Science.gov

Sample records for soft x-ray inelastic

  1. Highly efficient beamline and spectrometer for inelastic soft X-ray scattering at high resolution.

    PubMed

    Lai, C H; Fung, H S; Wu, W B; Huang, H Y; Fu, H W; Lin, S W; Huang, S W; Chiu, C C; Wang, D J; Huang, L J; Tseng, T C; Chung, S C; Chen, C T; Huang, D J

    2014-03-01

    The design, construction and commissioning of a beamline and spectrometer for inelastic soft X-ray scattering at high resolution in a highly efficient system are presented. Based on the energy-compensation principle of grating dispersion, the design of the monochromator-spectrometer system greatly enhances the efficiency of measurement of inelastic soft X-rays scattering. Comprising two bendable gratings, the set-up effectively diminishes the defocus and coma aberrations. At commissioning, this system showed results of spin-flip, d-d and charge-transfer excitations of NiO. These results are consistent with published results but exhibit improved spectral resolution and increased efficiency of measurement. The best energy resolution of the set-up in terms of full width at half-maximum is 108 meV at an incident photon energy tuned about the Ni L3-edge.

  2. A multiplexed high-resolution imaging spectrometer for resonant inelastic soft X-ray scattering spectroscopy.

    PubMed

    Warwick, Tony; Chuang, Yi De; Voronov, Dmitriy L; Padmore, Howard A

    2014-07-01

    The optical design of a two-dimensional imaging soft X-ray spectrometer is described. A monochromator will produce a dispersed spectrum in a narrow vertical illuminated stripe (∼2 µm wide by ∼2 mm tall) on a sample. The spectrometer will use inelastically scattered X-rays to image the extended field on the sample in the incident photon energy direction (vertical), resolving the incident photon energy. At the same time it will image and disperse the scattered photons in the orthogonal (horizontal) direction, resolving the scattered photon energy. The principal challenge is to design a system that images from the flat-field illumination of the sample to the flat field of the detector and to achieve sufficiently high spectral resolution. This spectrometer provides a completely parallel resonant inelastic X-ray scattering measurement at high spectral resolution (∼30,000) over the energy bandwidth (∼5 eV) of a soft X-ray absorption resonance.

  3. Resonant inelastic soft x-ray scattering of CdS: a two-dimensional electronic structure map approach

    SciTech Connect

    Weinhardt, L.; Fuchs, O.; Fleszar, A.; Bar, M.; Blum, M.; Weigand, M.; Denlinger, J.D.; Yang, W.; Hanke, W.; Umbach, E.; Heske, C.

    2008-09-24

    Resonant inelastic x-ray scattering (RIXS) with soft x-rays is uniquely suited to study the elec-tronic structure of a variety of materials, but is currently limited by low (fluorescence yield) count rates. This limitation is overcome with a new high-transmission spectrometer that allows to measure soft x-ray RIXS"maps." The S L2,3 RIXS map of CdS is discussed and compared with density functional calculations. The map allows the extraction of decay channel-specific"absorp-tion spectra," giving detailed insight into the wave functions of occupied and unoccupied elec-tronic states.

  4. The SEXTANTS beamline at SOLEIL: a new facility for elastic, inelastic and coherent scattering of soft X-rays

    NASA Astrophysics Data System (ADS)

    Sacchi, M.; Jaouen, N.; Popescu, H.; Gaudemer, R.; Tonnerre, J. M.; Chiuzbaian, S. G.; Hague, C. F.; Delmotte, A.; Dubuisson, J. M.; Cauchon, G.; Lagarde, B.; Polack, F.

    2013-03-01

    SEXTANTS is a new SOLEIL beamline dedicated to soft X-ray scattering techniques. The beamline, covering the 50-1700 eV energy range, features two Apple-II undulators for polarization control and a fixed-deviation monochromator. Two branch-lines host three end-stations for elastic, inelastic and coherent scattering experiments.

  5. Electronic Structure in Thin Film Organic Semiconductors Studied using Soft X-ray Emission and Resonant Inelastic X-ray Scattering

    SciTech Connect

    Zhang,Y.; Downes, J.; Wang, S.; Learmonth, T.; Plucinski, L.; Matsuura, A.; McGuinness, C.; Glans, P.; Bernardis, S.; et al.

    2006-01-01

    The electronic structure of thin films of the organic semiconductors copper and vanadyl (VO) phthalocyanine (Pc) has been measured using resonant soft X-ray emission spectroscopy and resonant inelastic X-ray scattering. For Cu-Pc we report the observation of two discrete states near E{sub F}. This differs from published photoemission results, but is in excellent agreement with density functional calculations. For VO-Pc, the vanadyl species is shown to be highly localized. Both dipole forbidden V 3d to V 3d*, and O 2p to V 3d* charge transfer transitions are observed, and explained in a local molecular orbital model.

  6. A setup for resonant inelastic soft x-ray scattering on liquids at free electron laser light sources

    SciTech Connect

    Kunnus, Kristjan; Schreck, Simon; Foehlisch, Alexander; Eckert, Sebastian; Beye, Martin; Suljoti, Edlira; Weniger, Christian; Wernet, Philippe; Kalus, Christian; Nordlund, Dennis; Zhang, Wenkai; Hartsock, Robert W.; Gaffney, Kelly J.; Schlotter, William F.; Turner, Joshua J.; Kennedy, Brian; and others

    2012-12-15

    We present a flexible and compact experimental setup that combines an in vacuum liquid jet with an x-ray emission spectrometer to enable static and femtosecond time-resolved resonant inelastic soft x-ray scattering (RIXS) measurements from liquids at free electron laser (FEL) light sources. We demonstrate the feasibility of this type of experiments with the measurements performed at the Linac Coherent Light Source FEL facility. At the FEL we observed changes in the RIXS spectra at high peak fluences which currently sets a limit to maximum attainable count rate at FELs. The setup presented here opens up new possibilities to study the structure and dynamics in liquids.

  7. The simultaneous measurement of energy and linear polarization of the scattered radiation in resonant inelastic soft x-ray scattering

    SciTech Connect

    Braicovich, L. Minola, M.; Dellea, G.; Ghiringhelli, G.; Le Tacon, M.; Moretti Sala, M.; Morawe, C.; Peffen, J.-Ch.; Yakhou, F.; Brookes, N. B.; Supruangnet, R.

    2014-11-15

    Resonant Inelastic X-ray Scattering (RIXS) in the soft x-ray range is an element-specific energy-loss spectroscopy used to probe the electronic and magnetic excitations in strongly correlated solids. In the recent years, RIXS has been progressing very quickly in terms of energy resolution and understanding of the experimental results, but the interpretation of spectra could further improve, sometimes decisively, from a full knowledge of the polarization of incident and scattered photons. Here we present the first implementation, in a high resolution soft-RIXS spectrometer used to analyze the scattered radiation, of a device allowing the measurement of the degree of linear polarization. The system, based on a graded W/B{sub 4}C multilayer mirror installed in proximity of the CCD detector, has been installed on the AXES spectrometer at the ESRF (European Synchrotron Radiation Facility); it has been fully characterized and it has been used for a demonstration experiment at the Cu L{sub 3} edge on a high-T{sub c} superconducting cuprate. The loss in efficiency suffered by the spectrometer equipped with this test facility was a factor 17.5. We propose also a more advanced version, suitable for a routine use on the next generation of RIXS spectrometers and with an overall efficiency up to 10%.

  8. High-resolution soft X-ray beamline ADRESS at the Swiss Light Source for resonant inelastic X-ray scattering and angle-resolved photoelectron spectroscopies

    PubMed Central

    Strocov, V. N.; Schmitt, T.; Flechsig, U.; Schmidt, T.; Imhof, A.; Chen, Q.; Raabe, J.; Betemps, R.; Zimoch, D.; Krempasky, J.; Wang, X.; Grioni, M.; Piazzalunga, A.; Patthey, L.

    2010-01-01

    The concepts and technical realisation of the high-resolution soft X-ray beamline ADRESS operating in the energy range from 300 to 1600 eV and intended for resonant inelastic X-ray scattering (RIXS) and angle-resolved photoelectron spectroscopy (ARPES) are described. The photon source is an undulator of novel fixed-gap design where longitudinal movement of permanent magnetic arrays controls not only the light polarization (including circular and 0–180° rotatable linear polarizations) but also the energy without changing the gap. The beamline optics is based on the well established scheme of plane-grating monochromator operating in collimated light. The ultimate resolving power E/ΔE is above 33000 at 1 keV photon energy. The choice of blazed versus lamellar gratings and optimization of their profile parameters is described. Owing to glancing angles on the mirrors as well as optimized groove densities and profiles of the gratings, the beamline is capable of delivering high photon flux up to 1 × 1013 photons s−1 (0.01% BW)−1 at 1 keV. Ellipsoidal refocusing optics used for the RIXS endstation demagnifies the vertical spot size down to 4 µm, which allows slitless operation and thus maximal transmission of the high-resolution RIXS spectrometer delivering E/ΔE > 11000 at 1 keV photon energy. Apart from the beamline optics, an overview of the control system is given, the diagnostics and software tools are described, and strategies used for the optical alignment are discussed. An introduction to the concepts and instrumental realisation of the ARPES and RIXS endstations is given. PMID:20724785

  9. Improving the spatial resolution of a soft X-ray Charge Coupled Device used for Resonant Inelastic X-ray Scattering

    NASA Astrophysics Data System (ADS)

    Soman, M. R.; Hall, D. J.; Tutt, J. H.; Murray, N. J.; Holland, A. D.; Schmitt, T.; Raabe, J.; Schmitt, B.

    2011-11-01

    The Super Advanced X-ray Emission Spectrometer (SAXES) at the Advanced Resonant Scattering (ADRESS) beamline of the Swiss Light Source is a high-resolution X-ray spectrometer used as an end station for Resonant Inelastic X-ray Scattering from 400 eV to 1600 eV. Through the dispersion of photons across a CCD, the energy of scattered photons may be determined by their detected spatial position. The limiting factor of the energy resolution is currently the spatial resolution achieved with the CCD, reported at 24 μm FWHM. For this energy range the electron clouds are formed by interactions in the `field free' region of the back-illuminated CCD. These clouds diffuse in all directions whilst being attracted to the electrodes, leading to events that are made up of signals in multiple pixels. The spreading of the charge allows centroiding techniques to be used to improve the CCD spatial resolution and therefore improve the energy resolution of SAXES. The PolLux microscopy beamline at the SLS produces an X-ray beam with a diameter of 20 nm. The images produced from scanning the narrow beam across CCD pixels (13.5 × 13.5 μm2) can aid in the production of event recognition algorithms, allowing the matching of event profiles to photon interactions in a specific region of a pixel. Through the use of this information software analysis can be refined with the aim of improving the energy resolution.

  10. Soft x-ray lasers

    SciTech Connect

    Matthews, D.L.; Rosen, M.D.

    1988-12-01

    One of the elusive dreams of laser physicists has been the development of an x-ray laser. After 25 years of waiting, the x-ray laser has at last entered the scientific scene, although those now in operation are still laboratory prototypes. They produce soft x rays down to about five nanometers. X-ray lasers retain the usual characteristics of their optical counterparts: a very tight beam, spatial and temporal coherence, and extreme brightness. Present x-ray lasers are nearly 100 times brighter that the next most powerful x-ray source in the world: the electron synchrotron. Although Lawrence Livermore National Laboratory (LLNL) is widely known for its hard-x-ray laser program which has potential applications in the Strategic Defense Initiative, the soft x-ray lasers have no direct military applications. These lasers, and the scientific tools that result from their development, may one day have a place in the design and diagnosis of both laser fusion and hard x-ray lasers. The soft x-ray lasers now in operation at the LLNL have shown great promise but are still in the primitive state. Once x-ray lasers become reliable, efficient, and economical, they will have several important applications. Chief among them might be the creation of holograms of microscopic biological structures too small to be investigated with visible light. 5 figs.

  11. Soft-x-ray emission and inelastic electron-scattering study of the electronic excitations in amorphous and crystalline silicon dioxide

    NASA Astrophysics Data System (ADS)

    Nithianandam, V. Jeyasingh; Schnatterly, S. E.

    1988-09-01

    The valence-band electronic structures of amorphous and crystalline SiO2 are examined with soft-x-ray emission spectroscopy. In addition, the absorption spectra of a-SiO2 obtained by inelastic electron scattering (IES) near the interband threshold and Si L23 threshold regions are presented. Simple models used to describe the absorption in these spectral regions give consistent values for the size of the band gap of SiO2. An empirical model based on these results is presented to explain the positions of peaks in the ultraviolet optical spectrum and the IES valence excitation spectrum of SiO2. The Si 2p core exciton observed in both x-ray emission and absorption spectra is discussed.

  12. Electronic Structure of the ID Conductor K0.3MoO3 studied using resonant inelastic x-ray scattering and soft x-ray emission spectroscopy

    SciTech Connect

    Learmonth, T.; Glans, P.-A.; McGuinness, C.; Plucinski, L.; Zhang, Y.; Guo, J.-H.; Greenblatt, M.; Smith, K.E.

    2008-09-24

    The electronic structure of the quasi-one dimensional conductor K{sub 0.3}MoO{sub 3} has been measured using high resolution resonant inelastic x-ray scattering and x-ray absorption spectroscopy. The data is compared to that from the related two dimensional insulator {alpha}-MoO{sub 3}. Scattering features are observed from both oxides that are explained in terms of the band momentum selectivity of the scattering process, allowing a comparison of the scattering data to recent band structure calculations.

  13. Soft x-ray interferometry

    SciTech Connect

    Not Available

    1993-09-01

    The purpose of the soft x-ray interferometry workshop held at Lawrence Berkeley Laboratory was to discuss with the scientific community the proposed technical design of the soft x-ray Fourier-transform spectrometer being developed at the ALS. Different design strategies for the instrument`s components were discussed, as well as detection methods, signal processing issues, and how to meet the manufacturing tolerances that are necessary for the instrument to achieve the desired levels of performance. Workshop participants were encouraged to report on their experiences in the field of Fourier transform spectroscopy. The ALS is developing a Fourier transform spectrometer that is intended to operate up to 100 eV. The motivation is solely improved resolution and not the throughput (Jaquinot) or multiplex (Fellgett) advantage, neither of which apply for the sources and detectors used in this spectral range. The proposed implementation of this is via a Mach-Zehnder geometry that has been (1) distorted from a square to a rhombus to get grazing incidence of a suitable angle for 100 eV and (2) provided with a mirror-motion system to make the path difference between the interfering beams tunable. The experiment consists of measuring the emergent light intensity (I(x)) as a function of the path difference (x). The resolving power of the system is limited by the amount of path difference obtainable that is 1 cm (one million half-waves at 200{angstrom} wavelength) in the design thus allowing a resolving power of one million. The free spectral range of the system is limited by the closeness with which the function I(x) is sampled. It is proposed to illuminate a helium absorption cell with roughly 1%-band-width light from a monochromator thus allowing one hundred aliases without spectral overlap even for sampling of I(x) at one hundredth of the Nyquist frequency.

  14. Soft-x-ray spectroscopy study of nanoscale materials

    SciTech Connect

    Guo, J.-H.

    2005-07-30

    The ability to control the particle size and morphology of nanoparticles is of crucial importance nowadays both from a fundamental and industrial point of view considering the tremendous amount of high-tech applications. Controlling the crystallographic structure and the arrangement of atoms along the surface of nanostructured material will determine most of its physical properties. In general, electronic structure ultimately determines the properties of matter. Soft X-ray spectroscopy has some basic features that are important to consider. X-ray is originating from an electronic transition between a localized core state and a valence state. As a core state is involved, elemental selectivity is obtained because the core levels of different elements are well separated in energy, meaning that the involvement of the inner level makes this probe localized to one specific atomic site around which the electronic structure is reflected as a partial density-of-states contribution. The participation of valence electrons gives the method chemical state sensitivity and further, the dipole nature of the transitions gives particular symmetry information. The new generation synchrotron radiation sources producing intensive tunable monochromatized soft X-ray beams have opened up new possibilities for soft X-ray spectroscopy. The introduction of selectively excited soft X-ray emission has opened a new field of study by disclosing many new possibilities of soft X-ray resonant inelastic scattering. In this paper, some recent findings regarding soft X-ray absorption and emission studies of various nanostructured systems are presented.

  15. Applications of soft x-ray lasers

    SciTech Connect

    Skinner, C.H.

    1993-08-01

    The high brightness and short pulse duration of soft x-ray lasers provide unique advantages for novel applications. Imaging of biological specimens using x-ray lasers has been demonstrated by several groups. Other applications to fields such as chemistry, material science, plasma diagnostics, and lithography are beginning to emerge. We review the current status of soft x-ray lasers from the perspective of applications, and present an overview of the applications currently being developed.

  16. Reaction cell for in situ soft x-ray absorption spectroscopy and resonant inelastic x-ray scattering measurements of heterogeneous catalysis up to 1 atm and 250 °C

    SciTech Connect

    Kristiansen, P. T.; Rocha, T. C. R.; Knop-Gericke, A.; Guo, J. H.; Duda, L. C.

    2013-11-15

    We present a novel in situ reaction cell for heterogeneous catalysis monitored in situ by x-ray absorption spectroscopy (XAS) and resonant inelastic x-ray scattering (RIXS). The reaction can be carried out at a total pressure up to 1 atm, a regime that has not been accessible to comparable in situ techniques and thus closes the pressure gap to many industrial standard conditions. Two alternate catalyst geometries were tested: (A) a thin film evaporated directly onto an x-ray transparent membrane with a flowing reaction gas mixture behind it or (B) a powder placed behind both the membrane and a gap of flowing reaction gas mixture. To illustrate the working principle and feasibility of our reaction cell setup we have chosen ethylene epoxidation over a silver catalyst as a test case. The evolution of incorporated oxygen species was monitored by total electron/fluorescence yield O K-XAS as well as O K-RIXS, which is a powerful method to separate contributions from inequivalent sites. We find that our method can reliably detect transient species that exist during catalytic reaction conditions that are hardly accessible using other spectroscopic methods.

  17. Theory of time-resolved inelastic x-ray diffraction

    SciTech Connect

    Lorenz, Ulf; Moeller, Klaus B.; Henriksen, Niels E.

    2010-02-15

    Starting from a general theory of time-resolved x-ray scattering, we derive a convenient expression for the diffraction signal based on a careful analysis of the relevant inelastic scattering processes. We demonstrate that the resulting inelastic limit applies to a wider variety of experimental conditions than similar, previously derived formulas, and it directly allows the application of selection rules when interpreting diffraction signals. Furthermore, we present a simple extension to systems simultaneously illuminated by x rays and a laser beam.

  18. Resonant Soft X-ray Scattering for Soft Materials

    NASA Astrophysics Data System (ADS)

    Wang, Cheng; Young, Athony; Hexemer, Alexander; Padmore, Howard

    2015-03-01

    Over the past a few years, we have developed Resonant Soft X-ray Scattering (RSoXS) and constructed the first dedicated resonant soft x-ray scattering beamline at the Advanced Light Source, LBNL. RSoXS combines soft x-ray spectroscopy with x-ray scattering thus offers statistical information for 3D chemical morphology over a large length scale range from nanometers to micrometers. Its unique chemical sensitivity, large accessible size scale, molecular bond orientation sensitivity with polarized x-rays and high coherence have shown great potential for chemical/morphological structure characterization for many classes of materials. Some recent development of in-situ soft x-ray scattering with in-vacuum sample environment will be discussed. In order to study sciences in naturally occurring conditions, we need to overcome the sample limitations set by the low penetration depth of soft x-rays and requirement of high vacuum. Adapting to the evolving environmental cell designs utilized increasingly in the Electron Microscopy community, customized designed liquid/gas environmental cells will enable soft x-ray scattering experiments on biological, electro-chemical, self-assembly, and hierarchical functional systems in both static and dynamic fashion. Recent RSoXS results on organic electronics, block copolymer thin films, and membrane structure will be presented.

  19. European XFEL: Soft X-Ray instrumentation

    SciTech Connect

    Molodtsov, S. L.

    2011-12-15

    The currently constructed European X-Ray Free Electron Laser (XFEL) will generate new knowledge in almost all the technical and scientific disciplines that are shaping our daily life-including nanotechnology, medicine, pharmaceutics, chemistry, materials science, power engineering and electronics. On 8 January 2009, civil engineering work (tunnels, shafts, halls) has been started at all three construction sites. In this presentation status and parameters of the European XFEL facility and instrumentation as well as planned research applications particularly in the range of soft X-rays are reviewed.

  20. Reflection soft X-ray microscope and method

    DOEpatents

    Suckewer, S.; Skinner, C.H.; Rosser, R.

    1993-01-05

    A reflection soft X-ray microscope is provided by generating soft X-ray beams, condensing the X-ray beams to strike a surface of an object at a predetermined angle, and focusing the X-ray beams reflected from the surface onto a detector, for recording an image of the surface or near surface features of the object under observation.

  1. Reflection soft X-ray microscope and method

    DOEpatents

    Suckewer, Szymon; Skinner, Charles H.; Rosser, Roy

    1993-01-01

    A reflection soft X-ray microscope is provided by generating soft X-ray beams, condensing the X-ray beams to strike a surface of an object at a predetermined angle, and focusing the X-ray beams reflected from the surface onto a detector, for recording an image of the surface or near surface features of the object under observation.

  2. Soft x-ray laser microscope

    SciTech Connect

    Suckewer, P.I.

    1990-10-01

    The program consisted of two phases (Phase I and Phase II). The goal of the Phase I (first year program) was to design and construct the Soft X-ray Laser Contact Microscope. Such microscope was constructed and adapted to PPL's 18.2nm soft X-ray Laser (SXL), which in turn was modified and prepared for microscopy experiments. Investigation of the photoresist response to 18.2nm laser radiation and transmissivity of 0.1m thick silicion-nitride (Si[sub 3]N[sub 4]) windows were important initial works. The goal of the first year of Phase II was to construct X-ray contact microscope in combination with existing optical phase microscope, already used by biologists. In the second year of Phase II study of dehydrated Horeseshoe Crab and Hela cancer cells were performed with COXRALM. Also during Phase II, the Imaging X-Ray Laser Microscope (IXRALM) was designed and constructed. This paper describes the development of each of the microscopes and their application for research.

  3. Resonant Inelastic X-ray Scattering in Correlated Electron Systems

    NASA Astrophysics Data System (ADS)

    Kim, Young-June

    2006-03-01

    Extremely bright photons generated at the new generation of synchrotron light sources have made a huge impact on various scientific disciplines ranging from biology to materials science. One of the exciting new developments is the use of x-rays in the field of solid-state spectroscopy. Inelastic x-ray scattering, analogous to the well-known inelastic neutron scattering, is a powerful tool for studying momentum-dependent electronic excitations and phonons. In particular, resonant inelastic x-ray scattering in the hard x-ray regime has been widely utilized to study the momentum dependence of various electronic excitations in strongly correlated electron systems. For example, by tuning the incident photon energy to the Cu K-edge, one can gain a large intensity enhancement as well as element specific knowledge of the electronic excitations in various copper oxide compounds. Most of the work to date has been focused on the charge-transfer excitation between the bonding and antibonding molecular orbitals, the excitation across the Mott gap, and crystal field excitations between the d-orbitals. Recent improvements in instrumentation have allowed us to observe a new mode in the mid-infrared frequency region. We will discuss the momentum dependence of these excitations in prototypical cuprate superconductors, La2-xSrxCuO4, and also examine the evolution of such excitations as charge carriers are doped into the system.

  4. Surface recombination effects in soft X-ray efficiencies

    NASA Astrophysics Data System (ADS)

    Benitez, E. L.; Husk, D. E.; Tarrio, C.; Schnatterly, S. E.

    1991-07-01

    The soft X-ray efficiencies of a silicon p-i-n photodiode and an La2O2S:Tm phosphor were measured over a broad energy range. Also, the inelastic electron scattering spectra of the constituent materials were measured and values of optical absorption coefficients versus energy were obtained. The energy dependence of the efficiencies is well explained by a model based on surface recombination of electron hole pairs, and the quality of data which can now be obtained from synchrotrons makes possible quantitative fits from which diffusion length, surface recombination velocity, and bulk quantum efficiency are obtained.

  5. New soft x-ray emission spectrograph

    NASA Astrophysics Data System (ADS)

    Carson, R. D.; Franck, C. P.; Schnatterly, S.; Zutavern, F.

