High-symmetry organic scintillator systems

DOEpatents

Feng, Patrick L.

2017-07-18

An ionizing radiation detector or scintillator system includes a scintillating material comprising an organic crystalline compound selected to generate photons in response to the passage of ionizing radiation. The organic compound has a crystalline symmetry of higher order than monoclinic, for example an orthorhombic, trigonal, tetragonal, hexagonal, or cubic symmetry. A photodetector is optically coupled to the scintillating material, and configured to generate electronic signals having pulse shapes based on the photons generated in the scintillating material. A discriminator is coupled to the photon detector, and configured to discriminate between neutrons and gamma rays in the ionizing radiation based on the pulse shapes of the output signals.

High-symmetry organic scintillator systems

DOEpatents

Feng, Patrick L.

2017-06-14

An ionizing radiation detector or scintillator system includes a scintillating material comprising an organic crystalline compound selected to generate photons in response to the passage of ionizing radiation. The organic compound has a crystalline symmetry of higher order than monoclinic, for example an orthorhombic, trigonal, tetragonal, hexagonal, or cubic symmetry. A photodetector is optically coupled to the scintillating material, and configured to generate electronic signals having pulse shapes based on the photons generated in the scintillating material. A discriminator is coupled to the photon detector, and configured to discriminate between neutrons and gamma rays in the ionizing radiation based on the pulse shapes of the output signals.

High-symmetry organic scintillator systems

DOEpatents

Feng, Patrick L.

2017-09-05

An ionizing radiation detector or scintillator system includes a scintillating material comprising an organic crystalline compound selected to generate photons in response to the passage of ionizing radiation. The organic compound has a crystalline symmetry of higher order than monoclinic, for example an orthorhombic, trigonal, tetragonal, hexagonal, or cubic symmetry. A photodetector is optically coupled to the scintillating material, and configured to generate electronic signals having pulse shapes based on the photons generated in the scintillating material. A discriminator is coupled to the photon detector, and configured to discriminate between neutrons and gamma rays in the ionizing radiation based on the pulse shapes of the output signals.

High-symmetry organic scintillator systems

DOE Office of Scientific and Technical Information (OSTI.GOV)

Feng, Patrick L.

An ionizing radiation detector or scintillator system includes a scintillating material comprising an organic crystalline compound selected to generate photons in response to the passage of ionizing radiation. The organic compound has a crystalline symmetry of higher order than monoclinic, for example an orthorhombic, trigonal, tetragonal, hexagonal, or cubic symmetry. A photodetector is optically coupled to the scintillating material, and configured to generate electronic signals having pulse shapes based on the photons generated in the scintillating material. A discriminator is coupled to the photon detector, and configured to discriminate between neutrons and gamma rays in the ionizing radiation based onmore » the pulse shapes of the output signals.« less

Tomographic analysis of neutron and gamma pulse shape distributions from liquid scintillation detectors at Joint European Torus.

PubMed

Giacomelli, L; Conroy, S; Gorini, G; Horton, L; Murari, A; Popovichev, S; Syme, D B

2014-02-01

The Joint European Torus (JET, Culham, UK) is the largest tokamak in the world devoted to nuclear fusion experiments of magnetic confined Deuterium (D)/Deuterium-Tritium (DT) plasmas. Neutrons produced in these plasmas are measured using various types of neutron detectors and spectrometers. Two of these instruments on JET make use of organic liquid scintillator detectors. The neutron emission profile monitor implements 19 liquid scintillation counters to detect the 2.45 MeV neutron emission from D plasmas. A new compact neutron spectrometer is operational at JET since 2010 to measure the neutron energy spectra from both D and DT plasmas. Liquid scintillation detectors are sensitive to both neutron and gamma radiation but give light responses of different decay time such that pulse shape discrimination techniques can be applied to identify the neutron contribution of interest from the data. The most common technique consists of integrating the radiation pulse shapes within different ranges of their rising and/or trailing edges. In this article, a step forward in this type of analysis is presented. The method applies a tomographic analysis of the 3-dimensional neutron and gamma pulse shape and pulse height distribution data obtained from liquid scintillation detectors such that n/γ discrimination can be improved to lower energies and additional information can be gained on neutron contributions to the gamma events and vice versa.

A first comparison of the responses of a 4He-based fast-neutron detector and a NE-213 liquid-scintillator reference detector

NASA Astrophysics Data System (ADS)

Jebali, R.; Scherzinger, J.; Annand, J. R. M.; Chandra, R.; Davatz, G.; Fissum, K. G.; Friederich, H.; Gendotti, U.; Hall-Wilton, R.; Håkansson, E.; Kanaki, K.; Lundin, M.; Murer, D.; Nilsson, B.; Rosborg, A.; Svensson, H.

2015-09-01

A first comparison has been made between the pulse-shape discrimination characteristics of a novel 4He-based pressurized scintillation detector and a NE-213 liquid-scintillator reference detector using an Am/Be mixed-field neutron and gamma-ray source and a high-resolution scintillation-pulse digitizer. In particular, the capabilities of the two fast neutron detectors to discriminate between neutrons and gamma-rays were investigated. The NE-213 liquid-scintillator reference cell produced a wide range of scintillation-light yields in response to the gamma-ray field of the source. In stark contrast, due to the size and pressure of the 4He gas volume, the 4He-based detector registered a maximum scintillation-light yield of 750keVee to the same gamma-ray field. Pulse-shape discrimination for particles with scintillation-light yields of more than 750keVee was excellent in the case of the 4He-based detector. Above 750keVee its signal was unambiguously neutron, enabling particle identification based entirely upon the amount of scintillation light produced.

Polystyrene-based scintillator with pulse-shape discrimination capability

NASA Astrophysics Data System (ADS)

Zhmurin, P. N.; Lebedev, V. N.; Titskaya, V. D.; Adadurov, A. F.; Elyseev, D. A.; Pereymak, V. N.

2014-10-01

Polystyrene-based scintillators with 2-phenyl-5-(4-tert-butylephenyl)-1,3,4-oxadiazole (tert-BuPPD) or 2,5-di-(3-methylphenyl)-1,3,4 oxadiazole (m-DMePPD) are proposed for pulse-shape n/γ-discrimination. These scintillators have improved mechanical properties, long operational time and high n/γ discrimination parameter - figure of merit (1.49 and 1.81 in a wide energy region), so they can be used as detectors of fast neutrons in the presence of gamma radiation background.

Improving Depth, Energy and Timing Estimation in PET Detectors with Deconvolution and Maximum Likelihood Pulse Shape Discrimination.

PubMed

Berg, Eric; Roncali, Emilie; Hutchcroft, Will; Qi, Jinyi; Cherry, Simon R

2016-11-01

In a scintillation detector, the light generated in the scintillator by a gamma interaction is converted to photoelectrons by a photodetector and produces a time-dependent waveform, the shape of which depends on the scintillator properties and the photodetector response. Several depth-of-interaction (DOI) encoding strategies have been developed that manipulate the scintillator's temporal response along the crystal length and therefore require pulse shape discrimination techniques to differentiate waveform shapes. In this work, we demonstrate how maximum likelihood (ML) estimation methods can be applied to pulse shape discrimination to better estimate deposited energy, DOI and interaction time (for time-of-flight (TOF) PET) of a gamma ray in a scintillation detector. We developed likelihood models based on either the estimated detection times of individual photoelectrons or the number of photoelectrons in discrete time bins, and applied to two phosphor-coated crystals (LFS and LYSO) used in a previously developed TOF-DOI detector concept. Compared with conventional analytical methods, ML pulse shape discrimination improved DOI encoding by 27% for both crystals. Using the ML DOI estimate, we were able to counter depth-dependent changes in light collection inherent to long scintillator crystals and recover the energy resolution measured with fixed depth irradiation (~11.5% for both crystals). Lastly, we demonstrated how the Richardson-Lucy algorithm, an iterative, ML-based deconvolution technique, can be applied to the digitized waveforms to deconvolve the photodetector's single photoelectron response and produce waveforms with a faster rising edge. After deconvolution and applying DOI and time-walk corrections, we demonstrated a 13% improvement in coincidence timing resolution (from 290 to 254 ps) with the LFS crystal and an 8% improvement (323 to 297 ps) with the LYSO crystal.

[Low level alpha activity measurements with pulse shape discrimination--application to the determination of alpha-nuclides in environmental samples].

PubMed

Satoh, K; Noguchi, M; Higuchi, H; Kitamura, K

1984-12-01

Liquid scintillation counting of alpha rays with pulse shape discrimination was applied to the analysis of 226Ra and 239+240Pu in environmental samples and of alpha-emitters in/on a filter paper. The instrument used in this study was either a specially designed detector or a commercial liquid scintillation counter with an automatic sample changer, both of which were connected to the pulse shape discrimination circuit. The background counting rate in alpha energy region of 5-7 MeV was 0.01 or 0.04 cpm/MeV, respectively. The figure of merit indicating the resolving power for alpha- and beta-particles in time spectrum was found to be 5.7 for the commercial liquid scintillation counter.

Significantly different pulse shapes for γ- and α-rays in Gd3Al2Ga3O12:Ce3+ scintillating crystals

NASA Astrophysics Data System (ADS)

Kobayashi, Masaaki; Tamagawa, Yoichi; Tomita, Shougo; Yamamoto, Akihiro; Ogawa, Izumi; Usuki, Yoshiyuki

2012-12-01

We have found that scintillation in Gd3Al2Ga3O12 (GAGG):Ce3+ garnet single crystals has significantly different pulse shapes for 0.662 MeV γ- and 5.47 MeV α-rays. The decay and rise times for γ-rays are smaller by 50% and threefold, respectively, than those for α-rays. Because the GAGG:Ce is a dense, efficient and fast-response scintillator and because it can be grown in large-size single crystals, it should be a promising unified target and a detector material in the study of neutrinoless double beta decay of 160Gd through the use of pulse shape discrimination between the β-ray signals and the α-ray-induced backgrounds.

Signal pulse emulation for scintillation detectors using Geant4 Monte Carlo with light tracking simulation.

PubMed

Ogawara, R; Ishikawa, M

2016-07-01

The anode pulse of a photomultiplier tube (PMT) coupled with a scintillator is used for pulse shape discrimination (PSD) analysis. We have developed a novel emulation technique for the PMT anode pulse based on optical photon transport and a PMT response function. The photon transport was calculated using Geant4 Monte Carlo code and the response function with a BC408 organic scintillator. The obtained percentage RMS value of the difference between the measured and simulated pulse with suitable scintillation properties using GSO:Ce (0.4, 1.0, 1.5 mol%), LaBr3:Ce and BGO scintillators were 2.41%, 2.58%, 2.16%, 2.01%, and 3.32%, respectively. The proposed technique demonstrates high reproducibility of the measured pulse and can be applied to simulation studies of various radiation measurements.

The angular dependence of pulse shape discrimination and detection sensitivity in cylindrical and cubic EJ-309 organic liquid scintillators

NASA Astrophysics Data System (ADS)

Jones, A. R.; Joyce, M. J.

2017-01-01

Liquid scintillators are used widely for neutron detection and for the assay of nuclear materials. However, due to the constituents of the detector and the nitrogen void within the detector cell, usually incorporated to accommodate any expansion that might occur to avoid leakage, fluctuations in detector response have been observed associated with the orientation of the detector when in use. In this work the angular dependence of the pulse-shape discrimination performance in an EJ309 liquid scintillator has been investigated with 252Cf in terms of the separation of γ -ray and neutron events, described quantitatively by the figure-of-merit. A subtle dependence in terms of pulse-shape discrimination is observed. In contrast, a more significant dependence of detection sensitivity with the angle of orientation is evident.

Alpha/beta pulse shape discrimination in plastic scintillation using commercial scintillation detectors.

PubMed

Bagán, H; Tarancón, A; Rauret, G; García, J F

2010-06-18

Activity determination in different types of samples is a current need in many different fields. Simultaneously analysing alpha and beta emitters is now a routine option when using liquid scintillation (LS) and pulse shape discrimination. However, LS has an important drawback, the generation of mixed waste. Recently, several studies have shown the capability of plastic scintillation (PS) as an alternative to LS, but no research has been carried out to determine its capability for alpha/beta discrimination. The objective of this study was to evaluate the capability of PS to discriminate alpha/beta emitters on the basis of pulse shape analysis (PSA). The results obtained show that PS pulses had lower energy than LS pulses. As a consequence, a lower detection efficiency, a shift to lower energies and a better discrimination of beta and a worst discrimination of alpha disintegrations was observed for PS. Colour quenching also produced a decrease in the energy of the particles, as well as the effects described above. It is clear that in PS, the discrimination capability was correlated with the energy of the particles detected. Taking into account the discrimination capabilities of PS, a protocol for the measurement and the calculation of alpha and beta activities in mixtures using PS and commercial scintillation detectors has been proposed. The new protocol was applied to the quantification of spiked river water samples containing a pair of radionuclides ((3)H-(241)Am or (90)Sr/(90)Y-(241)Am) in different activity proportions. The relative errors in all determinations were lower than 7%. These results demonstrate the capability of PS to discriminate alpha/beta emitters on the basis of pulse shape and to quantify mixtures without generating mixed waste. 2010 Elsevier B.V. All rights reserved.

Signal pulse emulation for scintillation detectors using Geant4 Monte Carlo with light tracking simulation

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ogawara, R.; Ishikawa, M., E-mail: masayori@med.hokudai.ac.jp

The anode pulse of a photomultiplier tube (PMT) coupled with a scintillator is used for pulse shape discrimination (PSD) analysis. We have developed a novel emulation technique for the PMT anode pulse based on optical photon transport and a PMT response function. The photon transport was calculated using Geant4 Monte Carlo code and the response function with a BC408 organic scintillator. The obtained percentage RMS value of the difference between the measured and simulated pulse with suitable scintillation properties using GSO:Ce (0.4, 1.0, 1.5 mol%), LaBr{sub 3}:Ce and BGO scintillators were 2.41%, 2.58%, 2.16%, 2.01%, and 3.32%, respectively. The proposedmore » technique demonstrates high reproducibility of the measured pulse and can be applied to simulation studies of various radiation measurements.« less

DOE Office of Scientific and Technical Information (OSTI.GOV)

Mabe, Andrew N.; Glenn, Andrew M.; Carman, M. Leslie

Transparent plastic scintillators with pulse shape discrimination containing 6Li salicylate have been synthesized by bulk polymerization with a maximum 6Li loading of 0.40 wt%. Photoluminescence and scintillation responses to gamma-rays and neutrons are reported in this paper. Plastics containing 6Li salicylate exhibit higher light yields and permit a higher loading of 6Li as compared to previously reported plastics based on lithium 3-phenylsalicylate. However, pulse shape discrimination performance is reduced in lithium salicylate plastics due to the requirement of adding more nonaromatic monomers to the polymer matrix as compared to those based on lithium 3-phenylsalicylate. Finally, reduction in light yield andmore » pulse shape discrimination performance in lithium-loaded plastics as compared to pulse shape discrimination plastics without lithium is interpreted in terms of energy transfer interference by the aromatic lithium salts.« less

Radioanalytical Chemistry for Automated Nuclear Waste Process Monitoring

DOE Office of Scientific and Technical Information (OSTI.GOV)

Devol, Timothy A.

2005-06-01

Comparison of different pulse shape discrimination methods was performed under two different experimental conditions and the best method was identified. Beta/gamma discrimination of 90Sr/90Y and 137Cs was performed using a phoswich detector made of BC400 (2.5 cm OD x 1.2 cm) and BGO (2.5 cm O.D. x 2.5 cm ) scintillators. Alpha/gamma discrimination of 210Po and 137Cs was performed using a CsI:Tl (2.8 x 1.4 x 1.4 cm3) scintillation crystal. The pulse waveforms were digitized with a DGF-4c (X-Ray Instrumentation Associates) and analyzed offline with IGOR Pro software (Wavemetrics, Inc.). The four pulse shape discrimination methods that were compared include:more » rise time discrimination, digital constant fraction discrimination, charge ratio, and constant time discrimination (CTD) methods. The CTD method is the ratio of the pulse height at a particular time after the beginning of the pulse to the time at the maximum pulse height. The charge comparison method resulted in a Figure of Merit (FoM) of 3.3 (9.9 % spillover) and 3.7 (0.033 % spillover) for the phoswich and the CsI:Tl scintillator setups, respectively. The CTD method resulted in a FoM of 3.9 (9.2 % spillover) and 3.2 (0.25 % spillover), respectively. Inverting the pulse shape data typically resulted in a significantly higher FoM than conventional methods, but there was no reduction in % spillover values. This outcome illustrates that the FoM may not be a good scheme for the quantification of a system to perform pulse shape discrimination. Comparison of several pulse shape discrimination (PSD) methods was performed as a means to compare traditional analog and digital PSD methods on the same scintillation pulses. The X-ray Instrumentation Associates DGF-4C (40 Msps, 14-bit) was used to digitize waveforms from a CsI:Tl crystal and BC400/BGO phoswich detector.« less

Improving Depth, Energy and Timing Estimation in PET Detectors with Deconvolution and Maximum Likelihood Pulse Shape Discrimination

PubMed Central

Berg, Eric; Roncali, Emilie; Hutchcroft, Will; Qi, Jinyi; Cherry, Simon R.

2016-01-01

In a scintillation detector, the light generated in the scintillator by a gamma interaction is converted to photoelectrons by a photodetector and produces a time-dependent waveform, the shape of which depends on the scintillator properties and the photodetector response. Several depth-of-interaction (DOI) encoding strategies have been developed that manipulate the scintillator’s temporal response along the crystal length and therefore require pulse shape discrimination techniques to differentiate waveform shapes. In this work, we demonstrate how maximum likelihood (ML) estimation methods can be applied to pulse shape discrimination to better estimate deposited energy, DOI and interaction time (for time-of-flight (TOF) PET) of a gamma ray in a scintillation detector. We developed likelihood models based on either the estimated detection times of individual photoelectrons or the number of photoelectrons in discrete time bins, and applied to two phosphor-coated crystals (LFS and LYSO) used in a previously developed TOF-DOI detector concept. Compared with conventional analytical methods, ML pulse shape discrimination improved DOI encoding by 27% for both crystals. Using the ML DOI estimate, we were able to counter depth-dependent changes in light collection inherent to long scintillator crystals and recover the energy resolution measured with fixed depth irradiation (~11.5% for both crystals). Lastly, we demonstrated how the Richardson-Lucy algorithm, an iterative, ML-based deconvolution technique, can be applied to the digitized waveforms to deconvolve the photodetector’s single photoelectron response and produce waveforms with a faster rising edge. After deconvolution and applying DOI and time-walk corrections, we demonstrated a 13% improvement in coincidence timing resolution (from 290 to 254 ps) with the LFS crystal and an 8% improvement (323 to 297 ps) with the LYSO crystal. PMID:27295658

Stabilization of Particle Discrimination Efficiencies for Neutron Spectrum Unfolding With Organic Scintillators

NASA Astrophysics Data System (ADS)

Lawrence, Chris C.; Polack, J. K.; Febbraro, Michael; Kolata, J. J.; Flaska, Marek; Pozzi, S. A.; Becchetti, F. D.

2017-02-01

The literature discussing pulse-shape discrimination (PSD) in organic scintillators dates back several decades. However, little has been written about PSD techniques that are optimized for neutron spectrum unfolding. Variation in n-γ misclassification rates and in γ/n ratio of incident fields can distort the neutron pulse-height response of scintillators and these distortions can in turn cause large errors in unfolded spectra. New applications in arms-control verification call for detection of lower-energy neutrons, for which PSD is particularly problematic. In this article, we propose techniques for removing distortions on pulse-height response that result from the merging of PSD distributions in the low-pulse-height region. These techniques take advantage of the repeatable shapes of PSD distributions that are governed by the counting statistics of scintillation-photon populations. We validate the proposed techniques using accelerator-based time-of-flight measurements and then demonstrate them by unfolding the Watt spectrum from measurement with a 252Cf neutron source.

An algorithm for charge-integration, pulse-shape discrimination and estimation of neutron/photon misclassification in organic scintillators

NASA Astrophysics Data System (ADS)

Polack, J. K.; Flaska, M.; Enqvist, A.; Sosa, C. S.; Lawrence, C. C.; Pozzi, S. A.

2015-09-01

Organic scintillators are frequently used for measurements that require sensitivity to both photons and fast neutrons because of their pulse shape discrimination capabilities. In these measurement scenarios, particle identification is commonly handled using the charge-integration pulse shape discrimination method. This method works particularly well for high-energy depositions, but is prone to misclassification for relatively low-energy depositions. A novel algorithm has been developed for automatically performing charge-integration pulse shape discrimination in a consistent and repeatable manner. The algorithm is able to estimate the photon and neutron misclassification corresponding to the calculated discrimination parameters, and is capable of doing so using only the information measured by a single organic scintillator. This paper describes the algorithm and assesses its performance by comparing algorithm-estimated misclassification to values computed via a more traditional time-of-flight estimation. A single data set was processed using four different low-energy thresholds: 40, 60, 90, and 120 keVee. Overall, the results compared well between the two methods; in most cases, the algorithm-estimated values fell within the uncertainties of the TOF-estimated values.

Measurement of ortho-positronium properties in liquid scintillators

NASA Astrophysics Data System (ADS)

Perasso, S.; Consolati, G.; Franco, D.; Jollet, C.; Meregaglia, A.; Tonazzo, A.; Yeh, M.

2014-03-01

Pulse shape discrimination is a well-established technique for background rejection in liquid scintillator detectors. It is particularly effective in separating heavy particles from light particles, but not in distinguishing electrons from positrons. This inefficiency can be overtaken by exploiting the formation of ortho-positronium (o-Ps), which alters the time profile of light pulses induced by positrons. We characterized the o-Ps properties in the most commonly used liquid scintillators, i.e. PC, PXE, LAB, OIL and PC + PPO. In addition, we studied the effects of scintillator doping on the o-Ps properties for dopants used in neutrino-less double beta decay experiments (Nd and Te) and in anti-neutrino and neutron detection (Gd and Li respectively). We found that the o-Ps properties are similar in all the tested scintillators, with a lifetime around 3 ns and a formation probability of about 50%. This result indicates that an o-Ps-enhanced pulse shape discrimination can be applied in liquid scintillator detectors for neutrino and anti-neutrino detection and for neutrino-less double beta decay search.

Improved pulse shape discrimination in EJ-301 liquid scintillators

NASA Astrophysics Data System (ADS)

Lang, R. F.; Masson, D.; Pienaar, J.; Röttger, S.

2017-06-01

Digital pulse shape discrimination has become readily available to distinguish nuclear recoil and electronic recoil events in scintillation detectors. We evaluate digital implementations of pulse shape discrimination algorithms discussed in the literature, namely the Charge Comparison Method, Pulse-Gradient Analysis, Fourier Series and Standard Event Fitting. In addition, we present a novel algorithm based on a Laplace Transform. Instead of comparing the performance of these algorithms based on a single Figure of Merit, we evaluate them as a function of recoil energy. Specifically, using commercial EJ-301 liquid scintillators, we examined both the resulting acceptance of nuclear recoils at a given rejection level of electronic recoils, as well as the purity of the selected nuclear recoil event samples. We find that both a Standard Event fit and a Laplace Transform can be used to significantly improve the discrimination capabilities over the whole considered energy range of 0 - 800keVee . Furthermore, we show that the Charge Comparison Method performs poorly in accurately identifying nuclear recoils.

Real-Time, Digital Pulse-Shape Discrimination in Non-Hazardous Fast Liquid Scintillation Detectors: Prospects for Safety and Security

NASA Astrophysics Data System (ADS)

Joyce, Malcolm J.; Aspinall, Michael D.; Cave, Francis D.; Lavietes, Anthony D.

2012-08-01

Pulse-shape discrimination (PSD) in fast, organic scintillation detectors is a long-established technique used to separate neutrons and γ rays in mixed radiation fields. In the analogue domain the method can achieve separation in real time, but all knowledge of the pulses themselves is lost thereby preventing the possibility of any post- or repeated analysis. Also, it is typically reliant on electronic systems that are largely obsolete and which require significant experience to set up. In the digital domain, PSD is often more flexible but significant post-processing has usually been necessary to obtain neutron/γ-ray separation. Moreover, the scintillation media on which the technique relies usually have a low flashpoint and are thus deemed hazardous. This complicates the ease with which they are used in industrial applications. In this paper, results obtained with a new portable digital pulse-shape discrimination instrument are described. This instrument provides real-time, digital neutron/γ-ray separation whilst preserving the synchronization with the time-of-arrival for each event, and realizing throughputs of 3 × 106 events per second. Furthermore, this system has been tested with a scintillation medium that is non-flammable and not hazardous.

Determination of 243Am by pulse shape discrimination liquid scintillation spectrometry.

PubMed

Alamelu, D; Bhade, S P D; Reddy, P J; Narayan, K K; Shah, P M; Aggarwal, S K

2006-05-01

Alpha specific activity of 243Am was determined using pulse shape discrimination in liquid scintillation spectrometry. 238Pu, 36Cl and 239Np (purified from 243Am) were used for obtaining the spillover of alpha/beta particles into the beta/alpha channels, respectively. Synthetic mixtures of 241Am/243Am were prepared. Using the alpha-specific activity, weights of the stock solutions used and the half-life of 241Am and 243Am isotopes, the expected 241Am/243Am atom ratios in the mixtures were determined and compared with those obtained by thermal ionization mass spectrometry (TIMS). An agreement of about 1% was obtained between the 241Am/243Am atom ratios determined by the two methods. This shows that liquid scintillation counting with pulse shape discrimination can be used for 243Am determination with an accuracy better than 1%.

Recent developments in plastic scintillators with pulse shape discrimination

NASA Astrophysics Data System (ADS)

Zaitseva, N. P.; Glenn, A. M.; Mabe, A. N.; Carman, M. L.; Hurlbut, C. R.; Inman, J. W.; Payne, S. A.

2018-05-01

The paper reports results of studies conducted to improve scintillation performance of plastic scintillators capable of neutron/gamma pulse-shape discrimination (PSD). Compositional modifications made with the polymer matrix improved physical stability, allowing for increased loads of the primary dye that, in combination with selected secondary dyes, provided enhanced PSD especially important for the lower energy ranges. Additional measurements were made with a newly-introduced PSD plastic EJ-276, that replaces the first commercially produced EJ-299. Comparative studies conducted with the new materials and EJ-309 liquids at large scale (up to 10 cm) show that current plastics may provide scintillation and PSD performance sufficient for the replacement of liquid scintillators. Comparison to stilbene single crystals compliments the information about the status of the solid-state materials recently developed for fast neutron detection applications.

Improved (10)B-loaded liquid scintillator with pulse-shape discrimination.

PubMed

Greenwood, L R; Chellew, N R

1979-04-01

An improved (10)B-loaded liquid scintillator solution has been developed containing trimethylborate, 1-methylnaphthalene, and 9,10-diphenylanthracene. Cells up to 5 cm in diameter by 15.2 cm long have been prepared and tested with (10)B-loadings up to 7.2% by weight (80% trimethylborate). The solution has excellent light output and pulse-shape discrimination properties and is stable at temperatures as low as -17 degrees C. Neutron efficiency calculations are also presented.

Study of the peak shape in alpha spectra measured by liquid scintillation

NASA Astrophysics Data System (ADS)

Vera Tomé, F.; Gómez Escobar, V.; Martín Sánchez, A.

2002-06-01

Liquid-scintillation counting allows the measurement of alpha and beta activities jointly or only of the alpha-emitting nuclides in a sample. Although the resolution of the alpha spectra is poorer than that attained with semiconductor detectors, it is still an attractive alternative. We describe here attempts to fit a peak shape to experimental liquid-scintillation alpha spectra and discuss the parameters affecting this shape, such as the PSA (pulse-shape analyser) level, vial type, shaking the sample, etc. Spectral analysis has been applied for complex alpha spectra.

Light collection and pulse-shape discrimination in elongated scintillator cells for the PROSPECT reactor antineutrino experiment

NASA Astrophysics Data System (ADS)

Ashenfelter, J.; Balantekin, B.; Band, H. R.; Barclay, G.; Bass, C. D.; Berish, D.; Bowden, N. S.; Bowes, A.; Brodsky, J. P.; Bryan, C. D.; Cherwinka, J. J.; Chu, R.; Classen, T.; Commeford, K.; Davee, D.; Dean, D.; Deichert, G.; Diwan, M. V.; Dolinski, M. J.; Dolph, J.; Dwyer, D. A.; Gaison, J. K.; Galindo-Uribarri, A.; Gilje, K.; Glenn, A.; Goddard, B. W.; Green, M.; Han, K.; Hans, S.; Heeger, K. M.; Heffron, B.; Jaffe, D. E.; Langford, T. J.; Littlejohn, B. R.; Martinez Caicedo, D. A.; McKeown, R. D.; Mendenhall, M. P.; Mueller, P.; Mumm, H. P.; Napolitano, J.; Neilson, R.; Norcini, D.; Pushin, D.; Qian, X.; Romero, E.; Rosero, R.; Saldana, L.; Seilhan, B. S.; Sharma, R.; Sheets, S.; Stemen, N. T.; Surukuchi, P. T.; Varner, R. L.; Viren, B.; Wang, W.; White, B.; White, C.; Wilhelmi, J.; Williams, C.; Wise, T.; Yao, H.; Yeh, M.; Yen, Y. R.; Zangakis, G.; Zhang, C.; Zhang, X.

2015-11-01

A meter-long, 23-liter EJ-309 liquid scintillator detector has been constructed to study the light collection and pulse-shape discrimination performance of elongated scintillator cells for the PROSPECT reactor antineutrino experiment. The magnitude and uniformity of light collection and neutron-gamma discrimination power in the energy range of antineutrino inverse beta decay products have been studied using gamma and spontaneous fission calibration sources deployed along the cell axis. We also study neutron-gamma discrimination and light collection abilities for differing PMT and reflector configurations. Key design features for optimizing MeV-scale response and background rejection capabilities are identified.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Giacomelli, L.; Department of Physics, Università degli Studi di Milano-Bicocca, Milano; Conroy, S.

The Joint European Torus (JET, Culham, UK) is the largest tokamak in the world devoted to nuclear fusion experiments of magnetic confined Deuterium (D)/Deuterium-Tritium (DT) plasmas. Neutrons produced in these plasmas are measured using various types of neutron detectors and spectrometers. Two of these instruments on JET make use of organic liquid scintillator detectors. The neutron emission profile monitor implements 19 liquid scintillation counters to detect the 2.45 MeV neutron emission from D plasmas. A new compact neutron spectrometer is operational at JET since 2010 to measure the neutron energy spectra from both D and DT plasmas. Liquid scintillation detectorsmore » are sensitive to both neutron and gamma radiation but give light responses of different decay time such that pulse shape discrimination techniques can be applied to identify the neutron contribution of interest from the data. The most common technique consists of integrating the radiation pulse shapes within different ranges of their rising and/or trailing edges. In this article, a step forward in this type of analysis is presented. The method applies a tomographic analysis of the 3-dimensional neutron and gamma pulse shape and pulse height distribution data obtained from liquid scintillation detectors such that n/γ discrimination can be improved to lower energies and additional information can be gained on neutron contributions to the gamma events and vice versa.« less

Study of pulse shape discrimination for a neutron phoswich detector

NASA Astrophysics Data System (ADS)

Hartman, Jessica; Barzilov, Alexander

2017-09-01

A portable phoswich detector capable of differentiating between fast neutrons and thermal neutrons, and photons was developed. The detector design is based on the use of two solid-state scintillators with dissimilar scintillation time properties coupled with a single optical sensor: a 6Li loaded glass and EJ-299-33A plastic. The on-the-fly digital pulse shape discrimination and the wavelet treatment of measured waveforms were employed in the data analysis. The instrument enabled neutron spectrum evaluation.

Pulse-shape discrimination of the new plastic scintillators in neutron-gamma mixed field using fast digitizer card

NASA Astrophysics Data System (ADS)

Jančář, A.; Kopecký, Z.; Dressler, J.; Veškrna, M.; Matěj, Z.; Granja, C.; Solar, M.

2015-11-01

Recently invented plastic scintillator EJ-299-33 enables pulse-shape discrimination (PSD) and thus measurement of neutron and photon spectra in mixed fields. In this work we compare the PSD properties of EJ-299-33 plastic and the well-known NE-213 liquid scintillator in monoenergetic neutron fields generated by the Van de Graaff accelerator using the 3H(d, n)4He reaction. Pulses from the scintillators are processed by a newly developed digital measuring system employing the fast digitizer card. This card contains two AD converters connected to the measuring computer via 10 Gbps optical ethernet. The converters operate with a resolution of 12 bits and have two differential inputs with a sampling frequency 1 GHz. The resulting digital channels with different gains are merged into one composite channel with a higher digital resolution in a wide dynamic range of energies. Neutron signals are fully discriminated from gamma signals. Results are presented.

The light-yield response of a NE-213 liquid-scintillator detector measured using 2-6 MeV tagged neutrons

NASA Astrophysics Data System (ADS)

Scherzinger, J.; Al Jebali, R.; Annand, J. R. M.; Fissum, K. G.; Hall-Wilton, R.; Kanaki, K.; Lundin, M.; Nilsson, B.; Perrey, H.; Rosborg, A.; Svensson, H.

2016-12-01

The response of a NE-213 liquid-scintillator detector has been measured using tagged neutrons from 2 to 6 MeV originating from an Am/Be neutron source. The neutron energies were determined using the time-of-flight technique. Pulse-shape discrimination was employed to discern between gamma-rays and neutrons. The behavior of both the fast (35 ns) and the combined fast and slow (475 ns) components of the neutron scintillation-light pulses were studied. Three different prescriptions were used to relate the neutron maximum energy-transfer edges to the corresponding recoil-proton scintillation-light yields, and the results were compared to simulations. The overall normalizations of parametrizations which predict the fast or total light yield of the scintillation pulses were also tested. Our results agree with both existing data and existing parametrizations. We observe a clear sensitivity to the portion and length of the neutron scintillation-light pulse considered.

Light collection and pulse-shape discrimination in elongated scintillator cells for the PROSPECT reactor antineutrino experiment

DOE PAGES

Ashenfelter, J.; Jaffe, D.; Diwan, M. V.; ...

2015-11-06

A meter-long, 23-liter EJ-309 liquid scintillator detector has been constructed to study the light collection and pulse-shape discrimination performance of elongated scintillator cells for the PROSPECT reactor antineutrino experiment. The magnitude and uniformity of light collection and neutron-gamma discrimination power in the energy range of antineutrino inverse beta decay products have been studied using gamma and spontaneous fission calibration sources deployed along the cell axis. We also study neutron-gamma discrimination and light collection abilities for differing PMT and reflector configurations. As a result, key design features for optimizing MeV-scale response and background rejection capabilities are identified.

(6)Li-loaded liquid scintillators with pulse shape discrimination.

PubMed

Greenwood, L R; Chellew, N R; Zarwell, G A

1979-04-01

Excellent pulse height and pulse shape discrimination performance has been obtained for liquid scintillators containing as much as 10 wt.% (6)Li-salicylate dissolved in a toluene-methanol solvent system using naphthalene and 9,10 diphenylanthracene as intermediate and secondary solutes. This solution has improved performance at higher (6)Li-loading than solutions in dioxane-water solvent systems, and remains stable at temperatures as low as -10 degrees C. Cells as large as 5 cm in diameter and 15.2 deep have been prepared which have a higher light output for slow neutron detection than (10)B-loaded liquids. Neutron efficiency calculations are also presented.

Structural Origins of Scintillation: Metal Organic Frameworks as a Nanolaboratory

DTIC Science & Technology

2016-06-01

scintillation response and thus the ability to perform neutron/gamma particle discrimination via pulse-shape discrimination ( PSD ). Unfortunately, the...defined an alternative approach towards particle discrimination that addresses the limitations of conventional PSD organic scintillators. This approach...discrimination ( PSD ), for which the prompt component of the scintillation response is quenched for high specific energy loss (dE/dX) particles such as protons

Optimization of a Fast Neutron Scintillator for Real-Time Pulse Shape Discrimination in the Transient Reactor Test Facility (TREAT) Hodoscope

DOE Office of Scientific and Technical Information (OSTI.GOV)

Johnson, James T.; Thompson, Scott J.; Watson, Scott M.

We present a multi-channel, fast neutron/gamma ray detector array system that utilizes ZnS(Ag) scintillator detectors. The system employs field programmable gate arrays (FPGAs) to do real-time all digital neutron/gamma ray discrimination with pulse height and time histograms to allow count rates in excess of 1,000,000 pulses per second per channel. The system detector number is scalable in blocks of 16 channels.

Characterization of ParTI Phoswiches Using Charged Pion Beams

NASA Astrophysics Data System (ADS)

Churchman, Emily; Zarrella, Andrew; Youngs, Michael; Yennello, Sherry

2017-09-01

The Partial Truncated Icosahedron (ParTI) detector array consists of 15 phoswiches. Each phoswich is made of two scintillating components - a thallium-doped cesium iodide (CsI(Tl)) crystal and an EJ-212 scintillating plastic - coupled to a photomultiplier tube. Both materials have different scintillation times and are sensitive to both charged and neutral particles. The type of particle and amount of energy deposited determine the shape of the scintillation pulse as a function of time. By integrating the fast and slow signals of the scintillation pulses, a ``Fast vs. Slow Integration'' plot can be created that produces particle identification lines based on the energy deposited in the scintillating materials. Four of these phoswiches were taken to the Paul Scherrer Institute (PSI) in Switzerland where π + , π-, and proton beams were scattered onto the phoswiches to demonstrate their particle identification (PID) capabilities. Using digitizers to record the detector response waveforms, pions can also be identified by the characteristic decay pulse of the muon daughters.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kelley, R.P., E-mail: rpkelley@ufl.edu; Ray, H.; Jordan, K.A.

An empirical investigation of the scintillation mechanism in a pressurized {sup 4}He gas fast neutron detector was conducted using pulse shape fitting. Scintillation signals from neutron interactions were measured and averaged to produce a single generic neutron pulse shape from both a {sup 252}Cf spontaneous fission source and a (d,d) neutron generator. An expression for light output over time was then developed by treating the decay of helium excited states in the same manner as the decay of radioactive isotopes. This pulse shape expression was fitted to the measured neutron pulse shape using a least-squares optimization algorithm, allowing an empiricalmore » analysis of the mechanism of scintillation inside the {sup 4}He detector. A further understanding of this mechanism in the {sup 4}He detector will advance the use of this system as a neutron spectrometer. For {sup 252}Cf neutrons, the triplet and singlet time constants were found to be 970 ns and 686 ns, respectively. For neutrons from the (d,d) generator, the time constants were found to be 884 ns and 636 ns. Differences were noted in the magnitude of these parameters compared to previously published data, however the general relationships were noted to be the same and checked with expected trends from theory. Of the excited helium states produced from a {sup 252}Cf neutron interaction, 76% were found to be born as triplet states, similar to the result from the neutron generator of 71%. The two sources yielded similar pulse shapes despite having very different neutron energy spectra, validating the robustness of the fits across various neutron energies.« less

Measurement of ortho-positronium properties in liquid scintillators

NASA Astrophysics Data System (ADS)

Perasso, S.; Consolati, G.; Franco, D.; Hans, S.; Jollet, C.; Meregaglia, A.; Tonazzo, A.; Yeh, M.

2013-08-01

Pulse shape discrimination in liquid scintillator detectors is a well-established technique for the discrimination of heavy particles from light particles. Nonetheless, it is not efficient in the separation of electrons and positrons, as they give rise to indistinguishable scintillator responses. This inefficiency can be overtaken through the exploitation of the formation of ortho-Positronium (o-Ps), which alters the time profile of light pulses induced by positrons. We characterized the o-Ps properties in the most commonly used liquid scintillators, i.e. PC, PXE, LAB, OIL and PC + PPO. In addition, we studied the effects of scintillator doping on the o-Ps properties for dopants currently used in neutrino experiments, Gd and Nd. Further measurements for Li-loaded and Tl-loaded liquid scintillators are foreseen. We found that the o-Ps properties are suitable for enhancing the electron-positron discrimination.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Dalla Palma, M.; Quaranta, A.; INFN, Laboratori Nazionali di Legnaro,Viale dell'Universita, 2, 35020 Legnaro - Padova

In the last decade, attention toward neutron detection has been growing in the scientific community, driven by new requirements in different fields of application ranging from homeland security to medical and material analysis, from research physics, to nuclear energy production. So far neutron detection, with particular attention to fast neutrons, has been mainly based on organic liquid scintillators, owing to their good efficiency and pulse shape discrimination (PSD) capability. Most of these liquids have however some main drawbacks given by toxicity, flammability, volatility and sensitivity to dissolved oxygen that limits the duration and the quality of their performances with worsemore » handiness and increased costs. Phenyl-substituted polysiloxanes could address most of these issues, being characterized by low toxicity, low volatility and low flammability. Their optical properties can be tailored by changing the phenyl distribution and concentration thus allowing to increase the solubility of organic dyes, to modify the fluorescence spectra and to vary the refractive index of the medium. Furthermore, polysiloxanes have been recently exploited for the production of plastic scintillators with very good chemical and thermal stability and very good radiation hardness and the development of polysiloxane liquid scintillators could allow to combine these interesting properties with the supremacy of liquid scintillators as regarding PSD over plastics. For these reasons, the properties of several phenyl-substituted polysiloxane with different phenyl amounts and different viscosities have been investigated, with particular attention to the scintillation response and the pulse shape discrimination capability, and the results of the investigation are reported in this work. More in details, the scintillation light yield towards gamma rays ({sup 60}Co and {sup 137}Cs) of several polysiloxane liquids has been analyzed and compared with the light yield of a commercial non-toxic liquid scintillator (EJ309). The results have been related to the optical characterization of these materials, especially as regarding the fluorescence response, and the best performing material (1,1,5,5-Tetraphenyl 1,3,3,5-Tetramethyl Trisiloxane) showed a scintillation light-yield only slightly lower than EJ309, proving to be a promising candidate for the production of an efficient polysiloxane based liquid scintillator. The results as regarding the neutron-gamma pulse shape discrimination capability of the best performing materials are also reported in this work and the scintillation decay time of these materials are compared to the results of fluorescence lifetime analysis. PSD tests have been performed at CN accelerator in Legnaro National Laboratories with a 2.2 MeV pulsed neutron beam using TOF procedure and the pulses have been analyzed in order to evidence the PSD capability of every sample. The reported results pave the way to the development of a new promising class of non-toxic liquid scintillating materials for neutron detection, with good light output and interesting PSD characteristics. (authors)« less

Energy calibration of organic scintillation detectors for. gamma. rays

DOE Office of Scientific and Technical Information (OSTI.GOV)

Gu Jiahui; Xiao Genlai; Liu Jingyi

1988-10-01

An experimental method of calibrating organic detectors is described. A NaI(T1) detector has some advantages of high detection efficiency, good energy resolution, and definite position of the back-scattering peak. The precise position of the Compton edge can be determined by coincidence measurement between the pulse of an organic scintillation detector and the pulse of the back-scattering peak from NaI(T1) detector. It can be used to calibrate various sizes and shapes of organic scintillation detectors simply and reliably. The home-made plastic and organic liquid scintillation detectors are calibrated and positions of the Compton edge as a function of ..gamma..-ray energies aremore » obtained.« less

Mixture quantification using PLS in plastic scintillation measurements.

PubMed

Bagán, H; Tarancón, A; Rauret, G; García, J F

2011-06-01

This article reports the capability of plastic scintillation (PS) combined with multivariate calibration (Partial least squares; PLS) to detect and quantify alpha and beta emitters in mixtures. While several attempts have been made with this purpose in mind using liquid scintillation (LS), no attempt was done using PS that has the great advantage of not producing mixed waste after the measurements are performed. Following this objective, ternary mixtures of alpha and beta emitters ((241)Am, (137)Cs and (90)Sr/(90)Y) have been quantified. Procedure optimisation has evaluated the use of the net spectra or the sample spectra, the inclusion of different spectra obtained at different values of the Pulse Shape Analysis parameter and the application of the PLS1 or PLS2 algorithms. The conclusions show that the use of PS+PLS2 applied to the sample spectra, without the use of any pulse shape discrimination, allows quantification of the activities with relative errors less than 10% in most of the cases. This procedure not only allows quantification of mixtures but also reduces measurement time (no blanks are required) and the application of this procedure does not require detectors that include the pulse shape analysis parameter. Copyright © 2011 Elsevier Ltd. All rights reserved.

Pulse Shape Analysis and Discrimination for Silicon-Photomultipliers in Helium-4 Gas Scintillation Neutron Detector

NASA Astrophysics Data System (ADS)

Barker, Cathleen; Zhu, Ting; Rolison, Lucas; Kiff, Scott; Jordan, Kelly; Enqvist, Andreas

2018-01-01

Using natural helium (helium-4), the Arktis 180-bar pressurized gas scintillator is capable of detecting and distinguishing fast neutrons and gammas. The detector has a unique design of three optically separated segments in which 12 silicon-photomultiplier (SiPM) pairs are positioned equilaterally across the detector to allow for them to be fully immersed in the helium-4 gas volume; consequently, no additional optical interfaces are necessary. The SiPM signals were amplified, shaped, and readout by an analog board; a 250 MHz, 14-bit digitizer was used to examine the output pulses from each SiPMpair channel. The SiPM over-voltage had to be adjusted in order to reduce pulse clipping and negative overshoot, which was observed for events with high scintillation production. Pulse shaped discrimination (PSD) was conducted by evaluating three different parameters: time over threshold (TOT), pulse amplitude, and pulse integral. In order to differentiate high and low energy events, a 30ns gate window was implemented to group pulses from two SiPM channels or more for the calculation of TOT. It was demonstrated that pulses from a single SiPM channel within the 30ns window corresponded to low-energy gamma events while groups of pulses from two-channels or more were most likely neutron events. Due to gamma pulses having lower pulse amplitude, the percentage of measured gamma also depends on the threshold value in TOT calculations. Similarly, the threshold values were varied for the optimal PSD methods of using pulse amplitude and pulse area parameters. Helium-4 detectors equipped with SiPMs are excellent for in-the-field radiation measurement of nuclear spent fuel casks. With optimized PSD methods, the goal of developing a fuel cask content monitoring and inspection system based on these helium-4 detectors will be achieved.

Neutron Spectroscopy for pulsed beams with frame overlap using a double time-of-flight technique

NASA Astrophysics Data System (ADS)

Harrig, K. P.; Goldblum, B. L.; Brown, J. A.; Bleuel, D. L.; Bernstein, L. A.; Bevins, J.; Harasty, M.; Laplace, T. A.; Matthews, E. F.

2018-01-01

A new double time-of-flight (dTOF) neutron spectroscopy technique has been developed for pulsed broad spectrum sources with a duty cycle that results in frame overlap, where fast neutrons from a given pulse overtake slower neutrons from previous pulses. Using a tunable beam at the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory, neutrons were produced via thick-target breakup of 16 MeV deuterons on a beryllium target in the cyclotron vault. The breakup spectral shape was deduced from a dTOF measurement using an array of EJ-309 organic liquid scintillators. Simulation of the neutron detection efficiency of the scintillator array was performed using both GEANT4 and MCNP6. The efficiency-corrected spectral shape was normalized using a foil activation technique to obtain the energy-dependent flux of the neutron beam at zero degrees with respect to the incoming deuteron beam. The dTOF neutron spectrum was compared to spectra obtained using HEPROW and GRAVEL pulse height spectrum unfolding techniques. While the unfolding and dTOF results exhibit some discrepancies in shape, the integrated flux values agree within two standard deviations. This method obviates neutron time-of-flight spectroscopy challenges posed by pulsed beams with frame overlap and opens new opportunities for pulsed white neutron source facilities.

Combination neutron-gamma ray detector

DOEpatents

Stuart, Travis P.; Tipton, Wilbur J.

1976-10-26

A radiation detection system capable of detecting neutron and gamma events and distinguishing therebetween. The system includes a detector for a photomultiplier which utilizes a combination of two phosphor materials, the first of which is in the form of small glass beads which scintillate primarily in response to neutrons and the second of which is a plastic matrix which scintillates in response to gammas. A combination of pulse shape and pulse height discrimination techniques is utilized to provide an essentially complete separation of the neutron and gamma events.

Continuous depth-of-interaction encoding using phosphor-coated scintillators.

PubMed

Du, Huini; Yang, Yongfeng; Glodo, Jarek; Wu, Yibao; Shah, Kanai; Cherry, Simon R

2009-03-21

We investigate a novel detector using a lutetium oxyorthosilicate (LSO) scintillator and YGG (yttrium-aluminum-gallium oxide:cerium, Y(3)(Al,Ga)(5)O(12):Ce) phosphor to construct a detector with continuous depth-of-interaction (DOI) information. The far end of the LSO scintillator is coated with a thin layer of YGG phosphor powder which absorbs some fraction of the LSO scintillation light and emits wavelength-shifted photons with a characteristic decay time of approximately 50 ns. The near end of the LSO scintillator is directly coupled to a photodetector. The photodetector detects a mixture of the LSO light and the light emitted by YGG. With appropriate placement of the coating, the ratio of the light converted from the YGG coating with respect to the unconverted LSO light can be made to depend on the interaction depth. DOI information can then be estimated by inspecting the overall light pulse decay time. Experiments were conducted to optimize the coating method. 19 ns decay time differences across the length of the detector were achieved experimentally when reading out a 1.5 x 1.5 x 20 mm(3) LSO crystal with unpolished surfaces and half-coated with YGG phosphor. The same coating scheme was applied to a 4 x 4 LSO array. Pulse shape discrimination (PSD) methods were studied to extract DOI information from the pulse shape changes. The DOI full-width-half-maximum (FWHM) resolution was found to be approximately 8 mm for this 2 cm thick array.

Continuous Depth-of-Interaction Encoding Using Phosphor-Coated Scintillators

PubMed Central

Du, Huini; Yang, Yongfeng; Glodo, Jarek; Wu, Yibao; Shah, Kanai; Cherry, Simon R.

2009-01-01

We investigate a novel detector using lutetium oxyorthosilicate (LSO) scintillator and YGG (yttrium aluminum gallium oxide:cerium, Y3(Al,Ga)5O12:Ce) phosphor to construct a detector with continuous depth-of-interaction (DOI) information. The far end of the LSO scintillator is coated with a thin layer of YGG phosphor powder which absorbs some fraction of the LSO scintillation light and emits wavelength-shifted photons with a characteristic decay time of ∼ 50 ns. The near end of the LSO scintillator is directly coupled to a photodetector. The photodetector detects a mixture of the LSO light and the light emitted by YGG. With appropriate placement of the coating, the ratio of the light converted from the YGG coating with respect to the unconverted LSO light can be made to depend on the interaction depth. DOI information can then be estimated by inspecting the overall light pulse decay time. Experiments were conducted to optimize the coating method. 19 ns decay time differences across the length of the detector were achieved experimentally when reading out a 1.5×1.5×20 mm3 LSO crystal with unpolished surfaces and half-coated with YGG phosphor. The same coating scheme was applied to a 4 by 4 LSO array. Pulse shape discrimination (PSD) methods were studied to extract DOI information from the pulse shape changes. The DOI full-width-half-maximum (FWHM) resolution was found to be ∼8 mm for this 2 cm thick array. PMID:19258685

Neutron spectroscopy for pulsed beams with frame overlap using a double time-of-flight technique

DOE Office of Scientific and Technical Information (OSTI.GOV)

Harrig, K. P.; Goldblum, B. L.; Brown, J. A.

A new double time-of- ight (dTOF) neutron spectroscopy technique has been developed for pulsed broad spectrum sources with a duty cycle that results in frame overlap, where fast neutrons from a given pulse overtake slower neutrons from previous pulses. Using a tunable beam at the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory, neutrons were produced via thick-target breakup of 16 MeV deuterons on a beryllium target in the cyclotron vault. The breakup spectral shape was deduced from a dTOF measurement using an array of EJ-309 organic liquid scintillators. Simulation of the neutron detection efficiency of the scintillator array was performedmore » using both GEANT4 and MCNP6. The efficiency- corrected spectral shape was normalized using a foil activation technique to obtain the energy-dependent flux of the neutron beam at zero degrees with respect to the incoming deuteron beam. The dTOF neutron spectrum was compared to spectra obtained using HEPROW and GRAVEL pulse height spectrum unfolding techniques. While the unfolding and dTOF results exhibit some discrepancies in shape, the integrated flux values agree within two standard deviations. As a result, this method obviates neutron time-of-flight spectroscopy challenges posed by pulsed beams« less

Pulse shape discrimination of Cs2LiYCl6:Ce3+ detectors at high count rate based on triangular and trapezoidal filters

NASA Astrophysics Data System (ADS)

Wen, Xianfei; Enqvist, Andreas

2017-09-01

Cs2LiYCl6:Ce3+ (CLYC) detectors have demonstrated the capability to simultaneously detect γ-rays and thermal and fast neutrons with medium energy resolution, reasonable detection efficiency, and substantially high pulse shape discrimination performance. A disadvantage of CLYC detectors is the long scintillation decay times, which causes pulse pile-up at moderate input count rate. Pulse processing algorithms were developed based on triangular and trapezoidal filters to discriminate between neutrons and γ-rays at high count rate. The algorithms were first tested using low-rate data. They exhibit a pulse-shape discrimination performance comparable to that of the charge comparison method, at low rate. Then, they were evaluated at high count rate. Neutrons and γ-rays were adequately identified with high throughput at rates of up to 375 kcps. The algorithm developed using the triangular filter exhibits discrimination capability marginally higher than that of the trapezoidal filter based algorithm irrespective of low or high rate. The algorithms exhibit low computational complexity and are executable on an FPGA in real-time. They are also suitable for application to other radiation detectors whose pulses are piled-up at high rate owing to long scintillation decay times.

Neutron spectroscopy for pulsed beams with frame overlap using a double time-of-flight technique

DOE PAGES

Harrig, K. P.; Goldblum, B. L.; Brown, J. A.; ...

2017-10-16

A new double time-of- ight (dTOF) neutron spectroscopy technique has been developed for pulsed broad spectrum sources with a duty cycle that results in frame overlap, where fast neutrons from a given pulse overtake slower neutrons from previous pulses. Using a tunable beam at the 88-Inch Cyclotron at Lawrence Berkeley National Laboratory, neutrons were produced via thick-target breakup of 16 MeV deuterons on a beryllium target in the cyclotron vault. The breakup spectral shape was deduced from a dTOF measurement using an array of EJ-309 organic liquid scintillators. Simulation of the neutron detection efficiency of the scintillator array was performedmore » using both GEANT4 and MCNP6. The efficiency- corrected spectral shape was normalized using a foil activation technique to obtain the energy-dependent flux of the neutron beam at zero degrees with respect to the incoming deuteron beam. The dTOF neutron spectrum was compared to spectra obtained using HEPROW and GRAVEL pulse height spectrum unfolding techniques. While the unfolding and dTOF results exhibit some discrepancies in shape, the integrated flux values agree within two standard deviations. As a result, this method obviates neutron time-of-flight spectroscopy challenges posed by pulsed beams« less

Pulse-shape discrimination with Cs2HfCl6 crystal scintillator

NASA Astrophysics Data System (ADS)

Cardenas, C.; Burger, A.; Goodwin, B.; Groza, M.; Laubenstein, M.; Nagorny, S.; Rowe, E.

2017-10-01

The results of investigation into cesium hafnium chloride (Cs2HfCl6) scintillating crystals as a promising detector to search for rare nuclear processes occurring in Hf isotopes is reported. The light output, quenching factor, and pulse-shape characteristics have been investigated at room temperature. The scintillation response of the crystal induced by α-particles and γ-quanta were studied to determine possibility of particle discrimination. Using the optimal filter method we obtained clear separation between signals with a factor of merit (FOM) = 9.3. This indicates that we are able to fully separate signals originating from α-particles and γ-quanta. Similar fruitful discrimination power was obtained by applying the mean time method (FOM = 7) and charge integration method (FOM = 7.5). The quenching factor for collimated 4 MeV α-particles is found to be 0.36, showing that α-particles generate more than a third of the light compared to γ-quanta at the same energy.

Shape of intrinsic alpha pulse height spectra in lanthanide halide scintillators

NASA Astrophysics Data System (ADS)

Wolszczak, W.; Dorenbos, P.

2017-06-01

Internal contamination with actinium-227 and its daughters is a serious drawback in low-background applications of lanthanide-based scintillators. In this work we showed the important role of nuclear γ de-excitations on the shape of the internal alpha spectrum measured in scintillators. We calculated with Bateman equations the activities of contamination isotopes and the time evolution of actinium-227 and its progenies. Next, we measured the intrinsic background spectra of LaBr3(Ce), LaBr3(Ce,Sr) and CeBr3 with a digital spectroscopy technique, and we analyzed them with a pulse shape discrimination method (PSD) and a time-amplitude analysis. Finally, we simulated the α background spectrum with Geant4 tool-kit, consequently taking into account complex α-γ-electron events, the α / β ratio dependence on the α energy, and the electron/γ nonproportionality. We found that α-γ mixed events have higher light yield than expected for alpha particles alone, which leads to overestimation of the α / β ratio when it is measured with internal 227Th and 223Ra isotopes. The time-amplitude analysis showed that the α peaks of 219Rn and 215Po in LaBr3(Ce) and LaBr3(Ce,Sr) are not symmetric. We compared the simulation results with the measured data and provided further evidence of the important role of mixed α-γ-electron events for understanding the shape of the internal α spectrum in scintillators.

Pulse shape discrimination of plastic scintillator EJ 299-33 with radioactive sources

NASA Astrophysics Data System (ADS)

Pagano, E. V.; Chatterjee, M. B.; De Filippo, E.; Russotto, P.; Auditore, L.; Cardella, G.; Geraci, E.; Gnoffo, B.; Guazzoni, C.; Lanzalone, G.; De Luca, S.; Maiolino, C.; Martorana, N. S.; Pagano, A.; Papa, M.; Parsani, T.; Pirrone, S.; Politi, G.; Porto, F.; Quattrocchi, L.; Rizzo, F.; Trifirò, A.; Trimarchi, M.

2018-05-01

The present study has been carried out in order to investigate about the possibility of using EJ 299-33 scintillator in a multi-detector array to detect neutrons along with light charged particles. In a reaction induced by stable and exotic heavy-ions beams, where copious production of neutrons and other light charged particles occurs, discrimination with low identification threshold of these particles are of great importance. In view of this, EJ 299-33 scintillator having dimension of 3 cm × 3 cm × 3 cm backed by a photomultiplier tube was tested and used under vacuum to detect neutrons, gamma-rays and alpha particles emitted by radioactive sources. Anode pulses from the photomultiplier tube were digitized through GET electronics, recorded and stored in a data acquisition system for the purpose of an off-line analysis. The measurements, under vacuum and low background conditions, show good pulse shape discrimination properties characterized by low identification threshold for neutrons, gamma-rays and alpha particles. The Figures of Merit for neutron-gamma and alpha particles-gamma discriminations have been evaluated together with the energy resolution for gamma-ray and alpha particles.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Joyce, M. J.; Aspinall, M. D.; Cave, F. D.

Pulse-shape discrimination (PSD) in fast, organic scintillation detectors is a long-established technique used to separate neutrons and {gamma} rays in mixed radiation fields. In the analogue domain the method can achieve separation in real time, but all knowledge of the pulses themselves is lost thereby preventing the possibility of any post- or repeated analysis. Also, it is typically reliant on electronic systems that are largely obsolete and which require significant experience to set up. In the digital domain, PSD is often more flexible but significant post-processing has usually been necessary to obtain neutron/{gamma}-ray separation. Moreover, the scintillation media on whichmore » the technique relies usually have a low flash point and are thus deemed hazardous. This complicates the ease with which they are used in industrial applications. In this paper, results obtained with a new portable digital pulse-shape discrimination instrument are described. This instrument provides real-time, digital neutron/{gamma} separation whilst preserving the synchronization with the time-of-arrival for each event, and realizing throughputs of 3 x 10{sup 6} events per second. Furthermore, this system has been tested with a scintillation medium that is non-flammable and not hazardous. (authors)« less

Optimal design of waveform digitisers for both energy resolution and pulse shape discrimination

NASA Astrophysics Data System (ADS)

Cang, Jirong; Xue, Tao; Zeng, Ming; Zeng, Zhi; Ma, Hao; Cheng, Jianping; Liu, Yinong

2018-04-01

Fast digitisers and digital pulse processing have been widely used for spectral application and pulse shape discrimination (PSD) owing to their advantages in terms of compactness, higher trigger rates, offline analysis, etc. Meanwhile, the noise of readout electronics is usually trivial for organic, plastic, or liquid scintillator with PSD ability because of their poor intrinsic energy resolution. However, LaBr3(Ce) has been widely used for its excellent energy resolution and has been proven to have PSD ability for alpha/gamma particles. Therefore, designing a digital acquisition system for such scintillators as LaBr3(Ce) with both optimal energy resolution and promising PSD ability is worthwhile. Several experimental research studies about the choice of digitiser properties for liquid scintillators have already been conducted in terms of the sampling rate and vertical resolution. Quantitative analysis on the influence of waveform digitisers, that is, fast amplifier (optional), sampling rates, and vertical resolution, on both applications is still lacking. The present paper provides quantitative analysis of these factors and, hence, general rules about the optimal design of digitisers for both energy resolution and PSD application according to the noise analysis of time-variant gated charge integration.

Deuterated scintillators and their application to neutron spectroscopy

NASA Astrophysics Data System (ADS)

Febbraro, M.; Lawrence, C. C.; Zhu, H.; Pierson, B.; Torres-Isea, R. O.; Becchetti, F. D.; Kolata, J. J.; Riggins, J.

2015-06-01

Deuterated scintillators have been used as a tool for neutron spectroscopy without Neutron Time-of-Flight (n-ToF) for more than 30 years. This article will provide a brief historical overview of the technique and current uses of deuterated scintillators in the UM-DSA and DESCANT arrays. Pulse-shape discrimination and spectrum unfolding with the maximum-likelihood expectation maximization algorithm will be discussed. Experimental unfolding and cross section results from measurements of (d,n), (3He,n) and (α,n) reactions are shown.

Coincidence measurements in α/β/γ spectrometry with phoswich detectors using digital pulse shape discrimination analysis

NASA Astrophysics Data System (ADS)

de Celis, B.; de la Fuente, R.; Williart, A.; de Celis Alonso, B.

2007-09-01

A novel system has been developed for the detection of low radioactivity levels using coincidence techniques. The device combines a phoswich detector for α/β/γ ray recognition with a fast digital card for electronic pulse analysis. The detector is able to discriminate different types of radiation in a mixed α/β/γ field and can be used in a coincidence mode by identifying the composite signal produced by the simultaneous detection of β particles in a plastic scintillator and γ rays in an NaI(Tl) scintillator. Use of a coincidence technique with phoswich detectors was proposed recently to verify the Nuclear Test Ban Treaty, which made it necessary to monitor the low levels of xenon radioisotopes produced by underground nuclear explosions. Previous studies have shown that combining CaF 2(Eu) for β ray detection and NaI(Tl) for γ ray detection makes it difficult to identify the coincidence signals because of the similar fluorescence decay times of the two scintillators. With the device proposed here, it is possible to identify the coincidence events owing to the short fluorescence decay time of the plastic scintillator. The sensitivity of the detector may be improved by employing liquid scintillators, which allow low radioactivity levels from actinides to be measured when present in environmental samples. The device developed is simpler to use than conventional coincidence equipment because it uses a single detector and electronic circuit, and it offers fast and precise analysis of the coincidence signals by employing digital pulse shape analysis.

Plastic scintillator with effective pulse shape discrimination for neutron and gamma detection

DOEpatents

Zaitseva, Natalia P.; Carman, M Leslie; Cherepy, Nerine; Glenn, Andrew M.; Hamel, Sebastien; Payne, Stephen A.; Rupert, Benjamin L.

2016-04-12

In one embodiment, a scintillator material includes a polymer matrix; and a primary dye in the polymer matrix, the primary dye being a fluorescent dye, the primary dye being present in an amount of 5 wt % or more; wherein the scintillator material exhibits an optical response signature for neutrons that is different than an optical response signature for gamma rays. In another embodiment, a scintillator material includes a polymer matrix; and a primary dye in the polymer matrix, the primary dye being a fluorescent dye, the primary dye being present in an amount greater than 10 wt %.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Hull, G; Zaitseva, N; Cherepy, N

Efficient, readily-available, low-cost, high-energy neutron detectors can play a central role in detecting illicit nuclear weapons since neutrons are a strong indication for the presence of fissile material such as Plutonium and Highly-Enriched Uranium. The main challenge in detecting fast neutrons consists in the discrimination of the signal from the gamma radiation background. At present, the only well-investigated organic crystal scintillator for fast neutron detection, in a n/{gamma} mixed field, is stilbene, which while offering good pulse shape discrimination, is not widely used because of its limited availability and high cost. In this work we report the results of ourmore » studies made with a number of new organic crystals, which exhibit pulse shape discrimination for detection of fast neutrons. In particular 1,1,4,4-tetraphenyl-1,3-butadiene features a light yield higher than anthracene and a Figure of Merit (FOM) for the pulse shape discrimination better than stilbene. New crystals are good candidates for the low-cost solution growth method, thus representing promising organic scintillators for widespread deployment for high-energy neutron detection.« less

DarkSide search for dark matter

NASA Astrophysics Data System (ADS)

Alexander, T.; Alton, D.; Arisaka, K.; Back, H. O.; Beltrame, P.; Benziger, J.; Bonfini, G.; Brigatti, A.; Brodsky, J.; Bussino, S.; Cadonati, L.; Calaprice, F.; Candela, A.; Cao, H.; Cavalcante, P.; Chepurnov, A.; Chidzik, S.; Cocco, A. G.; Condon, C.; D'Angelo, D.; Davini, S.; De Vincenzi, M.; De Haas, E.; Derbin, A.; Di Pietro, G.; Dratchnev, I.; Durben, D.; Empl, A.; Etenko, A.; Fan, A.; Fiorillo, G.; Franco, D.; Fomenko, K.; Forster, G.; Gabriele, F.; Galbiati, C.; Gazzana, S.; Ghiano, C.; Goretti, A.; Grandi, L.; Gromov, M.; Guan, M.; Guo, C.; Guray, G.; Hungerford, E. V.; Ianni, Al; Ianni, An; Joliet, C.; Kayunov, A.; Keeter, K.; Kendziora, C.; Kidner, S.; Klemmer, R.; Kobychev, V.; Koh, G.; Komor, M.; Korablev, D.; Korga, G.; Li, P.; Loer, B.; Lombardi, P.; Love, C.; Ludhova, L.; Luitz, S.; Lukyanchenko, L.; Lund, A.; Lung, K.; Ma, Y.; Machulin, I.; Mari, S.; Maricic, J.; Martoff, C. J.; Meregaglia, A.; Meroni, E.; Meyers, P.; Mohayai, T.; Montanari, D.; Montuschi, M.; Monzani, M. E.; Mosteiro, P.; Mount, B.; Muratova, V.; Nelson, A.; Nemtzow, A.; Nurakhov, N.; Orsini, M.; Ortica, F.; Pallavicini, M.; Pantic, E.; Parmeggiano, S.; Parsells, R.; Pelliccia, N.; Perasso, L.; Perasso, S.; Perfetto, F.; Pinsky, L.; Pocar, A.; Pordes, S.; Randle, K.; Ranucci, G.; Razeto, A.; Romani, A.; Rossi, B.; Rossi, N.; Rountree, S. D.; Saggese, P.; Saldanha, R.; Salvo, C.; Sands, W.; Seigar, M.; Semenov, D.; Shields, E.; Skorokhvatov, M.; Smirnov, O.; Sotnikov, A.; Sukhotin, S.; Suvarov, Y.; Tartaglia, R.; Tatarowicz, J.; Testera, G.; Thompson, J.; Tonazzo, A.; Unzhakov, E.; Vogelaar, R. B.; Wang, H.; Westerdale, S.; Wojcik, M.; Wright, A.; Xu, J.; Yang, C.; Zavatarelli, S.; Zehfus, M.; Zhong, W.; Zuzel, G.

2013-11-01

The DarkSide staged program utilizes a two-phase time projection chamber (TPC) with liquid argon as the target material for the scattering of dark matter particles. Efficient background reduction is achieved using low radioactivity underground argon as well as several experimental handles such as pulse shape, ratio of ionization over scintillation signal, 3D event reconstruction, and active neutron and muon vetos. The DarkSide-10 prototype detector has proven high scintillation light yield, which is a particularly important parameter as it sets the energy threshold for the pulse shape discrimination technique. The DarkSide-50 detector system, currently in commissioning phase at the Gran Sasso Underground Laboratory, will reach a sensitivity to dark matter spin-independent scattering cross section of 10-45 cm2 within 3 years of operation.

Separation of gamma-ray and neutron events with CsI(Tl) pulse shape analysis

NASA Astrophysics Data System (ADS)

Ashida, Y.; Nagata, H.; Koshio, Y.; Nakaya, T.; Wendell, R.

2018-04-01

Fast neutrons are a large background to measurements of gamma-rays emitted from excited nuclei, such that detectors that can efficiently distinguish between the two are essential. In this paper we describe the separation of gamma-rays from neutrons with the pulse shape information of the CsI(Tl) scintillator, using a fast neutron beam and several gamma-ray sources. We find that a figure of merit optimized for this separation takes on large and stable values (nearly 4) between 5 and 10 MeV of electron equivalent deposited energy, the region of most interest to the study of nuclear de-excitation gamma-rays. Accordingly, this work demonstrates the ability of CsI(Tl) scintillators to reject neutron backgrounds to gamma-ray measurements at these energies.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Lippincott, W. H.; McKinsey, D. N.; Nikkel, J. A.

Using a single-phase liquid argon detector with a signal yield of 4.85 photoelectrons per keV of electronic-equivalent recoil energy (keVee), we measure the scintillation time dependence of both electronic and nuclear recoils in liquid argon down to 5 keVee. We develop two methods of pulse shape discrimination to distinguish between electronic and nuclear recoils. Using one of these methods, we measure a background- and statistics-limited level of electronic recoil contamination to be 7.6x10{sup -7} between 52 and 110 keV of nuclear recoil energy (keVr) for a nuclear recoil acceptance of 50% with no nuclear recoil-like events above 62 keVr. Finally,more » we develop a maximum likelihood method of pulse shape discrimination based on the measured scintillation time dependence.« less

Pulse-shape discrimination scintillators for homeland security applications

NASA Astrophysics Data System (ADS)

Ellis, Mark E.; Duroe, Kirk; Kendall, Paul A.

2016-09-01

An extensive programme of research has been conducted for scintillation liquids and plastics capable of neutron-gamma discrimination for deployment in future passive and active Homeland Security systems to provide protection against radiological and nuclear threats. The more established detection materials such as EJ-301 and EJ-309 are compared with novel materials such as EJ-299-33 and p-terphenyl. This research also explores the benefits that can be gained from improvements in the analogue-to-digital sampling rate and sample bit resolution. Results are presented on the Pulse Shape Discrimination performance of various detector and data acquisition combinations and how optimum configurations from these studies have been developed into field-ready detector arrays. Early results from application-specific experimental configurations of multi-element detector arrays are presented.

Bismuth- and lithium-loaded plastic scintillators for gamma and neutron detection

NASA Astrophysics Data System (ADS)

Cherepy, Nerine J.; Sanner, Robert D.; Beck, Patrick R.; Swanberg, Erik L.; Tillotson, Thomas M.; Payne, Stephen A.; Hurlbut, Charles R.

2015-04-01

Transparent plastic scintillators based on polyvinyltoluene (PVT) have been fabricated with high loading of bismuth carboxylates for gamma spectroscopy, and with lithium carboxylates for neutron detection. When activated with a combination of standard fluors, 2,5-diphenyloxazole (PPO) and tetraphenylbutadiene (TPB), gamma light yields with 15 wt% bismuth tripivalate of 5000 Ph/MeV are measured. A PVT plastic formulation including 30 wt% lithium pivalate and 30 wt% PPO offers both pulse shape discrimination, and a neutron capture peak at 400 keVee. In another configuration, a bismuth-loaded PVT plastic is coated with ZnS(6Li) paint, permitting simultaneous gamma and neutron detection via pulse shape discrimination with a figure-of-merit of 3.8, while offering gamma spectroscopy with energy resolution of R(662 keV)=15%.

A Study of the quality of CsI detectors and pulse-shape discrimination of scintillators for ?[U+0251]-particles, ?[U+0263]-particles, and neutrons

NASA Astrophysics Data System (ADS)

Salyer, Kaitlin; Rogachev, Grigory; Hooker, Joshua

2016-09-01

This project studied the capabilities of two different scintillators, Cesium Iodide (CsI) and p-Terphenyl. First, the resolution of a CsI detector was investigated by exposing only very small areas of its surface at a time to an alpha source. Second, the abilities of p-Terphenyl to detect alpha particles, gamma particles, and neutrons were analyzed through pulse shape discrimination. p-Terphenyl is of particular interest because it will be used in the Mitchell Institute Neutrino Experiment at Reactor (MINER) at Texas A&M University for measuring background data. The information learned from conducting these tests will be useful in understanding and expanding the limits of the experiments in which these detectors will ultimately be used.

Hunting the Dark Matter with DEAP/CLEAN

DOE Office of Scientific and Technical Information (OSTI.GOV)

Giuliani, F.

2010-02-10

The potential of the DEAP/CLEAN program for direct Dark Matter detection to test various dark matter models is illustrated. The scintillation pulse of a noble liquid like Argon or Neon has two well distinguished time constants allowing a very reliable correlation between pulse shape and type of event. This pulse shape discrimination already provides the power of rejecting a background10{sup 8}-10{sup 9} times larger than the signal. MiniCLEAN, a 500 kg LAr detector, is currently under construction, and a 3.6 ton detector, DEAP-3600, under development.

Basic performance evaluation of a Si-PM array-based LGSO phoswich DOI block detector for a high-resolution small animal PET system.

