range from 3 to 74 nm. Our findings enable us to develop a theoretically framework that allows calculating the optical response of metal thin films in the IR by using their measured thickness and resistivity. An excellent agreement is found between experimental measurements and predicted values. This study also shows the theoretical lower limit for emissivity in Ag thin films according to their microstructure and thickness. Application of the model presented here will allow rapid characterization of the IR optical response of metal thin films, with important application in a broad spectrum of fundamental and industrial applications, including optical coatings, low-emissivity windows and semiconductor industry.« less

Quantum correlations and Bell’s inequality violation in a Heisenberg spin dimer via neutron scattering

NASA Astrophysics Data System (ADS)

Cruz, C.

The characterization of quantum information quantifiers has attracted a considerable attention of the scientific community, since they are a useful tool to verify the presence of quantum correlations in a quantum system. In this context, in the present work we show a theoretical study of some quantifiers, such as entanglement witness, entanglement of formation, Bell’s inequality violation and geometric quantum discord as a function of the diffractive properties of neutron scattering. We provide one path toward identifying the presence of quantum correlations and quantum nonlocality in a molecular magnet as a Heisenberg spin-1/2 dimer, by diffractive properties typically obtained via neutron scattering experiments.