    1984-12-01

    We have built a new soft x-ray emission spectrograph covering the photon energy range 20-800 eV. It incorporates toroidal holographic grazing incidence diffraction gratings and a position-sensitive photodiode array as a detector. The detector electronics are remote from the array which is under vacuum at nitrogen temperature, and features a double-correlated sampling scheme. The sample is excited with a Pierce-type electron gun using a quadrupole focusing lens. The performance of the instrument is described.

  6. Inelastic X-ray Scattering from Shocked Liquid Deuterium

    SciTech Connect

    Regan, S. P.; Falk, K.; Gregori, G.; Radha, P. B.; Hu, S. X.; Boehly, T. R.; Crowley, B.; Glenzer, S. H.; Landen, O.; Gericke, D. O.; Doeppner, T.; Meyerhofer, D. D.; Murphy, C. D.; Sangster, T. C.; Vorberger, J.

    2012-12-28

    The Fermi-degenerate plasma conditions created in liquid deuterium by a laser-ablation—driven shock wave were probed with noncollective, spectrally resolved, inelastic x-ray Thomson scattering employing Cl Lyα line emission at 2.96 keV. Thus, these first x-ray Thomson scattering measurements of the microscopic properties of shocked deuterium show an inferred spatially averaged electron temperature of 8±5 eV, an electron density of 2.2(±0.5)×1023 cm-3, and an ionization of 0.8 (-0.25, +0.15). Our two-dimensional hydrodynamic simulations using equation-of-state models suited for the extreme parameters occurring in inertial confinement fusion research and planetary interiors are consistent with the experimental results.

  7. Inelastic X-ray Scattering from Shocked Liquid Deuterium

    DOE PAGES

    Regan, S. P.; Falk, K.; Gregori, G.; Radha, P. B.; Hu, S. X.; Boehly, T. R.; Crowley, B.; Glenzer, S. H.; Landen, O.; Gericke, D. O.; et al

    2012-12-28

    The Fermi-degenerate plasma conditions created in liquid deuterium by a laser-ablation—driven shock wave were probed with noncollective, spectrally resolved, inelastic x-ray Thomson scattering employing Cl Lyα line emission at 2.96 keV. Thus, these first x-ray Thomson scattering measurements of the microscopic properties of shocked deuterium show an inferred spatially averaged electron temperature of 8±5 eV, an electron density of 2.2(±0.5)×1023 cm-3, and an ionization of 0.8 (-0.25, +0.15). Our two-dimensional hydrodynamic simulations using equation-of-state models suited for the extreme parameters occurring in inertial confinement fusion research and planetary interiors are consistent with the experimental results.

  8. Superconducting pairing in resonant inelastic x-ray scattering

    NASA Astrophysics Data System (ADS)

    Shi, Yifei; Benjamin, David; Demler, Eugene; Klich, Israel

    2016-09-01

    We develop a method to study the effect of the superconducting transition on the resonant inelastic x-ray scattering (RIXS) signal in superconductors with an order parameter with an arbitrary symmetry within a quasiparticle approach. As an example, we compare the direct RIXS signal below and above the superconducting transition for p -wave-type order parameters. For a p -wave order parameter with a nodal line, we show that, counterintuitively, the effect of the gap is most noticeable for momentum transfers in the nodal direction. This phenomenon may be naturally explained as a type of nesting effect.

  9. Technology development for soft X-ray spectroscopy

    NASA Astrophysics Data System (ADS)

    Törmä, P. T.; Sipilä, H. J.; Koskinen, T.; Mattila, M.

    2016-05-01

    X-ray spectroscopy instruments lose part of their performance due to the lack of suitable components for soft X-ray region below 1 keV. Therefore, in the analysis of low atomic number elements including lithium, beryllium, boron and carbon instrument sensitivity is often limited. In this work we describe how the performance of the spectroscopy of soft X-rays is significantly improved when all devices integrated in the spectroscopic instrument are suitable for both soft and hard X-rays. This concept is based on utilizing ultra-thin SiN X-ray windows with proven performance not only as a detector window but also as an X-ray source window. By including a soft-X-ray-sensitive silicon drift detector with efficient surface charge collection in this concept the sensitivity and performance of the instrument is significantly increased.

  10. Tunable Soft X-Ray Oscillators

    SciTech Connect

    Wurtele, Jonathan; Gandhi, Punut; Gu, X-W; Fawley, William M; Reinsch, Matthia; Penn, Gregory; Kim, K-J; Lindberg, Ryan; Zholents, Alexander

    2010-09-17

    A concept for a tunable soft x-ray free electron laser (FEL) photon source is presented and studied numerically. The concept is based on echo-enabled harmonic generation (EEHG), wherein two modulator-chicane sections impose high harmonic structure with much greater efficacy as compared to conventional high harmonic FELs that use only one modulator-chicane section. The idea proposed here is to replace the external laser power sources in the EEHG modulators with FEL oscillators, and to combine the bunching of the beam with the production of radiation. Tunability is accomplished by adjusting the magnetic chicanes while the two oscillators remain at a fixed frequency. This scheme eliminates the need to develop coherent sources with the requisite power, pulse length, and stability requirements by exploiting the MHz bunch repetition rates of FEL continuous wave (CW) sources driven by superconducting (SC) linacs. We present time-dependent GINGER simulation results for an EEHG scheme with an oscillator modulator at 43 nm employing 50percent reflective dielectric mirrors and a second modulator employing an external, 215-nm drive laser. Peak output of order 300 MW is obtained at 2.7 nm, corresponding to the 80th harmonic of 215 nm. An alternative single-cavity echo-oscillator scheme based on a 13.4 nm oscillator is investigated with time-independent simulations that a 180-MW peak power at final wavelength of 1.12 nm. Three alternate configurations that use separate bunches to produce the radiation for EEHG microbunching are also presented. Our results show that oscillator-based soft x-ray FELs driven by CWSC linacs are extremely attractive because of their potential to produce tunable radiation at high average power together with excellent longitudinal coherence and narrow spectral bandwidth.

  11. Effects of Galactic absorption on soft X-ray surveys

    NASA Technical Reports Server (NTRS)

    Zamorani, G.; Gioia, I. M.; Maccacaro, T.; Wolter, A.

    1988-01-01

    A bias in the spectral distribution of X-ray sources detected in X-ray surveys is discussed which is due to the combination of the intrinsic characteristics of X-ray telescopes and the effects of low-energy photoelectric absorption within the Galaxy. A statistical method for obtaining information on the average spectrum of X-ray sources detected in well-defined surveys is presented. This method can be applied to surveys performed with X-ray telescopes working at relatively soft X-ray energies, such as Einstein, Exosat, and Rosat.

  12. Dante Soft X-ray Power Diagnostic for NIF

    SciTech Connect

    Dewald, E; Campbell, K; Turner, R; Holder, J; Landen, O; Glenzer, S; Kauffman, R; Suter, L; Landon, M; Rhodes, M; Lee, D

    2004-04-15

    Soft x-ray power diagnostics are essential for measuring spectrally resolved the total x-ray flux, radiation temperature, conversion efficiency and albedo that are important quantities for the energetics of indirect drive hohlraums. At the Nova or Omega Laser Facilities, these measurements are performed mainly with Dante, but also with DMX and photo-conductive detectors (PCD's). The Dante broadband spectrometer is a collection of absolute calibrated vacuum x-ray diodes, thin filters and x-ray mirrors used to measure the soft x-ray emission for photon energies above 50 eV.

  13. CHEMICAL APPLICATIONS OF INELASTIC X-RAY SCATTERING

    SciTech Connect

    HAYASHI,H.; UDAGAWA,Y.; GILLET,J.M.; CALIEBE,W.A.; KAO,C.C.

    2001-08-01

    Inelastic x-ray scattering (IXS), complementary to other more established inelastic scattering probes, such as light scattering, electron scattering, and neutron scattering, is becoming an important experimental technique in the study of elementary excitations in condensed matters. Over the past decade, IXS with total energy resolution of few meV has been achieved, and is being used routinely in the study of phonon dispersions in solids and liquids as well as dynamics in disordered and biological systems. In the study of electronic excitations, IXS with total energy resolution on the order of 100 meV to 1 eV is gaining wider applications also. For example, IXS has been used to study collective excitations of valence electrons, single electron excitations of valence electrons, as well as core electron excitations. In comparison with the alternative scattering techniques mentioned above, IXS has several advantages. First, IXS probes the full momentum transfer range of the dielectric response of the sample, whereas light scattering is limited to very small momentum transfers, and electron scattering suffers the effects of multiple scattering at large momentum transfers. Second, since IXS measures the bulk properties of the sample it is not surface sensitive, therefore it does not require special preparation of the sample. The greater flexibility in sample conditions and environments makes IXS an ideal probe in the study of liquids and samples under extreme temperature, pressure, and magnetic field. Third, the tunability of synchrotron radiation sources enables IXS to exploit element specificity and resonant enhancement of scattering cross sections. Fourth, IXS is unique in the study of dynamics of liquids and amorphous solids because it can probe the particular region of energy-momentum transfer phase space, which is inaccessible to inelastic neutron scattering. On the other hand, the main disadvantages of IXS are the small cross sections and the strong absorption of

  14. Inelastic X-ray Scattering Studies of Zeolite Collapse

    SciTech Connect

    Greaves, G. Neville; Kargl, Florian; Ward, David; Holliman, Peter; Meneau, Florian

    2009-01-29

    In situ inelastic x-ray scattering (IXS) experiments have been used to probe heterogeneity and deformability in zeolte Y as this thermally collapses to a high density amorphous (HDA) aluminosilicate phase. The Landau-Placzek ratio R{sub LP} falls slowly as amorphisation advances, increasing in the later stages of collapse clearly showing how homogeneity improves non-linearly--behaviour linked closely with the decline in molar volume V{sub Molar}. The Brillouin frequency {omega}{sub Q} also decreases with amorphisation in a similar fashion, signifying a non-uniform decrease in the speed of sound v{sub l}. All of these changes with zeolite amorphisation infer formation of an intermediate low density amorphous (LDA) phase. This low entropy or 'perfect glass' has mechanical properties which are closer to the zeolite rather to the HDA glass--notably a very small value of Poisson's Ratio signifying unusually low resistance to deformation.

  15. The Origin of Soft X-rays in DQ Herculis

    NASA Technical Reports Server (NTRS)

    White, Nicholas E. (Technical Monitor); Mukai, K.; Still, M.; Ringwald, F. A.

    2002-01-01

    DQ Herculis (Nova Herculis 1934) is a deeply eclipsing cataclysmic variable containing a magnetic white dwarf primary. The accretion disk is thought to block our line of sight to the white dwarf at all orbital phases due to its extreme inclination angle. Nevertheless, soft X-rays were detected from DQ Her with ROSAT PSPC. To probe the origin of these soft X-rays, we have performed Chandra ACIS observations. We confirm that DQ Her is an X-ray source. The bulk of the X-rays are from a point-like source and exhibit a shallow partial eclipse. We interpret this as due to scattering of the unseen central X-ray source, probably in an accretion disk wind. At the same time, we detect weak extended X-ray features around DQ Her, which we interpret as an X-ray emitting knot in the nova shell.

  16. The hard X-ray perspective on the soft X-ray excess

    SciTech Connect

    Vasudevan, Ranjan V.; Mushotzky, Richard F.; Reynolds, Christopher S.; Lohfink, Anne M.; Zoghbi, Abderahmen; Fabian, Andrew C.; Gallo, Luigi C.; Walton, Dominic

    2014-04-10

    The X-ray spectra of many active galactic nuclei exhibit a 'soft excess' below 1 keV, whose physical origin remains unclear. Diverse models have been suggested to account for it, including ionized reflection of X-rays from the inner part of the accretion disk, ionized winds/absorbers, and Comptonization. The ionized reflection model suggests a natural link between the prominence of the soft excess and the Compton reflection hump strength above 10 keV, but it has not been clear what hard X-ray signatures, if any, are expected from the other soft X-ray candidate models. Additionally, it has not been possible up until recently to obtain high-quality simultaneous measurements of both soft and hard X-ray emission necessary to distinguish these models but upcoming joint XMM-NuSTAR programs provide precisely this opportunity. In this paper, we present an extensive analysis of simulations of XMM-NuSTAR observations, using two candidate soft excess models as inputs, to determine whether such campaigns can disambiguate between them by using hard and soft X-ray observations in tandem. The simulated spectra are fit with the simplest 'observer's model' of a blackbody and neutral reflection to characterize the strength of the soft and hard excesses. A plot of the strength of the hard excess against the soft excess strength provides a diagnostic plot which allows the soft excess production mechanism to be determined in individual sources and samples using current state-of-the-art and next generation hard X-ray enabled observatories. This approach can be straightforwardly extended to other candidate models for the soft excess.

  17. Soft x-ray scattering using FEL radiation for probing near-solid density plasmas at few electronvolt temperatures

    SciTech Connect

    Toleikis, S; Faustlin, R R; Cao, L; Doppner, T; Dusterer, S; Forster, E; Fortmann, C; Glenzer, S H; Gode, S; Gregori, G; Irsig, R; Laarmann, T; Lee, H J; Li, B; Meiwes-Broer, K; Przystawik, A; Radcliffe, P; Redmer, R; Tavella, F; Thiele, R; Tiggesbaumker, J; Truong, N X; Uschmann, I; Zastrau, U; Tschentscher, T

    2009-03-03

    We report on soft x-ray scattering experiments on cryogenic hydrogen and simple metal targets. As a source of intense and ultrashort soft x-ray pulses we have used free-electron laser radiation at 92 eV photon energy from FLASH at DESY, Hamburg. X-ray pulses with energies up to 100 {micro}J and durations below 50 fs provide interaction with the target leading simultaneously to plasma formation and scattering. Experiments exploiting both of these interactions have been carried out, using the same experimental setup. Firstly, recording of soft x-ray inelastic scattering from near-solid density hydrogen plasmas at few electronvolt temperatures confirms the feasibility of this diagnostics technique. Secondly, the soft x-ray excitation of few electronvolt solid-density plasmas in simple metals could be studied by recording soft x-ray line and continuum emission integrated over emission times from fs to ns.

  18. Soft X-ray telescope (SXRT)

    NASA Technical Reports Server (NTRS)

    Moore, R.

    1986-01-01

    The soft X-ray telescope (SXRT) will provide direct images of the solar corona with spatial resolution of about 1 arcsecond. These images will show the global structure of the corona, the location and area of coronal holes, and the presence of even the smallest active regions and flares. The good spatial resolution will show the fine scale magnetic structure and changes in these phenomena. These observations are essential for monitoring, predicting, and understanding the solar magnetic cycle, coronal heating, solar flares, coronal mass ejections, and the solar wind. These observations complement those of the White Light Coronagraph and Ultra-Violet Coronal Spectrometer; the SXRT will detect active regions and coronal holes near the east limb, thereby giving a week or more of advanced warning for disturbed geomagnetic conditions at Earth. The instrument consists of a grazing incidence collecting mirror with a full-disk film camera at the primary focus, and a secondary relay optic that feeds a CCD camera with a field of view about the size of an average active region.

  19. Soft X-Ray Telescope (SXRT)

    NASA Technical Reports Server (NTRS)

    Moore, R. L.

    1985-01-01

    The soft X-ray telescope (SXRT) will provide direct images of the solar corona with spatial resolution of about 1 arcsecond. These images will show the global structure of the corona, the location and area of coronal holes, and the presence of even the smallest active regions and flares. The good spatial resolution will show the fine scale magnetic structure and changes in these phenomena. These observations are essential for monitoring, predicting, and understanding the solar magnetic cycle, coronal heating, solar flares, coronal mass ejections, and the solar wind. These observations complement those of the White Light Coronagraph and Ultra-Violet Coronal Spectrometer; the SXRT will detect active regions and coronal holes near the east limb, thereby giving a week or more of advanced warning for disturbed geomagnetic conditions at Earth. The instrument consists of a grazing incidence collecting mirror with a full disk film camera at the primary focus, and a secondary relay optic that feeds a CCD camera with a field of view about the size of an average active region.

  20. Moon: lunar albedo for soft x-rays

    NASA Astrophysics Data System (ADS)

    Ibadov, Subhon

    2016-07-01

    Albedo of the Moon for soft X-rays (0.1-2 keV photons) is determined on the basis of the X-ray luminosity of the Moon detected and measured for the first time by orbital space telescope ROSAT in 1990. It is found that the lunar albedo for the solar soft X-rays is less than the lunar visual region albedo almost thousand times. The data allow to estimate more correctly X-ray luminosity of dusty comets like Hyakutake C/1996 B2 and Hale-Bopp C/1995 O1 due to scattering of solar soft X-rays and to reveal thus the dominant mechanism for production of X-rays in dusty comets.

  1. Multilayers for EUV, soft x-ray and x-ray optics

    NASA Astrophysics Data System (ADS)

    Wang, Zhanshan; Huang, Qiushi; Zhang, Zhong

    2016-02-01

    Driven by the requirements in synchrotron radiation applications, astronomical observation, and dense plasma diagnostics, the EUV, soft X-rays and X-rays multilayer optics have been tremendously developed. Based on the LAMP project for soft X-ray polarimetry, Co/C and Cr/C multilayers have been fabricated and characterized. Both Co/C and Cr/C multilayers reveal good optical performance working at 250 eV. Pd/Y multilayers have been successfully fabricated using reactive sputtering with nitrogen working at around 9.4 nm. EUV normal incidence Schwarzschild and soft X-ray grazing incidence KB microscopes were developed for ICF plasma diagnostics. This paper covers the outline of the multilayer optics and the current status in our lab.

  2. Soft X-Ray Absorption Spectroscopy at an X-ray Free Electron Laser

    NASA Astrophysics Data System (ADS)

    Higley, Daniel; Schlotter, William; Turner, Joshua; Moeller, Stefan; Mitra, Ankush; Tsukamoto, Arata; Marvel, Robert; Haglund, Richard; Durr, Hermann; Stohr, Joachim; Dakovski, Georgi

    2015-03-01

    X-ray free electron lasers, providing coherent, ultrafast, high intensity x-ray pulses, have enabled groundbreaking scattering experiments to probe the atomic structure of materials on femtosecond timescales. Nonetheless, x-ray absorption spectroscopy (XAS), one of the most fundamental and common x-ray techniques practiced at synchrotron light sources, has proven challenging to conduct with satisfactory signal-to-noise levels at soft x-ray energies using free electron laser sources. The ability to routinely collect high quality XAS spectra, especially in a time-resolved manner, will open many new scientific possibilities in the areas of ultrafast demagnetization, phase transitions and chemical dynamics to highlight a few. Here, we report how XAS using total fluorescence yield detection yields high signal-to-noise x-ray absorption spectra at an x-ray free electron laser source. Data were collected over multiple absorption edges on technologically relevant materials. These measurements were recorded on the Soft X-Ray Materials Science instrument at the Linac Coherent Light Source. The results are easily extendable to time-resolved measurements.

  3. Phase Resolved X-ray Spectral Analysis of Soft IPs

    NASA Astrophysics Data System (ADS)

    Pekon, Yakup

    2016-07-01

    As a subclass of Cataclysmic Variables, Intermediate Polars (IPs) are magnetic systems which mainly show hard X-ray emission. However, there have been an increasing number of systems that also show a soft emission component arising from reprocessed X-rays from the white dwarf limbs. Due to their relatively short periods, they pose as good canditates to perform phase resolved analysis. In this work, X-ray phase resolved spectral analysis of selected IPs with soft X-ray emission components (such as PQ Gem, V2069 Cyg etc.) over the orbital and/or spin periods will be presented. The analyses will help a better understanding of the complex absorption mechanisms and the nature of the soft X-ray emissions in soft IPs.

  4. Hard X-Ray, Soft X-Ray, and EUV Studies of Solar Eruptions

    NASA Technical Reports Server (NTRS)

    Sterling, Alphonse C.; Wagner, William (Technical Monitor)

    2003-01-01

    Document study the hard X-ray (HXR), soft X-ray (SXR) ,EUV, and magnetic nature of solar eruptions, with the objective of elucidating the physics of the eruption process. In particular, it was examine the viability of two specific eruption mechanisms, detailed in our proposal. These mechanisms are the "breakout model", and the "tether cutting model". During the second year, it was a significant progress in the goals to Data Sets Utilized. In the publications during this second year of the grant period, the data was used from the E W Imaging Telescope (EIT) and the Michelson Doppler Imager (MDI) instruments on SOHO, and from the Soft X-ray Telescope (SXT), Hard X-ray Telescope (HXT), and the Bragg Crystal Spectrometer (BCS) on Yooh.

  5. Soft-X-Ray Prefilter for Hot, Bright Objects

    NASA Technical Reports Server (NTRS)

    Davis, J. M.; Ortendahl, J. A.

    1985-01-01

    Prefilters consisting of beryllium foil supported on conductive silver mesh transmit soft x-rays but are nearly opaque to visible and infrared light. New Be/AG filters protect imaging X-ray detectors from damage by visible and longer wavelength radiation when viewing such hot, bright emitters as Sun or possibly certain industrial processes.

  6. HERMES: a soft X-ray beamline dedicated to X-ray microscopy.

    PubMed

    Belkhou, Rachid; Stanescu, Stefan; Swaraj, Sufal; Besson, Adrien; Ledoux, Milena; Hajlaoui, Mahdi; Dalle, Didier

    2015-07-01

    The HERMES beamline (High Efficiency and Resolution beamline dedicated to X-ray Microscopy and Electron Spectroscopy), built at Synchrotron SOLEIL (Saint-Auban, France), is dedicated to soft X-ray microscopy. The beamline combines two complementary microscopy methods: XPEEM (X-ray Photo Emitted Electron Microscopy) and STXM (Scanning Transmission X-ray Microscopy) with an aim to reach spatial resolution below 20 nm and to fully exploit the local spectroscopic capabilities of the two microscopes. The availability of the two methods within the same beamline enables the users to select the appropriate approach to study their specific case in terms of sample environment, spectroscopy methods, probing depth etc. In this paper a general description of the beamline and its design are presented. The performance and specifications of the beamline will be reviewed in detail. Moreover, the article is aiming to demonstrate how the beamline performances have been specifically optimized to fulfill the specific requirements of a soft X-ray microscopy beamline in terms of flux, resolution, beam size etc. Special attention has been dedicated to overcome some limiting and hindering problems that are usually encountered on soft X-ray beamlines such as carbon contamination, thermal stability and spectral purity.

  7. Resonant inelastic x-ray scattering in a Mott insulator

    NASA Astrophysics Data System (ADS)

    Pakhira, Nandan; Freericks, J. K.; Shvaika, A. M.

    2012-09-01

    We calculate the resonant inelastic x-ray scattering (RIXS) response in a Mott insulator, which is described by the Falicov-Kimball model. The model can be solved exactly within the single site dynamical mean-field theory (DMFT) approximation and the RIXS response can also be calculated accurately up to a local background correction. We find that on resonance the RIXS response is greatly enhanced. The response systematically evolves from a single-peak structure, arising due to relaxation processes within the lower Hubbard band, to a two-peak structure, arising due to relaxation processes within the upper Hubbard band and across the Mott gap into the lower Hubbard band. This occurs as we vary the incident photon frequency to allow excitations from the lower Hubbard band to the upper Hubbard band. The charge transfer excitations are found to disperse monotonically as we go from the center of the Brillouin zone towards the zone corner. These correlation-induced features have been observed by Hasan [Science0036-807510.1126/science.288.5472.1811 288, 1811 (2000)] and many other experimentalists in RIXS measurements over various transition-metal oxide compounds. They are found to be robust and survive even for large Auger lifetime broadening effects that can mask the many-body effects by smearing out spectral features. As a comparison, we also calculate the dynamic structure factor for this model, which is proportional to the nonresonant part of the response, and does not show these specific signatures.

  8. Ground state potential energy surfaces around selected atoms from resonant inelastic x-ray scattering

    NASA Astrophysics Data System (ADS)

    Schreck, Simon; Pietzsch, Annette; Kennedy, Brian; Såthe, Conny; Miedema, Piter S.; Techert, Simone; Strocov, Vladimir N.; Schmitt, Thorsten; Hennies, Franz; Rubensson, Jan-Erik; Föhlisch, Alexander

    2016-01-01

    Thermally driven chemistry as well as materials’ functionality are determined by the potential energy surface of a systems electronic ground state. This makes the potential energy surface a central and powerful concept in physics, chemistry and materials science. However, direct experimental access to the potential energy surface locally around atomic centers and to its long-range structure are lacking. Here we demonstrate how sub-natural linewidth resonant inelastic soft x-ray scattering at vibrational resolution is utilized to determine ground state potential energy surfaces locally and detect long-range changes of the potentials that are driven by local modifications. We show how the general concept is applicable not only to small isolated molecules such as O2 but also to strongly interacting systems such as the hydrogen bond network in liquid water. The weak perturbation to the potential energy surface through hydrogen bonding is observed as a trend towards softening of the ground state potential around the coordinating atom. The instrumental developments in high resolution resonant inelastic soft x-ray scattering are currently accelerating and will enable broad application of the presented approach. With this multidimensional potential energy surfaces that characterize collective phenomena such as (bio)molecular function or high-temperature superconductivity will become accessible in near future.