PubMed

Yamamoto, Seiichi

2013-07-01

The silicon photomultiplier (Si-PM) is a promising photodetector for PET. However, it remains unclear whether Si-PM can be used for a depth-of-interaction (DOI) detector based on the decay time differences of the scintillator where pulse shape analysis is used. For clarification, we tested the Hamamatsu 4 × 4 Si-PM array (S11065-025P) combined with scintillators that used different decay times to develop DOI block detectors using the pulse shape analysis. First, Ce-doped Gd(2)SiO(5) (GSO) scintillators of 0.5 mol% Ce were arranged in a 4 × 4 matrix and were optically coupled to the center of each pixel of the Si-PM array for measurement of the energy resolution as well as its gain variations according to the temperature. Then two types of Ce-doped Lu(1.9)Gd(0.1)Si0(5) (LGSO) scintillators, 0.025 mol% Ce (decay time: ~31 ns) and 0.75 mol% Ce (decay time: ~46 ns), were optically coupled in the DOI direction, arranged in a 11 × 7 matrix, and optically coupled to a Si-PM array for testing of the possibility of a high-resolution DOI detector. The energy resolution of the Si-PM array-based GSO block detector was 18 ± 4.4 % FWHM for a Cs-137 gamma source (662 keV). Less than 1 mm crystals were clearly resolved in the position map of the LGSO DOI block detector. The peak-to-valley ratio (P/V) derived from the pulse shape spectra of the LGSO DOI block detector was 2.2. These results confirmed that Si-PM array-based DOI block detectors are promising for high-resolution small animal PET systems.

Scintillation detector efficiencies for neutrons in the energy region above 20 MeV

DOE Office of Scientific and Technical Information (OSTI.GOV)

Dickens, J.K.

1991-01-01

The computer program SCINFUL (for SCINtillator FUL1 response) is a program designed to provide a calculated complete pulse-height response anticipated for neutrons being detected by either an NE-213 (liquid) scintillator or an NE-110 (solid) scintillator in the shape of a right circular cylinder. The point neutron source may be placed at any location with respect to the detector, even inside of it. The neutron source may be monoenergetic, or Maxwellian distributed, or distributed between chosen lower and upper bounds. The calculational method uses Monte Carlo techniques, and it is relativistically correct. Extensive comparisons with a variety of experimental data havemore » been made. There is generally overall good agreement (less than 10% differences) of results for SCINFUL calculations with measured integral detector efficiencies for the design incident neutron energy range of 0.1 to 80 MeV. Calculations of differential detector responses, i.e. yield versus response pulse height, are generally within about 5% on the average for incident neutron energies between 16 and 50 MeV and for the upper 70% of the response pulse height. For incident neutron energies between 50 and 80 MeV, the calculated shape of the response agrees with measurements, but the calculations tend to underpredict the absolute values of the measured responses. Extension of the program to compute responses for incident neutron energies greater than 80 MeV will require new experimental data on neutron interactions with carbon. 32 refs., 6 figs., 2 tabs.« less

Scintillation detector efficiencies for neutrons in the energy region above 20 MeV

NASA Astrophysics Data System (ADS)

Dickens, J. K.

The computer program SCINFUL (for SCINtillator FUL1 response) is a program designed to provide a calculated complete pulse-height response anticipated for neutrons being detected by either an NE-213 (liquid) scintillator or an NE-110 (solid) scintillator in the shape of a right circular cylinder. The point neutron source may be placed at any location with respect to the detector, even inside of it. The neutron source may be monoenergetic, or Maxwellian distributed, or distributed between chosen lower and upper bounds. The calculational method uses Monte Carlo techniques, and it is relativistically correct. Extensive comparisons with a variety of experimental data were made. There is generally overall good agreement (less than 10 pct. differences) of results for SCINFUL calculations with measured integral detector efficiencies for the design incident neutron energy range of 0.1 to 80 MeV. Calculations of differential detector responses, i.e., yield versus response pulse height, are generally within about 5 pct. on the average for incident neutron energies between 16 and 50 MeV and for the upper 70 pct. of the response pulse height. For incident neutron energies between 50 and 80 MeV, the calculated shape of the response agrees with measurements, but the calculations tend to underpredict the absolute values of the measured responses. Extension of the program to compute responses for incident neutron energies greater than 80 MeV will require new experimental data on neutron interactions with carbon.

Organic scintillators with pulse shape discrimination for detection of radiation (Conference Presentation)

NASA Astrophysics Data System (ADS)

Mabe, Andrew; Carman, M. Leslie; Glenn, Andrew M.; Zaitseva, Natalia P.; Payne, Stephen A.

2016-09-01

The detection of neutrons in the presence of gamma-ray fields has important applications in the fields of nuclear physics, homeland security, and medical imaging. Organic scintillators provide several attractive qualities as neutron detection materials including low cost, fast response times, ease of scaling, and the ability to implement pulse shape discrimination (PSD) to discriminate between neutrons and gamma-rays. This talk will focus on amorphous organic scintillators both in plastic form and small-molecule organic glass form. The first section of this talk will describe recent advances and improvements in the performance of PSD-capable plastic scintillators. The primary advances described in regard to modification of the polymer matrix, evaluation of new scintillating dyes, improved fabrication conditions, and implementation of additives which impart superior performance and mechanical properties to PSD-capable plastics as compared to commercially-available plastics and performance comparable to PSD-capable liquids. The second section of this talk will focus on a class of small-molecule organic scintillators based on modified indoles and oligophenylenes which form amorphous glasses as PSD-capable neutron scintillation materials. Though indoles and oligophenylenes have been known for many decades, their PSD properties have not been investigated and their scintillation properties only scantily investigated. Well-developed synthetic methodologies have permitted the synthesis of a library of structural analogs of these compounds as well as the investigation of their scintillation properties. The emission wavelengths of many indoles are in the sensitive region of common photomultiplier tubes, making them appropriate to be used as scintillators in either pure or doped form. This work was performed under the auspices of the U.S. Department of Energy by Lawrence Livermore National Laboratory under Contract DE-AC52-07NA27344. This work has been supported by the U.S. Department of Energy Office of Nonproliferation Research and Development (NA-22) and by the Defense Threat Reduction Agency (DTRA).

Basic performance of Mg co-doped new scintillator used for TOF-DOI-PET systems

NASA Astrophysics Data System (ADS)

Kobayashi, Takahiro; Yamamoto, Seiichi; Okumura, Satoshi; Yeom, Jung Yeol; Kamada, Kei; Yoshikawa, Akira

2017-01-01

Phoswich depth-of-interaction (DOI) detectors utilizing multiple scintillators with different decay time are a useful device for developing a high spatial resolution, high sensitivity PET scanner. However, in order to apply pulse shape discrimination (PSD), there are not many combinations of scintillators for which phoswich technique can be implemented. Ce doped Gd3Ga3Al2O12 (GFAG) is a recently developed scintillator with a fast decay time. This scintillator is similar to Ce doped Gd3Al2Ga3O12 (GAGG), which is a promising scintillator for PET detector with high light yield. By stacking these scintillators, it may be possible to realize a high spatial resolution and high timing resolution phoswich DOI detector. Such phoswich DOI detector may be applied to time-of-flight (TOF) systems with high timing performance. Therefore, in this study, we tested the basic performance of the new scintillator -GFAG for use in a TOF phoswich detector. The measured decay time of a GFAG element of 2.9 mmx2.9 mmx10 mm in dimension, which was optically coupled to a photomultiplier tube (PMT), was faster (66 ns) than that of same sized GAGG (103 ns). The energy resolution of the GFAG element was 5.7% FWHM which was slightly worse than that of GAGG with 4.9% FWHM for 662 keV gamma photons without saturation correction. Then we assembled the GFAG and the GAGG crystals in the depth direction to form a 20 mm long phoswich element (GFAG/GAGG). By pulse shape analysis, the two types of scintillators were clearly resolved. Measured timing resolution of a pair of opposing GFAG/GAGG phoswich scintillator coupled to Silicon Photomultipliers (Si-PM) was good with coincidence resolving time of 466 ps FWHM. These results indicate that the GFAG combined with GAGG can be a candidate for TOF-DOI-PET systems.

Portal radiation monitor

DOEpatents

Kruse, Lyle W.

1985-01-01

A portal radiation monitor combines 0.1% FAR with high sensitivity to special nuclear material. The monitor utilizes pulse shape discrimination, dynamic compression of the photomultiplier output and scintillators sized to maintain efficiency over the entire portal area.

Portal radiation monitor

DOEpatents

Kruse, L.W.

1982-03-23

A portal radiation monitor combines .1% FAR with high sensitivity to special nuclear material. The monitor utilizes pulse shape discrimination, dynamic compression of the photomultiplier output and scintillators sized to maintain efficiency over the entire portal area.

Bismuth- and lithium-loaded plastic scintillators for gamma and neutron detection

DOE PAGES

Cherepy, Nerine J.; Sanner, Robert D.; Beck, Patrick R.; ...

2015-01-09

In this paper, transparent plastic scintillators based on polyvinyltoluene (PVT) have been fabricated with high loading of bismuth carboxylates for gamma spectroscopy, and with lithium carboxylates for neutron detection. When activated with a combination of standard fluors, 2,5-diphenyloxazole (PPO) and tetraphenylbutadiene (TPB), gamma light yields with 15 wt% bismuth tripivalate of 5000 Ph/MeV are measured. A PVT plastic formulation including 30 wt% lithium pivalate and 30 wt% PPO offers both pulse shape discrimination, and a neutron capture peak at ~400 keVee. Finally, in another configuration, a bismuth-loaded PVT plastic is coated with ZnS( 6Li) paint, permitting simultaneous gamma and neutronmore » detection via pulse shape discrimination with a figure-of-merit of 3.8, while offering gamma spectroscopy with energy resolution of R(662 keV)=15%.« less

Particle discrimination of NaI(Tl) scintillator under high-energy neutron field to measure the photon energy spectrum

NASA Astrophysics Data System (ADS)

Kamada, So; Takada, Masashi; Suzuki, Toshikazu

2014-09-01

Photons are measured separately from neutrons in high-energy neutron fields using a NaI(Tl) scintillator, 7.62 cm in diameter and 7.62 cm in length, combined with a pulse-shape discrimination method. The particle discrimination capability for this scintillator is confirmed using a time-of-flight method. Neutron fields were produced by irradiating Li targets with 40 and 80 MeV proton beams at the cyclotron facility in the National Institute of Radiological Sciences. Figures of merit corresponding to particle discrimination for the scintillator at the two neutron fields are improved with higher neutron energies. Photon energy spectra for energies over 6.5 MeV can be measured using the NaI(Tl) scintillator.

Neutron-gamma discrimination via PSD plastic scintillator and SiPMs

NASA Astrophysics Data System (ADS)

Taggart, M. P.; Payne, C.; Sellin, P. J.

2016-10-01

The reduction in availability and inevitable increase in cost of traditional neutron detectors based on the 3He neutron capture reaction has resulted in a concerted effort to seek out new techniques and detection media to meet the needs of national nuclear security. Traditionally, the alternative has been provided through pulse shape discrimination (PSD) using liquid scintillators. However, these are not without their own inherent issues, primarily concerning user safety and ongoing maintenance. A potential system devised to separate neutron and gamma ray pulses utilising the PSD technique takes advantage of recent improvements in silicon photomultiplier (SiPM) technology and the development of plastic scintillators exhibiting the PSD phenomena. In this paper we present the current iteration of this ongoing work having achieved a Figure of Merit (FoM) of 1.39 at 1.5 MeVee.

DESCANT and β-delayed neutron measurements at TRIUMF

NASA Astrophysics Data System (ADS)

Bildstein, V.; Garrett, P. E.; Ashley, S. F.; Ball, G. C.; Bianco, L.; Bandyopadhyay, D.; Bangay, J.; Crider, B. P.; Demand, G.; Deng, G.; Dillmann, I.; Finlay, A.; Garnsworthy, A. B.; Hackman, G.; Hadinia, B.; Krücken, R.; Leach, K. G.; Martin, J.-P.; McEllistrem, M. T.; Pearson, C. J.; Peters, E. E.; Prados-Estévez, F. M.; Radich, A.; Sarazin, F.; Sumithrarachchi, C.; Svensson, C. E.; Vanhoy, J. R.; Wong, J.; Yates, S. W.

2015-05-01

The DESCANT array (Deuterated Scintillator Array for Neutron Tagging) consists of up to 70 detectors, each filled with approximately 2 liters of deuterated benzene. This scintillator material o_ers pulse-shape discrimination (PSD) capabilities to distinguish between neutrons and γ-rays interacting with the scintillator material. In addition, the anisotropic nature of n - d scattering allows for the determination of the neutron energy spectrum directly from the pulse height spectrum, complementing the traditional time-of-flight (ToF) information. DESCANT can be coupled either to the TIGRESS (TRIUMF-ISAC Gamma-Ray Escape Suppressed Spectrometer) γ-ray spectrometer [1] located in the ISAC-II [2] hall of TRIUMF for in-beam experiments, or to the GRIFFIN (Gamma-Ray Infrastructure For Fundamental Investigations of Nuclei) γ-ray spectrometer [3] located in the ISAC-I hall of TRIUMF for decay spectroscopy experiments.

Gain Shift Corrections at Chi-Nu

DOE Office of Scientific and Technical Information (OSTI.GOV)

Brown, Tristan Brooks; Devlin, Matthew James

Ambient conditions have the potential to cause changes in liquid scintillator detector gain that vary with time and temperature. These gain shifts can lead to poor resolution in both energy as well as pulse shape discrimination. In order to correct for these shifts in the Chi-Nu high energy array, a laser system has been developed for calibration of the pulse height signals.

Simple algorithms for digital pulse-shape discrimination with liquid scintillation detectors

NASA Astrophysics Data System (ADS)

Alharbi, T.

2015-01-01

The development of compact, battery-powered digital liquid scintillation neutron detection systems for field applications requires digital pulse processing (DPP) algorithms with minimum computational overhead. To meet this demand, two DPP algorithms for the discrimination of neutron and γ-rays with liquid scintillation detectors were developed and examined by using a NE213 liquid scintillation detector in a mixed radiation field. The first algorithm is based on the relation between the amplitude of a current pulse at the output of a photomultiplier tube and the amount of charge contained in the pulse. A figure-of-merit (FOM) value of 0.98 with 450 keVee (electron equivalent energy) energy threshold was achieved with this method when pulses were sampled at 250 MSample/s and with 8-bit resolution. Compared to the similar method of charge-comparison this method requires only a single integration window, thereby reducing the amount of computations by approximately 40%. The second approach is a digital version of the trailing-edge constant-fraction discrimination method. A FOM value of 0.84 with an energy threshold of 450 keVee was achieved with this method. In comparison with the similar method of rise-time discrimination this method requires a single time pick-off, thereby reducing the amount of computations by approximately 50%. The algorithms described in this work are useful for developing portable detection systems for applications such as homeland security, radiation dosimetry and environmental monitoring.

Melt-cast organic glasses as high-efficiency fast neutron scintillators

NASA Astrophysics Data System (ADS)

Carlson, Joseph S.; Feng, Patrick L.

2016-10-01

In this work we report a new class of organic-based scintillators that combines several of the desirable attributes of existing crystalline, liquid, and plastic organic scintillators. The prepared materials may be isolated in single crystalline form or melt-cast to produce highly transparent glasses that have been shown to provide high light yields of up to 16,000 photons/MeVee, as evaluated against EJ-200 plastic scintillators and solution-grown trans-stilbene crystals. The prepared organic glasses exhibit neutron/gamma pulse-shape discrimination (PSD) and are compatible with wavelength shifters to reduce optical self-absorption effects that are intrinsic to pure materials such as crystalline organics. The combination of high scintillation efficiency, PSD capabilities, and facile scale-up via melt-casting distinguishes this new class of amorphous materials from existing alternatives.

Some Experimental and Monte Carlo Investigations of the Plastic Scintillators for the Current Mode Measurements at Pulsed Neutron Sources

NASA Astrophysics Data System (ADS)

Rogov, A.; Pepyolyshev, Yu.; Carta, M.; d'Angelo, A.

Scintillation detector (SD) is widely used in neutron and gamma-spectrometry in a count mode. The organic scintillators for the count mode of the detector operation are investigated rather well. Usually, they are applied for measurement of amplitude and time distributions of pulses caused by single interaction events of neutrons or gamma's with scintillator material. But in a large area of scientific research scintillation detectors can alternatively be used on a current mode by recording the average current from the detector. For example,the measurements of the neutron pulse shape at the pulsed reactors or another pulsed neutron sources. So as to get a rather large volume of experimental data at pulsed neutron sources, it is necessary to use the current mode detector for registration of fast neutrons. Many parameters of the SD are changed with a transition from an accounting mode to current one. For example, the detector efficiency is different in counting and current modes. Many effects connected with time accuracy become substantial. Besides, for the registration of solely fast neutrons, as must be in many measurements, in the mixed radiation field of the pulsed neutron sources, SD efficiency has to be determined with a gamma-radiation shield present. Here is no calculations or experimental data on SD current mode operation up to now. The response functions of the detectors can be either measured in high-precision reference fields or calculated by a computer simulation. We have used the MCNP code [1] and carried out some experiments for investigation of the plastic performances in a current mode. There are numerous programs performing simulating similar to the MCNP code. For example, for neutrons there are [2-4], for photons - [5-8]. However, all known codes to use (SCINFUL, NRESP4, SANDYL, EGS49) have more stringent restrictions on the source, geometry and detector characteristics. In MCNP code a lot of these restrictions are absent and you need only to write special additions for proton and electron recoil and transfer energy to light output. These code modifications allow taking into account all processes in organic scintillator influence the light yield.

A compact pulse shape discriminator module for large neutron detector arrays

NASA Astrophysics Data System (ADS)

Venkataramanan, S.; Gupta, Arti; Golda, K. S.; Singh, Hardev; Kumar, Rakesh; Singh, R. P.; Bhowmik, R. K.

2008-11-01

A cost-effective high-performance pulse shape discriminator module has been developed to process signals from organic liquid scintillator-based neutron detectors. This module is especially designed for the large neutron detector array used for studies of nuclear reaction dynamics at the Inter University Accelerator Center (IUAC). It incorporates all the necessary pulse processing circuits required for neutron spectroscopy in a novel fashion by adopting the zero crossover technique for neutron-gamma (n- γ) pulse shape discrimination. The detailed layout of the circuit and different features of the module are described in the present paper. The quality of n- γ separation obtained with this electronics is much better than that of commercial modules especially in the low-energy region. The results obtained with our module are compared with similar setups available in other laboratories.

The spectrum of neutrons at 60 hg m(-2)

NASA Technical Reports Server (NTRS)

Barton, J. C.

1985-01-01

The rate of neutron interactions was measured for the energy range 7.5 to 60 MeV, using a 3.85 kg cell of liquid scintillator. The neutrons are selected by pulse shape discrimination, with anticoincidence counters used to reduce interference from muons transversing the scintillator. The observed flux is interpreted in terms of neutrons produced from environmental uranium and thorium, those resulting from the capture of negative muons in nuclei and those from fast muon interactions.

A novel intra-operative positron imager for rapid localization of tumor margins

NASA Astrophysics Data System (ADS)

Sabet, Hamid; Stack, Brendan C.; Nagarkar, Vivek V.

2014-03-01

We have developed an intra-operative and compact imaging tool for surgeons to detect PET- positive lesions. Currently, most such probes on the market are non-imaging, and provide no ancillary information of surveyed areas, such as clear delineations of malignant tissues. Our probe consists of a novel hybrid scintillator coupled to a compact silicon photomultiplier (SiPM) array with associated front-end electronics encapsulated in an ergonomic housing. Pulse shape discrimination electronics has been implemented and integrated into the downstream data acquisition system. The hybrid scintillator consists of a 0.4 mm thick layer of CsI:Tl scintillator coupled to a 1 mm thick LYSO crystal. To achieve high spatial resolution, CsI:Tl is pixelated to 0.5×0.5 mm2 pixels using laser ablation technique. While CsI:Tl act as beta-sensitive scintillator, LYSO senses the gamma radiation and can be used to navigate the probe to the locations of interest. The gamma response is also subtracted from the beta image for improved SNR and contrast. To achieve accurate centroid position estimation and uniform beta sensitivity over the entire imaging area, the LYSO thickness is optimized such that it acts as scintillation light diffuser by spreading CsI:Tl light over multiple SiPM pixels. The results show that the response of the two scintillators exposed to radiation could be easily distinguished based on their pulse shapes. The probe's spatial resolution is <1.5 mm FWHM in its 10×10 mm2 effective imaging area. The probe can rapidly detect and localize nCi levels of F-18 beta radiation even in presence of strong gamma background.

Digital pulse shape discrimination methods for n-γ separation in an EJ-301 liquid scintillation detector

NASA Astrophysics Data System (ADS)

Wan, Bo; Zhang, Xue-Ying; Chen, Liang; Ge, Hong-Lin; Ma, Fei; Zhang, Hong-Bin; Ju, Yong-Qin; Zhang, Yan-Bin; Li, Yan-Yan; Xu, Xiao-Wei

2015-11-01

A digital pulse shape discrimination system based on a programmable module NI-5772 has been established and tested with an EJ-301 liquid scintillation detector. The module was operated by running programs developed in LabVIEW, with a sampling frequency up to 1.6 GS/s. Standard gamma sources 22Na, 137Cs and 60Co were used to calibrate the EJ-301 liquid scintillation detector, and the gamma response function was obtained. Digital algorithms for the charge comparison method and zero-crossing method have been developed. The experimental results show that both digital signal processing (DSP) algorithms can discriminate neutrons from γ-rays. Moreover, the zero-crossing method shows better n-γ discrimination at 80 keVee and lower, whereas the charge comparison method gives better results at higher thresholds. In addition, the figure-of-merit (FOM) for detectors of two different dimensions were extracted at 9 energy thresholds, and it was found that the smaller detector presented better n-γ separation for fission neutrons. Supported by National Natural Science Foundation of China (91226107, 11305229) and the Strategic Priority Research Program of the Chinese Academy of Sciences (XDA03030300)

Pulse-shape discrimination and energy resolution of a liquid-argon scintillator with xenon doping

NASA Astrophysics Data System (ADS)

Wahl, C. G.; Bernard, E. P.; Lippincott, W. H.; Nikkel, J. A.; Shin, Y.; McKinsey, D. N.

2014-06-01

Liquid-argon scintillation detectors are used in fundamental physics experiments and are being considered for security applications. Previous studies have suggested that the addition of small amounts of xenon dopant improves performance in light or signal yield, energy resolution, and particle discrimination. In this study, we investigate the detector response for xenon dopant concentrations from 9 ± 5 ppm to 1100 ± 500 ppm xenon (by weight) in 6 steps. The 3.14-liter detector uses tetraphenyl butadiene (TPB) wavelength shifter with dual photomultiplier tubes and is operated in single-phase mode. Gamma-ray-interaction signal yield of 4.0 ± 0.1 photoelectrons/keV improved to 5.0 ± 0.1 photoelectrons/keV with dopant. Energy resolution at 662 keV improved from (4.4 ± 0.2)% (σ) to (3.5 ± 0.2)% (σ) with dopant. Pulse-shape discrimination performance degraded greatly at the first addition of dopant, slightly improved with additional additions, then rapidly improved near the end of our dopant range, with performance becoming slightly better than pure argon at the highest tested dopant concentration. Some evidence of reduced neutron scintillation efficiency with increasing dopant concentration was observed. Finally, the waveform shape outside the TPB region is discussed, suggesting that the contribution to the waveform from xenon-produced light is primarily in the last portion of the slow component.

Characterization of the scintillation anisotropy in crystalline stilbene scintillator detectors

DOE PAGES

Schuster, P.; Brubaker, E.

2016-11-23

This study reports a series of measurements that characterize the directional dependence of the scintillation response of crystalline melt-grown and solution-grown trans-stilbene to incident DT and DD neutrons. These measurements give the amplitude and pulse shape dependence on the proton recoil direction over one hemisphere of the crystal, confirming and extending previous results in the literature for melt-grown stilbene and providing the first measurements for solution-grown stilbene. In similar measurements of liquid and plastic detectors, no directional dependence was observed, confirming the hypothesis that the anisotropy in stilbene and other organic crystal scintillators is a result of internal effects duemore » to the molecular or crystal structure and not an external effect on the measurement system.« less

10B enriched plastic scintillators for application in thermal neutron detection

NASA Astrophysics Data System (ADS)

Mahl, Adam; Yemam, Henok A.; Fernando, Roshan; Koubek, Joshua T.; Sellinger, Alan; Greife, Uwe

2018-02-01

We report here on the synthesis and characterization of a novel 10B enriched aromatic molecule that can be incorporated into common poly(vinyltoluene) (PVT) based plastic scintillators to achieve enhanced thermal neutron detection. Starting from relatively inexpensive 10B enriched boric acid, we have prepared 4,4,5,5-tetramethyl-2-phenyl-1,3,2-dioxaborolane (MBB) in three high yield steps. MBB is soluble and compatible with PVT based formulations and results in stable plastic scintillators. Chemical synthesis, solubility limit in PVT, and the physical properties of the dopant were explored. The relevant response properties of the resulting scintillators when exposed to neutron and gamma radiation, including light yield and pulse shape discrimination properties were measured and analyzed.

Measurement of the scintillation time spectra and pulse-shape discrimination of low-energy β and nuclear recoils in liquid argon with DEAP-1

DOE PAGES

Amaudruz, P. -A.; Batygov, M.; Beltran, B.; ...

2016-09-17

The DEAP-1 low-background liquid argon detector has been used to measure scintillation pulse shapes of beta decays and nuclear recoil events and to demonstrate the feasibility of pulse-shape discrimination down to an electron-equivalent energy of 20 keV ee. The relative intensities of singlet/triplet states in liquid argon have been measured as a function of energy between 15 and 500 keVee for both beta and nuclear recoils. Using a triple-coincidence tag we find the fraction of beta events that are misidentified as nuclear recoils to be less than 6 x 10 -8 between 43-86 keV ee and that the discrimination parametermore » agrees with a simple analytic model. The discrimination measurement is currently limited by nuclear recoils induced by cosmic-ray generated neutrons, and is expected to improve by operating the detector underground at SNOLAB. The analytic model predicts a beta misidentification fraction of 10 -10 for an electron-equivalent energy threshold of 20 keV ee. This reduction allows for a sensitive search for spin-independent scattering of WIMPs from 1000 kg of liquid argon with a WIMP-nucleon cross-section sensitivity of 10 -46 cm 2.« less

Measurement of the scintillation time spectra and pulse-shape discrimination of low-energy β and nuclear recoils in liquid argon with DEAP-1

DOE Office of Scientific and Technical Information (OSTI.GOV)

Amaudruz, P. -A.; Batygov, M.; Beltran, B.

The DEAP-1 low-background liquid argon detector has been used to measure scintillation pulse shapes of beta decays and nuclear recoil events and to demonstrate the feasibility of pulse-shape discrimination down to an electron-equivalent energy of 20 keV ee. The relative intensities of singlet/triplet states in liquid argon have been measured as a function of energy between 15 and 500 keVee for both beta and nuclear recoils. Using a triple-coincidence tag we find the fraction of beta events that are misidentified as nuclear recoils to be less than 6 x 10 -8 between 43-86 keV ee and that the discrimination parametermore » agrees with a simple analytic model. The discrimination measurement is currently limited by nuclear recoils induced by cosmic-ray generated neutrons, and is expected to improve by operating the detector underground at SNOLAB. The analytic model predicts a beta misidentification fraction of 10 -10 for an electron-equivalent energy threshold of 20 keV ee. This reduction allows for a sensitive search for spin-independent scattering of WIMPs from 1000 kg of liquid argon with a WIMP-nucleon cross-section sensitivity of 10 -46 cm 2.« less

ZnO:Zn/6LiF scintillator-A low afterglow alternative to ZnS:Ag/6LiF for thermal neutron detection

NASA Astrophysics Data System (ADS)

Sykora, G. Jeff; Schooneveld, Erik M.; Rhodes, Nigel J.

2018-03-01

Current ZnS:Ag/6LiF based scintillation detectors are often count rate limited by the long lifetime afterglow in the scintillator. Despite this drawback, new instruments at neutron scattering facilities, like ISIS in the UK, would still like to use ZnS:Ag/6LiF detectors due to their low gamma sensitivity, high light output, simplicity of detector design and relatively inexpensive production. One particular advantage of ZnS:Ag/6LiF detectors is their ability to provide strong pulse shape discrimination between neutrons and gammas. Despite the advantages of these detectors, it is becoming clear that new and upgraded instruments will be limited by the count rate capability of ZnS:Ag/6LiF, so an alternative scintillator technology with equivalent simplicity is being sought. ZnO:Zn/6LiF is investigated here as a low afterglow alternative to ZnS:Ag/6LiF. Basic scintillation properties of ZnO:Zn are studied and are discussed. Pulse shape discrimination between neutrons and gammas is explored and taken advantage of through simple single photon counting methods. A further step toward a realistic detector for neutron scattering is also taken by fiber coupling the ZnO:Zn/6LiF to a PMT. In an initial study of this fiber coupled configuration, 60Co gamma sensitivity of ∼ 7 × 10-6 is shown and improvements in count rate capability of at least a factor of 6 over ZnS:Ag/6LiF based neutron detectors are demonstrated.

Melt-cast organic glasses as high-efficiency fast neutron scintillators

DOE PAGES

Carlson, Joseph S.; Feng, Patrick L.

2016-06-24

In this work we report a new class of organic-based scintillators that combines several of the desirable attributes of existing crystalline, liquid, and plastic organic scintillators. The prepared materials may be isolated in single crystalline form or melt-cast to produce highly transparent glasses that have been shown to provide high light yields of up to 16,000 photons/MeVee, as evaluated against EJ-200 plastic scintillators and solution-grown trans-stilbene crystals. The prepared organic glasses exhibit neutron/gamma pulse-shape discrimination (PSD) and are compatible with wavelength shifters to reduce optical self-absorption effects that are intrinsic to pure materials such as crystalline organics. In conclusion, themore » combination of high scintillation efficiency, PSD capabilities, and facile scale-up via melt-casting distinguishes this new class of amorphous materials from existing alternatives.« less

A Study of Nuclear Recoils in Liquid Argon Time Projection Chamber for the Direct Detection of WIMP Dark Matter

DOE Office of Scientific and Technical Information (OSTI.GOV)

Cao, Huajie

2014-11-01

Robust results of WIMP direct detection experiments depend on rm understandings of nuclear recoils in the detector media. This thesis documents the most comprehensive study to date on nuclear recoils in liquid argon - a strong candidate for the next generation multi-ton scale WIMP detectors. This study investigates both the energy partition from nuclear recoil energy to secondary modes (scintillation and ionization) and the pulse shape characteristics of scintillation from nuclear recoils.

Deuterated-xylene (xylene-d10; EJ301D): A new, improved deuterated liquid scintillator for neutron energy measurements without time-of-flight

NASA Astrophysics Data System (ADS)

Becchetti, F. D.; Raymond, R. S.; Torres-Isea, R. O.; Di Fulvio, A.; Clarke, S. D.; Pozzi, S. A.; Febbraro, M.

2016-06-01

In conjunction with Eljen Technology, Inc. (Sweetwater,TX) we have designed, constructed, and evaluated a 3 in. ×3 in. deuterated-xylene organic liquid scintillator (C8D10; EJ301D) as a fast neutron detector. Similar to deuterated benzene (C6D6; NE230, BC537, and EJ315) this scintillator can provide good pulse-shape discrimination between neutrons and gamma rays, has good timing characteristics, and can provide a light spectrum with peaks corresponding to discrete neutron energy groups up to ca. 20 MeV. Unlike benzene-based detectors, deuterated xylene is less volatile, less toxic, is not known to be carcinogenic, has a higher flashpoint, and hence is much safer for many applications. In addition EJ301D can provide slightly more light output and better PSD than deuterated-benzene scintillators. We show that, as with deuterated-benzene scintillators, the light-response spectra can be unfolded to provide useable neutron energy spectra without need for time-of-flight (ToF). An array of these detectors arranged at many angles close to a reaction target can be much more effective (×10 to ×100 or more) than an array of long-path ToF detectors which must utilize a narrowly-bunched and pulse-selected beam. As we demonstrate using a small Van de Graaff accelerator, measurements can thus be performed when a bunched and pulse-selected beam (as needed for time-of-flight) is not available.

Simultaneous beta and gamma spectroscopy

DOEpatents

Farsoni, Abdollah T.; Hamby, David M.

2010-03-23

A phoswich radiation detector for simultaneous spectroscopy of beta rays and gamma rays includes three scintillators with different decay time characteristics. Two of the three scintillators are used for beta detection and the third scintillator is used for gamma detection. A pulse induced by an interaction of radiation with the detector is digitally analyzed to classify the type of event as beta, gamma, or unknown. A pulse is classified as a beta event if the pulse originated from just the first scintillator alone or from just the first and the second scintillator. A pulse from just the third scintillator is recorded as gamma event. Other pulses are rejected as unknown events.

Fast neutron tomography with real-time pulse-shape discrimination in organic scintillation detectors

NASA Astrophysics Data System (ADS)

Joyce, Malcolm J.; Agar, Stewart; Aspinall, Michael D.; Beaumont, Jonathan S.; Colley, Edmund; Colling, Miriam; Dykes, Joseph; Kardasopoulos, Phoevos; Mitton, Katie

2016-10-01

A fast neutron tomography system based on the use of real-time pulse-shape discrimination in 7 organic liquid scintillation detectors is described. The system has been tested with a californium-252 source of dose rate 163 μSv/h at 1 m and neutron emission rate of 1.5×107 per second into 4π and a maximum acquisition time of 2 h, to characterize two 100×100×100 mm3 concrete samples. The first of these was a solid sample and the second has a vertical, cylindrical void. The experimental data, supported by simulations with both Monte Carlo methods and MATLAB®, indicate that the presence of the internal cylindrical void, corners and inhomogeneities in the samples can be discerned. The potential for fast neutron assay of this type with the capability to probe hydrogenous features in large low-Z samples is discussed. Neutron tomography of bulk porous samples is achieved that combines effective penetration not possible with thermal neutrons in the absence of beam hardening.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Carlson, Joseph S.; Feng, Patrick L.

In this work we report a new class of organic-based scintillators that combines several of the desirable attributes of existing crystalline, liquid, and plastic organic scintillators. The prepared materials may be isolated in single crystalline form or melt-cast to produce highly transparent glasses that have been shown to provide high light yields of up to 16,000 photons/MeVee, as evaluated against EJ-200 plastic scintillators and solution-grown trans-stilbene crystals. The prepared organic glasses exhibit neutron/gamma pulse-shape discrimination (PSD) and are compatible with wavelength shifters to reduce optical self-absorption effects that are intrinsic to pure materials such as crystalline organics. In conclusion, themore » combination of high scintillation efficiency, PSD capabilities, and facile scale-up via melt-casting distinguishes this new class of amorphous materials from existing alternatives.« less

Gamma ray spectroscopy employing divalent europium-doped alkaline earth halides and digital readout for accurate histogramming

DOEpatents

Cherepy, Nerine Jane; Payne, Stephen Anthony; Drury, Owen B; Sturm, Benjamin W

2014-11-11

A scintillator radiation detector system according to one embodiment includes a scintillator; and a processing device for processing pulse traces corresponding to light pulses from the scintillator, wherein pulse digitization is used to improve energy resolution of the system. A scintillator radiation detector system according to another embodiment includes a processing device for fitting digitized scintillation waveforms to an algorithm based on identifying rise and decay times and performing a direct integration of fit parameters. A method according to yet another embodiment includes processing pulse traces corresponding to light pulses from a scintillator, wherein pulse digitization is used to improve energy resolution of the system. A method in a further embodiment includes fitting digitized scintillation waveforms to an algorithm based on identifying rise and decay times; and performing a direct integration of fit parameters. Additional systems and methods are also presented.

Neutron response characterization for an EJ299-33 plastic scintillation detector

DOE PAGES

Lawrence, Chris C.; Febbraro, Michael; Massey, Thomas N.; ...

2014-05-10

Organic scintillation detectors have shown promise as neutron detectors for characterizing special nuclear materials in various arms-control and homeland security applications. Recent advances have yielded a new plastic scintillator - EJ299-33 - with pulse-shape-discrimination (PSD) capability. Plastic scintillators would have a much expanded range of deployment relative to liquids and crystals. Here in this paper, we present a full characterization of pulse height response to fission-energy neutrons for an EJ299-33 detector with 7.62-by-7.62-cm cylindrical active volume, and compare with an EJ309 liquid scintillator in the same assembly. Scintillation light output relations, energy resolutions, and response matrices are presented for bothmore » detectors. A Continuous spectrum neutron source, obtained via the bombardment of 27Al with 7.44-MeV deuterons at the Edwards Accelerator Facility at Ohio University, was used for the measurement. A new procedure for evaluating and comparing PSD performance is presented which accounts for the effect of the light output relation on the ability to detect low energy neutrons. The EJ299-33 is shown to have considerable deficit in matrix condition, and in PSD figure of merit when compared to EJ309, especially when neutron energy is taken into account. Furthermore the EJ299 is likely to bring a modest PSD capability into a array of held applications that are not accessible to liquids or crystals.« less

Rejection of randomly coinciding events in ZnMoO scintillating bolometers

NASA Astrophysics Data System (ADS)

Chernyak, D. M.; Danevich, F. A.; Giuliani, A.; Mancuso, M.; Nones, C.; Olivieri, E.; Tenconi, M.; Tretyak, V. I.

2014-06-01

Random coincidence of events (particularly from two neutrino double beta decay) could be one of the main sources of background in the search for neutrinoless double beta decay with cryogenic bolometers due to their poor time resolution. Pulse-shape discrimination by using front edge analysis, mean-time and methods were applied to discriminate randomly coinciding events in ZnMoO cryogenic scintillating bolometers. These events can be effectively rejected at the level of 99 % by the analysis of the heat signals with rise-time of about 14 ms and signal-to-noise ratio of 900, and at the level of 92 % by the analysis of the light signals with rise-time of about 3 ms and signal-to-noise ratio of 30, under the requirement to detect 95 % of single events. These rejection efficiencies are compatible with extremely low background levels in the region of interest of neutrinoless double beta decay of Mo for enriched ZnMoO detectors, of the order of counts/(y keV kg). Pulse-shape parameters have been chosen on the basis of the performance of a real massive ZnMoO scintillating bolometer. Importance of the signal-to-noise ratio, correct finding of the signal start and choice of an appropriate sampling frequency are discussed.

Liquid xenon scintillation measurements and pulse shape discrimination in the LUX dark matter detector

NASA Astrophysics Data System (ADS)

Akerib, D. S.; Alsum, S.; Araújo, H. M.; Bai, X.; Bailey, A. J.; Balajthy, J.; Beltrame, P.; Bernard, E. P.; Bernstein, A.; Biesiadzinski, T. P.; Boulton, E. M.; Brás, P.; Byram, D.; Carmona-Benitez, M. C.; Chan, C.; Currie, A.; Cutter, J. E.; Davison, T. J. R.; Dobi, A.; Druszkiewicz, E.; Edwards, B. N.; Fallon, S. R.; Fan, A.; Fiorucci, S.; Gaitskell, R. J.; Genovesi, J.; Ghag, C.; Gilchriese, M. G. D.; Hall, C. R.; Haselschwardt, S. J.; Hertel, S. A.; Hogan, D. P.; Horn, M.; Huang, D. Q.; Ignarra, C. M.; Jacobsen, R. G.; Ji, W.; Kamdin, K.; Kazkaz, K.; Khaitan, D.; Knoche, R.; Lenardo, B. G.; Lesko, K. T.; Liao, J.; Lindote, A.; Lopes, M. I.; Manalaysay, A.; Mannino, R. L.; Marzioni, M. F.; McKinsey, D. N.; Mei, D.-M.; Mock, J.; Moongweluwan, M.; Morad, J. A.; Murphy, A. St. J.; Nehrkorn, C.; Nelson, H. N.; Neves, F.; O'Sullivan, K.; Oliver-Mallory, K. C.; Palladino, K. J.; Pease, E. K.; Rhyne, C.; Shaw, S.; Shutt, T. A.; Silva, C.; Solmaz, M.; Solovov, V. N.; Sorensen, P.; Sumner, T. J.; Szydagis, M.; Taylor, D. J.; Taylor, W. C.; Tennyson, B. P.; Terman, P. A.; Tiedt, D. R.; To, W. H.; Tripathi, M.; Tvrznikova, L.; Utku, U.; Uvarov, S.; Velan, V.; Verbus, J. R.; Webb, R. C.; White, J. T.; Whitis, T. J.; Witherell, M. S.; Wolfs, F. L. H.; Xu, J.; Yazdani, K.; Young, S. K.; Zhang, C.; LUX Collaboration

2018-06-01

Weakly interacting massive particles (WIMPs) are a leading candidate for dark matter and are expected to produce nuclear recoil (NR) events within liquid xenon time-projection chambers. We present a measurement of the scintillation timing characteristics of liquid xenon in the LUX dark matter detector and develop a pulse shape discriminant to be used for particle identification. To accurately measure the timing characteristics, we develop a template-fitting method to reconstruct the detection times of photons. Analyzing calibration data collected during the 2013-2016 LUX WIMP search, we provide a new measurement of the singlet-to-triplet scintillation ratio for electron recoils (ER) below 46 keV, and we make, to our knowledge, a first-ever measurement of the NR singlet-to-triplet ratio at recoil energies below 74 keV. We exploit the difference of the photon time spectra for NR and ER events by using a prompt fraction discrimination parameter, which is optimized using calibration data to have the least number of ER events that occur in a 50% NR acceptance region. We then demonstrate how this discriminant can be used in conjunction with the charge-to-light discrimination to possibly improve the signal-to-noise ratio for nuclear recoils.

Pulse shape discrimination based on fast signals from silicon photomultipliers

NASA Astrophysics Data System (ADS)

Yu, Junhao; Wei, Zhiyong; Fang, Meihua; Zhang, Zixia; Cheng, Can; Wang, Yi; Su, Huiwen; Ran, Youquan; Zhu, Qingwei; Zhang, He; Duan, Kai; Chen, Ming; Liu, Meng

2018-06-01

Recent developments in organic plastic scintillators capable of pulse shape discrimination (PSD) enable a breakthrough in discrimination between neutrons and gammas. Plastic scintillator detectors coupled with silicon photomultipliers (SiPMs) offer many advantages, such as lower power consumption, smaller volume, and especially insensitivity to magnetic fields, compared with conventional photomultiplier tubes (PMTs). A SensL SiPM has two outputs: a standard output and a fast output. It is known that the charge injected into the fast output electrode is typically approximately 2% of the total charge generated during the avalanche, whereas the charge injected into the standard output electrode is nearly 98% of the total. Fast signals from SiPMs exhibit better performance in terms of timing and time-correlated measurements compared with standard signals. The pulse duration of a standard signal is on the order of hundreds of nanoseconds, whereas the pulse duration of the main monopole waveform of a fast signal is a few tens of nanoseconds. Fast signals are traditionally thought to be suitable for photon counting at very high speeds but unsuitable for PSD due to the partial charge collection. Meanwhile, the standard outputs of SiPMs coupled with discriminating scintillators have yielded nice PSD performances, but there have been no reports on PSD using fast signals. Our analysis shows that fast signals can also provide discrimination if the rate of charge injection into the fast output electrode is fixed for each event, even though only a portion of the charge is collected. In this work, we achieved successful PSD using fast signals; meanwhile, using a coincidence timing window of less 3 nanoseconds between the readouts from both ends of the detector reduced the influence of the high SiPM dark current. We experimentally achieved good timing performance and PSD capability simultaneously.

Single transmission-line readout method for silicon photomultiplier based time-of-flight and depth-of-interaction PET

NASA Astrophysics Data System (ADS)

Ko, Guen Bae; Lee, Jae Sung

2017-03-01

We propose a novel single transmission-line readout method for whole-body time-of-flight positron emission tomography applications, without compromising on performance. The basic idea of the proposed multiplexing method is the addition of a specially prepared tag signal ahead of the scintillation pulse. The tag signal is a square pulse that encodes photon arrival time and channel information. The 2D position of a silicon photomultiplier (SiPM) array is encoded by the specific width and height of the tag signal. A summing amplifier merges the tag and scintillation signals of each channel, and the final output signal can be acquired with a one-channel digitizer. The feasibility and performance of the proposed method were evaluated using a 1:1 coupled detector consisting of 4  ×  4 array of LGSO crystals and 16 channel SiPM. The sixteen 3 mm LGSO crystals were clearly separated in the crystal-positioning map with high reliability. The average energy resolution and coincidence resolving time were 11.31  ±  0.55% and 264.7  ±  10.7 ps, respectively. We also proved that the proposed method does not degrade timing performance with increasing multiplexing ratio. The two types of LGSO crystals (L0.95GSO and L0.20GSO) in phoswich detector were also clearly identified with the high-reliability using pulse shape discrimination, thanks to the well-preserved pulse shape information. In conclusion, the proposed multiplexing method allows decoding of the 3D interaction position of gamma rays in the scintillation detector with single-line readout.

Single transmission-line readout method for silicon photomultiplier based time-of-flight and depth-of-interaction PET.

PubMed

Ko, Guen Bae; Lee, Jae Sung

2017-03-21

We propose a novel single transmission-line readout method for whole-body time-of-flight positron emission tomography applications, without compromising on performance. The basic idea of the proposed multiplexing method is the addition of a specially prepared tag signal ahead of the scintillation pulse. The tag signal is a square pulse that encodes photon arrival time and channel information. The 2D position of a silicon photomultiplier (SiPM) array is encoded by the specific width and height of the tag signal. A summing amplifier merges the tag and scintillation signals of each channel, and the final output signal can be acquired with a one-channel digitizer. The feasibility and performance of the proposed method were evaluated using a 1:1 coupled detector consisting of 4  ×  4 array of LGSO crystals and 16 channel SiPM. The sixteen 3 mm LGSO crystals were clearly separated in the crystal-positioning map with high reliability. The average energy resolution and coincidence resolving time were 11.31  ±  0.55% and 264.7  ±  10.7 ps, respectively. We also proved that the proposed method does not degrade timing performance with increasing multiplexing ratio. The two types of LGSO crystals (L 0.95 GSO and L 0.20 GSO) in phoswich detector were also clearly identified with the high-reliability using pulse shape discrimination, thanks to the well-preserved pulse shape information. In conclusion, the proposed multiplexing method allows decoding of the 3D interaction position of gamma rays in the scintillation detector with single-line readout.

FAST NEUTRON SPECTROMETER

DOEpatents

Davis, F.J.; Hurst, G.S.; Reinhardt, P.W.

1959-08-18

An improved proton recoil spectrometer for determining the energy spectrum of a fast neutron beam is described. Instead of discriminating against and thereby"throwing away" the many recoil protons other than those traveling parallel to the neutron beam axis as do conventional spectrometers, this device utilizes protons scattered over a very wide solid angle. An ovoidal gas-filled recoil chamber is coated on the inside with a scintillator. The ovoidal shape of the sensitive portion of the wall defining the chamber conforms to the envelope of the range of the proton recoils from the radiator disposed within the chamber. A photomultiplier monitors the output of the scintillator, and a counter counts the pulses caused by protons of energy just sufficient to reach the scintillator.

Gamma ray spectroscopy employing divalent europium-doped alkaline earth halides and digital readout for accurate histogramming

DOEpatents

Cherepy, Nerine Jane; Payne, Stephen Anthony; Drury, Owen B.; Sturm, Benjamin W.

2016-02-09

According to one embodiment, a scintillator radiation detector system includes a scintillator, and a processing device for processing pulse traces corresponding to light pulses from the scintillator, where the processing device is configured to: process each pulse trace over at least two temporal windows and to use pulse digitization to improve energy resolution of the system. According to another embodiment, a scintillator radiation detector system includes a processing device configured to: fit digitized scintillation waveforms to an algorithm, perform a direct integration of fit parameters, process multiple integration windows for each digitized scintillation waveform to determine a correction factor, and apply the correction factor to each digitized scintillation waveform.

Fast-Neutron Survey With Compact Plastic Scintillation Detectors.

PubMed

Preston, Rhys M; Tickner, James R

2017-07-01

With the rise of the Silicon Photomultiplier (SiPM), it is now practical to build compact scintillation detectors well suited to portable use. A prototype survey meter for fast-neutrons and gamma-rays, based around an EJ-299-34 plastic scintillator with SiPM readout, has been developed and tested. A custom digital pulse processor was used to perform pulse shape discrimination on-the-fly. Ambient dose equivalent H*(10) was calculated by means of two energy-dependent 'G-functions'. The sensitivity was calculated to be between 0.10 and 0.22 cps/(µSv/hr) for fast-neutrons with energies above 2.5 MeV. The prototype was used to survey various laboratory radiation fields, with the readings compared with commercial survey meters. The high sensitivity and lightweight nature of this detector makes it promising for rapid survey of the mixed neutron/gamma-ray fields encountered in industry and homeland security. © The Author 2017. Published by Oxford University Press. All rights reserved. For Permissions, please email: journals.permissions@oup.com.

Development and operation of a 6LiF:ZnS(Ag)-scintillating plastic capture-gated detector

NASA Astrophysics Data System (ADS)

Wilhelm, K.; Nattress, J.; Jovanovic, I.

2017-01-01

We report on the design, construction, and operation of a capture-gated neutron detector based on a heterogeneous scintillating structure comprising two scintillator types. A flat, 500 μm thick sheet composed of a mixture of lithium-6-fluoride capture agent, 6LiF, and zinc sulfide phosphor, ZnS(Ag), is wrapped around scintillating polyvinyl toluene (PVT) in a form of cylinder. The 6LiF: ZnS(Ag) sheet uses an aluminum foil backing as a support for the scintillating material and as an optical reflector, and its optical properties have been characterized independently. The composite scintillator was tested using 252Cf, DD fusion, 137Cs, and 60Co sources. The intrinsic detection efficiency for neutrons from an unmoderated 252Cf source and rejection of gammas from 137Cs were measured to be 3.6 % and 10-6, respectively. A figure of merit for pulse shape discrimination of 4.6 was achieved, and capture-gated spectroscopic analysis is demonstrated.

Spectroscopic Investigations with Dual Neutron-Gamma Scintillators

NASA Astrophysics Data System (ADS)

Chowdhury, P.; Brown, T.; Doucet, E.; Lister, C. J.; Morse, C.; Rogers, A. M.; Wilson, G. L.; Devlin, M.; Fotiades, N.; Gomez, J. A.; Mosby, S.

2017-09-01

The spectroscopic capabilities of 7Li-enriched Cs27LiYCl6 (C7LYC) dual neutron-gamma scintillators are being tested in diverse application arenas to exploit the excellent pulse-shape discrimination together with the unprecedented pulse height resolution ( 10%) for fast neutrons in the < 8 MeV range via the 35Cl(n,p) reaction. Test experiments include both elastic and inelastic neutron scattering cross-sections on 56Fe at Los Alamos with a pulsed white neutron source, as well as (p,n) and (d,n) reactions on low-Z targets using mono-energetic proton and deuteron beams from the 5.5 MV Van de Graaff accelerator at the UMass Lowell Radiation Laboratory. Tests of waveform digitizers with different sampling rates are also being performed. A key goal is to evaluate whether the low intrinsic efficiency of C7LYC for fast neutrons compared to traditional neutron detectors, such as liquid scintillators, can be effectively offset by the gain in solid angle obtained by positioning the detectors much closer to the target, since the typical long time-of-flight arms for energy resolution are not necessary. Supported by the NNSA Stewardship Science Academic Alliance Program under Grant DE-NA0002932.

Tagging radon daughters in low-energy scintillation detectors

NASA Astrophysics Data System (ADS)

McCarty, Kevin B.

2011-12-01

One problematic source of background in scintillator-based low-energy solar neutrino experiments such as Borexino is the presence of radon gas and its daughters. The mean lifetime of the α-emitter 214Po in the radon chain is sufficiently short, 0.24 ms, that its decay, together with that immediately preceding of 214Bi, is easily recognized as a “coincidence event.” This fact, combined with the capability of α/β pulse-shape discrimination, makes it possible to tag decays of 222Rn and its first four daughters via a likelihood-based method.

Cerium-doped scintillating fused-silica fibers

NASA Astrophysics Data System (ADS)

Akchurin, N.; Cowden, C.; Damgov, J.; Dragoiu, C.; Dudero, P.; Faulkner, J.; Kunori, S.

2018-04-01

We report on a set of measurements made on (scintillating) cerium-doped fused-silica fibers using high-energy particle beams. These fibers were uniformly embedded in a copper absorber in order to utilize electromagnetic showers as a source of charged particles for generating signals. This new type of cerium-doped fiber potentially offers myriad new applications in calorimeters in high-energy physics, tracking systems, and beam monitoring detectors for future applications. The light yield, pulse shape, attenuation length, and light propagation speeds are given and discussed. Possible future applications are also explored.

Investigation of BCF-12 Plastic Scintillating Coherent Fiber Bundle Timing Properties

DTIC Science & Technology

2012-03-22

spread in transit time. The shape of the voltage pulse produced at the anode of a PM following a scin - tillation event depends on the time constant of...Choong, G. Hull, and B.W. Reutter. “ Scin - tillator Non-Proportionality: Present Understanding and Future Challenges”. Nuclear Science, IEEE

Apparatuses for large area radiation detection and related method

DOEpatents

Akers, Douglas W; Drigert, Mark W

2015-04-28

Apparatuses and a related method relating to radiation detection are disclosed. In one embodiment, an apparatus includes a first scintillator and a second scintillator adjacent to the first scintillator, with each of the first scintillator and second scintillator being structured to generate a light pulse responsive to interacting with incident radiation. The first scintillator is further structured to experience full energy deposition of a first low-energy radiation, and permit a second higher-energy radiation to pass therethrough and interact with the second scintillator. The apparatus further includes a plurality of light-to-electrical converters operably coupled to the second scintillator and configured to convert light pulses generated by the first scintillator and the second scintillator into electrical signals. The first scintillator and the second scintillator exhibit at least one mutually different characteristic for an electronic system to determine whether a given light pulse is generated by the first scintillator or the second scintillator.

Performance evaluation for 120 four-layer DOI block detectors of the jPET-D4.

PubMed

Inadama, Naoko; Murayama, Hideo; Ono, Yusuke; Tsuda, Tomoaki; Hamamoto, Manabu; Yamaya, Taiga; Yoshida, Eiji; Shibuya, Kengo; Nishikido, Fumihiko; Takahashi, Kei; Kawai, Hideyuki

2008-01-01

The jPET-D4 is a brain positron emission tomography (PET) scanner that we have developed to meet user demands for high sensitivity and high spatial resolution. For this scanner, we developed a four-layer depth-of-interaction (DOI) detector. The four-layer DOI detector is a key component for the jPET-D4, its performance has great influence on the overall system performance. Previously, we reported the original technique for encoding four-layer DOI. Here, we introduce the final design of the jPET-D4 detector and present the results of an investigation on uniformity in performance of the detector. The performance evaluation was done over the 120 DOI crystal blocks for the detectors, which are to be assembled into the jPET-D4 scanner. We also introduce the crystal assembly method, which is simple enough, even though each DOI crystal block is composed of 1,024 crystal elements. The jPET-D4 detector consists of four layers of 16 x 16 Gd(2)SiO(5) (GSO) crystals and a 256-channel flat-panel position-sensitive photomultiplier tube (256ch FP-PMT). To identify scintillated crystals in the four-layer DOI detector, we use pulse shape discrimination and position discrimination on the two-dimensional (2D) position histogram. For pulse shape discrimination, two kinds of GSO crystals that show different scintillation decay time constants are used in the upper two and lower two layers, respectively. Proper reflector arrangement in the crystal block then allows the scintillated crystals to be identified in these two-layer groupings with two 2D position histograms. We produced the 120 DOI crystal blocks for the jPET-D4 system, and measured their characteristics such as the accuracy of pulse shape discrimination, energy resolution, and the pulse height of the full energy peak. The results show a satisfactory and uniform performance of the four-layer DOI crystal blocks; for example, misidentification rate in each GSO layer is <5% based on pulse shape discrimination, the averaged energy resolutions for the central four crystals of the first (farthest from the FP-PMT), second, third, and 4th layers are 15.7 +/- 1.0, 15.8 +/- 0.6, 17.7 +/- 1.2, and 17.3 +/- 1.4%, respectively, and variation in pulse height of the full energy peak among the four layers is <5% on average.

Plastic Scintillators for Pulse Shape Discrimination of Particle Types in Radiation Detection

NASA Astrophysics Data System (ADS)

Hajagos, Tibor Jacob

Organic scintillators have a long history in the field of radiation detection, dating back to some of the earliest studies of organic photophysics and optoelectronic properties. In particular, plastics have come to dominate the commercial market for organic scintillators, due to their low cost and ease of use and manufacturing, and more notably in spite of their poorer performance in many metrics. While there has been decades of active research since their inception, little progress has been made to improve upon the now well established compositions of commercial plastics, a notable exception being the recent development of plastic scintillators capable of pulse shape discrimination (PSD) of n/gamma radiation, which is of particular interest among governments and industry for the detection of illicit nuclear material and weapons. In recent years, much attention has been paid towards the study of luminescent organic materials, in particular due to the invention and widespread adoption of organic light emitting diode (OLED) based electronic devices, and the knowledge and lessons that have been fundamental to such fields have recently begun to be adopted by the organic scintilator community. In this work, new approaches to the design of both plastic scintillator components, and of the materials as a whole, are described, with particular emphasis paid towards the design and synthesis of small molecule scintillating dyes that are specifically tailored towards the development of PSD-capable plastic scintilators. In the first of these approaches, the design and synthesis of a highly soluble and polymerizable derivative of 9,10-diphenylanthracene is described, and the properties of plastic scintilators fabricated from this dye when copolymerized with poly(vinyl toluene) were investigated. This particular approach was used to demonstrate a proof-of-concept of PSD in highly loaded plastics stabilized through copolymerization of the primary dye, a strategy conceived to address the particular shortcomings of the current generation of PSD plastics. The second general approach investigated is the application of the phenomenon of thermally activated delayed fluorescence (TADF)--most notably a key innovation among the latest developments in OLED technologies--to the enhancement of the performance of organic sicntillators. Several key observations about the potential and efficacy of TADF dyes as novel organic scintillators were made, including a demonstration of the profound effects the TADF phenomenon can have on scintillation properties. These findings suggest that it is quite possible that TADF dyes could eventually enable an entirely new generation of high performance organic scintillators, and PSD-capable plastics in particular.

DESCANT--The DEuterated SCintillator Array for Neutron Tagging

NASA Astrophysics Data System (ADS)

Bildstein, Vinzenz; Garrett, P. E.; Bandyopadhay, D.; Bangay, J.; Bianco, L.; Demand, G.; Hadinia, B.; Leach, K. G.; Sumithrarachchi, C.; Wong, J.; Ashley, S. F.; Crider, B. P.; McEllistrem, M. T.; Peters, E. E.; Prados-Estévez, F. M.; Yates, S. W.; Vanhoy, J. R.; Ball, G. C.; Garnsworthy, A. B.; Hackman, G.; Pearson, C. J.; Sarazin, F.

2014-09-01

The DESCANT array at TRIUMF is designed to track neutrons from RIB experiments. DESCANT is composed of 70 close-packed deuterated organic liquid scintillators coupled to digital fast read-out ADC modules. This configuration will permit online pulse-shape discrimination between neutron and γ-ray events. The anisotropy of the n - d scattering will allow distinction of higher neutron multiplicities from scattering within the array and determination of the neutron energy spectrum directly from the pulse-height spectrum without using TOF. A prototype detector has been tested with monoenergetic neutrons at the accelerator laboratory of the University of Kentucky and a 24Mg(3He, n)26Si experiment has been performed with eight DESCANT detectors and two HPGe detectors. The results of the tests and the status of DESCANT will be presented.

Characterization of a tin-loaded liquid scintillator for gamma spectroscopy and neutron detection

NASA Astrophysics Data System (ADS)

Wen, Xianfei; Harvey, Taylor; Weinmann-Smith, Robert; Walker, James; Noh, Young; Farley, Richard; Enqvist, Andreas

2018-07-01

A tin-loaded liquid scintillator has been developed for gamma spectroscopy and neutron detection. The scintillator was characterized in regard to energy resolution, pulse shape discrimination, neutron light output function, and timing resolution. The loading of tin into scintillators with low effective atomic number was demonstrated to provide photopeaks with acceptable energy resolution. The scintillator was shown to have reasonable neutron/gamma discrimination capability based on the charge comparison method. The effect on the discrimination quality of the total charge integration time and the initial delay time for tail charge integration was studied. To obtain the neutron light output function, the time-of-flight technique was utilized with a 252Cf source. The light output function was validated with the MCNPX-PoliMi code by comparing the measured and simulated pule height spectra. The timing resolution of the developed scintillator was also evaluated. The tin-loading was found to have negligible impact on the scintillation decay times. However, a relatively large degradation of timing resolution was observed due to the reduced light yield.

Method, apparatus and system for low-energy beta particle detection

DOEpatents

Akers, Douglas W.; Drigert, Mark W.

2012-09-25

An apparatus, method, and system relating to radiation detection of low-energy beta particles are disclosed. An embodiment includes a radiation detector with a first scintillator and a second scintillator operably coupled to each other. The first scintillator and the second scintillator are each structured to generate a light pulse responsive to interaction with beta particles. The first scintillator is structured to experience full energy deposition of low-energy beta particles, and permit a higher-energy beta particle to pass therethrough and interact with the second scintillator. The radiation detector further includes a light-to-electrical converter operably coupled to the second scintillator and configured to convert light pulses generated by the first scintillator and the second scintillator into electrical signals. The first scintillator and the second scintillator have at least one mutually different characteristic to enable an electronic system to determine whether a given light pulse is generated in the first scintillator or the second scintillator.

Pulse-shape discrimination and energy quenching of alpha particles in Cs 2LiLaBr 6:Ce 3+

DOE PAGES

Mesick, Katherine Elizabeth; Coupland, Daniel David S.; Stonehill, Laura Catherine

2016-10-19

Cs 2LiLaBr 6:Ce 3+ (CLLB) is an elpasolite scintillator that offers excellent linearity and gamma-ray energy resolution and sensitivity to thermal neutrons with the ability to perform pulse-shape discrimination (PSD) to distinguish gammas and neutrons. Our investigation of CLLB has indicated the presence of intrinsic radioactive alpha background that we have determined to be from actinium contamination of the lanthanum component. We measured the pulse shapes for gamma, thermal neutron, and alpha events and determined that PSD can be performed to separate the alpha background with a moderate figure of merit of 0.98. Here, we also measured the electron-equivalent-energy ofmore » the alpha particles in CLLB and simulated the intrinsic alpha background from 227Ac to determine the quenching factor of the alphas.« less

Functionalization of Polymers with Fluorescent and Neutron Sensitive Groups for Efficient Neutron and Gamma Detection

NASA Astrophysics Data System (ADS)

Mahl, Adam; Yemam, Henok; Remedes, Tyler; Stuntz, Jack; Koldemir, Unsal; Sellinger, Alan; Greife, Uwe

2015-10-01

This presentation will review the efforts made by an interdisciplinary development project aimed at cost-effective, thermal neutron sensitive, plastic scintillators as part of the communities efforts towards replacing 3He based detectors. Colorado School of Mines researchers with backgrounds in Physics and Chemistry have worked on the incorporation of 10B in plastics through admixture of various commercial and novel dopants developed at CSM. In addition, new fluorescent dopants have been developed for plastic scintillators in an effort towards better understanding quenching effects and scintillator response to thermal neutrons via pulse shape discrimination methods. Results on transparent samples using fluorescent spectroscopy and gamma/neutron excitation will be presented. Funded via Department of Homeland Security - Domestic Nuclear Detection Office.

Neutron spectroscopy with scintillation detectors using wavelets

NASA Astrophysics Data System (ADS)

Hartman, Jessica

The purpose of this research was to study neutron spectroscopy using the EJ-299-33A plastic scintillator. This scintillator material provided a novel means of detection for fast neutrons, without the disadvantages of traditional liquid scintillation materials. EJ-299-33A provided a more durable option to these materials, making it less likely to be damaged during handling. Unlike liquid scintillators, this plastic scintillator was manufactured from a non-toxic material, making it safer to use, as well as easier to design detectors. The material was also manufactured with inherent pulse shape discrimination abilities, making it suitable for use in neutron detection. The neutron spectral unfolding technique was developed in two stages. Initial detector response function modeling was carried out through the use of the MCNPX Monte Carlo code. The response functions were developed for a monoenergetic neutron flux. Wavelets were then applied to smooth the response function. The spectral unfolding technique was applied through polynomial fitting and optimization techniques in MATLAB. Verification of the unfolding technique was carried out through the use of experimentally determined response functions. These were measured on the neutron source based on the Van de Graff accelerator at the University of Kentucky. This machine provided a range of monoenergetic neutron beams between 0.1 MeV and 24 MeV, making it possible to measure the set of response functions of the EJ-299-33A plastic scintillator detector to neutrons of specific energies. The response of a plutonium-beryllium (PuBe) source was measured using the source available at the University of Nevada, Las Vegas. The neutron spectrum reconstruction was carried out using the experimentally measured response functions. Experimental data was collected in the list mode of the waveform digitizer. Post processing of this data focused on the pulse shape discrimination analysis of the recorded response functions to remove the effects of photons and allow for source characterization based solely on the neutron response. The unfolding technique was performed through polynomial fitting and optimization techniques in MATLAB, and provided an energy spectrum for the PuBe source.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Lawrence, Chris C.; Febbraro, Michael; Massey, Thomas N.

Organic scintillation detectors have shown promise as neutron detectors for characterizing special nuclear materials in various arms-control and homeland security applications. Recent advances have yielded a new plastic scintillator - EJ299-33 - with pulse-shape-discrimination (PSD) capability. Plastic scintillators would have a much expanded range of deployment relative to liquids and crystals. Here in this paper, we present a full characterization of pulse height response to fission-energy neutrons for an EJ299-33 detector with 7.62-by-7.62-cm cylindrical active volume, and compare with an EJ309 liquid scintillator in the same assembly. Scintillation light output relations, energy resolutions, and response matrices are presented for bothmore » detectors. A Continuous spectrum neutron source, obtained via the bombardment of 27Al with 7.44-MeV deuterons at the Edwards Accelerator Facility at Ohio University, was used for the measurement. A new procedure for evaluating and comparing PSD performance is presented which accounts for the effect of the light output relation on the ability to detect low energy neutrons. The EJ299-33 is shown to have considerable deficit in matrix condition, and in PSD figure of merit when compared to EJ309, especially when neutron energy is taken into account. Furthermore the EJ299 is likely to bring a modest PSD capability into a array of held applications that are not accessible to liquids or crystals.« less

Scintillator Development for the PROSPECT Experiment

NASA Astrophysics Data System (ADS)

Yeh, Minfang

2014-03-01

Doped scintillator is the target material of choice for antineutrino detection as it utilizes the time-delayed coincidence signature of the positron annihilation and neutron capture resulting from the Inverse Beta Decay (IBD) interaction. Additionally, the multiple gamma rays or heavy ions emitted after neutron capture on either Gd or 6Li respectively provide a distinct signal for the identification of antineutrino events and therefore significantly enhance accidental background reduction. The choice of scintillator and dopant depends on the detector requirements and scintillator performance criteria. Both Gd and 6Li doped scintillators have been used in past reactor antineutrino experiments such as Double Chooz, Daya Bay, RENO, and Bugey3 and are currently under investigation by the PROSPECT collaboration. Their properties in terms of light yield, optical transparency, chemical stability and background rejection efficiency using Pulse Shape Discrimination (PSD) will be reported. Research sponsored by the U.S. Department of Energy, Office of Nuclear Physics and Office of High Energy Physics, under contract with Brookhaven National Laboratory-Brookhaven Science Associates.

Organic Scintillator Detector Response Simulations with DRiFT

DOE PAGES

Andrews, Madison Theresa; Bates, Cameron Russell; Mckigney, Edward Allen; ...

2016-06-11

Here, this work presents the organic scintillation simulation capabilities of DRiFT, a post-processing Detector Response Function Toolkit for MCNPR output. DRiFT is used to create realistic scintillation detector response functions to incident neutron and gamma mixed- field radiation. As a post-processing tool, DRiFT leverages the extensively validated radiation transport capabilities of MCNPR ®6, which also provides the ability to simulate complex sources and geometries. DRiFT is designed to be flexible, it allows the user to specify scintillator material, PMT type, applied PMT voltage, and quenching data used in simulations. The toolkit's capabilities, which include the generation of pulse shape discriminationmore » plots and full-energy detector spectra, are demonstrated in a comparison of measured and simulated neutron contributions from 252Cf and PuBe, and photon spectra from 22Na and 228Th sources. DRiFT reproduced energy resolution effects observed in EJ-301 measurements through the inclusion of scintillation yield variances, photon transport noise, and PMT photocathode and multiplication noise.« less

Organic scintillator detector response simulations with DRiFT

NASA Astrophysics Data System (ADS)

Andrews, M. T.; Bates, C. R.; McKigney, E. A.; Solomon, C. J.; Sood, A.

2016-09-01

This work presents the organic scintillation simulation capabilities of DRiFT, a post-processing Detector Response Function Toolkit for MCNP® output. DRiFT is used to create realistic scintillation detector response functions to incident neutron and gamma mixed-field radiation. As a post-processing tool, DRiFT leverages the extensively validated radiation transport capabilities of MCNP® 6 , which also provides the ability to simulate complex sources and geometries. DRiFT is designed to be flexible, it allows the user to specify scintillator material, PMT type, applied PMT voltage, and quenching data used in simulations. The toolkit's capabilities, which include the generation of pulse shape discrimination plots and full-energy detector spectra, are demonstrated in a comparison of measured and simulated neutron contributions from 252Cf and PuBe, and photon spectra from 22Na and 228Th sources. DRiFT reproduced energy resolution effects observed in EJ-301 measurements through the inclusion of scintillation yield variances, photon transport noise, and PMT photocathode and multiplication noise.

Comparing the response of PSD-capable plastic scintillator to standard liquid scintillator

NASA Astrophysics Data System (ADS)

Woolf, Richard S.; Hutcheson, Anthony L.; Gwon, Chul; Phlips, Bernard F.; Wulf, Eric A.

2015-06-01

This work discusses a test campaign to characterize the response of the recently developed plastic scintillator with pulse shape discrimination (PSD) capabilities (EJ-299-33). PSD is a property exhibited by certain types of scintillating material in which incident stimuli (fast neutrons or γ rays) can be separated by exploiting differences in the scintillation light pulse tail. Detector geometries used were: a 10 cm×10 cm×10 cm cube and a 10-cm diameter×10-cm long cylinder. EJ-301 and EJ-309 liquid scintillators with well-known responses were also tested. The work was conducted at the University of Massachusetts Lowell Van De Graaff accelerator. The facility accelerated protons on a thin Li target to yield quasi-monoenergetic neutrons from the 7Li(p,n)7Be reaction (Q-value: -1.644 MeV). Collimated fast neutrons were obtained by placing detectors behind a neutron spectrometer. Rotating the spectrometer, and thus changing the neutron energy, allowed us to achieve 0.5-3.2 MeV neutrons in 200-300 keV steps. Data were acquired through a flash analog-to-digital converter (ADC) capable of performing digital PSD measurements. By using the PSD technique to separate the neutron events from unwanted γ background, we constructed a pulse height spectrum at each energy. Obtaining a relationship of the relative light output versus energy allowed us to construct the response function for the EJ-299-33 and liquid scintillator. The EJ-299-33 response in terms of electron equivalent energy (Ee.e.) vs. proton equivalent energy (Ep.e.), how it compared with the standard xylene-based EJ-301 (or, NE-213/BC-501 A equivalent) and EJ-309 liquid scintillator response, and how the EJ-301 and EJ-309 compared, are presented. We find that the EJ-299-33 demonstrated a lower light output by up to 40% for <1.0 MeV neutrons; and ranging between a 5-35% reduction for 2.5-3.0 MeV neutrons compared to the EJ-301/309, depending on the scintillator and geometry. Monte Carlo modeling techniques were used to investigate how the neutron beam and accelerator background environment affected the detector response. We find relatively good agreement between our results and the modeling; however, the observed response could not be fully accounted for due to events with pulse pile up, thus leading to contamination of the neutron PSD selected events.

Cherenkov and Scintillation Properties of Cubic Zirconium

NASA Technical Reports Server (NTRS)

Christl, M.J.; Adams, J.H.; Parnell, T.A.; Kuznetsov, E.N.

2008-01-01

Cubic zirconium (CZ) is a high index of refraction (n =2.17) material that we have investigated for Cherenkov counter applications. Laboratory and proton accelerator tests of an 18cc sample of CZ show that the expected fast Cherenkov response is accompanied by a longer scintillation component that can be separated by pulse shaping. This presents the possibility of novel particle spectrometers which exploits both properties of CZ. Other high index materials being examined for Cherenkov applications will be discussed. Results from laboratory tests and an accelerator exposure will be presented and a potential application in solar energetic particle instruments will be discussed

Light detection and the wavelength shifter deposition in DEAP-3600

NASA Astrophysics Data System (ADS)

Broerman, B.; Retière, F.

2016-02-01

The Dark matter Experiment using Argon Pulse-shape discrimination (DEAP) uses liquid argon as a target medium to perform a direct-detection dark matter search. The 3600 kg liquid argon target volume is housed in a spherical acrylic vessel and viewed by a surrounding array of photomultiplier tubes. Ionizing particles in the argon volume produce scintillation light which must be wavelength shifted to be detected by the photomultiplier tubes. Argon scintillation and wavelength shifting, along with details on the application of the wavelength shifter to the inner surface of the acrylic vessel are presented.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ashenfelter, J.; Jaffe, D.; Diwan, M. V.

A meter-long, 23-liter EJ-309 liquid scintillator detector has been constructed to study the light collection and pulse-shape discrimination performance of elongated scintillator cells for the PROSPECT reactor antineutrino experiment. The magnitude and uniformity of light collection and neutron-gamma discrimination power in the energy range of antineutrino inverse beta decay products have been studied using gamma and spontaneous fission calibration sources deployed along the cell axis. We also study neutron-gamma discrimination and light collection abilities for differing PMT and reflector configurations. As a result, key design features for optimizing MeV-scale response and background rejection capabilities are identified.