  9. Ground state potential energy surfaces around selected atoms from resonant inelastic x-ray scattering

    PubMed Central

    Schreck, Simon; Pietzsch, Annette; Kennedy, Brian; Såthe, Conny; Miedema, Piter S.; Techert, Simone; Strocov, Vladimir N.; Schmitt, Thorsten; Hennies, Franz; Rubensson, Jan-Erik; Föhlisch, Alexander

    2016-01-01

    Thermally driven chemistry as well as materials’ functionality are determined by the potential energy surface of a systems electronic ground state. This makes the potential energy surface a central and powerful concept in physics, chemistry and materials science. However, direct experimental access to the potential energy surface locally around atomic centers and to its long-range structure are lacking. Here we demonstrate how sub-natural linewidth resonant inelastic soft x-ray scattering at vibrational resolution is utilized to determine ground state potential energy surfaces locally and detect long-range changes of the potentials that are driven by local modifications. We show how the general concept is applicable not only to small isolated molecules such as O2 but also to strongly interacting systems such as the hydrogen bond network in liquid water. The weak perturbation to the potential energy surface through hydrogen bonding is observed as a trend towards softening of the ground state potential around the coordinating atom. The instrumental developments in high resolution resonant inelastic soft x-ray scattering are currently accelerating and will enable broad application of the presented approach. With this multidimensional potential energy surfaces that characterize collective phenomena such as (bio)molecular function or high-temperature superconductivity will become accessible in near future. PMID:26821751

  10. Ground state potential energy surfaces around selected atoms from resonant inelastic x-ray scattering.

    PubMed

    Schreck, Simon; Pietzsch, Annette; Kennedy, Brian; Såthe, Conny; Miedema, Piter S; Techert, Simone; Strocov, Vladimir N; Schmitt, Thorsten; Hennies, Franz; Rubensson, Jan-Erik; Föhlisch, Alexander

    2016-01-01

    Thermally driven chemistry as well as materials' functionality are determined by the potential energy surface of a systems electronic ground state. This makes the potential energy surface a central and powerful concept in physics, chemistry and materials science. However, direct experimental access to the potential energy surface locally around atomic centers and to its long-range structure are lacking. Here we demonstrate how sub-natural linewidth resonant inelastic soft x-ray scattering at vibrational resolution is utilized to determine ground state potential energy surfaces locally and detect long-range changes of the potentials that are driven by local modifications. We show how the general concept is applicable not only to small isolated molecules such as O2 but also to strongly interacting systems such as the hydrogen bond network in liquid water. The weak perturbation to the potential energy surface through hydrogen bonding is observed as a trend towards softening of the ground state potential around the coordinating atom. The instrumental developments in high resolution resonant inelastic soft x-ray scattering are currently accelerating and will enable broad application of the presented approach. With this multidimensional potential energy surfaces that characterize collective phenomena such as (bio)molecular function or high-temperature superconductivity will become accessible in near future.

  11. Soft x-ray reduction camera for submicron lithography

    DOEpatents

    Hawryluk, A.M.; Seppala, L.G.

    1991-03-26

    Soft x-ray projection lithography can be performed using x-ray optical components and spherical imaging lenses (mirrors), which form an x-ray reduction camera. The x-ray reduction is capable of projecting a 5x demagnified image of a mask onto a resist coated wafer using 4.5 nm radiation. The diffraction limited resolution of this design is about 135 nm with a depth of field of about 2.8 microns and a field of view of 0.2 cm[sup 2]. X-ray reflecting masks (patterned x-ray multilayer mirrors) which are fabricated on thick substrates and can be made relatively distortion free are used, with a laser produced plasma for the source. Higher resolution and/or larger areas are possible by varying the optic figures of the components and source characteristics. 9 figures.

  12. Soft x-ray reduction camera for submicron lithography

    DOEpatents

    Hawryluk, Andrew M.; Seppala, Lynn G.

    1991-01-01

    Soft x-ray projection lithography can be performed using x-ray optical components and spherical imaging lenses (mirrors), which form an x-ray reduction camera. The x-ray reduction is capable of projecting a 5x demagnified image of a mask onto a resist coated wafer using 4.5 nm radiation. The diffraction limited resolution of this design is about 135 nm with a depth of field of about 2.8 microns and a field of view of 0.2 cm.sup.2. X-ray reflecting masks (patterned x-ray multilayer mirrors) which are fabricated on thick substrates and can be made relatively distortion free are used, with a laser produced plasma for the source. Higher resolution and/or larger areas are possible by varying the optic figures of the components and source characteristics.

  13. An imaging photoemission polarimeter for soft X-rays

    NASA Technical Reports Server (NTRS)

    Kaaret, Philip; Novick, Robert; Heckler, A.; Shaw, P.; Fraser, G. W.

    1990-01-01

    Results of investigations are reviewed to assess the polarization dependence of photoemission in the optical, UV, and soft X-ray bands, as well as present a design for an imaging photoelectric polarimeter. Data regarding the effect of the dependence in the soft X-ray band are emphasized including the quantity of photons produced by each X-ray. The phase shift encountered in some experiments indicates that a third axis is present; the importance of the phase shift in understanding the vectoral photoeffect is emphasized. Measurements of the pulse height show that this measure is proportional to the number of electrons photoemitted by the incident X-ray. The development of X-ray polarimeters can be significantly improved as a result of the study of polarization sensitivity in the photoelectric effect. The design of a photoelectric polarimeter is presented, and the potential uses for the instrument include measuring the polarization of supernova remnants, AGN, and black hole candidates.

  14. Resonant soft X-ray scattering on protein solutions

    NASA Astrophysics Data System (ADS)

    Ye, Dan; Le, Thinh; Wang, Cheng; Zwart, Peter; Gomez, Esther; Gomez, Enrique

    Protein structure is crucial for biological function, such that characterizing protein folding and packing is important for the design of therapeutics and enzymes. We propose resonant soft X-ray scattering (RSOXS) as an approach to study proteins and other biological assemblies in solution. Calculations of the scattering contrast suggest that soft X-ray scattering is more sensitive than hard X-ray scattering, because of contrast generated at the absorption edges of constituent elements such as carbon, nitrogen and oxygen. We have examined the structure of bovine serum albumin (BSA) in solution by RSOXS. We find that by varying incident X-ray energies, we are able to achieve higher scattering contrast near the absorption edge. From our RSOXS scattering result we are able to reconstruct the structure of BSA in 3D. These RSOXS results also agree with hard X-ray experiments, including crystallographic data. Our study demonstrates the potential of RSOXS for studying protein structure in solution.

  15. Soft X-Ray Emissions from Planets and Moons

    NASA Technical Reports Server (NTRS)

    Bhardwaj, A.; Gladstone, G. R.; Elsner, R. F.; Waite, J. H., Jr.; Grodent, D.; Cravens, T. E.; Howell, R. R.; Metzger, A. E.; Ostgaard, N.; Maurellis, A.; Six, N. Frank (Technical Monitor)

    2002-01-01

    A wide variety of solar system planetary bodies are now known to radiate in the soft x-ray energy (<5 keV) regime. These include planets (Earth, Jupiter, Venus, Saturn): bodies having thick atmosphere and with/without intrinsic magnetic field; planetary satellites (Moon, Io, Europa, Ganymede): bodies with no/thin atmosphere; and comets and Io plasma torus: bodies having extended tenuous atmosphere. Several different mechanisms have been proposed to explain the generation of soft x-rays from these objects. whereas in the hard x-ray energy range (>10 keV) x-rays mainly result from electron bremsstrahlung process. In this paper we present a brief review of the x-ray observations on each of the planetary bodies and discuss their characteristics and proposed source mechanisms.

  16. X-Ray Emission from the Soft X-Ray Transient Aquila X-1

    NASA Technical Reports Server (NTRS)

    Tavani, Marco

    1998-01-01

    Aquila X-1 is the most prolific of soft X-ray transients. It is believed to contain a rapidly spinning neutron star sporadically accreting near the Eddington limit from a low-mass companion star. The interest in studying the repeated X-ray outbursts from Aquila X-1 is twofold: (1) studying the relation between optical, soft and hard X-ray emission during the outburst onset, development and decay; (2) relating the spectral component to thermal and non-thermal processes occurring near the magnetosphere and in the boundary layer of a time-variable accretion disk. Our investigation is based on the BATSE monitoring of Aquila X-1 performed by our group. We observed Aquila X-1 in 1997 and re-analyzed archival information obtained in April 1994 during a period of extraordinary outbursting activity of the source in the hard X-ray range. Our results allow, for the first time for this important source, to obtain simultaneous spectral information from 2 keV to 200 keV. A black body (T = 0.8 keV) plus a broken power-law spectrum describe accurately the 1994 spectrum. Substantial hard X-ray emission is evident in the data, confirming that the accretion phase during sub-Eddington limit episodes is capable of producing energetic hard emission near 5 x 10(exp 35) ergs(exp -1). A preliminary paper summarizes our results, and a more comprehensive account is being written. We performed a theoretical analysis of possible emission mechanisms, and confirmed that a non-thermal emission mechanism triggered in a highly sheared magnetosphere at the accretion disk inner boundary can explain the hard X-ray emission. An anticorrelation between soft and hard X-ray emission is indeed prominently observed as predicted by this model.

  17. The soft X-ray diffuse background

    NASA Technical Reports Server (NTRS)

    Mccammon, D.; Burrows, D. N.; Sanders, W. T.; Kraushaar, W. L.

    1982-01-01

    Maps of the diffuse X-ray background intensity covering essentially the entire sky with approx. 7 deg spatial resolution are presented for seven energy bands. The data were obtained on a series of ten sounding rocket flights conducted over a seven-year period. The different nature of the spatial distributions in different bands implies at least three distinct origins for the diffuse X-rays, none of which is well-understood. At energies or approx. 2000 eV, an isotropic and presumably extraglalactic 500 and 1000 eV, an origin which is at least partially galactic seems called for. At energies 284 eV, the observed intensity is anticorrelated with neutral hydrogen column density, but we find it unlikely that this anticorrelation is simply due to absorption of an extragalactic or halo source.

  18. Soft X-ray Polarimetry Development

    NASA Astrophysics Data System (ADS)

    Marshall, Herman; Schulz, Norbert S.; Heine, Sarah

    2016-07-01

    We present continued development of a telescope for measuring linear X-ray polarization over the 0.2-0.8 keV band. We employ multilayer-coated mirrors as Bragg reflectors at the Brewster angle. By matching to the dispersion of a spectrometer, one may take advantage of high multilayer reflectivities and achieve polarization modulation factors over 95%. We have constructed a source of polarized X-rays that operates at a wide range of energies with a selectable polarization angle. We will present results from measurements of new laterally graded multilayer mirrors and new gratings essential to the design. Finally, we will present a design for a small telescope for suborbital or orbital missions. A suborbital mission could measure the polarization of a blazar such as Mk 421 to 5-10 percent while an orbital version could measure the polarizations of neutron stars, active galactic nuclei, and blazars.

  19. A diffuse soft X-ray spectrometer

    NASA Technical Reports Server (NTRS)

    Mccammon, D.

    1981-01-01

    A design for a diffuse X-ray spectrometer utilizing Bragg reflection is described. The geometry has a very high throughput for a given physical size and allows simultaneous observation at all wavelengths within its range. Spectral resolving power is about 35 to 50. A similar unit equipped with thallium acid pthallate crystals will cover the 11 - 24 A-range with about half this throughput and twice the resolving power.

  20. X-ray induced dimerization of cinnamic acid: Time-resolved inelastic X-ray scattering study

    PubMed Central

    Inkinen, Juho; Niskanen, Johannes; Talka, Tuomas; Sahle, Christoph J.; Müller, Harald; Khriachtchev, Leonid; Hashemi, Javad; Akbari, Ali; Hakala, Mikko; Huotari, Simo

    2015-01-01

    A classic example of solid-state topochemical reactions is the ultraviolet-light induced photodimerization of α-trans-cinnamic acid (CA). Here, we report the first observation of an X-ray-induced dimerization of CA and monitor it in situ using nonresonant inelastic X-ray scattering spectroscopy (NRIXS). The time-evolution of the carbon core-electron excitation spectra shows the effects of two X-ray induced reactions: dimerization on a short time-scale and disintegration on a long time-scale. We used spectrum simulations of CA and its dimerization product, α-truxillic acid (TA), to gain insight into the dimerization effects. From the time-resolved spectra, we extracted component spectra and time-dependent weights corresponding to CA and TA. The results suggest that the X-ray induced dimerization proceeds homogeneously in contrast to the dimerization induced by ultraviolet light. We also utilized the ability of NRIXS for direct tomography with chemical-bond contrast to image the spatial progress of the reactions in the sample crystal. Our work paves the way for other time-resolved studies on chemical reactions using inelastic X-ray scattering. PMID:26568420

  1. X-ray induced dimerization of cinnamic acid: Time-resolved inelastic X-ray scattering study

    NASA Astrophysics Data System (ADS)

    Inkinen, Juho; Niskanen, Johannes; Talka, Tuomas; Sahle, Christoph J.; Müller, Harald; Khriachtchev, Leonid; Hashemi, Javad; Akbari, Ali; Hakala, Mikko; Huotari, Simo

    2015-11-01

    A classic example of solid-state topochemical reactions is the ultraviolet-light induced photodimerization of α-trans-cinnamic acid (CA). Here, we report the first observation of an X-ray-induced dimerization of CA and monitor it in situ using nonresonant inelastic X-ray scattering spectroscopy (NRIXS). The time-evolution of the carbon core-electron excitation spectra shows the effects of two X-ray induced reactions: dimerization on a short time-scale and disintegration on a long time-scale. We used spectrum simulations of CA and its dimerization product, α-truxillic acid (TA), to gain insight into the dimerization effects. From the time-resolved spectra, we extracted component spectra and time-dependent weights corresponding to CA and TA. The results suggest that the X-ray induced dimerization proceeds homogeneously in contrast to the dimerization induced by ultraviolet light. We also utilized the ability of NRIXS for direct tomography with chemical-bond contrast to image the spatial progress of the reactions in the sample crystal. Our work paves the way for other time-resolved studies on chemical reactions using inelastic X-ray scattering.

  2. Rapid soft X-ray fluctuations in solar flares observed with the X-ray polychromator

    NASA Technical Reports Server (NTRS)

    Zarro, D. M.; Saba, J. L. R.; Strong, K. T.

    1986-01-01

    Three flares observed by the Soft X-Ray Polychromator on the Solar Maximum Mission were studied. Flare light curves from the Flat Crystal Spectrometer and Bent Crystal Spectrometer were examined for rapid signal variations. Each flare was characterized by an initial fast (less than 1 min) burst, observed by the Hard X-Ray Burst Spectrometer (HXRBS), followed by softer gradual X-ray emission lasting several minutes. From an autocorrelation function analysis, evidence was found for quasi-periodic fluctuations with rise and decay times of 10 s in the Ca XIX and Fe XXV light curves. These variations were of small amplitude (less than 20%), often coincided with hard X-ray emissions, and were prominent during the onset of the gradual phase after the initial hard X-ray burst. It is speculated that these fluctuations were caused by repeated energy injections in a coronal loop that had already been heated and filled with dense plasma associated with the initial hard X-ray burst.

  3. Review of soft x-ray lasers and their applications

    SciTech Connect

    Skinner, C.H.

    1991-03-01

    The emerging technology of soft x-ray lasers is in a transition phase between the first laboratory demonstrations of gain and the acceptance of soft x-ray lasers as practical tools for novel applications. Current research is focused on several fronts. The operational wavelength range has been extended to the water window'', important for applications in the life sciences. Gain has also been generated with substantially simpler technology (such as a 6J laser) and this augurs well for the commercially availability in the near future of soft x-ray lasers for a variety of applications. Advanced soft x-ray laser concepts are being developed from investigations into ultra-high intensity laser/matter interactions. The first paper a brief historical perspective of x-ray microscopy and holography have begun. In this paper a brief historical perspective of x-ray laser development will be followed by a review of recent advances in recombination, collisional and photo-pumped systems and applications. A summary of current gain-length performance achieved in laboratories worldwide is presented. Near term prospects for applications to novel fields are discussed. 81 refs., 9 figs., 1 tab.

  4. Super-soft X-ray Spectral Evolution in Novae

    NASA Astrophysics Data System (ADS)

    Page, K. L.; Osborne, J. P.

    2014-12-01

    Swift has performed intensive monitoring of a number of novae as they pass through their super-soft X-ray phase. While Chandra and XMM-Newton can provide high-resolution grating spectra, important for identifying individual emission and absorption features and placing constraints on abundances, few observations are obtained with these instruments, thus providing only rare snapshots of the super-soft spectral evolution. With Swift, however, we can perform daily (if not hourly) monitoring, allowing us to follow the entirety of the super-soft phase in great detail. Spectral evolution is clear, often even when simply comparing the unfitted spectra. Here, we fit stellar atmosphere models to the X-ray spectra of some of the densely-observed Swift novae, investigating the evolution of temperature, emitting radius and X-ray luminosity throughout their super-soft phases.

  5. Resource Letter on Stimulated Inelastic X-ray Scattering at an XFEL

    SciTech Connect

    Patterson, Bruce D.; /SLAC

    2010-09-02

    At sufficient X-ray intensity, stimulated effects in inelastic scattering will become important. These coherent, non-linear optical phenomena may be used to impulsively produce a high degree of collective excitation in, for example, correlated electron materials, suitable for performing ultrafast time-resolved spectroscopy. This Resource Letter collects information on fundamental aspects of stimulated X-ray scattering and evaluates the prospect for successful experiments at a present or future X-ray free electron laser (XFEL) facility.

  6. Fabrication of a focusing soft X-ray collector payload

    NASA Technical Reports Server (NTRS)

    Davis, J. M.; Decaprio, A. R.; Manko, H.; Ting, J. W. S.

    1976-01-01

    A large area X-ray focusing collector with arc minute resolution and a position sensitive detector capable of operating in the soft X-ray region was developed for use on sounding rockets in studying stellar X-ray sources. The focusing payload consists of the following components, which are described: (1) a crossed paraboloid mirror assembly; (2) an aspect camera and star tracker; (3) a focal plane assembly containing an imaging proportional counter and its preamplifiers, high voltage power supplies and gas system; (4) a fiducial system; and (5) housekeeping, data handling, instrumentation and telemetry electronics. The design, tests, and operation are described.

  7. The very soft X-ray emission of X-ray-faint early-type galaxies

    NASA Technical Reports Server (NTRS)

    Pellegrini, S.; Fabbiano, G.

    1994-01-01

    A recent reanaylsis of Einstein data, and new ROSAT observations, have revealed the presence of at least two components in the X-ray spectra of X-ray faint early-type galaxies: a relatively hard component (kT greater than 1.5 keV), and a very soft component (kT approximately 0.2-0.3 keV). In this paper we address the problem of the nature of the very soft component and whether it can be due to a hot interstellar medium (ISM), or is most likely originated by the collective emission of very soft stellar sources. To this purpose, hydrodynamical evolutionary sequences for the secular behavior of gas flows in ellipticals have been performed, varying the Type Ia supernovae rate of explosion, and the dark matter amount and distribution. The results are compared with the observational X-ray data: the average Einstein spectrum for six X-ray faint early-type galaxies (among which are NGC 4365 and NGC 4697), and the spectrum obtained by the ROSAT pointed observation of NGC 4365. The very soft component could be entirely explained with a hot ISM only in galaxies such as NGC 4697, i.e., when the depth of the potential well-on which the average ISM temperature strongly depends-is quite shallow; in NGC 4365 a diffuse hot ISM would have a temperature larger than that of the very soft component, because of the deeper potential well. So, in NGC 4365 the softest contribution to the X-ray emission comes certainly from stellar sources. As stellar soft X-ray emitters, we consider late-type stellar coronae, supersoft sources such as those discovered by ROSAT in the Magellanic Clouds and M31, and RS CVn systems. All these candidates can be substantial contributors to the very soft emission, though none of them, taken separately, plausibly accounts entirely for its properties. We finally present a model for the X-ray emission of NGC 4365, to reproduce in detail the results of the ROSAT pointed observation, including the Position Sensitive Proportional Counter (PSPC) spectrum and radial

  8. Contact microscopy with a soft x-ray laser

    SciTech Connect

    DiCicco, D.S.; Kim, D.; Rosser, R.J.; Skinner, C.H.; Suckewer, S.; Gupta, A.P.; Hirschberg, J.G.

    1989-03-01

    A soft x-ray laser of output energy 1-3 mJ at 19.2 nm has been used to record high resolution images of biological specimens. The contact images were recorded on photoresist which was later viewed in a scanning electron microscope. We also present a Composite Optical X- ray Laser Microscope ''COXRALM'' of novel design. 14 refs., 8 figs., 1 tab.

  9. Soft X-ray Spectromicroscopy of Polymers

    NASA Astrophysics Data System (ADS)

    Ade, Harald

    1997-03-01

    The development of Near Edge X-ray Absorption Fine Structure (NEXAFS) microscopy^1 and linear dichroism microscopy^2 over the last few years utilizing the X1-Scanning Transmission X-ray Microscope (X1-STXM) at the National Synchrotron Light Source provides excellent specificity to various functional groups and moieties in organic molecules and polymeric materials at a spatial resolution of 50 nm. This chemical specificity can be utilized to map the distribution of various compounds in a material, or to micro-chemically analyze small sample areas. Examples of applications include the study of various phase-separated polymers (polyurethanes, liquid crystalline polyesters), multicomponent polymer blends, polymer laminates, and other organic materials such as coal^3. Linear dichroism microscopy furthermore explores the polarization dependence of NEXAFS in (partially) oriented materials, and can determine the orientation of specific functional groups. Applications of linear dichroism microscopy have focused so far on determining the relative degree of radial orientation in Kevlar fibers^3. ^1 H. Ade, X. Zhang, S. Cameron, C. Costello, J. Kirz, and S. Williams, Science 258, 972 (1992). ^2 H. Ade and B. Hsiao, Science 262, 1427 (1993). ^3 Acknowledgement: My callaborators are B. Hsiao, S. Subramoney, B. Wood, I. Plotzker, E. Rightor, G. Mitchell, C. Sloop, D.-J. Liu, S.-C. Liu, J. Marti, C. Zimba, A. P. Smith, R. Spontak, R. Fornes, R. Gilbert, C. Cody, A. Hitchcock and S. Urquhart. The X1-STXM is built and maintained by J. Kirz and C. Jacobsen and their groups. Work supported by: NSF Young Investigator Award (DMR-9458060), DuPont Young Professor Grant, and Dow Chemical.

  10. Electronic Properties of Hydrogen Storage Materials with Photon-in/Photon-out Soft-X-Ray Spectroscopy

    SciTech Connect

    Guo, Jinghua

    2008-09-22

    The applications of resonant soft X-ray emission spectroscopy on a variety of carbon systems have yielded characteristic fingerprints. With high-resolution monochromatized synchrotron radiation excitation, resonant inelastic X-ray scattering has emerged as a new source of information about electronic structure and excitation dynamics. Photon-in/photon-out soft-X-ray spectroscopy is used to study the electronic properties of fundamental materials, nanostructure, and complex hydrides and will offer potential in-depth understanding of chemisorption and/or physisorption mechanisms of hydrogen adsorption/desorption capacity and kinetics.

  11. Picosecond resolution soft x-ray laser plasma interferometry

    SciTech Connect

    Moon, S; Nilsen, J; Ng, A; Shlyaptsev, V; Dunn, J; Hunter, J; Keenan, R; Marconi, M; Filevich, J; Rocca, J; Smith, R

    2003-12-01

    We describe a soft x-ray laser interferometry technique that allows two-dimensional diagnosis of plasma electron density with picosecond time resolution. It consists of the combination of a robust high throughput amplitude division interferometer and a 14.7 nm transient inversion soft x-ray laser that produces {approx} 5 ps pulses. Due to its picosecond resolution and short wavelength scalability, this technique has potential for extending the high inherent precision of soft x-ray laser interferometry to the study of very dense plasmas of significant fundamental and practical interest, such as those investigated for inertial confined fusion. Results of its use in the diagnostics of dense large scale laser-created plasmas are presented.

  12. Bright circularly polarized soft X-ray high harmonics for X-ray magnetic circular dichroism

    PubMed Central

    Fan, Tingting; Grychtol, Patrik; Knut, Ronny; Hernández-García, Carlos; Hickstein, Daniel D.; Zusin, Dmitriy; Gentry, Christian; Dollar, Franklin J.; Mancuso, Christopher A.; Hogle, Craig W.; Kfir, Ofer; Legut, Dominik; Carva, Karel; Ellis, Jennifer L.; Dorney, Kevin M.; Chen, Cong; Shpyrko, Oleg G.; Fullerton, Eric E.; Cohen, Oren; Oppeneer, Peter M.; Milošević, Dejan B.; Becker, Andreas; Jaroń-Becker, Agnieszka A.; Popmintchev, Tenio; Murnane, Margaret M.; Kapteyn, Henry C.

    2015-01-01

    We demonstrate, to our knowledge, the first bright circularly polarized high-harmonic beams in the soft X-ray region of the electromagnetic spectrum, and use them to implement X-ray magnetic circular dichroism measurements in a tabletop-scale setup. Using counterrotating circularly polarized laser fields at 1.3 and 0.79 µm, we generate circularly polarized harmonics with photon energies exceeding 160 eV. The harmonic spectra emerge as a sequence of closely spaced pairs of left and right circularly polarized peaks, with energies determined by conservation of energy and spin angular momentum. We explain the single-atom and macroscopic physics by identifying the dominant electron quantum trajectories and optimal phase-matching conditions. The first advanced phase-matched propagation simulations for circularly polarized harmonics reveal the influence of the finite phase-matching temporal window on the spectrum, as well as the unique polarization-shaped attosecond pulse train. Finally, we use, to our knowledge, the first tabletop X-ray magnetic circular dichroism measurements at the N4,5 absorption edges of Gd to validate the high degree of circularity, brightness, and stability of this light source. These results demonstrate the feasibility of manipulating the polarization, spectrum, and temporal shape of high harmonics in the soft X-ray region by manipulating the driving laser waveform. PMID:26534992

  13. Bright circularly polarized soft X-ray high harmonics for X-ray magnetic circular dichroism.

    PubMed

    Fan, Tingting; Grychtol, Patrik; Knut, Ronny; Hernández-García, Carlos; Hickstein, Daniel D; Zusin, Dmitriy; Gentry, Christian; Dollar, Franklin J; Mancuso, Christopher A; Hogle, Craig W; Kfir, Ofer; Legut, Dominik; Carva, Karel; Ellis, Jennifer L; Dorney, Kevin M; Chen, Cong; Shpyrko, Oleg G; Fullerton, Eric E; Cohen, Oren; Oppeneer, Peter M; Milošević, Dejan B; Becker, Andreas; Jaroń-Becker, Agnieszka A; Popmintchev, Tenio; Murnane, Margaret M; Kapteyn, Henry C

    2015-11-17

    We demonstrate, to our knowledge, the first bright circularly polarized high-harmonic beams in the soft X-ray region of the electromagnetic spectrum, and use them to implement X-ray magnetic circular dichroism measurements in a tabletop-scale setup. Using counterrotating circularly polarized laser fields at 1.3 and 0.79 µm, we generate circularly polarized harmonics with photon energies exceeding 160 eV. The harmonic spectra emerge as a sequence of closely spaced pairs of left and right circularly polarized peaks, with energies determined by conservation of energy and spin angular momentum. We explain the single-atom and macroscopic physics by identifying the dominant electron quantum trajectories and optimal phase-matching conditions. The first advanced phase-matched propagation simulations for circularly polarized harmonics reveal the influence of the finite phase-matching temporal window on the spectrum, as well as the unique polarization-shaped attosecond pulse train. Finally, we use, to our knowledge, the first tabletop X-ray magnetic circular dichroism measurements at the N4,5 absorption edges of Gd to validate the high degree of circularity, brightness, and stability of this light source. These results demonstrate the feasibility of manipulating the polarization, spectrum, and temporal shape of high harmonics in the soft X-ray region by manipulating the driving laser waveform.

  14. Soft X-ray contact microscopy of nematode Caenorhabditis elegans

    NASA Astrophysics Data System (ADS)

    Poletti, G.; Orsini, F.; Batani, D.; Bernardinello, A.; Desai, T.; Ullschmied, J.; Skala, J.; Kralikova, B.; Krousky, E.; Juha, L.; Pfeifer, M.; Kadlec, Ch.; Mocek, T.; Präg, A.; Renner, O.; Cotelli, F.; Lora Lamia, C.; Zullini, A.

    2004-08-01

    Soft X-ray Contact Microscopy (SXCM) of Caenorhabditis elegans nematodes with typical length ~800 μ m and diameter ~30 μ m has been performed using the PALS laser source of wavelength λ = 1.314~μ m and pulse duration τ (FWHM) = 400 ps. Pulsed soft X-rays were generated using molybdenum and gold targets with laser intensities I ≥ 1014 W/cm2. Images have been recorded on PMMA photo resists and analyzed using an atomic force microscope operating in contact mode. Cuticle features and several internal organs have been identified in the SXCM images including lateral field, cuticle annuli, pharynx, and hypodermal and neuronal cell nuclei.

  15. Fast fluctuations of soft X-rays from active regions

    NASA Technical Reports Server (NTRS)

    Simnett, G. F.; Dennis, B. R.

    1986-01-01

    A selection of short lived small soft X-ray bursts is studied using data from the Hard X-ray Imaging Spectrometer (HXIS), and the results are compared with the data from the Hard X-Ray Burst Spectrometer (HXRBS) with a view to understanding conditions at the onset of flares. Short-lived events provide an opportunity to study the radiation from the primary energy transfer process without confusion from the slowly-varying thermal X-ray emission which characterizes the decay of a large flare. The fast decay of the soft X-rays, only a few tens of seconds, suggests that they occur in the dense chromosphere. The results indicate that the short events may be signatures of several different phenomena, depending on their characteristics. Some events occur in association with reverse-drift type III bursts and simultaneous flaring elsewhere on the Sun, thus suggesting dumping of particles accelerated at a remote site. Some events have hard X-ray bursts and normal type III bursts associated with them, while others have neither. The latter events place strong constraints on the nonthermal electron population present.

  16. Soft x-ray streak camera for laser fusion applications

    SciTech Connect

    Stradling, G.L.

    1981-04-01

    This thesis reviews the development and significance of the soft x-ray streak camera (SXRSC) in the context of inertial confinement fusion energy development. A brief introduction of laser fusion and laser fusion diagnostics is presented. The need for a soft x-ray streak camera as a laser fusion diagnostic is shown. Basic x-ray streak camera characteristics, design, and operation are reviewed. The SXRSC design criteria, the requirement for a subkilovolt x-ray transmitting window, and the resulting camera design are explained. Theory and design of reflector-filter pair combinations for three subkilovolt channels centered at 220 eV, 460 eV, and 620 eV are also presented. Calibration experiments are explained and data showing a dynamic range of 1000 and a sweep speed of 134 psec/mm are presented. Sensitivity modifications to the soft x-ray streak camera for a high-power target shot are described. A preliminary investigation, using a stepped cathode, of the thickness dependence of the gold photocathode response is discussed. Data from a typical Argus laser gold-disk target experiment are shown.

  17. Soft X ray properties of the Geminga pulsar

    NASA Astrophysics Data System (ADS)

    Halpern, J. P.; Ruderman, M.

    1993-01-01

    The ROSAT soft x ray spectrum and pulse profile of the Geminga pulsar are analyzed and interpreted in terms of thermal emission from the surface of the neutron star. The x ray spectrum appears to consist of two blackbody components with T1 = (5.2 +/- 1.0) x 10 5 K and T2 approximately 3 x 106 K, respectively. The inferred ratio of surface areas, A2/A1, is approximately 3 x 10-5. Both components are highly modulated at the pulsar rotation period, but the harder x ray pulse is narrower, and leads the main (soft) x ray pulse by about 105 deg of phase. The soft x ray component is interpreted as photospheric cooling of much of the neutron star's surface area, while the small, hot region could be part of the much smaller polar cap heated by energetic particles flowing inward from the magnetospheric accelerator which is responsible for the production of Geminga's gamma rays. Geminga's gamma ray emission is consistent with outer-magnetosphere accelerator models for highly inclined dipoles. These predict the beaming of energetic gamma rays close enough to the star to give copious e(+/-) production in the stellar magnetic field and a large circumstellar pair density from pair inflow toward the surface. These pairs may quench radio emission, and also reflect most of the hard polar cap x rays back to the stellar surface by cyclotron resonance scattering. They are then reemitted from that much larger area at the lower temperature T1. The single-peaked nature of the x ray pulse and its energy-dependent phase suggest an off-center dipole geometry for the surface magnetic field. Under the assumption that the soft x ray emission comes from the full surface of a neutron star of radius R = 10 km, a distance estimate of (150-400) pc is derived. This range is consistent with the fit interstellar column density of (1.5 +/- 0.5) x 1020 cm-2. Distances less than 150 pc are probably ruled out both by the lower limit on the column density, and also by the requirement that the Rayleigh

  18. Soft X-ray spectroscopy of astrophysical plasmas

    NASA Astrophysics Data System (ADS)

    Kahn, Steven M.

    These lectures are intended to provide a review of the basic physics necessary for the interpretation of high resolution soft X-ray spectra of astrophysical sources. While many of the topics I discuss can be found at the requisite level of sophistication in standard textbooks on atomic physics and spectroscopy, I have made an attempt to highlight those aspects which are especially important for X-ray transitions, and which are relevant at the characteristic temperatures and densities typically found in various types of X-ray emitting astrophysical plasmas. My emphasis is on discrete atomic transitions, which dominate the spectra of most cosmic sources in the soft X-ray band (100eV≤E≤10 keV). I do not discuss basic continuum processes like bremsstrahlung, synchrotron emission, and inverse Compton emission, as these are covered well in the usual texts used to introduce students to radiative processes in astrophysics. The organization is as follows: I provide a brief introduction to the role of X-ray spectroscopy in astrophysics, and the physical conditions in various types of cosmic X-ray sources. Chapters 1 through 3 cover the essentials of atomic physics: classical and quantum radiation theory, atomic structure, and electron-ion collisional processes, respectively. In Chap. 4, I discuss the various types of equilibria that apply in astrophysical plasmas, and in Chap. 5, I provide a relatively brief review of the most important discrete-line spectral diagnostics that fall in the soft X-ray band. Chapter 6 includes a set of concluding remarks and some thoughts on where this field might be headed in the future.

  19. Microspectroscopic soft X-ray analysis of keratin based biofibers.

    PubMed

    Späth, Andreas; Meyer, Markus; Semmler, Sonja; Fink, Rainer H

    2015-03-01

    Scanning soft X-ray transmission microspectroscopy (STXM) and transmission electron microscopy (TEM) have been employed for a high-resolution morphological and chemical analysis of hair fibers from human, sheep and alpaca. STXM allows optimum contrast imaging of the main hair building blocks due to tuneable photon energy. Chemical similarities and deviations for the human hair building blocks as well as for the three investigated species are discussed on the basis of the local near-edge X-ray absorption fine structure (NEXAFS). The spectra of melanosomes corroborate the state-of-the-art model for the chemical structure of eumelanin. Complementary TEM micrographs reveal the occurrence of cortex sectioning in alpaca hair to some extent. A spectroscopic analysis for human hair cortex indicates low mass loss upon soft X-ray irradiation, but transformation of chemical species with decreasing amount of peptide bonds and increasing NEXAFS signal for unsaturated carbon-carbon bonds.

  20. Phase measurement of soft x-ray multilayer mirrors.

    PubMed

    de Rossi, Sébastien; Bourassin-Bouchet, Charles; Meltchakov, Evgueni; Giglia, Angelo; Nannarone, Stefano; Delmotte, Franck

    2015-10-01

    We propose a new model enabling the extraction of the phase of a multilayer mirror from photocurrent measurements in the soft x rays. In this range, the effects of the mean free path of the electrons inside the stack can no longer be neglected, which prevents the phase reconstruction by conventional photocurrent measurements. The new model takes into account this phenomenon and thus extends up to the x rays the applicability range of the technique. This approach has been validated through a numerical and experimental study of chromium/scandium multilayers used near 360 eV. To our knowledge, this work constitutes the first measurement of the phase of a multilayer mirror in the soft x-ray range. PMID:26421544

  1. Phase measurement of soft x-ray multilayer mirrors.

    PubMed

    de Rossi, Sébastien; Bourassin-Bouchet, Charles; Meltchakov, Evgueni; Giglia, Angelo; Nannarone, Stefano; Delmotte, Franck

    2015-10-01

    We propose a new model enabling the extraction of the phase of a multilayer mirror from photocurrent measurements in the soft x rays. In this range, the effects of the mean free path of the electrons inside the stack can no longer be neglected, which prevents the phase reconstruction by conventional photocurrent measurements. The new model takes into account this phenomenon and thus extends up to the x rays the applicability range of the technique. This approach has been validated through a numerical and experimental study of chromium/scandium multilayers used near 360 eV. To our knowledge, this work constitutes the first measurement of the phase of a multilayer mirror in the soft x-ray range.

  2. Lensless imaging of nanoporous glass with soft X-rays

    DOE PAGES

    Turner, Joshua J.; Nelson, Johanna; Huang, Xiaojing; Steinbrener, Jan; Jacobsen, Chris

    2013-06-01

    Coherent soft X-ray diffraction has been used to image nanoporous glass structure in two dimensions using different methods. The merit of the reconstructions was judged using a new method of Fourier phase correlation with a final, refined image. The porous structure was found to have a much larger average size then previously believed.

  3. Soft x-ray virtual diagnostics for tokamak simulations

    SciTech Connect

    Kim, J. S.; Zhao, L.; Bogatu, I. N.; In, Y.; Turnbull, A.; Osborne, T.; Maraschek, M.; Comer, K.

    2009-11-15

    The numerical toolset, FAR-TECH Virtual Diagnostic Utility, for generating virtual experimental data based on theoretical models and comparing it with experimental data, has been developed for soft x-ray diagnostics on DIII-D. The virtual (or synthetic) soft x-ray signals for a sample DIII-D discharge are compared with the experimental data. The plasma density and temperature radial profiles needed in the soft x-ray signal modeling are obtained from experimental data, i.e., from Thomson scattering and electron cyclotron emission. The virtual soft x-ray diagnostics for the equilibriums have a good agreement with the experimental data. The virtual diagnostics based on an ideal linear instability also agree reasonably well with the experimental data. The agreements are good enough to justify the methodology presented here for utilizing virtual diagnostics for routine comparison of experimental data. The agreements also motivate further detailed simulations with improved physical models such as the nonideal magnetohydrodynamics contributions (resistivity, viscosity, nonaxisymmetric error fields, etc.) and other nonlinear effects, which can be tested by virtual diagnostics with various stability modeling.

  4. Lasers, extreme UV and soft X-ray

    SciTech Connect

    Nilsen, Joseph

    2015-09-20

    Three decades ago, large ICF lasers that occupied entire buildings were used as the energy sources to drive the first X-ray lasers. Today X-ray lasers are tabletop, spatially coherent, high-repetition rate lasers that enable many of the standard optical techniques such as interferometry to be extended to the soft X-ray regime between wavelengths of 10 and 50 nm. Over the last decade X-ray laser performance has been improved by the use of the grazing incidence geometry, diode-pumped solid-state lasers, and seeding techniques. The dominant X-ray laser schemes are the monopole collisional excitation lasers either driven by chirped pulse amplification (CPA) laser systems or capillary discharge. The CPA systems drive lasing in neon-like or nickel-like ions, typically in the 10 – 30 nm range, while the capillary system works best for neon-like argon at 46.9 nm. Most researchers use nickel-like ion lasers near 14 nm because they are well matched to the Mo:Si multilayer mirrors that have peak reflectivity near 13 nm and are used in many applications. As a result, the last decade has seen the birth of the X-ray free electron laser (XFEL) that can reach wavelengths down to 0.15 nm and the inner-shell Ne laser at 1.46 nm.

  5. Lasers, extreme UV and soft X-ray

    DOE PAGES

    Nilsen, Joseph

    2015-09-20

    Three decades ago, large ICF lasers that occupied entire buildings were used as the energy sources to drive the first X-ray lasers. Today X-ray lasers are tabletop, spatially coherent, high-repetition rate lasers that enable many of the standard optical techniques such as interferometry to be extended to the soft X-ray regime between wavelengths of 10 and 50 nm. Over the last decade X-ray laser performance has been improved by the use of the grazing incidence geometry, diode-pumped solid-state lasers, and seeding techniques. The dominant X-ray laser schemes are the monopole collisional excitation lasers either driven by chirped pulse amplification (CPA)more » laser systems or capillary discharge. The CPA systems drive lasing in neon-like or nickel-like ions, typically in the 10 – 30 nm range, while the capillary system works best for neon-like argon at 46.9 nm. Most researchers use nickel-like ion lasers near 14 nm because they are well matched to the Mo:Si multilayer mirrors that have peak reflectivity near 13 nm and are used in many applications. As a result, the last decade has seen the birth of the X-ray free electron laser (XFEL) that can reach wavelengths down to 0.15 nm and the inner-shell Ne laser at 1.46 nm.« less

  6. A soft X-ray lag detected in Centaurus A

    NASA Astrophysics Data System (ADS)

    Tachibana, Yutaro; Kawamuro, Taiki; Ueda, Yoshihiro; Shidatsu, Megumi; Arimoto, Makoto; Yoshii, Taketoshi; Yatsu, Yoichi; Saito, Yoshihiko; Pike, Sean; Kawai, Nobuyuki

    2016-06-01

    We performed time-lag analysis on the X-ray light curves of Centaurus A (Cen A) obtained by the Gas Slit Camera (GSC) aboard the Monitor of All-sky X-ray Image (MAXI) in three energy bands (2-4 keV, 4-10 keV, and 10-20 keV). We discovered a soft X-ray lag relative to higher energies (soft lag) on a timescale of days in a flaring episode by employing the discrete correlation function (DCF) and the z-transformed discrete correlation function (ZDCF) method. In the episode, a peak and a centroid in the DCF and the ZDCF was observed at a soft lag of ˜ 5 d in 2-4 keV versus 4-10 keV and in 4-10 keV versus 10-20 keV, and ˜ 10 d in 2-4 keV versus 10-20 keV. We found it difficult to explain the observed X-ray variation by a single energy injection with the one-zone synchrotron self-Compton (SSC) model, in which the soft lags in these three energy bands reflect the different cooling times of the relativistic electrons, by assuming the magnetic field and minimum Lorentz factor estimated from a broad-band spectral energy distribution. Alternatively, if the phenomenon is interpreted as cooling of Comptonizing electrons in a corona covering the accretion disk, the temperature of the corona producing the variable X-rays should be ˜ 10 keV for reconciliation with the soft lag in the energy range of 2-20 keV.

  7. Shakeup in soft-x-ray emission. II. Plasmon satellites and x-ray photoemission spectroscopy

    NASA Astrophysics Data System (ADS)

    Livins, Peteris; Schnatterly, S. E.

    1988-04-01

    We report the first observation of a plasmon satellite in the K emission spectrum of diamond. The previously identified plasmon satellites of Al and graphite are also presented, and data is compared with an oscillator model applicable to soft-x-ray emission and photoemission. The graphite satellite is shown to exhibit an anomalous location with respect to the parent emission. We report for the Al LI-LII,III core-core transitions a spin-orbit splitting of 0.42+/-0.02 eV with a Lorentzian width of 0.67+/-0.02 eV. The oscillator model applied to x-ray photoemission predicts a shift of the plasmon satellite with respect to the zero loss line as the final-electron kinetic energy is varied.

  8. A soft X-ray spectrometer for diffuse cosmic sources

    NASA Technical Reports Server (NTRS)

    Borken, R. J.; Kraushaar, W. L.

    1976-01-01

    The design of a Bragg crystal spectrometer for the diffuse soft X-ray background is described. The instrument has no moving parts; a 6 degree x 20 degree FWHM field of view; resolution in the range 20-100; and spans wavelength ranges 44-80 A or 13-23 A when lead stearate or KAP crystals are used. If placed on a small spacecraft, integration times of approximately 1000 s will be required to detect the existence of the stronger lines expected in the X-ray background.

  9. The Diffuse Soft X-ray Background: Trials and Tribulations

    NASA Astrophysics Data System (ADS)

    Ulmer, Melville P.

    2013-01-01

    I joined the University of Wisconsin-Madison sounding rocket group at its inception. It was an exciting time, as nobody knew what the X-ray sky looked like. Our group focused on the soft X-ray background, and built proportional counters with super thin (2 micron thick) windows. As the inter gas pressure of the counters was about 1 atmosphere, it was no mean feat to get payload to launch without the window bursting. On top of that we built all our own software from space solutions to unfolding the spectral data. For we did it then as now: Our computer code modeled the detector response and then folded various spectral shapes through the response and compared the results with the raw data. As far as interpretation goes, here are examples of how one can get things wrong: The Berkeley group published a paper of the soft X-ray background that disagreed with ours. Why? It turned out they had **assumed** the galactic plane was completely opaque to soft X-ray and hence corrected for detector background that way. It turns out that the ISM emits in soft X-rays! Another example was the faux pas of the Calgary group. They didn’t properly shield their detector from the sounding rocket telemetry. Thus they got an enormous signal, which to our amusement some (ambulance chaser) theoreticians tried to explain! So back then as now, mistakes were made, but at least we all knew how our X-ray systems worked from soup (the detectors) to nuts (the data analysis code) where as toady “anybody” with a good idea but only a vague inkling of how detectors, mirrors and software work, can be an X-ray astronomer. On the one hand, this has made the field accessible to all, and on the other, errors in interpretation can be made as the X-ray telescope user can fall prey to running black box software. Furthermore with so much funding going into supporting observers, there is little left to make the necessary technology advances or keep the core expertise in place to even to stay even with

  10. Transition radiation very soft X-ray source

    NASA Astrophysics Data System (ADS)

    Umiastowski, K.; Nguyen, A.

    1994-05-01

    There is a growing interest in the transition radiation (TR), as a soft X-ray source, in the last few years. Many papers have been published on calculations or experiments in the 1-10 keV X-ray energy range using 50-200 MeV electron accelerators. We investigate the possibility to generate very soft X-rays (λ = 12 nm) with low-energy electron accelerator (5-20 MeV). Very little information is available on TR in this range of photon wavelength and electron energy. A stack of 20 foils of beryllium placed in vacuum was used in our computer simulation. Calculation shows that for 1 mA electron beam current, radiation with few mW intensity can be produced. Emitted photons are quasi-monoenergetic (FWHM less than 5%), and well collimated. The aim of our study is to investigate the possibility of fabricate a soft X-ray source, much more compact than synchrotron source and producing an intense and quasi-coherent radiation, for industrial applications.

  11. Soft x-ray diagnostics for pulsed power machines

    SciTech Connect

    Idzorek, G.C.; Coulter, W.L.; Walsh, P.J.; Montoya, R.R.

    1995-08-01

    A variety of soft x-ray diagnostics are being fielded on the Los Alamos National Laboratory Pegasus and Procyon pulsed power systems and also being fielded on joint US/Russian magnetized target fusion experiments known as MAGO (Magnitoye Obzhatiye). The authors have designed a low-cost modular photoemissive detector designated the XRD-96 that uses commercial 1100 series aluminum for the photocathode. In addition to photocathode detectors a number of designs using solid state silicon photodiodes have been designed and fielded. They also present a soft x-ray time-integrated pinhole camera system that uses standard type TMAX-400 photographic film that obviates the need for expensive and no longer produced zero-overcoat soft x-ray emulsion film. In a typical experiment the desired spectral energy cuts, signal intensity levels, and desired field of view will determine diagnostic geometry and x-ray filters selected. The authors have developed several computer codes to assist in the diagnostic design process and data deconvolution. Examples of the diagnostic design process and data analysis for a typical pulsed power experiment are presented.