On the Relationship Between Scintillation Anisotropy and Crystal Structure in Pure Crystalline Organic Scintillator Materials

DOE Office of Scientific and Technical Information (OSTI.GOV)

Schuster, Patricia; Feng, Patrick; Brubaker, Erik

We report the scintillation anisotropy effect for proton recoil events has been investigated in five pure organic crystalline materials: anthracene, trans-stilbene, p-terphenyl, bibenzyl, and diphenylacetylene. These measurements include characterization of the scintillation response for one hemisphere of proton recoil directions in each crystal. In addition to standard measurements of the total light output and pulse shape at each angle, the prompt and delayed light anisotropies are analyzed, allowing for investigation of the singlet and triplet molecular excitation behaviors independently. This work provides new quantitative and qualitative observations that make progress toward understanding the physical mechanisms behind the scintillation anisotropy. Thesemore » measurements show that the relationship between the prompt and delayed light anisotropies is correlated with crystal structure, as it changes between the pi-stacked crystal structure materials (anthracene and p-terphenyl) and the herringbone crystal structure materials (stilbene, bibenzyl, and diphenylacetylene). The observations are consistent with a model in which there are preferred directions of kinetic processes for the molecular excitations. Finally, these processes and the impact of their directional dependencies on the scintillation anisotropy are discussed.« less

On the Relationship Between Scintillation Anisotropy and Crystal Structure in Pure Crystalline Organic Scintillator Materials

DOE PAGES

Schuster, Patricia; Feng, Patrick; Brubaker, Erik

2018-05-03

We report the scintillation anisotropy effect for proton recoil events has been investigated in five pure organic crystalline materials: anthracene, trans-stilbene, p-terphenyl, bibenzyl, and diphenylacetylene. These measurements include characterization of the scintillation response for one hemisphere of proton recoil directions in each crystal. In addition to standard measurements of the total light output and pulse shape at each angle, the prompt and delayed light anisotropies are analyzed, allowing for investigation of the singlet and triplet molecular excitation behaviors independently. This work provides new quantitative and qualitative observations that make progress toward understanding the physical mechanisms behind the scintillation anisotropy. Thesemore » measurements show that the relationship between the prompt and delayed light anisotropies is correlated with crystal structure, as it changes between the pi-stacked crystal structure materials (anthracene and p-terphenyl) and the herringbone crystal structure materials (stilbene, bibenzyl, and diphenylacetylene). The observations are consistent with a model in which there are preferred directions of kinetic processes for the molecular excitations. Finally, these processes and the impact of their directional dependencies on the scintillation anisotropy are discussed.« less

A Deuterated Neutron Detector Array For Nuclear (Astro)Physics Studies

NASA Astrophysics Data System (ADS)

Almaraz-Calderon, Sergio; Asher, B. W.; Barber, P.; Hanselman, K.; Perello, J. F.

2016-09-01

The properties of neutron-rich nuclei are at the forefront of research in nuclear structure, nuclear reactions and nuclear astrophysics. The advent of intense rare isotope beams (RIBs) has opened a new door for studies of systems with very short half-lives and possible fascinating properties. Neutron spectroscopic techniques become increasingly relevant when these neutron rich nuclei are used in a variety of experiments. At Florida State University, we are developing a neutron detector array that will allow us to perform high-resolution neutron spectroscopic studies with stable and radioactive beams. The neutron detection system consists of 16 deuterated organic liquid scintillation detectors with fast response and pulse-shape discrimination capabilities. In addition to these properties, there is the potential to use the structure in the pulse-height spectra to extract the energy of the neutrons and thus produce directly excitation spectra. This type of detector uses deuterated benzene (C6D6) as the liquid scintillation medium. The asymmetric nature of the scattering between a neutron and a deuterium in the center of mass produces a pulse-height spectrum from the deuterated scintillator which contains useful information on the initial energy of the neutron. Work supported in part by the State of Florida and NSF Grant No. 1401574.

Spectroscopic neutron detection using composite scintillators

NASA Astrophysics Data System (ADS)

Jovanovic, I.; Foster, A.; Kukharev, V.; Mayer, M.; Meddeb, A.; Nattress, J.; Ounaies, Z.; Trivelpiece, C.

2016-09-01

Shielded special nuclear material (SNM), especially highly enriched uranium, is exceptionally difficult to detect without the use of active interrogation (AI). We are investigating the potential use of low-dose active interrogation to realize simultaneous high-contrast imaging and photofission of SNM using energetic gamma-rays produced by low-energy nuclear reactions, such as 11B(d,nγ)12C and 12C(p,p‧)12C. Neutrons produced via fission are one reliable signature of the presence of SNM and are usually identified by their unique timing characteristics, such as the delayed neutron die-away. Fast neutron spectroscopy may provide additional useful discriminating characteristics for SNM detection. Spectroscopic measurements can be conducted by recoil-based or thermalization and capture-gated detectors; the latter may offer unique advantages since they facilitate low-statistics and event-by-event neutron energy measurements without spectrum unfolding. We describe the results of the development and characterization of a new type of capture-gated spectroscopic neutron detector based on a composite of scintillating polyvinyltoluene and lithium-doped scintillating glass in the form of millimeter-thick rods. The detector achieves >108 neutron-gamma discrimination resulting from its geometric properties and material selection. The design facilitates simultaneous pulse shape and pulse height discrimination, despite the fact that no materials intrinsically capable of pulse shape discrimination have been used to construct the detector. Accurate single-event measurements of neutron energy may be possible even when the energy is relatively low, such as with delayed fission neutrons. Simulation and preliminary measurements using the new composite detector are described, including those conducted using radioisotope sources and the low-dose active interrogation system based on low-energy nuclear reactions.

High-efficiency scintillation detector for combined detection of thermal and fast neutrons and gamma radiation

DOEpatents

Chiles, M.M.; Mihalczo, J.T.; Blakeman, E.D.

1987-02-27

A scintillation based radiation detector for the combined detection of thermal neutrons, high-energy neutrons and gamma rays in a single detecting unit. The detector consists of a pair of scintillators sandwiched together and optically coupled to the light sensitive face of a photomultiplier tube. A light tight radiation pervious housing is disposed about the scintillators and a portion of the photomultiplier tube to hold the arrangement in assembly and provides a radiation window adjacent the outer scintillator through which the radiation to be detected enters the detector. The outer scintillator is formed of a material in which scintillations are produced by thermal-neutrons and the inner scintillator is formed of a material in which scintillations are produced by high-energy neutrons and gamma rays. The light pulses produced by events detected in both scintillators are coupled to the photomultiplier tube which produces a current pulse in response to each detected event. These current pulses may be processed in a conventional manner to produce a count rate output indicative of the total detected radiation event count rate. Pulse discrimination techniques may be used to distinguish the different radiations and their energy distribution.

High-efficiency scintillation detector for combined of thermal and fast neutrons and gamma radiation

DOEpatents

Chiles, Marion M.; Mihalczo, John T.; Blakeman, Edward D.

1989-02-07

A scintillation based radiation detector for the combined detection of thermal neutrons, high-energy neutrons and gamma rays in a single detecting unit. The detector consists of a pair of scintillators sandwiched together and optically coupled to the light sensitive face of a photomultiplier tube. A light tight radiation pervious housing is disposed about the scintillators and a portion of the photomultiplier tube to hold the arrangement in assembly and provides a radiation window adjacent the outer scintillator through which the radiation to be detected enters the detector. The outer scintillator is formed of a material in which scintillations are produced by thermal-neutrons and the inner scintillator is formed of a material in which scintillations are produced by high-energy neutrons and gamma rays. The light pulses produced by events detected in both scintillators are coupled to the photomultiplier tube which produces a current pulse in response to each detected event. These current pulses may be processed in a conventional manner to produce a count rate output indicative of the total detected radiation even count rate. Pulse discrimination techniques may be used to distinguish the different radiations and their energy distribution.

High-efficiency scintillation detector for combined of thermal and fast neutrons and gamma radiation

DOEpatents

Chiles, Marion M.; Mihalczo, John T.; Blakeman, Edward D.

1989-01-01

A scintillation based radiation detector for the combined detection of thermal neutrons, high-energy neutrons and gamma rays in a single detecting unit. The detector consists of a pair of scintillators sandwiched together and optically coupled to the light sensitive face of a photomultiplier tube. A light tight radiation pervious housing is disposed about the scintillators and a portion of the photomultiplier tube to hold the arrangement in assembly and provides a radiation window adjacent the outer scintillator through which the radiation to be detected enters the detector. The outer scintillator is formed of a material in which scintillations are produced by thermal-neutrons and the inner scintillator is formed of a material in which scintillations are produced by high-energy neutrons and gamma rays. The light pulses produced by events detected in both scintillators are coupled to the photomultiplier tube which produces a current pulse in response to each detected event. These current pulses may be processed in a conventional manner to produce a count rate output indicative of the total detected radiation even count rate. Pulse discrimination techniques may be used to distinguish the different radiations and their energy distribution.

Neutron assay in mixed radiation fields with a 6Li-loaded plastic scintillator

NASA Astrophysics Data System (ADS)

Balmer, M. J. I.; Gamage, K. A. A.; Taylor, G. C.

2015-08-01

A novel technique for assay of thermal and fast neutrons in a 6Li-loaded plastic scintillator is presented. Existing capture-gated thermal neutron detection techniques were evaluated with the 6Li-loaded plastic scintillator studied in this work. Using simulations and experimental work, shortcomings in its performance were highlighted. As a result, it was proposed that by separating the combined fast and thermal neutron events from gamma events, using established pulse shape discrimination techniques, the thermal neutron events could then be assayed. Experiments were conducted at the National Physical Laboratory, Teddington, performing neutron assays with seven different neutron fields using the proposed technique. For each field, thermal and fast neutron content was estimated and were shown to corroborate with the seven synthesised fields.

Improved lithium iodide neutron scintillator with Eu 2+ activation: The elimination of Suzuki-Phase precipitates

DOE PAGES

Boatner, Lynn A.; Comer, Eleanor P.; Wright, Gomez W.; ...

2017-02-21

Monovalent alkali halides such as NaI, CsI, and LiI are widely used as inorganic scintillators for radiation detection due to their light yield, the capability for the growth of large single crystals, relatively low cost, and other favorable characteristics. These materials are frequently activated through the addition of small amounts (e.g., a few hundred ppm) of elements such as thallium - or sodium in the case of CsI. The monovalent alkali halide scintillators can also be activated with low concentrations of Eu 2+, however Eu activation has previously not been widely employed due to the non-uniform segregation of the divalentmore » Eu dopant that leads to the formation of unwanted phases during Bridgman or other solidification crystal-growth methods. Specifically, for Eu concentrations near and above ~0.5%, Suzuki Phase precipitates form in the course of the melt-growth process, and these Suzuki Phase particles scatter the scintillation light. This adversely affects the scintillator performance via reduction in the optical transmission of the material, and depending on the crystal thickness and precipitated-particle concentration, this reduction can occur up to the point of opacity. Here we describe a post-growth process for the removal of Suzuki Phase precipitates from single crystals of the neutron scintillator LiI activated with Eu 2+ at concentrations up to and in excess of 3 wt.%, and we correlate the resulting neutron-detection performance with the thermal processing methods used to remove the Suzuki Phase particles. Furthermore, the resulting improved scintillator properties using increased Eu activator levels are applicable to neutron imaging and active interrogation systems, and pulse-height gamma-ray spectroscopy rather than pulse-shape discrimination can be used to discriminate between gamma ray and neutron interaction events.« less

Measurement of Scintillation and Ionization Yield and Scintillation Pulse Shape from Nuclear Recoils in Liquid Argon

DOE PAGES

Cao, H.

2015-05-26

We have measured the scintillation and ionization yield of recoiling nuclei in liquid argon as a function of applied electric field by exposing a dual-phase liquid argon time projection chamber (LAr-TPC) to a low energy pulsed narrow band neutron beam produced at the Notre Dame Institute for Structure and Nuclear Astrophysics. Liquid scintillation counters were arranged to detect and identify neutrons scattered in the TPC and to select the energy of the recoiling nuclei. We also report measurements of the scintillation yields for nuclear recoils with energies from 10.3 to 57.3 keV and for median applied electric fields from 0more » to 970 V/cm. For the ionization yields, we report measurements from 16.9 to 57.3 keV and for electric fields from 96.4 to 486 V/cm. Furthermore, we report the observation of an anticorrelation between scintillation and ionization from nuclear recoils, which is similar to the anticorrelation between scintillation and ionization from electron recoils. Assuming that the energy loss partitions into excitons and ion pairs from 83mKr internal conversion electrons is comparable to that from 207Bi conversion electrons, we obtained the numbers of excitons (N ex) and ion pairs (N i) and their ratio (N ex/N i) produced by nuclear recoils from 16.9 to 57.3 keV. Motivated by arguments suggesting direction sensitivity in LAr-TPC signals due to columnar recombination, a comparison of the light and charge yield of recoils parallel and perpendicular to the applied electric field is presented for the first time.« less

Improved lithium iodide neutron scintillator with Eu2+ activation: The elimination of Suzuki-Phase precipitates

NASA Astrophysics Data System (ADS)

Boatner, L. A.; Comer, E. P.; Wright, G. W.; Ramey, J. O.; Riedel, R. A.; Jellison, G. E.; Kolopus, J. A.

2017-05-01

Monovalent alkali halides such as NaI, CsI, and LiI are widely used as inorganic scintillators for radiation detection due to their light yield, the capability for the growth of large single crystals, relatively low cost, and other favorable characteristics. These materials are frequently activated through the addition of small amounts (e.g., a few hundred ppm) of elements such as thallium - or sodium in the case of CsI. The monovalent alkali halide scintillators can also be activated with low concentrations of Eu2+, however Eu activation has previously not been widely employed due to the non-uniform segregation of the divalent Eu dopant that leads to the formation of unwanted phases during Bridgman or other solidification crystal-growth methods. Specifically, for Eu concentrations near and above 0.5%, Suzuki Phase precipitates form in the course of the melt-growth process, and these Suzuki Phase particles scatter the scintillation light. This adversely affects the scintillator performance via reduction in the optical transmission of the material, and depending on the crystal thickness and precipitated-particle concentration, this reduction can occur up to the point of opacity. Here we describe a post-growth process for the removal of Suzuki Phase precipitates from single crystals of the neutron scintillator LiI activated with Eu2+ at concentrations up to and in excess of 3 wt%, and we correlate the resulting neutron-detection performance with the thermal processing methods used to remove the Suzuki Phase particles. The resulting improved scintillator properties using increased Eu activator levels are applicable to neutron imaging and active interrogation systems, and pulse-height gamma-ray spectroscopy rather than pulse-shape discrimination can be used to discriminate between gamma ray and neutron interaction events.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Osovizky, A.; Rotem Industries Ltd, Rotem Industrial Park; University of Maryland, College park, Maryland

A Chromatic Analysis Neutron Diffractometer Or Reflectometer (CANDOR) is under development at the NIST Center for Neutron Research (NCNR). The CANDOR neutron sensor will rely on scintillator material for detecting the neutrons scattered by the sample under test. It consists of {sup 6}LiF:ZnS(Ag) scintillator material into which wavelength shifting (WLS) fibers have been embedded. Solid state photo-sensors (silicon photomultipliers) coupled to the WLS fibers are used to detect the light produced by the neutron capture event ({sup 6}Li (n,α) {sup 3}H reaction) and ionization of the ZnS(Ag). This detector configuration has the potential to accomplish the CANDOR performance requirements formore » efficiency of 90% for 5 A (3.35 meV) neutrons with high gamma rejection (10{sup 7}) along with compact design, affordable cost and materials availability. However this novel design includes challenges for precise neutron detection. The recognizing of the neutron signature versus the noise event produce by gamma event cannot be easy overcome by pulse height discrimination obstacle as can be achieved with {sup 3}He gas tube. Furthermore the selection of silicon photomultipliers (SiPM) as the light sensor maintains the obstacle of dark noise that does not exist when a photomultiplier tube is coupled to the scintillator. A proper selection of SiPM should focus on increasing the output signal and reducing the dark noise in order to optimize the detection sensitivity and to provide a clean signal pulse shape discrimination. The main parameters for evaluation are: - Quantum Efficiency (QE) - matching the SiPM peak QE with the peak transmission wavelength emission of the WLS. - Recovery time - a short recovery time is preferred to minimize the pulse width beyond the intrinsic decay time of the scintillator crystal (improves the gamma rejection based output pulse shape (time)). - Diode dimensions -The dark noise is proportional to the diode active area while the signal is provided by the WLS fibers; therefore the diode area should ideally be only minimally larger than fiber bundle area. - Low dark noise - it is desirable to minimize the dark noise during the pulse integration period so as to minimize the background for pulse shape discrimination. - Photon Detection Efficiency - it is desirable to increase the SiPM PDE in order to enhance light collection. This will increase the likelihood of detecting neutron events with lower light production and will present a cleaner raw signal for pulse shape discrimination. We will present the SiPM optimization process and studies of dark noise and gamma and neutron sensitivity as a function of bias voltage and operating temperature that have enabled us to optimize the detector sensitivity and gamma rejection. The gamma rejection performance goal requires to overcome the challenge of discriminating between the light signature accepted by neutron event to the one received by the noise. In addition there is a huge variation between the number of light photons that reaching the WLS fibers for different neutron events caused by the heavy ions energy losses prior to ionizing the ZnS(Ag) and the high light attenuation of the scintillation mixture. This variation in the light signal along with the long decay time of the ZnS(Ag) (tens of microseconds) can cause double counting of the same neutron event in the case of high light output signature or preventing the detection of low sequential light output signature neutron event. We will presents the algorithm developed for {sup 6}LiF:ZnS(Ag) sensor readout and the results achieved by an off-line analysis by Matlab software code that successfully achieved both the high gamma rejection with a sensitive and accurate neutron event detection. (authors)« less

Pulse-Shape Analysis of Neutron-Induced Scintillation Light in Ni-doped 6LiF/ZnS

DOE Office of Scientific and Technical Information (OSTI.GOV)

Cowles, Christian C.; Behling, Richard S.; Imel, G. R.

Abstract–Alternatives to 3He are being investigated for gamma-ray insensitive neutron detection applications, including plutonium assay. One promising material is lithium-6 fluoride with silver activated zinc sulfide 6LiF/ZnS(Ag) in conjunction with a wavelength shifting plastic. Doping the 6LiF/ZnS(Ag) with nickel (Ni) has been proposed as a means of reducing the decay time of neutron signal pulses. This research performed a pulse shape comparison between Ni-doped and non-doped 6LiF/ZnS(Ag) neutron pulses. The Ni-doped 6LiF/ZnS(Ag) had a 32.7% ± 0.3 increase in neutron pulse height and a 32.4% ± 0.3 decrease in neutron pulse time compared to the non-doped 6LiF/ZnS(Ag). Doping 6LiF/ZnS(Ag) withmore » nickel may allow neutron detector operation with improved signal to noise ratios, and reduced pulse pileup affects, increasing the accuracy and range of source activities with which such a detector could operate.« less

Scintillation efficiency measurement of Na recoils in NaI(Tl) below the DAMA/LIBRA energy threshold

NASA Astrophysics Data System (ADS)

Xu, Jingke; Shields, Emily; Calaprice, Frank; Westerdale, Shawn; Froborg, Francis; Suerfu, Burkhant; Alexander, Thomas; Aprahamian, Ani; Back, Henning O.; Casarella, Clark; Fang, Xiao; Gupta, Yogesh K.; Ianni, Aldo; Lamere, Edward; Lippincott, W. Hugh; Liu, Qian; Lyons, Stephanie; Siegl, Kevin; Smith, Mallory; Tan, Wanpeng; Kolk, Bryant Vande

2015-07-01

The dark matter interpretation of the DAMA modulation signal depends on the NaI(Tl) scintillation efficiency of nuclear recoils. Previous measurements for Na recoils have large discrepancies, especially in the DAMA/LIBRA modulation energy region. We report a quenching effect measurement of Na recoils in NaI(Tl) from 3 to 52 keVnr, covering the whole DAMA/LIBRA energy region for dark matter-Na scattering interpretations. By using a low-energy, pulsed neutron beam, a double time-of-flight technique, and pulse-shape discrimination methods, we obtained the most accurate measurement of this kind for NaI(Tl) to date. The results differ significantly from the DAMA reported values at low energies but fall between the other previous measurements. We present the implications of the new quenching results for the dark matter interpretation of the DAMA modulation signal.

Scintillation efficiency measurement of Na recoils in NaI(Tl) below the DAMA/LIBRA energy threshold

DOE Office of Scientific and Technical Information (OSTI.GOV)

Xu, Jingke; Shields, Emily; Calaprice, Frank

2015-07-01

The dark matter interpretation of the DAMA modulation signal depends on the NaI(Tl) scintillation efficiency of nuclear recoils. Previous measurements for Na recoils have large discrepancies, especially in the DAMA/LIBRA modulation energy region. We report a quenching effect measurement of Na recoils in NaI(Tl) from 3 to 52 keVnr, covering the whole DAMA/LIBRA energy region for dark matter-Na scattering interpretations. By using a low-energy, pulsed neutron beam, a double time-of-flight technique, and pulse-shape discrimination methods, we obtained the most accurate measurement of this kind for NaI(Tl) to date. The results differ significantly from the DAMA reported values at low energies butmore » fall between the other previous measurements. We present the implications of the new quenching results for the dark matter interpretation of the DAMA modulation signal.« less

A digital acquisition and elaboration system for nuclear fast pulse detection

NASA Astrophysics Data System (ADS)

Esposito, B.; Riva, M.; Marocco, D.; Kaschuck, Y.

2007-03-01

A new digital acquisition and elaboration system has been developed and assembled in ENEA-Frascati for the direct sampling of fast pulses from nuclear detectors such as scintillators and diamond detectors. The system is capable of performing the digital sampling of the pulses (200 MSamples/s, 14-bit) and the simultaneous (compressed) data transfer for further storage and software elaboration. The design (FPGA-based) is oriented to real-time applications and has been developed in order to allow acquisition with no loss of pulses and data storage for long-time intervals (tens of s at MHz pulse count rates) without the need of large on-board memory. A dedicated pulse analysis software, written in LabVIEWTM, performs the treatment of the acquired pulses, including pulse recognition, pile-up rejection, baseline removal, pulse shape particle separation and pulse height spectra analysis. The acquisition and pre-elaboration programs have been fully integrated with the analysis software.

Pulse shape discrimination and classification methods for continuous depth of interaction encoding PET detectors.

PubMed

Roncali, Emilie; Phipps, Jennifer E; Marcu, Laura; Cherry, Simon R

2012-10-21

In previous work we demonstrated the potential of positron emission tomography (PET) detectors with depth-of-interaction (DOI) encoding capability based on phosphor-coated crystals. A DOI resolution of 8 mm full-width at half-maximum was obtained for 20 mm long scintillator crystals using a delayed charge integration linear regression method (DCI-LR). Phosphor-coated crystals modify the pulse shape to allow continuous DOI information determination, but the relationship between pulse shape and DOI is complex. We are therefore interested in developing a sensitive and robust method to estimate the DOI. Here, linear discriminant analysis (LDA) was implemented to classify the events based on information extracted from the pulse shape. Pulses were acquired with 2×2×20 mm(3) phosphor-coated crystals at five irradiation depths and characterized by their DCI values or Laguerre coefficients. These coefficients were obtained by expanding the pulses on a Laguerre basis set and constituted a unique signature for each pulse. The DOI of individual events was predicted using LDA based on Laguerre coefficients (Laguerre-LDA) or DCI values (DCI-LDA) as discriminant features. Predicted DOIs were compared to true irradiation depths. Laguerre-LDA showed higher sensitivity and accuracy than DCI-LDA and DCI-LR and was also more robust to predict the DOI of pulses with higher statistical noise due to low light levels (interaction depths further from the photodetector face). This indicates that Laguerre-LDA may be more suitable to DOI estimation in smaller crystals where lower collected light levels are expected. This novel approach is promising for calculating DOI using pulse shape discrimination in single-ended readout depth-encoding PET detectors.

Pulse Shape Discrimination and Classification Methods for Continuous Depth of Interaction Encoding PET Detectors

PubMed Central

Roncali, Emilie; Phipps, Jennifer E.; Marcu, Laura; Cherry, Simon R.

2012-01-01

In previous work we demonstrated the potential of positron emission tomography (PET) detectors with depth-of-interaction (DOI) encoding capability based on phosphor-coated crystals. A DOI resolution of 8 mm full-width at half-maximum was obtained for 20 mm long scintillator crystals using a delayed charge integration linear regression method (DCI-LR). Phosphor-coated crystals modify the pulse shape to allow continuous DOI information determination, but the relationship between pulse shape and DOI is complex. We are therefore interested in developing a sensitive and robust method to estimate the DOI. Here, linear discriminant analysis (LDA) was implemented to classify the events based on information extracted from the pulse shape. Pulses were acquired with 2 × 2 × 20 mm3 phosphor-coated crystals at five irradiation depths and characterized by their DCI values or Laguerre coefficients. These coefficients were obtained by expanding the pulses on a Laguerre basis set and constituted a unique signature for each pulse. The DOI of individual events was predicted using LDA based on Laguerre coefficients (Laguerre-LDA) or DCI values (DCI-LDA) as discriminant features. Predicted DOIs were compared to true irradiation depths. Laguerre-LDA showed higher sensitivity and accuracy than DCI-LDA and DCI-LR and was also more robust to predict the DOI of pulses with higher statistical noise due to low light levels (interaction depths further from the photodetector face). This indicates that Laguerre-LDA may be more suitable to DOI estimation in smaller crystals where lower collected light levels are expected. This novel approach is promising for calculating DOI using pulse shape discrimination in single-ended readout depth-encoding PET detectors. PMID:23010690

Fast neutron flux analyzer with real-time digital pulse shape discrimination

NASA Astrophysics Data System (ADS)

Ivanova, A. A.; Zubarev, P. V.; Ivanenko, S. V.; Khilchenko, A. D.; Kotelnikov, A. I.; Polosatkin, S. V.; Puryga, E. A.; Shvyrev, V. G.; Sulyaev, Yu. S.

2016-08-01

Investigation of subthermonuclear plasma confinement and heating in magnetic fusion devices such as GOL-3 and GDT at the Budker Institute (Novosibirsk, Russia) requires sophisticated equipment for neutron-, gamma- diagnostics and upgrading data acquisition systems with online data processing. Measurement of fast neutron flux with stilbene scintillation detectors raised the problem of discrimination of the neutrons (n) from background cosmic particles (muons) and neutron-induced gamma rays (γ). This paper describes a fast neutron flux analyzer with real-time digital pulse-shape discrimination (DPSD) algorithm FPGA-implemented for the GOL-3 and GDT devices. This analyzer was tested and calibrated with the help of 137Cs and 252Cf radiation sources. The Figures of Merit (FOM) calculated for different energy cuts are presented.

Digital pulse shape discrimination.

PubMed

Miller, L F; Preston, J; Pozzi, S; Flaska, M; Neal, J

2007-01-01

Pulse-shape discrimination (PSD) has been utilised for about 40 years as a method to obtain estimates for dose in mixed neutron and photon fields. Digitizers that operate close to GHz are currently available at a reasonable cost, and they can be used to directly sample signals from photomultiplier tubes. This permits one to perform digital PSD rather than the traditional, and well-established, analogoue techniques. One issue that complicates PSD for neutrons in mixed fields is that the light output characteristics of typical scintillators available for PSD, such as BC501A, vary as a function of energy deposited in the detector. This behaviour is more easily accommodated with digital processing of signals than with analogoue signal processing. Results illustrate the effectiveness of digital PSD.

Methacrylate based cross-linkers for improved thermomechanical properties and retention of radiation detection response in plastic scintillators

NASA Astrophysics Data System (ADS)

Mahl, Adam; Lim, Allison; Latta, Joseph; Yemam, Henok A.; Greife, Uwe; Sellinger, Alan

2018-03-01

Pulse shape discrimination (PSD) is an important method that can efficiently sort and separate neutron and gamma radiation signals. PSD is currently achieved in plastic scintillators by over-doping poly(vinyl toluene) (PVT) matrices with fluorescent molecules. Meaningful separation of the signals requires addition of >20 wt% 2,5-diphenyloxazole (PPO) fluor in PVT. At these concentrations PPO acts as a plasticizer, negatively affecting the physical properties of the final plastic such as hardness, machinability, and thermomechanical stability. This work addresses these issues by implementing a cost-effective solution using cross-linking chemistry via commercially available bisphenol A dimethacrylate (BPA-DM), and a synthesized fluorinated analogue. Both improve the physical properties of over-doped PPO based plastic scintillators without degrading the measured light yield or PSD and Figure of Merit (FoM). In addition, the fluorinated analogue appears to enhance the hydrophobicity of the surface of the plastic scintillators, which may improve the scintillators' resistance to water diffusion and subsequent radiation response degradation. The new formulations improve the feasibility of widely deploying long lifetime PSD capable plastic scintillators in large area coverage assemblies.

Development of a flexible γ-ray detector using a liquid scintillation light guide (LSLG).

PubMed

Nomura, Kiyoshi; Yunoki, Akira; Hara, Masayuki; Morito, Yuko; Fujishima, Akira

2018-04-10

A flexible γ detector using a liquid scintillation light guide (LSLG) was developed. The analyzed pulse height (PHA) spectrum depended on the diameter, length and scintillator concentration of the LSLG, and the distance of a γ ray irradiation point from the head of photomultiplier tube (PMT). From the analysis of PHA spectrum, it was found that the count ratio of two divided channel regions linearly decreases as the distance from the PMT head increases. It was further found that the radiation dose rate can be estimated by setting the flexible LSLG tube to a circular shape since the count rate is proportional to the dose rate measured by a conventional NaI (Tl) scintillation detector. Therefore, a flexible and long LSLG detector using a single PMT is useful for determination of the dose rate and has a potential to detect local contaminations in a certain narrow space. Copyright © 2018. Published by Elsevier Ltd.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Andrews, Madison Theresa; Bates, Cameron Russell; Mckigney, Edward Allen

Here, this work presents the organic scintillation simulation capabilities of DRiFT, a post-processing Detector Response Function Toolkit for MCNPR output. DRiFT is used to create realistic scintillation detector response functions to incident neutron and gamma mixed- field radiation. As a post-processing tool, DRiFT leverages the extensively validated radiation transport capabilities of MCNPR ®6, which also provides the ability to simulate complex sources and geometries. DRiFT is designed to be flexible, it allows the user to specify scintillator material, PMT type, applied PMT voltage, and quenching data used in simulations. The toolkit's capabilities, which include the generation of pulse shape discriminationmore » plots and full-energy detector spectra, are demonstrated in a comparison of measured and simulated neutron contributions from 252Cf and PuBe, and photon spectra from 22Na and 228Th sources. DRiFT reproduced energy resolution effects observed in EJ-301 measurements through the inclusion of scintillation yield variances, photon transport noise, and PMT photocathode and multiplication noise.« less

Systematic studies of small scintillators for new sampling calorimeter

NASA Astrophysics Data System (ADS)

Jacosalem, E. P.; Iba, S.; Nakajima, N.; Ono, H.; Sanchez, A. L. C.; Bacala, A. M.; Miyata, H.

2007-12-01

A new sampling calorimeter using very thin scintillators and the multi-pixel photon counter (MPPC) has been proposed to produce better position resolution for the international linear collider (ILC) experiment. As part of this R&D study, small plastic scintillators of different sizes, thickness and wrapping reflectors are systematically studied. The scintillation light due to beta rays from a collimated ^{90}Sr source are collected from the scintillator by wavelength-shifting (WLS) fiber and converted into electrical signals at the PMT. The wrapped scintillator that gives the best light yield is determined by comparing the measured pulse height of each 10 × 40 × 2 mm strip scintillator covered with 3M reflective mirror film, teflon, white paint, black tape, gold, aluminum and white paint+teflon. The pulse height dependence on position, length and thickness of the 3M reflective mirror film and teflon wrapped scintillators are measured. Results show that the 3M radiant mirror film-wrapped scintillator has the greatest light yield with an average of 9.2 photoelectrons. It is observed that light yield slightly increases with scintillator length, but increases to about 100% when WLS fiber diameter is increased from 1.0 mm to 1.6 mm. The position dependence measurement along the strip scintillator showed the uniformity of light transmission from the sensor to the PMT. A dip across the strip is observed which is 40% of the maximum pulse height. The block type scintillator pulse height, on the other hand, is found to be almost proportional to scintillator thickness.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Lombigit, L., E-mail: lojius@nm.gov.my; Yussup, N., E-mail: nolida@nm.gov.my; Ibrahim, Maslina Mohd

A digital n/γ pulse shape discrimination (PSD) system is currently under development at Instrumentation and Automation Centre, Malaysian Nuclear Agency. This system aims at simultaneous detection of fast neutron and gamma ray in mixed radiations environment. This work reports the system characterization performed on the liquid scintillation detector (BC-501A) and digital pulse shape discrimination (DPSD) system. The characterization involves measurement of electron light output from the BC-501A detector and energy channels calibration of the pulse height spectra acquired with DPSD system using set of photon reference sources. The main goal of this experiment is to calibrate the ADC channel ofmore » our DPSD system, characterized the BC-501 detector and find the position of Compton edge which later could be used as threshold for the n/γ PSD experiment. The detector resolution however is worse as compared to other published data but it is expected as our detector has a smaller active volume.« less

DOE Office of Scientific and Technical Information (OSTI.GOV)

Boatner, Lynn A.; Comer, Eleanor P.; Wright, Gomez W.

Monovalent alkali halides such as NaI, CsI, and LiI are widely used as inorganic scintillators for radiation detection due to their light yield, the capability for the growth of large single crystals, relatively low cost, and other favorable characteristics. These materials are frequently activated through the addition of small amounts (e.g., a few hundred ppm) of elements such as thallium - or sodium in the case of CsI. The monovalent alkali halide scintillators can also be activated with low concentrations of Eu 2+, however Eu activation has previously not been widely employed due to the non-uniform segregation of the divalentmore » Eu dopant that leads to the formation of unwanted phases during Bridgman or other solidification crystal-growth methods. Specifically, for Eu concentrations near and above ~0.5%, Suzuki Phase precipitates form in the course of the melt-growth process, and these Suzuki Phase particles scatter the scintillation light. This adversely affects the scintillator performance via reduction in the optical transmission of the material, and depending on the crystal thickness and precipitated-particle concentration, this reduction can occur up to the point of opacity. Here we describe a post-growth process for the removal of Suzuki Phase precipitates from single crystals of the neutron scintillator LiI activated with Eu 2+ at concentrations up to and in excess of 3 wt.%, and we correlate the resulting neutron-detection performance with the thermal processing methods used to remove the Suzuki Phase particles. Furthermore, the resulting improved scintillator properties using increased Eu activator levels are applicable to neutron imaging and active interrogation systems, and pulse-height gamma-ray spectroscopy rather than pulse-shape discrimination can be used to discriminate between gamma ray and neutron interaction events.« less

Development of New High Resolution Neutron Detector

NASA Astrophysics Data System (ADS)

Mostella, L. D., III; Rajabali, M.; Loureiro, D. P.; Grzywacz, R.

2017-09-01

Beta-delayed neutron emission is a prevalent form of decay for neutron-rich nuclei. This occurs when an unstable nucleus undergoes beta decay, but produces a daughter nucleus in an excited state above the neutron separation energy. The daughter nucleus then de-excites by ejecting one or more neutrons. We wish to map the states from which these nuclei decay via neutron spectroscopy using NEXT, a new high resolution neutron detector. NEXT utilizes silicon photomultipliers and 6 mm thick pulse-shape discriminating plastic scintillators, allowing for smaller and more compact modular geometries in the NEXT array. Timing measurements for the detector were performed and a resolution of 893 ps (FWHM) has been achieved so far. Aspects of the detector that were investigated and will be presented here include scintillator geometry, wrapping materials, fitting functions for the digitized signals, and electronic components coupled to the silicon photomultipliers for signal shaping.

A triple-crystal phoswich detector with digital pulse shape discrimination for alpha/beta/gamma spectroscopy

NASA Astrophysics Data System (ADS)

White, Travis L.; Miller, William H.

1999-02-01

Researchers at the University of Missouri - Columbia have developed a three-crystal phoswich detector coupled to a digital pulse shape discrimination system for use in alpha/beta/gamma spectroscopy. Phoswich detectors use a sandwich of scintillators viewed by a single photomultiplier tube to simultaneously detect multiple types of radiation. Separation of radiation types is based upon pulse shape difference among the phosphors, which has historically been performed with analog circuitry. The system uses a GaGe CompuScope 1012, 12 bit, 10 MHz computer-based oscilloscope that digitally captures the pulses from a phoswich detector and subsequently performs pulse shape discrimination with cross-correlation analysis. The detector, based partially on previous phoswich designs by Usuda et al., uses a 10 mg/cm 2 thick layer of ZnS(Ag) for alpha detection, followed by a 0.254 cm CaF 2(Eu) crystal for beta detection, all backed by a 2.54 cm NaI(Tl) crystal for gamma detection. Individual energy spectra and count rate information for all three radiation types are displayed and updated periodically. The system shows excellent charged particle discrimination with an accuracy of greater than 99%. Future development will include a large area beta probe with gamma-ray discrimination, systems for low-energy photon detection (e.g. Bremsstrahlung or keV-range photon emissions), and other health physics instrumentation.

The impact of photon flight path on S1 pulse shape analysis in liquid xenon two-phase detectors

NASA Astrophysics Data System (ADS)

Moongweluwan, M.

2016-02-01

The LUX dark matter search experiment is a 350 kg dual-phase xenon time projection chamber located at the 4850 ft level of the Sanford Underground Research Facility in Lead, SD. The success of two-phase xenon detectors for dark matter searches relies on their ability to distinguish electron recoil (ER) background events from nuclear recoil (NR) signal events. Typically, the NR-ER discrimination is obtained from the ratio of the electroluminescence light (S2) to the prompt scintillation light (S1). Analysis of the S1 pulse shape is an additional discrimination technique that can be used to distinguish NR from ER. Pulse-shape NR-ER discrimination can be achieved based on the ratio of the de-excitation processes from singlet and triplet states that generate the S1. The NR S1 is dominated by the de-excitation process from singlet states with a time constant of about 3 ns while the ER S1 is dominated by the de-excitation process from triplet states with a time constant of about 24 ns. As the size of the detectors increases, the variation in the S1 photon flight path can become comparable to these decay constants, reducing the utility of pulse-shape analysis to separate NR from ER. The effect of path length variations in the LUX detector has been studied using the results of simulations and the impact on the S1 pulse shape analysis is discussed.

A new scalable modular data acquisition system for SPECT (PET)

NASA Astrophysics Data System (ADS)

Stenstrom, P.; Rillbert, A.; Bergquist, M.; Habte, F.; Bohm, C.; Larsson, S. A.

1998-06-01

Describes a modular decentralized data acquisition system that continuously samples shaped PMT pulses from a SPECT detector. The pulse waveform data are used by signal processors to accurately reconstruct amplitude and time for each scintillation event. Data acquisition for a PMT channel is triggered in two alternative ways, either when its own signal exceeds a selected digital threshold, or when it receives a trigger pulse from one of its neighboring PMTs. The triggered region is restricted to seven, thirteen or nineteen neighboring PMT channels. Each acquisition module supports three PMT channels and connects to all other modules and a reconstruction computer via Firewire to cover the 72 channels in the Stockholm University/Karolinska Hospital cylindrical SPECT camera.

Fission-neutrons source with fast neutron-emission timing

NASA Astrophysics Data System (ADS)

Rusev, G.; Baramsai, B.; Bond, E. M.; Jandel, M.

2016-05-01

A neutron source with fast timing has been built to help with detector-response measurements. The source is based on the neutron emission from the spontaneous fission of 252Cf. The time is provided by registering the fission fragments in a layer of a thin scintillation film with a signal rise time of 1 ns. The scintillation light output is measured by two silicon photomultipliers with rise time of 0.5 ns. Overall time resolution of the source is 0.3 ns. Design of the source and test measurements using it are described. An example application of the source for determining the neutron/gamma pulse-shape discrimination by a stilbene crystal is given.

Scintillation properties of Gd3Al2Ga3O12:Ce3+ single crystal scintillators

NASA Astrophysics Data System (ADS)

Sakthong, Ongsa; Chewpraditkul, Weerapong; Wanarak, Chalerm; Kamada, Kei; Yoshikawa, Akira; Prusa, Petr; Nikl, Martin

2014-07-01

The scintillation properties of Gd3Al2Ga3O12:Ce3+ (GAGG:Ce) single crystals grown by the Czochralski method with 1 at% cerium in the melt were investigated and results were compared with so far published results in the literature. The light yield (LY) and energy resolution were measured using a XP5200B photomultiplier. Despite about twice higher LY for GAGG:Ce, the energy resolution is only slightly better than that of LuAG:Ce due to its worse intrinsic resolution and non-proportionality of LY. The LY dependences on the sample thickness and amplifier shaping time were measured. The estimated photofraction in pulse height spectra of 320 and 662 keV γ-rays and the total mass attenuation coefficient at 662 keV γ-rays were also determined and compared with the theoretical ones calculated using the WinXCom program.

Handheld readout electronics to fully exploit the particle discrimination capabilities of elpasolite scintillators

DOE PAGES

Budden, B. S.; Stonehill, L. C.; Warniment, A.; ...

2015-06-10

In this study, a new class of elpasolite scintillators has garnered recent attention due to the ability to perform as simultaneous gamma spectrometers and thermal neutron detectors. Such a dual-mode capability is made possible by pulse-shape discrimination (PSD), whereby the emission waveform profiles of gamma and neutron events are fundamentally unique. To take full advantage of these materials, we have developed the Compact Advanced Readout Electronics for Elpasolites (CAREE). This handheld instrument employs a multi-channel PSD-capable ASIC, custom micro-processor board, front-end electronics, power supplies, and a 2 in. photomultiplier tube for readout of the scintillator. The unit is highly configurablemore » to allow for performance optimization amongst a wide sample of elpasolites which provide PSD in fundamentally different ways. We herein provide an introduction to elpasolites, then describe the motivation for the work, mechanical and electronic design, and preliminary performance results.« less

Handheld readout electronics to fully exploit the particle discrimination capabilities of elpasolite scintillators

NASA Astrophysics Data System (ADS)

Budden, B. S.; Stonehill, L. C.; Warniment, A.; Michel, J.; Storms, S.; Dallmann, N.; Coupland, D. D. S.; Stein, P.; Weller, S.; Borges, L.; Proicou, M.; Duran, G.; Kamto, J.

2015-09-01

A new class of elpasolite scintillators has garnered recent attention due to the ability to perform as simultaneous gamma spectrometers and thermal neutron detectors. Such a dual-mode capability is made possible by pulse-shape discrimination (PSD), whereby the emission waveform profiles of gamma and neutron events are fundamentally unique. To take full advantage of these materials, we have developed the Compact Advanced Readout Electronics for Elpasolites (CAREE). This handheld instrument employs a multi-channel PSD-capable ASIC, custom micro-processor board, front-end electronics, power supplies, and a 2 in. photomultiplier tube for readout of the scintillator. The unit is highly configurable to allow for performance optimization amongst a wide sample of elpasolites which provide PSD in fundamentally different ways. We herein provide an introduction to elpasolites, then describe the motivation for the work, mechanical and electronic design, and preliminary performance results.

Synthesis of plastic scintillation microspheres: alpha/beta discrimination.

PubMed

Santiago, L M; Bagán, H; Tarancón, A; Garcia, J F

2014-11-01

Plastic scintillation microspheres (PSm) have been developed as an alternative for liquid scintillation cocktails due to their ability to avoid the mixed waste, besides other strengths in which the possibility for alpha/beta discrimination is included. The aim of this work was to evaluate the capability of PSm containing two combinations of fluorescence solutes (PPO/POPOP and pT/Bis-MSB) and variable amounts of a second organic solvent (naphthalene) to enhance the alpha/beta discrimination. Two commercial detectors with different Pulse Shape Discrimination performances (Quantulus and Triathler) were used to evaluate the alpha/beta discrimination. An optimal discrimination of alpha/beta particles was reached, with very low misclassification values (2% for beta particles and 0.5% for alpha particles), when PSm containing PPO/POPOP and between 0.6 and 2.0 g of naphthalene were evaluated using Triathler and the appropriate programme for data processing. Copyright © 2014 Elsevier Ltd. All rights reserved.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Mesick, Katherine Elizabeth; Coupland, Daniel David S.; Stonehill, Laura Catherine

Cs 2LiLaBr 6:Ce 3+ (CLLB) is an elpasolite scintillator that offers excellent linearity and gamma-ray energy resolution and sensitivity to thermal neutrons with the ability to perform pulse-shape discrimination (PSD) to distinguish gammas and neutrons. Our investigation of CLLB has indicated the presence of intrinsic radioactive alpha background that we have determined to be from actinium contamination of the lanthanum component. We measured the pulse shapes for gamma, thermal neutron, and alpha events and determined that PSD can be performed to separate the alpha background with a moderate figure of merit of 0.98. Here, we also measured the electron-equivalent-energy ofmore » the alpha particles in CLLB and simulated the intrinsic alpha background from 227Ac to determine the quenching factor of the alphas.« less

DOE Office of Scientific and Technical Information (OSTI.GOV)

Cherepy, Nerine J.; Sanner, Robert D.; Beck, Patrick R.

In this paper, transparent plastic scintillators based on polyvinyltoluene (PVT) have been fabricated with high loading of bismuth carboxylates for gamma spectroscopy, and with lithium carboxylates for neutron detection. When activated with a combination of standard fluors, 2,5-diphenyloxazole (PPO) and tetraphenylbutadiene (TPB), gamma light yields with 15 wt% bismuth tripivalate of 5000 Ph/MeV are measured. A PVT plastic formulation including 30 wt% lithium pivalate and 30 wt% PPO offers both pulse shape discrimination, and a neutron capture peak at ~400 keVee. Finally, in another configuration, a bismuth-loaded PVT plastic is coated with ZnS( 6Li) paint, permitting simultaneous gamma and neutronmore » detection via pulse shape discrimination with a figure-of-merit of 3.8, while offering gamma spectroscopy with energy resolution of R(662 keV)=15%.« less

Fast neutron-gamma discrimination on neutron emission profile measurement on JT-60U.

PubMed

Ishii, K; Shinohara, K; Ishikawa, M; Baba, M; Isobe, M; Okamoto, A; Kitajima, S; Sasao, M

2010-10-01

A digital signal processing (DSP) system is applied to stilbene scintillation detectors of the multichannel neutron emission profile monitor in JT-60U. Automatic analysis of the neutron-γ pulse shape discrimination is a key issue to diminish the processing time in the DSP system, and it has been applied using the two-dimensional (2D) map. Linear discriminant function is used to determine the dividing line between neutron events and γ-ray events on a 2D map. In order to verify the validity of the dividing line determination, the pulse shape discrimination quality is evaluated. As a result, the γ-ray contamination in most of the beam heating phase was negligible compared with the statistical error with 10 ms time resolution.

Fast neutron-gamma discrimination on neutron emission profile measurement on JT-60U

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ishii, K.; Okamoto, A.; Kitajima, S.

2010-10-15

A digital signal processing (DSP) system is applied to stilbene scintillation detectors of the multichannel neutron emission profile monitor in JT-60U. Automatic analysis of the neutron-{gamma} pulse shape discrimination is a key issue to diminish the processing time in the DSP system, and it has been applied using the two-dimensional (2D) map. Linear discriminant function is used to determine the dividing line between neutron events and {gamma}-ray events on a 2D map. In order to verify the validity of the dividing line determination, the pulse shape discrimination quality is evaluated. As a result, the {gamma}-ray contamination in most of themore » beam heating phase was negligible compared with the statistical error with 10 ms time resolution.« less

Pulse-shape discrimination and energy quenching of alpha particles in Cs2LiLaBr6:Ce3+

NASA Astrophysics Data System (ADS)

Mesick, K. E.; Coupland, D. D. S.; Stonehill, L. C.

2017-01-01

Cs2LiLaBr6:Ce3+(CLLB) is an elpasolite scintillator that offers excellent linearity and gamma-ray energy resolution and sensitivity to thermal neutrons with the ability to perform pulse-shape discrimination (PSD) to distinguish gammas and neutrons. Our investigation of CLLB has indicated the presence of intrinsic radioactive alpha background that we have determined to be from actinium contamination of the lanthanum component. We measured the pulse shapes for gamma, thermal neutron, and alpha events and determined that PSD can be performed to separate the alpha background with a moderate figure of merit of 0.98. We also measured the electron-equivalent-energy of the alpha particles in CLLB and simulated the intrinsic alpha background from 227Ac to determine the quenching factor of the alphas. A linear quenching relationship Lα =Eα × q +L0 was found at alpha particle energies above 5 MeV, with a quenching factor q = 0.71 MeVee / MeV and an offset L0 = - 1.19 MeVee .

Laftr

NASA Astrophysics Data System (ADS)

Barghi, M. R., Sr.; Sample, J.; Forouzani, A.; Delaney, N.; Wells, E.; Parab, A.; Bowers, G. S.; Smith, D.; Martinez-McKinney, F.

2017-12-01

The Light and Fast TGF Recorder (LAFTR), is a joint institutional NASA balloon borne gamma-ray detector between undergraduates at Montana State University(MSU) and University of California Santa Cruz (UCSC) designed to record an extremely bright sub-millisecond burst of gamma-rays observed to originate inside thunderstorms called Terrestrial Gamma-ray Flashes (TGFs). The detector employs a fast small plastic scintillator(BC-408) to avoid oversaturation. The Scintillator output is read out by the SensL Silicon Photomultiplier (SiPm) complemented by a custom shaping circuit to narrow long exponential pulses outputted from the SiPm into a semi-gaussian pulse with a 40 ns FWHM to be read into a 6 channel discriminator board for coarse spectroscopy and output a Low Voltage Differential Signal(LVDS). The presentation will primarily focus on the significant experiences and skills acquired from the project by several team members such as the importance of team coordination in joint institutional projects,clear documentation, communication, and planning such detector systems under the NASA Guidelines.

Compensated gadolinium-loaded plastic scintillators for thermal neutron detection (and counting)

DOE Office of Scientific and Technical Information (OSTI.GOV)

Dumazert, Jonathan; Coulon, Romain; Bertrand, Guillaume H. V.

2015-07-01

Plastic scintillator loading with gadolinium-rich organometallic complexes shows a high potential for the deployment of efficient and cost-effective neutron detectors. Due to the low-energy photon and electron signature of thermal neutron capture by gadolinium-155 and gadolinium-157, alternative treatment to Pulse Shape Discrimination has to be proposed in order to display a trustable count rate. This paper discloses the principle of a compensation method applied to a two-scintillator system: a detection scintillator interacts with photon radiation and is loaded with gadolinium organometallic compound to become a thermal neutron absorber, while a non-gadolinium loaded compensation scintillator solely interacts with the photon partmore » of the incident radiation. Posterior to the nonlinear smoothing of the counting signals, a hypothesis test determines whether the resulting count rate after photon response compensation falls into statistical fluctuations or provides a robust image of a neutron activity. A laboratory prototype is tested under both photon and neutron irradiations, allowing us to investigate the performance of the overall compensation system in terms of neutron detection, especially with regards to a commercial helium-3 counter. The study reveals satisfactory results in terms of sensitivity and orientates future investigation toward promising axes. (authors)« less

A rapid method for the simultaneous determination of gross alpha and beta activities in water samples using a low background liquid scintillation counter.

PubMed

Sanchez-Cabeza, J A; Pujol, L

1995-05-01

The radiological examination of water requires a rapid screening technique that permits the determination of the gross alpha and beta activities of each sample in order to decide if further radiological analyses are necessary. In this work, the use of a low background liquid scintillation system (Quantulus 1220) is proposed to simultaneously determine the gross activities in water samples. Liquid scintillation is compared to more conventional techniques used in most monitoring laboratories. In order to determine the best counting configuration of the system, pulse shape discrimination was optimized for 6 scintillant/vial combinations. It was concluded that the best counting configuration was obtained with the scintillation cocktail Optiphase Hisafe 3 in Zinsser low diffusion vials. The detection limits achieved were 0.012 Bq L-1 and 0.14 Bq L-1 for gross alpha and beta activity respectively, after a 1:10 concentration process by simple evaporation and for a counting time of only 360 min. The proposed technique is rapid, gives spectral information, and is adequate to determine gross activities according to the World Health Organization (WHO) guideline values.

Optimisation of nasal swab analysis by liquid scintillation counting.

PubMed

Dai, Xiongxin; Liblong, Aaron; Kramer-Tremblay, Sheila; Priest, Nicholas; Li, Chunsheng

2012-06-01

When responding to an emergency radiological incident, rapid methods are needed to provide the physicians and radiation protection personnel with an early estimation of possible internal dose resulting from the inhalation of radionuclides. This information is needed so that appropriate medical treatment and radiological protection control procedures can be implemented. Nasal swab analysis, which employs swabs swiped inside a nostril followed by liquid scintillation counting of alpha and beta activity on the swab, could provide valuable information to quickly identify contamination of the affected population. In this study, various parameters (such as alpha/beta discrimination, swab materials, counting time and volume of scintillation cocktail etc) were evaluated in order to optimise the effectiveness of the nasal swab analysis method. An improved nasal swab procedure was developed by replacing cotton swabs with polyurethane-tipped swabs. Liquid scintillation counting was performed using a Hidex 300SL counter with alpha/beta pulse shape discrimination capability. Results show that the new method is more reliable than existing methods using cotton swabs and effectively meets the analysis requirements for screening personnel in an emergency situation. This swab analysis procedure is also applicable to wipe tests of surface contamination to minimise the source self-absorption effect on liquid scintillation counting.

Pulsed neutron detector

DOEpatents

Robertson, deceased, J. Craig; Rowland, Mark S.

1989-03-21

A pulsed neutron detector and system for detecting low intensity fast neutron pulses has a body of beryllium adjacent a body of hydrogenous material the latter of which acts as a beta particle detector, scintillator, and moderator. The fast neutrons (defined as having En>1.5 MeV) react in the beryllium and the hydrogenous material to produce larger numbers of slow neutrons than would be generated in the beryllium itself and which in the beryllium generate hellium-6 which decays and yields beta particles. The beta particles reach the hydrogenous material which scintillates to yield light of intensity related to the number of fast neutrons. A photomultiplier adjacent the hydrogenous material (scintillator) senses the light emission from the scintillator. Utilization means, such as a summing device, sums the pulses from the photo-multiplier for monitoring or other purposes.

Development of a three-layer phoswich alpha-beta-gamma imaging detector

NASA Astrophysics Data System (ADS)

Yamamoto, Seiichi; Ishibashi, Hiroyuki

2015-06-01

For radiation monitoring at the sites of such nuclear power plant accidents as Fukushima Daiichi, radiation detectors are needed not only for gamma photons but also for alpha and beta particles because some nuclear fission products emit beta particles and gamma photons and some nuclear fuels contain plutonium that emits alpha particles. In some applications, imaging detectors are required to detect the distribution of plutonium particles that emit alpha particles and radiocesium in foods that emits beta particles and gamma photons. To solve these requirements, we developed an imaging detector that can measure the distribution of alpha and beta particles as well as gamma photons. The imaging detector consists of three-layer scintillators optically coupled to each other and to a position sensitive photomultiplier tube (PSPMT). The first layer, which is made of a thin plastic scintillator (decay time: 5 ns), detects alpha particles. The second layer, which is made of a thin Gd2SiO5 (GSO) scintillator with 1.5 mol% Ce (decay time: 35 ns), detects beta particles. The third layer made of a thin GSO scintillator with 0.4 mol% Ce (decay time: 70 ns) detects gamma photons. Using pulse shape discrimination, the images of these layers can be separated. The position information is calculated by the Anger principle from 8×8 anode signals from the PSPMT. The images for the alpha and beta particles and the gamma photons are individually formed by the pulse shape discriminations for each layer. We detected alpha particle images in the first layer and beta particle images in the second layer. Gamma photon images were detected in the second and third layers. The spatial resolution for the alpha and beta particles was 1.25 mm FWHM and less than 2 mm FWHM for the gamma photons. We conclude that our developed alpha-beta-gamma imaging detector is promising for imaging applications not only for the environmental monitoring of radionuclides but also for medical and molecular imaging.

Measurement of the scintillation time spectra and pulse-shape discrimination of low-energy β and nuclear recoils in liquid argon with DEAP-1

NASA Astrophysics Data System (ADS)

Amaudruz, P.-A.; Batygov, M.; Beltran, B.; Bonatt, J.; Boudjemline, K.; Boulay, M. G.; Broerman, B.; Bueno, J. F.; Butcher, A.; Cai, B.; Caldwell, T.; Chen, M.; Chouinard, R.; Cleveland, B. T.; Cranshaw, D.; Dering, K.; Duncan, F.; Fatemighomi, N.; Ford, R.; Gagnon, R.; Giampa, P.; Giuliani, F.; Gold, M.; Golovko, V. V.; Gorel, P.; Grace, E.; Graham, K.; Grant, D. R.; Hakobyan, R.; Hallin, A. L.; Hamstra, M.; Harvey, P.; Hearns, C.; Hofgartner, J.; Jillings, C. J.; Kuźniak, M.; Lawson, I.; La Zia, F.; Li, O.; Lidgard, J. J.; Liimatainen, P.; Lippincott, W. H.; Mathew, R.; McDonald, A. B.; McElroy, T.; McFarlane, K.; McKinsey, D. N.; Mehdiyev, R.; Monroe, J.; Muir, A.; Nantais, C.; Nicolics, K.; Nikkel, J.; Noble, A. J.; O'Dwyer, E.; Olsen, K.; Ouellet, C.; Pasuthip, P.; Peeters, S. J. M.; Pollmann, T.; Rau, W.; Retière, F.; Ronquest, M.; Seeburn, N.; Skensved, P.; Smith, B.; Sonley, T.; Tang, J.; Vázquez-Jáuregui, E.; Veloce, L.; Walding, J.; Ward, M.

2016-12-01

The DEAP-1 low-background liquid argon detector was used to measure scintillation pulse shapes of electron and nuclear recoil events and to demonstrate the feasibility of pulse-shape discrimination down to an electron-equivalent energy of 20 keVee. In the surface dataset using a triple-coincidence tag we found the fraction of β events that are misidentified as nuclear recoils to be < 1.4 ×10-7 (90% C.L.) for energies between 43-86 keVee and for a nuclear recoil acceptance of at least 90%, with 4% systematic uncertainty on the absolute energy scale. The discrimination measurement on surface was limited by nuclear recoils induced by cosmic-ray generated neutrons. This was improved by moving the detector to the SNOLAB underground laboratory, where the reduced background rate allowed the same measurement to be done with only a double-coincidence tag. The combined data set contains 1.23 × 108 events. One of those, in the underground data set, is in the nuclear-recoil region of interest. Taking into account the expected background of 0.48 events coming from random pileup, the resulting upper limit on the level of electronic recoil contamination is < 2.7 ×10-8 (90% C.L.) between 44-89 keVee and for a nuclear recoil acceptance of at least 90%, with 6% systematic uncertainty on the absolute energy scale. We developed a general mathematical framework to describe pulse-shape-discrimination parameter distributions and used it to build an analytical model of the distributions observed in DEAP-1. Using this model, we project a misidentification fraction of approximately 10-10 for an electron-equivalent energy threshold of 15 keVee for a detector with 8 PE/keVee light yield. This reduction enables a search for spin-independent scattering of WIMPs from 1000 kg of liquid argon with a WIMP-nucleon cross-section sensitivity of 10-46 cm2, assuming negligible contribution from nuclear recoil backgrounds.

Plutonium and uranium determination in environmental samples: combined solvent extraction-liquid scintillation method.

PubMed

McDowell, W J; Farrar, D T; Billings, M R

1974-12-01

A method for the determination of uranium and plutonium by a combined high-resolution liquid scintillation-solvent extraction method is presented. Assuming a sample count equal to background count to be the detection limit, the lower detection limit for these and other alpha-emitting nuclides is 1.0 dpm with a Pyrex sample tube, 0.3 dpm with a quartz sample tube using present detector shielding or 0.02 d.p.m. with pulse-shape discrimination. Alpha-counting efficiency is 100%. With the counting data presented as an alpha-energy spectrum, an energy resolution of 0.2-0.3 MeV peak half-width and an energy identification to +/-0.1 MeV are possible. Thus, within these limits, identification and quantitative determination of a specific alpha-emitter, independent of chemical separation, are possible. The separation procedure allows greater than 98% recovery of uranium and plutonium from solution containing large amounts of iron and other interfering substances. In most cases uranium, even when present in 10(8)-fold molar ratio, may be quantitatively separated from plutonium without loss of the plutonium. Potential applications of this general analytical concept to other alpha-counting problems are noted. Special problems associated with the determination of plutonium in soil and water samples are discussed. Results of tests to determine the pulse-height and energy-resolution characteristics of several scintillators are presented. Construction of the high-resolution liquid scintillation detector is described.

Highly Soluble p-Terphenyl and Fluorene Derivatives as Efficient Dopants in Plastic Scintillators for Sensitive Nuclear Material Detection.

PubMed

Yemam, Henok A; Mahl, Adam; Tinkham, Jonathan S; Koubek, Joshua T; Greife, Uwe; Sellinger, Alan

2017-07-03

Plastic scintillators are commonly used as first-line detectors for special nuclear materials. Current state-of-the-art plastic scintillators based on poly(vinyltoluene) (PVT) matrices containing high loadings (>15.0 wt %) of 2,5-diphenyloxazole (PPO) offer neutron signal discrimination in gamma radiation background (termed pulse shape discrimination, PSD), however, they suffer from poor mechanical properties. In this work, a series of p-terphenyl and fluorene derivatives were synthesized and tested as dopants in PVT based plastic scintillators as possible alternatives to PPO to address the mechanical property issue and to study the PSD mechanism. The derivatives were synthesized from low cost starting materials in high yields using simple chemistry. The photophysical and thermal properties were investigated for their influence on radiation sensitivity/detection performance, and mechanical stability. A direct correlation was found between the melting point of the dopants and the subsequent mechanical properties of the PVT based plastic scintillators. For example, select fluorene derivatives used as dopants produced scintillator samples with mechanical properties exceeding those of the commercial PPO-based scintillators while producing acceptable PSD capabilities. The physical properties of the synthesized dopants were also investigated to examine their effect on the final scintillator samples. Planar derivatives of fluorene were found to be highly soluble in PVT matrices with little to no aggregation induced effects. © 2017 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

Cross-correlation measurements with the EJ-299-33 plastic scintillator

NASA Astrophysics Data System (ADS)

Bourne, Mark M.; Whaley, Jeff; Dolan, Jennifer L.; Polack, John K.; Flaska, Marek; Clarke, Shaun D.; Tomanin, Alice; Peerani, Paolo; Pozzi, Sara A.

2015-06-01

New organic-plastic scintillation compositions have demonstrated pulse-shape discrimination (PSD) of neutrons and gamma rays. We present cross-correlation measurements of 252Cf and mixed uranium-plutonium oxide (MOX) with the EJ-299-33 plastic scintillator. For comparison, equivalent measurements were performed with an EJ-309 liquid scintillator. Offline, digital PSD was applied to each detector. These measurements show that EJ-299-33 sacrifices a factor of 5 in neutron-neutron efficiency relative to EJ-309, but could still utilize the difference in neutron-neutron efficiency and neutron single-to-double ratio to distinguish 252Cf from MOX. These measurements were modeled with MCNPX-PoliMi, and MPPost was used to convert the detailed collision history into simulated cross-correlation distributions. MCNPX-PoliMi predicted the measured 252Cf cross-correlation distribution for EJ-309 to within 10%. Greater photon uncertainty in the MOX sample led to larger discrepancy in the simulated MOX cross-correlation distribution. The modeled EJ-299-33 plastic also gives reasonable agreement with measured cross-correlation distributions, although the MCNPX-PoliMi model appears to under-predict the neutron detection efficiency.

Status of LUMINEU program to search for neutrinoless double beta decay of 100Mo with cryogenic ZnMoO4 scintillating bolometers

NASA Astrophysics Data System (ADS)

Danevich, F. A.; Bergé, L.; Boiko, R. S.; Chapellier, M.; Chernyak, D. M.; Coron, N.; Devoyon, L.; Drillien, A.-A.; Dumoulin, L.; Enss, C.; Fleischmann, A.; Gastaldo, L.; Giuliani, A.; Gray, D.; Gros, M.; Hervé, S.; Humbert, V.; Ivanov, I. M.; Juillard, A.; Kobychev, V. V.; Koskas, F.; Loidl, M.; Magnier, P.; Makarov, E. P.; Mancuso, M.; de Marcillac, P.; Marnieros, S.; Marrache-Kikuchi, C.; Navick, X.-F.; Nones, C.; Olivieri, E.; Paul, B.; Penichot, Y.; Pessina, G.; Plantevin, O.; Poda, D. V.; Redon, T.; Rodrigues, M.; Shlegel, V. N.; Strazzer, O.; Tenconi, M.; Torres, L.; Tretyak, V. I.; Vasiliev, Ya. V.; Velazquez, M.; Viraphong, O.

2015-10-01

The LUMTNEU program aims at performing a pilot experiment on 0ν2β decay of 100Mo using radiopure ZnMoO4 crystals enriched in 100Mo operated as cryogenic scintillating bolometers. Large volume ZnMoO4 crystal scintillators (˜ 0.3 kg) were developed and tested showing high performance in terms of radiopurity, energy resolution and α/β particle discrimination capability. Zinc molybdate crystal scintillators enriched in 100Mo were grown for the first time by the low-thermal-gradient Czochralski technique with a high crystal yield and an acceptable level of enriched molybdenum irrecoverable losses. A background level of ˜ 0.5 counts/(yr keV ton) in the region of interest can be reached in a large detector array thanks to the excellent detectors radiopurity and particle discrimination capability, suppression of randomly coinciding events by pulse-shape analysis, and anticoincidence cut. These results pave the way to future sensitive searches based on the LUMTNEU technology, capable of approachingand exploring the inverted hierarchy region of the neutrino mass pattern.

Development of neutron-monitor detector using liquid organic scintillator coupled with 6Li + ZnS(Ag) Sheet.

PubMed

Sato, Tatsuhiko; Endo, Akira; Yamaguchi, Yasuhiro; Takahashi, Fumiaki

2004-01-01

A phoswitch-type detector has been developed for monitoring neutron doses in high-energy accelerator facilities. The detector is composed of a liquid organic scintillator (BC501A) coupled with ZnS(Ag) sheets doped with 6Li. The dose from neutrons with energies above 1 MeV is evaluated from the light output spectrum of the BC501A by applying the G-function, which relates the spectrum to the neutron dose directly. The dose from lower energy neutrons, on the other hand, is estimated from the number of scintillations emitted from the ZnS(Ag) sheets. Characteristics of the phoswitch-type detector were studied experimentally in some neutron fields. It was found from the experiments that the detector has an excellent property of pulse-shape discrimination between the scintillations of BC501A and the ZnS(Ag) sheets. The experimental results also indicate that the detector is capable of reproducing doses from thermal neutrons as well as neutrons with energies from one to several tens of megaelectronvolts (MeV).

DOE Office of Scientific and Technical Information (OSTI.GOV)

Miller, C A; Clarke, S D; Pozzi, S A

Purpose: To develop an instrument for measuring neutron and photon dose rates from mixed fields with a single device. Methods: Stilbene organic scintillators can be used to detect fast neutrons and photons. Stilbene was used to measure emission from mixed particle sources californium-252 (Cf-252) and plutonium-beryllium (PuBe). Many source detector configurations were used, along with varying amounts of shielding. Collected spectra were analyzed using pulse shape discrimination software, to separate neutron and photon interactions. With a measured light output to energy relationship the pulse height spectrum was converted to energy deposited in the detector. Energy deposited was converted to dosemore » with a variety of standard dose factors, for comparison to current methods. For validation, all measurements and processing was repeated using an EJ-309 liquid scintillator detector. Dose rates were also measured in the same configuration with commercially available dose meters for further validation. Results: Measurements of dose rates will show agreement across all methods. Higher accuracy of pulse shape discrimination at lower energies with stilbene leads to more accurate measurement of neutron and photon deposited dose. In strong fields of mixed particles discrimination can be performed well at a very low energy threshold. This shows accurate dose measurements over a large range of incident particle energy. Conclusion: Stilbene shows promise as a material for dose rate measurements due to its strong ability for separating neutrons and photon pulses and agreement with current methods. A dual particle dose meter would simplify methods which are currently limited to the measurement of only one particle type. Future work will investigate the use of a silicon photomultiplier to reduce the size and required voltage of the assembly, for practical use as a handheld survey meter, room monitor, or phantom installation. Funding From the United States Department of Energy and the National Nuclear Security Administration.« less

Measuring and Validating Neutron Capture Cross Sections Using a Lead Slowing-Down Spectrometer

NASA Astrophysics Data System (ADS)

Thompson, Nicholas

Accurate nuclear data is essential for the modeling, design, and operation of nuclear systems. In this work, the Rensselaer Polytechnic Institute (RPI) Lead Slowing-Down Spectrometer (LSDS) at the Gaerttner Linear Accelerator Center (LINAC) was used to measure neutron capture cross sections and validate capture cross sections in cross section libraries. The RPI LINAC was used to create a fast burst of neutrons in the center of the LSDS, a large cube of high purity lead. A sample and YAP:Ce scintillator were placed in the LSDS, and as neutrons lost energy through scattering interactions with the lead, the scintillator detected capture gammas resulting from neutron capture events in the sample. Samples of silver, gold, cobalt, iron, indium, molybdenum, niobium, nickel, tin, tantalum, and zirconium were measured. Data was collected as a function of time after neutron pulse, or slowing-down time, which is correlated to average neutron energy. An analog and a digital data acquisition system collected data simultaneously, allowing for collection of pulse shape information as well as timing. Collection of digital data allowed for pulse shape analysis after the experiment. This data was then analyzed and compared to Monte Carlo simulations to validate the accuracy of neutron capture cross section libraries. These measurements represent the first time that neutron capture cross sections have been measured using an LSDS in the United States, and the first time tools such as coincidence measurements and pulse height weighting have been applied to measurements of neutron capture cross sections using an LSDS. Significant differences between measurement results and simulation results were found in multiple materials, and some errors in nuclear data libraries have already been identified due to these measurements.

A remotely triggered fast neutron detection instrument based on a plastic organic scintillator

NASA Astrophysics Data System (ADS)

Jones, A. R.; Aspinall, M. D.; Joyce, M. J.

2018-02-01

A detector system for the characterization of radiation fields of both fast neutrons and γ rays is described comprising of a gated photomultiplier tube (PMT), an EJ299-33 solid organic scintillator detector, and an external trigger circuit. The objective of this development was to conceive a means by which the PMT in such a system can be actuated remotely during the high-intensity bursts of pulsed γ-ray contamination that can arise during active interrogation procedures. The system is used to detect neutrons and γ rays using established pulse-shape discrimination (PSD) techniques. The gating circuit enables the PMT to be switched off remotely. This is compatible with use during intense radiation transients to avoid saturation and the disruption of the operation of the PMT during the burst. Data are presented in the form of pulse-height spectra and PSD scatter plots for the system triggered with a strobed light source. These confirm that the gain of the system and the throughput for both triggered and un-triggered scenarios are as expected, given the duty cycle of the stimulating radiation. This demonstrates that the triggering function does not perturb the system response of the detector.

A remotely triggered fast neutron detection instrument based on a plastic organic scintillator.

PubMed

Jones, A R; Aspinall, M D; Joyce, M J

2018-02-01

A detector system for the characterization of radiation fields of both fast neutrons and γ rays is described comprising of a gated photomultiplier tube (PMT), an EJ299-33 solid organic scintillator detector, and an external trigger circuit. The objective of this development was to conceive a means by which the PMT in such a system can be actuated remotely during the high-intensity bursts of pulsed γ-ray contamination that can arise during active interrogation procedures. The system is used to detect neutrons and γ rays using established pulse-shape discrimination (PSD) techniques. The gating circuit enables the PMT to be switched off remotely. This is compatible with use during intense radiation transients to avoid saturation and the disruption of the operation of the PMT during the burst. Data are presented in the form of pulse-height spectra and PSD scatter plots for the system triggered with a strobed light source. These confirm that the gain of the system and the throughput for both triggered and un-triggered scenarios are as expected, given the duty cycle of the stimulating radiation. This demonstrates that the triggering function does not perturb the system response of the detector.

A high-speed scintillation-based electronic portal imaging device to quantitatively characterize IMRT delivery.

PubMed

Ranade, Manisha K; Lynch, Bart D; Li, Jonathan G; Dempsey, James F

2006-01-01

We have developed an electronic portal imaging device (EPID) employing a fast scintillator and a high-speed camera. The device is designed to accurately and independently characterize the fluence delivered by a linear accelerator during intensity modulated radiation therapy (IMRT) with either step-and-shoot or dynamic multileaf collimator (MLC) delivery. Our aim is to accurately obtain the beam shape and fluence of all segments delivered during IMRT, in order to study the nature of discrepancies between the plan and the delivered doses. A commercial high-speed camera was combined with a terbium-doped gadolinium-oxy-sulfide (Gd2O2S:Tb) scintillator to form an EPID for the unaliased capture of two-dimensional fluence distributions of each beam in an IMRT delivery. The high speed EPID was synchronized to the accelerator pulse-forming network and gated to capture every possible pulse emitted from the accelerator, with an approximate frame rate of 360 frames-per-second (fps). A 62-segment beam from a head-and-neck IMRT treatment plan requiring 68 s to deliver was recorded with our high speed EPID producing approximately 6 Gbytes of imaging data. The EPID data were compared with the MLC instruction files and the MLC controller log files. The frames were binned to provide a frame rate of 72 fps with a signal-to-noise ratio that was sufficient to resolve leaf positions and segment fluence. The fractional fluence from the log files and EPID data agreed well. An ambiguity in the motion of the MLC during beam on was resolved. The log files reported leaf motions at the end of 33 of the 42 segments, while the EPID observed leaf motions in only 7 of the 42 segments. The static IMRT segment shapes observed by the high speed EPID were in good agreement with the shapes reported in the log files. The leaf motions observed during beam-on for step-and-shoot delivery were not temporally resolved by the log files.