  12. Towards practical soft X-ray spectromicroscopy of biomaterials.

    PubMed

    Hitchcock, A P; Morin, C; Heng, Y M; Cornelius, R M; Brash, J L

    2002-01-01

    Scanning transmission X-ray microscopy (STXM) is being developed as a new tool to study the surface chemical morphology and biointeractions of candidate biomaterials with emphasis on blood compatible polymers. STXM is a synchrotron based technique which provides quantitative chemical mapping at a spatial resolution of 50 nm. Chemical speciation is provided by the near edge X-ray absorption spectral (NEXAFS) signal. We show that STXM can detect proteins on soft X-ray transparent polymer thin films with monolayer sensitivity. Of great significance is the fact that measurements can be made in situ, i.e. in the presence of an overlayer of the protein solution. The strengths, limitations and future potential of STXM for studies of biomaterials are discussed.

  13. Soft X-Ray Polarimetry with a CubeSat

    NASA Astrophysics Data System (ADS)

    Kaaret, Philip

    2016-07-01

    We describe an instrument capable of measuring the polarization of astrophysical sources in soft X-rays that can be accomplished at modest cost by exploiting CubeSats as novel vehicles for high energy astrophysics. The instrument would re-use technologies that will be demonstrated on the HaloSat cubesat that is currently under construction. Potential target include thermally-emitting isolated neutron stars and blazars. Measurement of the polarization of X-rays emitted from the surface of a highly magnetized neutron star provides a means to test a unique signature of strong-field quantum electrodynamics and probe the neutron star magnetic field and X-ray emission geometry. Polarization measurements of blazars should strongly constrain jet emission models.

  14. High spatial resolution soft-x-ray microscopy

    SciTech Connect

    Meyer-Ilse, W.; Medecki, H.; Brown, J.T.

    1997-04-01

    A new soft x-ray microscope (XM-1) with high spatial resolution has been constructed by the Center for X-ray Optics. It uses bending magnet radiation from beamline 6.1 at the Advanced Light Source, and is used in a variety of projects and applications in the life and physical sciences. Most of these projects are ongoing. The instrument uses zone plate lenses and achieves a resolution of 43 nm, measured over 10% to 90% intensity with a knife edge test sample. X-ray microscopy permits the imaging of relatively thick samples, up to 10 {mu}m thick, in water. XM-1 has an easy to use interface, that utilizes visible light microscopy to precisely position and focus the specimen. The authors describe applications of this device in the biological sciences, as well as in studying industrial applications including structured polymer samples.

  15. Soft x-ray holographic tomography for biological specimens

    NASA Astrophysics Data System (ADS)

    Gao, Hongyi; Chen, Jianwen; Xie, Honglan; Li, Ruxin; Xu, Zhizhan; Jiang, Shiping; Zhang, Yuxuan

    2003-10-01

    In this paper, we present some experimental results on X -ray holography, holographic tomography, and a new holographic tomography method called pre-amplified holographic tomography is proposed. Due to the shorter wavelength and the larger penetration depths, X-rays provide the potential of higher resolution in imaging techniques, and have the ability to image intact, living, hydrated cells w ithout slicing, dehydration, chemical fixation or stain. Recently, using X-ray source in National Synchrotron Radiation Laboratory in Hefei, we have successfully performed some soft X-ray holography experiments on biological specimen. The specimens used in the experiments was the garlic clove epidermis, we got their X-ray hologram, and then reconstructed them by computer programs, the feature of the cell walls, the nuclei and some cytoplasm were clearly resolved. However, there still exist some problems in realization of practical 3D microscopic imaging due to the near-unity refractive index of the matter. There is no X-ray optics having a sufficient high numerical aperture to achieve a depth resolution that is comparable to the transverse resolution. On the other hand, computer tomography needs a record of hundreds of views of the test object at different angles for high resolution. This is because the number of views required for a densely packed object is equal to the object radius divided by the desired depth resolution. Clearly, it is impractical for a radiation-sensitive biological specimen. Moreover, the X-ray diffraction effect makes projection data blur, this badly degrades the resolution of the reconstructed image. In order to observe 3D structure of the biological specimens, McNulty proposed a new method for 3D imaging called "holographic tomography (HT)" in which several holograms of the specimen are recorded from various illumination directions and combined in the reconstruction step. This permits the specimens to be sampled over a wide range of spatial

  16. Viewing spin structures with soft x-ray microscopy

    SciTech Connect

    Fischer, Peter

    2010-06-01

    The spin of the electron and its associated magnetic moment marks the basic unit for magnetic properties of matter. Magnetism, in particular ferromagnetism and antiferromagnetism is described by a collective order of these spins, where the interaction between individual spins reflects a competition between exchange, anisotropy and dipolar energy terms. As a result the energetically favored ground state of a ferromagnetic system is a rather complex spin configuration, the magnetic domain structure. Magnetism is one of the eldest scientific phenomena, yet it is one of the most powerful and versatile utilized physical effects in modern technologies, such as in magnetic storage and sensor devices. To achieve highest storage density, the relevant length scales, such as the bit size in disk drives is now approaching the nanoscale and as such further developments have to deal with nanoscience phenomena. Advanced characterization tools are required to fully understand the underlying physical principles. Magnetic microscopes using polarized soft X-rays offer a close-up view into magnetism with unique features, these include elemental sensitivity due to X-ray magnetic dichroism effects as contrast mechanism, high spatial resolution provided by state-of-the-art X-ray optics and fast time resolution limited by the inherent time structure of current X-ray sources, which will be overcome with the introduction of ultrafast and high brilliant X-ray sources.

  17. Inelastic x-ray scattering from polycrystalline materials at low momentum transfer

    SciTech Connect

    Bosak, Alexey; Krisch, Michael; Fischer, Irmengard; Huotari, Simo; Monaco, Giulio

    2007-02-01

    The inelastic x-ray scattering from polycrystalline materials at low momentum transfer is analyzed with respect to the orientation-averaged acoustic phonon dispersion and the relationship between the derived sound velocities and their corresponding macroscopic entities. The effect of texturing on the sound dispersion is discussed and illustrated using the examples of hcp cobalt and hexagonal graphite. Our theoretical considerations are supported by experimental results and emphasize the importance to carefully consider the effects of elastic anisotropy when data obtained by inelastic x-ray scattering are compared or confronted with macroscopic measurements.

  18. Focusing polycapillary to reduce parasitic scattering for inelastic x-ray measurements at high pressure

    SciTech Connect

    Chow, P. Xiao, Y. M.; Rod, E.; Bai, L. G.; Shen, G. Y.; Sinogeikin, S.; Gao, N.; Ding, Y.; Mao, H.-K.

    2015-07-15

    The double-differential scattering cross-section for the inelastic scattering of x-ray photons from electrons is typically orders of magnitude smaller than that of elastic scattering. With samples 10-100 μm size in a diamond anvil cell at high pressure, the inelastic x-ray scattering signals from samples are obscured by scattering from the cell gasket and diamonds. One major experimental challenge is to measure a clean inelastic signal from the sample in a diamond anvil cell. Among the many strategies for doing this, we have used a focusing polycapillary as a post-sample optic, which allows essentially only scattered photons within its input field of view to be refocused and transmitted to the backscattering energy analyzer of the spectrometer. We describe the modified inelastic x-ray spectrometer and its alignment. With a focused incident beam which matches the sample size and the field of view of polycapillary, at relatively large scattering angles, the polycapillary effectively reduces parasitic scattering from the diamond anvil cell gasket and diamonds. Raw data collected from the helium exciton measured by x-ray inelastic scattering at high pressure using the polycapillary method are compared with those using conventional post-sample slit collimation.

  19. Soft x-ray laser microscope. Final report

    SciTech Connect

    Suckewer, P.I.

    1990-10-01

    The program consisted of two phases (Phase I and Phase II). The goal of the Phase I (first year program) was to design and construct the Soft X-ray Laser Contact Microscope. Such microscope was constructed and adapted to PPL`s 18.2nm soft X-ray Laser (SXL), which in turn was modified and prepared for microscopy experiments. Investigation of the photoresist response to 18.2nm laser radiation and transmissivity of 0.1m thick silicion-nitride (Si{sub 3}N{sub 4}) windows were important initial works. The goal of the first year of Phase II was to construct X-ray contact microscope in combination with existing optical phase microscope, already used by biologists. In the second year of Phase II study of dehydrated Horeseshoe Crab and Hela cancer cells were performed with COXRALM. Also during Phase II, the Imaging X-Ray Laser Microscope (IXRALM) was designed and constructed. This paper describes the development of each of the microscopes and their application for research.

  20. Soft X-ray polarimeter-spectrometer SOLPEX

    NASA Astrophysics Data System (ADS)

    Steslicki, Marek; Sylwester, Janusz; Plocieniak, Stefan; Bakala, Jaroslaw; Szaforz, Zaneta Anna; Scislowski, Daniel; Kowalinski, Miroslaw; Hernandez, Jose; Vadimovich Kuzin, Sergey; Shestov, Sergey

    2015-08-01

    We present an innovative soft X-ray polarimeter and spectrometer SOLPEX. The instrument will be mounted aboard the ISS within the Russian science complex KORTES. The measurements to be made by SOLPEX are expected to be of unprecedented quality in terms of sensitivity to detect the soft-X- ray polarization of solar emission emanating from active regions and flares in particular. Simultaneous measurements of the polarization degree and the other characteristics (eg. evolution of the spectra) constitute the last, rather unexplored area of solar X-ray spectroscopy providing substantial diagnostic potential. Second important science task to be addressed are the measurements of Doppler shifts in selected X-ray spectral emission lines formed in hot flaring sources. The novel-type Dopplerometer (flat Bragg crystal drum unit) is planned to be a part of SOLPEX and will allow to measure line Doppler shifts in absolute terms with unprecedented time resolution (fraction of a second) during the impulsive flare phases. We shall present some details of the SolpeX instrument and discuss observing sequences in a view of science objectives to be reached.

  1. PSPC soft x-ray observations of Seyfert 2 galaxies

    NASA Technical Reports Server (NTRS)

    Turner, T. J.; Urry, C. M.; Mushotzky, R. F.

    1993-01-01

    We present the results from ROSAT PSPC soft x-ray (0.1-2.0 keV) observations of six Seyfert 2 galaxies, chosen from the brightest Seyfert 2s detected with the Einstein Imaging Proportional Counter. All of the targets were detected with the ROSAT PSPC. Spatial analysis shows that the source density within a few arcmin of each Seyfert 2 galaxy is a factor of approximately eight higher than in the rest of the inner field of view of the PSPC images. In NGC1365 it appears that the serendipitous sources may be x-ray binary systems in the host galaxy. The proximity of the serendipitous sources, typically within a few arcmin of the target Seyfert 2, means that previous x-ray observations of the Seyfert 2 galaxies have been significantly contaminated, and that source confusion is important on a spatial scale of approximately 1 arcmin. Some spectra, most notably Mrk3 and NGC1365, indicate the presence of a high equivalent width soft x-ray line blend consistent with unresolved iron L and oxygen K emission.

  2. X-ray edge singularity in resonant inelastic x-ray scattering (RIXS)

    NASA Astrophysics Data System (ADS)

    Markiewicz, Robert; Rehr, John; Bansil, Arun

    2013-03-01

    We develop a lattice model based on the theory of Mahan, Noziéres, and de Dominicis for x-ray absorption to explore the effect of the core hole on the RIXS cross section. The dominant part of the spectrum can be described in terms of the dynamic structure function S (q , ω) dressed by matrix element effects, but there is also a weak background associated with multi-electron-hole pair excitations. The model reproduces the decomposition of the RIXS spectrum into well- and poorly-screened components. An edge singularity arises at the threshold of both components. Fairly large lattice sizes are required to describe the continuum limit. Supported by DOE Grant DE-FG02-07ER46352 and facilitated by the DOE CMCSN, under grant number DE-SC0007091.

  3. Aperiodic multilayer structures in soft X-ray radiation optics

    SciTech Connect

    Vishnyakov, E A; Kamenets, F F; Kondratenko, V V; Lugin, M S; Panchenko, A V; Pershin, Yu P; Pirozhkov, A S; Ragozin, Evgenii N

    2012-02-28

    We review the works related to the development of aperiodic multilayer structures - optical elements for the soft X-ray range. The potentialities of aperiodic multilayer mirrors as regards reflection of soft X-ray radiation in a broad wavelength range, first and foremost at normal radiation incidence, as well as the capabilities of broadband polariser mirrors are investigated. The results of multiparametric optimisation and experimental results for Mo/Si aperiodic mirrors ({lambda} {>=} 12.5 nm) as well as calculations for several promising material pairs (Pd/Y, Ag/Y, etc.) for {lambda} {<=} 12.5 nm are outlined. The effect of transition layers on the reflectivity is considered, in particular by taking into account the smooth variation of the permittivity near interfacial boundaries. The use of broadband mirrors in laser-plasma spectroscopic experiments is discussed.

  4. The soft X ray excess in Einstein quasar spectra

    NASA Technical Reports Server (NTRS)

    Wilkes, Belinda J.; Masnou, Jean-Louis; Elvis, Martin; Mcdowell, Jonathan; Arnaud, Keith

    1989-01-01

    The soft X-ray excess component is studied for a signal to noise limited subsample of 14 quasars from the WE87 sample observed with the Einstein Imaging Proportional Counter (IPC). Detailed analysis of the IPC data, combined with Einstein Monitor Proportional Counter (MPC) data where possible, and use of accurate galactic N sub H values allows estimation of the strength of any excess and improvement of constraints on the spectral slope at higher X-ray energies. A significant excess in 9 of the 14 objects is found. It is confined in all but one case to below 0.6 keV and variable in the two cases where there are multiple observations. The relation of the soft excess to other continuum properties of the quasars is investigated.

  5. The Soft X-ray Spectromicroscopy Beamline at SSRF

    SciTech Connect

    Guo, Z.; Tai, R.; Wand, Y.; Yan, R.; Chen, M.; Wu, Y.; Chen, J.; Xue, S.; Xu, H.

    2011-09-09

    Commissioning of the soft x-ray spectromicroscopy beanmline at SSRF was formally started on Dec 26, 2008. Beamline performance has reached or surpassed the designing goals according to the measurements by domestic experts, especially for its high energy resolution and high spatial resolution. Since its first operation by users on May 6, 2009, tens of experiments have been conducted, and some preliminary exciting results have been acquired.

  6. ASTRO-H Soft X-ray Telescope (SXT)

    NASA Astrophysics Data System (ADS)

    Soong, Yang; Okajima, Takashi; Serlemitsos, Peter J.; Odell, Stephen L.; Ramsey, Brian D.; Gubarev, Mikhail V.; Ishida, Manabu; Maeda, Yoshitomo; Iizuka, Ryo; Hayashi, Takayuki; Tawara, Yuzuru; Furuzawa, Akihiro; Mori, Hideyuki; Miyazawa, Takuya; Kunieda, Hideyo; Awaki, Hisamitsu; Sugita, Satoshi; Tamura, Keisuke; Ishibashi, Kazunori; Izumiya, Takanori; Minami, Sari; Sato, Toshiki; Tomikawa, Kazuki; Kikuchi, Naomichi; Iwase, Toshihiro

    2014-07-01

    ASTRO-H is an astrophysics satellite dedicated for non-dispersive X-ray spectroscopic study on selective celestial X-ray sources. Among the onboard instruments there are four Wolter-I X-ray mirrors of their reflectors' figure in conical approximation. Two of the four are soft X-ray mirrors1, of which the energy range is from a few hundred eV to 15 keV within the effective aperture being defined by the nested reflectors' radius ranging between 5.8 cm to 22.5 cm. The focal point instruments will be a calorimeter (SXS) and a CCD camera (SXI), respectively. The mirrors were in quadrant configuration with photons being reflected consecutively in the primary and secondary stage before converging on the focal plane of 5.6 m away from the interface between the two stages. The reflectors of the mirror are made of heat-formed aluminum substrate of the thickness gauged of 152 μm, 229 μm, and 305 μm of the alloy 5052 H-19, followed by epoxy replication on gold-sputtered smooth Pyrex cylindrical mandrels to acquire the X-ray reflective surface. The epoxy layer is 10 m nominal and surface gold layer of 0.2 μm. Improvements on angular response over its predecessors, e.g. Astro-E1/Suzaku mirrors, come from error reduction on the figure, the roundness, and the grazing angle/radius mismatching of the reflecting surface, and tighter specs and mechanical strength on supporting structure to reduce the reflector positioning and the assembly errors. Each soft x-ray telescope (SXT), SXT-1 or SXT-2, were integrated from four independent quadrants of mirrors. The stray-light baffles, in quadrant configuration, were mounted onto the integrated mirror. Thermal control units were attached to the perimeter of the integrated mirror to keep the mirror within operating temperature in space. The completed instrument went through a series of optical alignment, thus made the quadrant images confocal and their optical axes in parallel to achieve highest throughput possible. Environmental tests

  7. Soft X-ray measurements in magnetic fusion plasma physics

    NASA Astrophysics Data System (ADS)

    Botrugno, A.; Gabellieri, L.; Mazon, D.; Pacella, D.; Romano, A.

    2010-11-01

    Soft X-ray diagnostic systems and their successful application in the field of magnetic fusion plasma physics are discussed. Radiation with wavelength in the region of Soft X-Ray (1-30 keV) is largely produced by high temperature plasmas, carrying important information on many processes during a plasma discharge. Soft X-ray diagnostics are largely used in various fusion devices all over the world. These diagnostic systems are able to obtain information on electron temperature, electron density, impurity transport, Magneto Hydro Dynamic instabilities. We will discuss the SXR diagnostic installed on FTU in Frascati (Italy) and on Tore Supra in Cadarache (France), with special emphasis on diagnostic performances. Moreover, we will discuss the two different inversion methods for tomographic reconstruction used in Frascati and in Cadarache, the first one is relied on a guessed topology of iso-emissivity surfaces, the second one on regularization techniques, like minimum Fisher or maximum entropy. Finally, a new and very fast 2D imaging system with energy discrimination and high time resolution will be summarized as an alternative approach of SXR detection system.

  8. Soft x ray properties of the Geminga pulsar

    NASA Technical Reports Server (NTRS)

    Halpern, J. P.; Ruderman, M.

    1993-01-01

    The ROSAT soft x ray spectrum and pulse profile of the Geminga pulsar are analyzed and interpreted in terms of thermal emission from the surface of the neutron star. The x ray spectrum appears to consist of two blackbody components with T(sub 1) = (5.2 +/- 1.0) x 10 (exp 5) K and T(sub 2) approximately 3 x 10(exp 6) K, respectively. The inferred ratio of surface areas, A(sub 2)/A(sub 1), is approximately 3 x 10(exp -5). Both components are highly modulated at the pulsar rotation period, but the harder x ray pulse is narrower, and leads the main (soft) x ray pulse by about 105 deg of phase. The soft x ray component is interpreted as photospheric cooling of much of the neutron star's surface area, while the small, hot region could be part of the much smaller polar cap heated by energetic particles flowing inward from the magnetospheric accelerator which is responsible for the production of Geminga's gamma rays. Geminga's gamma ray emission is consistent with outer-magnetosphere accelerator models for highly inclined dipoles. These predict the beaming of energetic gamma rays close enough to the star to give copious e(+/-) production in the stellar magnetic field and a large circumstellar pair density from pair inflow toward the surface. These pairs may quench radio emission, and also reflect most of the hard polar cap x rays back to the stellar surface by cyclotron resonance scattering. They are then reemitted from that much larger area at the lower temperature T(sub 1). The single-peaked nature of the x ray pulse and its energy-dependent phase suggest an off-center dipole geometry for the surface magnetic field. Under the assumption that the soft x ray emission comes from the full surface of a neutron star of radius R = 10 km, a distance estimate of (150-400) pc is derived. This range is consistent with the fit interstellar column density of (1.5 +/- 0.5) x 10(exp 20) cm(exp -2). Distances less than 150 pc are probably ruled out both by the lower limit on the column

  9. X-ray microscopy of soft and hard human tissues

    NASA Astrophysics Data System (ADS)

    Müller, Bert; Schulz, Georg; Deyhle, Hans; Stalder, Anja K.; Ilgenstein, Bernd; Holme, Margaret N.; Weitkamp, Timm; Beckmann, Felix; Hieber, Simone E.

    2016-01-01

    The simultaneous post mortem visualization of soft and hard tissues using absorption-based CT remains a challenge. If the photon energy is optimized for the visualization of hard tissue, the surrounding soft tissue components are almost X-ray transparent. Therefore, the combination with other modalities such as phase-contrast CT, magnetic resonance microscopy, and histology is essential to detect the anatomical features. The combination of the 2D and 3D data sets using sophisticated segmentation and registration tools allows for conclusions about otherwise inaccessible anatomical features essential for improved patient treatments.

  10. Soft x-ray holography and microscopy of biological cells

    NASA Astrophysics Data System (ADS)

    Chen, Jianwen; Gao, Hongyi; Xie, Honglan; Li, Ruxin; Xu, Zhizhan

    2003-10-01

    Some experimental results on soft X-ray microscopy and holography imaging of biological specimens are presented in the paper. As we know, due to diffraction effects, there exists a resolution limit determined by wavelength λ and numerical aperture NA in conventional optical microscopy. In order to improve resolution, the num erical aperture should be made as large as possible and the wavelength as short as possible. Owing to the shorter wavelength, X-rays provide the potential of higher resolution in X-ray microscopy, holography image and allow for exam ination the interior structures of thicker specimens. In the experiments, we used synchrotron radiation source in Hefei as light source. Soft X-rays come from a bending magnet in 800 M eV electron storage ring with characteristic wavelength of 2.4 nm. The continuous X-ray spectrums are monochromatized by a zone-plate and a pinhole with 300 m diameter. The experimental set-up is typical contact microscopic system, its main advantage is simplicity and no special optical element is needed. The specimens used in the experiments of microscopic imaging are the colibacillus, the gingko vascular hundle and the fritillaries ovary karyon. The specimen for holographic imaging is the spider filam ents. The basic structures of plant cells such as the cell walls, the cytoplasm and the karyon especially the joint structures between the cells are observed clearly. An experimental study on a thick biological specimen that is a whole sporule w ith the thickness of about 30 μm is performed. In the holographic experiments, the experimental setup is typical Gabor in-line holography. The specimen is placed in line with X-ray source, which provides both the reference w aves and specimen illum ination. The specimen is some spider filament, which adhere to a Si3N4 film. The recording medium is PM M A, which is placed at recording distance of about 400 μm from the specimen. The hologram s were reconstructed by digital method with 300 nm

  11. Soft x-ray measurements from the PDX tokamak

    SciTech Connect

    Silver, E.H.; Bitter, M.; Brau, K.; Eames, D.; Greenberger, A.; Hill, K.W.; Meade, D.M.; Roney, W.; Sauthoff, N.R.; von Goeler, S.

    1982-05-01

    Temporally and spatially-resolved profiles of the PDX soft x-ray spectra have been measured during single tokamak pulses of circular and divertor plasmas with a recently developed pulse height analyzer. This detection system incorporates an array of five vertically displaced sets of lithium-drifted silicon detectors, each consisting of three independent channels optimized for rapid data collection in adjacent energy regions. Simultaneous measurement of x-ray emission integrated along five chords of the plasma cross section can thereby be achieved. Abel inversion of these data yields temporally-resolved radial profiles of the local electron temperature from the slope of the continuum, concentrations of high-Z impurities from the characteristic line intensities, and a measure of Z/sub eff/ from the continuum intensity. The techniques of x-ray pulse height analysis, with illustrations featuring the results from the initial PDX circular plasma experiments are discussed in detail. In addition, comparisons between circular and divertor plasmas on PDX, derived from the x-ray measurements, are also presented.

  12. Coherent X-ray diffraction from collagenous soft tissues

    SciTech Connect

    Berenguer de la Cuesta, Felisa; Wenger, Marco P.E.; Bean, Richard J.; Bozec, Laurent; Horton, Michael A.; Robinson, Ian K.

    2009-09-11

    Coherent X-ray diffraction has been applied in the imaging of inorganic materials with great success. However, its application to biological specimens has been limited to some notable exceptions, due to the induced radiation damage and the extended nature of biological samples, the last limiting the application of most part of the phasing algorithms. X-ray ptychography, still under development, is a good candidate to overcome such difficulties and become a powerful imaging method for biology. We describe herein the feasibility of applying ptychography to the imaging of biological specimens, in particular collagen rich samples. We report here speckles in diffraction patterns from soft animal tissue, obtained with an optimized small angle X-ray setup that exploits the natural coherence of the beam. By phasing these patterns, dark field images of collagen within tendon, skin, bone, or cornea will eventually be obtained with a resolution of 60-70 nm. We present simulations of the contrast mechanism in collagen based on atomic force microscope images of the samples. Simulations confirmed the 'speckled' nature of the obtained diffraction patterns. Once inverted, the patterns will show the disposition and orientation of the fibers within the tissue, by enhancing the phase contrast between protein and no protein regions of the sample. Our work affords the application of the most innovative coherent X-ray diffraction tools to the study of biological specimens, and this approach will have a significant impact in biology and medicine because it overcomes many of the limits of current microscopy techniques.