Apparatus and method for temperature correction and expanded count rate of inorganic scintillation detectors

DOEpatents

Ianakiev, Kiril D [Los Alamos, NM; Hsue, Sin Tao [Santa Fe, NM; Browne, Michael C [Los Alamos, NM; Audia, Jeffrey M [Abiquiu, NM

2006-07-25

The present invention includes an apparatus and corresponding method for temperature correction and count rate expansion of inorganic scintillation detectors. A temperature sensor is attached to an inorganic scintillation detector. The inorganic scintillation detector, due to interaction with incident radiation, creates light pulse signals. A photoreceiver processes the light pulse signals to current signals. Temperature correction circuitry that uses a fast light component signal, a slow light component signal, and the temperature signal from the temperature sensor to corrected an inorganic scintillation detector signal output and expanded the count rate.

A DSP equipped digitizer for online analysis of nuclear detector signals

NASA Astrophysics Data System (ADS)

Pasquali, G.; Ciaranfi, R.; Bardelli, L.; Bini, M.; Boiano, A.; Giannelli, F.; Ordine, A.; Poggi, G.

2007-01-01

In the framework of the NUCL-EX collaboration, a DSP equipped fast digitizer has been implemented and it has now reached the production stage. Each sampling channel is implemented on a separate daughter-board to be plugged on a VME mother-board. Each channel features a 12-bit, 125 MSamples/s ADC and a Digital Signal Processor (DSP) for online analysis of detector signals. A few algorithms have been written and successfully tested on detectors of different types (scintillators, solid-state, gas-filled), implementing pulse shape discrimination, constant fraction timing, semi-Gaussian shaping, gated integration.

Skin contamination dosimeter

DOEpatents

Hamby, David M [Corvallis, OR; Farsoni, Abdollah T [Corvallis, OR; Cazalas, Edward [Corvallis, OR

2011-06-21

A technique and device provides absolute skin dosimetry in real time at multiple tissue depths simultaneously. The device uses a phoswich detector which has multiple scintillators embedded at different depths within a non-scintillating material. A digital pulse processor connected to the phoswich detector measures a differential distribution (dN/dH) of count rate N as function of pulse height H for signals from each of the multiple scintillators. A digital processor computes in real time from the differential count-rate distribution for each of multiple scintillators an estimate of an ionizing radiation dose delivered to each of multiple depths of skin tissue corresponding to the multiple scintillators embedded at multiple corresponding depths within the non-scintillating material.

Fast scintillation counter system and performance

NASA Technical Reports Server (NTRS)

Sasaki, H.; Nishioka, A.; Ohmori, N.; Kusumose, M.; Nakatsuka, T.; Horiki, T.; Hatano, Y.

1985-01-01

An experimental study of the fast scintillation counter (FS) system to observe a shower disk structure at Mt. Norikura is described, especially the system performance and a pulse wave-form by a single charge particles. The photomultiplier tube (PT) pulse appears at the leading edge of the main pulse. To remove this PT-pulse from the main pulse, the frame of the scintillator vessel was changed. The fast triggering system was made to decrease the dead time which came from the use of the function of the self triggering of the storage oscilloscope (OSC). To provide a new field on the multi-parameter study of the cosmic ray showers, the system response of the FS system also improved as a result of many considerations.

Measurements of response functions of EJ-299-33A plastic scintillator for fast neutrons

NASA Astrophysics Data System (ADS)

Hartman, J.; Barzilov, A.; Peters, E. E.; Yates, S. W.

2015-12-01

Monoenergetic neutron response functions were measured for an EJ-299-33A plastic scintillator. The 7-MV Van de Graaff accelerator at the University of Kentucky Accelerator Laboratory was used to produce proton and deuteron beams for reactions with gaseous tritium and deuterium targets, yielding monoenergetic neutrons by means of the 3H(p,n)3He, 2H(d,n)3He, and 3H(d,n)4He reactions. The neutron energy was selected by tuning the charged-particle's energy and using the angular dependence of the neutron emission. The resulting response functions were measured for 0.1-MeV steps in neutron energy from 0.1 MeV to 8.2 MeV and from 12.2 MeV to 20.2 MeV. Experimental data were processed using a procedure for digital pulse-shape discrimination, which allowed characterization of the response functions of the plastic scintillator to neutrons only. The response functions are intended for use in neutron spectrum unfolding methods.

Positronium signature in organic liquid scintillators for neutrino experiments

DOE Office of Scientific and Technical Information (OSTI.GOV)

Franco, D.; Consolati, G.; Trezzi, D.

2011-01-15

Electron antineutrinos are commonly detected in liquid scintillator experiments via inverse {beta} decay by looking at the coincidence between the reaction products: neutrons and positrons. Prior to positron annihilation, an electron-positron pair may form an orthopositronium (o-Ps) state, with a mean lifetime of a few nanoseconds. Even if the o-Ps decay is speeded up by spin-flip or pick-off effects, it may introduce distortions in the photon emission time distribution, crucial for position reconstruction and pulse shape discrimination algorithms in antineutrino experiments. Reversing the problem, the o-Ps-induced time distortion represents a new signature for tagging antineutrinos in liquid scintillator. In thismore » article, we report the results of measurements of the o-Ps formation probability and lifetime for the most used solvents for organic liquid scintillators in neutrino physics (pseudocumene, linear alkyl benzene, phenylxylylethane, and dodecane). We characterize also a mixture of pseudocumene +1.5 g/l of 2,5-diphenyloxazole, a fluor acting as wavelength shifter. In the second part of the article, we demonstrate that the o-Ps-induced distortion of the scintillation photon emission time distributions represent an optimal signature for tagging positrons on an event by event basis, potentially enhancing the antineutrino detection.« less

Neutron detection with plastic scintillators coupled to solid state photomultiplier detectors

NASA Astrophysics Data System (ADS)

Christian, James F.; Johnson, Erik B.; Fernandez, Daniel E.; Vogel, Samuel; Frank, Rebecca; Stoddard, Graham; Stapels, Christopher; Pereira, Jorge; Zegers, Remco

2017-09-01

The recent reduction of dark current in Silicon Solid-state photomultipliers (SiSSPMs) makes them an attractive alternative to conventional photomultiplier tubes (PMTs) for scintillation detection applications. Nuclear Physics experiments often require large detector volumes made using scintillation materials, which require sensitive photodetectors, such as a PMTs. PMTs add to the size, fragility, and high-voltage requirements as well as distance requirements for experiments using magnetic fields. This work compares RMD's latest detector modules, denoted as the "year 2 prototype", of plastic scintillators that discriminate gamma and high-energy particle events from neutron events using pulse shape discrimination (PSD) coupled to a SiSSPM to the following two detector modules: a similar "year 1 prototype" and a scintillator coupled to a PMT module. It characterizes the noise floor, relative signal-to-noise ratio (SNR), the timing performance, the PSD figure-of-merit (FOM) and the neutron detection efficiency of RMD's detectors. This work also evaluates the scaling of SiSSPM detector modules to accommodate the volumes needed for many Nuclear Physics experiments. The Si SSPM detector module provides a clear advantage in Nuclear Physics experiments that require the following attributes: discrimination of neutron and gamma-ray events, operation in or near strong magnetic fields, and segmentation of the detector.

Gadolinium-loaded Plastic Scintillators for Thermal Neutron Detection using Compensation

NASA Astrophysics Data System (ADS)

Dumazert, Jonathan; Coulon, Romain; Hamel, Matthieu; Carrel, Frédérick; Sguerra, Fabien; Normand, Stéphane; Méchin, Laurence; Bertrand, Guillaume H. V.

2016-06-01

Plastic scintillator loading with gadolinium-rich organometallic complexes shows a high potential for the deployment of efficient and cost-effective neutron detectors. Due to the low-energy photon and electron signature of thermal neutron capture by Gd-155 and Gd-157, alternative treatment to pulse-shape discrimination has to be proposed in order to display a count rate. This paper discloses the principle of a compensation method applied to a two-scintillator system: a detection scintillator interacts with photon and fast neutron radiation and is loaded with gadolinium organometallic compound to become a thermal neutron absorber, while a not-gadolinium loaded compensation scintillator solely interacts with the fast neutron and photon part of incident radiation. After the nonlinear smoothing of the counting signals, a hypothesis test determines whether the resulting count rate post-background response compensation falls into statistical fluctuations or provides a robust indication of neutron activity. Laboratory samples are tested under both photon and neutron irradiations, allowing the authors to investigate the performance of the overall detection system in terms of sensitivity and detection limits, especially with regards to a similar-active volume He-3 based commercial counter. The study reveals satisfactory figures of merit in terms of sensitivity and directs future investigation toward promising paths.

Development of a thin scintillation films fission-fragment detector and a novel neutron source

NASA Astrophysics Data System (ADS)

Rusev, G.; Jandel, M.; Baramsai, B.; Bond, E. M.; Bredeweg, T. A.; Couture, A.; Daum, J. K.; Favalli, A.; Ianakiev, K. D.; Iliev, M. L.; Mosby, S.; Roman, A. R.; Springs, R. K.; Ullmann, J. L.; Walker, C. L.

2015-08-01

Investigation of prompt fission and neutron-capture Υ rays from fissile actinide samples at the Detector for Advanced Neutron Capture Experiments (DANCE) requires use of a fission-fragment detector to provide a trigger or a veto signal. A fission-fragment detector based on thin scintillating films and silicon photomultipliers has been built to serve as a trigger/veto detector in neutron-induced fission measurements at DANCE. The fissile material is surrounded by scintillating films providing a 4π detection of the fission fragments. The scintillations were registered with silicon photomultipliers. A measurement of the 235U(n,f) reaction with this detector at DANCE revealed a correct time-of-flight spectrum and provided an estimate for the efficiency of the prototype detector of 11.6(7)%. Design and test measurements with the detector are described. A neutron source with fast timing has been built to help with detector-response measurements. The source is based on the neutron emission from the spontaneous fission of 252Cf and the same type of scintillating films and silicon photomultipliers. Overall time resolution of the source is 0.3 ns. Design of the source and test measurements with it are described. An example application of the source for determining the neutron/gamma pulse-shape discrimination by a stilbene crystal is given.

PRESCILA: a new, lightweight neutron rem meter.

PubMed

Olsher, Richard H; Seagraves, David T; Eisele, Shawna L; Bjork, Christopher W; Martinez, William A; Romero, Leonard L; Mallett, Michael W; Duran, Michael A; Hurlbut, Charles R

2004-06-01

Conventional neutron rem meters currently in use are based on 1960's technology that relies on a large neutron moderator assembly surrounding a thermal detector to achieve a rem-like response function over a limited energy range. Such rem meters present an ergonomic challenge, being heavy and bulky, and have caused injuries during radiation protection surveys. Another defect of traditional rem meters is a poor high-energy response above 10 MeV, which makes them unsuitable for applications at high-energy accelerator facilities. Proton Recoil Scintillator-Los Alamos (PRESCILA) was developed as a low-weight (2 kg) alternative capable of extended energy response, high sensitivity, and moderate gamma rejection. An array of ZnS(Ag) based scintillators is located inside and around a Lucite light guide, which couples the scintillation light to a sideview bialkali photomultiplier tube. The use of both fast and thermal scintillators allows the energy response function to be optimized for a wide range of operational spectra. The light guide and the borated polyethylene frame provide moderation for the thermal scintillator element. The scintillators represent greatly improved versions of the Hornyak and Stedman designs from the 1950's, and were developed in collaboration with Eljen Technology. The inherent pulse height advantage of proton recoils over electron tracks in the phosphor grains eliminates the need for pulse shape discrimination and makes it possible to use the PRESCILA probe with standard pulse height discrimination provided by off-the-shelf health physics counters. PRESCILA prototype probes have been extensively tested at both Los Alamos and the German Bureau of Standards, Physikalisch-Technische Bundesanstalt. Test results are presented for energy response, directional dependence, linearity, sensitivity, and gamma rejection. Initial field tests have been conducted at Los Alamos and these results are also given. It is concluded that PRESCILA offers a viable, ergonomically superior, alternative to traditional rem meters that is effective for a wide range of neutron fields. The probe is capable of excellent sensitivity (40 counts per minute per microSv h-1 for 241AmBe) and extended energy response to beyond 20 MeV. Directional response is uniform (+/-15%) over a wide range of energies. Response linearity has been characterized to over 20 mSv h-1. Gamma rejection is effective in gamma fields up to 2 mSv h-1. The PRESCILA technology has been commercialized and is now offered under license by Ludlum Measurements, Inc.

SCINFUL: A Monte Carlo based computer program to determine a scintillator full energy response to neutron detection for E/sub n/ between 0. 1 and 80 MeV: Program development and comparisons of program predictions with experimental data

DOE Office of Scientific and Technical Information (OSTI.GOV)

Dickens, J.K.

1988-04-01

This document provides a discussion of the development of the FORTRAN Monte Carlo program SCINFUL (for scintillator full response), a program designed to provide a calculated full response anticipated for either an NE-213 (liquid) scintillator or an NE-110 (solid) scintillator. The program may also be used to compute angle-integrated spectra of charged particles (p, d, t, /sup 3/He, and ..cap alpha..) following neutron interactions with /sup 12/C. Extensive comparisons with a variety of experimental data are given. There is generally overall good agreement (<10% differences) of results from SCINFUL calculations with measured detector responses, i.e., N(E/sub r/) vs E/sub r/more » where E/sub r/ is the response pulse height, reproduce measured detector responses with an accuracy which, at least partly, depends upon how well the experimental configuration is known. For E/sub n/ < 16 MeV and for E/sub r/ > 15% of the maximum pulse height response, calculated spectra are within +-5% of experiment on the average. For E/sub n/ up to 50 MeV similar good agreement is obtained with experiment for E/sub r/ > 30% of maximum response. For E/sub n/ up to 75 MeV the calculated shape of the response agrees with measurements, but the calculations underpredicts the measured response by up to 30%. 65 refs., 64 figs., 3 tabs.« less

DOE Office of Scientific and Technical Information (OSTI.GOV)

Andrews, Madison Theresa; Bates, Cameron Russell; Mckigney, Edward Allen

Accurate detector modeling is a requirement to design systems in many non-proliferation scenarios; by determining a Detector’s Response Function (DRF) to incident radiation, it is possible characterize measurements of unknown sources. DRiFT is intended to post-process MCNP® output and create realistic detector spectra. Capabilities currently under development include the simulation of semiconductor, gas, and (as is discussed in this work) scintillator detector physics. Energy spectra and pulse shape discrimination (PSD) trends for incident photon and neutron radiation have been reproduced by DRiFT.

Time-over-threshold for pulse shape discrimination in a time-of-flight phoswich PET detector.

PubMed

Chang, Chen-Ming; Cates, Joshua W; Levin, Craig S

2017-01-07

It is well known that a PET detector capable of measuring both photon time-of-flight (TOF) and depth-of-interaction (DOI) improves the image quality and accuracy. Phoswich designs have been realized in PET detectors to measure DOI for more than a decade. However, PET detectors based on phoswich designs put great demand on the readout circuits, which have to differentiate the pulse shape produced by different crystal layers. A simple pulse shape discrimination approach is required to realize the phoswich designs in a clinical PET scanner, which consists of thousands of scintillation crystal elements. In this work, we studied time-over-threshold (ToT) as a pulse shape parameter for DOI. The energy, timing and DOI performance were evaluated for a phoswich detector design comprising [Formula: see text] mm LYSO:Ce crystal optically coupled to [Formula: see text] mm calcium co-doped LSO:Ce,Ca(0.4%) crystal read out by a silicon photomultiplier (SiPM). A DOI accuracy of 97.2% has been achieved for photopeak events using the proposed time-over-threshold (ToT) processing. The energy resolution without correction for SiPM non-linearity was [Formula: see text]% and [Formula: see text]% FWHM at 511 keV for LYSO and LSO crystal layers, respectively. The coincidence time resolution for photopeak events ranges from 164.6 ps to 183.1 ps FWHM, depending on the layer combinations. The coincidence time resolution for inter-crystal scatter events ranges from 214.6 ps to 418.3 ps FWHM, depending on the energy windows applied. These results show great promises of using ToT for pulse shape discrimination in a TOF phoswich detector since a ToT measurement can be easily implemented in readout electronics.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Gao, Fei; Kerisit, Sebastien N.; Xie, YuLong

This annual report presents work carried out during Fiscal Year (FY) 2013 at Pacific Northwest National Laboratory (PNNL) under the project entitled “Science-Driven Candidate Search for New Scintillator Materials” (Project number: PL13-SciDriScintMat-PD05) and led by Dr. Fei Gao. This project is divided into three tasks, namely (1) Ab initio calculations of electronic properties, electronic response functions and secondary particle spectra; (2) Intrinsic response properties, theoretical light yield, and microscopic description of ionization tracks; and (3) Kinetics and efficiency of scintillation: nonlinearity, intrinsic energy resolution, and pulse shape discrimination. Detailed information on the findings and insights obtained in each of thesemore » three tasks are provided in this report. Additionally, papers published this fiscal year or currently in review are included in Appendix together with presentations given this fiscal year.« less

DESCANT - The DEuterated SCintillator Array for Neutron Tagging

NASA Astrophysics Data System (ADS)

Bildstein, Vinzenz; Garrett, P. E.; Bandyopadhay, D.; Bangay, J.; Bianco, L.; Demand, G.; Hadinia, B.; Leach, K. G.; Sumithrarachchi, C.; Turko, J.; Wong, J.; Ashley, S. F.; Crider, B. P.; McEllistrem, M. T.; Peters, E. E.; Prados-Estévez, F. M.; Yates, S. W.; Vanhoy, J. R.; Ball, G. C.; Bishop, D. P.; Garnsworthy, A. B.; Hackman, G.; Pearson, C. J.; Shaw, B.; Saran, F.

2016-09-01

The DESCANT array at TRIUMF is designed to detect neutrons from RIB experiments. DESCANT is composed of 70 close-packed deuterated organic liquid scintillators coupled to digital fast read-out ADC modules. This configuration will permit online pulse-shape discrimination between neutron and γ-ray events. A prototype detector has been tested with monoenergetic neutrons at the accelerator laboratory of the University of Kentucky. A first commissioning experiment of the full array, using the decay of 145-146Cs, will be performed in August 2016. The results of the tests and a preliminary analysis of the commissioning experiment will be presented. Work supported by the Canada Foundation for Innovation, the Natural Sciences and Engineering Research Council of Canada, the National Research Council of Canada and the Canadian Research Chairs program.

The 3H(d,γ)5He Reaction for Ec.m. ≤ 300 keV

NASA Astrophysics Data System (ADS)

Parker, C. E.; Brune, C. R.; Massey, T. N.; O'Donnell, J. E.; Richard, A. L.; Sayre, D. B.

2016-03-01

The 3H(d, γ)5He reaction has been measured using a 500-keV pulsed deuteron beam incident on a stopping titanium tritide target at Ohio University's Edwards Accelerator Laboratory. The time-of-flight (TOF) technique has been used to distinguish the γ-rays from neutrons detected in the bismuth germinate (BGO) γ-ray detector. A stilbene scintillator and an NE-213 scintillator have been used to detect the neutrons from the 3H(d, n)4He reaction using both the pulse-shape discrimination and TOF techniques. A newly-designed target holder with a silicon surface barrier detector to simultaneously measure α-particles to normalize the neutron count was incorporated for subsequent measurements. The γ-rays have been measured at laboratory angles of 0°, 45°, 90°, and 135°. Information about the γ-ray energy distribution for the unbound ground state and first excited state of 5He can be obtained experimentally by comparing the BGO data to Monte Carlo simulations. The 3H(d, γ)/3H(d, n) branching ratio has also been determined.

Active Well Counting Using New PSD Plastic Detectors

DOE Office of Scientific and Technical Information (OSTI.GOV)

Hausladen, Paul; Newby, Jason; McElroy, Robert Dennis

This report presents results and analysis from a series of proof-of-concept measurements to assess the suitability of segmented detectors constructed from Eljen EJ-299-34 PSD-plastic scintillator with pulse-shape discrimination capability for the purposes of quantifying uranium via active neutron coincidence counting. Present quantification of bulk uranium materials for international safeguards and domestic materials control and accounting relies on active neutron coincidence counting systems, such as the Active Well Coincidence Counter (AWCC) and the Uranium Neutron Coincidence Collar (UNCL), that use moderated He-3 proportional counters along with necessarily low-intensity 241Am(Li) neutron sources. Scintillation-based fast-neutron detectors are a potentially superior technology to themore » existing AWCC and UNCL designs due to their spectroscopic capability and their inherently short neutron coincidence times that largely eliminate random coincidences and enable interrogation by stronger sources. One of the past impediments to the investigation and adoption of scintillation counters for the purpose of quantifying bulk uranium was the commercial availability of scintillators having the necessary neutron-gamma pulse-shape discrimination properties only as flammable liquids. Recently, Eljen EJ-299-34 PSD-plastic scintillator became commercially available. The present work is the first assessment of an array of PSD-plastic detectors for the purposes of quantifying bulk uranium. The detector panel used in the present work was originally built as the focal plane for a fast-neutron imager, but it was repurposed for the present investigation by construction of a stand to support the inner well of an AWCC immediately in front of the detector panel. The detector panel and data acquisition of this system are particularly well suited for performing active-well fast-neutron counting of LEU and HEU samples because the active detector volume is solid, the 241Am(Li) interrogating neutrons are largely below the detector threshold, and the segmented construction of the detector modules allow for separation of true neutron-neutron coincidences from inter-detector scattering using the kinematics of neutron scattering. The results from a series of measurements of a suite of uranium standards are presented, and compared to measurements of the same standards and source configurations using the AWCC. Using these results, the performance of the segmented detectors reconfigured as a well counter is predicted and outperforms the AWCC.« less

Luminescence properties and scintillation response in Ce3+-doped Y2Gd1Al5-xGaxO12 (x = 2, 3, 4) single crystals

NASA Astrophysics Data System (ADS)

Chewpraditkul, Warut; Pánek, Dalibor; Brůža, Petr; Chewpraditkul, Weerapong; Wanarak, Chalerm; Pattanaboonmee, Nakarin; Babin, Vladimir; Bartosiewicz, Karol; Kamada, Kei; Yoshikawa, Akira; Nikl, Martin

2014-08-01

The compositional dependence of luminescence properties and scintillation response were investigated in Ce3+-doped Y2Gd1Al5-xGaxO12 (x = 2, 3, 4) single crystals. The Gd3+ → Ce3+ energy transfer was evidenced by photoluminescence excitation spectra of Ce3+ emission. With increasing Ga content in the garnet host, the Ce3+ luminescence from the lowest 5d level (5d1) is shifted toward higher energy due to the decrease in the crystal field splitting of the 5d levels. Light yield (LY) and its dependence on the amplifier shaping time were measured under excitation with γ-rays. High LY value of ˜38 000 ph/MeV was obtained for a Y2Gd1Al3Ga2O12:Ce sample. Scintillation decay was measured with an extended dynamical and temporal scale under the nanosecond pulse soft X-ray excitation. The decrease of both LY value and relative contribution of slower decay component in the scintillation response was observed with increasing Ga content in the garnet host.

Measured neutron and gamma spectra from californium-252 in a tissue-equivalent medium.

PubMed

Elson, H R; Stupar, T A; Shapiro, A; Kereiakes, J G

1979-01-01

A method of experimentally obtaining both neutron and gamma-ray spectra in a scattering medium is described. The method utilizes a liquid-organic scintillator (NE-213) coupled with a pulse-shape discrimination circuit. This allows the separation of the neutron-induced pulse-height data from the gamma-ray pulse-height data. Using mathematical unfolding techniques, the two sets of pulse-height data were transformed to obtain the neutron and gamma-ray energy spectra. A small spherical detector was designed and constructed to reduce the errors incurred by attempting spectral measurements in a scattering medium. Demonstration of the utility of the system to obtain the neutron and gamma-ray spectra in a scattering medium was performed by characterizing the neutron and gamma-ray spectra at various sites about a 3.7-microgram (1.5 cm active length) californium-252 source in a tissue-equivalent medium.

Calibration of LiBaF3: Ce Scintillator for Fission Spectrum Neutrons

DOE Office of Scientific and Technical Information (OSTI.GOV)

Reeder, Paul L.; Bowyer, Sonya M.

2002-05-21

The scintillator LiBaF3 doped with small amounts of Ce+3 has the ability to distinguish heavy charged particles (p, d, t, or a) from beta and/or gamma radiation based on the presence or absence of ns components in the scintillation light output. Because the neutron capture reaction on 6Li produces recoil alphas and tritons, this scintillator also discriminates between neutron induced events and beta or gamma interactions. An experimental technique using a time-tagged 252Cf source has been used to measure the efficiency of this scintillator for neutron capture, the calibration of neutron capture pulse height, and the pulse height resolution -more » all as a function of incident neutron energy.« less

DOE Office of Scientific and Technical Information (OSTI.GOV)

Agnes, P.; et al.

The DarkSide-50 experiment, located at the “Laboratori Nazionali del Gran Sasso (INFN)”, is based on low-radioactivity argon double phase time projection chamber, surrounded by an active liquid scintillator veto, designed for the zero background achievement. The liquid argon features sufficient self shielding and easy scalability to multi-tons scale. The impressive reduction of the 39Ar isotope (compared to the atmospheric argon), along with the excellent pulse shape discrimination, make this technology a possible candidate for the forthcoming generation of multi-ton Dark Matter experiments.

Measuring the dependence of the decay curve on the electron energy deposit in NaI(Tl)

NASA Astrophysics Data System (ADS)

Choong, W.-S.; Bizarri, G.; Cherepy, N. J.; Hull, G.; Moses, W. W.; Payne, S. A.

2011-08-01

We report on the first measurement of the decay times of NaI(Tl) as a function of the deposited electron energy. It has been suggested that the decay curve depends on the ionization density, which is correlated with the electron energy deposit in the scintillator. The ionization creates excitation states, which can decay radiatively and non-radiatively through a number of competing processes. As a result, the rate at which the excitation decays depends on the ionization density. A measurement of the decay curve as a function of the ionization density will allow us to probe the kinetic rates of the competing processes. The Scintillator Light Yield Non-proportionality Characterization Instrument (SLYNCI) measures the electron response of scintillators utilizing fast sampling ADCs to digitize the raw signals from the detectors, and so can provide a measurement of the light pulse shape from the scintillator. Using data collected with the SLYNCI instrument, the intrinsic scintillation profile is extracted on an event-by-event basis by deconvolving the raw signal with the impulse response of the system. Scintillation profiles with the same electron energy deposit are summed to obtain decay curves as a function of the deposited electron energy. The decay time constants are obtained by fitting the decay curves with a two-component exponential decay. While a slight dependence of the decay time constants on the electron energy deposit is observed, the results are not statistically significant.

Theoretical and experimental investigations of coincidences in Poisson distributed pulse trains and spectral distortion caused by pulse pileup

NASA Astrophysics Data System (ADS)

Bristow, Quentin

1990-03-01

The occurrence rates of pulse strings, or sequences of pulses with interarrival times less than the resolving time of the pulse-height analysis system used to acquire spectra, are derived from theoretical considerations. Logic circuits were devised to make experimental measurements of multiple pulse string occurrence rates in the output from a scintillation detector over a wide range of count rates. Markov process theory was used to predict state transition rates in the logic circuits, enabling the experimental data to be checked rigorously for conformity with those predicted for a Poisson distribution. No fundamental discrepancies were observed. Monte Carlo simulations, incorporating criteria for pulse pileup inherent in the operation of modern analog to digital converters, were used to generate pileup spectra due to coincidences between two pulses (first order pileup) and three pulses (second order pileup) for different semi-Gaussian pulse shapes. Coincidences between pulses in a single channel produced a basic probability density function spectrum. The use of a flat spectrum showed the first order pileup distorted the spectrum to a linear ramp with a pileup tail. A correction algorithm was successfully applied to correct entire spectra (simulated and real) for first and second order pileups.

Photon-induced positron annihilation lifetime spectroscopy using ultrashort laser-Compton-scattered gamma-ray pulses

NASA Astrophysics Data System (ADS)

Taira, Y.; Toyokawa, H.; Kuroda, R.; Yamamoto, N.; Adachi, M.; Tanaka, S.; Katoh, M.

2013-05-01

High-energy ultrashort gamma-ray pulses can be generated via laser Compton scattering with 90° collisions at the UVSOR-II electron storage ring. As an applied study of ultrashort gamma-ray pulses, a new photon-induced positron annihilation lifetime spectroscopy approach has been developed. Ultrashort gamma-ray pulses with a maximum energy of 6.6 MeV and pulse width of 2.2 ps created positrons throughout bulk lead via pair production. Annihilation gamma rays were detected by a BaF2 scintillator mounted on a photomultiplier tube. A positron lifetime spectrum was obtained by measuring the time difference between the RF frequency of the electron storage ring and the detection time of the annihilation gamma rays. We calculated the response of the BaF2 scintillator and the time jitter caused by the variation in the total path length of the ultrashort gamma-ray pulses, annihilation gamma rays, and scintillation light using a Monte Carlo simulation code. The positron lifetime for bulk lead was successfully measured.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Brubaker, Erik; Dibble, Dean C.; Mengesha, Wondwosen

An ideal 3He detector replacement for the near- to medium-term future will use materials that are easy to produce and well understood, while maintaining thermal neutron detection efficiency and gamma rejection close to the 3He standard. Toward this end, we investigated the use of standard alkali halide scintillators interfaced with 6Li and read out with photomultiplier tubes (PMTs). Thermal neutrons are captured on 6Li with high efficiency, emitting high-energy and triton ( 3H) reaction products. These particles deposit energy in the scintillator, providing a thermal neutron signal; discrimination against gamma interactions is possible via pulse shape discrimination (PSD), since heavymore » particles produce faster pulses in alkali halide crystals. We constructed and tested two classes of detectors based on this concept. In one case 6Li is used as a dopant in polycrystalline NaI; in the other case a thin Li foil is used as a conversion layer. In the configurations studied here, these systems are sensitive to both gamma and neutron radiation, with discrimination between the two and good energy resolution for gamma spectroscopy. We present results from our investigations, including measurements of the neutron efficiency and gamma rejection for the two detector types. We also show a comparison with Cs 2LiYCl 6:Ce (CLYC), which is emerging as the standard scintillator for simultaneous gamma and thermal neutron detection, and also allows PSD. We conclude that 6Li foil with CsI scintillating crystals has near-term promise as a thermal neutron detector in applications previously dominated by 3He detectors. The other approach, 6Li-doped alkali halides, has some potential, but require more work to understand material properties and improve fabrication processes.« less

Development of a thin scintillation films fission-fragment detector and a novel neutron source

DOE PAGES

Rusev, Gencho Yordanov; Jandel, Marian; Baramsai, Bayarbadrakh; ...

2015-08-26

Here, investigation of prompt fission and neutron-capture Υ rays from fissile actinide samples at the Detector for Advanced Neutron Capture Experiments (DANCE) requires use of a fission-fragment detector to provide a trigger or a veto signal. A fission-fragment detector based on thin scintillating films and silicon photomultipliers has been built to serve as a trigger/veto detector in neutron-induced fission measurements at DANCE. The fissile material is surrounded by scintillating films providing a 4π detection of the fission fragments. The scintillations were registered with silicon photomultipliers. A measurement of the 235U(n,f) reaction with this detector at DANCE revealed a correct time-of-flightmore » spectrum and provided an estimate for the efficiency of the prototype detector of 11.6(7)%. Design and test measurements with the detector are described. A neutron source with fast timing has been built to help with detector-response measurements. The source is based on the neutron emission from the spontaneous fission of 252Cf and the same type of scintillating films and silicon photomultipliers. Overall time resolution of the source is 0.3 ns. Design of the source and test measurements with it are described. An example application of the source for determining the neutron/gamma pulse-shape discrimination by a stilbene crystal is given.« less

1987 Nuclear Science Symposium, 34th, and 1987 Symposium on Nuclear Power Systems, 19th, San Francisco, CA, Oct. 21-23, 1987, Proceedings

NASA Astrophysics Data System (ADS)

Armantrout, Guy A.

1988-02-01

The present conference consideres topics in radiation detectors, advanced electronic circuits, data acquisition systems, radiation detector systems, high-energy and nuclear physics radiation detection, spaceborne instrumentation, health physics and environmental radiation detection, nuclear medicine, nuclear well logging, and nuclear reactor instrumentation. Attention is given to the response of scintillators to heavy ions, phonon-mediated particle detection, ballistic deficits in pulse-shaping amplifiers, fast analog ICs for particle physics, logic cell arrays, the CERN host interface, high performance data buses, a novel scintillating glass for high-energy physics applications, background events in microchannel plates, a tritium accelerator mass spectrometer, a novel positron tomograph, advancements in PET, cylindrical positron tomography, nuclear techniques in subsurface geology, REE borehole neutron activation, and a continuous tritium monitor for aqueous process streams.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Budden, B. S.; Stonehill, L. C.; Warniment, A.

In this study, a new class of elpasolite scintillators has garnered recent attention due to the ability to perform as simultaneous gamma spectrometers and thermal neutron detectors. Such a dual-mode capability is made possible by pulse-shape discrimination (PSD), whereby the emission waveform profiles of gamma and neutron events are fundamentally unique. To take full advantage of these materials, we have developed the Compact Advanced Readout Electronics for Elpasolites (CAREE). This handheld instrument employs a multi-channel PSD-capable ASIC, custom micro-processor board, front-end electronics, power supplies, and a 2 in. photomultiplier tube for readout of the scintillator. The unit is highly configurablemore » to allow for performance optimization amongst a wide sample of elpasolites which provide PSD in fundamentally different ways. We herein provide an introduction to elpasolites, then describe the motivation for the work, mechanical and electronic design, and preliminary performance results.« less

Response of Cs 2LiYCl 6:Ce (CLYC) to High Energy Protons

DOE Office of Scientific and Technical Information (OSTI.GOV)

Coupland, Daniel David Schechtman; Stonehill, Laura Catherine; Goett III, John Jerome

2015-11-23

Cs 2LiYCl 6:Ce (CLYC) is a promising new inorganic scintillator for gamma and neutron detection. As a gamma-ray detector, it exhibits bright light output and better resolution and proportionality of response than traditional gamma-ray scintillators such as NaI. It is also highly sensitive to thermal neutrons through capture on 6Li, and recent experiments have demonstrated sensitivity to fast neutrons through interactions with 35Cl. The response of CLYC to other forms of radiation has not been reported. We have performed the first measurements of the response of CLYC to several-hundred MeV protons. We have collected digitized waveforms from proton events, andmore » compare to those produced by gammas and thermal neutrons. Finally, we discuss the potential for pulse shape discrimination between them.« less

High fluence neutron radiation of plastic scintillators for the TileCal of the ATLAS detector.

NASA Astrophysics Data System (ADS)

Mdhluli, J. E.; Davydov, Yu I.; Baranov, V.; Mthembu, S.; Erasmus, R.; Jivan, H.; Khanye, N.; Tlou, H.; Tjale, B.; Starchenko, J.; Solovyanov, O.; Mellado, B.; Sideras-Haddad, E.

2017-09-01

We report on structural and optical properties of neutron irradiated plastic scintillators. These scintillators were subjected to a neutron beam with wide energy range of up to 10MeV and a neutron flux range of 1.2 × 1012 - 9.4 × 1012 n/cm 2 using the IBR-2 pulsed reactor at the Joint Institute for Nuclear Research in Dubna. A study between polyvinyl toluene based commercial scintillators EJ200, EJ208 and EJ260 as well as polystyrene based scintillator from Kharkov is conducted. Light transmission, Raman spectroscopy, fluorescence spectroscopy and light yield testing was performed to characterize the damage induced in the samples. Preliminary results from the tests performed indicate no change in the optical and structural properties of the scintillators. The polystyrene based scintillators were further subjected to a higher neutron flux range of 3.8 × 1012 - 1.8 × 1014 n/cm 2 using the IBR-2 pulsed reactor.

Organic Scintillator for Real-Time Neutron Dosimetry

DOE PAGES

Beyer, Kyle A.; Di Fulvio, Angela; Stolarczyk, Liliana; ...

2017-11-15

We have developed a radiation detector based on an organic scintillator for spectrometry and dosimetry of out-of-field secondary neutrons from clinical proton beams. The detector consists of an EJ-299-34 crystalline organic scintillator, coupled by fiber optic cable to a silicon photomultiplier (SiPM). Proof of concept measurements were taken with 137Cs and 252Cf, and corresponding simulations were performed in MCNPX-PoliMi. Despite its small size, the detector is able to discriminate between neutron and gamma-rays via pulse shape discrimination. We simulated the response function of the detector to monoenergetic neutrons in the 100 keV–0 MeV range using MCNPX-PoliMi. The measured unfolded 252Cfmore » neutron spectrum is in good agreement with the theoretical Watt fission spectrum. We determined the ambient dose equivalent by folding the spectrum with the fluence-to-ambient dose conversion coefficient, with a 1.4% deviation from theory. Some preliminary proton beam experiments were preformed at the Bronowice Cyclotron Center patient treatment facility using a clinically relevant proton pencil beam for brain tumor and craino-spinal treatment directed at a child phantom.« less

Science-Driven Candidate Search for New Scintillator Materials: FY 2014 Annual Report

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kerisit, Sebastien N.; Gao, Fei; Xie, YuLong

2014-10-01

This annual reports presents work carried out during Fiscal Year (FY) 2014 at Pacific Northwest National Laboratory (PNNL) under the project entitled “Science-Driven Candidate Search for New Scintillator Materials” (Project number: PL13-SciDriScintMat-PD05) and led by Drs. Fei Gao and Sebastien N. Kerisit. This project is divided into three tasks: 1) Ab initio calculations of electronic properties, electronic response functions and secondary particle spectra; 2) Intrinsic response properties, theoretical light yield, and microscopic description of ionization tracks; and 3) Kinetics and efficiency of scintillation: nonproportionality, intrinsic energy resolution, and pulse shape discrimination. Detailed information on the results obtained in each ofmore » the three tasks is provided in this Annual Report. Furthermore, peer-reviewed articles published this FY or currently under review and presentations given this FY are included in Appendix. This work was supported by the National Nuclear Security Administration, Office of Nuclear Nonproliferation Research and Development (DNN R&D/NA-22), of the U.S. Department of Energy (DOE).« less

Temperature behavior of CLYC/MPPC detectors

NASA Astrophysics Data System (ADS)

Glodo, Jarek; McClish, Mickel; Hawrami, Rastgo; O'Dougherty, Patrick; Tower, Josh; Gueorguiev, Andrey; Shah, Kanai S.

2013-09-01

He-3 tubes are the most popular thermal neutron detectors. They are easy to use, have good sensitivity for neutron detection, and are insensitive to gamma radiation. Due to low stockpiles of the He-3 gas, alternatives are being sought to replace these devices in many applications. One of the possible alternatives to these devices are scintillators incorporating isotopes with high cross-section for neutron capture (e.g. Li-6 or B-10). Cs2LiYCl6:Ce (CLYC) is one of the scintillators that recently has been considered for neutron detection. This material offers good detection efficiency (~80%), bright response (70,000 photons/neutron), high gamma ray equivalent energy of the neutron signal (>3MeV), and excellent separation between gamma and neutron radiation with pulse shape discrimination. A He-3 tube alternative based on a CLYC scintillator was constructed using a silicon photomultiplier (SiPM) for the optical readout. SiPMs are very compact optical detectors that are an alternative to usually bulky photomultiplier tubes. Constructed detector was characterized for its behavior across a temperature range of -20°C to 50°C.

Bis(pinacolato)diboron as an additive for the detection of thermal neutrons in plastic scintillators

NASA Astrophysics Data System (ADS)

Mahl, Adam; Yemam, Henok A.; Stuntz, John; Remedes, Tyler; Sellinger, Alan; Greife, Uwe

2016-04-01

A readily available and inexpensive boron compound was tested as an additive for the detection of thermal neutrons in plastic scintillators. Bis(pinacolato)diboron (B2Pin2) was determined to be a compatible boron source (8.51 wt% boron, 1.70 wt% 10B) in poly(vinyltoluene) based matrices. Plastic scintillator blends of 1-20 wt% 2,5-diphenyloxazole (PPO), 0.1 wt% 1,4-bis(5-phenyloxazol-2-yl) benzene (POPOP) and 1-15 wt% B2Pin2 were prepared that provided optical clarity, good mechanical properties, and the capability of thermal neutron detection. Independent of B2Pin2 concentration, strong 10B neutron capture signals around 90 keVee were observed at essentially constant light output. Increasing PPO concentration allowed for the use of pulse shape discrimination (PSD) in both fast and thermal neutron detection. High PPO concentrations appear to cause additional alpha quenching that affected the 10B neutron capture signal. Aging effects after storage in air for several months were observed, which led to degradation of performance and in some samples of mechanical stability.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Danevich, F. A., E-mail: danevich@kinr.kiev.ua; Boiko, R. S.; Chernyak, D. M.

The LUMTNEU program aims at performing a pilot experiment on 0ν2β decay of {sup 100}Mo using radiopure ZnMoO{sub 4} crystals enriched in {sup 100}Mo operated as cryogenic scintillating bolometers. Large volume ZnMoO{sub 4} crystal scintillators (∼ 0.3 kg) were developed and tested showing high performance in terms of radiopurity, energy resolution and α/β particle discrimination capability. Zinc molybdate crystal scintillators enriched in {sup 100}Mo were grown for the first time by the low-thermal-gradient Czochralski technique with a high crystal yield and an acceptable level of enriched molybdenum irrecoverable losses. A background level of ∼ 0.5 counts/(yr keV ton) in the regionmore » of interest can be reached in a large detector array thanks to the excellent detectors radiopurity and particle discrimination capability, suppression of randomly coinciding events by pulse-shape analysis, and anticoincidence cut. These results pave the way to future sensitive searches based on the LUMTNEU technology, capable of approachingand exploring the inverted hierarchy region of the neutrino mass pattern.« less

Organic Scintillator for Real-Time Neutron Dosimetry

DOE Office of Scientific and Technical Information (OSTI.GOV)

Beyer, Kyle A.; Di Fulvio, Angela; Stolarczyk, Liliana

We have developed a radiation detector based on an organic scintillator for spectrometry and dosimetry of out-of-field secondary neutrons from clinical proton beams. The detector consists of an EJ-299-34 crystalline organic scintillator, coupled by fiber optic cable to a silicon photomultiplier (SiPM). Proof of concept measurements were taken with 137Cs and 252Cf, and corresponding simulations were performed in MCNPX-PoliMi. Despite its small size, the detector is able to discriminate between neutron and gamma-rays via pulse shape discrimination. We simulated the response function of the detector to monoenergetic neutrons in the 100 keV–0 MeV range using MCNPX-PoliMi. The measured unfolded 252Cfmore » neutron spectrum is in good agreement with the theoretical Watt fission spectrum. We determined the ambient dose equivalent by folding the spectrum with the fluence-to-ambient dose conversion coefficient, with a 1.4% deviation from theory. Some preliminary proton beam experiments were preformed at the Bronowice Cyclotron Center patient treatment facility using a clinically relevant proton pencil beam for brain tumor and craino-spinal treatment directed at a child phantom.« less

Investigating the anisotropic scintillation response in anthracene through neutron, gamma-ray, and muon measurements

DOE PAGES

Schuster, Patricia; Brubaker, Erik

2016-05-05

Our paper reports a series of measurements that characterize the directional dependence of the scintillation response of crystalline anthracene to incident DT neutrons, DD neutrons, 137Cs gamma rays, and, for the first time, cosmic ray muons. Moreover, the neutron measurements give the amplitude and pulse shape dependence on the proton recoil direction over one hemisphere of the crystal, confirming and extending previous results in the literature. In similar measurements using incident gamma rays, no directional effect is evident, and any anisotropy with respect to the electron recoil direction is constrained to have a magnitude of less than a tenth ofmore » that present in the proton recoil events. Cosmic muons are measured at two directions, and no anisotropy is observed. Our set of observations indicates that high dE/dx is necessary for an anisotropy to be present for a given type of scintillation event, which in turn could be used to discriminate among different hypotheses for the underlying causes of the anisotropy, which are not well understood.« less

Development of a homogeneous pulse shape discriminating flow-cell radiation detection system

NASA Astrophysics Data System (ADS)

Hastie, K. H.; DeVol, T. A.; Fjeld, R. A.

1999-02-01

A homogeneous flow-cell radiation detection system which utilizes coincidence counting and pulse shape discrimination circuitry was assembled and tested with five commercially available liquid scintillation cocktails. Two of the cocktails, Ultima Flo (Packard) and Mono Flow 5 (National Diagnostics) have low viscosities and are intended for flow applications; and three of the cocktails, Optiphase HiSafe 3 (Wallac), Ultima Gold AB (Packard), and Ready Safe (Beckman), have higher viscosities and are intended for static applications. The low viscosity cocktails were modified with 1-methylnaphthalene to increase their capability for alpha/beta pulse shape discrimination. The sample loading and pulse shape discriminator setting were optimized to give the lowest minimum detectable concentration for alpha radiation in a 30 s count time. Of the higher viscosity cocktails, Optiphase HiSafe 3 had the lowest minimum detectable activities for alpha and beta radiation, 0.2 and 0.4 Bq/ml for 233U and 90Sr/ 90Y, respectively, for a 30 s count time. The sample loading was 70% and the corresponding alpha/beta spillover was 5.5%. Of the low viscosity cocktails, Mono Flow 5 modified with 2.5% (by volume) 1-methylnaphthalene resulted in the lowest minimum detectable activities for alpha and beta radiation; 0.3 and 0.5 Bq/ml for 233U and 90Sr/ 90Y, respectively, for a 30 s count time. The sample loading was 50%, and the corresponding alpha/beta spillover was 16.6%. HiSafe 3 at a 10% sample loading was used to evaluate the system under simulated flow conditions.

New Opportunities in Decay Spectroscopy with the GRIFFIN and DESCANT Arrays

NASA Astrophysics Data System (ADS)

Bildstein, V.; Andreoiu, C.; Ball, G. C.; Ballast, T.; Bartlett, C.; Bender, P. C.; Bernier, N.; Bianco, L.; Bishop, D.; Brennan, D.; Bruhn, T.; Cheeseman, A.; Churchman, R.; Ciccone, S.; Davids, B.; Demand, G.; Dillmann, I.; Garnsworthy, A. B.; Garrett, P. E.; Georges, S.; Hackman, G.; Hadinia, B.; Kokke, R.; Krücken, R.; Linn, Y.; Lim, C.; Martin, J.-P.; Miller, D.; Mills, W. J.; Morrison, L. N.; Ohlmann, C. A.; Park, J.; Pearson, C. J.; Pore, J. L.; Rajabali, M. M.; Rand, E. T.; Rizwan, U.; Sarazin, F.; Shaw, B.; Starosta, K.; Svensson, C. E.; Sumithrarachchi, C.; Unsworth, C.; Voss, P.; Wang, Z. M.; Williams, J.; Wong, J.; Wong, S.

The GRIFFIN (Gamma-Ray Infrastructure For Fundamental Investigations of Nuclei) project is a major upgrade of the decay spectroscopy capabilities at TRIUMF-ISAC. GRIFFIN will replace the 8π spectrometer with an array of up to 16 large-volume HPGe clover detectors and use a state-of-the-art digital data acquisition system. The existing ancillary detector systems that had been developed for 8π, such as the SCEPTAR array for β-tagging, PACES for high-resolution internal conversion electron spectroscopy, and the DANTE array of LaBr3/BaF2 scintillators for fast γ-ray timing, will be used with GRIFFIN. GRIFFIN can also accommodate the new neutron detector array DESCANT (Deuterated Scintillator Array for Neutron Tagging), enabling the study of β-delayed neutron emitters. DESCANT consists of up to 70 detectors, each filled with approximately 2 liters of deuterated benzene, a liquid scintillator that provides pulse-shape discrimination (PSD) capabilities to distinguish between neutrons and γ-rays interacting with the detector. In addition, the anisotropic nature of n-d scattering as compared to the isotropic n-p scattering allows for the determination of the neutron energy spectrum directly from the pulse-height spectrum, complementing the time-of-flight (TOF) information. The installation of GRIFFIN is under way and first experiments are planned for the fall of 2014. The array will be completed in 2015 with the full complement of 16 clovers. DESCANT will be tested coupled with GRIFFIN in spring of 2015.

NeuRad detector prototype pulse shape study

NASA Astrophysics Data System (ADS)

Muzalevsky, I.; Chudoba, V.; Belogurov, S.; Kiselev, O.; Bezbakh, A.; Fomichev, A.; Krupko, S.; Slepnev, R.; Kostyleva, D.; Gorshkov, A.; Ovcharenko, E.; Schetinin, V.

2018-04-01

The EXPERT setup located at the Super-FRS facility, the part of the FAIR complex in Darmstadt, Germany, is intended for investigation of properties of light exotic nuclei. One of its modules, the high granularity neutron detector NeuRad assembled from a large number of the scintillating fiber is intended for registration of neutrons emitted by investigated nuclei in low-energy decays. Feasibility of the detector strongly depends on its timing properties defined by the spatial distribution of ionization, light propagation inside the fibers, light emission kinetics and transition time jitter in the multi-anode photomultiplier tube. The first attempt of understanding the pulse formation in the prototype of the NeuRad detector by comparing experimental results and Monte Carlo (MC) simulations is reported in this paper.

A Hand-Held, Intra-Operative Positron Imaging Probe for Surgical Applications

NASA Astrophysics Data System (ADS)

Sabet, Hamid; Stack, Brendan C.; Nagarkar, Vivek V.

2015-10-01

We have developed a prototype intra-operative β+ imaging probe to help tumor removal and malignant tissue resection. The probe can be used during surgery to provide clear delineation of malignant tissues. Our probe consists of a hybrid scintillator coupled to a silicon photomultiplier (SiPM) array with associated front-end electronics encapsulated in an ergonomic aluminum housing. Pulse shape discrimination electronics has been implemented and integrated into the downstream data acquisition system. The field of view of the probe is 10 ×10 mm2 realized by a 0.4 mm thick CsI:Tl scintillator coupled to a 1 mm thick LYSO. While CsI:Tl layer acts as β+ sensitive detector, LYSO detects gamma radiation where the gamma response can be subtracted from the total signal to improve SNR and contrast. The thickness of the LYSO scintillator is optimized such that it acts as light diffuser to spread the scintillation light generated in CsI:Tl over multiple SiPM pixels for accurate estimation of the β+ interaction location. The probe shows FWHM spatial resolution in the presence of large background radiation. The probe was used to study rabbits with tongue tumors. The experimental results show that the probe can successfully locate the tongue tumors in its active imaging area.

Radionuclide detection devices and associated methods

DOEpatents

Mann, Nicholas R [Rigby, ID; Lister, Tedd E [Idaho Falls, ID; Tranter, Troy J [Idaho Falls, ID

2011-03-08

Radionuclide detection devices comprise a fluid cell comprising a flow channel for a fluid stream. A radionuclide collector is positioned within the flow channel and configured to concentrate one or more radionuclides from the fluid stream onto at least a portion of the radionuclide collector. A scintillator for generating scintillation pulses responsive to an occurrence of a decay event is positioned proximate at least a portion of the radionuclide collector and adjacent to a detection system for detecting the scintillation pulses. Methods of selectively detecting a radionuclide are also provided.

Simultaneous determination of radionuclides separable into natural decay series by use of time-interval analysis.

PubMed

Hashimoto, Tetsuo; Sanada, Yukihisa; Uezu, Yasuhiro

2004-05-01

A delayed coincidence method, time-interval analysis (TIA), has been applied to successive alpha- alpha decay events on the millisecond time-scale. Such decay events are part of the (220)Rn-->(216)Po ( T(1/2) 145 ms) (Th-series) and (219)Rn-->(215)Po ( T(1/2) 1.78 ms) (Ac-series). By using TIA in addition to measurement of (226)Ra (U-series) from alpha-spectrometry by liquid scintillation counting (LSC), two natural decay series could be identified and separated. The TIA detection efficiency was improved by using the pulse-shape discrimination technique (PSD) to reject beta-pulses, by solvent extraction of Ra combined with simple chemical separation, and by purging the scintillation solution with dry N(2) gas. The U- and Th-series together with the Ac-series were determined, respectively, from alpha spectra and TIA carried out immediately after Ra-extraction. Using the (221)Fr-->(217)At ( T(1/2) 32.3 ms) decay process as a tracer, overall yields were estimated from application of TIA to the (225)Ra (Np-decay series) at the time of maximum growth. The present method has proven useful for simultaneous determination of three radioactive decay series in environmental samples.

Update on the MiniCLEAN dark matter experiment

DOE PAGES

Rielage, K.; Akashi-Ronquest, M.; Bodmer, M.; ...

2015-03-24

The direct search for dark matter is entering a period of increased sensitivity to the hypothetical Weakly Interacting Massive Particle (WIMP). One such technology that is being examined is a scintillation only noble liquid experiment, MiniCLEAN. MiniCLEAN utilizes over 500 kg of liquid cryogen to detect nuclear recoils from WIMP dark matter and serves as a demonstration for a future detector of order 50 to 100 tonnes. The liquid cryogen is interchangeable between argon and neon to study the A² dependence of the potential signal and examine backgrounds. MiniCLEAN utilizes a unique modular design with spherical geometry to maximize themore » light yield using cold photomultiplier tubes in a single-phase detector. Pulse shape discrimination techniques are used to separate nuclear recoil signals from electron recoil backgrounds. MiniCLEAN will be spiked with additional ³⁹Ar to demonstrate the effective reach of the pulse shape discrimination capability. Assembly of the experiment is underway at SNOLAB and an update on the project is given.« less

CHELSI: a portable neutron spectrometer for the 20-800 MeV region.

PubMed

McLean, T D; Olsher, R H; Romero, L L; Miles, L H; Devine, R T; Fallu-Labruyere, A; Grudberg, P

2007-01-01

CHELSI is a CsI-based portable spectrometer being developed at Los Alamos National Laboratory for use in high-energy neutron fields. Based on the inherent pulse shape discrimination properties of CsI(Tl), the instrument flags charged particle events produced via neutron-induced spallation events. Scintillation events are processed in real time using digital signal processing and a conservative estimate of neutron dose rate is made based on the charged particle energy distribution. A more accurate dose estimate can be made by unfolding the 2D charged particle versus pulse height distribution to reveal the incident neutron spectrum from which dose is readily obtained. A prototype probe has been assembled and data collected in quasi-monoenergetic fields at The Svedberg Laboratory (TSL) in Uppsala as well as at the Los Alamos Neutron Science Center (LANSCE). Preliminary efforts at deconvoluting the shape/energy data using empirical response functions derived from time-of-flight measurements are described.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Rielage, K.; Akashi-Ronquest, M.; Bodmer, M.

The direct search for dark matter is entering a period of increased sensitivity to the hypothetical Weakly Interacting Massive Particle (WIMP). One such technology that is being examined is a scintillation only noble liquid experiment, MiniCLEAN. MiniCLEAN utilizes over 500 kg of liquid cryogen to detect nuclear recoils from WIMP dark matter and serves as a demonstration for a future detector of order 50 to 100 tonnes. The liquid cryogen is interchangeable between argon and neon to study the A² dependence of the potential signal and examine backgrounds. MiniCLEAN utilizes a unique modular design with spherical geometry to maximize themore » light yield using cold photomultiplier tubes in a single-phase detector. Pulse shape discrimination techniques are used to separate nuclear recoil signals from electron recoil backgrounds. MiniCLEAN will be spiked with additional ³⁹Ar to demonstrate the effective reach of the pulse shape discrimination capability. Assembly of the experiment is underway at SNOLAB and an update on the project is given.« less

Time-over-threshold for pulse shape discrimination in a time-of-flight phoswich PET detector

PubMed Central

Chang, Chen-Ming; Cates, Joshua W.; Levin, Craig S.

2016-01-01

It is well known that a PET detector capable of measuring both photon time-of-flight (TOF) and depth-of-interaction (DOI) improves the image quality and accuracy. Phoswich designs have been realized in PET detectors to measure DOI for more than a decade. However, PET detectors based on phoswich designs put great demand on the readout circuits, which have to differentiate the pulse shape produced by different crystal layers. A simple pulse shape discrimination approach is required to realize the phoswich designs in a clinical PET scanner, which consists of thousands of scintillation crystal elements. In this work, we studied time-over-threshold (ToT) as a pulse shape parameter for DOI. The energy, timing and DOI performance were evaluated for a phoswich detector design comprising 3 mm × 3 mm × 10 mm LYSO:Ce crystal optically coupled to 3 mm × 3 mm × 10 mm calcium co-doped LSO:Ce,Ca(0.4%) crystal read out by a silicon photomultiplier (SiPM). A DOI accuracy of 97.2% has been achieved for photopeak events using the proposed time-over-threshold (ToT) processing. The energy resolution without correction for SiPM non-linearity was 9.7 ± 0.2% and 11.3 ± 0.2% FWHM at 511 keV for LYSO and LSO crystal layers, respectively. The coincidence time resolution for photopeak events ranges from 164.6 ps to 183.1 ps FWHM, depending on the layer combinations. The coincidence time resolution for inter-crystal scatter events ranges from 214.6 ps to 418.3 ps FWHM, depending on the energy windows applied. These results show great promises of using ToT for pulse shape discrimination in a TOF phoswich detector since a ToT measurement can be easily implemented in readout electronics. PMID:27991437

Electronics for the STEREO experiment

NASA Astrophysics Data System (ADS)

HÉLAINE, Victor; STEREO Collaboration

2017-09-01

The STEREO experiment, aiming to probe short baseline neutrino oscillations by precisely measuring reactor anti-neutrino spectrum, is currently under installation. It is located at short distance from the compact research reactor core of the Institut Laue-Langevin, Grenoble, France. Dedicated electronics, hosted in a single µTCA crate, were designed for this experiment. In this article, the electronics requirements, architecture and the performances achieved are described. It is shown how intrinsic Pulse Shape Discrimination properties of the liquid scintillator are preserved and how custom adaptable logic is used to improve the muon veto efficiency.

Standardization of 237Np by the CIEMAT/NIST LSC tracer method

PubMed

Gunther

2000-03-01

The standardization of 237Np presents some difficulties: several groups of alpha, beta and gamma radiation, chemical problems with the daughter nuclide 233Pa, an incomplete radioactive equilibrium after sample preparation, high conversion of some gamma transitions. To solve the chemical problems, a sample composition involving the Ultima Gold AB scintillator and a high concentration of HCl is used. Standardization by the CIEMAT/NIST method and by pulse shape discrimination is described. The results agree within 0.1% with those obtained by two other methods.

A prototype of a portable TDCR system at ENEA.

PubMed

Capogni, Marco; De Felice, Pierino

2014-11-01

A prototype of a portable liquid scintillation counting system based on the Triple-to-Double Coincidence Ratio (TDCR) technique was developed at ENEA-INMRI in the framework of the European Metrofission project. The new device equipped with the CAEN digitizers was tested for the activity measurements of pure β-emitters ((99)Tc and (63)Ni). The list-mode data recorded by the digitizers were analyzed by software implemented in the CERN ROOT environment, which allows the application of pulse shape discrimination using the new device. Copyright © 2014 Elsevier Ltd. All rights reserved.

The evaluation of uncertainty in low-level LSC measurements of water samples.

PubMed

Rusconi, R; Forte, M; Caresana, M; Bellinzona, S; Cazzaniga, M T; Sgorbati, G

2006-01-01

The uncertainty in measurements of gross alpha and beta activities in water samples by liquid scintillation counting with alpha/beta discrimination has been evaluated considering the problems typical of low-level measurements of environmental samples. The use of a pulse shape analysis device to discriminate alpha and beta events introduces a correlation between some of the input quantities, and it has to be considered. Main contributors to total uncertainty have been assessed by specifically designed experimental tests. Results have been fully examined and discussed.

Neutron emission in 19F-induced reactions

NASA Astrophysics Data System (ADS)

Acharya, Jaimin; Mukherjee, S.; Chatterjee, A.; Singh, N. L.; Ramachandran, K.; Rout, P. C.; Mahata, K.; Desai, Vishal; Mirgule, E. T.; Suryanarayana, S. V.; Nayak, B. K.; Saxena, A.; Steyn, G. F.

2018-03-01

We measured neutron emission spectra for 19F-induced reactions on 181Ta, 89Y, and 51V at beam energies of 130, 140, 145, and 150 MeV. Measurements were made using liquid scintillator detectors at eight angles in the range of 25∘-143∘ using time-of-flight and pulse-shape discrimination. A comparison has been made with alice2014 and pace4 calculations to understand the role of incomplete fusion and pre-equilibrium effects. Global predictions with alice2014 without parameter adjustment gives a fair agreement with the measured data.

A Monte Carlo simulation study for the gamma-ray/neutron dual-particle imager using rotational modulation collimator (RMC).

PubMed

Kim, Hyun Suk; Choi, Hong Yeop; Lee, Gyemin; Ye, Sung-Joon; Smith, Martin B; Kim, Geehyun

2018-03-01

The aim of this work is to develop a gamma-ray/neutron dual-particle imager, based on rotational modulation collimators (RMCs) and pulse shape discrimination (PSD)-capable scintillators, for possible applications for radioactivity monitoring as well as nuclear security and safeguards. A Monte Carlo simulation study was performed to design an RMC system for the dual-particle imaging, and modulation patterns were obtained for gamma-ray and neutron sources in various configurations. We applied an image reconstruction algorithm utilizing the maximum-likelihood expectation-maximization method based on the analytical modeling of source-detector configurations, to the Monte Carlo simulation results. Both gamma-ray and neutron source distributions were reconstructed and evaluated in terms of signal-to-noise ratio, showing the viability of developing an RMC-based gamma-ray/neutron dual-particle imager using PSD-capable scintillators.

Fast neutron detection with a segmented spectrometer

NASA Astrophysics Data System (ADS)

Langford, T. J.; Bass, C. D.; Beise, E. J.; Breuer, H.; Erwin, D. K.; Heimbach, C. R.; Nico, J. S.

2015-01-01

A fast neutron spectrometer consisting of segmented plastic scintillator and 3He proportional counters was constructed for the measurement of neutrons in the energy range 1-200 MeV. We discuss its design, principles of operation, and the method of analysis. The detector is capable of observing very low neutron fluxes in the presence of ambient gamma background and does not require scintillator pulse-shape discrimination. The spectrometer was characterized for its energy response in fast neutron fields of 2.5 MeV and 14 MeV, and the results are compared with Monte Carlo simulations. Measurements of the fast neutron flux and energy response at 120 m above sea-level (39.130°N, 77.218°W) and at a depth of 560 m in a limestone mine are presented. Finally, the design of a spectrometer with improved sensitivity and energy resolution is discussed.

Time encoded radiation imaging

DOEpatents

Marleau, Peter; Brubaker, Erik; Kiff, Scott

2014-10-21

The various technologies presented herein relate to detecting nuclear material at a large stand-off distance. An imaging system is presented which can detect nuclear material by utilizing time encoded imaging relating to maximum and minimum radiation particle counts rates. The imaging system is integrated with a data acquisition system that can utilize variations in photon pulse shape to discriminate between neutron and gamma-ray interactions. Modulation in the detected neutron count rates as a function of the angular orientation of the detector due to attenuation of neighboring detectors is utilized to reconstruct the neutron source distribution over 360 degrees around the imaging system. Neutrons (e.g., fast neutrons) and/or gamma-rays are incident upon scintillation material in the imager, the photons generated by the scintillation material are converted to electrical energy from which the respective neutrons/gamma rays can be determined and, accordingly, a direction to, and the location of, a radiation source identified.

A novel phoswich imaging detector for simultaneous beta and coincidence-gamma imaging of plant leaves.

PubMed

Wu, Heyu; Tai, Yuan-Chuan

2011-09-07

To meet the growing demand for functional imaging technology for use in studying plant biology, we are developing a novel technique that permits simultaneous imaging of escaped positrons and coincidence gammas from annihilation of positrons within an intake leaf. The multi-modality imaging system will include two planar detectors: one is a typical PET detector array and the other is a phoswich imaging detector that detects both beta and gamma. The novel phoswich detector is made of a plastic scintillator, a lutetium oxyorthosilicate (LSO) array, and a position sensitive photomultiplier tube (PS-PMT). The plastic scintillator serves as a beta detector, while the LSO array serves as a gamma detector and light guide that couples scintillation light from the plastic detector to the PMT. In our prototype, the PMT signal was fed into the Siemens QuickSilver electronics to achieve shaping and waveform sampling. Pulse-shape discrimination based on the detectors' decay times (2.1 ns for plastic and 40 ns for LSO) was used to differentiate beta and gamma events using the common PMT signals. Using our prototype phoswich detector, we simultaneously measured a beta image and gamma events (in single mode). The beta image showed a resolution of 1.6 mm full-width-at-half-maximum using F-18 line sources. Because this shows promise for plant-scale imaging, our future plans include development of a fully functional simultaneous beta-and-coincidence-gamma imager with sub-millimeter resolution imaging capability for both modalities.

Scintillation-based Search for Off-pulse Radio Emission from Pulsars

NASA Astrophysics Data System (ADS)

Ravi, Kumar; Deshpande, Avinash A.

2018-05-01

We propose a new method to detect off-pulse (unpulsed and/or continuous) emission from pulsars using the intensity modulations associated with interstellar scintillation. Our technique involves obtaining the dynamic spectra, separately for on-pulse window and off-pulse region, with time and frequency resolutions to properly sample the intensity variations due to diffractive scintillation and then estimating their mutual correlation as a measure of off-pulse emission, if any. We describe and illustrate the essential details of this technique with the help of simulations, as well as real data. We also discuss the advantages of this method over earlier approaches to detect off-pulse emission. In particular, we point out how certain nonidealities inherent to measurement setups could potentially affect estimations in earlier approaches and argue that the present technique is immune to such nonidealities. We verify both of the above situations with relevant simulations. We apply this method to the observation of PSR B0329+54 at frequencies of 730 and 810 MHz made with the Green Bank Telescope and present upper limits for the off-pulse intensity at the two frequencies. We expect this technique to pave the way for extensive investigations of off-pulse emission with the help of existing dynamic spectral data on pulsars and, of course, with more sensitive long-duration data from new observations.

Neutron/Gamma-ray discrimination through measures of fit

DOE Office of Scientific and Technical Information (OSTI.GOV)

Amiri, Moslem; Prenosil, Vaclav; Cvachovec, Frantisek

2015-07-01

Statistical tests and their underlying measures of fit can be utilized to separate neutron/gamma-ray pulses in a mixed radiation field. In this article, first the application of a sample statistical test is explained. Fit measurement-based methods require true pulse shapes to be used as reference for discrimination. This requirement makes practical implementation of these methods difficult; typically another discrimination approach should be employed to capture samples of neutrons and gamma-rays before running the fit-based technique. In this article, we also propose a technique to eliminate this requirement. These approaches are applied to several sets of mixed neutron and gamma-ray pulsesmore » obtained through different digitizers using stilbene scintillator in order to analyze them and measure their discrimination quality. (authors)« less

Light output function and assembly of the time-of-flight enhanced diagnostics neutron spectrometer plastic scintillators for background reduction by double kinematic selection at EAST

DOE Office of Scientific and Technical Information (OSTI.GOV)

Peng, X. Y.; Chen, Z. J.; Zhang, X.

The 2.5 MeV neutron spectrometer TOFED (Time-Of-Flight Enhanced Diagnostics) has been constructed to perform advanced neutron emission spectroscopy diagnosis of deuterium plasmas on EAST. The instrument has a double-ring structure which, in combination with pulse shape digitization, allows for a dual kinematic selection in the time-of-flight/recoil proton energy (tof/E{sub p}) space, thus improving the spectrometer capability to resolve fast ion signatures in the neutron spectrum, in principle up to a factor ≈100. The identification and separation of features from the energetic ions in the neutron spectrum depends on the detailed knowledge of the instrument response function, both in terms ofmore » the light output function of the scintillators and the effect of undesired multiple neutron scatterings in the instrument. This work presents the determination of the light output function of the TOFED plastic scintillator detectors and their geometrical assembly. Results from dedicated experiments with γ-ray sources and quasi-monoenergetic neutron beams are presented. Implications on the instrument capability to perform background suppression based on double kinematic selection are discussed.« less

Detectors for Active Interrogation Applications

NASA Astrophysics Data System (ADS)

Clarke, S. D.; Hamel, M. C.; Bourne, M. M.; Pozzi, S. A.

Active interrogation creates an environment that is particularly challenging from a radiation-detection standpoint: the elevated background levels from the source can mask the desired signatures from the SNM. Neutron based interrogation experiments have shown that nanosecond-level timing is required to discriminate induced-fission neutrons from the scattered source neutrons. Previous experiments using high-energy bremsstrahlung X-rays have demonstrated the ability to induce and detect prompt photofission neutrons from single target materials; however, a real-world application would require spectroscopic capability to discern between photofission neutrons emitted by SNM and neutrons emitted by other reactions in non-SNM. Using digital pulse-shape discrimination, organic liquid scintillators are capable of reliably detecting neutrons in an intense gamma-ray field. Photon misclassification rates as low as 1 in 106 have been achieved, which is approaching the level of gaseous neutron detectors such as 3He without the need for neutron moderation. These scintillators also possess nanosecond-timing resolution, making them candidates for both neutron-and photon-driven active interrogation systems. We have applied an array of liquid and NaI(Tl) scintillators to successfully image 13.7 kg of HEU interrogated by a DT neutron generator; the system was in the direct presence of the accelerator during the experiment.

ORGANIC SCINTILLATOR FOR REAL-TIME NEUTRON DOSIMETRY.

PubMed

Beyer, Kyle A; Di Fulvio, Angela; Stolarczyk, Liliana; Parol, Wiktor; Mojzeszek, Natalia; Kopéc, Renata; Clarke, Shaun D; Pozzi, Sara A

2017-11-15

We developed a radiation detector based on an organic scintillator for spectrometry and dosimetry of out-of-field secondary neutrons from clinical proton beams. The detector consists of an EJ-299-34 crystalline organic scintillator, coupled by fiber optic cable to a silicon photomultiplier (SiPM). Proof of concept measurements were taken with 137Cs and 252Cf, and corresponding simulations were performed in MCNPX-PoliMi. Despite its small size, the detector is able to discriminate between neutron and gamma-rays via pulse shape discrimination. We simulated the response function of the detector to monoenergetic neutrons in the 100 keV-0 MeV range using MCNPX-PoliMi. The measured unfolded 252Cf neutron spectrum is in good agreement with the theoretical Watt fission spectrum. We determined the ambient dose equivalent by folding the spectrum with the fluence-to-ambient dose conversion coefficient, with a 1.4% deviation from theory. Some preliminary proton beam experiments were preformed at the Bronowice Cyclotron Center patient treatment facility using a clinically relevant proton pencil beam for brain tumor and craino-spinal treatment directed at a child phantom. © The Author 2017. Published by Oxford University Press. All rights reserved. For Permissions, please email: journals.permissions@oup.com.

Plastic scintillator detector for pulsed flux measurements

NASA Astrophysics Data System (ADS)

Kadilin, V. V.; Kaplun, A. A.; Taraskin, A. A.

2017-01-01

A neutron detector, providing charged particle detection capability, has been designed. The main purpose of the detector is to measure pulsed fluxes of both charged particles and neutrons during scientific experiments. The detector consists of commonly used neutron-sensitive ZnS(Ag) / 6LiF scintillator screens wrapping a layer of polystyrene based scintillator (BC-454, EJ-254 or equivalent boron loaded plastic). This type of detector design is able to log a spatial distribution of events and may be scaled to any size. Different variations of the design were considered and modelled in specialized toolkits. The article presents a review of the detector design features as well as simulation results.

Development of MCNPX-ESUT computer code for simulation of neutron/gamma pulse height distribution

NASA Astrophysics Data System (ADS)

Abolfazl Hosseini, Seyed; Vosoughi, Naser; Zangian, Mehdi

2015-05-01

In this paper, the development of the MCNPX-ESUT (MCNPX-Energy Engineering of Sharif University of Technology) computer code for simulation of neutron/gamma pulse height distribution is reported. Since liquid organic scintillators like NE-213 are well suited and routinely used for spectrometry in mixed neutron/gamma fields, this type of detectors is selected for simulation in the present study. The proposed algorithm for simulation includes four main steps. The first step is the modeling of the neutron/gamma particle transport and their interactions with the materials in the environment and detector volume. In the second step, the number of scintillation photons due to charged particles such as electrons, alphas, protons and carbon nuclei in the scintillator material is calculated. In the third step, the transport of scintillation photons in the scintillator and lightguide is simulated. Finally, the resolution corresponding to the experiment is considered in the last step of the simulation. Unlike the similar computer codes like SCINFUL, NRESP7 and PHRESP, the developed computer code is applicable to both neutron and gamma sources. Hence, the discrimination of neutron and gamma in the mixed fields may be performed using the MCNPX-ESUT computer code. The main feature of MCNPX-ESUT computer code is that the neutron/gamma pulse height simulation may be performed without needing any sort of post processing. In the present study, the pulse height distributions due to a monoenergetic neutron/gamma source in NE-213 detector using MCNPX-ESUT computer code is simulated. The simulated neutron pulse height distributions are validated through comparing with experimental data (Gohil et al. Nuclear Instruments and Methods in Physics Research Section A: Accelerators, Spectrometers, Detectors and Associated Equipment, 664 (2012) 304-309.) and the results obtained from similar computer codes like SCINFUL, NRESP7 and Geant4. The simulated gamma pulse height distribution for a 137Cs source is also compared with the experimental data.

A scintillator-based approach to monitor secondary neutron production during proton therapy.