  13. Soft x-ray measurements from the PDX tokamak

    NASA Astrophysics Data System (ADS)

    Silver, E. H.; Bitter, M.; Brau, K.; Eames, D.; Greenberger, A.; Hill, K. W.; Meade, D. M.; Roney, W.; Sauthoff, N. R.; Von Goeler, S.

    1982-08-01

    Temporally and spatially resolved profiles of the PDX soft x-ray spectra have been measured during single tokamak pulses of circular divertor plasmas with a recently developed pulse-height analyzer. This detection system incorporates an array of five vertically displaced sets of lithium-drifted silicon detectors, each consisting of three independent channels optimized for rapid data collection in adjacent energy regions. Simultaneous measurements of x-ray emission integrated along five chords of the plasma cross section can, thereby, be achieved. Abel inversion of these data yields temporally resolved radial profiles of the local electron temperature from the slope of the continuum, concentrations of high-Z impurities from the characteristic line intensities, and a measure of Zeff from the continuum intensity. The techniques of x-ray pulse-height analysis, with illustrations featuring the results from the initial PDX circular plasma experiments, are discussed in detail. In addition, comparisons between circular and divertor plasmas on PDX, derived from the x-ray measurements, are also presented.

  14. Soft x-ray measurements from the PDX tokamak

    SciTech Connect

    Silver, E.H.; Bitter, M.; Brau, K.; Eames, D.; Greenberger, A.; Hill, K.W.; Meade, D.M.; Roney, W.; Sauthoff, N.R.; Von Goeler, S.

    1982-08-01

    Temporally and spatially resolved profiles of the PDX soft x-ray spectra have been measured during single tokamak pulses of circular divertor plasmas with a recently developed pulse-height analyzer. This detection system incorporates an array of five vertically displaced sets of lithium-drifted silicon detectors, each consisting of three independent channels optimized for rapid data collection in adjacent energy regions. Simultaneous measurements of x-ray emission integrated along five chords of the plasma cross section can, thereby, be achieved. Abel inversion of these data yields temporally resolved radial profiles of the local electron temperature from the slope of the continuum, concentrations of high-Z impurities from the characteristic line intensities, and a measure of Z/sub eff/ from the continuum intensity. The techniques of x-ray pulse-height analysis, with illustrations featuring the results from the initial PDX circular plasma experiments, are discussed in detail. In addition, comparisons between circular and divertor plasmas on PDX, derived from the x-ray measurements, are also presented.

  15. Laboratory soft x-ray source with foil target

    NASA Astrophysics Data System (ADS)

    Stephan, Karl-Heinz; Braeuninger, Heinrich W.

    1993-02-01

    We have developed a comparatively small soft x-ray source for application in our test facilities, which are used at present to support the developments of the astrophysical space projects XMM and AXAF. The instrument comprises a commercially available color television tube for generation of the electron beam, which is focused on exchangeable metal films serving as targets. The x rays are taken off after having transversed the foil target and have a sufficient spectral purity with regard to the experimental requirements. The maximum electric operating parameters correspond to an emission current of 100 (mu) A generated by a filament heating power of 6.6 watt at an accelerating voltage of 25 kV. The technical advantages of the instrument are lightweight construction, no water cooling, small size electric supply, cost efficient manufacturing, small sized focus, and quick access to the desired characteristic spectral line by exchange of a complete tube. We describe the measurements on the local x-ray intensity profile of the focus, the spectral features of the beam, and present the resulting performance data. A special development could be used as calibration sources in x-ray telescopes.

  16. The correlation of solar flare hard X-ray bursts with Doppler blueshifted soft X-ray flare emission

    NASA Technical Reports Server (NTRS)

    Bentley, R. D.; Doschek, G. A.; Simnett, G. M.; Rilee, M. L.; Mariska, J. T.; Culhane, J. L.; Kosugi, T.; Watanabe, T.

    1994-01-01

    We have investigated the temporal correlation between hard X-ray bursts and the intensity of Doppler blueshifted soft X-ray spectral line emission. We find a strong correlation for many events that have intense blueshifted spectral signatures and some correlation in events with modest blueshifts. The onset of hard X-rays frequently coincides to within a few seconds with the onset of blueshifted emission. The peak intensity of blueshifted emission is frequently close in time to the peak of the hard X-ray emission. Decay rates of the blueshifted and hard X-ray emission are similar, with the decay of the blueshifted emission tending to lag behind the hard X-ray emission in some cases. There are, however, exceptions to these conclusions, and, therefore, the results should not be generalized to all flares. Most of the data for this work were obtained from instruments flown on the Japanese Yohkoh solar spacecraft.

  17. Soft X-ray scanning transmission X-ray microscopy (STXM) of actinide particles.

    PubMed

    Nilsson, Hans J; Tyliszczak, Tolek; Wilson, Richard E; Werme, Lars; Shuh, David K

    2005-09-01

    A descriptive account is given of our most recent research on the actinide dioxides with the Advanced Light Source Molecular Environmental Science (ALS-MES) Beamline 11.0.2 soft X-ray scanning transmission X-ray microscope (STXM) at the Lawrence Berkeley National Laboratory (LBNL). The ALS-MES STXM permits near-edge X-ray absorption fine structure (NEXAFS) and imaging with 30-nm spatial resolution. The first STXM spectromicroscopy NEXAFS spectra at the actinide 4d5/2 edges of the imaged transuranic particles, NpO2 and PuO2, have been obtained. Radiation damage induced by the STXM was observed in the investigation of a mixed oxidation state particle (Np(V,VI)) and was minimized during collection of the actual spectra at the 4d5/2 edge of the Np(V,VI) solid. A plutonium elemental map was obtained from an irregular PuO2 particle with the dimensions of 650 x 650 nm. The Pu 4d5/2 NEXAFS spectra were collected at several different locations from the PuO2 particle and were identical. A representative oxygen K-edge spectrum from UO2 was collected and resembles the oxygen K-edge from the bulk material. The unique and current performance of the ALS-MES STXM at extremely low energies (ca. 100 eV) that may permit the successful measurement of the actinide 5d edge is documented. Finally, the potential of STXM as a tool for actinide investigations is briefly discussed. PMID:16021423

  18. Soft X-ray scanning transmission X-ray microscopy (STXM) of actinide particles.

    PubMed

    Nilsson, Hans J; Tyliszczak, Tolek; Wilson, Richard E; Werme, Lars; Shuh, David K

    2005-09-01

    A descriptive account is given of our most recent research on the actinide dioxides with the Advanced Light Source Molecular Environmental Science (ALS-MES) Beamline 11.0.2 soft X-ray scanning transmission X-ray microscope (STXM) at the Lawrence Berkeley National Laboratory (LBNL). The ALS-MES STXM permits near-edge X-ray absorption fine structure (NEXAFS) and imaging with 30-nm spatial resolution. The first STXM spectromicroscopy NEXAFS spectra at the actinide 4d5/2 edges of the imaged transuranic particles, NpO2 and PuO2, have been obtained. Radiation damage induced by the STXM was observed in the investigation of a mixed oxidation state particle (Np(V,VI)) and was minimized during collection of the actual spectra at the 4d5/2 edge of the Np(V,VI) solid. A plutonium elemental map was obtained from an irregular PuO2 particle with the dimensions of 650 x 650 nm. The Pu 4d5/2 NEXAFS spectra were collected at several different locations from the PuO2 particle and were identical. A representative oxygen K-edge spectrum from UO2 was collected and resembles the oxygen K-edge from the bulk material. The unique and current performance of the ALS-MES STXM at extremely low energies (ca. 100 eV) that may permit the successful measurement of the actinide 5d edge is documented. Finally, the potential of STXM as a tool for actinide investigations is briefly discussed.

  19. Inelastic x-ray scattering at modest energy resolution

    SciTech Connect

    Finkelstein, K. D.; Tischler, J. Z.; Larson, B. C.

    1997-07-01

    We report results from the development of an inelastic scattering spectrometer designed to take advantage of high energy synchrotron radiation available at CHESS. The device allows a large increase of the effective scattering volume in the sample by permitting measurements to be made in an energy range up to 25 KeV. The highest useable energy appears limited by the efficiency of the analyzers under consideration. At 20 KeV a novel 4-bounce, sagittal focusing monochromator passes 10e11 photons/second with Darwin width limited energy resolution. In the scattering plane, the monochromator images the electron beam producing a small scattering source for the analyzing optics. Analyzer systems under study include a cooled mosaic crystal in para-focusing geometry, and an adjustable spherically bent silicon crystal respectively for parallel and point-by-point collection of the energy loss spectrum. This paper discusses the optical configurations presents results from our early measurements and suggests directions for improvements.

  20. A Soft X-ray Spectrometer using a Highly Dispersive Multilayer Grating

    NASA Astrophysics Data System (ADS)

    Warwick, Tony; Padmore, Howard; Voronov, Dmitriy; Yashchuk, Valeriy

    2010-06-01

    There is a need for higher resolution spectrometers as a tool for inelastic x-ray scattering. Currently, resolving power around R = 10,000 is advertised. Measured RIXS spectra are often limited by this instrumental resolution and higher resolution spectrometers using conventional gratings would be prohibitively large. We are engaged in a development program to build blazed multilayer grating structures for diffracting soft x-rays in high order. This leads to spectrometers with dispersion much higher than is possible using metal coated-gratings. The higher dispersion then provides higher resolution and the multilayer gratings are capable of operating away from grazing incidence as required. A spectrometer design is presented with a total length 3.8 m and capable of 105 resolving power.

  1. A Soft X-ray Spectrometer using a Highly Dispersive Multilayer Grating

    SciTech Connect

    Warwick, Tony; Padmore, Howard; Voronov, Dmitriy; Yashchuk, Valeriy

    2010-01-31

    There is a need for higher resolution spectrometers as a tool for inelastic x-ray scattering. Currently, resolving power around R = 10,000 is advertised. Measured RIXS spectra are often limited by this instrumental resolution and higher resolution spectrometers using conventional gratings would be prohibitively large. We are engaged in a development program to build blazed multilayer grating structures for diffracting soft x-rays in high order. This leads to spectrometers with dispersion much higher than is possible using metal coated-gratings. The higher dispersion then provides higher resolution and the multilayer gratings are capable of operating away from grazing incidence as required. A spectrometer design is presented with a total length 3.8m and capable of 10{sup 5} resolving power.

  2. Characterizing automotive fuel cell materials by soft x-ray scanning transmission x-ray microscopy

    NASA Astrophysics Data System (ADS)

    Hitchcock, A. P.; Lee, V.; Wu, J.; West, M. M.; Cooper, G.; Berejnov, V.; Soboleva, T.; Susac, D.; Stumper, J.

    2016-01-01

    Proton-Exchange Membrane Fuel Cell (PEM-FC) based engines are being developed rapidly for near-term implementation in hydrogen fueled, mass production, personal automobiles. Research is focused on understanding and controlling various degradation processes (carbon corrosion, Pt migration, cold start), and reducing cost by reducing or eliminating Pt catalyst. We are using soft X-ray scanning transmission X-ray microscopy (STXM) at the S 2p, C 1s, O 1s and F 1s edges to study a variety of issues related to optimization of PEM-FC materials for automotive applications. A method to efficiently and accurately measure perfluorosulfonic acid distributions was developed and is being used to better understand how different loadings and preparation methods affect the ionomer distribution in the cathode. Progress towards an environmental cell capable of controlling the temperature and humidity of a PEM-FC sample in the STXM is described. Methods for studying the 3D chemical structure of PEM-FC are outlined.

  3. ASTRO-H Soft X-ray Telescope (SXT)

    NASA Astrophysics Data System (ADS)

    Soong, Yang; Serlemitsos, Peter J.; Okajima, Takashi; Hahne, Devin

    2011-09-01

    ASTRO-H is an astrophysics satellite dedicated for X-ray spectroscopic study non-dispersively and to carry out survey complementally, which will be borne out of US-Japanese collaborative effort. Among the onboard instruments there are four conically approximated Wolter-I X-ray mirrors, among which two of them are soft X-ray mirrors1, of which the energy range is from a few hundred eV to 15 keV, currently being fabricated in the X-ray Optics Lab at Goddard Space Flight Center. The focal point instruments will be a calorimeter (SXS) and a CCD camera (SXI), respectively. The reflectors of the mirror are made of heat-formed aluminum substrate of the thickness gauged of 152 μm, 229 μm, and 305 μm of the alloy 5052 H-19, followed by epoxy replication on gold-sputtered smooth Pyrex cylindrical mandrels to acquire the X-ray reflective surface. The epoxy layer is 10 μm nominal and surface gold layer of 0.2 μm. Improvements on angular response over the Astro-E1/Suzaku mirrors come from error reduction on the figure, the roundness, and the grazing angle/radius mismatching of the reflecting surface, and tighter specs and mechanical strength on supporting structure to reduce the reflector positioning and the assembly errors. In this paper, we report the results of calibration of the engineering model of SXT (EM), and project the quality of the flight mirrors.

  4. Goldhelox: a soft x-ray solar telescope.

    PubMed

    Durfee, D S; Moody, J W; Brady, K D; Brown, C; Campbell, B; Durfee, M K; Early, D; Hansen, E; Madsen, D W; Morey, D B; Roming, P W; Savage, M B; Eastman, P F; Jensen, V

    1995-01-01

    The Goldhelox Project is the construction and use of a near-normal incidence soft x-ray robotic solar telescope by undergraduate students at Brigham Young University. Once it is completed and tested, it will be deployed from a Get-Away-Special (GAS) canister in the bay of a space shuttle. It will image the sun at a wavelength of 171-181Å with a time resolution of 1 sec and a spatial resolution of 2.5 arcsec. The observational bandpass was chosen to image x-rays from highly ionized coronal Fe lines. The data will be an aid in better understanding the beginning phases of solar flares and how flaring relates to the physics of the corona-chromosphere transition region. Goldhelox is tentatively scheduled to fly on a space shuttle sometime in 1995 or 1996. This paper outlines the project goals, basic instrument design, and the unique aspects of making this an undergraduate endeavor. PMID:21307474

  5. Soft X-ray photoemission studies of Hf oxidation

    SciTech Connect

    Suzer, S.; Sayan, S.; Banaszak Holl, M.M.; Garfunkel, E.; Hussain, Z.; Hamdan, N.M.

    2002-02-01

    Soft X-Ray Photoemission Spectroscopy using surface sensitive Synchrotron Radiation has been applied to accurately determine the binding energy shifts and the valence band offset of the HfO2 grown on Hf metal. Charging of oxide films under x-rays (or other irradiation) is circumvented by controlled and sequential in-situ oxidation. Photoemission results show the presence of metallic Hf (from the substrate) with the 4f7/2 binding energy of 14.22 eV, fully oxidized Hf (from HfO2) with the 4f7/2 binding energy of 18.16 eV, and at least one clear suboxide peak. The position of the valence band of HfO2 with respect to the Hf(m) Fermi level is determined as 4.05 eV.

  6. DISENTANGLING AGN AND STAR FORMATION IN SOFT X-RAYS

    SciTech Connect

    LaMassa, Stephanie M.; Heckman, T. M.; Ptak, A.

    2012-10-20

    We have explored the interplay of star formation and active galactic nucleus (AGN) activity in soft X-rays (0.5-2 keV) in two samples of Seyfert 2 galaxies (Sy2s). Using a combination of low-resolution CCD spectra from Chandra and XMM-Newton, we modeled the soft emission of 34 Sy2s using power-law and thermal models. For the 11 sources with high signal-to-noise Chandra imaging of the diffuse host galaxy emission, we estimate the luminosity due to star formation by removing the AGN, fitting the residual emission. The AGN and star formation contributions to the soft X-ray luminosity (i.e., L{sub x,AGN} and L{sub x,SF}) for the remaining 24 Sy2s were estimated from the power-law and thermal luminosities derived from spectral fitting. These luminosities were scaled based on a template derived from XSINGS analysis of normal star-forming galaxies. To account for errors in the luminosities derived from spectral fitting and the spread in the scaling factor, we estimated L{sub x,AGN} and L{sub x,SF} from Monte Carlo simulations. These simulated luminosities agree with L{sub x,AGN} and L{sub x,SF} derived from Chandra imaging analysis within a 3{sigma} confidence level. Using the infrared [Ne II]12.8 {mu}m and [O IV]26 {mu}m lines as a proxy of star formation and AGN activity, respectively, we independently disentangle the contributions of these two processes to the total soft X-ray emission. This decomposition generally agrees with L{sub x,SF} and L{sub x,AGN} at the 3{sigma} level. In the absence of resolvable nuclear emission, our decomposition method provides a reasonable estimate of emission due to star formation in galaxies hosting type 2 AGNs.

  7. Disentangling AGN and Star Formation in Soft X-Rays

    NASA Technical Reports Server (NTRS)

    LaMassa, Stephanie M.; Heckman, T. M.; Ptak, A.

    2012-01-01

    We have explored the interplay of star formation and active galactic nucleus (AGN) activity in soft X-rays (0.5-2 keV) in two samples of Seyfert 2 galaxies (Sy2s). Using a combination of low-resolution CCD spectra from Chandra and XMM-Newton, we modeled the soft emission of 34 Sy2s using power-law and thermal models. For the 11 sources with high signal-to-noise Chandra imaging of the diffuse host galaxy emission, we estimate the luminosity due to star formation by removing the AGN, fitting the residual emission. The AGN and star formation contributions to the soft X-ray luminosity (i.e., L(sub x,AGN) and L(sub x,SF)) for the remaining 24 Sy2s were estimated from the power-law and thermal luminosities derived from spectral fitting. These luminosities were scaled based on a template derived from XSINGS analysis of normal star-forming galaxies. To account for errors in the luminosities derived from spectral fitting and the spread in the scaling factor, we estimated L(sub x,AGN) and L(sub x,SF))from Monte Carlo simulations. These simulated luminosities agree with L(sub x,AGN) and L(sub x,SF) derived from Chandra imaging analysis within a 3sigma confidence level. Using the infrared [Ne ii]12.8 micron and [O iv]26 micron lines as a proxy of star formation and AGN activity, respectively, we independently disentangle the contributions of these two processes to the total soft X-ray emission. This decomposition generally agrees with L(sub x,SF) and L(sub x,AGN) at the 3 sigma level. In the absence of resolvable nuclear emission, our decomposition method provides a reasonable estimate of emission due to star formation in galaxies hosting type 2 AGNs.

  8. Inelastic x-ray scattering at modest energy resolution

    SciTech Connect

    Finkelstein, K.D.; Larson, B.C.

    1997-07-01

    We report results from the development of an inelastic scattering spectrometer designed to take advantage of high energy synchrotron radiation available at CHESS. The device allows a large increase of the effective scattering volume in the sample by permitting measurements to be made in an energy range up to 25 KeV. The highest useable energy appears limited by the efficiency of the analyzers under consideration. At 20 KeV a novel 4-bounce, sagittal focusing monochromator passes 10e11 photons/second with Darwin width limited energy resolution. In the scattering plane, the monochromator images the electron beam producing a small scattering source for the analyzing optics. Analyzer systems under study include a cooled mosaic crystal in para-focusing geometry, and an adjustable spherically bent silicon crystal respectively for parallel and point-by-point collection of the energy loss spectrum. This paper discusses the optical configurations presents results from our early measurements and suggests directions for improvements. {copyright} {ital 1997 American Institute of Physics.}

  9. Comparison of hard and soft x-ray photoelectron spectra of silicon

    NASA Astrophysics Data System (ADS)

    Offi, F.; Werner, W. S. M.; Sacchi, M.; Torelli, P.; Cautero, M.; Cautero, G.; Fondacaro, A.; Huotari, S.; Monaco, G.; Paolicelli, G.; Smekal, W.; Stefani, G.; Panaccione, G.

    2007-08-01

    A detailed comparison of the surface sensitivity of x-ray photoemission spectroscopy for hard and soft x rays is presented and discussed. Electron scattering parameters and their energy dependence are given for Si and two Si spectra are analyzed: a MgKα (hν=1253.6eV) excited spectrum of the Si2p and 2s lines and a hard x-ray excited spectrum (hν=5925eV) of the Si1s line. The differential inelastic scattering characteristics for Si are extracted from reflection electron energy loss spectra taken at energies of 1500 and 4000eV . Using these scattering characteristics and electron mean free paths from the literature, simulated spectra are compared with experiment. The experimental spectra are deconvoluted to give the true intrinsic line shape corresponding to the theoretical collision statistics when interference effects between intrinsic and extrinsic scattering are neglected. The magnitude of interference effects cannot be assessed by our analysis. Within the (unknown) uncertainty introduced by neglecting interference effects, it is possible to determine the relative intensity of intrinsic and extrinsic excitations. In this way, it is found that in the case of the soft x-ray excited photoelectron spectrum of the shallower electronic shells ( 2p and 2s ), intrinsic plasmon creation is rather weak, and the apparent asymmetric line shape of the spectrum might be interpreted as the fact that electron-hole pair creation dominates the intrinsic loss spectrum, while an alternative explanation in terms of surface core level shifted components is also proposed. For the deeper core electronic shell, probed with hard x rays, the opposite situation is observed: while intrinsic electron-hole pair creation was not observed, a strong contribution of intrinsic plasmon losses of about 30% was seen.

  10. Toroidal silicon polarization analyzer for resonant inelastic x-ray scattering

    NASA Astrophysics Data System (ADS)

    Gao, Xuan; Casa, Diego; Kim, Jungho; Gog, Thomas; Li, Chengyang; Burns, Clement

    2016-08-01

    Resonant Inelastic X-ray Scattering (RIXS) is a powerful probe for studying electronic excitations in materials. Standard high energy RIXS measurements do not measure the polarization of the scattered x-rays, which is unfortunate since it carries information about the nature and symmetry of the excitations involved in the scattering process. Here we report the fabrication of thin Si-based polarization analyzers with a double-concave toroidal surface, useful for L-edge RIXS studies in heavier atoms such as the 5-d transition metals.

  11. Toroidal silicon polarization analyzer for resonant inelastic x-ray scattering.

    PubMed

    Gao, Xuan; Casa, Diego; Kim, Jungho; Gog, Thomas; Li, Chengyang; Burns, Clement

    2016-08-01

    Resonant Inelastic X-ray Scattering (RIXS) is a powerful probe for studying electronic excitations in materials. Standard high energy RIXS measurements do not measure the polarization of the scattered x-rays, which is unfortunate since it carries information about the nature and symmetry of the excitations involved in the scattering process. Here we report the fabrication of thin Si-based polarization analyzers with a double-concave toroidal surface, useful for L-edge RIXS studies in heavier atoms such as the 5-d transition metals. PMID:27587100

  12. Energy calibration of a high-resolution inelastic x-ray scattering spectrometer

    SciTech Connect

    Verbeni, Roberto; D'Astuto, Matteo; Krisch, Michael; Lorenzen, Maren; Mermet, Alain; Monaco, Giulio; Requardt, Herwig; Sette, Francesco

    2008-08-15

    The energy scale of a triple-axis x-ray spectrometer with meV energy resolution based on perfect silicon crystal optics is calibrated, utilizing the most recent determination of the silicon lattice parameter and its thermal expansion coefficient and recording the dispersion of longitudinal acoustic and optical phonons in a diamond single crystal and the molecular vibration mode in liquid nitrogen. Comparison of the x-ray results with previous inelastic neutron and Raman scattering results as well as with ab initio phonon dispersion calculations yields an overall agreement better than 2%.

  13. Resonant inelastic x-ray scattering at the limit of subfemtosecond natural lifetime

    SciTech Connect

    Marchenko, T.; Journel, L.; Marin, T.; Guillemin, R.; Carniato, S.; Simon, M.; Zitnik, M.; Kavcic, M.; Bucar, K.; Mihelic, A.; Hoszowska, J.; Cao, W.

    2011-04-14

    We present measurements of the resonant inelastic x-ray scattering (RIXS) spectra of the CH{sub 3}I molecule in the hard-x-ray region near the iodine L{sub 2} and L{sub 3} absorption edges. We show that dispersive RIXS spectral features that were recognized as a fingerprint of dissociative molecular states can be interpreted in terms of ultrashort natural lifetime of {approx}200 attoseconds in the case of the iodine L-shell core-hole. Our results demonstrate the capacity of the RIXS technique to reveal subtle dynamical effects in molecules with sensitivity to nuclear rearrangement on a subfemtosecond time scale.

  14. Toroidal silicon polarization analyzer for resonant inelastic x-ray scattering.

    PubMed

    Gao, Xuan; Casa, Diego; Kim, Jungho; Gog, Thomas; Li, Chengyang; Burns, Clement

    2016-08-01

    Resonant Inelastic X-ray Scattering (RIXS) is a powerful probe for studying electronic excitations in materials. Standard high energy RIXS measurements do not measure the polarization of the scattered x-rays, which is unfortunate since it carries information about the nature and symmetry of the excitations involved in the scattering process. Here we report the fabrication of thin Si-based polarization analyzers with a double-concave toroidal surface, useful for L-edge RIXS studies in heavier atoms such as the 5-d transition metals.

  15. A wide-field soft X-ray camera

    NASA Technical Reports Server (NTRS)

    Petre, R.

    1981-01-01

    A wide-field soft X-ray camera (WFSXC) sensitive in the 50 to 250 eV band is described. The camera features Wolter-Schwarzschild optics with an 8 degree field of view and 300 cu cu collecting area. The focal plane instrument is a microchannel plate detector. Broad-band energy discrimination is provided by thin-film filters mounted immediately in front of the focal plane. The WFSXC is capable of detecting sources with intensities greater than 5 percent of HZ 43 during typical sounding rocket exposures, and it would approach the same sensitivity range as EUVE during a typical exposure from the Shuttle.

  16. Soft X-ray microscopy to characterize polyelectrolyte assemblies.

    PubMed

    Köhler, Karen; Déjugnat, Christophe; Dubois, Monique; Zemb, Thomas; Sukhorukov, Gleb B; Guttmann, Peter; Möhwald, Helmuth

    2007-07-26

    Transmission microscopy with soft X-rays (TXM) is applied to image in-situ polyelectrolyte assemblies in aqueous environment. The method is element specific and at this stage exhibits a lateral resolution of 20 nm. With the specific examples of hollow capsules and full spheres made of PAH/PSS polyelectrolyte multilayers, it is shown quantitatively that heat treatment irreversibly reduces the water content in the membrane. These experiments complement those reported recently on the polyion system PDADMAC/PSS, which shows a different glass-transition behavior. Finally, the potential and present limitations of TXM are discussed. PMID:17428089

  17. Soft X-ray Microscopy of Green Cements

    NASA Astrophysics Data System (ADS)

    Monteiro, P. J. M.; Mancio, M.; Kirchheim, A. P.; Chae, R.; Ha, J.; Fischer, P.; Tyliszczak, T.

    2011-09-01

    The present status of the cement and concrete industry is not sustainable. The production of Portland cement is responsible for 7% of the CO2 emissions in the world and existing reinforced concrete infrastructure is deteriorating at a fast pace. The change in the existing technology requires new developments in our understanding of the nanostructure of hydration products and the complex deterioration reactions. We have been developing an elaborate research program to advance the existing cement and concrete science by characterizing its nanostructure by synchrotron radiation. A new generation of green cements is being studied using high-resolution soft x-ray microscopy at the nano-level.

  18. Soft X-ray Microscopy of Green Cements

    SciTech Connect

    Monteiro, P. J. M.; Mancio, M.; Chae, R.; Ha, J.; Kirchheim, A. P.; Fischer, P.; Tyliszczak, T.

    2011-09-09

    The present status of the cement and concrete industry is not sustainable. The production of Portland cement is responsible for 7% of the CO{sub 2} emissions in the world and existing reinforced concrete infrastructure is deteriorating at a fast pace. The change in the existing technology requires new developments in our understanding of the nanostructure of hydration products and the complex deterioration reactions. We have been developing an elaborate research program to advance the existing cement and concrete science by characterizing its nanostructure by synchrotron radiation. A new generation of green cements is being studied using high-resolution soft x-ray microscopy at the nano-level.

  19. Superconducting tunnel junction detectors for soft x-ray astrophysics

    NASA Astrophysics Data System (ADS)

    Verhoeve, P.; Hijmering, R. A.; Martin, D. D. E.; Jerjen, I.; Peacock, A.; Venn, R.

    2006-06-01

    The requirement on energy resolution for detectors in future X-ray satelite missions such as XEUS (X-ray Evolving Universe Spectroscopy mission) is <2eV in the soft x-ray range of 50-2000 eV, with a detection efficiency >80%. In addition, the requirements for field of view and angular resolution demand a detector array of typically 150x150 micron sized pixels in a 30x30 pixel format. DROIDs (Distributed Read Out Imaging Devices), consisting of a superconducting absorber strip with superconducting tunnel junctions (STJs) as read-out devices on either end, can fulfill these requirements. The amplitudes of the two signals from the STJs provide information on the absorption position and the energy of the incoming photon in the absorber. In this paper we present the development status of Ta/Al 1-D DROIDs, as well as the the short term development program that should result in a full size XEUS array.

  20. Soft x-rays measurements in a dense plasma focus

    SciTech Connect

    Castillo, F.; Milanese, M.; Moroso, R.; Pouzo, J.

    1994-12-31

    Soft X-Rays emitted from a 2 kJ DPF are detected. Deuterium or a mixture of deuterium and argon is used as filling gas. The DPF is operated in static filling D{sub 2} gas pressure ({approximately} 2 mb) or in gas-puff mode. The image of the emitting area (time integrated) is taken with a 5 holes X-Rays pin-hole camera. The visible light is filtered using Al foils of different thickness in each one of the 5 holes. The image is a fine line ({approximately} 1 cm long) on the PF axis, into which several bright points can be observed. An estimation of the emitting zone temperature is performed through measurements of transmittance in each hole using radiographic plates densitometry. The background plasma emission corresponds to a temperature between 1 and 2 keV, in both normal and gas-puff modes. The temperature estimated for the bright points results higher by a factor 2 respect to the plasma bulk. Simultaneous measurements of time resolved X-Rays pulses using a PIN diode with Be filter, and both time resolved and time integrated neutron flux detection are performed.

  1. The Astro-H Soft X-ray Spectrometer (SXS)

    NASA Astrophysics Data System (ADS)

    Porter, F. Scott; Fujimoto, Ryuichi; Kelley, Richard L.; Kilbourne, Caroline A.; Mitsuda, Kazuhiasa; Ohashi, Takaya; Astro-H/SXS Collaboration

    2009-12-01

    The Soft-X-ray Spectrometer (SXS) is a high spectral resolution, cryogenic x-ray spectrometer that will fly on the Japan/U.S. Astro-H observatory in 2014. The SXS is composed of a 36 pixel, imaging, x-ray calorimeter array that will operate at 0.05 K utilizing a 2-stage adiabatic demagnetization refrigerator and a redundant pre-cooler design using both a 40 liter liquid helium tank and a 1.7 K Joule-Thomson (JT) cryocooler. Additional redundant Stirling cycle coolers provide pre-cooling for the (JT) and cool the outer thermal shields for the JT and the helium tank. The detector system, while similar to that flown on Suzaku, is composed of larger 0.81×0.81mm pixels, but has significantly better performance, currently predicted to be better than 4 eV FWHM at 6 keV with 95% quantum efficiency. This instrument is the result of a close collaboration between many institutions in the U.S. and Japan over the last 25 years. Here we will present an overview of the SXS instrument, the SXS cooling system, and recent laboratory improvements to the detector system.

  2. Synoptic IPS and Yohkoh soft X-ray observations

    NASA Technical Reports Server (NTRS)

    Hick, P.; Jackson, B. V.; Rappoport, S.; Woan, G.; Slater, G.; Strong, K.; Uchida, Y.

    1995-01-01

    Interplanetary scintillation measurements of the disturbance factor, g, from October 1991 to October 1992 are used to construct synoptic Carrington maps. These maps, which show the structure of the quiet solar wind, are compared with X-ray Carrington maps from the Yohkoh Soft X-ray Telescope (SXT) instrument. For the period studied the global structure outlined by (weakly) enhanced g-values apparent in the interplanetary scintillation (IPS) maps tend to match the active regions (as shown in the X-ray maps) significantly better than the heliospheric current sheet. Contrary to traditional opinion, which views active regions as magnetically closed structures that do not have any significant impact on the solar wind flow, our results suggest that density fluctuations in the solar wind are significantly enhanced over active regions. These results support the suggestion by Uchida et al. (1992), based on Yohkoh observations of expanding active regions, that active regions play a role in feeding mass into the quiet solar wind.

  3. Laser produced plasma soft x-ray generation

    SciTech Connect

    Cerjan, C.; Rosen, M.D.

    1991-05-20

    The efficiency of soft x-ray production from laser-irradiated plasmas is simulated for two different spectral regions. These two regions, 14{Angstrom} {plus minus} 15% and 130{Angstrom} {plus minus} 1%, were chosen for proximity mask or point-projection technological applications. Relatively large conversion efficiencies were obtained from irradiation of a stainless steel target using the conditions suggested by recent Hampshire Instruments' experiments for proximity masking. Pulse-width and laser frequency parameter studies were performed for point-projection applications which suggest that the conversion applications which suggest that the conversion efficiency is sensitive to pulse-width but not to laser frequency. One of the critical components of any x-ray lithographic scheme is of course the x-ray laser source. There are two primary contenders for a reliable, efficient source currently: synchrotron radiation and spectral emission from laser produced plasma. The dominant issue for laser-plasma emission is the conversion efficiency -- output in the intended operating spectral region relative the required incident laser energy. Simulations are described in the following for both high and low energy spectral regions which have been suggested by either the proximity masking or point-projection technology.

  4. The Astro-H Soft X-Ray Mirror

    NASA Technical Reports Server (NTRS)

    Robinson, David; Okajima, Takashi; Serlemitsos, Peter; Soong, Yang

    2012-01-01

    The Astro-H is led by the Japanese Space Agency (JAXA) in collaboration with many other institutions including the NASA Goddard Space Flight Center. Goddard's contributions include two soft X-ray telescopes (SXTs). The telescopes have an effective area of 562 square cm at 1 keV and 425 square cm at 6 keV with an image quality requirement of 1.7 arc-minutes half power diameter (HPD). The engineering model has demonstrated 1.1 arc-minutes HPD error. The design of the SXT is based on the successful Suzaku mission mirrors with some enhancements to improve the image quality. Two major enhancements are bonding the X-ray mirror foils to alignment bars instead of allowing the mirrors to float, and fabricating alignment bars with grooves within 5 microns of accuracy. An engineering model SXT was recently built and subjected to several tests including vibration, thermal, and X-ray performance in a beamline. Several lessons were learned during this testing that will be incorporated in the flight design. Test results and optical performance are discussed, along with a description of the design of the SXT.

  5. Observing soft X-ray line emission from the interstellar medium with X-ray calorimeter on a sounding rocket

    NASA Technical Reports Server (NTRS)

    Zhang, J.; Edwards, B.; Juda, M.; Mccammon, D.; Skinner, M.; Kelley, R.; Moseley, H.; Schoelkopf, R.; Szymkowiak, A.

    1990-01-01

    For an X-ray calorimeter working at 0.1 K, the energy resolution ideally can be as good as one eV for a practical detector. A detector with a resolution of 17 eV FWHM at 6 keV has been constructed. It is expected that this can be improved by a factor of two or more. With X-ray calorimeters flown on a sounding rocket, it should be possible to observe soft X-ray line emission from the interstellar medium over the energy range 0.07 to 1 keV. Here, a preliminary design for an X-ray calorimeter rocket experiment and the spectrum which might be observed from an equilibrium plasma are presented. For later X-ray calorimeter sounding rocket experiments, it is planned to add an aluminum foil mirror with collecting area of about 400 sq cm to observe line features from bright supernova remnants.

  6. Soft X-Ray and Vacuum Ultraviolet Based Spectroscopy of the Actinides

    SciTech Connect

    Tobin, J G

    2011-03-17

    The subjects of discussion included: VUV photoelectron spectroscopy, X-ray photoelectron spectroscopy, Synchrotron-radiation-based photoelectron spectroscopy, Soft x-ray absorption spectroscopy, Soft x-ray emission spectroscopy, Inverse photoelectron spectroscopy, Bremstrahlung Isochromat Spectroscopy, Low energy IPES, Resonant inverse photoelectron spectroscopy.

  7. Opening the Field of Soft X-ray Polarimetry

    NASA Astrophysics Data System (ADS)

    Marshall, Herman L.; Schulz, Norbert; Windt, David; Gullikson, Eric

    2015-08-01

    We present development of a telescope for measuring linear X-ray polarization over the 0.2-0.8 keV band. We employ multilayer-coated mirrors as Bragg reflectors at the Brewster angle. By matching to the dispersion of a spectrometer, one may take advantage of high multilayer reflectivities and achieve polarization modulation factors over 90%. We have constructed a source of polarized X-rays that operates at a wide range of energies with a selectable polarization angle. Previously, we demonstrated that the polarimetry beam-line provides 100% polarized X-rays at 0.525 keV (Marshall et al. 2013). Recently, we upgraded the source by installing a mirror with a laterally graded multilayer (LGML) coating, providing a wide energy range. Here, we will present results from continued development that includes LGMls of new material combinations (C/CrCo and La/B4C) with high efficiencies in different soft X-ray bands. We have also sponsored the development of new gratings and anticipate showing results from testing these new gratings. Finally, we will present a design for a small telescope for suborbital or orbital missions. A suborbital mission would be limited to measuring the polarization of a blazar such as Mk 421 to a few percent while an orbital version could measure the polarizations of neutron stars, active galactic nuclei, and blazars.Support for this work was provided by the National Aeronautics and Space Administration through grant NNX12AH12G and by Research Investment Grants from the MIT Kavli Institute.

  8. Resonant magnetic scattering of polarized soft x rays

    SciTech Connect

    Sacchi, M.; Hague, C.F.; Gullikson, E.M.; Underwood, J.

    1997-04-01

    Magnetic effects on X-ray scattering (Bragg diffraction, specular reflectivity or diffuse scattering) are a well known phenomenon, and they also represent a powerful tool for investigating magnetic materials since it was shown that they are strongly enhanced when the photon energy is tuned across an absorption edge (resonant process). The resonant enhancement of the magnetic scattering has mainly been investigated at high photon energies, in order to match the Bragg law for the typical lattice spacings of crystals. In the soft X-ray range, even larger effects are expected, working for instance at the 2p edges of transition metals of the first row or at the 3d edges of rare earths (300-1500 eV), but the corresponding long wavelengths prevent the use of single crystals. Two approaches have been recently adopted in this energy range: (i) the study of the Bragg diffraction from artificial structures of appropriate 2d spacing; (ii) the analysis of the specular reflectivity, which contains analogous information but has no constraints related to the lattice spacing. Both approaches have their own specific advantages: for instance, working under Bragg conditions provides information about the (magnetic) periodicity in ordered structures, while resonant reflectivity can easily be related to electronic properties and absorption spectra. An important aspect common to all the resonant X-ray scattering techniques is the element selectivity inherent to the fact of working at a specific absorption edge: under these conditions, X-ray scattering becomes in fact a spectroscopy. Results are presented for films of iron and cobalt.

  9. Coherent X-ray diffraction from collagenous soft tissues

    PubMed Central

    Berenguer de la Cuesta, Felisa; Wenger, Marco P. E.; Bean, Richard J.; Bozec, Laurent; Horton, Michael A.; Robinson, Ian K.

    2009-01-01

    Coherent X-ray diffraction has been applied in the imaging of inorganic materials with great success. However, its application to biological specimens has been limited to some notable exceptions, due to the induced radiation damage and the extended nature of biological samples, the last limiting the application of most part of the phasing algorithms. X-ray ptychography, still under development, is a good candidate to overcome such difficulties and become a powerful imaging method for biology. We describe herein the feasibility of applying ptychography to the imaging of biological specimens, in particular collagen rich samples. We report here speckles in diffraction patterns from soft animal tissue, obtained with an optimized small angle X-ray setup that exploits the natural coherence of the beam. By phasing these patterns, dark field images of collagen within tendon, skin, bone, or cornea will eventually be obtained with a resolution of 60–70 nm. We present simulations of the contrast mechanism in collagen based on atomic force microscope images of the samples. Simulations confirmed the ‘speckled’ nature of the obtained diffraction patterns. Once inverted, the patterns will show the disposition and orientation of the fibers within the tissue, by enhancing the phase contrast between protein and no protein regions of the sample. Our work affords the application of the most innovative coherent X-ray diffraction tools to the study of biological specimens, and this approach will have a significant impact in biology and medicine because it overcomes many of the limits of current microscopy techniques. PMID:19706395

  10. Soft x-ray spectroscopy studies of novel electronic materials using synchrotron radiation

    NASA Astrophysics Data System (ADS)

    Newby, David, Jr.

    surface evolution of these films is discussed, and the effects of different gas environments on oxygen vacancy concentration are elucidated. LSMO is commonly used in commercial fuel cell devices. Here the resonant soft x-ray emission (RIXS) spectrum of LSMO is examined, and it is shown that the inelastic x-ray emission structure of LSMO arises from local atomic multiplet effects.

  11. Investigation of the Ionic Hydration in Aqueous Salt Solutions by Soft X-ray Emission Spectroscopy.

    PubMed

    Jeyachandran, Y L; Meyer, F; Benkert, A; Bär, M; Blum, M; Yang, W; Reinert, F; Heske, C; Weinhardt, L; Zharnikov, M

    2016-08-11

    Understanding the molecular structure of the hydration shells and their impact on the hydrogen bond (HB) network of water in aqueous salt solutions is a fundamentally important and technically relevant question. In the present work, such hydration effects were studied for a series of representative salt solutions (NaCl, KCl, CaCl2, MgCl2, and KBr) by soft X-ray emission spectroscopy (XES) and resonant inelastic soft X-ray scattering (RIXS). The oxygen K-edge XES spectra could be described with three components, attributed to initial state HB configurations in pure water, water molecules that have undergone an ultrafast dissociation initiated by the X-ray excitation, and water molecules in contact with salt ions. The behavior of the individual components, as well as the spectral shape of the latter component, has been analyzed in detail. In view of the role of ions in such effects as protein denaturation (i.e., the Hofmeister series), we discuss the ion-specific nature of the hydration shells and find that the results point to a predominant role of anions as compared to cations. Furthermore, we observe a concentration-dependent suppression of ultrafast dissociation in all salt solutions, associated with a significant distortion of intact HB configurations of water molecules facilitating such a dissociation. PMID:27442708

  12. Molecular orientation in soft matter thin films studied by resonant soft X-ray reflectivity

    SciTech Connect

    Mezger, Markus; Jerome, Blandine; Kortright, Jeffrey B.; Valvidares, Manuel; Gullikson, Eric; Giglia, Angelo; Mahne, Nicola; Nannarone, Stefano

    2011-01-12

    We present a technique to study depth profiles of molecular orientation in soft matter thin films with nanometer resolution. The method is based on dichroism in resonant soft X-ray reflectivity using linear s- and p-polarization. It combines the chemical sensitivity of Near-Edge X-ray Absorption Fine Structure spectroscopy to specific molecular bonds and their orientation relative to the polarization of the incident beam with the precise depth profiling capability of X-ray reflectivity. We demonstrate these capabilities on side chain liquid crystalline polymer thin films with soft X-ray reflectivity data at the carbon K edge. Optical constants of the anisotropic refractive index ellipsoid were obtained from a quantitative analysis using the Berreman formalism. For films up to 50 nm thickness we find that the degree of orientation of the long axis exhibits no depth variation and isindependent of the film thickness.

  13. Soft X-Ray Pulsations in Solar Flares

    NASA Astrophysics Data System (ADS)

    Simões, P. J. A.; Hudson, H. S.; Fletcher, L.

    2015-12-01

    The soft X-ray emissions ( hν>1.5 keV) of solar flares mainly come from the bright coronal loops at the highest temperatures normally achieved in the flare process. Their ubiquity has led to their use as a standard measure of flare occurrence and energy, although the overwhelming bulk of the total flare energy goes elsewhere. Recently Dolla et al. ( Astrophys. J. Lett. 749, L16, 2012) noted quasi-periodic pulsations (QPP) in the soft X-ray signature of the X-class flare SOL2011-02-15, as observed by the standard photometric data from the GOES ( Geostationary Operational Environmental Satellite) spacecraft. In this article we analyse the suitability of the GOES data for this type of analysis and find them to be generally valuable after September, 2010 (GOES-15). We then extend the result of Dolla et al. to a complete list of X-class flares from Cycle 24 and show that most of them (80 %) display QPPs in the impulsive phase. The pulsations show up cleanly in both channels of the GOES data, making use of time-series of irradiance differences (the digital time derivative on the 2-s sampling). We deploy different techniques to characterise the periodicity of GOES pulsations, considering the red-noise properties of the flare signals, finding a range of characteristic time scales of the QPPs for each event, but usually with no strong signature of a single period dominating in the power spectrum. The QPP may also appear on somewhat longer time scales during the later gradual phase, possibly with a greater tendency towards coherence, but the sampling noise in GOES difference data for high irradiance values (X-class flares) makes these more uncertain. We show that there is minimal phase difference between the differenced GOES energy channels, or between them and the hard X-ray variations on short time scales. During the impulsive phase, the footpoints of the newly forming flare loops may also contribute to the observed soft X-ray variations.

  14. Imaging bacterial spores by soft-x-ray microscopy

    SciTech Connect

    Stead, A.D.; Ford, T.W.; Judge, J.

    1997-04-01

    Bacterial spores are able to survive dehydration, but neither the physiological nor structural basis of this have been fully elucidated. Furthermore, once hydrated, spores often require activation before they will germinate. Several treatments can be used to activate spores, but in the case of Bacillus subtlis the most effective is heat treatment. The physiological mechanism associated with activation is also not understood, but some workers suggest that the loss of calcium from the spores may be critical. However, just prior to germination, the spores change from being phase bright to phase dark when viewed by light microscopy. Imaging spores by soft x-ray microscopy is possible without fixation. Thus, in contrast to electron microscopy, it is possible to compare the structure of dehydrated and hydrated spores in a manner not possible previously. A further advantage is that it is possible to monitor individual spores by phase contrast light microscopy immediately prior to imaging with soft x-rays; whereas, with both electron microscopy and biochemical studies, it is a population of spores being studied without knowledge of the phase characteristics of individual spores. This study has therefore tried to compare dehydrated and hydrated spores and to determine if there is a mass loss from individual spores as they pass the transition from being phase bright to phase dark.

  15. Phase-resolved X-ray spectroscopy and spectral energy distribution of the X-ray soft polar RS Caeli

    NASA Astrophysics Data System (ADS)

    Traulsen, I.; Reinsch, K.; Schwope, A. D.; Schwarz, R.; Walter, F. M.; Burwitz, V.

    2014-02-01

    Context. RS Cae is the third target in our series of XMM-Newton observations of soft X-ray-dominated polars. Aims: Our observational campaign aims to better understand and describe the multiwavelength data, the physical properties of the system components, and the short- and long-term behavior of the component fluxes in RS Cae. Methods: We employ stellar atmosphere, stratified accretion-column, and widely used X-ray spectral models. We fit the XMM-Newton spectra, model the multiband light curves, and opt for a mostly consistent description of the spectral energy distribution. Results: Our XMM-Newton data of RS Cae are clearly dominated by soft X-ray emission. The X-ray light curves are shaped by emission from the main accretion region, which is visible over the whole orbital cycle, interrupted only by a stream eclipse. The optical light curves are formed by cyclotron and stream emission. The XMM-Newton X-ray spectra comprise a black-body-like and a plasma component at mean temperatures of 36 eV and 7 keV. The spectral fits give evidence of a partially absorbing and a reflection component. Multitemperature models, covering a broader temperature range in the X-ray emitting accretion regions, reproduce the spectra appropriately well. Including archival data, we describe the spectral energy distribution with a combination of models based on a consistent set of parameters and derive a lower limit estimate of the distance d ≳ 750 pc. Conclusions: The high bolometric soft-to-hard flux ratios and short-term variability of the (X-ray) light curves are characteristic of inhomogeneous accretion. RS Cae clearly belongs in the group of polars that show a very strong soft X-ray flux compared to their hard X-ray flux. The different black-body fluxes and similar hard X-ray and optical fluxes during the XMM-Newton and ROSAT observations show that soft and hard X-ray emission are not directly correlated. Based on observations obtained with XMM-Newton, an ESA science mission with

  16. Structure and dynamics of cadmium telluride studied by x-ray and inelastic neutron scattering

    SciTech Connect

    Niedziela, Jennifer L; Stone, Matthew B

    2014-01-01

    We present a combined study of density functional theory, x-ray diffraction, and inelastic neutron scattering examining the temperature dependent structure and lattice dynamics of commercially available cadmium telluride. A subtle change in the structure is evinced near 80~K, which manifests also in the measured phonon density of states. There is no change to the long-range ordered structure. The implications of the change in relation to structural defects are discussed.