PubMed

Clarke, S D; Pryser, E; Wieger, B M; Pozzi, S A; Haelg, R A; Bashkirov, V A; Schulte, R W

2016-11-01

The primary objective of this work is to measure the secondary neutron field produced by an uncollimated proton pencil beam impinging on different tissue-equivalent phantom materials using organic scintillation detectors. Additionally, the Monte Carlo code mcnpx-PoliMi was used to simulate the detector response for comparison to the measured data. Comparison of the measured and simulated data will validate this approach for monitoring secondary neutron dose during proton therapy. Proton beams of 155- and 200-MeV were used to irradiate a variety of phantom materials and secondary particles were detected using organic liquid scintillators. These detectors are sensitive to fast neutrons and gamma rays: pulse shape discrimination was used to classify each detected pulse as either a neutron or a gamma ray. The mcnpx-PoliMi code was used to simulate the secondary neutron field produced during proton irradiation of the same tissue-equivalent phantom materials. An experiment was performed at the Loma Linda University Medical Center proton therapy research beam line and corresponding models were created using the mcnpx-PoliMi code. The authors' analysis showed agreement between the simulations and the measurements. The simulated detector response can be used to validate the simulations of neutron and gamma doses on a particular beam line with or without a phantom. The authors have demonstrated a method of monitoring the neutron component of the secondary radiation field produced by therapeutic protons. The method relies on direct detection of secondary neutrons and gamma rays using organic scintillation detectors. These detectors are sensitive over the full range of biologically relevant neutron energies above 0.5 MeV and allow effective discrimination between neutron and photon dose. Because the detector system is portable, the described system could be used in the future to evaluate secondary neutron and gamma doses on various clinical beam lines for commissioning and prospective data collection in pediatric patients treated with proton therapy.

C7LYC Scintillators and Fast Neutron Spectroscopy

NASA Astrophysics Data System (ADS)

Chowdhury, P.; Brown, T.; Doucet, E.; Lister, C. J.; Wilson, G. L.; D'Olympia, N.; Devlin, M.; Mosby, S.

2016-09-01

Cs2 LiYCl6 (CLYC) scintillators detect both gammas and neutrons with excellent pulse shape discrimination. At UML, fast neutron measurements with a 16-element 1''x1'' CLYC array show promise for low energy nuclear science. CLYC detects fast neutrons via the 35Cl (n,p) reaction (resolution < 10 % at < 8 MeV). In our 7Li-enriched C7LYC, the thermal neutron response from the 6Li(n, α)t reaction is virtually eliminated. The low intrinsic efficiency of CLYC for fast neutrons (< 1 %) is offset by increased solid angle with the array placed near the target, since TOF is not needed for energy resolution. The array was tested at LANL for measuring elastic and inelastic neutron scattering on 56Fe. The incident energy from the white neutron source was measured via TOF, and the scattered neutron energy via the pulse height in CLYC. The array was also tested at CARIBU for measuring beta-delayed neutrons. Larger CLYC crystals are now a reality. Measurements with the first 3'' x 3'' C7LYC crystal are in progress at UML. Results will be discussed in the context of constructing a C7LYC array at FRIB for reaction and decay spectroscopy of neutron-rich fragments. Supported by the NNSA Stewardship Science Academic Alliance Program under Grant DE-NA00013008.

Fast collimated neutron flux measurement using stilbene scintillator and flashy analog-to-digital converter in JT-60U

NASA Astrophysics Data System (ADS)

Ishikawa, M.; Itoga, T.; Okuji, T.; Nakhostin, M.; Shinohara, K.; Hayashi, T.; Sukegawa, A.; Baba, M.; Nishitani, T.

2006-10-01

A line-integrated neutron emission profile is routinely measured using the radial neutron collimator system in JT-60U tokamak. Stilbene neuron detectors (SNDs), which combine a stilbene organic crystal scintillation detector (SD) with an analog neutron-gamma pulse shape discrimination (PSD) circuit, have been used to measure collimated neutron flux. Although the SND has many advantages as a neutron detector, the maximum count rate is limited up to ˜1×105counts/s due to the analog PSD circuit. To overcome this issue, a digital signal processing system (DSPS) using a flash analog-to-digital converter (Acqiris DC252, 8GHz, 10bits) has been developed at Cyclotron and Radioisotope Center in Tohoku University. In this system anode signals from photomultiplier of the SD are directory stored and digitized. Then, the PSD between neutrons and gamma rays is performed using software. The DSPS has been installed in the vertical neutron collimator system in JT-60U and applied to deuterium experiments. It is confirmed that the PSD is sufficiently performed and collimated neutron flux is successfully measured with count rate up to ˜5×105counts/s without the effect of pileup of detected pulses. The performance of the DSPS as a neutron detector, which supersedes the SND, is demonstrated.

A novel pulse height analysis technique for nuclear spectroscopic and imaging systems

NASA Astrophysics Data System (ADS)

Tseng, H. H.; Wang, C. Y.; Chou, H. P.

2005-08-01

The proposed pulse height analysis technique is based on the constant and linear relationship between pulse width and pulse height generated from front-end electronics of nuclear spectroscopic and imaging systems. The present technique has successfully implemented into the sump water radiation monitoring system in a nuclear power plant. The radiation monitoring system uses a NaI(Tl) scintillator to detect radioactive nuclides of Radon daughters brought down by rain. The technique is also used for a nuclear medical imaging system. The system uses a position sensitive photomultiplier tube coupled with a scintillator. The proposed techniques has greatly simplified the electronic design and made the system a feasible one for potable applications.

RADIATION-MEASURING SYSTEMS OF SOVIET ROCKETS

DOE Office of Scientific and Technical Information (OSTI.GOV)

Vakulov, P.V.; Goryunov, N.N.; Logachev, Yu.I.

1961-11-01

The second and third Sputniks and all Soviet space rockets and spaceship- satellites were equipped with radiationmeasuring systems comprising scintillation and gasdischarge counters and shaping, amplification, and scaling circuits. The scintillation counters use photomultipliers having either 40 x 40 Nal(Tl) or 20 x 20 Csl(Tl) cylindrical crystals. Both types have a gain of ~5.10/sup 4/. The highvoltage battery supplies voltages to the photomultipliers without the use of voltage dividers. Pulses from the 11th, 9th, and 8th dynodes are used for counting the number of particles which produce energy yields from the crystal exceeding ~50 and 500 kev and 5 Mev,more » respectively. Fourstage transistor amplifiers with an over-all gain of ~100 are used for amplification of the counting pulses. The trigger-discriminator, together with the amplifier, is capable of counting (2.5 -- 3.0) x 10/sup 5/ pulses/sec and of insuring a threshold stability of 10% at ambient temperatures of --30 to +50 deg C and voltage variations of plus or minus 20%. Ionization is measured from the current of the 7th dynode and the photomultiplier collector, which permits readings as low as 10/sup -10/ amp to be made by the method of charge storage (in the capacitor) with subsequent discharge through a neon tube. A gas-disoharge counter with 50 mg/cm/sup 2/ stainless-steel walls, operating at 400 v, also measures ionization. Before coming to the scaling circuit, the 50 v negative pulses from this counter pass through a transistor amplifier which changes their polarity and reduces their duration to 8 to 10 mu sec. (OTS)« less

Synthesis of plastic scintillation microspheres: Evaluation of scintillators

NASA Astrophysics Data System (ADS)

Santiago, L. M.; Bagán, H.; Tarancón, A.; Garcia, J. F.

2013-01-01

The use of plastic scintillation microspheres (PSm) appear to be an alternative to liquid scintillation for the quantification of alpha and beta emitters because it does not generate mixed wastes after the measurement (organic and radioactive). In addition to routine radionuclide determinations, PSm can be used for further applications, e.g. for usage in a continuous monitoring equipment, for measurements of samples with a high salt concentration and for an extractive scintillation support which permits the separation, pre-concentration and measurement of the radionuclides without additional steps of elution and sample preparation. However, only a few manufacturers provide PSm, and the low number of regular suppliers reduces its availability and restricts the compositions and sizes available. In this article, a synthesis method based on the extraction/evaporation methodology has been developed and successfully used for the synthesis of plastic scintillation microspheres. Seven different compositions of plastic scintillation microspheres have been synthesised; PSm1 with polystyrene, PSm2 with 2,5-Diphenyloxazol(PPO), PSm3 with p-terphenyl (pT), PSm4 with PPO and 1,4-bis(5-phenyloxazol-2-yl) (POPOP), PSm5 pT and (1,4-bis [2-methylstyryl] benzene) (Bis-MSB), PSm6 with PPO, POPOP and naphthalene and PSm7 with pT, Bis-MSB and naphthalene. The synthesised plastic scintillation microspheres have been characterised in terms of their morphology, detection capabilities and alpha/beta separation capacity. The microspheres had a median diameter of approximately 130 μm. Maximum detection efficiency values were obtained for the PSm4 composition as follows 1.18% for 3H, 51.2% for 14C, 180.6% for 90Sr/90Y and 76.7% for 241Am. Values of the SQP(E) parameter were approximately 790 for PSm4 and PSm5. These values show that the synthesised PSm exhibit good scintillation properties and that the spectra are at channel numbers higher than in commercial PSm. Finally, the addition of naphthalene modifies the shape of the pulses produced by alpha and beta particles leading to better alpha/beta separation.

Development of a digital method for neutron/gamma-ray discrimination based on matched filtering

NASA Astrophysics Data System (ADS)

Korolczuk, S.; Linczuk, M.; Romaniuk, R.; Zychor, I.

2016-09-01

Neutron/gamma-ray discrimination is crucial for measurements with detectors sensitive to both neutron and gamma-ray radiation. Different techniques to discriminate between neutrons and gamma-rays based on pulse shape analysis are widely used in many applications, e.g., homeland security, radiation dosimetry, environmental monitoring, fusion experiments, nuclear spectroscopy. A common requirement is to improve a radiation detection level with a high detection reliability. Modern electronic components, such as high speed analog to digital converters and powerful programmable digital circuits for signal processing, allow us to develop a fully digital measurement system. With this solution it is possible to optimize digital signal processing algorithms without changing any electronic components in an acquisition signal path. We report on results obtained with a digital acquisition system DNG@NCBJ designed at the National Centre for Nuclear Research. A 2'' × 2'' EJ309 liquid scintillator was used to register mixed neutron and gamma-ray radiation from PuBe sources. A dedicated algorithm for pulse shape discrimination, based on real-time filtering, was developed and implemented in hardware.

A real-time neutron-gamma discriminator based on the support vector machine method for the time-of-flight neutron spectrometer

NASA Astrophysics Data System (ADS)

Wei, ZHANG; Tongyu, WU; Bowen, ZHENG; Shiping, LI; Yipo, ZHANG; Zejie, YIN

2018-04-01

A new neutron-gamma discriminator based on the support vector machine (SVM) method is proposed to improve the performance of the time-of-flight neutron spectrometer. The neutron detector is an EJ-299-33 plastic scintillator with pulse-shape discrimination (PSD) property. The SVM algorithm is implemented in field programmable gate array (FPGA) to carry out the real-time sifting of neutrons in neutron-gamma mixed radiation fields. This study compares the ability of the pulse gradient analysis method and the SVM method. The results show that this SVM discriminator can provide a better discrimination accuracy of 99.1%. The accuracy and performance of the SVM discriminator based on FPGA have been evaluated in the experiments. It can get a figure of merit of 1.30.

PMT-scintillator system set up for D-D neutron TOF measurements in INTI plasma focus device

NASA Astrophysics Data System (ADS)

Damideh, V.; Saw, S. H.; Sadighzadeh, A.; Ali, J.; Rawat, R. S.; Lee, P.; Lee, S.

2017-03-01

This paper summarizes a Photomultiplier-Scintillator diagnostic system for use in our plasma focus experiments at the Center for Plasma Research INTI IU. The system features an anode-grounded high pulse linearity voltage divider and uses NE102A plastic scintillators. It has detected D-D neutrons in INTI plasma focus device with clear and high signal to noise ratio. Neutron TOF of 120 ns has been measured from the time difference between hard x-ray pulse peak and neutron peak time over a flight path of 2.6±0.01 m; giving energy of 2.5±0.1 MeV for these side-on neutrons.

Searching for dark matter with single phase liquid argon

NASA Astrophysics Data System (ADS)

Caldwell, Thomas S., Jr.

The first hint that we fail to understand the nature of a large fraction of the gravitating matter in the universe came from Fritz Zwicky's measurements of the velocity distribution of the Coma cluster in 1933. Using the Virial theorem, Zwicky found that galaxies in the cluster were orbiting far too fast to remain gravitationally bound when their mass was estimated by the brightness of the visible matter. This led to the postulation that some form of non-luminous dark matter is present in galaxies comprising a large fraction of the galactic mass. The nature of this dark matter remains yet unknown over 80 years after Zwicky's measurements despite the efforts of many experiments. Dark matter is widely believed to be a beyond the Standard Model particle which brings the dark matter problem into the realm of particle physics. Supersymmetry is one widely explored extension of the Standard model, from which particles meeting the constraints on dark matter properties can naturally arise. These particles are generically termed weakly interacting massive particles (WIMPs), and are a currently favored dark matter candidate. A variety of experimental efforts are underway aimed towards direct detection of dark matter through observation of rare scattering of WIMPs in terrestrial detectors. Single phase liquid argon detectors are an appealing WIMP detection technique due to the scintillation properties of liquid argon and the scalability of the single phase approach. The MiniCLEAN dark matter detector is a single phase liquid argon scintillation scintillation detector with a 500 kg active mass. The modular design offers 4pi coverage with 92 optical cassettes, each containing TPB coated acrylic and a cryogenic photomultiplier tube. The MiniCLEAN detector has recently completed construction at SNOLAB. The detector is currently being commissioned, and will soon begin operation with the liquid argon target. Utilizing advanced pulse-shape discrimination techniques, MiniCLEAN will probe the WIMP-nucleon cross section parameter space to the level of 10--44 cm2 and demonstrate the pulse-shape discrimination required for next generation experiments capable of further probing the WIMP parameter space in search of WIMP dark matter.

A wearable sensor based on CLYC scintillators

NASA Astrophysics Data System (ADS)

McDonald, Benjamin S.; Myjak, Mitchell J.; Zalavadia, Mital A.; Smart, John E.; Willett, Jesse A.; Landgren, Peter C.; Greulich, Christopher R.

2016-06-01

We have developed a wearable radiation sensor using Cs2LiYCl6:Ce (CLYC) for simultaneous gamma-ray and neutron detection. The system includes two ∅ 2.5 × 2.5cm3 crystals coupled to small, metal-body photomultiplier tubes. A custom, low-power electronics base digitizes the output signal at three time points and enables both pulse height and pulse shape discrimination of gamma rays and neutrons. The total counts, anomaly detection metrics, and identified isotopes are displayed on a small screen. Users may leave the device in unattended mode to collect long-dwell energy spectra. The system stores up to 18 h of one-second data, including energy spectra, and may transfer the data to a remote computer via a wired or wireless connection. The prototype is 18 × 13 × 7.5cm3, weighs 1.3 kg, not including the protective pouch, and runs on six AA alkaline batteries for 29 h with the wireless link active, or 41 h with the wireless link disabled. In this paper, we summarize the system design and present characterization results from the detector modules. The energy resolution is about 6.5% full width at half maximum at 662 keV due to the small photomultiplier tube selected, and the linearity and pulse shape discrimination performance are very good.

Timing and Pulse Shape Discrimination Comparison Against Legacy TDC & QDC and the JLab F250 FADC

NASA Astrophysics Data System (ADS)

Milkeris-Zellar, Tyler; Sawatzky, Brad

2017-09-01

The F250 Flash Analog to Digital Convertor (FADC) is a relatively new module used in Data Acquisition Systems (DAQ) at Jefferson Lab. The FADC will replace or supplement older DAQ modules like Time to Digital Converters (TDCs) and Charge Analog to Digital Converters (QDCs). The TDC has a certain known timing resolution and the QDC can integrate a pulse's charge, a feature which can also be used for particle identification between photons and neutrons using pulse shape discrimination (PSD). The focus of this project is developing a test stand to study timing and PSD performance of legacy modules TDC and QDC, and the new F250 FADC. A cosmic telescope was used to extract timing resolution from the TDC and FADC. Through PSD with the QDC and FADC, using a liquid scintillator, we plan to identify photons and neutrons from an americium-beryllium (AmBe) source. Through PSD, we found that the FADC allows for flexible data analysis compared to the QDC. The results indicate that the TDC provides a more accurate measurement of timing resolution than the FADC. This improvement allows for a clear distinction of what module to use when wanting precision of measurement in a DAQ for a cosmic ray telescope. NSF.

A wearable sensor based on CLYC scintillators

DOE Office of Scientific and Technical Information (OSTI.GOV)

McDonald, Benjamin S.; Myjak, Mitchell J.; Zalavadia, Mital A.

We developed a wearable radiation sensor using Cs 2LiYCl 6:Ce (CLYC) for simultaneous gamma-ray and neutron detection. The system includes two ø2.5×2.5 cm 3 crystals coupled to small, metal-body photomultiplier tubes. A custom, low-power electronics base digitizes the output signal at three time points and enables both pulse height and pulse shape discrimination of neutrons and gamma-rays. Data, including spectra, can be transferred via a wired or wireless connection. The total gamma-ray and neutron counts, anomaly detection metrics, and identified isotopes are displayed on a small screen on the device. Users may leave the system in unattended mode to collectmore » long-dwell energy spectra. The prototype system has overall dimensions of 13×7.5×18 cm 3 and weight of 1.3 kg, not including the protective pouch, and runs on six AA alkaline batteries for 29 hours with a 1% wireless transmission duty cycle and 41 hours with the wireless turned off . In this paper, we summarize the system design and present characterization results from the detector modules. The energy resolution is about 6.5% full width at half maximum at 662 keV due to the small photomultiplier tube selected, and the linearity and pulse shape discrimination performance are very good.« less

Plastic scintillators with high loading of one or more metal carboxylates

DOE Office of Scientific and Technical Information (OSTI.GOV)

Cherepy, Nerine; Sanner, Robert Dean

In one embodiment, a material includes at least one metal compound incorporated into a polymeric matrix, where the metal compound includes a metal and one or more carboxylate ligands, where at least one of the one or more carboxylate ligands includes a tertiary butyl group, and where the material is optically transparent. In another embodiment, a method includes: processing pulse traces corresponding to light pulses from a scintillator material; and outputting a result of the processing, where the scintillator material comprises at least one metal compound incorporated into a polymeric matrix, the at least one metal compound including a metalmore » and one or more carboxylate ligands, where at least one of the one or more carboxylate ligands has a tertiary butyl group, and where the scintillator material is optically transparent and has an energy resolution at 662 keV of less than about 20%.« less

Microprocessor-based single particle calibration of scintillation counter

NASA Technical Reports Server (NTRS)

Mazumdar, G. K. D.; Pathak, K. M.

1985-01-01

A microprocessor-base set-up is fabricated and tested for the single particle calibration of the plastic scintillator. The single particle response of the scintillator is digitized by an A/D converter, and a 8085 A based microprocessor stores the pulse heights. The digitized information is printed. Facilities for CRT display and cassette storing and recalling are also made available.

Pulse pile-up identification and reconstruction for liquid scintillator based neutron detectors

NASA Astrophysics Data System (ADS)

Luo, X. L.; Modamio, V.; Nyberg, J.; Valiente-Dobón, J. J.; Nishada, Q.; de Angelis, G.; Agramunt, J.; Egea, F. J.; Erduran, M. N.; Ertürk, S.; de France, G.; Gadea, A.; González, V.; Goasduff, A.; Hüyük, T.; Jaworski, G.; Moszyński, M.; Di Nitto, A.; Palacz, M.; Söderström, P.-A.; Sanchis, E.; Triossi, A.; Wadsworth, R.

2018-07-01

The issue of pulse pile-up is frequently encountered in nuclear experiments involving high counting rates, which will distort the pulse shapes and the energy spectra. A digital method of off-line processing of pile-up pulses is presented. The pile-up pulses were firstly identified by detecting the downward-going zero-crossings in the first-order derivative of the original signal, and then the constituent pulses were reconstructed based on comparing the pile-up pulse with four models that are generated by combining pairs of neutron and γ standard pulses together with a controllable time interval. The accuracy of this method in resolving the pile-up events was investigated as a function of the time interval between two pulses constituting a pile-up event. The obtained results show that the method is capable of disentangling two pulses with a time interval among them down to 20 ns, as well as classifying them as neutrons or γ rays. Furthermore, the error of reconstructing pile-up pulses could be kept below 6% when successive peaks were separated by more than 50 ns. By applying the method in a high counting rate of pile-up events measurement of the NEutron Detector Array (NEDA), it was empirically found that this method can reconstruct the pile-up pulses and perform neutron- γ discrimination quite accurately. It can also significantly correct the distorted pulse height spectrum due to pile-up events.

Real-Time Wavelength Discrimination for Improved Neutron Discrimination in CLYC

DOE Office of Scientific and Technical Information (OSTI.GOV)

Hornback, Donald Eric; Hu, Michael Z.; Bell, Zane W.

We investigated the effects of optical filters on the pulse shape discrimination properties of Cs 2LiYCl 6:Ce (CLYC) scintillator crystals. By viewing the scintillation light through various optical filters, we attempted to better distinguish between neutron and gamma ray events in the crystal. We applied commercial interference and colored glass filters in addition to fabricating quantum dot (QD) filters by suspending QDs in plastic films and glass. QD filters ultimately failed because of instability of the QDs with respect to oxidation when exposed to ambient air, and the tendency of the QDs to aggregate in the plastic. Of the commercialmore » filters, the best results were obtained with a bandpass interference filter covering the spectral region containing core-valence luminescence (CVL) light. However, the PSD response of filtered CLYC light was always poorer than the response exhibited by unfiltered light because filters always reduced the amount of light available for signal processing.« less

Rejection of randomly coinciding 2ν2β events in ZnMoO4 scintillating bolometers

NASA Astrophysics Data System (ADS)

Chernyak, D. M.; Danevich, F. A.; Giuliani, A.; Mancuso, M.; Nones, C.; Olivieri, E.; Tenconi, M.; Tretyak, V. I.

2014-01-01

Random coincidence of 2ν2β decay events could be one of the main sources of background for 0ν2β decay in cryogenic bolometers due to their poor time resolution. Pulse-shape discrimination by using front edge analysis, the mean-time and χ2 methods was applied to discriminate randomly coinciding 2ν2β events in ZnMoO4 cryogenic scintillating bolometers. The background can be effectively rejected on the level of 99% by the mean-time analysis of heat signals with the rise time about 14 ms and the signal-to-noise ratio 900, and on the level of 98% for the light signals with 3 ms rise time and signal-to-noise ratio of 30 (under a requirement to detect 95% of single events). Importance of the signal-to-noise ratio, correct finding of the signal start and choice of an appropriate sampling frequency are discussed.

Theoretical and Experimental Investigations of Coincidences in Poisson Distributed Pulse Trains and Spectral Distortion Caused by Pulse Pileup.

NASA Astrophysics Data System (ADS)

Bristow, Quentin

1990-01-01

Part one of this two-part study is concerned with the multiple coincidences in pulse trains from X-ray and gamma radiation detectors which are the cause of pulse pileup. A sequence of pulses with inter-arrival times less than tau, the resolving time of the pulse-height analysis system used to acquire spectra, is called a multiple pulse string. Such strings can be classified on the basis of the number of pulses they contain, or the number of resolving times they cover. The occurrence rates of such strings are derived from theoretical considerations. Logic circuits were devised to make experimental measurements of multiple pulse string occurrence rates in the output from a NaI(Tl) scintillation detector over a wide range of count rates. Markov process theory was used to predict state transition rates in the logic circuits, enabling the experimental data to be checked rigorously for conformity with those predicted for a Poisson distribution. No fundamental discrepancies were observed. Part two of the study is concerned with a theoretical analysis of pulse pileup and the development of a discrete correction algorithm, based on the use of a function to simulate the coincidence spectrum produced by partial sums of pulses. Monte Carlo simulations, incorporating criteria for pulse pileup inherent in the operation of modern ADC's, were used to generate pileup spectra due to coincidences between two pulses, (1st order pileup) and three pulses (2nd order pileup), for different semi-Gaussian pulse shapes. Coincidences between pulses in a single channel produced a basic probability density function spectrum which can be regarded as an impulse response for a particular pulse shape. The use of a flat spectrum (identical count rates in all channels) in the simulations, and in a parallel theoretical analysis, showed the 1st order pileup distorted the spectrum to a linear ramp with a pileup tail. The correction algorithm was successfully applied to correct entire spectra for 1st and 2nd order pileup; both those generated by Monte Carlo simulations and in addition some real spectra acquired with a laboratory multichannel analysis system.

A Sub-Sampling Approach for Data Acquisition in Gamma Ray Emission Tomography

NASA Astrophysics Data System (ADS)

Fysikopoulos, Eleftherios; Kopsinis, Yannis; Georgiou, Maria; Loudos, George

2016-06-01

State of the art data acquisition systems for small animal imaging gamma ray detectors often rely on free running Analog to Digital Converters (ADCs) and high density Field Programmable Gate Arrays (FPGA) devices for digital signal processing. In this work, a sub-sampling acquisition approach, which exploits a priori information regarding the shape of the obtained detector pulses is proposed. Output pulses shape depends on the response of the scintillation crystal, photodetector's properties and amplifier/shaper operation. Using these known characteristics of the detector pulses prior to digitization, one can model the voltage pulse derived from the shaper (a low-pass filter, last in the front-end electronics chain), in order to reduce the desirable sampling rate of ADCs. Fitting with a small number of measurements, pulse shape estimation is then feasible. In particular, the proposed sub-sampling acquisition approach relies on a bi-exponential modeling of the pulse shape. We show that the properties of the pulse that are relevant for Single Photon Emission Computed Tomography (SPECT) event detection (i.e., position and energy) can be calculated by collecting just a small fraction of the number of samples usually collected in data acquisition systems used so far. Compared to the standard digitization process, the proposed sub-sampling approach allows the use of free running ADCs with sampling rate reduced by a factor of 5. Two small detectors consisting of Cerium doped Gadolinium Aluminum Gallium Garnet (Gd3Al2Ga3O12 : Ce or GAGG:Ce) pixelated arrays (array elements: 2 × 2 × 5 mm3 and 1 × 1 × 10 mm3 respectively) coupled to a Position Sensitive Photomultiplier Tube (PSPMT) were used for experimental evaluation. The two detectors were used to obtain raw images and energy histograms under 140 keV and 661.7 keV irradiation respectively. The sub-sampling acquisition technique (10 MHz sampling rate) was compared with a standard acquisition method (52 MHz sampling rate), in terms of energy resolution and image signal to noise ratio for both gamma ray energies. The Levenberg-Marquardt (LM) non-linear least-squares algorithm was used, in post processing, in order to fit the acquired data with the proposed model. The results showed that analog pulses prior to digitization are being estimated with high accuracy after fitting with the bi-exponential model.

Elpasolite Planetary Ice and Composition Spectrometer (EPICS): A Low-Resource Combined Gamma-Ray and Neutron Spectrometer for Planetary Science

NASA Astrophysics Data System (ADS)

Stonehill, L. C.; Coupland, D. D. S.; Dallmann, N. A.; Feldman, W. C.; Mesick, K.; Nowicki, S.; Storms, S.

2017-12-01

The Elpasolite Planetary Ice and Composition Spectrometer (EPICS) is an innovative, low-resource gamma-ray and neutron spectrometer for planetary science missions, enabled by new scintillator and photodetector technologies. Neutrons and gamma rays are produced by cosmic ray interactions with planetary bodies and their subsequent interactions with the near-surface materials produce distinctive energy spectra. Measuring these spectra reveals details of the planetary near-surface composition that are not accessible through any other phenomenology. EPICS will be the first planetary science instrument to fully integrate the neutron and gamma-ray spectrometers. This integration is enabled by the elpasolite family of scintillators that offer gamma-ray spectroscopy energy resolutions as good as 3% FWHM at 662 keV, thermal neutron sensitivity, and the ability to distinguish gamma-ray and neutron signals via pulse shape differences. This new detection technology will significantly reduce size, weight, and power (SWaP) while providing similar neutron performance and improved gamma energy resolution compared to previous scintillator instruments, and the ability to monitor the cosmic-ray source term. EPICS will detect scintillation light with silicon photomultipliers rather than traditional photomultiplier tubes, offering dramatic additional SWaP reduction. EPICS is under development with Los Alamos National Laboratory internal research and development funding. Here we report on the EPICS design, provide an update on the current status of the EPICS development, and discuss the expected sensitivity and performance of EPICS in several potential missions to airless bodies.

Observation of 67 keV x-rays with a scintillation detector using proportional-mode silicon avalanche photodiode

DOE Office of Scientific and Technical Information (OSTI.GOV)

Inoue, Keisuke; Kishimoto, Shunji, E-mail: syunji.kishimoto@kek.jp; Inst. of Materials Structure Science, KEK, 1-1 Oho, Tsukuba, Ibaraki 305-0801

2016-07-27

We developed a scintillation X-ray detector using a proportional-mode silicon avalanche photodiode (Si-APD). We report a prototype detector using a lead-loaded plastic scintillator mounted on a proportional-mode Si-APD (active area size: 3 mm in diameter), which is operated at a low temperature. Using 67.41 keV X-rays, we could measure pulse-height spectra of scintillation light with a charge-sensitive preamplifier at 20, 0, and −35°C. Time spectra of the X-ray bunch structure were successfully recorded using a wideband and 60-dB-gain amplifier in hybrid-mode operation of the Photon Factory ring. We obtained a better time resolution of 0.51 ns (full width at half-maximum)more » for the single-bunch X-ray peak at −35°C. We were also able to observe a linear response of the scintillation pulses up to 8 Mcps for input photon rates up to 1.4 × 10{sup 8} photons/s.« less

Scintillator and solid-state neutron detectors and their applications

NASA Astrophysics Data System (ADS)

Carturan, Sara Maria; Marchi, Tommaso; Fanchini, Erica; De Vita, Raffaella; Finocchiaro, Paolo; Pappalardo, Alfio

2014-10-01

The application range of neutron detectors covers many topics, not only involving experimental research, but spanning tens of industrial, health, transport, cultural heritage fields of interest. Several studies focus on new scintillating materials where the light response, under fast and slow neutrons exposure, is triggered by proton recoil or by the presence of neutron capture materials as 10B, 6Li or 157Gd. Neutron monitors, where the robustness of silicon-based detectors can be fully exploited by coupling with suitable neutron absorber/converter materials, have recently proved their outstanding performances. Discrimination between neutron signals from other radiations, such as - or cosmic rays, is achieved through timing techniques or with pulse shape analysis. Furthermore, the choice of the detection/discrimination techniques depends on the type of application the detector will be used for. An example is Radiation Portal Monitors (RPM) for cargo inspection or luggage control that are required to satisfy specific international standards for and neutron detection efficiencies. This paper is an overview of some of the National Institute of Nuclear Physics (INFN) activities in the field of neutron detection, involving novel technologies. We will describe the most recent advances related to scintillators and silicon-based detectors coupled with thin films of suitable converters for neutron detection and we will discuss applications in the field of nuclear security.

Improved LabPET Detectors Using Lu1.8Gd0.2SiO5:Ce (LGSO) Scintillator Blocks

NASA Astrophysics Data System (ADS)

Bergeron, Mélanie; Pepin, Catherine M.; Cadorette, Jules; Loignon-Houle, Francis; Fontaine, Réjean; Lecomte, Roger

2015-02-01

The scintillator is one of the key building blocks that critically determine the physical performance of PET detectors. The quest for scintillation crystals with improved characteristics has been crucial in designing scanners with superior imaging performance. Recently, it was shown that the decay time constant of high lutetium content Lu1.8Gd0.2SiO5: Ce (LGSO) scintillators can be adjusted by varying the cerium concentration from 0.025 mol% to 0.75 mol%, thus providing interesting characteristics for phoswich detectors. The high light output (90%-120% NaI) and the improved spectral match of these scintillators with avalanche photodiode (APD) readout promise superior energy and timing resolutions. Moreover, their improved mechanical properties, as compared to conventional LGSO ( Lu0.4Gd1.6SiO5: Ce), make block array manufacturing readily feasible. To verify these assumptions, new phoswich block arrays made of LGSO-90%Lu with low and high mol% Ce concentrations were fabricated and assembled into modules dedicated to the LabPET scanner. Typical crystal decay time constants were 31 ns and 47 ns, respectively. Phoswich crystal identification performed using a digital pulse shape discrimination algorithm yielded an average 8% error. At 511 keV, an energy resolution of 17-21% was obtained, while coincidence timing resolution between 4.6 ns and 5.2 ns was achieved. The characteristics of this new LGSO-based phoswich detector module are expected to improve the LabPET scanner performance. The higher stopping power would increase the detection efficiency. The better timing resolution would also allow the use of a narrower coincidence window, thus minimizing the random event rate. Altogether, these two improvements will significantly enhance the noise equivalent count rate performance of an all LGSO-based LabPET scanner.

DESCANT - Testing and Commissioning

NASA Astrophysics Data System (ADS)

Bildstein, Vinzenz; Garrett, P. E.; Bandyopadhay, D.; Bangay, J.; Bianco, L.; Demand, G.; Hadinia, B.; Leach, K. G.; Sumithrarachchi, C.; Turko, J.; Wong, J.; Ashley, S. F.; Crider, B. P.; McEllistrem, M. T.; Peters, E. E.; Prados-Estévez, F. M.; Yates, S. W.; Vanhoy, J. R.; Ball, G. C.; Bishop, D. P.; Garnsworthy, A. B.; Hackman, G.; Pearson, C. J.; Shaw, B.; Sarazin, F.

2017-09-01

The DESCANT array at TRIUMF is designed to detect neutrons from RIB experiments. DESCANT is composed of 70 close-packed deuterated organic liquid scintillators coupled to digital fast read-out ADC modules. This configuration permits online pulse-shape discrimination between neutron and γ-ray events. A prototype detector was tested with monoenergetic neutrons at the University of Kentucky Accelerator Laboratory. The data from these tests was compared to Geant4 simulations. A first commissioning experiment of the full array, using the decay of Cs 145 - 146 , was performed in August 2016. The results of the tests and a preliminary analysis of the commissioning experiment will be presented.

The GSFC Advanced Compton Telescope (ACT)

NASA Technical Reports Server (NTRS)

Hartman, R.; Fichtel, C.; Kniffen, D.; Trombka, J.; Stacy, G.

1983-01-01

A new telescope is being developed at GSFC for the study of point sources of gamma rays in the energy range 1-30 MeV. Using the detection principle of a Compton scatter in a 2.5 cm thick NaI(Tl) detector followed by absorption in a 15 cm thick NaI(Tl) detector, the telescope uses a rocking collimator for field-of-view reduction and background subtraction. Background reduction techniques include lead-plastic scintillator shielding, pulse shape discrimination and Anger camera operation to both NaI detectors, as well as a time-of-flight measurement between them. The instrument configuration and status is described.

Scattering analysis of LOFAR pulsar observations

NASA Astrophysics Data System (ADS)

Geyer, M.; Karastergiou, A.; Kondratiev, V. I.; Zagkouris, K.; Kramer, M.; Stappers, B. W.; Grießmeier, J.-M.; Hessels, J. W. T.; Michilli, D.; Pilia, M.; Sobey, C.

2017-09-01

We measure the effects of interstellar scattering on average pulse profiles from 13 radio pulsars with simple pulse shapes. We use data from the LOFAR High Band Antennas, at frequencies between 110 and 190 MHz. We apply a forward fitting technique, and simultaneously determine the intrinsic pulse shape, assuming single Gaussian component profiles. We find that the constant τ, associated with scattering by a single thin screen, has a power-law dependence on frequency τ ∝ ν-α, with indices ranging from α = 1.50 to 4.0, despite simplest theoretical models predicting α = 4.0 or 4.4. Modelling the screen as an isotropic or extremely anisotropic scatterer, we find anisotropic scattering fits lead to larger power-law indices, often in better agreement with theoretically expected values. We compare the scattering models based on the inferred, frequency-dependent parameters of the intrinsic pulse, and the resulting correction to the dispersion measure (DM). We highlight the cases in which fits of extreme anisotropic scattering are appealing, while stressing that the data do not strictly favour either model for any of the 13 pulsars. The pulsars show anomalous scattering properties that are consistent with finite scattering screens and/or anisotropy, but these data alone do not provide the means for an unambiguous characterization of the screens. We revisit the empirical τ versus DM relation and consider how our results support a frequency dependence of α. Very long baseline interferometry, and observations of the scattering and scintillation properties of these sources at higher frequencies, will provide further evidence.

Development of the Fast Scintillation Detector with Programmable High Voltage Adjustment Suitable for Moessbauer Spectroscopy

DOE Office of Scientific and Technical Information (OSTI.GOV)

Prochazka, R.; Frydrych, J.; Pechousek, J.

2010-07-13

This work is focused on a development of a compact fast scintillation detector suitable for Moessbauer spectroscopy (low energy X-ray/{gamma}-ray detection) where high counting rates are inevitable. Optimization of this part was necessary for a reliable function, better time resolution and to avoid a detector pulses pile-up effect. The pile-up effect decreases the measurement performance, significantly depends on the source activity and also on the pulse duration. Our new detection unit includes a fast scintillation crystal YAP:Ce, an R6095 photomultiplier tube, a high voltage power supply socket C9028-01 assembly, an AD5252 digital potentiometer with an I2C interface and an AD8000more » ultra fast operation preamplifier. The main advantages of this solution lie in a short pulse duration (less than 200 ns), stable operation for high activities, programmable gain of the high voltage supply and compact design in the aluminum housing.« less

Cs2LiLa(Br,Cl)6 Crystals for Nuclear Security Applications

NASA Astrophysics Data System (ADS)

Hawrami, R.; Pandian, L. Soundara; Ariesanti, E.; Glodo, J.; Finkelstein, J.; Tower, J.; Shah, K.

2016-04-01

Properties of dual-mode scintillation detectors based on CLLBC crystals are reported. Energy resolution and light yield are measured at 2.9% (FWHM) at 662 keV and 45000 photons/MeV, respectively, for a 1-in-diameter and 1-in-long crystal. With less than 2% variation in light yield as a function of energy, CLLBC has better proportionality than LaBr3 and NaI:Tl. Neutron peak resulting from reactions with neutrons emitted by 252Cf (moderated) is measured at a gamma energy equivalent of 3.1 MeVee (electron energy equivalent), making pulse height discrimination between gamma-rays and neutrons easy. The material is also of effective pulse shape discrimination. The figure-of-merit for discrimination of gamma rays and thermal neutrons in CLLBC can be as high as 3.2, which is comparable to that of CLYC.

Observation of hard X-rays from the Crab pulsar and A0535+26

NASA Technical Reports Server (NTRS)

Wu, M.; Dai, C.; Lu, Z.; Ma, Y.; Li, G.; Fan, Z.; Zhang, C.; Xu, C.; Zhang, X.; Gu, Y.

1985-01-01

The Crab pulsar PSR0531+21 was observed in a balloon flight from the Xianghe Balloon Station (China). Data were obtained in the range 20 to 200 keV with a poswish hard X-ray telescope which comprised a 150 sq cm primary crystal of 5 mm thick CsI(T1) which actively shielded the lower 2 pi steradians by a 5 cm thick NaI(T1) crystal. The scintillation pulses originating in CsI and NaI crystals are distinguished by pulse shape discrimination. The telescope has a field of view of approximately 4 deg H psi H pi determined by graded shield and collimator. The effective geometric area of the detector is 116 sq cm. It is noted that when folding a data flow on a long period interference from the data acquisition, transmission and recording system considerably affect the result.

Deriving depth-dependent light escape efficiency and optical Swank factor from measured pulse height spectra of scintillators.

PubMed

Howansky, Adrian; Peng, Boyu; Lubinsky, Anthony R; Zhao, Wei

2017-03-01

Pulse height spectroscopy has been used by investigators to deduce the imaging properties of scintillators. Pulse height spectra (PHS) are used to compute the Swank factor, which describes the variation in scintillator light output per x-ray interaction. The spread in PHS measured below the K-edge is related to the optical component of the Swank factor, i.e., variations in light escape efficiency from different depths of x-ray interaction in the scintillator, denoted ε¯(z). Optimizing scintillators for medical imaging applications requires understanding of these optical properties, as they determine tradeoffs between parameters such as x-ray absorption, light yield, and spatial resolution. This work develops a model for PHS acquisition such that the effect of measurement uncertainty can be removed. This method allows ε¯(z) to be quantified on an absolute scale and permits more accurate estimation of the optical Swank factor of scintillators. The pulse height spectroscopy acquisition chain was modeled as a linear system of stochastic gain stages. Analytical expressions were derived for signal and noise propagation through the PHS chain, accounting for deterministic and stochastic aspects of x-ray absorption, scintillation, and light detection with a photomultiplier tube. The derived expressions were used to calculate PHS of thallium-doped cesium iodide (CsI) scintillators using parameters that were measured, calculated, or known from literature. PHS were measured at 25 and 32 keV of CsI samples designed with an optically reflective or absorptive backing, with or without a fiber-optic faceplate (FOP), and with thicknesses ranging from 150-1000 μm. Measured PHS were compared with calculated PHS, then light escape model parameters were varied until measured and modeled results reached agreement. Resulting estimates of ε¯(z) were used to calculate each scintillator's optical Swank factor. For scintillators of the same optical design, only minor differences in light escape efficiency were observed between samples with different thickness. As thickness increased, escape efficiency decreased by up to 20% for interactions furthest away from light collection. Optical design (i.e., backing and FOP) predominantly affected the magnitude and relative variation in ε¯(z). Depending on interaction depth and scintillator thickness, samples with an absorptive backing and FOP were estimated to yield 4.1-13.4 photons/keV. Samples with a reflective backing and FOP yielded 10.4-18.4 keV -1 , while those with a reflective backing and no FOP yielded 29.5-52.0 keV -1 . Optical Swank factors were approximately 0.9 and near-unity in samples featuring an absorptive or reflective backing, respectively. This work uses a modeling approach to remove the noise introduced by the measurement apparatus from measured PHS. This method allows absolute quantification of ε¯(z) and more accurate estimation of the optical Swank factor of scintillators. The method was applied to CsI scintillators with different thickness and optical design, and determined that optical design more strongly affects ε¯(z) and Swank factor than differences in CsI thickness. Despite large variations in ε¯(z) between optical designs, the Swank factor of all evaluated samples is above 0.9. Information provided by this methodology can help validate Monte Carlo simulations of structured CsI and optimize scintillator design for x-ray imaging applications. © 2016 American Association of Physicists in Medicine.

The 3 H(d , γ) Reaction at Ec . m . <= 300 keV

NASA Astrophysics Data System (ADS)

Parker, C. E.; Brune, C. R.; Massey, T. N.; O'Donnell, J. E.; Richard, A. L.; Sayre, D. B.

2015-04-01

The 3 H(d , γ) 5He reaction has been measured using a 500-keV pulsed deuteron beam incident on a stopping titanium tritide target at the Edwards Accelerator Laboratory. The time-of-flight technique has been used to distinguish the γ-rays from neutrons in the bismuth germinate (BGO) γ-ray detector. A stilbene scintillator and an NE-213 scintillator have been used to detect the neutrons from the 3 H(d , n) α reaction using both the pulse-shape discrimination and time-of-flight techniques. A newly designed target holder with a silicon surface barrier detector to simultaneously measure α-particles to normalize the number of neutrons, along with a new titanium tritide target, was incorporated for subsequent measurements. The γ-rays have been measured at laboratory angles of 0 °, 45 °, 90 °, and 135 °. Information about the γ-ray energy distribution for the unbound ground state and first excited state of 5He can be obtained experimentally by comparing the BGO data to Monte Carlo simulations. The 3 H(d , γ) /3 H(d , n) branching ratio has also been measured. Data analysis is currently underway for the subsequent measurements. This work is supported in part by Lawrence Livermore National Laboratory and the U.S. D.O.E. (NNSA) through Grant No. DE-NA0001837.

The 3H(d,gamma) Reaction and the 3 H(d,gamma)/ 3H(d, n) Branching Ratio for Ec.m. 300 keV

NASA Astrophysics Data System (ADS)

Parker, Cody E.

The 3H(d, gamma)5He reaction and the 3H(d, gamma)/3H(d, n) branching ratio have been measured using a 500-keV pulsed deuteron beam incident on a titanium tritide target of stopping thickness at the Edwards Accelerator Laboratory. The time-of-flight technique has been used to distinguish the gamma-rays from neutrons in the bismuth germinate (BGO) gamma-ray detector. A stilbene scintillator and an NE-213 scintillator have been used to detect the neutrons from the 3H(d, n)alpha reaction using both the pulse-shape discrimination and time-of-flight techniques. A target holder with an ion-implanted silicon detector at a fixed angle of 135° to the beam axis to simultaneously measure alpha-particles as a normalization for the number of neutrons was incorporated to reduce the uncertainty in the neutron yield over the preliminary measurement. The gamma-rays have been measured at laboratory angles of 0°, 4°, 9°, and 15°. Information about the gamma-ray energy distribution for the unbound ground state and first excited state of 5He have been obtained experimentally by comparing the BGO data to Monte Carlo simulations. The reported branching ratios for each angle contain only contributions from the ground-state gamma-ray branch.

Development of a miniature phoswich-based detector for 1-10 MeV solar neutrons

NASA Astrophysics Data System (ADS)

McKibben, R. Bruce; Connell, James; Bancroft, Christopher M.; Bravar, Ulisse; Pirard, Benoit; Wood, Joshua R.

We report on the initial development and test of a simple miniaturized detector for 1-10 MeV neutrons using phoswich techniques to isolate neutrons from background caused by energetic charged particles. The basic concept consists of a small plastic scintillator completely surrounded by an inorganic scintillator (CsI(Tl)) and viewed by a single compact PM tube. An incident neutron usually passes through the CsI(Tl) without producing a signal and then, through elastic scattering with a proton in the plastic, can produce a scintillation signal in the plastic. An energetic charged particle, on the other hand, would always produce scintillation in both the plastic and CsI(Tl). Making use of the pronounced difference in scintillation speeds between the plastic scintillator (nano-seconds) and the CsI(Tl) scintillator (microseconds), we exclude energetic charged particles by rejecting any signal that lasts more than a few 10s of nanoseconds. The amplitude of the signal from the plastic provides information about the energy of the scattered neutron which, though not definitive event-by-event, can be used to derive information about the neutron spectrum by applying a fitting procedure to the distribution of pulse sizes. The ultimate goal is to develop a detector that will enable studies of low energy solar neutrons on severely mass and power constrained deep space missions that approach the Sun. At energies below 10 MeV, neutrons produced at the Sun do not survive in significant numbers to reach a radius of 1 AU, and are therefore measurable only from observation points well inside the orbit of Earth. These low energy neutrons provide unique information on fluxes of energetic protons and helium nuclei interacting with the denser regions of the lower corona and chromosphere, whether or not these accelerated particles escape the strong magnetic fields in the lower corona to reach interplanetary space. Our efforts to date have consisted of design and construction of a proto-type sensor, including breadboard front-end electronics to make the pulse-shape discrimination, simulation of its response to mono-energetic neutrons using the GEANT-4 Monte Carlo code, and experimental studies of the response of the sensor to radioactive sources and to nearly monoenergetic beams of neutrons produced at the Crocker Nuclear Laboratory at the University of California at Davis. We report the results of our efforts to date, and discuss further work that remains to be done, as well as possible alternative applications for the sensor. This work was supported in part by NASA Grant NNG06GD56G. We are grateful for many useful discussions with James Ryan of the University of New Hampshire and members of his group.

Plastic Scintillator Based Detector for Observations of Terrestrial Gamma-ray Flashes.

NASA Astrophysics Data System (ADS)

Barghi, M. R., Sr.; Delaney, N.; Forouzani, A.; Wells, E.; Parab, A.; Smith, D.; Martinez, F.; Bowers, G. S.; Sample, J.

2017-12-01

We present an overview of the concept and design of the Light and Fast TGF Recorder (LAFTR), a balloon borne gamma-ray detector designed to observe Terrestrial Gamma-Ray Flashes (TGFs). Terrestrial Gamma-Ray Flashes (TGFs) are extremely bright, sub-millisecond bursts of gamma-rays observed to originate inside thunderclouds coincident with lightning. LAFTR is joint institutional project built by undergraduates at the University of California Santa Cruz and Montana State University. It consists of a detector system fed into analog front-end electronics and digital processing. The presentation focuses specifically on the UCSC components, which consists of the detector system and analog front-end electronics. Because of the extremely high count rates observed during TGFs, speed is essential for both the detector and electronics of the instrument. The detector employs a fast plastic scintillator (BC-408) read out by a SensL Silicon Photomultiplier (SiPM). BC-408 is chosen for its speed ( 4 ns decay time) and low cost and availability. Furthermore, GEANT3 simulations confirm the scintillator is sensitive to 500 counts at 7 km horizontal distance from the TGF source (for a 13 km source altitude and 26 km balloon altitude) and to 5 counts out to 20 km. The signal from the SiPM has a long exponential decay tail and is sent to a custom shaping circuit board that amplifies and shapes the signal into a semi-Gaussian pulse with a 40 ns FWHM. The signal is then input to a 6-channel discriminator board that clamps the signal and outputs a Low Voltage Differential Signal (LVDS) for processing by the digital electronics.

A neutron Albedo system with time rejection for landmine and IED detection

NASA Astrophysics Data System (ADS)

Kovaltchouk, V. D.; Andrews, H. R.; Clifford, E. T. H.; Faust, A. A.; Ing, H.; McFee, J. E.

2011-10-01

A neutron Albedo system has been developed for imaging of buried landmines and improvised explosive devices (IEDs). It involves irradiating the ground with fast neutrons and subsequently detecting the thermalized neutrons that return. A scintillating 6Li loaded ZnS(Ag) screen with a sensitive area of 40 cm×40 cm is used as a thermal neutron detector. Scintillation light is captured by orthogonal arrays of wavelength-shifting fibers placed on either side of the scintillator surface and then transferred to X and Y multi-pixel PMTs. A timing circuit, used with pulsed neutron sources, records the time when a neutron detection takes place relative to an external synchronization pulse from the pulsed source. Experimental tests of the Albedo system performance have been done in a sand box with a 252Cf neutron source (no time gating) and with pulsed D-D (2.6 MeV) neutrons from the Defense R&D Ottawa Van de Graaff accelerator (with time gating). Information contained in the time evolution of the thermal neutron field provided improved detection capability and image reconstruction. The detector design is described and experimental results are discussed.

Deriving depth-dependent light escape efficiency and optical Swank factor from measured pulse height spectra of scintillators

PubMed Central

Howansky, Adrian; Peng, Boyu; Lubinsky, Anthony R.; Zhao, Wei

2017-01-01

Purpose Pulse height spectroscopy has been used by investigators to deduce the imaging properties of scintillators. Pulse height spectra (PHS) are used to compute the Swank factor, which describes the variation in scintillator light output per x-ray interaction. The spread in PHS measured below the K-edge is related to the optical component of the Swank factor, i.e. variations in light escape efficiency from different depths of x-ray interaction in the scintillator, denoted ε̄(z). Optimizing scintillators for medical imaging applications requires understanding of these optical properties, as they determine tradeoffs between parameters such as x-ray absorption, light yield, and spatial resolution. This work develops a model for PHS acquisition such that the effect of measurement uncertainty can be removed. This method allows ε̄(z) to be quantified on an absolute scale and permits more accurate estimation of the optical Swank factor of scintillators. Methods The pulse height spectroscopy acquisition chain was modeled as a linear system of stochastic gain stages. Analytical expressions were derived for signal and noise propagation through the PHS chain, accounting for deterministic and stochastic aspects of x-ray absorption, scintillation, and light detection with a photomultiplier tube. The derived expressions were used to calculate PHS of thallium-doped cesium iodide (CsI) scintillators using parameters that were measured, calculated, or known from literature. PHS were measured at 25 and 32 keV of CsI samples designed with an optically-reflective or absorptive backing, with or without a fiber-optic faceplate (FOP), and with thicknesses ranging from 150–1000 μm. Measured PHS were compared with calculated PHS, then light escape model parameters were varied until measured and modeled results reached agreement. Resulting estimates of ε̄(z) were used to calculate each scintillator’s optical Swank factor. Results For scintillators of the same optical design, only minor differences in light escape efficiency were observed between samples with different thickness. As thickness increased, escape efficiency decreased by up to 20% for interactions furthest away from light collection. Optical design (i.e. backing and FOP) predominantly affected the magnitude and relative variation in ε̄(z). Depending on interaction depth and scintillator thickness, samples with an absorptive backing and FOP were estimated to yield 4.1–13.4 photons/keV. Samples with a reflective backing and FOP yielded 10.4–18.4 keV−1, while those with a reflective backing and no FOP yielded 29.5–52.0 keV−1. Optical Swank factors were approximately 0.9 and near-unity in samples featuring an absorptive or reflective backing, respectively. Conclusions This work uses a modeling approach to remove the noise introduced by the measurement apparatus from measured PHS. This method allows absolute quantification of ε̄(z) and more accurate estimation of the optical Swank factor of scintillators. The method was applied to CsI scintillators with different thickness and optical design, and determined that optical design more strongly affects ε̄(z) and Swank factor than differences in CsI thickness. Despite large variations in ε̄(z) between optical designs, the Swank factor of all evaluated samples is above 0.9. Information provided by this methodology can help validate Monte Carlo simulations of structured CsI and optimize scintillator design for x-ray imaging applications. PMID:28039881

Elastic and Inelastic Scattering of Neutrons using a CLYC array

NASA Astrophysics Data System (ADS)

Brown, Tristan; Doucet, E.; Chowdhury, P.; Lister, C. J.; Wilson, G. L.; Devlin, M.; Mosby, S.

2015-10-01

CLYC scintillators, which have dual neutron and gamma response, have recently ushered in the possibility of fast neutron spectroscopy without time-of-flight (TOF). A 16-element array of 1'' x 1'' 6Li-depleted CLYC crystals, where pulse-shape-discrimination is achieved via digital pulse processing, has been commissioned at UMass Lowell. In an experiment at LANSCE, high energy neutrons were used to bombard 56Fe and 238U targets, in order to measure elastic and inelastic neutron scattering cross sections as a function of energy and angle with the array. The array is placed very close to the targets for enhanced geometrical solid angles for scattered neutrons compared to standard neutron-TOF measurements. A pulse-height spectrum of scattered neutrons in the detectors is compared to the energy of the incident neutrons, which is measured via the TOF of the pulsed neutrons from the source to the detectors. Recoil corrections are necessary to combine the energy spectra from all the detectors to obtain angle-integrated elastic and inelastic cross-sections. The detection techniques, analysis procedures and results will be presented. Supported by NNSA-SSAA program through DOE Grant DE-NA00013008.

Radon backgrounds in the DEAP-1 liquid-argon-based Dark Matter detector

NASA Astrophysics Data System (ADS)

Amaudruz, P.-A.; Batygov, M.; Beltran, B.; Boudjemline, K.; Boulay, M. G.; Cai, B.; Caldwell, T.; Chen, M.; Chouinard, R.; Cleveland, B. T.; Contreras, D.; Dering, K.; Duncan, F.; Ford, R.; Gagnon, R.; Giuliani, F.; Gold, M.; Golovko, V. V.; Gorel, P.; Graham, K.; Grant, D. R.; Hakobyan, R.; Hallin, A. L.; Harvey, P.; Hearns, C.; Jillings, C. J.; Kuźniak, M.; Lawson, I.; Li, O.; Lidgard, J.; Liimatainen, P.; Lippincott, W. H.; Mathew, R.; McDonald, A. B.; McElroy, T.; McFarlane, K.; McKinsey, D.; Muir, A.; Nantais, C.; Nicolics, K.; Nikkel, J.; Noble, T.; O'Dwyer, E.; Olsen, K. S.; Ouellet, C.; Pasuthip, P.; Pollmann, T.; Rau, W.; Retiere, F.; Ronquest, M.; Skensved, P.; Sonley, T.; Tang, J.; Vázquez-Jáuregui, E.; Veloce, L.; Ward, M.

2015-03-01

The DEAP-1 7 kg single phase liquid argon scintillation detector was operated underground at SNOLAB in order to test the techniques and measure the backgrounds inherent to single phase detection, in support of the DEAP-3600 Dark Matter detector. Backgrounds in DEAP are controlled through material selection, construction techniques, pulse shape discrimination, and event reconstruction. This report details the analysis of background events observed in three iterations of the DEAP-1 detector, and the measures taken to reduce them. The 222 Rn decay rate in the liquid argon was measured to be between 16 and 26 μBq kg-1. We found that the background spectrum near the region of interest for Dark Matter detection in the DEAP-1 detector can be described considering events from three sources: radon daughters decaying on the surface of the active volume, the expected rate of electromagnetic events misidentified as nuclear recoils due to inefficiencies in the pulse shape discrimination, and leakage of events from outside the fiducial volume due to imperfect position reconstruction. These backgrounds statistically account for all observed events, and they will be strongly reduced in the DEAP-3600 detector due to its higher light yield and simpler geometry.

Detector optimization for hand-held CsI(Tl)/HgI{sub 2} gamma-ray scintillation spectrometer applications

DOE Office of Scientific and Technical Information (OSTI.GOV)

Wang, Y.J.; Patt, B.E.; Iwanczyk, J.S.

Gamma-ray spectrometers using mercuric iodide (HgI{sub 2}) photodetectors (PDs) coupled with CsI(Tl) scintillators have shown excellent energy resolutions and high detection efficiency at room temperature. Additionally HgI{sub 2} semiconductor PDs allow for extreme miniaturization of the detector packaging compared with photomultiplier tube (PMT) based detectors. These advantages make possible the construction of a new generation of hand-held gamma-ray spectrometers. Studies of detector optimization for this application have been undertaken. Several contact materials including hydrogen and semi-transparent metal films have been evaluated and compared for their performances and long term stability. In order to provide higher gamma-ray detection efficiency (i.e., largermore » scintillator volume), but without causing significant degradation of the excellent response achieved with the matched scintillator/PD interface, the scintillator/PD configuration has been studied. A Monte Carlo simulation model has been developed so that the spectral shape can be predicted for various scintillator shapes and surface treatments.« less

Configuring and Characterizing X-Rays for Laser-Driven Compression Experiments at the Dynamic Compression Sector

NASA Astrophysics Data System (ADS)

Li, Y.; Capatina, D.; D'Amico, K.; Eng, P.; Hawreliak, J.; Graber, T.; Rickerson, D.; Klug, J.; Rigg, P. A.; Gupta, Y. M.

2017-06-01

Coupling laser-driven compression experiments to the x-ray beam at the Dynamic Compression Sector (DCS) at the Advanced Photon Source (APS) of Argonne National Laboratory requires state-of-the-art x-ray focusing, pulse isolation, and diagnostics capabilities. The 100J UV pulsed laser system can be fired once every 20 minutes so precise alignment and focusing of the x-rays on each new sample must be fast and reproducible. Multiple Kirkpatrick-Baez (KB) mirrors are used to achieve a focal spot size as small as 50 μm at the target, while the strategic placement of scintillating screens, cameras, and detectors allows for fast diagnosis of the beam shape, intensity, and alignment of the sample to the x-ray beam. In addition, a series of x-ray choppers and shutters are used to ensure that the sample is exposed to only a single x-ray pulse ( 80ps) during the dynamic compression event and require highly precise synchronization. Details of the technical requirements, layout, and performance of these instruments will be presented. Work supported by DOE/NNSA.

The Effect of Photon Statistics and Pulse Shaping on the Performance of the Wiener Filter Crystal Identification Algorithm Applied to LabPET Phoswich Detectors

NASA Astrophysics Data System (ADS)

Yousefzadeh, Hoorvash Camilia; Lecomte, Roger; Fontaine, Réjean

2012-06-01

A fast Wiener filter-based crystal identification (WFCI) algorithm was recently developed to discriminate crystals with close scintillation decay times in phoswich detectors. Despite the promising performance of WFCI, the influence of various physical factors and electrical noise sources of the data acquisition chain (DAQ) on the crystal identification process was not fully investigated. This paper examines the effect of different noise sources, such as photon statistics, avalanche photodiode (APD) excess multiplication noise, and front-end electronic noise, as well as the influence of different shaping filters on the performance of the WFCI algorithm. To this end, a PET-like signal simulator based on a model of the LabPET DAQ, a small animal APD-based digital PET scanner, was developed. Simulated signals were generated under various noise conditions with CR-RC shapers of order 1, 3, and 5 having different time constants (τ). Applying the WFCI algorithm to these simulated signals showed that the non-stationary Poisson photon statistics is the main contributor to the identification error of WFCI algorithm. A shaping filter of order 1 with τ = 50 ns yielded the best WFCI performance (error 1%), while a longer shaping time of τ = 100 ns slightly degraded the WFCI performance (error 3%). Filters of higher orders with fast shaping time constants (10-33 ns) also produced good WFCI results (error 1.4% to 1.6%). This study shows the advantage of the pulse simulator in evaluating various DAQ conditions and confirms the influence of the detection chain on the WFCI performance.

Ames collaborative study of cosmic ray neutrons

NASA Technical Reports Server (NTRS)

Hewitt, J. E.; Hughes, L.; Mccaslin, J. B.; Stephens, L. D.; Rindi, A.; Smith, A. R.; Thomas, R. H.; Griffith, R. V.; Welles, C. G.; Baum, J. W.

1976-01-01

The results of a collaborative study to define both the neutron flux and the spectrum more precisely and to develop a dosimetry package that can be flown quickly to altitude for solar flare events are described. Instrumentation and analysis techniques were used which were developed to measure accelerator-produced radiation. The instruments were flown in the Ames Research Center high altitude aircraft. Neutron instrumentation consisted of Bonner spheres with both active and passive detector elements, threshold detectors of both prompt-counter and activation-element types, a liquid scintillation spectrometer based on pulse-shape discrimination, and a moderated BF3 counter neutron monitor. In addition, charged particles were measured with a Reuter-Stokes ionization chamber system and dose equivalent with another instrument. Preliminary results from the first series of flights at 12.5 km (41,000 ft) are presented, including estimates of total neutron flux intensity and spectral shape and of the variation of intensity with altitude and geomagnetic latitude.

Time correlated measurements using plastic scintillators with neutron-photon pulse shape discrimination

NASA Astrophysics Data System (ADS)

Richardson, Norman E., IV

Since the beginning of the nuclear age, there has been a strong demand for the development of efficient technologies for the detection of ionizing radiation. According to the United States' Department of Energy, the accurate assessment of fissile materials is essential in achieving the nonproliferation goals of enhancing safety and security of nuclear fuel cycle and nuclear energy facilities. Nuclear materials can be characterized by the measurement of prompt and delayed neutrons and gamma rays emitted in spontaneous or induced fission reactions and neutrons emitted in fission reactions are the distinctive signatures of nuclear materials. Today, the most widely used neutron detection technologies rely on thermal neutron capture reactions using a moderating material to cause the neutron to lose its energy prior to the detection event. This is necessary because as the fission event occurs, neutrons are emitted carrying high amounts of energy, typically on the order of mega electron volts (MeV). These energetic particles are classified as "fast" neutrons. For detecting the thermal neutrons, the Helium-3 (3He) gas-filled counters are arguably the most widely used technology of neutron detection. 3He counters have been the scientific standard for the nuclear engineering community for several decades, and have earned their place as a reliable technique for the detection of neutrons. However, 3He gas-filled counters have several disadvantages. First, gas-filled counters are not rigid and are sensitive to vibrations. Secondly, gas-filled counters are prone to the count rate limitations due to the physical processes of charge multiplication and transport in the gas medium in the electric field. Lastly, 3He gas-filled counters suffer from a supply shortage of the 3He isotope. As it is stated in [3], this shortage is created by the new demand for Helium-3 due to the deployment of neutron detectors at the borders after the 9/11 attack to help secure the nation against smuggled nuclear and radiological material. Moreover, the production of 3He isotope as a byproduct of security programs was drastically decreased. This isotope shortage coupled with the disadvantages of relying on a detector that requires neutron moderation before the detection of fission neutrons, poses a significant challenge in supporting the existing detection systems and the development of future technologies. To address this problem, a reliable and accurate alternative technology to detect neutrons emitted in fissions must be developed. One such alternative technology that shows promise in this application is the use of scintillators based on solid state materials (plastics) which are sensitive to fast neutrons. However, plastic scintillators are also sensitive to photons. Hence, it is necessary to separate the neutron signals from the photon signals, using the pulse shape discrimination (PSD) analysis. The PSD is based on the comparison of the pulse shapes of digitized signal waveforms. This approach allows for the measurement of fast neutrons without the necessity of their moderation. Because the fission spectrum neutrons are mainly fast, methods employing fast neutron detection are applicable for the assay of fissile materials. In addition, the average time of scintillation of the plastic medium is much shorter than those of the gaseous counters, thus allowing scintillation detectors to be used in high count rate environments. Furthermore, the temporal information of the fast neutron detection using multiple sensors enables the time correlation analysis of the fission neutron multiplicity. The study of time correlation measurements of fast neutrons using the array of plastic scintillators is the basis of this work. The array of four plastic scintillator detectors equipped with the digital data acquisition and analysis system was developed. The digital PSD analysis of detector signals "on-the-fly" was implemented for the array. The time coincidence measurement technique using the list mode was employed for two detectors operating on the single time scale. This was necessary as no fission source was available to be used as a fast neutron multiplicity source. The detection technology was tested using isotopic photon sources and a plutonium-beryllium neutron source. It was shown that the system can be effectively used for fast-neutron multiplicity measurements, through a "proof-of-concept" model, enabling a shorter width of the time coincidence window compared to the 3He counters. This result opens prospects to reduce the false coincidence rates in the neutron multiplicity measurements, thus increasing the sensitivity of nuclear material detection.

Optimum design calculations for detectors based on ZnSe(Те,О) scintillators

NASA Astrophysics Data System (ADS)

Katrunov, K.; Ryzhikov, V.; Gavrilyuk, V.; Naydenov, S.; Lysetska, O.; Litichevskyi, V.

2013-06-01

Light collection in scintillators ZnSe(X), where X is an isovalent dopant, was studied using Monte Carlo calculations. Optimum design was determined for detectors of "scintillator—Si-photodiode" type, which can involve either one scintillation element or scintillation layers of large area made of small-crystalline grains. The calculations were carried out both for determination of the optimum scintillator shape and for design optimization of light guides, on the surface of which the layer of small-crystalline grains is formed.

PSA discriminator influence on (222)Rn efficiency detection in waters by liquid scintillation counting.

PubMed

Stojković, Ivana; Todorović, Nataša; Nikolov, Jovana; Tenjović, Branislava

2016-06-01

A procedure for the (222)Rn determination in aqueous samples using liquid scintillation counting (LSC) was evaluated and optimized. Measurements were performed by ultra-low background spectrometer Quantulus 1220™ equipped with PSA (Pulse Shape Analysis) circuit which discriminates alpha/beta spectra. Since calibration procedure is carried out with (226)Ra standard, which has both alpha and beta progenies, it is clear that PSA discriminator has vital importance in order to provide precise spectra separation. Improvement of calibration procedure was done through investigation of PSA discriminator level and, consequentially, the activity of (226)Ra calibration standard influence on (222)Rn efficiency detection. Quench effects on generated spectra i.e. determination of radon efficiency detection were also investigated with quench calibration curve obtained. Radon determination in waters based on modified procedure according to the activity of (226)Ra standard used, dependent on PSA setup, was evaluated with prepared (226)Ra solution samples and drinking water samples with assessment of measurement uncertainty variation included. Copyright © 2016 Elsevier Ltd. All rights reserved.

Real-Time, Fast Neutron Coincidence Assay of Plutonium With a 4-Channel Multiplexed Analyzer and Organic Scintillators

NASA Astrophysics Data System (ADS)

Joyce, Malcolm J.; Gamage, Kelum A. A.; Aspinall, M. D.; Cave, F. D.; Lavietes, A.

2014-06-01

The design, principle of operation and the results of measurements made with a four-channel organic scintillator system are described. The system comprises four detectors and a multiplexed analyzer for the real-time parallel processing of fast neutron events. The function of the real-time, digital multiple-channel pulse-shape discrimination analyzer is described together with the results of laboratory-based measurements with 252Cf, 241Am-Li and plutonium. The analyzer is based on a single-board solution with integrated high-voltage supplies and graphical user interface. It has been developed to meet the requirements of nuclear materials assay of relevance to safeguards and security. Data are presented for the real-time coincidence assay of plutonium in terms of doubles count rate versus mass. This includes an assessment of the limiting mass uncertainty for coincidence assay based on a 100 s measurement period and samples in the range 0-50 g. Measurements of count rate versus order of multiplicity for 252Cf and 241Am-Li and combinations of both are also presented.

Evaluation of a digital data acquisition system and optimization of n-γ discrimination for a compact neutron spectrometer.

PubMed

Giacomelli, L; Zimbal, A; Reginatto, M; Tittelmeier, K

2011-01-01

A compact NE213 liquid scintillation neutron spectrometer with a new digital data acquisition (DAQ) system is now in operation at the Physikalisch-Technische Bundesanstalt (PTB). With the DAQ system, developed by ENEA Frascati, neutron spectrometry with high count rates in the order of 5×10(5) s(-1) is possible, roughly an order of magnitude higher than with an analog acquisition system. To validate the DAQ system, a new data analysis code was developed and tests were done using measurements with 14-MeV neutrons made at the PTB accelerator. Additional analysis was carried out to optimize the two-gate method used for neutron and gamma (n-γ) discrimination. The best results were obtained with gates of 35 ns and 80 ns. This indicates that the fast and medium decay time components of the NE213 light emission are the ones that are relevant for n-γ discrimination with the digital acquisition system. This differs from what is normally implemented in the analog pulse shape discrimination modules, namely, the fast and long decay emissions of the scintillating light.

Advances in Neutron Spectroscopy with Deuterated Organic Scintillators

NASA Astrophysics Data System (ADS)

Febbraro, Michael; Pain, Steve; Becchetti, Frederick

2015-10-01

Deuterated organic scintillators have shown promise as neutron detectors for nuclear science as well as applications in nuclear non-proliferation and safeguards. In particular, they can extract neutron spectra without the use of neutron time-of-flight measurement (n-ToF) utilizing spectrum unfolding techniques. This permits the measure of cross sections of bound and unbound states with high efficiency and angular coverage. In the case of measurements with radioactive ion beams where low beam intensities limit long path n-ToF, short path n-ToF can be used to discriminate neutrons of interest from room return and background neutrons. This presentation will provide recent advances with these types of detectors. Digital pulse-shape discrimination using fast waveform digitizers, spectrum unfolding methods for extraction of neutron spectra, and a new safer deuterated-xylene formulation EJ-301D will be discussed. In addition, experimental results from measurements of discrete and continuous neutron spectra which illustrate the advantage of these detectors for certain applications in nuclear physics research and nuclear security will be shown. This work is supported by NSF and DOE.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ramirez, A. P. D.; Vanhoy, J. R.; Hicks, S. F.

Elastic and inelastic differential cross sections for neutron scattering from 56Fe have been measured for several incident energies from 1.30 to 7.96 MeV at the University of Kentucky Accelerator Laboratory. Scattered neutrons were detected using a C 6D 6 liquid scintillation detector using pulse-shape discrimination and time-of-flight techniques. The deduced cross sections have been compared with previously reported data, predictions from evaluation databases ENDF, JENDL, and JEFF, and theoretical calculations performed using different optical model potentials using the TALYS and EMPIRE nuclear reaction codes. The coupled-channel calculations based on the vibrational and soft-rotor models are found to describe the experimentalmore » (n,n 0) and (n,n 1) cross sections well.« less

LArGe: active background suppression using argon scintillation for the Gerda 0ν β β -experiment

NASA Astrophysics Data System (ADS)

Agostini, M.; Barnabé-Heider, M.; Budjáš, D.; Cattadori, C.; Gangapshev, A.; Gusev, K.; Heisel, M.; Junker, M.; Klimenko, A.; Lubashevskiy, A.; Pelczar, K.; Schönert, S.; Smolnikov, A.; Zuzel, G.

2015-10-01

LArGe is a Gerda low-background test facility to study novel background suppression methods in a low-background environment, for future application in the Gerda experiment. Similar to Gerda, LArGe operates bare germanium detectors submersed into liquid argon (1 m^3, 1.4 tons), which in addition is instrumented with photomultipliers to detect argon scintillation light. The scintillation signals are used in anti-coincidence with the germanium detectors to effectively suppress background events that deposit energy in the liquid argon. The background suppression efficiency was studied in combination with a pulse shape discrimination (PSD) technique using a BEGe detector for various sources, which represent characteristic backgrounds to Gerda. Suppression factors of a few times 10^3 have been achieved. First background data of LArGe with a coaxial HPGe detector (without PSD) yield a background index of (0.12-4.6)× 10^{-2} cts/(keV kg year) (90 % C.L.), which is at the level of Gerda Phase I. Furthermore, for the first time we monitor the natural ^{42}Ar abundance (parallel to Gerda), and have indication for the 2ν β β -decay in natural germanium. These results show the effectivity of an active liquid argon veto in an ultra-low background environment. As a consequence, the implementation of a liquid argon veto in Gerda Phase II is pursued.

Development and deployment of the Collimated Directional Radiation Detection System

NASA Astrophysics Data System (ADS)

Guckes, Amber L.; Barzilov, Alexander

2017-09-01

The Collimated Directional Radiation Detection System (CDRDS) is capable of imaging radioactive sources in two dimensions (as a directional detector). The detection medium of the CDRDS is a single Cs2LiYCl6:Ce3+ scintillator cell enriched in 7Li (CLYC-7). The CLYC-7 is surrounded by a heterogeneous high-density polyethylene (HDPE) and lead (Pb) collimator. These materials make-up a coded aperture inlaid in the collimator. The collimator is rotated 360° by a stepper motor which enables time-encoded imaging of a radioactive source. The CDRDS is capable of spectroscopy and pulse shape discrimination (PSD) of photons and fast neutrons. The measurements of a radioactive source are carried out in discrete time steps that correlate to the angular rotation of the collimator. The measurement results are processed using a maximum likelihood expectation (MLEM) algorithm to create an image of the measured radiation. This collimator design allows for the directional detection of photons and fast neutrons simultaneously by utilizing only one CLYC-7 scintillator. Directional detection of thermal neutrons can also be performed by utilizing another suitable scintillator. Moreover, the CDRDS is portable, robust, and user friendly. This unit is capable of utilizing wireless data transfer for possible radiation mapping and network-centric applications. The CDRDS was tested by performing laboratory measurements with various gamma-ray and neutron sources.

Neutron kinetics in moderators and SNM detection through epithermal-neutron-induced fissions

NASA Astrophysics Data System (ADS)

Gozani, Tsahi; King, Michael J.

2016-01-01

Extension of the well-established Differential Die Away Analysis (DDAA) into a faster time domain, where more penetrating epithermal neutrons induce fissions, is proposed and demonstrated via simulations and experiments. In the proposed method the fissions stimulated by thermal, epithermal and even higher-energy neutrons are measured after injection of a narrow pulse of high-energy 14 MeV (d,T) or 2.5 MeV (d,D) source neutrons, appropriately moderated. The ability to measure these fissions stems from the inherent correlation of neutron energy and time ("E-T" correlation) during the process of slowing down of high-energy source neutrons in common moderating materials such as hydrogenous compounds (e.g., polyethylene), heavy water, beryllium and graphite. The kinetic behavior following injection of a delta-function-shaped pulse (in time) of 14 MeV neutrons into such moderators is studied employing MCNPX simulations and, when applicable, some simple "one-group" models. These calculations served as a guide for the design of a source moderator which was used in experiments. Qualitative relationships between slowing-down time after the pulse and the prevailing neutron energy are discussed. A laboratory system consisting of a 14 MeV neutron generator, a polyethylene-reflected Be moderator, a liquid scintillator with pulse-shape discrimination (PSD) and a two-parameter E-T data acquisition system was set up to measure prompt neutron and delayed gamma-ray fission signatures in a 19.5% enriched LEU sample. The measured time behavior of thermal and epithermal neutron fission signals agreed well with the detailed simulations. The laboratory system can readily be redesigned and deployed as a mobile inspection system for SNM in, e.g., cars and vans. A strong pulsed neutron generator with narrow pulse (<75 ns) at a reasonably high pulse frequency could make the high-energy neutron induced fission modality a realizable SNM detection technique.

YAP:Ce scintillator characteristics for neutron detection

DOE Office of Scientific and Technical Information (OSTI.GOV)

Viererbl, L.; Klupak, V.; Vins, M.

2015-07-01

YAP:Ce (YAlO{sub 3}:Ce{sup +}, Yttrium Aluminum Perovskite, Ce{sup +} doped) crystals with appropriate converters seem like prospective scintillators for neutron detection. An important aspect for neutron detection with inorganic scintillators is the ability to discriminate neutron radiation from gamma radiation by pulse height of signals. For a detailed measurement of the aspect, a YAP:Ce crystal scintillator with lithium or hydrogen converters and a photomultiplier was used. A plutonium-beryllium neutron source and horizontal neutron channel beams of the LVR-15 research reactor were used as neutron sources. The measurement confirmed the possibility to use the YAP:Ce scintillator for neutron radiation detection. Themore » degree of discrimination between neutron and gamma radiation for different detection configurations was studied. (authors)« less

Sub-luminal pulses from cosmic ray air showers

NASA Technical Reports Server (NTRS)

Linsley, J.

1985-01-01

Some of the signals produced by air showers in scintillators possess a distinctive feature, a sub-luminal pulse (SLP) following the normal one with a time delay of approximately 1.5 r/c. The average amplitude of the SLP corresponds to an energy deposit of about 50 MeV, three times as much as is deposited in a typical scintillator by vertical minimum ionizing muons. The SLP account for approximately 5% of the energy deposited in the atmosphere by IR showers with energy 10 to the 10th power GeV at impact parameters 1 km. Assuming that these pulses are due to neutrons travelling with a speed slightly less than c, they provide a unique means of estimating E sub h, the energy deposited by slow hadrons, in showers of this very high energy. On the other hand, if not allowed for properly, these pulses are liable to cause errors in estimating the impact parameters of large showers from pulse width observations.

A Wavelet Packet Transform Inspired Method of Neutron-Gamma Discrimination

NASA Astrophysics Data System (ADS)

Shippen, David I.; Joyce, Malcolm J.; Aspinall, Michael D.

2010-10-01

A Simplified Digital Charge Collection (SDCC) method of discrimination between neutron and gamma pulses in an organic scintillator is presented and compared to the Pulse Gradient Analysis (PGA) discrimination method. Data used in this research were gathered from events arising from the 7Li(p,n)7Be reaction detected by an EJ-301 organic liquid scintillator recorded with a fast digital oscilloscope. Time-of-Flight (TOF) data were also recorded and used as a second means of identification. The SDCC method is found to improve on the figure of merit (FOM) given by PGA method at the equivalent sampling rate.

Study on the Characteristics of a Scintillator for Beta-ray Detection using Epoxy Resin

NASA Astrophysics Data System (ADS)

Nam, Jong Soo; Choi, Yong Seok; Hong, Sang Bum; Seo, Bum Kyung; Moon, Jei Kwon; Choi, Jong Won

2017-09-01

A thin plate of a plastic scintillator for detecting a beta-ray was developed. The plastic scintillator was made using epoxy resin and organic scintillators such as 2.5-diphenyloxazole (PPO) and 1,4-bis [5-phenyl-2-oxazole] benzene (POPOP). The mixture ratio of epoxy resin and the organic scintillators was determined using their absorbance, transmittance, emission spectra, and transparency. Their optimal weight percentage of PPO and POPOP in the organic scintillators was adjusted to 0.2 wt%:0.01 wt%. The prepared plastic scintillator was used to measure the standard source of Sr-90. The pulse height spectra and total counts of the prepared plastic scintillator were similar to a commercial plastic scintillator. Based on the above results, a large-area plastic scintillator was prepared for rapid investigation of a site contaminated with Sr-90. The prepared large-area plastic scintillator was evaluated for the characteristics in the laboratory. The evaluation results are expected to be usefully utilized in the development of a large-area plastic scintillation detector. The large-area plastic scintillation detector developed on the basis of the evaluation results is expected to be utilized to quickly measure the contamination of Sr-90 in the grounds used as a nuclear power facility.

Novel scintillating material 2-(4-styrylphenyl)benzoxazole for the fully digital and MRI compatible J-PET tomograph based on plastic scintillators

PubMed Central

Dulski, Kamil; Niedźwiecki, Szymon; Alfs, Dominika; Białas, Piotr; Curceanu, Catalina; Czerwiński, Eryk; Danel, Andrzej; Gajos, Aleksander; Głowacz, Bartosz; Gorgol, Marek; Hiesmayr, Beatrix; Jasińska, Bożena; Kacprzak, Krzysztof; Kamińska, Daria; Kapłon, Łukasz; Kochanowski, Andrzej; Korcyl, Grzegorz; Kowalski, Paweł; Kozik, Tomasz; Krzemień, Wojciech; Kubicz, Ewelina; Kucharek, Mateusz; Mohammed, Muhsin; Pawlik-Niedźwiecka, Monika; Pałka, Marek; Raczyński, Lech; Rudy, Zbigniew; Rundel, Oleksandr; Sharma, Neha G.; Silarski, Michał; Uchacz, Tomasz; Wiślicki, Wojciech; Zgardzińska, Bożena; Zieliński, Marcin; Moskal, Paweł

2017-01-01

A novel plastic scintillator is developed for the application in the digital positron emission tomography (PET). The novelty of the concept lies in application of the 2-(4-styrylphenyl)benzoxazole as a wavelength shifter. The substance has not been used as scintillator dopant before. A dopant shifts the scintillation spectrum towards longer wavelengths making it more suitable for applications in scintillators of long strips geometry and light detection with digital silicon photomultipliers. These features open perspectives for the construction of the cost-effective and MRI-compatible PET scanner with the large field of view. In this article we present the synthesis method and characterize performance of the elaborated scintillator by determining its light emission spectrum, light emission efficiency, rising and decay time of the scintillation pulses and resulting timing resolution when applied in the positron emission tomography. The optimal concentration of the novel wavelength shifter was established by maximizing the light output and it was found to be 0.05 ‰ for cuboidal scintillator with dimensions of 14 mm x 14 mm x 20 mm. PMID:29176834

Novel scintillating material 2-(4-styrylphenyl)benzoxazole for the fully digital and MRI compatible J-PET tomograph based on plastic scintillators.

PubMed

Wieczorek, Anna; Dulski, Kamil; Niedźwiecki, Szymon; Alfs, Dominika; Białas, Piotr; Curceanu, Catalina; Czerwiński, Eryk; Danel, Andrzej; Gajos, Aleksander; Głowacz, Bartosz; Gorgol, Marek; Hiesmayr, Beatrix; Jasińska, Bożena; Kacprzak, Krzysztof; Kamińska, Daria; Kapłon, Łukasz; Kochanowski, Andrzej; Korcyl, Grzegorz; Kowalski, Paweł; Kozik, Tomasz; Krzemień, Wojciech; Kubicz, Ewelina; Kucharek, Mateusz; Mohammed, Muhsin; Pawlik-Niedźwiecka, Monika; Pałka, Marek; Raczyński, Lech; Rudy, Zbigniew; Rundel, Oleksandr; Sharma, Neha G; Silarski, Michał; Uchacz, Tomasz; Wiślicki, Wojciech; Zgardzińska, Bożena; Zieliński, Marcin; Moskal, Paweł

2017-01-01

A novel plastic scintillator is developed for the application in the digital positron emission tomography (PET). The novelty of the concept lies in application of the 2-(4-styrylphenyl)benzoxazole as a wavelength shifter. The substance has not been used as scintillator dopant before. A dopant shifts the scintillation spectrum towards longer wavelengths making it more suitable for applications in scintillators of long strips geometry and light detection with digital silicon photomultipliers. These features open perspectives for the construction of the cost-effective and MRI-compatible PET scanner with the large field of view. In this article we present the synthesis method and characterize performance of the elaborated scintillator by determining its light emission spectrum, light emission efficiency, rising and decay time of the scintillation pulses and resulting timing resolution when applied in the positron emission tomography. The optimal concentration of the novel wavelength shifter was established by maximizing the light output and it was found to be 0.05 ‰ for cuboidal scintillator with dimensions of 14 mm x 14 mm x 20 mm.

Optimizing ZnS/6LiF scintillators for wavelength-shifting-fiber neutron detectors

DOE Office of Scientific and Technical Information (OSTI.GOV)

Crow, Lowell; Funk, Loren L; Hannan, Bruce W

2016-01-01

In this paper we compare the performance of grooved and flat ZnS/6LiF scintillators in a wavelength shifting-fiber (WLSF) detector. Flat ZnS/6LiF scintillators with the thickness L=0.2-0.8 mm were characterized using photon counting and pulse-height analysis and compared to a grooved scintillator of approximately 0.8 mm thick. While a grooved scintillator considerably increases the apparent thickness of the scintillator to neutrons for a given coating thickness, we find that the flat scintillators perform better than the grooved scintillators in terms of both light yield and neutron detection efficiency. The flat 0.8-mm-thick scintillator has the highest light output, and it is 52%more » higher compared with a grooved scintillator of same thickness. The lower light output of the grooved scintillator as compared to the flat scintillator is consistent with the greater scintillator-WLSF separation and the much larger average emission angle of the grooved scintillator. We also find that the average light cone width, or photon travel-length as measured using time-of-flight powder diffraction of diamond and vanadium, decreases with increasing L in the range of L=0.6-0.8 mm. This result contrasts with the traditional Swank diffusion model for micro-composite scintillators, and could be explained by a decrease in photon diffusion-coefficient or an increase in micro-particle content in the flat scintillator matrix for the thicker scintillators.« less

Predicting the timing properties of phosphor-coated scintillators using Monte Carlo light transport simulation

PubMed Central

Roncali, Emilie; Schmall, Jeffrey P.; Viswanath, Varsha; Berg, Eric; Cherry, Simon R.

2014-01-01

Current developments in positron emission tomography (PET) focus on improving timing performance for scanners with time-of-flight (TOF) capability, and incorporating depth-of-interaction (DOI) information. Recent studies have shown that incorporating DOI correction in TOF detectors can improve timing resolution, and that DOI also becomes more important in long axial field-of-view scanners. We have previously reported the development of DOI-encoding detectors using phosphor-coated scintillation crystals; here we study the timing properties of those crystals to assess the feasibility of providing some level of DOI information without significantly degrading the timing performance. We used Monte Carlo simulations to provide a detailed understanding of light transport in phosphor-coated crystals which cannot be fully characterized experimentally. Our simulations used a custom reflectance model based on 3D crystal surface measurements. Lutetium oxyorthosilicate (LSO) crystals were simulated with a phosphor coating in contact with the scintillator surfaces and an external diffuse reflector (teflon). Light output, energy resolution, and pulse shape showed excellent agreement with experimental data obtained on 3 × 3 × 10 mm3 crystals coupled to a photomultiplier tube (PMT). Scintillator intrinsic timing resolution was simulated with head-on and side-on configurations, confirming the trends observed experimentally. These results indicate that the model may be used to predict timing properties in phosphor-coated crystals and guide the coating for optimal DOI resolution/timing performance trade-off for a given crystal geometry. Simulation data suggested that a time stamp generated from early photoelectrons minimizes degradation of the timing resolution, thus making this method potentially more useful for TOF-DOI detectors than our initial experiments suggested. Finally, this approach could easily be extended to the study of timing properties in other scintillation crystals, with a range of treatments and materials attached to the surface. PMID:24694727

Light yield in DarkSide-10: A prototype two-phase argon TPC for dark matter searches

NASA Astrophysics Data System (ADS)

Alexander, T.; Alton, D.; Arisaka, K.; Back, H. O.; Beltrame, P.; Benziger, J.; Bonfini, G.; Brigatti, A.; Brodsky, J.; Cadonati, L.; Calaprice, F.; Candela, A.; Cao, H.; Cavalcante, P.; Chavarria, A.; Chepurnov, A.; Cline, D.; Cocco, A. G.; Condon, C.; D'Angelo, D.; Davini, S.; De Haas, E.; Derbin, A.; Di Pietro, G.; Dratchnev, I.; Durben, D.; Empl, A.; Etenko, A.; Fan, A.; Fiorillo, G.; Fomenko, K.; Gabriele, F.; Galbiati, C.; Gazzana, S.; Ghag, C.; Ghiano, C.; Goretti, A.; Grandi, L.; Gromov, M.; Guan, M.; Guo, C.; Guray, G.; Hungerford, E. V.; Ianni, Al.; Ianni, An.; Kayunov, A.; Keeter, K.; Kendziora, C.; Kidner, S.; Kobychev, V.; Koh, G.; Korablev, D.; Korga, G.; Shields, E.; Li, P.; Loer, B.; Lombardi, P.; Love, C.; Ludhova, L.; Lukyanchenko, L.; Lund, A.; Lung, K.; Ma, Y.; Machulin, I.; Maricic, J.; Martoff, C. J.; Meng, Y.; Meroni, E.; Meyers, P. D.; Mohayai, T.; Montanari, D.; Montuschi, M.; Mosteiro, P.; Mount, B.; Muratova, V.; Nelson, A.; Nemtzow, A.; Nurakhov, N.; Orsini, M.; Ortica, F.; Pallavicini, M.; Pantic, E.; Parmeggiano, S.; Parsells, R.; Pelliccia, N.; Perasso, L.; Perfetto, F.; Pinsky, L.; Pocar, A.; Pordes, S.; Ranucci, G.; Razeto, A.; Romani, A.; Rossi, N.; Saggese, P.; Saldanha, R.; Salvo, C.; Sands, W.; Seigar, M.; Semenov, D.; Skorokhvatov, M.; Smirnov, O.; Sotnikov, A.; Sukhotin, S.; Suvorov, Y.; Tartaglia, R.; Tatarowicz, J.; Testera, G.; Teymourian, A.; Thompson, J.; Unzhakov, E.; Vogelaar, R. B.; Wang, H.; Westerdale, S.; Wojcik, M.; Wright, A.; Xu, J.; Yang, C.; Zavatarelli, S.; Zehfus, M.; Zhong, W.; Zuzel, G.

2013-09-01

As part of the DarkSide program of direct dark matter searches using two-phase argon TPCs, a prototype detector with an active volume containing 10 kg of liquid argon, DarkSide-10, was built and operated underground in the Gran Sasso National Laboratory in Italy. A critically important parameter for such devices is the scintillation light yield, as photon statistics limits the rejection of electron-recoil backgrounds by pulse shape discrimination. We have measured the light yield of DarkSide-10 using the readily-identifiable full-absorption peaks from gamma ray sources combined with single-photoelectron calibrations using low-occupancy laser pulses. For gamma lines of energies in the range 122-1275 keV, we get light yields averaging 8.887±0.003(stat)±0.444(sys) p.e./keVee. With additional purification, the light yield measured at 511 keV increased to 9.142±0.006(stat) p.e./keVee.

Investigating the origins of double photopeaks in CsI:Tl samples through activator mapping

NASA Astrophysics Data System (ADS)

Onken, Drew R.; Gridin, Sergii; Williams, Richard T.; Williams, Charles B.; Donati, George L.; Gayshan, Vadim; Vasyukov, Sergey; Gektin, Alex

2018-06-01

Careful examination of the origins of double photopeaks in CsI:Tl provides a foundation for exploring the relationship between activator homogeneity and photopeak resolution in scintillators. In rare cases, certain CsI:Tl crystals exhibit a second photopeak in the pulse-height spectrum. A combination of optical mapping and ICP-MS measurements reveals the presence of two distinct regions with differing Tl concentrations in these crystals. The oscillator strength of the 299 nm absorption A-band of Tl in CsI was measured to be 0.0526 ± 0.0008; this parameter can be used to quantify activator concentration from the optical absorption. Using published measurements of luminescence intensity versus Tl concentration, the distributions of Tl measured from optical absorption maps of the samples were reconstructed into photopeaks in good agreement with experiment. The distribution of Tl concentrations in these particular crystals allowed examining luminescence pulse shape as a function of Tl concentration.

Development of an alpha/beta/gamma detector for radiation monitoring

NASA Astrophysics Data System (ADS)

Yamamoto, Seiichi; Hatazawa, Jun

2011-11-01

For radiation monitoring at the site of nuclear power plant accidents such as Fukushima Daiichi, radiation detectors not only for gamma photons but also for alpha and beta particles are needed because some nuclear fission products emit beta particles and gamma photons and some nuclear fuels contain plutonium that emits alpha particles. We developed a radiation detector that can simultaneously monitor alpha and beta particles and gamma photons for radiation monitoring. The detector consists of three-layered scintillators optically coupled to each other and coupled to a photomultiplier tube. The first layer, which is made of a thin plastic scintillator (decay time: 2.4 ns), detects alpha particles. The second layer, which is made of a thin Gd2SiO5 (GSO) scintillator with 1.5 mol.% Ce (decay time: 35 ns), detects beta particles. The third layer made of a thin GSO scintillator with 0.4 mol.% Ce (decay time: 70 ns) detects gamma photons. By using pulse shape discrimination, the count rates of these layers can be separated. With individual irradiation of alpha and beta particles and gamma photons, the count rate of the first layer represented the alpha particles, the second layer represented the beta particles, and the third layer represented the gamma photons. Even with simultaneous irradiation of the alpha and beta particles and the gamma photons, these three types of radiation can be individually monitored using correction for the gamma detection efficiency of the second and third layers. Our developed alpha, beta, and gamma detector is simple and will be useful for radiation monitoring, especially at nuclear power plant accident sites or other applications where the simultaneous measurements of alpha and beta particles and gamma photons are required.

Development of high resolution phoswich depth-of-interaction block detectors utilizing Mg co-doped new scintillators

NASA Astrophysics Data System (ADS)

Kobayashi, Takahiro; Yamamoto, Seiichi; Yeom, Jung-Yeol; Kamada, Kei; Yoshikawa, Akira

2017-12-01

To correct for parallax error in positron emission tomography (PET), phoswich depth-of-interaction (DOI) detector using multiple scintillators with different decay times is a practical approach. However not many scintillator combinations suitable for phoswich DOI detector have been reported. Ce doped Gd3Ga3Al2O12 (GFAG) is a newly developed promising scintillator for PET detector, which has high density, high light output, appropriate light emission wavelength for silicon-photomultiplier (Si-PM) and faster decay time than that of Ce doped Gd3Al2Ga3O12 (GAGG). In this study, we developed a Si-PM based phoswich DOI block detector of GFAG with GAGG crystal arrays and evaluated its performance. We assembled a GFAG block and a GAGG block and they were optically coupled in depth direction to form a phoswich detector block. The phoswich block was optically coupled to a Si-PM array with a 1 mm thick light guide. The sizes of the GFAG and GAGG pixels were 0.9 mm x 0.9 mm x 7.5 mm and they were arranged into 24 x 24 matrix with 0.1 mm thick BaSO4 as reflector. We conducted the performance evaluation for two types of configurations; GFAG block arranged in upper layer (GFAG/GAGG) and GAGG arranged in upper layer (GAGG/GFAG). The measured two dimensional position histograms of these block detectors showed good separation and pulse shape spectra produced two distinct peaks for both configurations although some difference in energy spectra were observed. These results indicate phoswich block detectors composed of GFAG and GAGG are promising for high resolution DOI PET systems.

Development of an alpha/beta/gamma detector for radiation monitoring.

PubMed

Yamamoto, Seiichi; Hatazawa, Jun

2011-11-01

For radiation monitoring at the site of nuclear power plant accidents such as Fukushima Daiichi, radiation detectors not only for gamma photons but also for alpha and beta particles are needed because some nuclear fission products emit beta particles and gamma photons and some nuclear fuels contain plutonium that emits alpha particles. We developed a radiation detector that can simultaneously monitor alpha and beta particles and gamma photons for radiation monitoring. The detector consists of three-layered scintillators optically coupled to each other and coupled to a photomultiplier tube. The first layer, which is made of a thin plastic scintillator (decay time: 2.4 ns), detects alpha particles. The second layer, which is made of a thin Gd(2)SiO(5) (GSO) scintillator with 1.5 mol.% Ce (decay time: 35 ns), detects beta particles. The third layer made of a thin GSO scintillator with 0.4 mol.% Ce (decay time: 70 ns) detects gamma photons. By using pulse shape discrimination, the count rates of these layers can be separated. With individual irradiation of alpha and beta particles and gamma photons, the count rate of the first layer represented the alpha particles, the second layer represented the beta particles, and the third layer represented the gamma photons. Even with simultaneous irradiation of the alpha and beta particles and the gamma photons, these three types of radiation can be individually monitored using correction for the gamma detection efficiency of the second and third layers. Our developed alpha, beta, and gamma detector is simple and will be useful for radiation monitoring, especially at nuclear power plant accident sites or other applications where the simultaneous measurements of alpha and beta particles and gamma photons are required. © 2011 American Institute of Physics

Neutron scattering cross section measurements for Fe 56

DOE PAGES

Ramirez, A. P. D.; Vanhoy, J. R.; Hicks, S. F.; ...

2017-06-09

Elastic and inelastic differential cross sections for neutron scattering from 56Fe have been measured for several incident energies from 1.30 to 7.96 MeV at the University of Kentucky Accelerator Laboratory. Scattered neutrons were detected using a C 6D 6 liquid scintillation detector using pulse-shape discrimination and time-of-flight techniques. The deduced cross sections have been compared with previously reported data, predictions from evaluation databases ENDF, JENDL, and JEFF, and theoretical calculations performed using different optical model potentials using the TALYS and EMPIRE nuclear reaction codes. The coupled-channel calculations based on the vibrational and soft-rotor models are found to describe the experimentalmore » (n,n 0) and (n,n 1) cross sections well.« less

Neutron scattering cross section measurements for 56Fe

NASA Astrophysics Data System (ADS)

Ramirez, A. P. D.; Vanhoy, J. R.; Hicks, S. F.; McEllistrem, M. T.; Peters, E. E.; Mukhopadhyay, S.; Harrison, T. D.; Howard, T. J.; Jackson, D. T.; Lenzen, P. D.; Nguyen, T. D.; Pecha, R. L.; Rice, B. G.; Thompson, B. K.; Yates, S. W.

2017-06-01

Elastic and inelastic differential cross sections for neutron scattering from 56Fe have been measured for several incident energies from 1.30 to 7.96 MeV at the University of Kentucky Accelerator Laboratory. Scattered neutrons were detected using a C6D6 liquid scintillation detector using pulse-shape discrimination and time-of-flight techniques. The deduced cross sections have been compared with previously reported data, predictions from evaluation databases ENDF, JENDL, and JEFF, and theoretical calculations performed using different optical model potentials using the talys and empire nuclear reaction codes. The coupled-channel calculations based on the vibrational and soft-rotor models are found to describe the experimental (n ,n0 ) and (n ,n1 ) cross sections well.

Note: Coincidence measurements of 3He and neutrons from a compact D-D neutron generator.

PubMed

Ji, Q; Lin, C-J; Tindall, C; Garcia-Sciveres, M; Schenkel, T; Ludewigt, B A

2017-05-01

Tagging of neutrons (2.45 MeV) with their associated 3 He particles from deuterium-deuterium (D-D) fusion reactions has been demonstrated in a compact neutron generator setup enabled by a high brightness, microwave-driven ion source with a high fraction of deuterons. Energy spectra with well separated peaks of the D-D fusion reaction products, 3 He, tritons, and protons, were measured with a silicon PIN diode. The neutrons were detected using a liquid scintillator detector with pulse shape discrimination. By correlating the 3 He detection events with the neutron detection in time, we demonstrated the tagging of emitted neutrons with 3 He particles detected with a Si PIN diode detector mounted inside the neutron generator vacuum vessel.

A neutron camera system for MAST.

PubMed

Cecconello, M; Turnyanskiy, M; Conroy, S; Ericsson, G; Ronchi, E; Sangaroon, S; Akers, R; Fitzgerald, I; Cullen, A; Weiszflog, M

2010-10-01

A prototype neutron camera has been developed and installed at MAST as part of a feasibility study for a multichord neutron camera system with the aim to measure the spatial and time resolved 2.45 MeV neutron emissivity profile. Liquid scintillators coupled to a fast digitizer are used for neutron/gamma ray digital pulse shape discrimination. The preliminary results obtained clearly show the capability of this diagnostic to measure neutron emissivity profiles with sufficient time resolution to study the effect of fast ion loss and redistribution due to magnetohydrodynamic activity. A minimum time resolution of 2 ms has been achieved with a modest 1.5 MW of neutral beam injection heating with a measured neutron count rate of a few 100 kHz.

Ultrahigh resolution radiation imaging system using an optical fiber structure scintillator plate.

PubMed

Yamamoto, Seiichi; Kamada, Kei; Yoshikawa, Akira

2018-02-16

High resolution imaging of radiation is required for such radioisotope distribution measurements as alpha particle detection in nuclear facilities or high energy physics experiments. For this purpose, we developed an ultrahigh resolution radiation imaging system using an optical fiber structure scintillator plate. We used a ~1-μm diameter fiber structured GdAlO 3 :Ce (GAP) /α-Al 2 O 3 scintillator plate to reduce the light spread. The fiber structured scintillator plate was optically coupled to a tapered optical fiber plate to magnify the image and combined with a lens-based high sensitivity CCD camera. We observed the images of alpha particles with a spatial resolution of ~25 μm. For the beta particles, the images had various shapes, and the trajectories of the electrons were clearly observed in the images. For the gamma photons, the images also had various shapes, and the trajectories of the secondary electrons were observed in some of the images. These results show that combining an optical fiber structure scintillator plate with a tapered optical fiber plate and a high sensitivity CCD camera achieved ultrahigh resolution and is a promising method to observe the images of the interactions of radiation in a scintillator.

Laser micromachining of cadmium tungstate scintillator for high energy X-ray imaging

NASA Astrophysics Data System (ADS)

Richards, Sion Andreas

Pulsed laser ablation has been investigated as a method for the creation of thick segmented scintillator arrays for high-energy X-ray radiography. Thick scintillators are needed to improve the X-ray absorption at high energies, while segmentation is required for spatial resolution. Monte-Carlo simulations predicted that reflections at the inter-segment walls were the greatest source of loss of scintillation photons. As a result of this, fine pitched arrays would be inefficient as the number of reflections would be significantly higher than in large pitch arrays. Nanosecond and femtosecond pulsed laser ablation was investigated as a method to segment cadmium tungstate (CdWO_4). The effect of laser parameters on the ablation mechanisms, laser induced material changes and debris produced were investigated using optical and electron microscopy, energy dispersive X-ray spectroscopy and X-ray photoelectron spectroscopy for both types of lasers. It was determined that nanosecond ablation was unsuitable due to the large amount of cracking and a heat affected zone created during the ablation process. Femtosecond pulsed laser ablation was found to induce less damage. The optimised laser parameters for a 1028 nm laser was found to be a pulse energy of 54 μJ corresponding to a fluence of 5.3 J cm. -2 a pulse duration of 190 fs, a repetition rate of 78.3 kHz and a laser scan speed of 707 mm s. -1 achieving a normalised pulse overlap of 0.8. A serpentine scan pattern was found to minimise damage caused by anisotropic thermal expansion. Femtosecond pulsed ablation was also found to create a layer of tungsten and cadmium sub-oxides on the surface of the crystals. The CdWO_4 could be cleaned by immersing the CdWO_4 in ammonium hydroxide at 45°C for 15 minutes. However, XPS indicated that the ammonium hydroxide formed a thin layer of CdCO_3 and Cd(OH)_2 on the surface. Prototype arrays were shown to be able to resolve features as small as 0.5 mm using keV energy X-rays. The most efficient prototype showed low detective quantum efficiency of 0.08±0.01 at 0 lp/mm using a tube voltage of 160 kVp.

Scintillation Counters

NASA Astrophysics Data System (ADS)

Bell, Zane W.

Scintillators find wide use in radiation detection as the detecting medium for gamma/X-rays, and charged and neutral particles. Since the first notice in 1895 by Roentgen of the production of light by X-rays on a barium platinocyanide screen, and Thomas Edison's work over the following 2 years resulting in the discovery of calcium tungstate as a superior fluoroscopy screen, much research and experimentation have been undertaken to discover and elucidate the properties of new scintillators. Scintillators with high density and high atomic number are prized for the detection of gamma rays above 1 MeV; lower atomic number, lower-density materials find use for detecting beta particles and heavy charged particles; hydrogenous scintillators find use in fast-neutron detection; and boron-, lithium-, and gadolinium-containing scintillators are used for slow-neutron detection. This chapter provides the practitioner with an overview of the general characteristics of scintillators, including the variation of probability of interaction with density and atomic number, the characteristics of the light pulse, a list and characteristics of commonly available scintillators and their approximate cost, and recommendations regarding the choice of material for a few specific applications. This chapter does not pretend to present an exhaustive list of scintillators and applications.

Staged Z-pinch Experiments at the 1MA Zebra pulsed-power generator: Neutron measurements

NASA Astrophysics Data System (ADS)

Ruskov, Emil; Darling, T.; Glebov, V.; Wessel, F. J.; Anderson, A.; Beg, F.; Conti, F.; Covington, A.; Dutra, E.; Narkis, J.; Rahman, H.; Ross, M.; Valenzuela, J.

2017-10-01

We report on neutron measurements from the latest Staged Z-pinch experiments at the 1MA Zebra pulsed-power generator. In these experiments a hollow shell of argon or krypton gas liner, injected between the 1 cm anode-cathode gap, compresses a deuterium plasma target of varying density. Axial magnetic field Bz <= 2 kGs, applied throughout the pinch region, stabilizes the Rayleigh-Taylor instability. The standard silver activation diagnostics and 4 plastic scintillator neutron Time of Flight (nTOF) detectors are augmented with a large area ( 1400 cm2) liquid scintillator detector to which fast gatedPhotek photomultipliers are attached. Sample data from these neutron diagnostics systems is presented. Consistently high neutron yields YDD >109 are measured, with highest yield of 2.6 ×109 . A pair of horizontally and vertically placed plastic scintillator nTOFs suggest isotropic i.e. thermonuclear origin of the neutrons produced. nTOF data from the liquid scintillator detector was cross-calibrated with the silver activation detector, and can be used for accurate calculation of the neutron yield. Funded by the Advanced Research Projects Agency - Energy, under Grant Number DE-AR0000569.

Scintillating Cocktail Mixtures and the Role of Water on the Optophysical Properties.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Cordaro, Joseph Gabriel; Feng, Patrick L.; Mengesha, Wondwosen

2015-10-01

Two types of water - containing liquid scinti llation mixtures were prepared in the present work. In the first, m ixtures of 2 - phenylethanol, water, diphenyl phosphate, sodium phenyl phosphate dibasic dihydrate, and the dye 2,5 - diphenyloxazole (PPO) have been investigated as liquid scintillators. In th e second system, nonionic and mixed surfactant systems were investigated in conjunction with water and small amounts of toluene. In both cases, increasing amounts of water led to reductions in the scintillation light yield. Understanding what factors contr ibute to this phenomenon is the focus of this report. Changes in the solutionmore » microphase structure, diminishing aromatic content of the cocktail mixtures, and inefficient energy transfer to the dye a ppear to be responsible for the decreased light yield as more water is added . In the 2 - phenylethanol system, the observed experimental results are consistent with the formation of a bicontinuous microemulsion at higher water concentrations, which incorporates PPO and shields it from the quenching effects of the increasing polar matrix. Evidence for this proposed phase chan ge c ome s from light scattering data, photo - and x - ray luminescence measurements, and optical transparency measurements . In the surfactant - based system, the quenching effect of water was found to be less than both commercially - available dioxane - naphthalene mixtures used for scintillation counting as well as the 2 - phenylethanol mixtures described above. The effect of different surfactant mixtures and concentrations were studied, revealing a benefic ial effect upon the scintillation light yield for mixed surfactant mixtures. These results are interpreted in the context of r eactive radical species formation following water ionization , which leads to light - yield quenching in aqueous systems . The presenc e of surfactant(s) in these mixtures enables the formation of organic - rich regions that are spatially separated from the reactive radicals. This hypothesis is consistent with subsequent experiments that showed reduced light - yield quenching in the presence of radical - trapping additives. A notable result from these surfactant studies was the preparation of an aqueous scintillator that was transparent and showed neutron/gamma pulse - shape discrimination. Section II below provides background information on the s ignificance of this finding. The combined work described herein has implications on other efforts to make water - based solution scintillators -- without aromatic content an efficient mechanism for ionizing radiation to sensitize emission from a dye is limited.« less

microPMT-A New Photodetector for Gamma Spectrometry and Fast Timing?

NASA Astrophysics Data System (ADS)

Szczęśniak, T.; Grodzicka, M.; Moszyński, M.; Szawłowski, M.; Baszak, J.

2014-10-01

A micro photomultiplier (microPMT or μPMT) works like a classic photomultiplier but the whole device is made directly in a silicon wafer sandwiched between two glass layers. A microPMT has dimensions of only 13x10x2 mm and its photocathode has a size of 3x1 mm. The aim of the work is to check usefulness of a microPMT in gamma spectrometry with scintillators and fast timing. In the first part of the study analysis of the energy resolution obtained with 3x3x1 mm LSO, BGO and CsI(Tl) scintillators is made. The recorded values for 662 keV are equal to 22.9% and 13.5% for CsI and LSO, respectively. The light pulse shapes of a single photoelectron and scintillation signal of LSO are also shown. The important part of the study is measurement of the number of photoelectrons and estimation of the excess noise factor. Only 2200 phe/MeV were obtained for LSO coupled with the tested microPMT. The calculated excess noise factor is equal to 1.4. In the second part, measurements of the time jitter and timing resolution with LSO crystal for 511 keV annihilation quanta are reported. The timing characteristics of the tested device is poor. Its time jitter equals to 1.5 ns, whereas timing resolution for 22Na is 620 ps. All the results are compared with data obtained with classic PMTs.

Rejection of randomly coinciding events in Li_2^{100}MoO_4 scintillating bolometers using light detectors based on the Neganov-Luke effect

NASA Astrophysics Data System (ADS)

Chernyak, D. M.; Danevich, F. A.; Dumoulin, L.; Giuliani, A.; Mancuso, M.; Marcillac, P. de; Marnieros, S.; Nones, C.; Olivieri, E.; Poda, D. V.; Tretyak, V. I.

2017-01-01

Random coincidences of nuclear events can be one of the main background sources in low-temperature calorimetric experiments looking for neutrinoless double-beta decay, especially in those searches based on scintillating bolometers embedding the promising double-beta candidate ^{100} Mo, because of the relatively short half-life of the two-neutrino double-beta decay of this nucleus. We show in this work that randomly coinciding events of the two-neutrino double-beta decay of ^{100} Mo in enriched Li_2^{100} MoO_4 detectors can be effectively discriminated by pulse-shape analysis in the light channel if the scintillating bolometer is provided with a Neganov-Luke light detector, which can improve the signal-to-noise ratio by a large factor, assumed here at the level of {˜ }750 on the basis of preliminary experimental results obtained with these devices. The achieved pile-up rejection efficiency results in a very low contribution, of the order of {˜ }6× 10^{-5} counts/(keV\\cdot kg\\cdot y), to the background counting rate in the region of interest for a large volume ({˜ }90 cm^3) Li_2^{100} MoO_4 detector. This background level is very encouraging in view of a possible use of the Li_2^{100} MoO_4 solution for a bolometric tonne-scale next-generation experiment as that proposed in the CUPID project.

An integrated circuit/microsystem/nano-enhanced four species radiation sensor for inexpensive fissionable material detection

NASA Astrophysics Data System (ADS)

Waguespack, Randy Paul

2011-12-01

Small scale radiation detectors sensitive to alpha, beta, electromagnetic, neutron radiation are needed to combat the threat of nuclear terrorism and maintain national security. There are many types of radiation detectors on the market, and the type of detector chosen is usually determined by the type of particle to be detected. In the case of fissionable material, an ideal detector needs to detect all four types of radiation, which is not the focus of many detectors. For fissionable materials, the two main types of radiation that must be detected are gamma rays and neutrons. Our detector uses a glass or quartz scintillator doped with 10B nanoparticles to detect all four types of radiation particles. Boron-10 has a thermal neutron cross section of 3,840 barns. The interaction between the neutron and boron results in a secondary charge particle in the form of an alpha particle to be emitted, which is detectable by the scintillator. Radiation impinging on the scintillator matrix produces varying optical pulses dependent on the energy of the particles. The optical pulses are then detected by a photomultiplier (PM) tube, creating a current proportional to the energy of the particle. Current pulses from the PM tube are differentiated by on-chip pulse height spectroscopy, allowing for source discrimination. The pulse height circuitry has been fabricated with discrete circuits and designed into an integrated circuit package. The ability to replace traditional PM tubes with a smaller, less expensive photomultiplier will further reduce the size of the device and enhance the cost effectiveness and portability of the detector.

Methodology for the neutron time of flight measurement of 120-GeV proton-induced reactions on a thick copper target

DOE PAGES

Sanami, T.; Iwamoto, Y.; Kajimoto, T.; ...

2011-12-06

Our methodology for the time-of-flight measurement of the neutron energy spectrum for a high-energy proton-beam-induced reaction was established at the Fermilab Test Beam Facility of the Fermi National Accelerator Laboratory. The 120-GeV proton beam with 3 × 10 5 protons/spill was prepared for event-by-event counting of incident protons and emitted neutrons for time-of-flight energy determination. An NE213 organic liquid scintillator (12.7 cm in diameter by 12.7 cm in length) was employed with a veto plastic scintillator and a pulse-shape discrimination technique to identify neutrons. Raw waveforms of NE213, veto and beam detectors were recorded to discriminate the effects of multi-protonmore » beam events by considering different time windows. The neutron energy spectrum ranging from 10 to 800 MeV was obtained for a 60-cm-long copper target at 90° with respect to the beam axis. Finally our obtained spectrum was consistent with that deduced employing the conventional unfolding technique as well as that obtained in a 40-GeV/c thin-target experiment.« less

Measurement of seeing and the atmospheric time constant by differential scintillations.

PubMed

Tokovinin, Andrei

2002-02-20

A simple differential analysis of stellar scintillations measured simultaneously with two apertures opens the possibility to estimate seeing. Moreover, some information on the vertical turbulence distribution can be obtained. A general expression for the differential scintillation index for apertures of arbitrary shape and for finite exposure time is derived, and its applications are studied. Correction for exposure time bias by use of the ratio of scintillation indices with and without time binning is studied. A bandpass-filtered scintillation in a small aperture (computed as the differential-exposure index) provides a reasonably good estimate of the atmospheric time constant for adaptive optics.

Luminescence and scintillation properties of XPO4:Nd3+ (X = Y, Lu, Sc, La) crystals

NASA Astrophysics Data System (ADS)

Makowski, Michał; Witkowski, Marcin E.; Drozdowski, Winicjusz; Wojtowicz, Andrzej J.; Wisniewski, Krzysztof; Boatner, Lynn A.

2018-05-01

Due to their very fast short-wavelength emission, neodymium-doped materials are a subject of current interest as potential scintillators. Although the initial reports regarding neodymium-doped orthophosphates (in crystalline form) and their scintillation properties appeared almost twenty years ago, they remain an interesting class of materials since there is no in-depth understanding of their fundamental scintillation mechanism. In the present research, we focus on the crystalline systems: XPO4:Nd3+, where X = Y, Lu, La, Sc. The pulse height, optical absorption, radioluminescence and photoluminescence spectra were investigated and are reported here for various temperatures from 10 to 350 K. Additionally, results of both low and high temperature thermoluminescence measurements are reported in this communication.

RADIATION COUNTER

DOEpatents

Goldsworthy, W.W.

1958-02-01

This patent relates to a radiation counter, and more particularly, to a scintillation counter having high uniform sensitivity over a wide area and capable of measuring alpha, beta, and gamma contamination over wide energy ranges, for use in quickly checking the contami-nation of personnel. Several photomultiplier tubes are disposed in parallel relationship with a light tight housing behind a wall of scintillation material. Mounted within the housing with the photomultipliers are circuit means for producing an audible sound for each pulse detected, and a range selector developing a voltage proportional to the repetition rate of the detected pulses and automatically altering its time constant when the voltage reaches a predetermined value, so that manual range adjustment of associated metering means is not required.

Photon statistics in scintillation crystals

NASA Astrophysics Data System (ADS)

Bora, Vaibhav Joga Singh

Scintillation based gamma-ray detectors are widely used in medical imaging, high-energy physics, astronomy and national security. Scintillation gamma-ray detectors are eld-tested, relatively inexpensive, and have good detection eciency. Semi-conductor detectors are gaining popularity because of their superior capability to resolve gamma-ray energies. However, they are relatively hard to manufacture and therefore, at this time, not available in as large formats and much more expensive than scintillation gamma-ray detectors. Scintillation gamma-ray detectors consist of: a scintillator, a material that emits optical (scintillation) photons when it interacts with ionization radiation, and an optical detector that detects the emitted scintillation photons and converts them into an electrical signal. Compared to semiconductor gamma-ray detectors, scintillation gamma-ray detectors have relatively poor capability to resolve gamma-ray energies. This is in large part attributed to the "statistical limit" on the number of scintillation photons. The origin of this statistical limit is the assumption that scintillation photons are either Poisson distributed or super-Poisson distributed. This statistical limit is often dened by the Fano factor. The Fano factor of an integer-valued random process is dened as the ratio of its variance to its mean. Therefore, a Poisson process has a Fano factor of one. The classical theory of light limits the Fano factor of the number of photons to a value greater than or equal to one (Poisson case). However, the quantum theory of light allows for Fano factors to be less than one. We used two methods to look at the correlations between two detectors looking at same scintillation pulse to estimate the Fano factor of the scintillation photons. The relationship between the Fano factor and the correlation between the integral of the two signals detected was analytically derived, and the Fano factor was estimated using the measurements for SrI2:Eu, YAP:Ce and CsI:Na. We also found an empirical relationship between the Fano factor and the covariance as a function of time between two detectors looking at the same scintillation pulse. This empirical model was used to estimate the Fano factor of LaBr3:Ce and YAP:Ce using the experimentally measured timing-covariance. The estimates of the Fano factor from the time-covariance results were consistent with the estimates of the correlation between the integral signals. We found scintillation light from some scintillators to be sub-Poisson. For the same mean number of total scintillation photons, sub-Poisson light has lower noise. We then conducted a simulation study to investigate whether this low-noise sub-Poisson light can be used to improve spatial resolution. We calculated the Cramer-Rao bound for dierent detector geometries, position of interactions and Fano factors. The Cramer-Rao calculations were veried by generating simulated data and estimating the variance of the maximum likelihood estimator. We found that the Fano factor has no impact on the spatial resolution in gamma-ray imaging systems.

Application of photodiodes to the detection of electromagnetic bursts

NASA Technical Reports Server (NTRS)

Fukushima, Y.; Saito, T.; Sakata, M.; Shima, M.; Yamamoto, Y.

1985-01-01

A new type of photodiode + scintillator (1 m2 x 1 cm) detector is developed to detect the large electro-magnetic burst under an EX-chamber. The threshold burst size is found to be 4.3 x 10 the 5 particles at the center of the scintillator. Therefore a gamma-ray family of 10 TeV is detectable by it, when it is set under 14 r.1. of iron. In addition, a very fast (2.4 nsec width) and very bright (correspond to 10 to the 6 particles) scintillation pulse has become avarable for this study.

Novel methods for measuring afterglow in developmental scintillators for X-ray and neutron detection

NASA Astrophysics Data System (ADS)

Bartle, C. M.; Edgar, A.; Dixie, L.; Varoy, C.; Piltz, R.; Buchanan, S.; Rutherford, K.

2011-09-01

In this paper we discuss two novel methods of measuring afterglow in scintillators. One method is designed for X-ray detection and the other for neutron detection applications. In the first method a commercial fan-beam scanner of basic design similar to those seen at airports is used to deliver a typically 12 ms long X-ray pulse to a scintillator by passing the test equipment through the scanner on the conveyor belt. In the second method the thermal neutron beam from a research reactor is incident on the scintillator. The beam is cut-off in about 1 ms using a 10B impregnated aluminum pneumatic shutter, and the afterglow is recorded on a dual range storage oscilloscope to capture both the steady state intensity and the weak decay. We describe these measurement methods and the results obtained for a range of developmental ceramic and glass scintillators, as well as some standard scintillators such as NaI(Tl), LiI(Eu) and the plastic scintillator NE102A. Preliminary modeling of the afterglow is presented.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Divani, Nazila, E-mail: n-divani@birjand.ac.ir; Firoozabadi, Mohammad M.; Bayat, Esmail

Scintillators are almost used in any nuclear laboratory. These detectors combine of scintillation materials, PMT and a voltage divider. Voltage dividers are different in resistive ladder design. But the effect of decoupling capacitors and damping resistors haven’t discussed yet. In this paper at first a good equilibrium circuit designed for PMT, and it was used for investigating about capacitors and resistors in much manner. Results show that decoupling capacitors have great effect on PMT output pulses. In this research, it was tried to investigate the effect of Capacitor’s value and places on PMT voltage divider in Neutron-Gamma discrimination capability. Therefore,more » the voltage divider circuit for R329-02 Hamamatsu PMT was made and Zero Cross method used for neutron-gamma discrimination. The neutron source was a 20Ci Am-Be. Anode and Dynode pulses and discrimination spectrum were saved. The results showed that the pulse height and discrimination quality change with the value and setting of capacitors.« less

Improved neutron-gamma discrimination for a 6Li-glass neutron detector using digital signal analysis methods

DOE PAGES

Wang, Cai -Lin; Riedel, Richard A.

2016-01-14

A 6Li-glass scintillator (GS20) based neutron Anger camera was developed for time-of-flight single-crystal diffraction instruments at SNS. Traditional pulse-height analysis (PHA) for neutron-gamma discrimination (NGD) resulted in the neutron-gamma efficiency ratio (defined as NGD ratio) on the order of 10 4. The NGD ratios of Anger cameras need to be improved for broader applications including neutron reflectometers. For this purpose, five digital signal analysis methods of individual waveforms from PMTs were proposed using: i). pulse-amplitude histogram; ii). power spectrum analysis combined with the maximum pulse amplitude; iii). two event parameters (a 1, b 0) obtained from Wiener filter; iv). anmore » effective amplitude (m) obtained from an adaptive least-mean-square (LMS) filter; and v). a cross-correlation (CC) coefficient between an individual waveform and a reference. The NGD ratios can be 1-102 times those from traditional PHA method. A brighter scintillator GS2 has better NGD ratio than GS20, but lower neutron detection efficiency. The ultimate NGD ratio is related to the ambient, high-energy background events. Moreover, our results indicate the NGD capability of neutron Anger cameras can be improved using digital signal analysis methods and brighter neutron scintillators.« less

Performance of Large Neutron Detectors Containing Lithium-Gadolinium-Borate Scintillator

DOE Office of Scientific and Technical Information (OSTI.GOV)

Slaughter, David M.; Stuart, Cory R.; Klaass, R. Fred

2015-07-01

This paper describes the development and testing of a neutron counter, spectrometer, and dosimeter that is compact, efficient, and accurate. A self-contained neutron detection instrument has wide applications in health physics, scientific research, and programs to detect, monitor, and control strategic nuclear materials (SNM). The 1.3 liter detector head for this instrument is a composite detector with an organic scintillator containing uniformly distributed {sup 6}Li{sub 6}{sup nat}Gd{sup 10}B{sub 3}O{sub 9}:Ce (LGB:Ce) microcrystals. The plastic scintillator acts to slow impinging neutrons and emits light proportional to the energy lost by the neutrons as they moderate in the detector body. Moderating neutronsmore » that have slowed sufficiently capture in one of the Lithium-6, Boron-10, or Gadolinium-157 atoms in the LGB:Ce scintillator, which then releases the capture energy in a characteristic cerium emission pulse. The measured captured pulses indicate the presence of neutrons. When a scintillating fluor is present in the plastic, the light pulse resulting from the neutron moderating in the plastic is paired with the LGB:Ce capture pulse to identify the energy of the neutron. About 2% of the impinging neutrons lose all of their energy in a single collision with the detector. There is a linear relationship between the pulse areas of this group of neutrons and energy. The other 98% of neutrons have a wide range of collision histories within the detector body. When these neutrons are 'binned' into energy groups, each group contains a distribution of pulse areas. This data was used to assist in the unfolding of the neutron spectra. The unfolded spectra were then validated with known spectra, at both neutron emitting isotopes and fission/accelerator facilities. Having validated spectra, the dose equivalent and dose rate are determined by applying standard, regulatory damage coefficients to the measured neutron counts for each energy bin of the spectra. Testing at the Los Alamos Neutron Science Center (LANSCE), Edwards Accelerator Laboratory (EAL) at Ohio University and the Radiation Center at University of Massachusetts-Lowell has demonstrated that the instrument can measure neutrons and their spectra over the range between 0.8 MeV and 150 MeV with an uncertainty of only ± 8%. An independent test of the LGB:Ce neutron spectrometer was conducted by a US Defense Threat Reduction Agency (DTRA) team at the Idaho National Laboratory (INL). The results of this evaluation showed that the neutron spectrometer accurately identified bare radioactive isotopes by their spectra. Further, masking and shielding materials alter those spectra in predictable ways that permit an extrapolation from the observed spectra back to the identity of the isotopic spectrum. (authors)« less

The beam test of muon detector parameters for the SHiP experiment at CERN

NASA Astrophysics Data System (ADS)

Likhacheva, V. L.; Kudenko, Yu. G.; Mefodiev, A. V.; Mineev, O. V.; Khotyantsev, A. N.

2018-01-01

Scintillation detectors based on extruded plastics have been tested in a 10 GeV/c beam at CERN. The scintillation signal readout was provided using optical wavelength shifting fibers Y11 Kuraray and Hamamatsu MPPC micropixel avalanche photodiodes. The light yield was scanned along and across the detectors. Time resolution was found by fitting the MPPC digitized pulse rise and other methods.

Characterization of SiPM for cryogenic applications

NASA Astrophysics Data System (ADS)

Cervi, T.; Bonesini, M.; Falcone, A.; Menegolli, A.; Raselli, G. L.; Rossella, M.; Simonetta, M.; Torti, M.

2016-07-01

The development of detectors based on liquefied noble gas (LAr, LXe) is mandatory for experiments dedicated to study physics beyond the Standard Model. For this purpose, it is fundamental to detect the Vacuum Ultra Violet (VUV) scintillation light, produced after the passage of ionizing particles inside the detector sensitive volume, to be used for trigger, timing and calorimetric purposes. Besides the traditional cryogenic Photo-Multiplier Tubes (PMTs), one possibility is to adopt Silicon Photo-Multipliers (SiPMs). We present a comparison of the performance of a SiPM (mod. ASD-NUV3S-P Low Afterpulse) at various cryogenic temperatures, from 60 K up to room temperature, with particular emphasis on the LAr and LXe temperatures. SiPM were characterized in terms of breakdown voltage, gain, pulse shape response, dark count rate and correlated noise.

DEAP-3600 Dark Matter Search at SNOLAB

NASA Astrophysics Data System (ADS)

Boulay, Mark; DEAP Collaboration

2014-09-01

The DEAP-3600 experiment will search for dark matter particle interactions on 3.6 tonnes of liquid argon at SNOLAB. The argon is contained in a large ultralow-background acrylic vessel viewed by 255 8-inch photomultiplier tubes. Very good pulse-shape discrimination has been demonstrated for scintillation in argon, and the detector has been designed for a total background budget, including (alpha,n) and external neutron recoils, surface contamination from 210Pb and radon daughters, of 0.2 events per tonne-year, allowing an ultimate sensitivity to spin-independent scattering of 10-46 cm2 per nucleon at 100 GeV mass. Installation of the detector is currently being completed at SNOLAB. The status of the experiment and an overview of low background techniques employed will be presented.

Luminescence and scintillation properties of XPO 4:Nd 3+ (X = Y, Lu, Sc, La) crystals

DOE PAGES

Makowski, Michal; Witkowski, Marcin E.; Drozdowski, Winicjusz; ...

2018-04-12

Due to their very fast short-wavelength emission, neodymium-doped materials are a subject of current interest as potential scintillators. Although the initial reports regarding neodymium-doped orthophosphates (in crystalline form) and their scintillation properties appeared almost twenty years ago, they remain an interesting class of materials since there is no in-depth understanding of their fundamental scintillation mechanism. In the present research, we focus on the crystalline systems: XPO 4:Nd 3+, where X = Y, Lu, La, Sc. The pulse height, optical absorption, radioluminescence and photoluminescence spectra were investigated and are reported here for various temperatures from 10 to 350 K. Here, resultsmore » of both low and high temperature thermoluminescence measurements are reported in this communication.« less

Luminescence and scintillation properties of XPO 4:Nd 3+ (X = Y, Lu, Sc, La) crystals

DOE Office of Scientific and Technical Information (OSTI.GOV)

Makowski, Michal; Witkowski, Marcin E.; Drozdowski, Winicjusz

Due to their very fast short-wavelength emission, neodymium-doped materials are a subject of current interest as potential scintillators. Although the initial reports regarding neodymium-doped orthophosphates (in crystalline form) and their scintillation properties appeared almost twenty years ago, they remain an interesting class of materials since there is no in-depth understanding of their fundamental scintillation mechanism. In the present research, we focus on the crystalline systems: XPO 4:Nd 3+, where X = Y, Lu, La, Sc. The pulse height, optical absorption, radioluminescence and photoluminescence spectra were investigated and are reported here for various temperatures from 10 to 350 K. Here, resultsmore » of both low and high temperature thermoluminescence measurements are reported in this communication.« less

Methods for the continuous production of plastic scintillator materials

DOEpatents

Bross, Alan; Pla-Dalmau, Anna; Mellott, Kerry

1999-10-19

Methods for producing plastic scintillating material employing either two major steps (tumble-mix) or a single major step (inline-coloring or inline-doping). Using the two step method, the polymer pellets are mixed with silicone oil, and the mixture is then tumble mixed with the dopants necessary to yield the proper response from the scintillator material. The mixture is then placed in a compounder and compounded in an inert gas atmosphere. The resultant scintillator material is then extruded and pelletized or formed. When only a single step is employed, the polymer pellets and dopants are metered into an inline-coloring extruding system. The mixture is then processed under a inert gas atmosphere, usually argon or nitrogen, to form plastic scintillator material in the form of either scintillator pellets, for subsequent processing, or as material in the direct formation of the final scintillator shape or form.

Characterization of Fissile Assemblies Using Low-Efficiency Detection Systems

DOE PAGES

Chapline, George F.; Verbeke, Jerome M.

2017-02-02

Here, we have investigated the possibility that the amount, chemical form, multiplication, and shape of the fissile material in an assembly can be passively assayed using scintillator detection systems by only measuring the fast neutron pulse height distribution and distribution of time intervals Δt between fast neutrons. We have previously demonstrated that the alpha-ratio can be obtained from the observed pulse height distribution for fast neutrons. In this paper we report that we report that when the distribution of time intervals is plotted as a function of logΔt, the position of the correlated neutron peak is nearly independent of detectormore » efficiency and determines the internal relaxation rate for fast neutrons. If this information is combined with knowledge of the alpha-ratio, then the position of the minimum between the correlated and uncorrelated peaks can be used to rapidly estimate the mass, multiplication, and shape of fissile material. This method does not require a priori knowledge of either the efficiency for neutron detection or the alpha-ratio. Although our method neglects 3-neutron correlations, we have used previously obtained experimental data for metallic and oxide forms of Pu to demonstrate that our method yields good estimates for multiplications as large as 2, and that the only constraint on detector efficiency/observation time is that a peak in the interval time distribution due to correlated neutrons is visible.« less

Measurements of high energy photons in Z-pinch experiments on primary test stand

NASA Astrophysics Data System (ADS)

Si, Fenni; Zhang, Chuanfei; Xu, Rongkun; Yuan, Xi; Huang, Zhanchang; Xu, Zeping; Ye, Fan; Yang, Jianlun; Ning, Jiamin; Hu, Qingyuan; Zhu, Xuebin

2015-08-01

High energy photons are measured for the first time in wire-array Z-pinch experiments on the Primary Test Stand (PTS) which delivers a current up to 8 MA with a rise time of 70 ns. A special designed detecting system composed of three types of detectors is used to measure the average energy, intensity, and pulse waveform of high energy photons. Results from Pb-TLD (thermoluminescence dosimeter) detector indicate that the average energy is 480 keV (±15%). Pulse shape of high energy photons is measured by the photodiode detector consisted of scintillator coupled with a photodiode, and it is correlated with soft x-ray power by the same timing signal. Intensity is measured by both TLD and the photodiode detector, showing good accordance with each other, and it is 1010 cm-2 (±20%) at 2 m in the horizontal direction. Measurement results show that high energy photons are mainly produced in pinch regions due to accelerated electrons. PTS itself also produces high energy photons due to power flow electrons, which is one order smaller in amplitude than those from pinch region.

Measurements of high energy photons in Z-pinch experiments on primary test stand.

PubMed

Si, Fenni; Zhang, Chuanfei; Xu, Rongkun; Yuan, Xi; Huang, Zhanchang; Xu, Zeping; Ye, Fan; Yang, Jianlun; Ning, Jiamin; Hu, Qingyuan; Zhu, Xuebin

2015-08-01

High energy photons are measured for the first time in wire-array Z-pinch experiments on the Primary Test Stand (PTS) which delivers a current up to 8 MA with a rise time of 70 ns. A special designed detecting system composed of three types of detectors is used to measure the average energy, intensity, and pulse waveform of high energy photons. Results from Pb-TLD (thermoluminescence dosimeter) detector indicate that the average energy is 480 keV (±15%). Pulse shape of high energy photons is measured by the photodiode detector consisted of scintillator coupled with a photodiode, and it is correlated with soft x-ray power by the same timing signal. Intensity is measured by both TLD and the photodiode detector, showing good accordance with each other, and it is 10(10) cm(-2) (±20%) at 2 m in the horizontal direction. Measurement results show that high energy photons are mainly produced in pinch regions due to accelerated electrons. PTS itself also produces high energy photons due to power flow electrons, which is one order smaller in amplitude than those from pinch region.

A new gamma ray imaging diagnostic for runaway electron studies at DIII-D

NASA Astrophysics Data System (ADS)

Cooper, C. M.; Pace, D. C.; Eidietis, N. W.; Paz-Soldan, C.; Commaux, N.; Shiraki, D.; Hollmann, E. M.; Moyer, R. A.; Risov, V.

2015-11-01

A new Gamma Ray Imager (GRI) is developed to probe the electron distribution function with 2D spatial resolution during runaway electron (RE) experiments at DIII-D. The diagnostic is sensitive to 0.5 - 50 MeV gamma rays, allowing characterization of the RE distribution function evolution during RE dissipation from pellet injection. The GRI consists of a lead ``pinhole camera'' mounted on the midplane with 11x11 counter-current tangential chords 20 cm wide that span the vessel. Up to 30 bismuth germanate (BGO) scintillation detectors capture RE Bremsstrahlung radiation. Detectors operate in current saturation mode at 10 MHz, or the flux is attenuated for Pulse Height Analysis (PHA) capable of discriminating up to ~10k pulses per second. Digital signal processing routines combining shaping filters are performed during PHA to reject noise and record gamma ray energy. The GRI setup and PHA algorithms will be described and initial data from experiments will be presented. Work supported by the US DOE under DE-AC05-00OR22725, DE-FG02-07ER54917 & DE-FC02-04ER54698.

Digital pile-up rejection for plutonium experiments with solution-grown stilbene

NASA Astrophysics Data System (ADS)

Bourne, M. M.; Clarke, S. D.; Paff, M.; DiFulvio, A.; Norsworthy, M.; Pozzi, S. A.

2017-01-01

A solution-grown stilbene detector was used in several experiments with plutonium samples including plutonium oxide, mixed oxide, and plutonium metal samples. Neutrons from different reactions and plutonium isotopes are accompanied by numerous gamma rays especially by the 59-keV gamma ray of 241Am. Identifying neutrons correctly is important for nuclear nonproliferation applications and makes neutron/gamma discrimination and pile-up rejection necessary. Each experimental dataset is presented with and without pile-up filtering using a previously developed algorithm. The experiments were simulated using MCNPX-PoliMi, a Monte Carlo code designed to accurately model scintillation detector response. Collision output from MCNPX-PoliMi was processed using the specialized MPPost post-processing code to convert neutron energy depositions event-by-event into light pulses. The model was compared to experimental data after pulse-shape discrimination identified waveforms as gamma ray or neutron interactions. We show that the use of the digital pile-up rejection algorithm allows for accurate neutron counting with stilbene to within 2% even when not using lead shielding.

Light yield and energy resolution studies for SoLid phase 1

NASA Astrophysics Data System (ADS)

Boursette, Delphine; SoLid Collaboration

2017-09-01

The SoLid experiment is searching for sterile neutrinos at a nuclear research reactor. It looks for inverse beta decays (producing a positron and a neutron in delayed coincidence) with a very segmented detector made of thousands of scintillating cubes. SoLid has a very innovative hybrid technology with two different scintillators which have different light emissions: polyvynil-toluene cubes (PVT) to detect the positrons and 6LiF:ZnS sheets on two faces of each PVT cube to detect the neutrons. It allows us to do an efficient pulse shape analysis to identify the signals from neutrons and positrons. The 288 kg detector prototype (SM1) took data in 2015. It demonstrated the detection principle and background rejection efficiency. The construction of SoLid phase I (˜ 1.5 t) has now started. To improve the energy resolution of SoLid phase I, we have tried to increase the light yield studying separately the two scintillators: PVT and ZnS. A test bench has been built to fully characterize and improve the neutron detection with the ZnS using an AmBe source. To study the positron light yield on the PVT, we have built another test bench with a 207Bi source. We have improved the design of the cubes, their wrapping or the type and the configuration of the fibers. We managed to increase the PVT light yield by about 66 % and improve the resolution of the positron energy on the test bench from 21 % to 16 % at 1 MeV.

The Use of Fast Neutron Detection for Materials Accountability

NASA Astrophysics Data System (ADS)

Nakae, L. F.; Chapline, G. F.; Glenn, A. M.; Kerr, P. L.; Kim, K. S.; Ouedraogo, S. A.; Prasad, M. K.; Sheets, S. A.; Snyderman, N. J.; Verbeke, J. M.; Wurtz, R. E.

2014-02-01

For many years at LLNL, we have been developing time-correlated neutron detection techniques and algorithms for applications such as Arms Control, Threat Detection and Nuclear Material Assay. Many of our techniques have been developed specifically for the relatively low efficiency (a few percent) inherent in man-portable systems. Historically, thermal neutron detectors (mainly 3He) were used, taking advantage of the high thermal neutron interaction cross-sections, but more recently we have been investigating the use of fast neutron detection with liquid scintillators, inorganic crystals, and in the near future, pulse-shape discriminating plastics that respond over 1000 times faster (nanoseconds versus tens of microseconds) than thermal neutron detectors. Fast neutron detection offers considerable advantages, since the inherent nanosecond production timescales of fission and neutron-induced fission are preserved and measured instead of being lost in the thermalization of thermal neutron detectors. We are now applying fast neutron technology to the safeguards regime in the form of high efficiency counters. Faster detector response times and sensitivity to neutron momentum show promise in measuring, differentiating, and assaying samples that have modest to very high count rates, as well as mixed neutron sources (e.g., Pu oxide or Mixed Cm and Pu). Here we report on measured results with our existing liquid scintillator array and promote the design of a nuclear material assay system that incorporates fast neutron detection, including the surprising result that fast liquid scintillator becomes competitive and even surpasses the precision of 3He counters measuring correlated pairs in modest (kg) samples of plutonium.

Neutron induced radiation damage of plastic scintillators for the upgrade of the Tile Calorimeter of the ATLAS detector.

NASA Astrophysics Data System (ADS)

Mdhluli, J. E.; Jivan, H.; Erasmus, R.; Davydov, Yu I.; Baranov, V.; Mthembu, S.; Mellado, B.; Sideras-Haddad, E.; Solovyanov, O.; Sandrock, C.; Peter, G.; Tlou, S.; Khanye, N.; Tjale, B.

2017-07-01

With the prediction that the plastic scintillators in the gap region of the Tile Calorimeter will sustain a significantly large amount of radiation damage during the HL-LHC run time, the current plastic scintillators will need to be replaced during the phase 2 upgrade in 2018. The scintillators in the gap region were exposed to a radiation environment of up to 10 kGy/year during the first run of data taking and with the luminosity being increased by a factor of 10, the radiation environment will be extremely harsh. We report on the radiation damage to the optical properties of plastic scintillators following irradiation using a neutron beam of the IBR-2 pulsed reactor in Joint Institute for Nuclear Research (JINR), Dubna. A comparison is drawn between polyvinyl toluene based commercial scintillators EJ200, EJ208 and EJ260 as well as polystyrene based scintillator from Kharkov. The samples were subjected to irradiation with high energy neutrons and a flux density range of 1 × 106-7.7 × 106. Light transmission, Raman spectroscopy, fluorescence spectroscopy and light yield testing was performed to characterize the damage induced in the samples. Preliminary results from the tests done indicate a minute change in the optical properties of the scintillators with further studies underway to gain a better understanding of the interaction between neutrons with plastic scintillators.

Lithium Alkaline Halides—Next Generation of Dual Mode Scintillators

NASA Astrophysics Data System (ADS)

Soundara-Pandian, L.; Hawrami, R.; Glodo, J.; Ariesanti, E.; van Loef, E. V.; Shah, K.

2016-04-01

We report on a new family of scintillators - Lithium alkaline halides, developed based on the alkaline halides by introducing lithium for dual mode gamma-neutron detection. Many different compositions were grown, among which LiSr2I5 (LSI), LiCa2I5 (LCI), LiSr2Br5 (LSB) activated with divalent Europium show good gamma and neutron detection properties. LSI shows the main emission at 497 nm under X-ray excitation. It also shows good proportionality, which in combination with the light yield as high as 60000 photons/MeV, results in an energy resolution of 3.5% at 662 keV. The electron or gamma equivalent energy (GEE) of the thermal neutron peak due to the 6Li neutron capture is 4.1 MeV, which amounts to a very high neutron light yield of 245000 photons. The decay times for neutrons are faster compared to that for gamma-rays, hence we achieved good pulse shape discrimination (PSD) between gamma and neutron events. Our initial studies on the effects of Eu concentration on the properties of LSI show that 3%-4% Eu concentration is optimal for the best performance in terms of gamma and neutron light yields and pulse shape discrimination. LCI shows the main emission at 475 nm under X-ray excitation and a very high gamma light yield of 90000 photons/MeV. The measured energy resolution is 6% at 662 keV. The electron equivalent energy for neutron detection has been measured to be around 3 MeV, which gives a neutron light yield of 270 000 photons. The measured decay times for neutrons are faster compared to gamma decays and the PSD between the gamma-rays and neutrons is not as good as LSI. LSB shows two emissions at 410 and 475 nm under X-ray excitation. The measured light yield is 32000 ph/MeV gamma-ray with an energy resolution of 6% at 662 keV. The electron equivalent energy of the 6Li capture peak was measured to be 3.3 MeV.

Temporally separating Cherenkov radiation in a scintillator probe exposed to a pulsed X-ray beam.

PubMed

Archer, James; Madden, Levi; Li, Enbang; Carolan, Martin; Petasecca, Marco; Metcalfe, Peter; Rosenfeld, Anatoly

2017-10-01

Cherenkov radiation is generated in optical systems exposed to ionising radiation. In water or plastic devices, if the incident radiation has components with high enough energy (for example, electrons or positrons with energy greater than 175keV), Cherenkov radiation will be generated. A scintillator dosimeter that collects optical light, guided by optical fibre, will have Cherenkov radiation generated throughout the length of fibre exposed to the radiation field and compromise the signal. We present a novel algorithm to separate Cherenkov radiation signal that requires only a single probe, provided the radiation source is pulsed, such as a linear accelerator in external beam radiation therapy. We use a slow scintillator (BC-444) that, in a constant beam of radiation, reaches peak light output after 1 microsecond, while the Cherenkov signal is detected nearly instantly. This allows our algorithm to separate the scintillator signal from the Cherenkov signal. The relative beam profile and depth dose of a linear accelerator 6MV X-ray field were reconstructed using the algorithm. The optimisation method improved the fit to the ionisation chamber data and improved the reliability of the measurements. The algorithm was able to remove 74% of the Cherenkov light, at the expense of only 1.5% scintillation light. Further characterisation of the Cherenkov radiation signal has the potential to improve the results and allow this method to be used as a simpler optical fibre dosimeter for quality assurance in external beam therapy. Copyright © 2017 Associazione Italiana di Fisica Medica. Published by Elsevier Ltd. All rights reserved.

A new spectroscopic imager for X-rays from 0.5 keV to 150 keV combining a pnCCD and a columnar CsI(Tl) scintillator

NASA Astrophysics Data System (ADS)

Schlosser, D. M.; Hartmann, R.; Kalok, D.; Bechteler, A.; Abboud, A.; Shokr, M.; Çonka, T.; Pietsch, U.; Strüder, L.

2017-04-01

By combining a low noise fully depleted pnCCD detector with a columnar CsI(Tl) scintillator an energy dispersive spatial resolving detector can be realized with a high quantum efficiency in the range from below 0.5 keV to above 150 keV. The used scintillator system increases the pulse height of gamma-rays converted in the CsI(Tl), due to focusing properties of the columnar scintillator structure by reducing the event size in indirect detection mode (conversion in the scintillator). In case of direct detection (conversion in the silicon of the pnCCD) the relative energy resolution is 0.7% at 122 keV (FWHM = 850 eV) and the spatial resolution is less than 75 μm. In case of indirect detection the relative energy resolution, integrated over all event sizes is about 9% at 122 keV with an expected spatial precision of below 75 μm.

Performance of coincidence-based PSD on LiF/ZnS Detectors for Multiplicity Counting

DOE Office of Scientific and Technical Information (OSTI.GOV)

Robinson, Sean M.; Stave, Sean C.; Lintereur, Azaree

Abstract: Mass accountancy measurement is a nuclear nonproliferation application which utilizes coincidence and multiplicity counters to verify special nuclear material declarations. With a well-designed and efficient detector system, several relevant parameters of the material can be verified simultaneously. 6LiF/ZnS scintillating sheets may be used for this purpose due to a combination of high efficiency and short die-away times in systems designed with this material, but involve choices of detector geometry and exact material composition (e.g., the addition of Ni-quenching in the material) that must be optimized for the application. Multiplicity counting for verification of declared nuclear fuel mass involves neutronmore » detection in conditions where several neutrons arrive in a short time window, with confounding gamma rays. This paper considers coincidence-based Pulse-Shape Discrimination (PSD) techniques developed to work under conditions of high pileup, and the performance of these algorithms with different detection materials. Simulated and real data from modern LiF/ZnS scintillator systems are evaluated with these techniques and the relationship between the performance under pileup and material characteristics (e.g., neutron peak width and total light collection efficiency) are determined, to allow for an optimal choice of detector and material.« less

The AMoRE: Search for Neutrinoless Double Beta Decay in 100Mo

NASA Astrophysics Data System (ADS)

Park, HyangKyu; AMoRE Collaboration

2016-04-01

The AMoRE (Advanced Mo-based Rare process Experiment) collaboration is going to use calcium molybdate, 40Ca100MoO4 (CMO), crystal scintillators enriched in 100Mo and depleted in 48Ca to search for neutrinoless double-beta (0 νββ) decay of 100Mo using a technique of cryogenic scintillating bolometers at the underground laboratory in Korea. The collaboration is going to utilize metallic magnetic calorimeters (MMC) as temperature sensors both in heat and light channels of CMO detectors operated at milli-Kelvin temperature. Application of relatively fast MMC sensors provides excellent energy resolution, powerful discrimination of internal alpha particles, effective pulse-shape discrimination of randomly coinciding events of two-neutrino double-beta decay of 100Mo. In its first phase, the AMoRE-10 will use about 10 kg of CMO crystals. As a next step, the AMoRE-200 is going to build about 200 kg detector to reach a half-life sensitivity on the level of 1026 years with an aim to explore inverted hierarchy region of the effective Majorana neutrino mass 0.02 - 0.05 eV. Recent progress on the calcium molybdate detectors developments at room and milli-Kelvin temperatures as well as background study based on Monte Carlo simulations will be presented.

The compact neutron spectrometer at ASDEX Upgrade.

PubMed

Giacomelli, L; Zimbal, A; Tittelmeier, K; Schuhmacher, H; Tardini, G; Neu, R

2011-12-01

The first neutron spectrometer of ASDEX Upgrade (AUG) was installed in November 2008. It is a compact neutron spectrometer (CNS) based on a BC501A liquid scintillating detector, which can simultaneously measure 2.45-MeV and 14-MeV neutrons emitted from deuterium (D) plasmas and γ radiation. The scintillating detector is coupled to a digital pulse shape discrimination data acquisition (DPSD) system capable of count rates up to 10(6) s(-1). The DPSD system can operate in acquisition and processing mode. With the latter n-γ discrimination is performed off-line based on the two-gate method. The paper describes the tests of the CNS and its installation at AUG. The neutron emission from the D plasma measured during a discharge with high auxiliary heating power was used to validate the CNS performance. The study of the optimal settings for the DPSD data processing to maximize the n-γ discrimination capability of the CNS is reported. The CNS measured both 2.45-MeV and 14-MeV neutrons emitted in AUG D plasmas with a maximum count rate of 5.4 × 10(5) s(-1) (>10 times higher than similar spectrometers previously achieved) with an efficiency of 9.3 × 10(-10) events per AUG neutron.

Flexible composite radiation detector

DOEpatents

Cooke, D Wayne [Santa Fe, NM; Bennett, Bryan L [Los Alamos, NM; Muenchausen, Ross E [Los Alamos, NM; Wrobleski, Debra A [Los Alamos, NM; Orler, Edward B [Los Alamos, NM

2006-12-05

A flexible composite scintillator was prepared by mixing fast, bright, dense rare-earth doped powdered oxyorthosilicate (such as LSO:Ce, LSO:Sm, and GSO:Ce) scintillator with a polymer binder. The binder is transparent to the scintillator emission. The composite is seamless and can be made large and in a wide variety of shapes. Importantly, the composite can be tailored to emit light in a spectral region that matches the optimum response of photomultipliers (about 400 nanometers) or photodiodes (about 600 nanometers), which maximizes the overall detector efficiency.

Characterizing a pulse-resolved dosimetry system for complex radiotherapy beams using organic scintillators.

PubMed

Beierholm, Anders R; Ottosson, Rickard O; Lindvold, Lars R; Behrens, Claus F; Andersen, Claus E

2011-05-21

A fast-readout dosimetry system based on fibre-coupled organic scintillators has been developed for the purpose of conducting point measurements of absorbed dose in radiotherapy beams involving high spatial and temporal dose gradients. The system measures the dose for each linac radiation pulse with millimetre spatial resolution. To demonstrate the applicability of the system in complex radiotherapy fields, output factors and per cent depth dose measurements were performed in solid water for a 6 MV photon beam and compared with Monte Carlo simulated doses for square fields down to 0.6 cm × 0.6 cm size. No significant differences between measurements and simulations were observed. The temporal resolution of the system was demonstrated by measuring dose per pulse, beam start-up transients and the quality factor for 6 MV. The precision of dose per pulse measurements was within 2.7% (1 SD) for a 10 cm × 10 cm field at 10 cm depth. The dose per pulse behaviour compared well with linac target current measurements and accumulated dose measurements, and the system was able to resolve transient dose delivery differences between two Varian linac builds. The system therefore shows promise for reference dosimetry and quality assurance of complex radiotherapy treatments.

Scintillation properties of polycrystalline LaxY1-xO3 ceramic

NASA Astrophysics Data System (ADS)

Sahi, Sunil; Chen, Wei; Kenarangui, Rasool

2015-03-01

Scintillators are the material that absorbs the high-energy photons and emits visible photons. Scintillators are commonly used in radiation detector for security, medical imaging, industrial applications and high energy physics research. Two main types of scintillators are inorganic single crystals and organic (plastic or liquid) scintillators. Inorganic single crystals are expensive and difficult to grow in desire shape and size. Also, some efficient inorganic scintillator such as NaI and CsI are not environmental friendly. But on the other hand, organic scintillators have low density and hence poor energy resolution which limits their use in gamma spectroscopy. Polycrystalline ceramic can be a cost effective alternative to expensive inorganic single crystal scintillators. Here we have fabricated La0.2Y1.8O3 ceramic scintillator and studied their luminescence and scintillation properties. Ceramic scintillators were fabricated by vacuum sintering of La0.2Y1.8O3 nanoparticles at temperature below the melting point. La0.2Y1.8O3 ceramic were characterized structurally using XRD and TEM. Photoluminescence and radioluminescence studies were done using UV and X-ray as an excitation source. We have used gamma isotopes with different energy to studies the scintillation properties of La0.2Y1.8O3 scintillator. Preliminary studies of La0.2Y1.8O3 scintillator shows promising result with energy resolution comparable to that of NaI and CsI.

PROSPECT - A precision oscillation and spectrum experiment

NASA Astrophysics Data System (ADS)

Langford, T. J.; PROSPECT Collaboration

2015-08-01

Segmented antineutrino detectors placed near a compact research reactor provide an excellent opportunity to probe short-baseline neutrino oscillations and precisely measure the reactor antineutrino spectrum. Close proximity to a reactor combined with minimal overburden yield a high background environment that must be managed through shielding and detector technology. PROSPECT is a new experimental effort to detect reactor antineutrinos from the High Flux Isotope Reactor (HFIR) at Oak Ridge National Laboratory, managed by UT Battelle for the U.S. Department of Energy. The detector will use novel lithium-loaded liquid scintillator capable of neutron/gamma pulse shape discrimination and neutron capture tagging. These enhancements improve the ability to identify neutrino inverse-beta decays (IBD) and reject background events in analysis. Results from these efforts will be covered along with their implications for an oscillation search and a precision spectrum measurement.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Agnes, P.; et al.

A Geant4-based Monte Carlo package named G4DS has been developed to simulate the response of DarkSide-50, an experiment operating since 2013 at LNGS, designed to detect WIMP interactions in liquid argon. In the process of WIMP searches, DarkSide-50 has achieved two fundamental milestones: the rejection of electron recoil background with a power of ~10^7, using the pulse shape discrimination technique, and the measurement of the residual 39Ar contamination in underground argon, ~3 orders of magnitude lower with respect to atmospheric argon. These results rely on the accurate simulation of the detector response to the liquid argon scintillation, its ionization, andmore » electron-ion recombination processes. This work provides a complete overview of the DarkSide Monte Carlo and of its performance, with a particular focus on PARIS, the custom-made liquid argon response model.« less

Characterization of gamma rays existing in the NMIJ standard neutron field.

PubMed

Harano, H; Matsumoto, T; Ito, Y; Uritani, A; Kudo, K

2004-01-01

Our laboratory provides national standards on fast neutron fluence. Neutron fields are always accompanied by gamma rays produced in neutron sources and surroundings. We have characterised these gamma rays in the 5.0 MeV standard neutron field. Gamma ray measurement was performed using an NE213 liquid scintillator. Pulse shape discrimination was incorporated to separate the events induced by gamma rays from those by neutrons. The measured gamma ray spectra were unfolded with the HEPRO program package to obtain the spectral fluences using the response matrix prepared with the EGS4 code. Corrections were made for the gamma rays produced by neutrons in the detector assembly using the MCNP4C code. The effective dose equivalents were estimated to be of the order of 25 microSv at the neutron fluence of 10(7) neutrons cm(-2).

The MiniCLEAN Dark Matter Experiment

NASA Astrophysics Data System (ADS)

Schnee, Richard; Deap/Clean Collaboration

2011-10-01

The MiniCLEAN dark matter experiment exploits a single-phase liquid argon (LAr) detector, instrumented with photomultiplier tubes submerged in the cryogen with nearly 4 π coverage of a 500 kg target (150 kg fiducial) mass. The high light yield and large difference in singlet/triplet scintillation time-profiles in LAr provide effective defense against radioactive backgrounds through pulse-shape discrimination and event position reconstruction. The detector is also designed for a liquid neon target which, in the event of a positive signal in LAr, will enable an independent verification of backgrounds and provide a unique test of the expected A2 dependence of the WIMP interaction rate. The conceptually simple design can be scaled to target masses in excess of 10 tons in a relatively straightforward and economic manner. The experimental technique and current status of MiniCLEAN will be summarized.

Measured and calculated fast neutron spectra in a depleted uranium and lithium hydride shielded reactor

NASA Technical Reports Server (NTRS)

Lahti, G. P.; Mueller, R. A.

1973-01-01

Measurements of MeV neutron were made at the surface of a lithium hydride and depleted uranium shielded reactor. Four shield configurations were considered: these were assembled progressively with cylindrical shells of 5-centimeter-thick depleted uranium, 13-centimeter-thick lithium hydride, 5-centimeter-thick depleted uranium, 13-centimeter-thick lithium hydride, 5-centimeter-thick depleted uranium, and 3-centimeter-thick depleted uranium. Measurements were made with a NE-218 scintillation spectrometer; proton pulse height distributions were differentiated to obtain neutron spectra. Calculations were made using the two-dimensional discrete ordinates code DOT and ENDF/B (version 3) cross sections. Good agreement between measured and calculated spectral shape was observed. Absolute measured and calculated fluxes were within 50 percent of one another; observed discrepancies in absolute flux may be due to cross section errors.

Large surface scintillators as base of impact point detectors and their application in Space Weather

NASA Astrophysics Data System (ADS)

Ayuso, Sindulfo; Medina, José; Gómez-Herrero, Raul; José Blanco, Juan; García-Tejedor, Ignacio; García-Población, Oscar; Díaz-Romeral, Gonzalo

2016-04-01

The use of a pile of two 100 cm x 100 cm x 5 cm BC-400 organic scintillators is proposed as ground-based cosmic ray detector able to provide directional information on the incident muons. The challenge is to get in real time the muon impact point on the scintillator and its arrival direction using as few Photomultiplier Tubes (PMTs) as possible. The instrument is based on the dependence of attenuation of light with the traversed distance in each scintillator. For the time being, four photomultiplier tubes gather the light through the lateral faces (100 cm x 5 cm) of the scintillator. Several experiments have already been carried out. The results show how data contain information about the muon trajectory through the scintillator. This information can be extracted using the pulse heights collected by the PMTs working in coincidence mode. Reliability and accuracy of results strongly depend on the number of PMTs used and mainly on their appropriate geometrical arrangement with regard to the scintillator. In order to determine the optimal position and the minimum number of PMTs required, a Montecarlo simulation code has been developed. Preliminary experimental and simulation results are presented and the potential of the system for space weather monitoring is discussed.

Capture-gated Spectroscopic Measurements of Monoenergetic Neutrons with a Composite Scintillation Detector

NASA Astrophysics Data System (ADS)

Nattress, Jason; Mayer, M.; Foster, A.; Meddeb, A. Barhoumi; Trivelpiece, C.; Ounaies, Z.; Jovanovic, I.

2016-04-01

We report on the measurements of monoenergetic neutrons from DD and DT fusion reactions by use of the capture gating method in a heterogeneous plastic-glass composite scintillation detector. The cylindrical detector is 5.08 cm in diameter and 5.05 cm in height and was fabricated using 1-mm diameter Li-doped glass rods (GS20) and scintillating polyvinyl toluene (EJ-290). Different scintillation decay constants are used to identify energy depositions in two materials constituting the composite scintillator. Geant4 simulations of the neutron thermalization and capture process were conducted, finding a mean capture time of approximately 2.6 μs for both DD and DT neutrons. A capture gating time acceptance window based on simulation results was used to identify the neutron thermalization pulses. The total scintillation light yield produced in neutron thermalization was measured and found to show consistency on event-by-event basis despite the variety of neutron thermalization histories prior to capture. The ratio of light yields from thermalization of 14.1 MeV and 2.45 MeV neutrons in the EJ-290 scintillator was determined to be 14.6, and the light output from 2.45 MeV neutrons was also correlated to its electron equivalent, obtaining a value of 0.58±0.05 MeVee.

3D Printed Scintillators For Use in Field Emission Detection and Other Nuclear Physics Experiments

NASA Astrophysics Data System (ADS)

Ficenec, Karen

2015-10-01

In accelerator cavities, field emission electrons - electrons that get stripped away from the cavity walls due to the high electromagnetic field necessary to accelerate the main beam - are partially accelerated and can crash into the cavity walls, adding to the heat-load of the cryogenic system. Because these field electrons emit gamma rays when bent by the electromagnetic field, a scintillator, if made to fit the cavity enclosure, can detect their presence. Eliminating the waste of subtractive manufacturing techniques and allowing for the production of unique, varied shapes, 3D printing of scintillators may allow for an efficient detection system. UV light is used to start a chemical polymerization process that links the monomers of the liquid resin together into larger, intertwined molecules, forming the solid structure. Each shape requires slightly different calibration of its optimal printing parameters, such as slice thickness and exposure time to UV light. Thus far, calibration parameters have been optimized for cylinders of 20 mm diameter, cones of 30 mm diameter and 30 mm height, rectangular prisms 30 by 40 by 10 mm, and square pyramids 20 mm across. Calibration continues on creating holes in the prints (for optical fibers), as well as shapes with overhangs. Scintill This work was supported in part by the National Science Foundation under Grant No. PHY-1405857.

Temperature response of several scintillator materials to light ions

NASA Astrophysics Data System (ADS)

Rodríguez-Ramos, M.; Jiménez-Ramos, M. C.; García-Muñoz, M.; García López, J.

2017-07-01

Ion beam induced luminescence has been used to study the response of scintillator screens of Y2O3:Eu3+ (P56) and SrGa2S4:Eu2+ (TG-Green) when irradiated with light ions (protons, deuterium and helium particles). The absolute efficiency of the samples has been studied as a function of the ion energy (with energies up to 3.5 MeV), the beam current and the operating temperature. The evolution of the scintillator yield with ion fluence has been carried out for all the scintillators to estimate radiation damage. Finally, measurements of the decay time of these materials using a system of pulsed beam accelerated particles have been done. Among the screens under study, the TG-Green is the best suited material, in terms of absolute efficiency, temporal response and degradation with ion dose, for fast-ion loss detectors in fusion devices.

Doping of polysiloxane rubbers for the production of organic scintillators

NASA Astrophysics Data System (ADS)

Quaranta, A.; Carturan, S.; Marchi, T.; Cinausero, M.; Scian, C.; Kravchuk, V. L.; Degerlier, M.; Gramegna, F.; Poggi, M.; Maggioni, G.

2010-08-01

Polysiloxane rubbers have been produced with different concentrations of phenyl groups and of dye molecules in order to find the best synthesis conditions for reaching a high light yield. In particular, two different polymer compositions were examined, namely with 15% and 22% of phenyl units in the starting resin. 2,5-Diphenyl oxazole (PPO) as a primary dopant and Lumogen F Violet 570 as secondary dopant were dispersed in the polysiloxane. Ion beam induced luminescence (IBIL) technique was employed for studying radioluminescence and radiation hardness properties. The α and γ scintillation yields were analyzed by measuring the pulse height spectra from 241Am and 60Co radioactive sources. First tests on the suitability of these materials to the detection of fast neutrons were also performed with a TOF procedure. Preliminary results indicate that these materials exhibit a scintillation yield comparable with NE102 plastic scintillator.

Characterization of the Gamma Response of a Cadmium Capture-gated Neutron Spectrometer

NASA Astrophysics Data System (ADS)

Hogan, Nathaniel; Rees, Lawrence; Czirr, Bart; Bastola, Suraj

2010-10-01

We have studied the gamma response of a newly developed capture-gated neutron spectrometer. Such spectrometers detect a dual signal from incoming neutrons, allowing for differentiation between other particles, such as gamma rays. The neutron provides a primary light pulse in either plastic or liquid scintillator through neutron-proton collisions. A capture material then delivers a second pulse as the moderated neutron captures in the intended material, which then de-excites with the release of gamma energy. The presented spectrometer alternates one centimeter thick plastic scintillators with sheets of cadmium inserted in between for neutron capture. The neutron capture in cadmium offers a release of gamma energy ˜ 9 MeV. To verify that the interaction was caused by a neutron, the response functions of both events must be well known. Due to the prior existence of many capture-gated neutron spectrometers, the proton recoil pulse has already been studied, but the capture pulse is unique to each spectrometer and must be measured. Experimental results agree with theoretical Monte-Carlo code, both suggesting that the optics and geometry of the spectrometer play a large role in its efficiency. Results prove promising for the efficiency of the spectrometer.

Generation of programmable temporal pulse shape and applications in micromachining

NASA Astrophysics Data System (ADS)

Peng, X.; Jordens, B.; Hooper, A.; Baird, B. W.; Ren, W.; Xu, L.; Sun, L.

2009-02-01

In this paper we presented a pulse shaping technique on regular solid-state lasers and the application in semiconductor micromachining. With a conventional Q-switched laser, all of the parameters can be adjusted over only limited ranges, especially the pulse width and pulse shape. However, some laser link processes using traditional laser pulses with pulse widths of a few nanoseconds to a few tens of nanoseconds tend to over-crater in thicker overlying passivation layers and thereby cause IC reliability problems. Use of a laser pulse with a special shape and a fast leading edge, such as tailored pulse, is one technique for controlling link processing. The pulse shaping technique is based on light-loop controlled optical modulation to shape conventional Q-switched solid-state lasers. One advantage of the pulse shaping technique is to provide a tailored pulse shape that can be programmed to have more than one amplitude value. Moreover, it has the capability of providing programmable tailored pulse shapes with discrete amplitude and time duration components. In addition, it provides fast rising and fall time of each pulse at fairly high repetition rate at 355nm with good beam quality. The regular-to-shaped efficiency is up to 50%. We conclude with a discussion of current results for laser processing of semiconductor memory link structures using programmable temporal pulse shapes. The processing experiments showed promising results with shaped pulse.

Interactions between butterfly-shaped pulses in the inhomogeneous media

DOE Office of Scientific and Technical Information (OSTI.GOV)

Liu, Wen-Jun; Beijing National Laboratory for Condensed Matter Physics, Institute of Physics, Chinese Academy of Sciences, Beijing 100190; Huang, Long-Gang

2014-10-15

Pulse interactions affect pulse qualities during the propagation. Interactions between butterfly-shaped pulses are investigated to improve pulse qualities in the inhomogeneous media. In order to describe the interactions between butterfly-shaped pulses, analytic two-soliton solutions are derived. Based on those solutions, influences of corresponding parameters on pulse interactions are discussed. Methods to control the pulse interactions are suggested. - Highlights: • Interactions between butterfly-shaped pulses are investigated. • Methods to control the pulse interactions are suggested. • Analytic two-soliton solutions for butterfly-shaped pulses are derived.

An adaptation method to improve secret key rates of time-frequency QKD in atmospheric turbulence channels

NASA Astrophysics Data System (ADS)

Sun, Xiaole; Djordjevic, Ivan B.; Neifeld, Mark A.

2016-03-01

Free-space optical (FSO) channels can be characterized by random power fluctuations due to atmospheric turbulence, which is known as scintillation. Weak coherent source based FSO quantum key distribution (QKD) systems suffer from the scintillation effect because during the deep channel fading the expected detection rate drops, which then gives an eavesdropper opportunity to get additional information about protocol by performing photon number splitting (PNS) attack and blocking single-photon pulses without changing QBER. To overcome this problem, in this paper, we study a large-alphabet QKD protocol, which is achieved by using pulse-position modulation (PPM)-like approach that utilizes the time-frequency uncertainty relation of the weak coherent photon state, called here TF-PPM-QKD protocol. We first complete finite size analysis for TF-PPM-QKD protocol to give practical bounds against non-negligible statistical fluctuation due to finite resources in practical implementations. The impact of scintillation under strong atmospheric turbulence regime is studied then. To overcome the secure key rate performance degradation of TF-PPM-QKD caused by scintillation, we propose an adaptation method for compensating the scintillation impact. By changing source intensity according to the channel state information (CSI), obtained by classical channel, the adaptation method improves the performance of QKD system with respect to the secret key rate. The CSI of a time-varying channel can be predicted using stochastic models, such as autoregressive (AR) models. Based on the channel state predictions, we change the source intensity to the optimal value to achieve a higher secret key rate. We demonstrate that the improvement of the adaptation method is dependent on the prediction accuracy.

Measurement of Fission Neutron Spectrum and Multiplicity using a Gamma Tag Double Time-of-flight Setup

NASA Astrophysics Data System (ADS)

Blain, E.; Daskalakis, A.; Danon, Y.

2014-05-01

Recent efforts have been made to improve the prompt fission neutron spectrum and nu-bar measurements for Uranium and Plutonium isotopes particularly in the keV region. A system has been designed at Rensselaer Polytechnic Institute (RPI) utilizing an array of EJ-301 liquid scintillators as well as lithium glass and plastic scintillators to experimentally determine these values. An array of BaF2 detectors was recently obtained from Oak Ridge National Laboratory to be used in conjunction with the neutron detectors. The system uses a novel gamma tagging method for fission which can offer an improvement over conventional fission chambers due to increased sample mass. A coincidence requirement on the gamma detectors from prompt fission gammas is used as the fission tag for the system as opposed to fission fragments in a conventional fission chamber. The system utilizes pulse digitization using Acqiris 8 bit digitizer boards which allow for gamma/neutron pulse height discrimination on the liquid scintillators during post processing. Additionally, a 252Cf fission chamber was designed and constructed at RPI which allowed for optimization and testing of the system without the need for an external neutron source. The characteristics of the gamma tagging method such as false detection rate and detection efficiency were determined using this fission chamber and verified using MCNP Polimi modeling. Prompt fission neutron spectrum data has been taken using the fission chamber focusing on the minimum detectable neutron energy for each of the various detectors. Plastic scintillators were found to offer a significant improvement over traditional liquid scintillators allowing energy measurements down to 50 keV. Background was also characterized for all detectors and will be discussed.

A method for characterizing after-pulsing and dark noise of PMTs and SiPMs

NASA Astrophysics Data System (ADS)

Butcher, A.; Doria, L.; Monroe, J.; Retière, F.; Smith, B.; Walding, J.

2017-12-01

Photo-multiplier tubes (PMTs) and silicon photo-multipliers (SiPMs) are detectors sensitive to single photons that are widely used for the detection of scintillation and Cerenkov light in subatomic physics and medical imaging. This paper presents a method for characterizing two of the main noise sources that PMTs and SiPMs share: dark noise and correlated noise (after-pulsing). The proposed method allows for a model-independent measurement of the after-pulsing timing distribution and dark noise rate.

An investigation of the digital discrimination of neutrons and γ rays with organic scintillation detectors using an artificial neural network

NASA Astrophysics Data System (ADS)

Liu, G.; Aspinall, M. D.; Ma, X.; Joyce, M. J.

2009-08-01

The discrimination of neutron and γ-ray events in an organic scintillator has been investigated by using a method based on an artificial neural network (ANN). Voltage pulses arising from an EJ-301 organic liquid scintillation detector in a mixed radiation field have been recorded with a fast digital sampling oscilloscope. Piled-up events have been disentangled using a pile-up management unit based on a fitting method. Each individual pulse has subsequently been sent to a discrimination unit which discriminates neutron and γ-ray events with a method based on an artificial neural network. This discrimination technique has been verified by the corresponding mixed-field data assessed by time of flight (TOF). It is shown that the characterization of the neutrons and photons achieved by the discrimination method based on the ANN is consistent with that afforded by TOF. This approach enables events that are often as a result of scattering or pile-up to be identified and returned to the data set and affords digital discrimination of mixed radiation fields in a broad range of environments on the basis of training obtained with a single TOF dataset.

Scintillation properties of Gd3Al2Ga3O12:Ce (GAGG:Ce): a comparison between monocrystalline and nanoceramic samples

NASA Astrophysics Data System (ADS)

Drozdowski, Winicjusz; Witkowski, Marcin E.; Solarz, Piotr; Głuchowski, Paweł; Głowacki, Michał; Brylew, Kamil

2018-05-01

In this Communication the behavior of two types of Gd3Al2Ga3O12:Ce samples under gamma and X-ray excitation is compared. Single crystals of GAGG:1%Ce have been grown by the Czochralski technique, while nanoceramic pills of GAGG:1%Ce have been fabricated by the LTHP sintering from nanocrystalline powders prepared by the Pechini method. The results of pulse height, scintillation time profile, radioluminescence as a function of temperature, and low temperature thermoluminescence measurements, are reported, indicating that monocrystals are still a better choice for scintillator application, nevertheless some of the properties of nanoceramics are indeed promising and there should be a room for improvement.

On-line tritium production monitor

DOEpatents

Mihalczo, John T.

1993-01-01

A scintillation optical fiber system for the on-line monitoring of nuclear reactions in an event-by-event manner is described. In the measurement of tritium production one or more optical fibers are coated with enriched .sup.6 Li and connected to standard scintillation counter circuitry. A neutron generated .sup.6 Li(n )T reaction occurs in the coated surface of .sup.6 Li-coated fiber to produce energetic alpha and triton particles one of which enters the optical fiber and scintillates light through the fiber to the counting circuit. The coated optical fibers can be provided with position sensitivity by placing a mirror at the free end of the fibers or by using pulse counting circuits at both ends of the fibers.

On-line tritium production monitor

DOEpatents

Mihalczo, J.T.

1993-11-23

A scintillation optical fiber system for the on-line monitoring of nuclear reactions in an event-by-event manner is described. In the measurement of tritium production one or more optical fibers are coated with enriched {sup 6}Li and connected to standard scintillation counter circuitry. A neutron generated {sup 6}Li(n)T reaction occurs in the coated surface of {sup 6}Li-coated fiber to produce energetic alpha and triton particles one of which enters the optical fiber and scintillates light through the fiber to the counting circuit. The coated optical fibers can be provided with position sensitivity by placing a mirror at the free end of the fibers or by using pulse counting circuits at both ends of the fibers. 5 figures.

Pulse Shaped 8-PSK Bandwidth Efficiency and Spectral Spike Elimination

NASA Technical Reports Server (NTRS)

Tao, Jian-Ping

1998-01-01

The most bandwidth-efficient communication methods are imperative to cope with the congested frequency bands. Pulse shaping methods have excellent effects on narrowing bandwidth and increasing band utilization. The position of the baseband filters for the pulse shaping is crucial. Post-modulation pulse shaping (a low pass filter is located after the modulator) can change signals from constant envelope to non-constant envelope, and non-constant envelope signals through non-linear device (a SSPA or TWT) can further spread the power spectra. Pre-modulation pulse shaping (a filter is located before the modulator) will have constant envelope. These two pulse shaping methods have different effects on narrowing the bandwidth and producing bit errors. This report studied the effect of various pre-modulation pulse shaping filters with respect to bandwidth, spectral spikes and bit error rate. A pre-modulation pulse shaped 8-ary Phase Shift Keying (8PSK) modulation was used throughout the simulations. In addition to traditional pulse shaping filters, such as Bessel, Butterworth and Square Root Raised Cosine (SRRC), other kinds of filters or pulse waveforms were also studied in the pre-modulation pulse shaping method. Simulations were conducted by using the Signal Processing Worksystem (SPW) software package on HP workstations which simulated the power spectral density of pulse shaped 8-PSK signals, end to end system performance and bit error rates (BERS) as a function of Eb/No using pulse shaping in an AWGN channel. These results are compared with the post-modulation pulse shaped 8-PSK results. The simulations indicate traditional pulse shaping filters used in pre-modulation pulse shaping may produce narrower bandwidth, but with worse BER than those in post-modulation pulse shaping. Theory and simulations show pre- modulation pulse shaping could also produce discrete line power spectra (spikes) at regular frequency intervals. These spikes may cause interference with adjacent channel and reduce power efficiency. Some particular pulses (filters), such as trapezoid and pulses with different transits (such as weighted raised cosine transit) were found to reduce bandwidth and not generate spectral spikes. Although a solid state power amplifier (SSPA) was simulated in the non-linear (saturation) region, output power spectra did not spread due to the constant envelope 8-PSK signals.

A SPECT system simulator built on the SolidWorks TM 3D-Design package.

PubMed

Li, Xin; Furenlid, Lars R

2014-08-17

We have developed a GPU-accelerated SPECT system simulator that integrates into instrument-design workflow [1]. This simulator includes a gamma-ray tracing module that can rapidly propagate gamma-ray photons through arbitrary apertures modeled by SolidWorks TM -created stereolithography (.STL) representations with a full complement of physics cross sections [2, 3]. This software also contains a scintillation detector simulation module that can model a scintillation detector with arbitrary scintillation crystal shape and light-sensor arrangement. The gamma-ray tracing module enables us to efficiently model aperture and detector crystals in SolidWorks TM and save them as STL file format, then load the STL-format model into this module to generate list-mode results of interacted gamma-ray photon information (interaction positions and energies) inside the detector crystals. The Monte-Carlo scintillation detector simulation module enables us to simulate how scintillation photons get reflected, refracted and absorbed inside a scintillation detector, which contributes to more accurate simulation of a SPECT system.

A SPECT system simulator built on the SolidWorksTM 3D design package

NASA Astrophysics Data System (ADS)

Li, Xin; Furenlid, Lars R.

2014-09-01

We have developed a GPU-accelerated SPECT system simulator that integrates into instrument-design work flow [1]. This simulator includes a gamma-ray tracing module that can rapidly propagate gamma-ray photons through arbitrary apertures modeled by SolidWorksTM-created stereolithography (.STL) representations with a full com- plement of physics cross sections [2, 3]. This software also contains a scintillation detector simulation module that can model a scintillation detector with arbitrary scintillation crystal shape and light-sensor arrangement. The gamma-ray tracing module enables us to efficiently model aperture and detector crystals in SolidWorksTM and save them as STL file format, then load the STL-format model into this module to generate list-mode results of interacted gamma-ray photon information (interaction positions and energies) inside the detector crystals. The Monte-Carlo scintillation detector simulation module enables us to simulate how scintillation photons get reflected, refracted and absorbed inside a scintillation detector, which contributes to more accurate simulation of a SPECT system.

Modeling Photo-multiplier Gain and Regenerating Pulse Height Data for Application Development

NASA Astrophysics Data System (ADS)

Aspinall, Michael D.; Jones, Ashley R.

2018-01-01

Systems that adopt organic scintillation detector arrays often require a calibration process prior to the intended measurement campaign to correct for significant performance variances between detectors within the array. These differences exist because of low tolerances associated with photo-multiplier tube technology and environmental influences. Differences in detector response can be corrected for by adjusting the supplied photo-multiplier tube voltage to control its gain and the effect that this has on the pulse height spectra from a gamma-only calibration source with a defined photo-peak. Automated methods that analyze these spectra and adjust the photo-multiplier tube bias accordingly are emerging for hardware that integrate acquisition electronics and high voltage control. However, development of such algorithms require access to the hardware, multiple detectors and calibration source for prolonged periods, all with associated constraints and risks. In this work, we report on a software function and related models developed to rescale and regenerate pulse height data acquired from a single scintillation detector. Such a function could be used to generate significant and varied pulse height data that can be used to integration-test algorithms that are capable of automatically response matching multiple detectors using pulse height spectra analysis. Furthermore, a function of this sort removes the dependence on multiple detectors, digital analyzers and calibration source. Results show a good match between the real and regenerated pulse height data. The function has also been used successfully to develop auto-calibration algorithms.

Assessment of beryllium and molybdenum nuclear data files with the RPI neutron scattering system in the energy region from 0.5 to 20 MeV

NASA Astrophysics Data System (ADS)

Daskalakis, Adam; Blain, Ezekiel; Leinweber, Gregory; Rapp, Michael; Barry, Devin; Block, Robert; Danon, Yaron

2017-09-01

A series of neutron scattering benchmark measurements were performed on beryllium and molybdenum with the Rensselaer Polytechnic Institute's Neutron Scattering System. The pulsed neutron source was produced by the Rensselaer Polytechnic Institute's Linear Accelerator and a well collimated neutron beam was incident onto the samples located at a distance of 30.07 m. Neutrons that scattered from the sample were measured using the time-of-flight by eight EJ-301 liquid scintillator detectors positioned 0.5 m from the sample of interest. A total of eight experiments were performed with two sample thicknesses each, measured by detectors placed at two sets of angles. All data were processed using pulse shape analysis that separated the neutron and gamma ray events and included a gamma misclassification correction to account for erroneously identified gamma rays. A detailed model of the neutron scattering system simulated each experiment with several current evaluated nuclear data libraries and their predecessors. Results for each evaluation were compared to the experimental data using a figure-of-merit. The neutron scattering system has been used as a means to quantify a library's performance.

Gamma-ray detector employing scintillators coupled to semiconductor drift photodetectors

DOE Office of Scientific and Technical Information (OSTI.GOV)

Iwanczyk, Jan S.; Patt, Bradley E.

Radiation detectors according to one embodiment of the invention are implemented using scintillators combined with a semiconductor drift photodetectors wherein the components are specifically constructed in terms of their geometry, dimensions, and arrangement so that the scintillator decay time and drift time in the photodetector pairs are matched in order to achieve a greater signal-to-noise ratio. The detectors may include electronics for amplification of electrical signals produced by the silicon drift photodetector, the amplification having a shaping time optimized with respect to the decay time of the scintillator and time spread of the signal in the silicon drift photodetector tomore » substantially maximize the ratio of the signal to the electronic noise.« less

A novel design for scintillator-based neutron and gamma imaging in inertial confinement fusion

NASA Astrophysics Data System (ADS)

Geppert-Kleinrath, Verena; Cutler, Theresa; Danly, Chris; Madden, Amanda; Merrill, Frank; Tybo, Josh; Volegov, Petr; Wilde, Carl

2017-10-01

The LANL Advanced Imaging team has been providing reliable 2D neutron imaging of the burning fusion fuel at NIF for years, revealing possible multi-dimensional asymmetries in the fuel shape, and therefore calling for additional views. Adding a passive imaging system using image plate techniques along a new polar line of sight has recently demonstrated the merit of 3D neutron image reconstruction. Now, the team is in the process of designing a new active neutron imaging system for an additional equatorial view. The design will include a gamma imaging system as well, to allow for the imaging of carbon in the ablator of the NIF fuel capsules, constraining the burning fuel shape even further. The selection of ideal scintillator materials for a position-sensitive detector system is the key component for the new design. A comprehensive study of advanced scintillators has been carried out at the Los Alamos Neutron Science Center and the OMEGA Laser Facility in Rochester, NY. Neutron radiography using a fast-gated CCD camera system delivers measurements of resolution, light output and noise characteristics. The measured performance parameters inform the novel design, for which we conclude the feasibility of monolithic scintillators over pixelated counterparts.

Mitigation of ^{42}Ar/^{42}K background for the GERDA Phase II experiment

NASA Astrophysics Data System (ADS)

Lubashevskiy, A.; Agostini, M.; Budjáš, D.; Gangapshev, A.; Gusev, K.; Heisel, M.; Klimenko, A.; Lazzaro, A.; Lehnert, B.; Pelczar, K.; Schönert, S.; Smolnikov, A.; Walter, M.; Zuzel, G.

2018-01-01

Background coming from the ^{42}Ar decay chain is considered to be one of the most relevant for the Gerda experiment, which searches for the neutrinoless double beta decay of ^{76}Ge. The sensitivity strongly relies on the absence of background around the Q-value of the decay. Background coming from ^{42}K, a progeny of ^{42}Ar, can contribute to that background via electrons from the continuous spectrum with an endpoint at 3.5 MeV. Research and development on the suppression methods targeting this source of background were performed at the low-background test facility LArGe . It was demonstrated that by reducing ^{42}K ion collection on the surfaces of the broad energy germanium detectors in combination with pulse shape discrimination techniques and an argon scintillation veto, it is possible to suppress ^{42}K background by three orders of magnitude. This is sufficient for Phase II of the Gerda experiment.

The Goals and Status of SoLid Experiment

NASA Astrophysics Data System (ADS)

Park, Jaewon

2016-09-01

SoLid is a short baseline sterile neutrino oscillation search experiment using the BR2 compact core reactor in Belgium. Ruling out or confirming sterile neutrino is one of main interests in the neutrino physics field. Highly segmented scintillator cube detector with 6LiF:ZnS(Ag) neutron screen provides high purity neutron tagging by pulse shape discrimination (PSD), and capture position identification. These capabilities from this novel detector are critical to isolate neutrino interactions in a high background environment. The prototype detector (SM1) provides important feedback for validating the performance of the detector design. Recent results from SM1 will be presented. Construction of the SoLid Phase-1 detector is underway. The three-ton detector with three years running will allow us to reach the sterile neutrino exclusion limit of sin2 2 θ < 0 . 03 at Δm2 2eV2 at the 99% confidence level.

Simulation of argon response and light detection in the DarkSide-50 dual phase TPC

NASA Astrophysics Data System (ADS)

Agnes, P.; Albuquerque, I. F. M.; Alexander, T.; Alton, A. K.; Asner, D. M.; Back, H. O.; Biery, K.; Bocci, V.; Bonfini, G.; Bonivento, W.; Bossa, M.; Bottino, B.; Budano, F.; Bussino, S.; Cadeddu, M.; Cadoni, M.; Calaprice, F.; Canci, N.; Candela, A.; Caravati, M.; Cariello, M.; Carlini, M.; Catalanotti, S.; Cataudella, V.; Cavalcante, P.; Chepurnov, A.; Cicalò, C.; Cocco, A. G.; Covone, G.; D'Angelo, D.; D'Incecco, M.; Davini, S.; de Candia, A.; De Cecco, S.; De Deo, M.; De Filippis, G.; De Vincenzi, M.; Derbin, A. V.; De Rosa, G.; Devoto, A.; Di Eusanio, F.; Di Pietro, G.; Dionisi, C.; Edkins, E.; Empl, A.; Fan, A.; Fiorillo, G.; Fomenko, K.; Franco, D.; Gabriele, F.; Galbiati, C.; Giagu, S.; Giganti, C.; Giovanetti, G. K.; Goretti, A. M.; Granato, F.; Gromov, M.; Guan, M.; Guardincerri, Y.; Hackett, B. R.; Herner, K.; Hughes, D.; Humble, P.; Hungerford, E. V.; Ianni, An.; James, I.; Johnson, T. N.; Keeter, K.; Kendziora, C. L.; Koh, G.; Korablev, D.; Korga, G.; Kubankin, A.; Li, X.; Lissia, M.; Loer, B.; Longo, G.; Ma, Y.; Machado, A. A.; Machulin, I. N.; Mandarano, A.; Mari, S. M.; Maricic, J.; Martoff, C. J.; Meyers, P. D.; Milincic, R.; Monte, A.; Mount, B. J.; Muratova, V. N.; Musico, P.; Napolitano, J.; Navrer Agasson, A.; Oleinik, A.; Orsini, M.; Ortica, F.; Pagani, L.; Pallavicini, M.; Pantic, E.; Pelczar, K.; Pelliccia, N.; Pocar, A.; Pordes, S.; Pugachev, D. A.; Qian, H.; Randle, K.; Razeti, M.; Razeto, A.; Reinhold, B.; Renshaw, A. L.; Rescigno, M.; Riffard, Q.; Romani, A.; Rossi, B.; Rossi, N.; Sablone, D.; Sands, W.; Sanfilippo, S.; Savarese, C.; Schlitzer, B.; Segreto, E.; Semenov, D. A.; Singh, P. N.; Skorokhvatov, M. D.; Smirnov, O.; Sotnikov, A.; Stanford, C.; Suvorov, Y.; Tartaglia, R.; Testera, G.; Tonazzo, A.; Trinchese, P.; Unzhakov, E. V.; Verducci, M.; Vishneva, A.; Vogelaar, B.; Wada, M.; Walker, S.; Wang, H.; Wang, Y.; Watson, A. W.; Westerdale, S.; Wilhelmi, J.; Wojcik, M. M.; Xiang, X.; Xiao, X.; Yang, C.; Ye, Z.; Zhu, C.; Zuzel, G.

2017-10-01

A Geant4-based Monte Carlo package named G4DS has been developed to simulate the response of DarkSide-50, an experiment operating since 2013 at LNGS, designed to detect WIMP interactions in liquid argon. In the process of WIMP searches, DarkSide-50 has achieved two fundamental milestones: the rejection of electron recoil background with a power of ~107, using the pulse shape discrimination technique, and the measurement of the residual 39Ar contamination in underground argon, ~3 orders of magnitude lower with respect to atmospheric argon. These results rely on the accurate simulation of the detector response to the liquid argon scintillation, its ionization, and electron-ion recombination processes. This work provides a complete overview of the DarkSide Monte Carlo and of its performance, with a particular focus on PARIS, the custom-made liquid argon response model.

Radiation Templates of Spent Fuel in Casks

DOE Office of Scientific and Technical Information (OSTI.GOV)

Vanier, Peter

BNL and INL propose to perform a scoping study, using heavily collimated gamma and fast neutron detectors, to obtain passive radiation templates of dry storage casks containing spent fuel. The goal is to demonstrate sufficient spatial resolution and sensitivity to detect a missing fuel assembly. Such measurements, combined with detailed modeling and decay corrections should provide confidence that the cask contents have not been altered, despite loss of continuity of knowledge (CoK). The concept relies on the leakage of high energy gammas and neutrons through the shielding of the casks. Tests will emphasize organic scintillators with pulse shape discrimination, butmore » baseline comparisons will be made to high purity germanium (HPGe) and collimated moderated 3He detectors deployed in the same locations. Commercial off-the-shelf (COTS) detectors and data acquisition electronics will be used with custom-built collimators and shielding.« less

DOE Office of Scientific and Technical Information (OSTI.GOV)

Xu, Jingke; Stanford, Chris; Westerdale, Shawn

Here, one major background in direct searches for weakly interacting massive particles (WIMPs) comes from the deposition of radon progeny on detector surfaces. A dangerous surface background is the 206Pb nuclear recoils produced by 210Po decays. In this paper, we report the first characterization of this background in liquid argon. The scintillation signal of low energy Pb recoils is measured to be highly quenched in argon, and we estimate that the 103 keV 206Pb recoil background will produce a signal equal to that of a ~5 keV (30 keV) electron recoil ( 40Ar recoil). In addition, we demonstrate that thismore » dangerous 210Po surface background can be suppressed, using pulse shape discrimination methods, by a factor of ~100 or higher, which can make argon dark matter detectors near background-free and enhance their potential for discovery of medium- and high-mass WIMPs. Lastly, we also discuss the impact on other low background experiments.« less

PANDORA, a large volume low-energy neutron detector with real-time neutron-gamma discrimination

NASA Astrophysics Data System (ADS)

Stuhl, L.; Sasano, M.; Yako, K.; Yasuda, J.; Baba, H.; Ota, S.; Uesaka, T.

2017-09-01

The PANDORA (Particle Analyzer Neutron Detector Of Real-time Acquisition) system, which was developed for use in inverse kinematics experiments with unstable isotope beams, is a neutron detector based on a plastic scintillator coupled to a digital readout. PANDORA can be used for any reaction study involving the emission of low energy neutrons (100 keV-10 MeV) where background suppression and an increased signal-to-noise ratio are crucial. The digital readout system provides an opportunity for pulse shape discrimination (PSD) of the detected particles as well as intelligent triggering based on PSD. The figure of merit results of PANDORA are compared to the data in literature. Using PANDORA, 91 ± 1% of all detected neutrons can be separated, while 91 ± 1% of the detected gamma rays can be excluded, reducing the gamma ray background by one order of magnitude.

Pulse shaping with transmission lines

DOEpatents

Wilcox, Russell B.

1987-01-01

A method and apparatus for forming shaped voltage pulses uses passive reflection from a transmission line with nonuniform impedance. The impedance of the reflecting line varies with length in accordance with the desired pulse shape. A high voltage input pulse is transmitted to the reflecting line. A reflected pulse is produced having the desired shape and is transmitted by pulse removal means to a load. Light activated photoconductive switches made of silicon can be utilized. The pulse shaper can be used to drive a Pockels cell to produce shaped optical pulses.

Pulse shaping with transmission lines

DOEpatents

Wilcox, R.B.

1985-08-15

A method and apparatus for forming shaped voltage pulses uses passive reflection from a transmission line with nonuniform impedance. The impedance of the reflecting line varies with length in accordance with the desired pulse shape. A high voltage input pulse is transmitted to the reflecting line. A reflected pulse is produced having the desired shape and is transmitted by pulse removal means to a load. Light activated photoconductive switches made of silicon can be utilized. The pulse shaper can be used to drive a Pockels cell to produce shaped optical pulses.

PULSE AMPLIFIER

DOEpatents

Johnstone, C.W.

1958-06-17

The improvement of pulse amplifiers used with scintillation detectors is described. The pulse amplifier circuit has the advantage of reducing the harmful effects of overloading cause by large signal inputs. In general the pulse amplifier circuit comprises two amplifier tubes with the input pulses applied to one amplifier grid and coupled to the second amplifier tube through a common cathode load. The output of the second amplifier is coupled from the plate circuit to a cathode follower tube grid and a diode tube in connected from grid to cathode of the cathode follower tube. Degenerative feedback is provided in the second amplifier by coupling a signal from the cathode follower cathode to the second amplifier grid. The circuit proqides moderate gain stability, and overload protection for subsequent pulse circuits.

Low-background EN-detector for the investigation of the neutron component of EASs

NASA Astrophysics Data System (ADS)

Gromushkin, D. M.; Bogdanov, F. A.; Lakhonin, A. A.; Petrukhin, A. A.; Stenkin, Yu. V.; Shchegolev, O. B.; Yurin, K. O.; Yashin, I. I.

2018-01-01

Thermal neutrons are detected using a scintillator compound based on ZnS(Ag) with B2O3 added to it. The pulse height generated by single charged particles in a scintillator of small thickness (50 mg/cm2) is not larger than that of a noise signal due to a low sensitivity to single charged particles. As a result, the detector satisfies the requirements of a low-background one in the context of cosmic-ray experiments. The detector is to be used for neutron detection in extensive air showers.

A high-rate 10B-loaded liquid scintillation detector for parity-violation studies in neutron resonances

NASA Astrophysics Data System (ADS)

Yen, Yi-Fen; Bowman, J. D.; Bolton, R. D.; Crawford, B. E.; Delheij, P. P. J.; Hart, G. W.; Haseyama, T.; Frankle, C. M.; Iinuma, M.; Knudson, J. N.; Masaike, A.; Masuda, Y.; Matsuda, Y.; Mitchell, G. E.; Penttilä, S. I.; Roberson, N. R.; Seestrom, S. J.; Sharapov, E.; Shimizu, H. M.; Smith, D. A.; Stephenson, S. L.; Szymanski, J. J.; Yoo, S. H.; Yuan, V. W.

2000-06-01

We have developed a large-area 10B-loaded liquid scintillation detector for parity-violation studies in neutron resonances with high instantaneous neutron fluxes from the LANSCE short-pulse spallation source. The detector has an efficiency of 95%, 85% and 71% at neutron energies of 10, 100 and 1000 eV, respectively. The neutron mean capture time in the detector is (416±5) ns. We describe the detector and the current-mode signal processing system, that can handle neutron rates up to 500 MHz.

Above-ground Antineutrino Detection for Nuclear Reactor Monitoring

DOE PAGES

Sweany, Melinda; Brennan, James S.; Cabrera-Palmer, Belkis; ...

2014-08-01

Antineutrino monitoring of nuclear reactors has been demonstrated many times, however the technique has not as of yet been developed into a useful capability for treaty verification purposes. The most notable drawback is the current requirement that detectors be deployed underground, with at least several meters-water-equivalent of shielding from cosmic radiation. In addition, the deployment of liquid-based detector media presents a challenge in reactor facilities. We are currently developing a detector system that has the potential to operate above ground and circumvent deployment problems associated with a liquid detection media: the system is composed of segments of plastic scintillator surroundedmore » by 6LiF/ZnS:Ag. ZnS:Ag is a radio-luminescent phosphor used to detect the neutron capture products of lithium-6. Because of its long decay time compared to standard plastic scintillators, pulse-shape discrimination can be used to distinguish positron and neutron interactions resulting from the inverse beta decay (IBD) of antineutrinos within the detector volume, reducing both accidental and correlated backgrounds. Segmentation further reduces backgrounds by identifying the positron’s annihilation gammas, which are absent for most correlated and uncorrelated backgrounds. This work explores different configurations in order to maximize the size of the detector segments without reducing the intrinsic neutron detection efficiency. We believe this technology will ultimately be applicable to potential safeguards scenarios such as those recently described.« less

Darkside-20k: A 20 ton Liquid Argon Dark Matter Experiment

NASA Astrophysics Data System (ADS)

Back, Henning; Darkside-20k Collaboration

2016-03-01

The Darkside-20k detector is the next step in the Darkside dark matter search program at the Laboratori Nazionali del Gran Sasso in Italy. The Darkside detectors have grown in fiducial mass starting with 10kg in Darkside10, to 50 kg in Darkside50, and finally a proposed 20,000 kg fiducial mass, Darkside20k. The Darkside detectors are dual-phase argon TPCs that combine the very powerful scintillation pulse-shape analysis and ionization information to discriminate against background events. Two unique aspects to the Darkside program is the use of an external neutron veto based on borated liquid scintillator, and the use of low radioactivity argon from underground sources as the target. Argon from the atmosphere has an 39Ar activity of 1Bq/kg, which would be the limiting background, but the underground argon is essentially free of 39Ar. Additionally, the detector is placed in a water Cherenkov muon veto. Combining all these techniques allows Darkside-20k to achieve a background-free 100 t-yr exposure accumulated in a 5 yr run. Darkside-20k is expected to start operations in 2020 with data taking starting in 2021, and will be sensitive to WIMP-nucleon interaction cross sections of 1×10-47 cm2 (1x10-46 cm2) for WIMPs of 1 TeV/c2 (10 TeV/c2) mass.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Sweany, Melinda; Brennan, James S.; Cabrera-Palmer, Belkis

Antineutrino monitoring of nuclear reactors has been demonstrated many times, however the technique has not as of yet been developed into a useful capability for treaty verification purposes. The most notable drawback is the current requirement that detectors be deployed underground, with at least several meters-water-equivalent of shielding from cosmic radiation. In addition, the deployment of liquid-based detector media presents a challenge in reactor facilities. We are currently developing a detector system that has the potential to operate above ground and circumvent deployment problems associated with a liquid detection media: the system is composed of segments of plastic scintillator surroundedmore » by 6LiF/ZnS:Ag. ZnS:Ag is a radio-luminescent phosphor used to detect the neutron capture products of lithium-6. Because of its long decay time compared to standard plastic scintillators, pulse-shape discrimination can be used to distinguish positron and neutron interactions resulting from the inverse beta decay (IBD) of antineutrinos within the detector volume, reducing both accidental and correlated backgrounds. Segmentation further reduces backgrounds by identifying the positron’s annihilation gammas, which are absent for most correlated and uncorrelated backgrounds. This work explores different configurations in order to maximize the size of the detector segments without reducing the intrinsic neutron detection efficiency. We believe this technology will ultimately be applicable to potential safeguards scenarios such as those recently described.« less

Laser fusion pulse shape controller

DOEpatents

Siebert, Larry D.

1977-01-01

An apparatus for controlling the pulse shape, i.e., the pulse duration and intensity pattern, of a pulsed laser system, and which is particularly well adapted for controlling the pellet ignition pulse in a laser-driven fusion reaction system. The apparatus comprises a laser generator for providing an optical control pulse of the shape desired, a pulsed laser triggered by the control pulse, and a plurality of optical Kerr-effect gates serially disposed at the output of the pulsed laser and selectively triggered by the control pulse to pass only a portion of the pulsed laser output generally corresponding in shape to the control pulse.

Determination of the energy dependence of the BC-408 plastic scintillation detector in medium energy x-ray beams

NASA Astrophysics Data System (ADS)

Yücel, H.; Çubukçu, Ş.; Uyar, E.; Engin, Y.

2014-11-01

The energy dependence of the response of BC-408 plastic scintillator (PS), an approximately water-equivalent material, has been investigated by employing standardized x-ray beams. IEC RQA and ISO N series x-ray beam qualities, in the range of 40-100 kVp, were calibrated using a PTW-type ionization chamber. The energy response of a thick BC-408 PS detector was measured using the multichannel pulse height analysis method. The response of BC-408 PS increased gradually with increasing energy in the energy range of 40-80 kVp and then showed a flat behavior at about 80 to 120 kVp. This might be due to the self-attenuation of scintillation light by the scintillator itself and may also be partly due to the ionization quenching, leading to a reduction in the intensity of the light output from the scintillator. The results indicated that the sensitivity drop in BC-408 PS material at lower photon energies may be overcome by adding some high-Z elements to its polyvinyltoluene (PVT) base. The material modification may compensate for the drop in the response at lower photon energies. Thus plastic scintillation dosimetry is potentially suitable for applications in diagnostic radiology.

Determination of the energy dependence of the BC-408 plastic scintillation detector in medium energy x-ray beams.

PubMed

Yücel, H; Çubukçu, Ş; Uyar, E; Engin, Y

2014-11-21

The energy dependence of the response of BC-408 plastic scintillator (PS), an approximately water-equivalent material, has been investigated by employing standardized x-ray beams. IEC RQA and ISO N series x-ray beam qualities, in the range of 40-100 kVp, were calibrated using a PTW-type ionization chamber. The energy response of a thick BC-408 PS detector was measured using the multichannel pulse height analysis method. The response of BC-408 PS increased gradually with increasing energy in the energy range of 40-80 kVp and then showed a flat behavior at about 80 to 120 kVp. This might be due to the self-attenuation of scintillation light by the scintillator itself and may also be partly due to the ionization quenching, leading to a reduction in the intensity of the light output from the scintillator. The results indicated that the sensitivity drop in BC-408 PS material at lower photon energies may be overcome by adding some high-Z elements to its polyvinyltoluene (PVT) base. The material modification may compensate for the drop in the response at lower photon energies. Thus plastic scintillation dosimetry is potentially suitable for applications in diagnostic radiology.

Time and position sensitive single photon detector for scintillator read-out

NASA Astrophysics Data System (ADS)

Schössler, S.; Bromberger, B.; Brandis, M.; Schmidt, L. Ph H.; Tittelmeier, K.; Czasch, A.; Dangendorf, V.; Jagutzki, O.

2012-02-01

We have developed a photon counting detector system for combined neutron and γ radiography which can determine position, time and intensity of a secondary photon flash created by a high-energy particle or photon within a scintillator screen. The system is based on a micro-channel plate photomultiplier concept utilizing image charge coupling to a position- and time-sensitive read-out anode placed outside the vacuum tube in air, aided by a standard photomultiplier and very fast pulse-height analyzing electronics. Due to the low dead time of all system components it can cope with the high throughput demands of a proposed combined fast neutron and dual discrete energy γ radiography method (FNDDER). We show tests with different types of delay-line read-out anodes and present a novel pulse-height-to-time converter circuit with its potential to discriminate γ energies for the projected FNDDER devices for an automated cargo container inspection system (ACCIS).

Waveform synthesizer

DOEpatents

Franks, L.A.; Nelson, M.A.

1979-12-07

The invention is a method by which an optical pulse of an arbitrary but defined shape may be transformed into a virtual multitude of optical or electrical output pulse shapes. Since the method is not limited to any particular input pulse shape, the output pulse shapes that can be generated thereby are virtually unlimited. Moreover, output pulse widths as narrow as about 0.1 nsec can be readily obtained since optical pulses of less than a few picoseconds are available for use as driving pulses. The range of output pulse widths obtainable is very large, the limiting factors being the driving source energy and the particular shape of the desired output pulse.

Single-shot positron annihilation lifetime spectroscopy with LYSO scintillators

NASA Astrophysics Data System (ADS)

Alonso, A. M.; Cooper, B. S.; Deller, A.; Cassidy, D. B.

2016-08-01

We have evaluated the application of a lutetium yttrium oxyorthosilicate (LYSO) based detector to single-shot positron annihilation lifetime spectroscopy. We compare this detector directly with a similarly configured PbWO4 scintillator, which is the usual choice for such measurements. We find that the signal to noise ratio obtained using LYSO is around three times higher than that obtained using PbWO4 for measurements of Ps excited to longer-lived (Rydberg) levels, or when they are ionized soon after production. This is due to the much higher light output for LYSO (75% and 1% of NaI for LYSO and PbWO4 respectively). We conclude that LYSO is an ideal scintillator for single-shot measurements of positronium production and excitation performed using a low-intensity pulsed positron beam.

Tests of a solution-grown stilbene scintillator in mono-energetic neutron beams of 565 keV and 5 MeV

NASA Astrophysics Data System (ADS)

Dioni, Luca; Gressier, Vincent; Nardin, Gaëlle; Jacqmin, Robert; Stout, Brian; Sumini, Marco

2018-02-01

The results of measurements performed with a solution-grown stilbene scintillator placed in reference mono-energetic neutron fields are presented. The ∅ 25 mm organic scintillator was positioned in 5 MeV and 565 keV neutron fields delivered by the AIFIRA facility at CENBG. The goal of the experiment was to assess the performance of the solution-grown stilbene crystal (n- γ discrimination, response, anisotropy, sensitivity) relative to that of a BC501A liquid scintillator of larger size. Neutron pulse height spectra after gamma discrimination are compared. The results show that the stilbene crystal not only has a better discrimination capability than the BC501A (35% higher FoM) at 5 MeV, but is also able to separate neutrons from gamma-rays at 565 keV and below, a range where the BC501A is inoperative. This study also confirms the anisotropy of the crystal response, as already observed by other groups at different energies.

Monte Carlo simulations and measurements for efficiency determination of lead shielded plastic scintillator detectors

NASA Astrophysics Data System (ADS)

Yasin, Zafar; Negoita, Florin; Tabbassum, Sana; Borcea, Ruxandra; Kisyov, Stanimir

2017-12-01

The plastic scintillators are used in different areas of science and technology. One of the use of these scintillator detectors is as beam loss monitors (BLM) for new generation of high intensity heavy ion in superconducting linear accelerators. Operated in pulse counting mode with rather high thresholds and shielded by few centimeters of lead in order to cope with radiofrequency noise and X-ray background emitted by accelerator cavities, they preserve high efficiency for high energy gamma ray and neutrons produced in the nuclear reactions of lost beam particles with accelerator components. Efficiency calculation and calibration of detectors is very important before their practical usage. In the present work, the efficiency of plastic scintillator detectors is simulated using FLUKA for different gamma and neutron sources like, 60Co, 137Cs and 238Pu-Be. The sources are placed at different positions around the detector. Calculated values are compared with the measured values and a reasonable agreement is observed.

SATSIN System Manual.

DTIC Science & Technology

1995-01-01

This report outlines the design, functions and operation of the HAARP Diagnostic Satellite Scintillation (SATSIN) system that will be used to...be located so that the propagation path from satellite radio beacons passes through the heated volume created by HAARP . The signal, altered in phase...characteristics of the scintillation. From this information, the strength, shape and motion of the in situ irregularities generated by HAARP can be implied. The

Energy resolution experiments of conical organic scintillators and a comparison with Geant4 simulations

NASA Astrophysics Data System (ADS)

Sosa, C. S.; Thompson, S. J.; Chichester, D. L.; Clarke, S. D.; Di Fulvio, A.; Pozzi, S. A.

2018-08-01

An increase in light-collection efficiency (LCE) improves the energy resolution of scintillator-based detection systems. An improvement in energy resolution can benefit detector performance, for example by lowering the measurement threshold and achieving greater accuracy in light-output calibration. This work shows that LCE can be increased by modifying the scintillator shape to reduce optical-photon reflections, thereby decreasing transmission and absorption likelihood at the reflector boundary. The energy resolution of four organic scintillators (EJ200) were compared: two cones and two right-circular cylinders, all with equal base diameter and height (50 mm). The sides of each shape had two surface conditions: one was polished and the other was ground. Each scintillator was coupled to the center of four photomultiplier tube (PMT) configurations of different diameters. The photocathode response of all PMTs was assessed as a function of position using a small cube (5 mm height) of EJ200. The worst configuration, a highly polished conical scintillator mated to a PMT of equal base diameter, produced a smeared energy spectrum. The cause of spectrum smearing is explored in detail. Results demonstrate that a ground cone had the greatest improvement in energy resolution over a ground cylinder by approximately 16.2% at 478 keVee, when using the largest diameter (127 mm) PMT. This result is attributed to the greater LCE of the cone, its ground surface, and the uniform photocathode response near center of the largest PMT. Optical-photon transport simulations in Geant4 of the cone and cylinder assuming a diffuse reflector and a uniform photocathode were compared to the best experimental configuration and agreed well. If a detector application requires excellent energy resolution above all other considerations, a ground cone on a large PMT is recommended over a cylinder.

Two detector arrays for fast neutrons at LANSCE

NASA Astrophysics Data System (ADS)

Haight, R. C.; Lee, H. Y.; Taddeucci, T. N.; O'Donnell, J. M.; Perdue, B. A.; Fotiades, N.; Devlin, M.; Ullmann, J. L.; Laptev, A.; Bredeweg, T.; Jandel, M.; Nelson, R. O.; Wender, S. A.; White, M. C.; Wu, C. Y.; Kwan, E.; Chyzh, A.; Henderson, R.; Gostic, J.

2012-03-01

The neutron spectrum from neutron-induced fission needs to be known in designing new fast reactors, predicting criticality for safety analyses, and developing techniques for global security application. The experimental data base of fission neutron spectra is very incomplete and most present evaluated libraries are based on the approach of the Los Alamos Model. To validate these models and to provide improved data for applications, a program is underway to measure the fission neutron spectrum for a wide range of incident neutron energies using the spallation source of fast neutrons at the Weapons Neutron Research (WNR) facility at the Los Alamos Neutron Science Center (LANSCE). In a double time-of-flight experiment, fission neutrons are detected by arrays of neutron detectors to increase the solid angle and also to investigate possible angular dependence of the fission neutrons. The challenge is to measure the spectrum from low energies, down to 100 keV or so, to energies over 10 MeV, where the evaporation-like spectrum decreases by 3 orders of magnitude from its peak around 1 MeV. For these measurements, we are developing two arrays of neutron detectors, one based on liquid organic scintillators and the other on 6Li-glass detectors. The range of fission neutrons detected by organic liquid scintillators extends from about 600 keV to well over 10 MeV, with the lower limit being defined by the limit of pulse-shape discrimination. The 6Li-glass detectors have a range from very low energies to about 1 MeV, where their efficiency then becomes small. Various considerations and tests are in progress to understand important contributing factors in designing these two arrays and they include selection and characterization of photomultiplier tubes (PM), the performance of relatively thin (1.8 cm) 6Li-glass scintillators on 12.5 cm diameter PM tubes, use of 17.5 cm diameter liquid scintillators with 12.5 cm PM tubes, measurements of detector efficiencies with tagged neutrons from the WNR/LANSCE neutron beam, and efficiency calibration with 252Cf spontaneous fission neutrons. Design considerations and test results are presented.

TH-CD-207B-06: Swank Factor of Segmented Scintillators in Multi-Slice CT Detectors: Pulse Height Spectra and Light Escape

DOE Office of Scientific and Technical Information (OSTI.GOV)

Howansky, A; Peng, B; Lubinsky, A

Purpose: Pulse height spectra (PHS) have been used to determine the Swank factor of a scintillator by measuring fluctuations in its light output per x-ray interaction. The Swank factor and x-ray quantum efficiency of a scintillator define the upper limit to its imaging performance, i.e. DQE(0). The Swank factor below the K-edge is dominated by optical properties, i.e. variations in light escape efficiency from different depths of interaction, denoted e(z). These variations can be optimized to improve tradeoffs in x-ray absorption, light yield, and spatial resolution. This work develops a quantitative model for interpreting measured PHS, and estimating e(z) onmore » an absolute scale. The method is used to investigate segmented ceramic GOS scintillators used in multi-slice CT detectors. Methods: PHS of a ceramic GOS plate (1 mm thickness) and segmented GOS array (1.4 mm thick) were measured at 46 keV. Signal and noise propagation through x-ray conversion gain, light escape, detection by a photomultiplier tube and dynode amplification were modeled using a cascade of stochastic gain stages. PHS were calculated with these expressions and compared to measurements. Light escape parameters were varied until modeled PHS agreed with measurements. The resulting estimates of e(z) were used to calculate PHS without measurement noise to determine the inherent Swank factor. Results: The variation in e(z) was 67.2–89.7% in the plate and 40.2–70.8% in the segmented sample, corresponding to conversion gains of 28.6–38.1 keV{sup −1} and 17.1–30.1 keV{sup −1}, respectively. The inherent Swank factors of the plate and segmented sample were 0.99 and 0.95, respectively. Conclusion: The high light escape efficiency in the ceramic GOS samples yields high Swank factors and DQE(0) in CT applications. The PHS model allows the intrinsic optical properties of scintillators to be deduced from PHS measurements, thus it provides new insights for evaluating the imaging performance of segmented ceramic GOS scintillators.« less

Intrinsic radioactivity of KSr2I5:Eu2+

NASA Astrophysics Data System (ADS)

Rust, M.; Melcher, C.; Lukosi, E.

2016-10-01

A current need in nuclear security is an economical, yet high energy resolution (near 2%), scintillation detector suitable for gamma-ray spectroscopy. For current scintillators on the market, there is an inverse relationship between scintillator energy resolution and cost of production. A new promising scintillator, KSr2I5:Eu2+, under development at the University of Tennessee, has achieved an energy resolution of 2.4% at 662 keV at room temperature, with potential growth rates exceeding several millimeters per hour. However, the internal background due to the 40K content could present a hurdle for effective source detection/identification in nuclear security applications. As a first step in addressing this question, this paper reports on a computational investigation of the intrinsic differential pulse height spectrum (DPHS) generated by 40K within the KSr2I5:Eu2+ scintillator as a function of crystal geometry. It was found that the DPHS remains relatively equal to a constant multiplicative factor of the negatron emission spectrum with a direct increase of the 1.46 MeV photopeak relative height to the negatron spectrum with volume. Further, peak pileup does not readily manifest itself for practical KSr2I5:Eu2+ volumes.

Precise rise and decay time measurements of inorganic scintillators by means of X-ray and 511 keV excitation

NASA Astrophysics Data System (ADS)

Gundacker, S.; Turtos, R. M.; Auffray, E.; Lecoq, P.

2018-05-01

The emergence of new solid-state avalanche photodetectors, e.g. SiPMs, with unprecedented timing capabilities opens new ways to profit from ultrafast and prompt photon emission in scintillators. In time of flight positron emission tomography (TOF-PET) and high energy timing detectors based on scintillators the ultimate coincidence time resolution (CTR) achievable is proportional to the square root of the scintillation rise time, decay time and the reciprocal light yield, CTR ∝√{τrτd / LY }. Hence, the precise study of light emission in the very first tens of picoseconds is indispensable to understand time resolution limitations imposed by the scintillator. We developed a time correlated single photon counting setup having a Gaussian impulse response function (IRF) of 63ps sigma, allowing to precisely measure the scintillation rise time of various materials with 511keV excitation. In L(Y)SO:Ce we found two rise time components, the first below the resolution of our setup <10 ps and a second component being ∼380 ps. Co-doping with Ca2+ completely suppresses the slow rise component leading to a very fast initial scintillation emission with a rise time of <10ps. A very similar behavior is observed in LGSO:Ce crystals. The results are further confirmed by complementary measurements using a streak-camera system with pulsed X-ray excitation and additional 511 keV excited measurements of Mg2+ co-doped LuAG:Ce, YAG:Ce and GAGG:Ce samples.

Ballistic Deficits for Ionization Chamber Pulses in Pulse Shaping Amplifiers

NASA Astrophysics Data System (ADS)

Kumar, G. Anil; Sharma, S. L.; Choudhury, R. K.

2007-04-01

In order to understand the dependence of the ballistic deficit on the shape of rising portion of the voltage pulse at the input of a pulse shaping amplifier, we have estimated the ballistic deficits for the pulses from a two-electrode parallel plate ionization chamber as well as for the pulses from a gridded parallel plate ionization chamber. These estimations have been made using numerical integration method when the pulses are processed through the CR-RCn (n=1-6) shaping network as well as when the pulses are processed through the complex shaping network of the ORTEC Model 472 spectroscopic amplifier. Further, we have made simulations to see the effect of ballistic deficit on the pulse-height spectra under different conditions. We have also carried out measurements of the ballistic deficits for the pulses from a two-electrode parallel plate ionization chamber as well as for the pulses from a gridded parallel plate ionization chamber when these pulses are processed through the ORTEC 572 linear amplifier having a simple CR-RC shaping network. The reasonable matching of the simulated ballistic deficits with the experimental ballistic deficits for the CR-RC shaping network clearly establishes the validity of the simulation technique

SU-E-T-451: Accuracy and Application of the Standard Imaging W1 Scintillator Dosimeter

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kowalski, M; McEwen, M

2014-06-01

Purpose: To evaluate the Standard Imaging W1 scintillator dosimeter in a range of clinical radiation beams to determine its range of possible applications. Methods: The W1 scintillator is a small perturbation-free dosimeter which is of interest in absolute and relative clinical dosimetry due to its small size and water equivalence. A single version of this detector was evaluated in Co-60 and linac photon and electron beams to investigate the following: linearity, sensitivity, precision, and dependence on electrometer type. In addition, depth-dose and cross-plane profiles were obtained in both photon and electron beams and compared with data obtained with wellbehaved ionizationmore » chambers. Results: In linac beams the precision and linearity was very impressive, with typical values of 0.3% and 0.1% respectively. Performance in a Co-60 beam was much poorer (approximately three times worse) and it is not clear whether this is due to the lower signal current or the effect of the continuous beam (rather than pulsed beam of the linac measurements). There was no significant difference in the detector reading when using either the recommended SI Supermax electrometer or two independent high-quality electrometers, except for low signal levels, where the Supermax exhibited an apparent threshold effect, preventing the measurement of the bremsstrahlung background in electron depth-dose curves. Comparisons with ion chamber measurements in linac beams were somewhat variable: good agreement was seen for cross-profiles (photon and electron beams) and electron beam depth-dose curves, generally within the 0.3% precision of the scintillator but systematic differences were observed as a function of measurement depth in photon beam depth-dose curves. Conclusion: A first look would suggest that the W1 scintillator has applications beyond small field dosimetry but performance appears to be limited to higher doserate and/or pulsed radiation beams. Further work is required to resolve discrepancies compared to ion chambers.« less

Optimizing coherent anti-Stokes Raman scattering by genetic algorithm controlled pulse shaping

NASA Astrophysics Data System (ADS)

Yang, Wenlong; Sokolov, Alexei

2010-10-01

The hybrid coherent anti-Stokes Raman scattering (CARS) has been successful applied to fast chemical sensitive detections. As the development of femto-second pulse shaping techniques, it is of great interest to find the optimum pulse shapes for CARS. The optimum pulse shapes should minimize the non-resonant four wave mixing (NRFWM) background and maximize the CARS signal. A genetic algorithm (GA) is developed to make a heuristic searching for optimized pulse shapes, which give the best signal the background ratio. The GA is shown to be able to rediscover the hybrid CARS scheme and find optimized pulse shapes for customized applications by itself.

Simulation of the neutron response matrix of an EJ309 liquid scintillator

NASA Astrophysics Data System (ADS)

Bai, Huaiyong; Wang, Zhimin; Zhang, Luyu; Jiang, Haoyu; Lu, Yi; Chen, Jinxiang; Zhang, Guohui

2018-04-01

The neutron response matrix is the basis for measuring the neutron energy spectrum through unfolding the pulse height spectrum detected with a liquid scintillator. Based on the light output of the EJ309 liquid scintillator and the related reaction cross sections, a Monte Carlo code is developed to obtain the neutron response matrix. The effects of the related reactions, the contributions of different number of neutron interactions and the wall effect of the recoil proton are discussed. With the obtained neutron response matrix and the GRAVEL iterative unfolding method, the neutron energy spectra of the 252Cf and the 241AmBe neutron sources are measured, and the results are respectively compared with the theoretical prediction of the 252Cf neutron energy spectrum and the previous results of the 241AmBe neutron energy spectra.

Nuclear Science Symposium, 21st, Scintillation and Semiconductor Counter Symposium, 14th, and Nuclear Power Systems Symposium, 6th, Washington, D.C., December 11-13, 1974, Proceedings

NASA Technical Reports Server (NTRS)

1975-01-01

Papers are presented dealing with latest advances in the design of scintillation counters, semiconductor radiation detectors, gas and position sensitive radiation detectors, and the application of these detectors in biomedicine, satellite instrumentation, and environmental and reactor instrumentation. Some of the topics covered include entopistic scintillators, neutron spectrometry by diamond detector for nuclear radiation, the spherical drift chamber for X-ray imaging applications, CdTe detectors in radioimmunoassay analysis, CAMAC and NIM systems in the space program, a closed loop threshold calibrator for pulse height discriminators, an oriented graphite X-ray diffraction telescope, design of a continuous digital-output environmental radon monitor, and the optimization of nanosecond fission ion chambers for reactor physics. Individual items are announced in this issue.

Improved neutron-gamma discrimination for a {sup 6}Li-glass neutron detector using digital signal analysis methods

DOE Office of Scientific and Technical Information (OSTI.GOV)

Wang, C. L., E-mail: wangc@ornl.gov; Riedel, R. A.

2016-01-15

A {sup 6}Li-glass scintillator (GS20) based neutron Anger camera was developed for time-of-flight single-crystal diffraction instruments at Spallation Neutron Source. Traditional Pulse-Height Analysis (PHA) for Neutron-Gamma Discrimination (NGD) resulted in the neutron-gamma efficiency ratio (defined as NGD ratio) on the order of 10{sup 4}. The NGD ratios of Anger cameras need to be improved for broader applications including neutron reflectometers. For this purpose, six digital signal analysis methods of individual waveforms acquired from photomultiplier tubes were proposed using (i) charge integration, (ii) pulse-amplitude histograms, (iii) power spectrum analysis combined with the maximum pulse-amplitude, (iv) two event parameters (a{sub 1}, b{submore » 0}) obtained from a Wiener filter, (v) an effective amplitude (m) obtained from an adaptive least-mean-square filter, and (vi) a cross-correlation coefficient between individual and reference waveforms. The NGD ratios are about 70 times those from the traditional PHA method. Our results indicate the NGD capabilities of neutron Anger cameras based on GS20 scintillators can be significantly improved with digital signal analysis methods.« less

Arbitrary temporal shape pulsed fiber laser based on SPGD algorithm

NASA Astrophysics Data System (ADS)

Jiang, Min; Su, Rongtao; Zhang, Pengfei; Zhou, Pu

2018-06-01

A novel adaptive pulse shaping method for a pulsed master oscillator power amplifier fiber laser to deliver an arbitrary pulse shape is demonstrated. Numerical simulation has been performed to validate the feasibility of the scheme and provide meaningful guidance for the design of the algorithm control parameters. In the proof-of-concept experiment, information on the temporal property of the laser is exchanged and evaluated through a local area network, and the laser adjusted the parameters of the seed laser according to the monitored output of the system automatically. Various pulse shapes, including a rectangular shape, ‘M’ shape, and elliptical shape are achieved through experimental iterations.

FPGA-Based Pulse Pile-Up Correction With Energy and Timing Recovery.

PubMed

Haselman, M D; Pasko, J; Hauck, S; Lewellen, T K; Miyaoka, R S

2012-10-01

Modern field programmable gate arrays (FPGAs) are capable of performing complex discrete signal processing algorithms with clock rates well above 100 MHz. This, combined with FPGA's low expense, ease of use, and selected dedicated hardware make them an ideal technology for a data acquisition system for a positron emission tomography (PET) scanner. The University of Washington is producing a high-resolution, small-animal PET scanner that utilizes FPGAs as the core of the front-end electronics. For this scanner, functions that are typically performed in dedicated circuits, or offline, are being migrated to the FPGA. This will not only simplify the electronics, but the features of modern FPGAs can be utilized to add significant signal processing power to produce higher quality images. In this paper we report on an all-digital pulse pile-up correction algorithm that has been developed for the FPGA. The pile-up mitigation algorithm will allow the scanner to run at higher count rates without incurring large data losses due to the overlapping of scintillation signals. This correction technique utilizes a reference pulse to extract timing and energy information for most pile-up events. Using pulses acquired from a Zecotech Photonics MAPD-N with an LFS-3 scintillator, we show that good timing and energy information can be achieved in the presence of pile-up utilizing a moderate amount of FPGA resources.

Achieving a Linear Dose Rate Response in Pulse-Mode Silicon Photodiode Scintillation Detectors Over a Wide Range of Excitations

NASA Astrophysics Data System (ADS)

Carroll, Lewis

2014-02-01

We are developing a new dose calibrator for nuclear pharmacies that can measure radioactivity in a vial or syringe without handling it directly or removing it from its transport shield “pig”. The calibrator's detector comprises twin opposing scintillating crystals coupled to Si photodiodes and current-amplifying trans-resistance amplifiers. Such a scheme is inherently linear with respect to dose rate over a wide range of radiation intensities, but accuracy at low activity levels may be impaired, beyond the effects of meager photon statistics, by baseline fluctuation and drift inevitably present in high-gain, current-mode photodiode amplifiers. The work described here is motivated by our desire to enhance accuracy at low excitations while maintaining linearity at high excitations. Thus, we are also evaluating a novel “pulse-mode” analog signal processing scheme that employs a linear threshold discriminator to virtually eliminate baseline fluctuation and drift. We will show the results of a side-by-side comparison of current-mode versus pulse-mode signal processing schemes, including perturbing factors affecting linearity and accuracy at very low and very high excitations. Bench testing over a wide range of excitations is done using a Poisson random pulse generator plus an LED light source to simulate excitations up to ˜106 detected counts per second without the need to handle and store large amounts of radioactive material.

Investigation of FPGA-Based Real-Time Adaptive Digital Pulse Shaping for High-Count-Rate Applications

NASA Astrophysics Data System (ADS)

Saxena, Shefali; Hawari, Ayman I.

2017-07-01

Digital signal processing techniques have been widely used in radiation spectrometry to provide improved stability and performance with compact physical size over the traditional analog signal processing. In this paper, field-programmable gate array (FPGA)-based adaptive digital pulse shaping techniques are investigated for real-time signal processing. National Instruments (NI) NI 5761 14-bit, 250-MS/s adaptor module is used for digitizing high-purity germanium (HPGe) detector's preamplifier pulses. Digital pulse processing algorithms are implemented on the NI PXIe-7975R reconfigurable FPGA (Kintex-7) using the LabVIEW FPGA module. Based on the time separation between successive input pulses, the adaptive shaping algorithm selects the optimum shaping parameters (rise time and flattop time of trapezoid-shaping filter) for each incoming signal. A digital Sallen-Key low-pass filter is implemented to enhance signal-to-noise ratio and reduce baseline drifting in trapezoid shaping. A recursive trapezoid-shaping filter algorithm is employed for pole-zero compensation of exponentially decayed (with two-decay constants) preamplifier pulses of an HPGe detector. It allows extraction of pulse height information at the beginning of each pulse, thereby reducing the pulse pileup and increasing throughput. The algorithms for RC-CR2 timing filter, baseline restoration, pile-up rejection, and pulse height determination are digitally implemented for radiation spectroscopy. Traditionally, at high-count-rate conditions, a shorter shaping time is preferred to achieve high throughput, which deteriorates energy resolution. In this paper, experimental results are presented for varying count-rate and pulse shaping conditions. Using adaptive shaping, increased throughput is accepted while preserving the energy resolution observed using the longer shaping times.

Position and time resolution measurements with a microchannel plate image intensifier: A comparison of monolithic and pixelated CeBr3 scintillators

NASA Astrophysics Data System (ADS)

Ackermann, Ulrich; Eschbaumer, Stephan; Bergmaier, Andreas; Egger, Werner; Sperr, Peter; Greubel, Christoph; Löwe, Benjamin; Schotanus, Paul; Dollinger, Günther

2016-07-01

To perform Four Dimensional Age Momentum Correlation measurements in the near future, where one obtains the positron lifetime in coincidence with the three dimensional momentum of the electron annihilating with the positron, we have investigated the time and position resolution of two CeBr3 scintillators (monolithic and an array of pixels) using a Photek IPD340/Q/BI/RS microchannel plate image intensifier. The microchannel plate image intensifier has an active diameter of 40 mm and a stack of two microchannel plates in chevron configuration. The monolithic CeBr3 scintillator was cylindrically shaped with a diameter of 40 mm and a height of 5 mm. The pixelated scintillator array covered the whole active area of the microchannel plate image intensifier and the shape of each pixel was 2.5·2.5·8 mm3 with a pixel pitch of 3.3 mm. For the monolithic setup the measured mean single time resolution was 330 ps (FWHM) at a gamma energy of 511 keV. No significant dependence on the position was detected. The position resolution at the center of the monolithic scintillator was about 2.5 mm (FWHM) at a gamma energy of 662 keV. The single time resolution of the pixelated crystal setup reached 320 ps (FWHM) in the region of the center of the active area of the microchannel plate image intensifier. The position resolution was limited by the cross-section of the pixels. The gamma energy for the pixel setup measurements was 511 keV.

Applying the new gamma ray imager diagnostic to measurements of runaway electron Bremsstrahlung radiation in the DIII-D Tokamak (invited)

DOE Office of Scientific and Technical Information (OSTI.GOV)

Cooper, C. M., E-mail: coopercm@fusion.gat.com; Pace, D. C.; Paz-Soldan, C.

2016-11-15

A new gamma ray imager (GRI) is developed to probe the electron distribution function with 2D spatial resolution during runaway electron (RE) experiments at the DIII-D tokamak. The diagnostic is sensitive to 0.5–100 MeV gamma rays, allowing characterization of the RE distribution function evolution during RE growth and dissipation. The GRI consists of a lead “pinhole camera” mounted on the DIII-D midplane with 123 honeycombed tangential chords 20 cm wide that span the vessel interior. Up to 30 bismuth germanate (BGO) scintillation detectors capture RE bremsstrahlung radiation for Pulse Height Analysis (PHA) capable of discriminating up to 20 000 pulses permore » second. Digital signal processing routines combining shaping filters are performed during PHA to reject noise and record gamma ray energy. The GRI setup and PHA algorithms will be described and initial data from experiments will be presented. A synthetic diagnostic is developed to generate the gamma ray spectrum of a GRI channel given the plasma information and a prescribed distribution function. Magnetic reconstructions of the plasma are used to calculate the angle between every GRI sightline and orient and discriminate gamma rays emitted by a field-aligned RE distribution function.« less

Adaptive optics to enhance target recognition

NASA Astrophysics Data System (ADS)

McAulay, Alastair D.

2012-06-01

Target recognition can be enhanced by reducing image degradation due to atmospheric turbulence. This is accomplished by an adaptive optic system. We discuss the forms of degradation when a target is viewed through the atmosphere1: scintillation from ground targets on a hot day in visible or infrared light; beam spreading and wavering around in time; atmospheric turbulence caused by motion of the target or by weather. In the case of targets we can use a beacon laser that reflects back from the target into a wavefront detector to measure the effects of turbulence on propagation to and from the target before imaging.1 A deformable mirror then corrects the wavefront shape of the transmitted, reflected or scattered data for enhanced imaging. Further, recognition of targets is enhanced by performing accurate distance measurements to localized parts of the target using lidar. Distance is obtained by sending a short pulse to the target and measuring the time for the pulse to return. There is inadequate time to scan the complete field of view so that the beam must be steered to regions of interest such as extremities of the image during image recognition. Distance is particularly valuable to recognize fine features in range along the target or when segmentation is required to separate a target from background or from other targets. We discuss the issues involved.

Applying the new gamma ray imager diagnostic to measurements of runaway electron Bremsstrahlung radiation in the DIII-D Tokamak (invited)

NASA Astrophysics Data System (ADS)

Cooper, C. M.; Pace, D. C.; Paz-Soldan, C.; Commaux, N.; Eidietis, N. W.; Hollmann, E. M.; Shiraki, D.

2016-11-01

A new gamma ray imager (GRI) is developed to probe the electron distribution function with 2D spatial resolution during runaway electron (RE) experiments at the DIII-D tokamak. The diagnostic is sensitive to 0.5-100 MeV gamma rays, allowing characterization of the RE distribution function evolution during RE growth and dissipation. The GRI consists of a lead "pinhole camera" mounted on the DIII-D midplane with 123 honeycombed tangential chords 20 cm wide that span the vessel interior. Up to 30 bismuth germanate (BGO) scintillation detectors capture RE bremsstrahlung radiation for Pulse Height Analysis (PHA) capable of discriminating up to 20 000 pulses per second. Digital signal processing routines combining shaping filters are performed during PHA to reject noise and record gamma ray energy. The GRI setup and PHA algorithms will be described and initial data from experiments will be presented. A synthetic diagnostic is developed to generate the gamma ray spectrum of a GRI channel given the plasma information and a prescribed distribution function. Magnetic reconstructions of the plasma are used to calculate the angle between every GRI sightline and orient and discriminate gamma rays emitted by a field-aligned RE distribution function.

Applying the new gamma ray imager diagnostic to measurements of runaway electron Bremsstrahlung radiation in the DIII-D Tokamak (invited).

PubMed

Cooper, C M; Pace, D C; Paz-Soldan, C; Commaux, N; Eidietis, N W; Hollmann, E M; Shiraki, D

2016-11-01

A new gamma ray imager (GRI) is developed to probe the electron distribution function with 2D spatial resolution during runaway electron (RE) experiments at the DIII-D tokamak. The diagnostic is sensitive to 0.5-100 MeV gamma rays, allowing characterization of the RE distribution function evolution during RE growth and dissipation. The GRI consists of a lead "pinhole camera" mounted on the DIII-D midplane with 123 honeycombed tangential chords 20 cm wide that span the vessel interior. Up to 30 bismuth germanate (BGO) scintillation detectors capture RE bremsstrahlung radiation for Pulse Height Analysis (PHA) capable of discriminating up to 20 000 pulses per second. Digital signal processing routines combining shaping filters are performed during PHA to reject noise and record gamma ray energy. The GRI setup and PHA algorithms will be described and initial data from experiments will be presented. A synthetic diagnostic is developed to generate the gamma ray spectrum of a GRI channel given the plasma information and a prescribed distribution function. Magnetic reconstructions of the plasma are used to calculate the angle between every GRI sightline and orient and discriminate gamma rays emitted by a field-aligned RE distribution function.

Applying the new gamma ray imager diagnostic to measurements of runaway electron Bremsstrahlung radiation in the DIII-D Tokamak (invited)

DOE PAGES

Cooper, C. M.; Pace, D. C.; Paz-Soldan, C.; ...

2016-08-30

A new gamma ray imager (GRI) is developed to probe the electron distribution function with 2D spatial resolution during runaway electron (RE) experiments at the DIII-D tokamak. The diagnostic is sensitive to 0.5-100 MeV gamma rays, allowing characterization of the RE distribution function evolution during RE growth and dissipation. The GRI consists of a lead "pinhole camera" mounted on the DIII-D midplane with 123 honeycombed tangential chords 20 cm wide that span the vessel interior. Up to 30 bismuth germanate (BGO) scintillation detectors capture RE bremsstrahlung radiation for Pulse Height Analysis (PHA) capable of discriminating up to 20,000 pulses permore » second. Digital signal processing routines combining shaping filters are performed during PHA to reject noise and record gamma ray energy. The GRI setup and PHA algorithms will be described and initial data from experiments will be presented. A synthetic diagnostic is developed to generate the gamma ray spectrum of a GRI channel given the plasma information and a prescribed distribution function. Furthermore, magnetic reconstructions of the plasma are used to calculate the angle between every GRI sightline and orient and discriminate gamma rays emitted by a field-aligned RE distribution function.« less

Insulating epoxy/barite and polyester/barite composites for radiation attenuation.

PubMed

El-Sarraf, M A; El-Sayed Abdo, A

2013-09-01

A trial has been made to create insulating Epoxy/Barite (EP/Brt) (ρ=2.85 g cm(-3)) and Crosslinked Unsaturated Polyester/Barite (CUP/Brt) (ρ=3.25 g cm(-3)) composites with radiation attenuation and shielding capabilities. Experimental work regarding mechanical and physical properties was performed to study the composites integrity for practical applications. The properties were found to be reasonable. Radiation attenuation properties have been carried out using emitted collimated beam from a fission (252)Cf (100 µg) neutron source, and the neutron-gamma spectrometer with stilbene scintillator. The pulse shape discriminating (P.S.D) technique based on the zero cross-over method was used to discriminate between neutron and gamma-ray pulses. Thermal neutron fluxes, measured using the BF3 detector and thermal neutron detection system, were used to plot the attenuation relations. The fast neutron macroscopic effective removal cross-section ΣR, gamma ray total attenuation coefficient µ and thermal neutron macroscopic cross-section Σ have been evaluated. Theoretical calculations have been achieved using MCNP-4C2 code to calculate ΣR, µ and Σ. Also, MERCSF-N program was used to calculate macroscopic effective removal cross-section ΣR. Measured and calculated results have been compared and were found to be in reasonable agreement. Copyright © 2013 Elsevier Ltd. All rights reserved.

The Salinas Airshower Learning And Discovery Project (SALAD)

NASA Astrophysics Data System (ADS)

Hernandez, Victor; Niduaza, Rommel; Ruiz Castruita, Daniel; Knox, Adrian; Ramos, Daniel; Fan, Sewan; Fatuzzo, Laura

2015-04-01

The SALAD project partners community college and high school STEM students in order to develop and investigate cosmic ray detector telescopes and the physical concepts, using a new light sensor technology based on silicon photomultiplier (SiPM) detectors. Replacing the conventional photomultiplier with the SiPM, offers notable advantages in cost and facilitates more in depth, hands-on learning laboratory activities. The students in the SALAD project design, construct and extensively evaluate the SiPM detector modules. These SiPM modules, can be completed in a short time utilizing cost effective components. We describe our research to implement SiPM as read out light detectors for plastic scintillators in a cosmic ray detector telescope for use in high schools. In particular, we describe our work in the design, evaluation and the assembly of (1) a fast preamplifier, (2) a simple coincidence circuit using fast comparators, to discriminate the SiPM noise signal pulses, and (3) a monovibrator circuit to shape the singles plus the AND logic pulses for subsequent processing. To store the singles and coincidence counts data, an Arduino micro-controller with program sketches can be implemented. Results and findings from our work would be described and presented. US Department of Education Title V Grant Award PO31S090007

James Clerk Maxwell Prize Address: High Intensity Laser Propagation and Interactions

NASA Astrophysics Data System (ADS)

Sprangle, Phillip

2013-10-01

High intensity laser radiation sources cover a wide range of parameters, e.g., peak powers from tera to peta watts, pulse lengths from pico to femto seconds, repetition rates ranging from kilo to mega hertz and average powers of many tens of watts. This talk will cover, among other things, some of the unique physical processes which result when high intensity laser radiation interacts with gases and plasmas. One of the interesting topics to be discussed is the propagation of these laser pulses in a turbulent atmosphere which results in a multitude of coupled linear and nonlinear processes including filamentation and scintillation. Phase conjugation techniques to reduce the effects of atmospheric turbulence (scintillation) will be described. This talk will also discuss a range of potential applications of these high intensity lasers, including: electron acceleration in spatially periodic and tapered plasma channels, detection of radioactive material using electromagnetic signatures, atmospheric lasing of N2 molecules, as well as incoherent and coherent x-ray generation mechanisms. Research supported by NRL, ONR and UMD.

aCORN Beta Spectrometer and Electrostatic Mirror

NASA Astrophysics Data System (ADS)

Hassan, Md; aCORN Collaboration

2013-10-01

aCORN uses a high efficiency backscatter suppressed beta spectrometer to measure the electron-antineutrino correlation in neutron beta decay. We measure the correlation by counting protons and beta electrons in coincidence with precisely determined electron energy. There are 19 photomultiplier tubes arranged in a hexagonal array coupled to a single phosphor doped polystyrene scintillator. The magnetic field is shaped so that electrons that backscatter without depositing their full energy strike a tulip-shaped array of scintillator paddles and these events are vetoed. The detailed construction, performance and calibration of this beta spectrometer will be presented. I will also present the simulation, construction, and features of our novel electrostatic mirror. This work was supported by the National Science Foundation and the NIST Center for Neutron Research.

Above-ground antineutrino detection for nuclear reactor monitoring

NASA Astrophysics Data System (ADS)

Sweany, M.; Brennan, J.; Cabrera-Palmer, B.; Kiff, S.; Reyna, D.; Throckmorton, D.

2015-01-01

Antineutrino monitoring of nuclear reactors has been demonstrated many times (Klimov et al., 1994 [1]; Bowden et al., 2009 [2]; Oguri et al., 2014 [3]), however the technique has not as of yet been developed into a useful capability for treaty verification purposes. The most notable drawback is the current requirement that detectors be deployed underground, with at least several meters-water-equivalent of shielding from cosmic radiation. In addition, the deployment of liquid-based detection media presents a challenge in reactor facilities. We are currently developing a detector system that has the potential to operate above ground and circumvent deployment problems associated with a liquid detection media: the system is composed of segments of plastic scintillator surrounded by 6LiF/ZnS:Ag. ZnS:Ag is a radio-luminescent phosphor used to detect the neutron capture products of 6Li. Because of its long decay time compared to standard plastic scintillators, pulse-shape discrimination can be used to distinguish positron and neutron interactions resulting from the inverse beta decay (IBD) of antineutrinos within the detector volume, reducing both accidental and correlated backgrounds. Segmentation further reduces backgrounds by identifying the positron's annihilation gammas, a signature that is absent for most correlated and uncorrelated backgrounds. This work explores different configurations in order to maximize the size of the detector segments without reducing the intrinsic neutron detection efficiency. We believe that this technology will ultimately be applicable to potential safeguards scenarios such as those recently described by Huber et al. (2014) [4,5].

Effects of Ga substitution in Ce:Tb3Ga x Al5- x O12 single crystals for scintillator applications

NASA Astrophysics Data System (ADS)

Nakauchi, Daisuke; Okada, Go; Kawano, Naoki; Kawaguchi, Noriaki; Yanagida, Takayuki

2018-02-01

Bulk single crystals of Ce-doped Tb3Ga x Al5- x O12 (x = 0-4) were successfully synthesized by the floating zone method. The samples exhibit photoluminescence and scintillation with an intense broad emission due to the 5d-4f transitions of Ce3+ peaking around 550 nm as well as a few sharp peaks due to the 4f-4f transitions of Tb3+. Pulse height spectrum measurements under 137Cs γ-ray irradiation demonstrated a clear photoabsorption peak, in which the scintillation light yields were estimated to be 57,000 (x = 0), 28,000 (x = 1), 19,000 (x = 2), and 10,000 (x = 3) photons/MeV. Afterglow level can be suppressed with an appropriate addition of Ga, in which the optimum concertation is x = 2 leading an afterglow level of 23 ppm.

Mg,Ce co-doped Lu2Gd1(Ga,Al)5O12 by micro-pulling down method and their luminescence properties

NASA Astrophysics Data System (ADS)

Kamada, Kei; Yamaguchi, Hiroaki; Yoshino, Masao; Kurosawa, Shunsuke; Shoji, Yasuhiro; Yokota, Yuui; Ohashi, Yuji; Pejchal, Jan; Nikl, Martin; Yoshikawa, Akira

2018-04-01

The effects of Mg co-doping on the scintillation properties of Ce:Lu2Gd1(Ga,Al)5O12 (LGGAG) single crystals with different Ga/Al ratios were investigated. Mg co-doped and non co-doped Ce:LGGAG single crystals were grown by the micro-pulling down (µ-PD) method and then cut, polished and annealed for each measurement. Absorption spectra, radioluminescence (RL) spectra, pulse height spectra, and scintillation decay were measured to reveal the effect of Mg co-doping. Ce4+ charge transfer (CT) absorption band peaking at ∼260 nm was observed in Mg co-doped samples, which is in good agreement with previous reports for the Ce4+ CT absorption band in other garnet-based crystals. The scintillation decay time tended to be accelerated and the light yield tended to be decreased by Mg co-doping at higher Ga concentrations.

Characteristic evaluation of a Lithium-6 loaded neutron coincidence spectrometer.

PubMed

Hayashi, M; Kaku, D; Watanabe, Y; Sagara, K

2007-01-01

Characteristics of a (6)Li-loaded neutron coincidence spectrometer were investigated from both measurements and Monte Carlo simulations. The spectrometer consists of three (6)Li-glass scintillators embedded in a liquid organic scintillator BC-501A, which can detect selectively neutrons that deposit the total energy in the BC-501A using a coincidence signal generated from the capture event of thermalised neutrons in the (6)Li-glass scintillators. The relative efficiency and the energy response were measured using 4.7, 7.2 and 9.0 MeV monoenergetic neutrons. The measured ones were compared with the Monte Carlo calculations performed by combining the neutron transport code PHITS and the scintillator response calculation code SCINFUL. The experimental light output spectra were in good agreement with the calculated ones in shape. The energy dependence of the detection efficiency was reproduced by the calculation. The response matrices for 1-10 MeV neutrons were finally obtained.

Effect of annealing temperature on the photoluminescence and scintillation properties of ZnO nanorods

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kurudirek, Sinem V.; Menkara, H.; Klein, Benjamin D. B.

2018-01-01

The effect of the annealing to enhance the photoluminescence (PL) and scintillation properties, as determined by pulse height distribution of alpha particle irradiation, has been investigated for solution grown ZnO nanorods For this investigation the ZnO nanorod arrays were grown on glass for 22 h at 95 ◦ C as a substrate using a solution based hydrothermal technique. The samples were first annealed for different times (30, 60, 90 and 120 min) at 300 ◦ C and then at different temperatures (100 ◦ C–600 ◦ C) in order to determine the optimum annealing time and temperature, respectively. Before annealing, themore » ZnO nanorod arrays showed a broad yellow–orange visible and near-band gap UV emission peaks. After annealing in a forming gas atmosphere, the intensity of the sub-band gap PL was significantly reduced and the near-band gap PL emission intensity correspondingly increased (especially at temperatures higher than 100 ◦ C). Based on the ratio of the peak intensity ratio before and after annealing, it was concluded that samples at 350 ◦ C for 90 min resulted in the best near-band gap PL emission. Similarly, the analysis of the pulse height spectrum resulting from alpha particles revealed that ZnO nanorod arrays similarly annealed at 350 ◦ C for 90 min exhibited the highest scintillation response.« less

[INVITED] Control of femtosecond pulsed laser ablation and deposition by temporal pulse shaping

NASA Astrophysics Data System (ADS)

Garrelie, Florence; Bourquard, Florent; Loir, Anne--Sophie; Donnet, Christophe; Colombier, Jean-Philippe

2016-04-01

This study explores the effects of temporal laser pulse shaping on femtosecond pulsed laser deposition (PLD). The potential of laser pulses temporally tailored on ultrafast time scales is used to control the expansion and the excitation degree of ablation products including atomic species and nanoparticles. The ablation plume generated by temporally shaped femtosecond pulsed laser ablation of aluminum and graphite targets is studied by in situ optical diagnostic methods. Taking advantage of automated pulse shaping techniques, an adaptive procedure based on spectroscopic feedback regulates the irradiance for the enhancement of typical plasma features. Thin films elaborated by unshaped femtosecond laser pulses and by optimized sequence indicate that the nanoparticles generation efficiency is strongly influenced by the temporal shaping of the laser irradiation. The ablation processes leading either to the generation of the nanoparticles either to the formation of plasma can be favored by using a temporal shaping of the laser pulse. Insights are given on the possibility to control the quantity of the nanoparticles. The temporal laser pulse shaping is shown also to strongly modify the laser-induced plasma contents and kinetics for graphite ablation. Temporal pulse shaping proves its capability to reduce the number of slow radicals while increasing the proportion of monomers, with the addition of ionized species in front of the plume. This modification of the composition and kinetics of plumes in graphite ablation using temporal laser pulse shaping is discussed in terms of modification of the structural properties of deposited Diamond-Like Carbon films (DLC). This gives rise to a better understanding of the growth processes involved in femtosecond-PLD and picosecond-PLD of DLC suggesting the importance of neutral C atoms, which are responsible for the subplantation process.

DOI Determination by Rise Time Discrimination in Single-Ended Readout for TOF PET Imaging

PubMed Central

Wiener, R.I.; Surti, S.; Karp, J.S.

2013-01-01

Clinical TOF PET systems achieve detection efficiency using thick crystals, typically of thickness 2–3cm. The resulting dispersion in interaction depths degrades spatial resolution for increasing radial positions due to parallax error. Furthermore, interaction depth dispersion results in time pickoff dispersion and thus in degraded timing resolution, and is therefore of added concern in TOF scanners. Using fast signal digitization, we characterize the timing performance, pulse shape and light output of LaBr3:Ce, CeBr3 and LYSO. Coincidence timing resolution is shown to degrade by ~50ps/cm for scintillator pixels of constant cross section and increasing length. By controlling irradiation depth in a scintillator pixel, we show that DOI-dependence of time pickoff is a significant factor in the loss of timing performance in thick detectors. Using the correlated DOI-dependence of time pickoff and charge collection, we apply a charge-based correction to the time pickoff, obtaining improved coincidence timing resolution of <200ps for a uniform 4×4×30mm3 LaBr3 pixel. In order to obtain both DOI identification and improved timing resolution, we design a two layer LaBr3[5%Ce]/LaBr3[30%Ce] detector of total size 4×4×30mm3, exploiting the dependence of scintillator rise time on [Ce] in LaBr3:Ce. Using signal rise time to determine interaction layer, excellent interaction layer discrimination is achieved, while maintaining coincidence timing resolution of <250ps and energy resolution <7% using a R4998 PMT. Excellent layer separation and timing performance is measured with several other commercially-available TOF photodetectors, demonstrating the practicality of this design. These results indicate the feasibility of rise time discrimination as a technique for measuring event DOI while maintaining sensitivity, timing and energy performance, in a well-known detector architecture. PMID:24403611

DOI Determination by Rise Time Discrimination in Single-Ended Readout for TOF PET Imaging.

PubMed

Wiener, R I; Surti, S; Karp, J S

2013-06-01

Clinical TOF PET systems achieve detection efficiency using thick crystals, typically of thickness 2-3cm. The resulting dispersion in interaction depths degrades spatial resolution for increasing radial positions due to parallax error. Furthermore, interaction depth dispersion results in time pickoff dispersion and thus in degraded timing resolution, and is therefore of added concern in TOF scanners. Using fast signal digitization, we characterize the timing performance, pulse shape and light output of LaBr 3 :Ce, CeBr 3 and LYSO. Coincidence timing resolution is shown to degrade by ~50ps/cm for scintillator pixels of constant cross section and increasing length. By controlling irradiation depth in a scintillator pixel, we show that DOI-dependence of time pickoff is a significant factor in the loss of timing performance in thick detectors. Using the correlated DOI-dependence of time pickoff and charge collection, we apply a charge-based correction to the time pickoff, obtaining improved coincidence timing resolution of <200ps for a uniform 4×4×30mm 3 LaBr 3 pixel. In order to obtain both DOI identification and improved timing resolution, we design a two layer LaBr 3 [5%Ce]/LaBr 3 [30%Ce] detector of total size 4×4×30mm 3 , exploiting the dependence of scintillator rise time on [Ce] in LaBr 3 :Ce. Using signal rise time to determine interaction layer, excellent interaction layer discrimination is achieved, while maintaining coincidence timing resolution of <250ps and energy resolution <7% using a R4998 PMT. Excellent layer separation and timing performance is measured with several other commercially-available TOF photodetectors, demonstrating the practicality of this design. These results indicate the feasibility of rise time discrimination as a technique for measuring event DOI while maintaining sensitivity, timing and energy performance, in a well-known detector architecture.

System for generating shaped optical pulses and measuring optical pulses using spectral beam deflection (SBD)

DOEpatents

Skupsky, Stanley; Kessler, Terrance J.; Letzring, Samuel A.

1993-01-01

A temporally shaped or modified optical output pulse is generated from a bandwidth-encoded optical input pulse in a system in which the input pulse is in the form of a beam which is spectrally spread into components contained within the bandwidth, followed by deflection of the spectrally spread beam (SBD) thereby spatially mapping the components in correspondence with the temporal input pulse profile in the focal plane of a lens, and by spatially selective attenuation of selected components in that focal plane. The shaped or modified optical output pulse is then reconstructed from the attenuated spectral components. The pulse-shaping system is particularly useful for generating optical pulses of selected temporal shape over a wide range of pulse duration, such pulses finding application in the fields of optical communication, optical recording and data storage, atomic and molecular spectroscopy and laser fusion. An optical streak camera is also provided which uses SBD to display the beam intensity in the focal plane as a function of time during the input pulse.

System for generating shaped optical pulses and measuring optical pulses using spectral beam deflection (SBD)

DOEpatents

Skupsky, S.; Kessler, T.J.; Letzring, S.A.

1993-11-16

A temporally shaped or modified optical output pulse is generated from a bandwidth-encoded optical input pulse in a system in which the input pulse is in the form of a beam which is spectrally spread into components contained within the bandwidth, followed by deflection of the spectrally spread beam (SBD) thereby spatially mapping the components in correspondence with the temporal input pulse profile in the focal plane of a lens, and by spatially selective attenuation of selected components in that focal plane. The shaped or modified optical output pulse is then reconstructed from the attenuated spectral components. The pulse-shaping system is particularly useful for generating optical pulses of selected temporal shape over a wide range of pulse duration, such pulses finding application in the fields of optical communication, optical recording and data storage, atomic and molecular spectroscopy and laser fusion. An optical streak camera is also provided which uses SBD to display the beam intensity in the focal plane as a function of time during the input pulse. 10 figures.

BC404 scintillators as gamma locators studied via Geant4 simulations

NASA Astrophysics Data System (ADS)

Cortés, M. L.; Hoischen, R.; Eisenhauer, K.; Gerl, J.; Pietralla, N.

2014-05-01

In many applications in industry and academia, an accurate determination of the direction from where gamma rays are emitted is either needed or desirable. Ion-beam therapy treatments, the search for orphan sources, and homeland security applications are examples of fields that can benefit from directional sensitivity to gamma-radiation. Scintillation detectors are a good option for these types of applications as they have relatively low cost, are easy to handle and can be produced in a large range of different sizes. In this work a Geant4 simulation was developed to study the directional sensitivity of different BC404 scintillator geometries and arrangements. The simulation includes all the physical processes relevant for gamma detection in a scintillator. In particular, the creation and propagation of optical photons inside the scintillator was included. A simplified photomultiplier tube model was also simulated. The physical principle exploited is the angular dependence of the shape of the energy spectrum obtained from thin scintillator layers when irradiated from different angles. After an experimental confirmation of the working principle of the device and a check of the simulation, the possibilities and limitations of directional sensitivity to gamma radiation using scintillator layers was tested. For this purpose, point-like sources of typical energies expected in ion-beam therapy were used. Optimal scintillator thicknesses for different energies were determined and the setup efficiencies calculated. The use of arrays of scintillators to reconstruct the direction of incoming gamma rays was also studied. For this case, a spherical source emitting Bremsstrahlung radiation was used together with a setup consisting of scintillator layers. The capability of this setup to identify the center of the extended source was studied together with its angular resolution.

A pulse-shape discrimination method for improving Gamma-ray spectrometry based on a new digital shaping filter

NASA Astrophysics Data System (ADS)

Qin, Zhang-jian; Chen, Chuan; Luo, Jun-song; Xie, Xing-hong; Ge, Liang-quan; Wu, Qi-fan

2018-04-01

It is a usual practice for improving spectrum quality by the mean of designing a good shaping filter to improve signal-noise ratio in development of nuclear spectroscopy. Another method is proposed in the paper based on discriminating pulse-shape and discarding the bad pulse whose shape is distorted as a result of abnormal noise, unusual ballistic deficit or bad pulse pile-up. An Exponentially Decaying Pulse (EDP) generated in nuclear particle detectors can be transformed into a Mexican Hat Wavelet Pulse (MHWP) and the derivation process of the transform is given. After the transform is performed, the baseline drift is removed in the new MHWP. Moreover, the MHWP-shape can be discriminated with the three parameters: the time difference between the two minima of the MHWP, and the two ratios which are from the amplitude of the two minima respectively divided by the amplitude of the maximum in the MHWP. A new type of nuclear spectroscopy was implemented based on the new digital shaping filter and the Gamma-ray spectra were acquired with a variety of pulse-shape discrimination levels. It had manifested that the energy resolution and the peak-Compton ratio were both improved after the pulse-shape discrimination method was used.

Bright Eu2+-activated polycrystalline ceramic neutron scintillators

NASA Astrophysics Data System (ADS)

Wang, C. L.; Paranthaman, M. P.; Riedel, R. A.; Hodges, J. P.; Karlic, J. J.; Veatch, R. A.; Li, L.; Bridges, C. A.

2018-03-01

Scintillation properties of Eu2+-doped CaF2-AlF3-6LiF (Eu:CALF) polycrystalline ceramic thermal-neutron scintillators as a function of AlF3 concentration have been studied. The emission band peaked at a wavelength of 425-431 nm is due to the presence of Eu:CaF2 micro-crystallites. The highest light output from these samples is approximately 20,000 photons per thermal neutron, which is 3 times that of a GS20 6Li-glass scintillator. The pulse-decay lifetime and light output vs. AlF3 concentration may be understood using a radiation trapping model and the formation of a Li3AlF6 phase. At lower AlF3 concentration, Al3+ ions in Eu:CaF2 passivate the hole-trapping defects and enhance the light output; whereas at higher AlF3 concentration, Al3+ ions lead to the formation of electron trapping centers in Eu:CaF2 and the Li3AlF6 phase is formed, which reduces the light output. A neutron-gamma-discrimination (NGD) ratio of 9 × 108 was obtained from Principal Component Analysis (PCA) of digital waveforms, while Fisher Linear Discriminant Analysis (FLDA) can completely separate the thermal neutrons from 60Co gamma rays within the limit of gamma event statistics used in this work. Our results suggest that Eu:CALF scintillators can potentially replace the GS20 scintillator used for thermal and cold neutron detection systems.

Note: Neutron bang time diagnostic system on Shenguang-III prototype

DOE Office of Scientific and Technical Information (OSTI.GOV)

Tang, Qi; Chen, Jiabin; Liu, Zhongjie

A neutron bang time (NBT) diagnostic system has been implemented on Shenguang-III prototype. The bang time diagnostic system is based on a sensitive fusion neutron detector, which consists of a plastic scintillator and a micro-channel plate photomultiplier tube (PMT). An optical fiber bundle is used to couple the scintillator and the PMT. The bang time system is able to measure bang time above a neutron yield of 10{sup 7}. Bang times and start time of laser were related by probing x-ray pulses produced by 200 ps laser irradiating golden targets. Timing accuracy of the NBT is better than 60 ps.

Application of nonlinear pulse shaping of femtosecond pulse generation in a fiber amplifier at 500 MHz repetition rate

NASA Astrophysics Data System (ADS)

Liu, Yang; Luo, Daping; Wang, Chao; Zhu, Zhiwei; Li, Wenxue

2018-03-01

We numerically and experimentally demonstrate that a nonlinear pulse shaping technique based on pre-chirping management in a short gain fiber can be exploited to improve the quality of a compressed pulse. With prior tuning of the pulse chirp, the amplified pulse express different nonlinear propagating processes. A spectrum with s flat top and more smooth wings, showing a similariton feature, generates with the optimal initial pulse chirp, and the shortest pulses with minimal pulse pedestals are obtained. Experimental results show the ability of nonlinear pulse shaping to enhance the quality of compressed pulses, as theoretically expected.

Pulsed x-ray imaging of high-density objects using a ten picosecond high-intensity laser driver

NASA Astrophysics Data System (ADS)

Rusby, D. R.; Brenner, C. M.; Armstrong, C.; Wilson, L. A.; Clarke, R.; Alejo, A.; Ahmed, H.; Butler, N. M. H.; Haddock, D.; Higginson, A.; McClymont, A.; Mirfayzi, S. R.; Murphy, C.; Notley, M.; Oliver, P.; Allott, R.; Hernandez-Gomez, C.; Kar, S.; McKenna, P.; Neely, D.

2016-10-01

Point-like sources of X-rays that are pulsed (sub nanosecond), high energy (up to several MeV) and bright are very promising for industrial and security applications where imaging through large and dense objects is required. Highly penetrating X-rays can be produced by electrons that have been accelerated by a high intensity laser pulse incident onto a thin solid target. We have used a pulse length of 10ps to accelerate electrons to create a bright x-ray source. The bremsstrahlung temperature was measured for a laser intensity from 8.5-12×1018 W/cm2. These x-rays have sequentially been used to image high density materials using image plate and a pixelated scintillator system.

First measurement of surface nuclear recoil background for argon dark matter searches

DOE PAGES

Xu, Jingke; Stanford, Chris; Westerdale, Shawn; ...

2017-09-19

Here, one major background in direct searches for weakly interacting massive particles (WIMPs) comes from the deposition of radon progeny on detector surfaces. A dangerous surface background is the 206Pb nuclear recoils produced by 210Po decays. In this paper, we report the first characterization of this background in liquid argon. The scintillation signal of low energy Pb recoils is measured to be highly quenched in argon, and we estimate that the 103 keV 206Pb recoil background will produce a signal equal to that of a ~5 keV (30 keV) electron recoil ( 40Ar recoil). In addition, we demonstrate that thismore » dangerous 210Po surface background can be suppressed, using pulse shape discrimination methods, by a factor of ~100 or higher, which can make argon dark matter detectors near background-free and enhance their potential for discovery of medium- and high-mass WIMPs. Lastly, we also discuss the impact on other low background experiments.« less

Continued Data Acquisition Development

DOE Office of Scientific and Technical Information (OSTI.GOV)

Schwellenbach, David

This task focused on improving techniques for integrating data acquisition of secondary particles correlated in time with detected cosmic-ray muons. Scintillation detectors with Pulse Shape Discrimination (PSD) capability show the most promise as a detector technology based on work in FY13. Typically PSD parameters are determined prior to an experiment and the results are based on these parameters. By saving data in list mode, including the fully digitized waveform, any experiment can effectively be replayed to adjust PSD and other parameters for the best data capture. List mode requires time synchronization of two independent data acquisitions (DAQ) systems: the muonmore » tracker and the particle detector system. Techniques to synchronize these systems were studied. Two basic techniques were identified: real time mode and sequential mode. Real time mode is the preferred system but has proven to be a significant challenge since two FPGA systems with different clocking parameters must be synchronized. Sequential processing is expected to work with virtually any DAQ but requires more post processing to extract the data.« less

Measurement of intrinsic radioactive backgrounds from the 137Cs and U/Th chains in CsI(Tl) crystals

NASA Astrophysics Data System (ADS)

Liu, Shu-Kui; Yue, Qian; Lin, Shin-Ted; Li, Yuan-Jing; Tang, Chang-Jian; Wong Tsz-King, Henry; Xing, Hao-Yang; Yang, Chao-Wen; Zhao, Wei; Zhu, Jing-Jun

2015-04-01

The inorganic CsI(Tl) crystal scintillator is a candidate anti-compton detector for the China Dark matter Experiment. Studying the intrinsic radiopurity of the CsI(Tl) crystal is an issue of major importance. The timing, energy and spatial correlations, as well as the capability of pulse shape discrimination provide powerful methods for the measurement of intrinsic radiopurities. The experimental design, detector performance and event-selection algorithms are described. A total of 359×3 kg-days data from three prototypes of CsI(Tl) crystals were taken at China Jinping Underground Laboratory (CJPL), which offers a good shielding environment. The contamination levels of internal isotopes from 137Cs, 232Th and 238U series, as well as the upper bounds of 235U series are reported. Identification of the whole α peaks from U/Th decay chains and derivation of those corresponding quenching factors are achieved. Supported by National Natural Science Foundation of China (11275107, 11175099)

DOE Office of Scientific and Technical Information (OSTI.GOV)

Furuta, H.; Imura, A.; Furuta, Y.

Recently, technique of Gadolinium loaded liquid scintillator (Gd-LS) for reactor neutrino oscillation experiments has attracted attention as a monitor of reactor operation and 'nuclear Gain (GA)' for IAEA safeguards. For the practical use, R and D of the 1 ton class compact detector, which is measurable above ground, is necessary. Especially, it is important to reduce much amount of fast neutron background induced by cosmic muons with data analysis for the measurement above ground. We developed a prototype of the Gd-LS detector with 200 L of the target volume, which has Pulse Shape Discrimination (PSD) ability for the fast neutronmore » reduction with data analysis. Usually, it is well known that it is difficult to keep high fast neutron reduction power of PSD with the large volume size such as the neutrino reactor monitor. We evaluated the PSD ability of our prototype with real fast neutrons induced by the muons in our laboratory above ground, and we could confirm to keep the high fast neutron reduction power with even our large detector size. (authors)« less

Constraining the Origin of Phobos with the Elpasolite Planetary Ice and Composition Spectrometer (EPICS) - Simulated Performance

NASA Astrophysics Data System (ADS)

Nowicki, S. F.; Mesick, K.; Coupland, D. D. S.; Dallmann, N. A.; Feldman, W. C.; Stonehill, L. C.; Hardgrove, C.; Dibb, S.; Gabriel, T. S. J.; West, S.

2017-12-01

Elpasolites are a promising new family of inorganic scintillators that can detect both gamma rays and neutrons within a single detector volume, reducing the instrument size, weight, and power (SWaP), all of which are critical for planetary science missions. The ability to distinguish between neutron and gamma events is done through pulse shape discrimination (PSD). The Elpasolite Planetary Ice and Composition Spectrometer (EPICS) utilizes elpasolites in a next-generation, highly capable, low-SWaP gamma-ray and neutron spectrometer. We present simulated capabilities of EPICS sensitivities to neutron and gamma-rays, and demonstrate how EPICS can constrain the origin of Phobos between the following three main hypotheses: 1) accretion after a giant impact with Mars, 2) co-accretion with Mars, and 3) capture of an external body. The MCNP6 code was used to calculate the neutron and gamma-ray flux that escape the surface of Phobos, and GEANT4 to model the response of the EPICS instrument on orbit around Phobos.

Generation of first hard X-ray pulse at Tsinghua Thomson Scattering X-ray Source.

PubMed

Du, Yingchao; Yan, Lixin; Hua, Jianfei; Du, Qiang; Zhang, Zhen; Li, Renkai; Qian, Houjun; Huang, Wenhui; Chen, Huaibi; Tang, Chuanxiang

2013-05-01

Tsinghua Thomson Scattering X-ray Source (TTX) is the first-of-its-kind dedicated hard X-ray source in China based on the Thomson scattering between a terawatt ultrashort laser and relativistic electron beams. In this paper, we report the experimental generation and characterization of the first hard X-ray pulses (51.7 keV) via head-on collision of an 800 nm laser and 46.7 MeV electron beams. The measured yield is 1.0 × 10(6) per pulse with an electron bunch charge of 200 pC and laser pulse energy of 300 mJ. The angular intensity distribution and energy spectra of the X-ray pulse are measured with an electron-multiplying charge-coupled device using a CsI scintillator and silicon attenuators. These measurements agree well with theoretical and simulation predictions. An imaging test using the X-ray pulse at the TTX is also presented.

Generation of arbitrarily shaped picosecond optical pulses using an integrated electrooptic waveguide modulator.

PubMed

Haner, M; Warren, W S

1987-09-01

We have produced complex software adjustable laser pulse shapes with ~10-ps resolution, and pulse energies up to 100 microJ for spectroscopic applications. The key devices are a high damage threshold electrooptic directional coupler and a GaAs circuit for synthesizing arbitrarily shaped microwave pulses.

Neutron threshold activation detectors (TAD) for the detection of fissions

NASA Astrophysics Data System (ADS)

Gozani, Tsahi; Stevenson, John; King, Michael J.

2011-10-01

Prompt fission neutrons are one of the strongest signatures of the fission process. Depending on the fission inducing radiation, their average number ranges from 2.5 to 4 neutrons per fission. They are more energetic and abundant, by about 2 orders of magnitude, than the delayed neutrons (≈3 vs. ≈0.01) that are commonly used as indicators for the presence of fissionable materials. The detection of fission prompt neutrons, however, has to be done in the presence of extremely intense probing radiation that stimulated them. During irradiation, the fission stimulation radiation, X-rays or neutrons, overwhelms the neutron detectors and temporarily incapacitate them. Consequently, by the time the detectors recover from the source radiation, fission prompt neutrons are no longer emitted. In order to measure the prompt fission signatures under these circumstances, special measures are usually taken with the detectors such as heavy shielding with collimation, use of inefficient geometries, high pulse height bias and gamma-neutron separation via pulse-shape discrimination with an appropriate organic scintillator. These attempts to shield the detector from the flash of radiation result in a major loss of sensitivity. It can lead to a complete inability to detect the fission prompt neutrons. In order to overcome the blinding induced background from the source radiation, the detection of prompt fission neutrons needs to occur long after the fission event and after the detector has fully recovered from the source overload. A new approach to achieve this is to detect the delayed activation induced by the fission neutrons. The approach demonstrates a good sensitivity in adverse overload situations (gamma and neutron "flash") where fission prompt neutrons could normally not be detected. The new approach achieves the required temporal separation between the detection of prompt neutrons and the detector overload by the neutron activation of the detector material. The technique, called Threshold Activation Detection (TAD), is to utilize appropriate substances that can be selectively activated by the fission neutrons and not by the source radiation and then measure the radioactively decaying activation products (typically beta and gamma rays) well after the source pulse. The activation material should possess certain properties: a suitable half-life of the order of seconds; an energy threshold below which the numerous source neutrons will not activate it (e.g., 3 MeV); easily detectable activation products (typically >1 MeV beta and gamma rays) and have a usable cross-section for the selected reaction. Ideally the substance would be a part of the scintillator. There are several good material candidates for the TAD, including fluorine, which is a major constituent of available scintillators such as BaF 2, CaF 2 and hydrogen free liquid fluorocarbon. Thus the fluorine activation products, in particular the beta particles, can be measured with a very high efficiency in the detector. The principles, applications and experimental results obtained with the fluorine based TAD are discussed.

PULSE AMPLITUDE ANALYZER

DOEpatents

Gray, G.W.; Jensen, A.S.

1957-10-22

A pulse-height analyzer system of improved design for sorting and counting a series of pulses, such as provided by a scintillation detector in nuclear radiation measurements, is described. The analyzer comprises a main transmission line, a cathode-ray tube for each section of the line with its deflection plates acting as the line capacitance; means to bias the respective cathode ray tubes so that the beam strikes a target only when a prearranged pulse amplitude is applied, with each tube progressively biased to respond to smaller amplitudes; pulse generating and counting means associated with each tube to respond when the beam is deflected; a control transmission line having the same time constant as the first line per section with pulse generating means for each tube for initiating a pulse on the second transmission line when a pulse triggers the tube of corresponding amplitude response, the former pulse acting to prevent successive tubes from responding to the pulse under test. This arrangement permits greater deflection sensitivity in the cathode ray tube and overcomes many of the disadvantages of prior art pulse-height analyzer circuits.

A 24 hr global campaign to assess precision timing of the millisecond pulsar J1713+0747

DOE Office of Scientific and Technical Information (OSTI.GOV)

Dolch, T.; Lam, M. T.; Cordes, J.

2014-10-10

The radio millisecond pulsar J1713+0747 is regarded as one of the highest-precision clocks in the sky and is regularly timed for the purpose of detecting gravitational waves. The International Pulsar Timing Array Collaboration undertook a 24 hr global observation of PSR J1713+0747 in an effort to better quantify sources of timing noise in this pulsar, particularly on intermediate (1-24 hr) timescales. We observed the pulsar continuously over 24 hr with the Arecibo, Effelsberg, GMRT, Green Bank, LOFAR, Lovell, Nançay, Parkes, and WSRT radio telescopes. The combined pulse times-of-arrival presented here provide an estimate of what sources of timing noise, excludingmore » DM variations, would be present as compared to an idealized √N improvement in timing precision, where N is the number of pulses analyzed. In the case of this particular pulsar, we find that intrinsic pulse phase jitter dominates arrival time precision when the signal-to-noise ratio of single pulses exceeds unity, as measured using the eight telescopes that observed at L band/1.4 GHz. We present first results of specific phenomena probed on the unusually long timescale (for a single continuous observing session) of tens of hours, in particular interstellar scintillation, and discuss the degree to which scintillation and profile evolution affect precision timing. This paper presents the data set as a basis for future, deeper studies.« less

Smaller, Lower-Power Fast-Neutron Scintillation Detectors

NASA Technical Reports Server (NTRS)

Patel, Jagdish; Blaes, Brent

2008-01-01

Scintillation-based fast-neutron detectors that are smaller and less power-hungry than mainstream scintillation-based fast-neutron detectors are undergoing development. There are numerous applications for such detectors in monitoring fast-neutron fluxes from nuclear reactors, nuclear materials, and natural sources, both on Earth and in outer space. A particularly important terrestrial application for small, low-power, portable fast-neutron detectors lies in the requirement to scan for nuclear materials in cargo and baggage arriving at international transportation facilities. The present development of miniature, low-power scintillation-based fast-neutron detectors exploits recent advances in the fabrication of avalanche photodiodes (APDs). Basically, such a detector includes a plastic scintillator, typically between 300 and 400 m thick with very thin silver mirror coating on all its faces except the one bonded to an APD. All photons generated from scintillation are thus internally reflected and eventually directed to the APD. This design affords not only compactness but also tight optical coupling for utilization of a relatively large proportion of the scintillation light. The combination of this tight coupling and the avalanche-multiplication gain (typically between 750 and 1,000) of the APD is expected to have enough sensitivity to enable monitoring of a fast-neutron flux as small as 1,000 cm(exp -2)s(exp -1). Moreover, pulse-height analysis can be expected to provide information on the kinetic energies of incident neutrons. It has been estimated that a complete, fully developed fast-neutron detector of this type, would be characterized by linear dimensions of the order of 10 cm or less, a mass of no more than about 0.5 kg, and a power demand of no more than a few watts.

Systems and methods for detecting nuclear radiation in the presence of backgrounds

DOEpatents

Bross, Alan D.; Mellott, Kerry L.; Pla-Dalmau, Anna

2005-06-21

Systems and methods for the simultaneous detection and identification of radiation species, including neutrons, gammas/x-rays and minimum ionizing particles (MIPs). A plurality of rectangular and/or triangularly shaped radiation sensitive scintillators can be configured from a plurality of nano-sized particles, dopants and an extruded plastic material. A wavelength-shifting fiber can then be located within a central hole of each extruded scintillator, wherein the wavelength-shifting fiber absorbs scintillation light and re-emits the light at a longer wavelength, thereby piping the light to a photodetector whose response to the light indicates the presence of radiation The resulting method and system can simultaneously detect neutrons, gamma rays, x-rays and cosmic rays (MIPs) and identify each.

Scintillation properties of the Ce-doped multicomponent garnet epitaxial films

NASA Astrophysics Data System (ADS)

Prusa, P.; Kucera, M.; Mares, J. A.; Hanus, M.; Beitlerova, A.; Onderisinova, Z.; Nikl, M.

2013-10-01

(Lu,Y,Gd)3(Al,Ga)5O12:Ce garnet scintillator single crystalline films were grown onto LuAG, YAG and GGG substrates by liquid phase epitaxy method. Absorption, radioluminescence spectra and photoluminescence excitation, emission spectra, and decay kinetics were measured. Photoelectron yield, its dependence on amplifier shaping time and energy resolution were determined to evaluate scintillation performance. Most of the samples exhibited strong UV emission caused by trapped excitons and/or Gd3+ 4f-4f transition. However, emission spectrum of the best performing Gd2YAl5O12:Ce is dominated by the Ce3+ fast 5d-4f luminescence. This sample has outperformed photoelectron yield of all the garnet films studied so far.

Characterization of spectral and intensity changes with measurement geometry in various light guides used in scintillation dosimetry.

PubMed

Simiele, Eric A; DeWerd, Larry A

2018-05-24

To characterize response changes of various light guides used in megavoltage (MV) photon beam scintillation dosimetry as a function of irradiation conditions. Particular emphasis was placed on quantifying the impact of response changes on the Čerenkov light ratio (CLR). Intensity and spectral response measurements as a function of dose, depth, and fiber-beam angle were performed with a commercial scintillation detector stripped of its scintillation material and five different custom-made light guides. The core materials of the light guides investigated consisted of polymethyl methacrylate (PMMA), low- and high-hydroxyl content silica, and polystyrene. Dose levels ranging from 50 monitor units (MU) to 1000 MU, depths ranging from 1 to 20 cm, and fiber-beam angles ranging from 10° to 90° were investigated. All measurements were performed at a photon beam energy of 6 MV. The CLR was calculated by taking the ratio of the responses in the blue to green spectral regions. There was no significant change in the CLR measured with the modified commercial scintillation detector as a function of delivered dose. In addition, increases in the CLR as functions of depth and fiber-beam angle were observed where the maximum changes were 4.2% and 3.6%, respectively. The spectrum measurements showed no observable changes in spectral shape with depth except for the low-hydroxyl content silica fiber. Variations in the measured spectral shape with fiber-beam angle were observed for all fibers investigated. The magnitude of the changes in the spectral shape varied with fiber type, where the silica fibers exhibited the largest changes and the plastic fibers exhibited the smallest changes. Increases in the CLR were observed for the silica fibers with depth and for all fibers with fiber-beam angle. The plastic fibers showed no significant change in the CLR as a function of depth. Increases of 3.1% and 9.5% in the CLR were observed for the high- and low-hydroxyl content silica fibers, respectively, over the range of depths investigated. Variations of 2.3%, 6.1%, 5.1% and 11.9% were observed for the PMMA, polystyrene, high-hydroxyl, and low-hydroxyl content silica fiber CLR values as a function of fiber-beam angle, respectively. The insignificant change in the CLR with delivered dose indicates that a single CLR value over the investigated dose range is sufficient for accurate Čerenkov subtraction. Variations in the stem-effect spectrum shape can occur with changes in irradiation geometry. The magnitude of the changes are governed by the fiber construction and the optical properties of the fiber. The observed spectral shape changes can be explained by a combination of variations in optical path length through the fiber and the fiber fluorescent signal contribution to the stem-effect. These spectral shape variations directly influence the calculated CLR values. This work confirms that careful characterization of scintillation detectors is important as changes in the stem-effect spectrum can cause changes in the CLR. If the CLR changes between the reference and measurement conditions, this could result in an incorrect stem-effect subtraction and reduced measurement accuracy. © 2018 American Association of Physicists in Medicine.

Effect of the combination of different welding parameters on melting characteristics of grade 1 titanium with a pulsed Nd-Yag laser.

PubMed

Bertrand, C; Laplanche, O; Rocca, J P; Le Petitcorps, Y; Nammour, S

2007-11-01

The laser is a very attractive tool for joining dental metallic alloys. However, the choice of the setting parameters can hardly influence the welding performances. The aim of this research was to evaluate the impact of several parameters (pulse shaping, pulse frequency, focal spot size...) on the quality of the microstructure. Grade 1 titanium plates have been welded with a pulsed Nd-Yag laser. Suitable power, pulse duration, focal spot size, and flow of argon gas were fixed by the operator. Five different pulse shapes and three pulse frequencies were investigated. Two pulse shapes available on this laser unit were eliminated because they considerably hardened the metal. As the pulse frequency rose, the metal was more and more ejected, and a plasma on the surface of the metal increased the oxygen contamination in the welded area. Frequencies of 1 or 2 Hz are optimum for a dental use. Three pulse shapes can be used for titanium but the rectangular shape gives better results.

High-speed pulse-shape generator, pulse multiplexer

DOEpatents

Burkhart, Scott C.

2002-01-01

The invention combines arbitrary amplitude high-speed pulses for precision pulse shaping for the National Ignition Facility (NIF). The circuitry combines arbitrary height pulses which are generated by replicating scaled versions of a trigger pulse and summing them delayed in time on a pulse line. The combined electrical pulses are connected to an electro-optic modulator which modulates a laser beam. The circuit can also be adapted to combine multiple channels of high speed data into a single train of electrical pulses which generates the optical pulses for very high speed optical communication. The invention has application in laser pulse shaping for inertial confinement fusion, in optical data links for computers, telecommunications, and in laser pulse shaping for atomic excitation studies. The invention can be used to effect at least a 10.times. increase in all fiber communication lines. It allows a greatly increased data transfer rate between high-performance computers. The invention is inexpensive enough to bring high-speed video and data services to homes through a super modem.

Waveform synthesizer

DOEpatents

Franks, Larry A.; Nelson, Melvin A.

1981-01-01

A method of producing optical and electrical pulses of desired shape. An optical pulse of arbitrary but defined shape illuminates one end of an array of optical fiber waveguides of differing lengths to time differentiate the input pulse. The optical outputs at the other end of the array are combined to form a synthesized pulse of desired shape.

TH-C-19A-11: Toward An Optimized Multi-Point Scintillation Detector

DOE Office of Scientific and Technical Information (OSTI.GOV)

Duguay-Drouin, P; Delage, ME; Centre Hospitalier University de Quebec, Quebec, QC

Purpose: The purpose of this work is to characterize a 2-points mPSDs' optical chain using a spectral analysis to help selecting the optimal components for the detector. Methods: Twenty different 2-points mPSD combinations were built using 4 plastic scintillators (BCF10, BCF12, BCF60, BC430; St-Gobain) and quantum dots (QDs). The scintillator is said to be proximal when near the photodetector, and distal otherwise. A 15m optical fiber (ESKA GH-4001) was coupled to the scintillating component and connected to a spectrometer (Shamrock, Andor and QEPro, OceanOptics). These scintillation components were irradiated at 125kVp; a spectrum for each scintillator was obtained by irradiationmore » of individual scintillator and shielding the second component, thus talking into account light propagation in all components and interfaces. The combined total spectrum was also acquired and involved simultaneous irradiation of the two scintillators for each possible combination. The shape and intensity were characterized. Results: QDs in proximal position absorb almost all the light signal from distal plastic scintillators and emit in its own emission wavelength, with 100% of the signal in the QD range (625–700nm) for the combination BCF12/QD. However, discrimination is possible when QD is in distal position in combination with blue scintillators, total signal being 73% in the blue range (400-550nm) and 27% in QD range. Similar results are obtained with the orange scintillator (BC430). For optimal signal intensity, BCF12 should always be in proximal position, e.g. having 50% more intensity when coupled with BCF60 in distal position (BCF12/BCF60) compared to the BCF60/BCF12 combination. Conclusion: Different combinations of plastic scintillators and QD were built and their emission spectra were studied. We established a preferential order for the scintillating components in the context of an optimized 2-points mPSD. In short, the components with higher wavelength emission spectrum should be distal and lower wavelength in the proximal position.« less

A logarithmic detection system suitable for a 4π array

NASA Astrophysics Data System (ADS)

Westfall, G. D.; Yurkon, J. E.; van der Plicht, J.; Koenig, Z. M.; Jacak, B. V.; Fox, R.; Crawley, G. M.; Maier, M. R.; Hasselquist, B. E.; Tickle, R. S.; Horn, D.

1985-08-01

A low pressure multiwire proportional counter, a Bragg curve counter, and an array of CaF2/plastic scintillator telescopes have been developed in a geometry suitable for close packing into a 4π detector designed to study nucleus-nucleus reactions at 100-200 MeV/nucleon. The multiwire counter is hexagonal in shape and gives X-Y position information using resistive charge division from nichrome-coated stretched polypropylene foils. The Bragg curve counter is a hexagonal pyramid with the charge taken from a Frisch gridded anode. A field shaping grid gives the Bragg curve counter a radial field. The scintillator telescopes are shaped as truncated triangular pyramids such that when stacked together they form a truncated hexagonal pyramid. The light signal of the CaF2-plastic combination is read with one phototube using a phoswich technique to separate the ΔE signal from the E signal. The entire system has been tested so far for particles with 1 <= Z <= 18 and gives good position, charge, and time resolution.

Characterizations of Pr-doped Yb3Al5O12 single crystals for scintillator applications

NASA Astrophysics Data System (ADS)

Yoshida, Yasuki; Shinozaki, Kenji; Igashira, Takuya; Kawano, Naoki; Okada, Go; Kawaguchi, Noriaki; Yanagida, Takayuki

2018-04-01

Yb3Al5O12 (YbAG) single crystals doped with different concentrations of Pr were synthesized by the Floating Zone (FZ) method. Then, we evaluated their basic optical and scintillation properties. All the samples showed photoluminescence (PL) with two emission bands appeared approximately 300-500 nm and 550-600 nm due to the charge transfer luminescence of Yb3+ and intrinsic luminescence of the garnet structure, respectively. A PL decay profile of each sample was approximated by a sum of two exponential decay functions, and the obtained decay times were 1 ns and 3-4 ns. In the scintillation spectra, we observed emission peaks in the ranges from 300 to 400 nm and from 450 to 550 nm for all the samples. The origins of these emissions were attributed to charge transfer luminescence of Yb3+ and intrinsic luminescence of the garnet structure, respectively. The scintillation decay times became longer with increasing the Pr concentrations. Among the present samples, the 0.1% Pr-doped sample showed the lowest scintillation afterglow level. In addition, pulse height spectrum of 5.5 MeV α-rays was demonstrated using the Pr-doped YbAG, and we confirmed that all the samples showed a full energy deposited peak. Above all, the 0.1% Pr-doped sample showed the highest light yield with a value of 14 ph/MeV under α-rays excitation.

Power Spectrum of Atmospheric Scintillation for the Deep Space Network Goldstone Ka-Band Downlink

NASA Technical Reports Server (NTRS)

Ho, C.; Wheelon, A.

2004-01-01

Dynamic signal fluctuations due to atmospheric scintillations may impair the Ka-band (around 32-GHz) link sensitivities for a low-margin Deep Space Network (DSN) receiving system. The ranges of frequency and power of the fast fluctuating signals (time scale less than 1 min) are theoretically investigated using the spatial covariance and turbulence theory. Scintillation power spectrum solutions are derived for both a point receiver and a finite-aperture receiver. The aperture-smoothing frequency ((omega(sub s)), corner frequency ((omega(sub c)), and damping rate are introduced to define the shape of the spectrum for a finite-aperture antenna. The emphasis is put on quantitatively describing the aperture-smoothing effects and graphically estimating the corner frequency for a large aperture receiver. Power spectral shapes are analyzed parametrically in detail through both low- and high-frequency approximations. It is found that aperture-averaging effects become significant when the transverse correlation length of the scintillation is smaller than the antenna radius. The upper frequency or corner frequency for a finite-aperture receiver is controlled by both the Fresnel frequency and aperture-smoothing frequency. Above the aperture-smoothing frequency, the spectrum rolls off at a much faster rate of exp (-omega(sup 2)/omega(sup 2, sub s), rather than omega(sup -8/3), which is customary for a point receiver. However, a relatively higher receiver noise level can mask the fast falling-off shape and make it hard to be identified. We also predict that when the effective antenna radius a(sub r) less than or = 6 m, the corner frequency of its power spectrum becomes the same as that for a point receiver. The aperture-smoothing effects are not obvious. We have applied these solutions to the scenario of a DSN Goldstone 34-m-diameter antenna and predicted the power spectrum shape for the receiving station. The maximum corner frequency for the receiver (with omega(sub s) = 0.79 omega(sub 0) is found to be 0.44 Hz (or 1.0 omega(sub 0), while the fading rate (or fading slope) is about 0.06 dB/s.

Resolving the shape of a sonoluminescence pulse in sulfuric acid by the use of streak camera.

PubMed

Huang, Wei; Chen, Weizhong; Cui, Weicheng

2009-06-01

A streak camera is used to measure the shape of sonoluminescence pulses from a cavitation bubble levitated stably in a sulfuric acid solution. The shape and response to an acoustic pressure field of the sonoluminescence pulse in 85% by weight sulfuric acid are qualitatively similar to those in water. However, the pulse width in sulfuric acid is wider than that in water by over one order of magnitude. The width of the sonoluminescence pulse is strongly dependent on the concentration of the sulfuric acid solution, while the skewed distribution of the shape remains unchanged.

Neutron coincidence detectors employing heterogeneous materials

DOEpatents

Czirr, J. Bartley; Jensen, Gary L.

1993-07-27

A neutron detector relies upon optical separation of different scintillators to measure the total energy and/or number of neutrons from a neutron source. In pulse mode embodiments of the invention, neutrons are detected in a first detector which surrounds the neutron source and in a second detector surrounding the first detector. An electronic circuit insures that only events are measured which correspond to neutrons first detected in the first detector followed by subsequent detection in the second detector. In spectrometer embodiments of the invention, neutrons are thermalized in the second detector which is formed by a scintillator-moderator and neutron energy is measured from the summed signals from the first and second detectors.

Comparative study of nondoped and Eu-doped SrI2 scintillator

NASA Astrophysics Data System (ADS)

Yanagida, Takayuki; Koshimizu, Masanori; Okada, Go; Kojima, Takahiro; Osada, Junya; Kawaguchi, Noriaki

2016-11-01

Optical and scintillation properties of nondoped and Eu 3% doped SrI2 crystals grown by the Vertical Bridgman method were investigated. Eu-doped crystal showed an intense single band emission at 430 nm due to the Eu2+ 5d-4f transitions in both photoluminescence and scintillation while the nondoped crystal had a complex spectral shape. The latter emission consists of mainly four bands: 360 nm, 540 nm, 410 nm and 430 nm. The origins of 360 nm and 540 nm were self-trapped exciton and unexpected impurity, respectively. The origins of 410 and 430 nm lines were ascribed to F center in different I sites. Under 137Cs γ-ray irradiations, both crystals showed a clear photoabsorption peak. The scintillation light yields of the nondoped and Eu-doped SrI2 resulted 33,000 ph/MeV and 82,000 ph/MeV, respectively. The energy resolution at 662 keV of Eu-doped was 4% while that of the non-doped SrI2 was 8%.

Composition and apparatus for detecting gamma radiation

DOEpatents

Hofstetter, Kenneth J.

1994-01-01

A gamma radiation detector and a radioluminiscent composition for use therein. The detector includes a radioluminscent composition that emits light in a characteristic wavelength region when exposed to gamma radiation, and means for detecting said radiation. The composition contains a scintillant such as anglesite (PbSO.sub.4) or cerussite (PbCO.sub.3) incorporated into an inert, porous glass matrix via a sol-gel process. Particles of radiation-sensitive scintillant are added to, a sol solution. The mixture is polymerized to form a gel, then dried under conditions that preserve the structural integrity and radiation sensitivity of the scintillant. The final product is a composition containing the uniformly-dispersed scintillant in an inert, optically transparent and highly porous matrix. The composition is chemically inert and substantially impervious to environmental conditions including changes in temperature, air pressure, and so forth. It can be fabricated in cylinders, blocks with holes therethrough for flow of fluid, sheets, surface coatings, pellets or other convenient shapes.

Composition and apparatus for detecting gamma radiation

DOEpatents

Hofstetter, K.J.

1994-08-09

A gamma radiation detector and a radioluminescent composition for use therein. The detector includes a radioluminescent composition that emits light in a characteristic wavelength region when exposed to gamma radiation, and means for detecting said radiation. The composition contains a scintillant such as anglesite (PbSO[sub 4]) or cerussite (PbCO[sub 3]) incorporated into an inert, porous glass matrix via a sol-gel process. Particles of radiation-sensitive scintillant are added to, a sol solution. The mixture is polymerized to form a gel, then dried under conditions that preserve the structural integrity and radiation sensitivity of the scintillant. The final product is a composition containing the uniformly-dispersed scintillant in an inert, optically transparent and highly porous matrix. The composition is chemically inert and substantially impervious to environmental conditions including changes in temperature, air pressure, and so forth. It can be fabricated in cylinders, blocks with holes therethrough for flow of fluid, sheets, surface coatings, pellets or other convenient shapes. 3 figs.

Electron multiplier-ion detector system

DOEpatents

Dietz, L.A.

1975-08-01

This patent relates to an improved ion detector for use in mass spectrometers for pulse counting signal ions which may have a positive or a negative charge. The invention combines a novel electron multiplier with a scintillator type of ion detector. It is a high vacuum, high voltage device intended for use in ion microprobe mass spectrometers. (auth)

Designing a new type of neutron detector for neutron and gamma-ray discrimination via GEANT4.

PubMed

Shan, Qing; Chu, Shengnan; Ling, Yongsheng; Cai, Pingkun; Jia, Wenbao

2016-04-01

Design of a new type of neutron detector, consisting of a fast neutron converter, plastic scintillator, and Cherenkov detector, to discriminate 14-MeV fast neutrons and gamma rays in a pulsed n-γ mixed field and monitor their neutron fluxes is reported in this study. Both neutrons and gamma rays can produce fluorescence in the scintillator when they are incident on the detector. However, only the secondary charged particles of the gamma rays can produce Cherenkov light in the Cherenkov detector. The neutron and gamma-ray fluxes can be calculated by measuring the fluorescence and Cherenkov light. The GEANT4 Monte Carlo simulation toolkit is used to simulate the whole process occurring in the detector, whose optimum parameters are known. Analysis of the simulation results leads to a calculation method of neutron flux. This method is verified by calculating the neutron fluxes using pulsed n-γ mixed fields with different n/γ ratios, and the results show that the relative errors of all calculations are <5%. Copyright © 2016 Elsevier Ltd. All rights reserved.

Improving photoelectron counting and particle identification in scintillation detectors with Bayesian techniques

NASA Astrophysics Data System (ADS)

Akashi-Ronquest, M.; Amaudruz, P.-A.; Batygov, M.; Beltran, B.; Bodmer, M.; Boulay, M. G.; Broerman, B.; Buck, B.; Butcher, A.; Cai, B.; Caldwell, T.; Chen, M.; Chen, Y.; Cleveland, B.; Coakley, K.; Dering, K.; Duncan, F. A.; Formaggio, J. A.; Gagnon, R.; Gastler, D.; Giuliani, F.; Gold, M.; Golovko, V. V.; Gorel, P.; Graham, K.; Grace, E.; Guerrero, N.; Guiseppe, V.; Hallin, A. L.; Harvey, P.; Hearns, C.; Henning, R.; Hime, A.; Hofgartner, J.; Jaditz, S.; Jillings, C. J.; Kachulis, C.; Kearns, E.; Kelsey, J.; Klein, J. R.; Kuźniak, M.; LaTorre, A.; Lawson, I.; Li, O.; Lidgard, J. J.; Liimatainen, P.; Linden, S.; McFarlane, K.; McKinsey, D. N.; MacMullin, S.; Mastbaum, A.; Mathew, R.; McDonald, A. B.; Mei, D.-M.; Monroe, J.; Muir, A.; Nantais, C.; Nicolics, K.; Nikkel, J. A.; Noble, T.; O'Dwyer, E.; Olsen, K.; Orebi Gann, G. D.; Ouellet, C.; Palladino, K.; Pasuthip, P.; Perumpilly, G.; Pollmann, T.; Rau, P.; Retière, F.; Rielage, K.; Schnee, R.; Seibert, S.; Skensved, P.; Sonley, T.; Vázquez-Jáuregui, E.; Veloce, L.; Walding, J.; Wang, B.; Wang, J.; Ward, M.; Zhang, C.

2015-05-01

Many current and future dark matter and neutrino detectors are designed to measure scintillation light with a large array of photomultiplier tubes (PMTs). The energy resolution and particle identification capabilities of these detectors depend in part on the ability to accurately identify individual photoelectrons in PMT waveforms despite large variability in pulse amplitudes and pulse pileup. We describe a Bayesian technique that can identify the times of individual photoelectrons in a sampled PMT waveform without deconvolution, even when pileup is present. To demonstrate the technique, we apply it to the general problem of particle identification in single-phase liquid argon dark matter detectors. Using the output of the Bayesian photoelectron counting algorithm described in this paper, we construct several test statistics for rejection of backgrounds for dark matter searches in argon. Compared to simpler methods based on either observed charge or peak finding, the photoelectron counting technique improves both energy resolution and particle identification of low energy events in calibration data from the DEAP-1 detector and simulation of the larger MiniCLEAN dark matter detector.

Pulse Shaped Constant Envelope 8-PSK Modulation Study

NASA Technical Reports Server (NTRS)

Tao, Jianping; Horan, Sheila

1997-01-01

This report provides simulation results for constant envelope pulse shaped 8 Level Phase Shift Keying (8 PSK) modulation for end to end system performance. In order to increase bandwidth utilization, pulse shaping is applied to signals before they are modulated. This report provides simulation results of power spectra and measurement of bit errors produced by pulse shaping in a non-linear channel with Additive White Gaussian Noise (AWGN). The pulse shaping filters can placed before (Type B) or after (Type A) signals are modulated. Three kinds of baseband filters, 5th order Butterworth, 3rd order Bessel and Square-Root Raised Cosine with different BTs or roll off factors, are utilized in the simulations. The simulations were performed on a Signal Processing Worksystem (SPW).