  17. Structure and dynamics of cadmium telluride studied by x-ray and inelastic neutron scattering

    SciTech Connect

    Niedziela, J. L.; Stone, M. B.

    2014-09-08

    We present a combined study of density functional theory, x-ray diffraction, and inelastic neutron scattering examining the temperature dependent structure and lattice dynamics of commercially available cadmium telluride. A subtle change in the structure is evinced near 80 K, which manifests also in the measured phonon density of states. There is no change to the long-range ordered structure. The implications of the change in relation to structural defects are discussed.

  18. Soft X-Ray Microscopy: Imaging Magnetism at Small Sizes

    NASA Astrophysics Data System (ADS)

    Fischer, Peter

    2010-03-01

    The manipulation of spins on the nanoscale is of both fundamental and technological interest. In spin based electronics the observation that spin currents can exert a torque onto local spin configurations which can e.g. push a domain wall has stimulated significant research activities in order to provide a fundamental understanding of the physical processes involved. Magnetic soft X-ray microscopy is a unique analytical technique combining X-ray magnetic circular dichroism (X-MCD) as element specific magnetic contrast mechanism with high spatial and temporal resolution. Fresnel zone plates used as X-ray optical elements provide a spatial resolution down to currently <12nm [1] thus approaching fundamental magnetic length scales such as the grain size [2] and magnetic exchange lengths. Images can be recorded in external magnetic fields giving access to study magnetization reversal phenomena on the nanoscale and its stochastic character [3] with elemental sensitivity [4]. Utilizing the inherent time structure of current synchrotron sources fast magnetization dynamics with 70ps time resolution, limited by the lengths of the electron bunches, can be performed with a stroboscopic pump-probe scheme. In this talk I will review recent achievements with magnetic soft X-ray microscopy with focus on current induced wall [5] and vortex dynamics in ferromagnetic elements [6]. Future magnetic microscopies are faced with the challenge to provide both spatial resolution in the nanometer regime, a time resolution on a ps to fs scale and elemental specificity to be able to study novel multicomponent and multifunctional magnetic nanostructures and their ultrafast spin dynamics.[4pt] References[0pt] [1] W. Chao, et al., Optics Express 17(20) 17669 (2009) [0pt] [2] M.-Y. Im, et al, Advanced Materials 20 1750 (2008) [0pt] [3] M.-Y. Im, et al., Phys Rev Lett 102 147204 (2009) [0pt] [4] M.-Y. Im, et al., Appl Phys Lett 95 182504 (2009) [0pt] [5] L. Bocklage, et al., Phys Rev B 78 180405(R

  19. X-ray emission from cataclysmic variables with accretion disks. I - Hard X-rays. II - EUV/soft X-ray radiation

    NASA Technical Reports Server (NTRS)

    Patterson, J.; Raymond, J. C.

    1985-01-01

    Theoretical models explaining the hard-X-ray, soft-X-ray, and EUV emission of accretion-disk cataclysmic variables in terms of the disk boundary layer (DBL) are developed on the basis of a survey of the published observational data. The data are compared with model predictions in graphs for systems with high or low (greater than or less than 10-Pg/s) accretion rates. Good agreement is obtained both at low accretion rates, where an optically thin rarefied hot (Te = 10 to the 8th K) DBL radiates most of its energy as hard X-rays, and at high accretion rates, where an optically thick 100,000-K DBL radiates most of its energy in the EUV and as soft X-rays. Detailed analysis of the old nova V603 Aql suggests that previous models predicting more detections of soft-X-ray/EUV emissions from thick-DBL objects (Ferland et al., 1982) used inappropriate dwarf masses, interstellar column densities, or classical-nova space densities.

  20. SAS 3 survey of the soft X-ray background

    NASA Technical Reports Server (NTRS)

    Marshall, F. J.; Clark, G. W.

    1984-01-01

    The results of a survey of the soft X-ray sky in the C band (0.10-0.28keV) are reported. The observations were carried out using two independent flow proportional counters on board the SAS 3 X-ray satellite which had a total angular resolution of 2.9 deg FWHM, and a total exposure of 2.2 x 10 to the 4th per sq cm s sr. It is found that C band counting rates were generally inversely correlated with the column density of the neutral hydrogen on all angular scales down to the lowest angular resolution of the detectors. In the region 90-180 deg l and 0-10 deg b, the relation between C-band rates and the column densities of neutral hydrogen was fitted with a residual rms deviation of less than 13 percent by a two-component numerical model of the X-ray background. For the apparent attenuation column density a value of 2.7 x 10 to the 20th per sq cm was obtained. On the basis of a computer simulation of the SAS 3 data, it is shown that the observed clumping of interstellar matter was consistent with the magnitude of spatial fluctuations in the C-band map. When the background rates were subtracted from the survey map, the subsequent map showed foreground emission and absorption features with improved sensitivity and clarity. A series of computer-generated maps incorporating the SAS 3 data is given in an appendix.

  1. Refraction effects in soft x-ray multilayer blazed gratings.

    PubMed

    Voronov, D L; Salmassi, F; Meyer-Ilse, J; Gullikson, E M; Warwick, T; Padmore, H A

    2016-05-30

    A 2500 lines/mm Multilayer Blazed Grating (MBG) optimized for the soft x-ray wavelength range was fabricated and tested. The grating coated with a W/B4C multilayer demonstrated a record diffraction efficiency in the 2nd blazed diffraction order in the energy range from 500 to 1200 eV. Detailed investigation of the diffraction properties of the grating demonstrated that the diffraction efficiency of high groove density MBGs is not limited by the normal shadowing effects that limits grazing incidence x-ray grating performance. Refraction effects inherent in asymmetrical Bragg diffraction were experimentally confirmed for MBGs. The refraction affects the blazing properties of the MBGs and results in a shift of the resonance wavelength of the gratings and broadening or narrowing of the grating bandwidth depending on diffraction geometry. The true blaze angle of the MBGs is defined by both the real structure of the multilayer stack and by asymmetrical refraction effects. Refraction effects can be used as a powerful tool in providing highly efficient suppression of high order harmonics.

  2. Design and analysis of soft X-ray imaging microscopes

    NASA Technical Reports Server (NTRS)

    Shealy, David L.; Cheng, Wang; Wu, Jiang; Hoover, Richard B.

    1992-01-01

    The spherical Schwarzschild microscope for soft X-ray applications in microscopy and projection lithography consists of two concentric spherical mirrors configured such that the third-order spherical aberration and coma are zero. Since multilayers are used on the mirror substrates for X-ray applications, it is desirable to have only two reflecting surfaces in a microscope. To reduce microscope aberrations and increase the field of view, generalized mirror surface profiles are here considered. Based on incoherent and sine wave modulation transfer function calculations, the object plane resolution of a microscope has been analyzed as a function of the object height and numerical aperture (NA) of the primary for several spherical Schwarzschild, conic, and aspherical Head reflecting two-mirror microscope configurations. The Head microscope with a NA of 0.4 achieves diffraction limited performance for objects with a diameter of 40 microns. Thus, it seems possible to record images with a feature size less than 100 A with a 40x microscope when using 40 A radiation.

  3. Ultrahigh-resolution soft x-ray tomography

    NASA Astrophysics Data System (ADS)

    Haddad, Waleed S.; Trebes, James E.; Goodman, Dennis M.; Lee, Heung-Rae; McNulty, Ian; Anderson, Erik H.; Zalensky, Andrei O.

    1995-09-01

    Ultra high resolution three-dimensional images of a microscopic test object were made with soft x rays using a scanning transmission x-ray microscope. The test object consisted of two different patterns of gold bars on silicon nitride windows that were separated by approximately 5 micrometer. A series of nine 2-D images of the object were recorded at angles between -5 to +55 degrees with respect to the beam axis. The projections were then combined tomographically to form a 3-D image by means of an algebraic reconstruction technique (ART) algorithm. A transverse resolution of approximately 1000 angstrom was observed. Artifacts in the reconstruction limited the overall depth resolution to approximately 6000 angstrom, however some features were clearly reconstructed with a depth resolution of approximately 1000 angstrom. A specially modified ART algorithm and a constrained conjugate gradient (CCG) code were also developed as improvements over the standard ART algorithm. Both of these methods made significant improvements in the overall depth resolution, bringing it down to approximately 1200 angstrom overall. Preliminary projection data sets were also recorded with both dry and re-hydrated human sperm cells over a similar angular range.

  4. ComIXS on BACH: a compact soft x-ray spectrometer operating at Elettra

    SciTech Connect

    Cocco, Daniele; Matteucci, Maurizio; Zangrando, Marco; Bondino, Federica; Zacchigna, Michele; Plate, Mauro; Parmigiani, Fulvio; Nelles, Bruno; Prince, Kevin C.

    2004-05-12

    To accommodate increasing interest in soft x-ray inelastic scattering, a new spectrometer has been designed, constructed and commissioned at Elettra. This instrument uses as the dispersive element one of two interchangeable Variable Line Spacing (VLS) spherical gratings. The energy scan is performed by a 7 cm linear translation of a back illuminated CCD which also collects the zero order light, facilitating alignment and calibration. The two gratings have the same radius of curvature while the groove densities and the groove density variations differ by a factor four. Thus the energies focused by the gratings at a particular position differ by a factor of four. The total length of the instrument is 60 cm, the energy range covered is roughly 25-1000 eV and the expected resolving power ranges from 1000 to 5000. The spectrometer is now operating on the beamline Bach. It takes advantage of the small size of the photon spot in the experimental chamber and of the possibility to control the polarization of the incoming radiation. The small spot constitutes the virtual entrance slit, and the spectrometer collects the photons emitted in a solid angle of about 30x10 mrad2. The instrument, named ComIXS (Compact Inelastic X-ray Spectrometer), has been routinely operating since October 2002. Several experiments have already been carried out, and some results illustrating the characteristics of the instrument are described. The manufacture and testing of the blaze gratings are also discussed.

  5. ComIXS on BACH: a compact soft x-ray spectrometer operating at Elettra

    NASA Astrophysics Data System (ADS)

    Cocco, Daniele; Zangrando, Marco; Matteucci, Maurizio; Bondino, Federica; Platè, Mauro; Zacchigna, Michele; Parmigiani, Fulvio; Nelles, Bruno; Prince, Kevin C.

    2004-05-01

    To accommodate increasing interest in soft x-ray inelastic scattering, a new spectrometer has been designed, constructed and commissioned at Elettra. This instrument uses as the dispersive element one of two interchangeable Variable Line Spacing (VLS) spherical gratings. The energy scan is performed by a 7 cm linear translation of a back illuminated CCD which also collects the zero order light, facilitating alignment and calibration. The two gratings have the same radius of curvature while the groove densities and the groove density variations differ by a factor four. Thus the energies focused by the gratings at a particular position differ by a factor of four. The total length of the instrument is 60 cm, the energy range covered is roughly 25-1000 eV and the expected resolving power ranges from 1000 to 5000. The spectrometer is now operating on the beamline Bach. It takes advantage of the small size of the photon spot in the experimental chamber and of the possibility to control the polarization of the incoming radiation. The small spot constitutes the virtual entrance slit, and the spectrometer collects the photons emitted in a solid angle of about 30×10 mrad2. The instrument, named ComIXS (Compact Inelastic X-ray Spectrometer), has been routinely operating since October 2002. Several experiments have already been carried out, and some results illustrating the characteristics of the instrument are described. The manufacture and testing of the blaze gratings are also discussed.

  6. Soft X-Ray Thomson Scattering in Warm Dense Hydrogen at FLASH

    SciTech Connect

    Faustlin, R R; Toleikis, S; Bornath, T; Doppner, T; Dusterer, S; Forster, E; Fortmann, C; Glenzer, S H; Gode, S; Gregori, G; Irsig, R; Laarmann, T; Lee, H J; Li, B; Meiwes-Broer, K; Mithen, J; Przystawik, A; Redlin, H; Redmer, R; Reinholz, H; Ropke, G; Tavella, F; Thiele, R; Tiggesbaumker, J; Uschmann, I; Zastrau, U; Tschentscher, T

    2009-07-15

    We present collective Thomson scattering with soft x-ray free electron laser radiation as a method to track the evolution of warm dense matter plasmas with {approx}200 fs time resolution. In a pump-probe scheme an 800 nm laser heats a 20 {micro}m hydrogen droplet to the plasma state. After a variable time delay in the order of ps the plasma is probed by an x-ray ultra violet (XUV) pulse which scatters from the target and is recorded spectrally. Alternatively, in a self-Thomson scattering experiment, a single XUV pulse heats the target while a portion of its photons are being scattered probing the target. From such inelastic x-ray scattering spectra free electron temperature and density can be inferred giving insight on relaxation time scales in plasmas as well as the equation of state. We prove the feasibility of this method in the XUV range utilizing the free electron laser facility in Hamburg, FLASH. We recorded Thomson scattering spectra for hydrogen plasma, both in the self-scattering and in the pump-probe mode using optical laser heating.

  7. 2-D soft x-ray arrays in the EAST

    NASA Astrophysics Data System (ADS)

    Chen, Kaiyun; Xu, Liqing; Hu, Liqun; Duan, Yanmin; Li, Xueqin; Yuan, Yi; Mao, Songtao; Sheng, Xiuli; Zhao, Jinlong

    2016-06-01

    A high spatial and temporal resolution soft x-ray (SXR) imaging diagnostic has been installed in EAST for the study of magnetohydrodynamics activities and core high-Z impurity transport. Up to 122 lines of sight view the poloidal plasma from three directions (two up-down symmetrical horizontal arrays and one vertical array), which renders the diagnostic able to provide detailed tomographic reconstructions under various conditions. Fourier-Bessel method based on flux coordinates was employed for 2-D SXR tomographic reconstruction. Examples of several events measured by SXR diagnostic in EAST are shown, namely the crash patterns of sawtooth, periodical burst of edge localized modes, and the transport of high-Z intrinsic impurities.

  8. G-133: A soft X ray solar telescope

    NASA Astrophysics Data System (ADS)

    Williams, Memorie K.; Campbell, Branton; Roming, Peter W. A.; Spute, Mark K.; Moody, J. Ward

    1992-10-01

    The GOLDHELOX Project, NASA payload number G-133, is a robotic soft x ray solar telescope designed and built by an organization of undergraduate students. The telescope is designed to observe the sun at a wavelength of 171 to 181 A. Since we require observations free from atmospheric interference, the telescope will be launched in a NASA Get-Away-Special (GAS) canister with a Motorized Door Assembly (MDA). In this paper we primarily discuss the most important elements of the telescope itself. We also elaborate on some of the technical difficulties associated with doing good science in space on a small budget (about $100,000) and mention ways in which controlling the instrument environment has reduced the complexity of the system and thus saved us money.

  9. VUV and soft x-ray spectroscopy of actinides

    SciTech Connect

    Olson, C. G.; Joyce, J. J.; Durakiewicz, T.; Guziewicz, E.

    2004-01-01

    Optical and photoelectron spectroscopies using VUV and Soft X-ray photons are powerful tools for studies of elemental and compound actinides. Large changes in the relative atomic cross sections of the 5f, 6d and sp electrons allow decomposition of the character of the valence bands using photoemission. Resonant enhancement of photoelectrons and Auger electrons at the 5d core threshold further aids the decomposition and gives a measure of elemental specificity. Angle-resolved photoemission can be used to map the momentum dependence of the electronic states. The large changes in relative cross section with photon energy yields further details when the mapping is done at equivalent points in multiple zones. Spectra for well understood rare earth materials will be presented to establish spectral characteristics for known atomic character initial states. These signatures will be applied to the case of USb to investigate f-d hybridization near the Fermi level.

  10. Soft x-ray microscope with zone plates at UVSOR

    NASA Astrophysics Data System (ADS)

    Watanabe, Norio; Shimanuki, Yoshio; Taniguchi, Mieko; Kihara, Hiroshi

    1993-01-01

    A soft x-ray microscope with zone plates was set up at UVSOR (Okazaki, Japan). A 0.41 micrometers line and space pattern was clearly distinguished using an objective zone plate with the outermost zone width of 0.41 micrometers . Modulation transfer functions were measured at wavelengths of 3.1 nm and 5.4 nm, and compared with theoretical calculations. Considering the resolution of a microchannel plate used as a detector, the agreement is fairly good. With this microscope, some biological specimens such as diatoms, spicule of trepang, crab and rabbit muscles, human blood cells, human chromosomes, and magnetotactic bacterium were observed at 3.1 nm and 5.4 nm. With an environmental chamber (wet cell) using polypropylene foils as windows, wet specimens were observed at a wavelength of 4.6 nm. Images of spicule of trepang, human blood cell, and cultured protoplast of plant cell stained by methyl mercury were observed with good contrast.

  11. Holography-guided ptychography with soft X-rays.

    PubMed

    Hessing, Piet; Pfau, Bastian; Guehrs, Erik; Schneider, Michael; Shemilt, Laura; Geilhufe, Jan; Eisebitt, Stefan

    2016-01-25

    Ptychography is a lensless imaging technique that aims to reconstruct an object from a set of coherent diffraction patterns originating from different and partially overlapping sample illumination areas. For a successful convergence of the iterative algorithms used, the sample scan positions have to be known with very high accuracy. Here, we present a method that allows to directly encode this information in the diffraction patterns without the need of accurate position encoders. Our approach relies on combining ptychography with another coherent imaging method, namely Fourier-transform holography. We have imaged two different objects using coherent soft-X-ray illumination and investigate the influence of experimental and numerical position refinement on the reconstruction result. We demonstrate that holographically encoded positions significantly reduce the experimental and numerical requirements. Our ptychographic reconstructions cover a large field of view with diffraction-limited resolution and high sensitivity in the reconstructed phase shift and absorption of the objects.

  12. Optical pseudomotors for soft x-ray beamlines.

    PubMed

    Pedreira, P; Sics, I; Sorrentino, A; Pereiro, E; Aballe, L; Foerster, M; Pérez-Dieste, V; Escudero, C; Nicolas, J

    2016-05-01

    Optical elements of soft x-ray beamlines usually have motorized translations and rotations that allow for the fine alignment of the beamline. This is to steer the photon beam at some positions and to correct the focus on slits or on sample. Generally, each degree of freedom of a mirror induces a change of several parameters of the beam. Inversely, several motions are required to actuate on a single optical parameter, keeping the others unchanged. We define optical pseudomotors as combinations of physical motions of the optical elements of a beamline, which allow modifying one optical parameter without affecting the others. We describe a method to obtain analytic relationships between physical motions of mirrors and the corresponding variations of the beam parameters. This method has been implemented and tested at two beamlines at ALBA, where it is used to control the focus of the photon beam and its position independently.

  13. Surface Slope Metrology on Deformable Soft X-ray Mirrors

    SciTech Connect

    Yuan, Sheng; Yashchuk, Valeriy V.; Goldberg, Kenneth A.; Celestre, Rich; Church, Matthew; McKinney, Wayne R.; Morrison, Greg; Warwick, Tony

    2010-01-31

    We report on the current state of surface slope metrology on deformable mirrors for soft x-rays at the Advanced Light Source (ALS). While we are developing techniques for in situ at-wavelength tuning, we are refining methods of ex situ visible-light optical metrology to achieve sub-100-nrad accuracy. This paper reports on laboratory studies, measurements and tuning of a deformable test-KB mirror prior to its use. The test mirror was bent to a much different optical configuration than its original design, achieving a 0.38 micro-radian residual slope error. Modeling shows that in some cases, by including the image conjugate distance as an additional free parameter in the alignment, along with the two force couples, fourth-order tangential shape errors (the so-called bird shape) can be reduced or eliminated.

  14. Surface Slope Metrology on Deformable Soft X-ray Mirrors

    SciTech Connect

    Yuan, S.; Yashchuk, V.V.; Goldberg, K.A.; Celestre, R.; Church, M.; McKinney, W.R.; Morrison, G.; Warwick, T.

    2009-09-18

    We report on the current state of surface slope metrology on deformable mirrors for soft x-rays at the Advanced Light Source (ALS). While we are developing techniques for in situ at-wavelength tuning, we are refining methods of ex situvisible-light optical metrology to achieve sub-100-nrad accuracy. This paper reports on laboratory studies, measurements and tuning of a deformable test-KB mirror prior to its use. The test mirror was bent to a much different optical configuration than its original design, achieving a 0.38 micro-radian residual slope error. Modeling shows that in some cases, by including the image conjugate distance as an additional free parameter in the alignment, along with the two force couples, fourth-order tangential shape errors (the so-called bird shape) can be reduced or eliminated.

  15. Resonant soft x-ray fluorescence studies of novel materials

    SciTech Connect

    Carlisle, J.A.; Terminello, L.J.; Hudson, E.A.; Shirley, E.L.; Jia, J.J.; Callcott, T.A.; Himpsel, F.J.; Ederer, D.L.; Perera, R.C.C.

    1995-02-08

    The authors are using resonant soft x-ray fluorescence at the Advanced Light Source to probe the electronic and geometric structure of novel materials. In the resonant process, a core electron is excited by a photon whose energy is near the core binding energy. In this energy regime the absorption and emission processes are coupled, and this coupling manifests itself in several ways. In boron nitride (BN), the resonant emission spectra reflect the influence of a ``spectator`` electron in an unoccupied excitonic state. The resonant emission can be used to distinguish between the various bulk phases of BN, and can also be used to probe the electronic structure of a monolayer of BN buried in a bulk environment, where it is inaccessible to electron spectroscopies. For highly-oriented pyrolytic graphite (HOPG) a coherent absorption-emission process takes place in the resonant regime, whereby crystalline momentum is conserved between the core excited electron and the valence hole which remains after emission.

  16. G-133: A soft x ray solar telescope

    NASA Technical Reports Server (NTRS)

    Williams, Memorie K.; Campbell, Branton; Roming, Peter W. A.; Spute, Mark K.; Moody, J. Ward

    1992-01-01

    The GOLDHELOX Project, NASA payload number G-133, is a robotic soft x ray solar telescope designed and built by an organization of undergraduate students. The telescope is designed to observe the sun at a wavelength of 171 to 181 A. Since we require observations free from atmospheric interference, the telescope will be launched in a NASA Get-Away-Special (GAS) canister with a Motorized Door Assembly (MDA). In this paper we primarily discuss the most important elements of the telescope itself. We also elaborate on some of the technical difficulties associated with doing good science in space on a small budget (about $100,000) and mention ways in which controlling the instrument environment has reduced the complexity of the system and thus saved us money.

  17. Soft-x-ray experiment revisited: a theoretical analysis

    SciTech Connect

    Brenner, D.J.; Zaider, M.

    1982-01-01

    The generalized formulation of the Theory of Dual Radiation Action (TDRA) deals quantitatively with the process of sublesion-lesion production in sensitive sites irradiated with uniform fields of ionizing radiation. In this paper modifications of this formalism necessary to treat the case of attenuated fields of radiations are described. As an application, recent survival data obtained with soft x-ray experiments are analyzed. It is shown that: (1) given a linear-quadratic dose-effect relation with constant ..beta..; (2) the function ..gamma..(x) can be obtained with the aid of Monte-Carlo generated proximity functions; and (3) this ..gamma..(x) may be successfully utilized to account for survival results obtained, with the same cell line, using ..cap alpha.. particles.

  18. Divergence measurements of soft x-ray laser beam

    SciTech Connect

    Suckewer, S.; Skinner, C.H.; Kim, D.; Valeo, E.; Voorhees, D.; Wouters, A.

    1986-07-01

    The divergence of the CVI 182 A lasing line generated in a rapidly recombining, magnetically confined plasma column was measured using soft x-ray spectrometers equipped with multichannel detectors. In addition to measurements of the relative divergence, an absolute divergence of approx.9 mrad at a magnetic field of 20 kG and approx.5 mrad at a magnetic field of 35 or 50 kG was obtained by a direct scan of the 182 A axial radiation. Based on this data a peak 182 A intensity of approx.100 kW is obtained. Calculations of the spatial distribution of gain in the plasma were in very good agreement with the experimental data.

  19. Tracing Chromospheric Evaporation in Radio and Soft X-rays

    NASA Technical Reports Server (NTRS)

    Aschwanden, Markus J.

    1997-01-01

    There are three publications in refereed journals and several presentations at scientific conferences resulted from this work, over a period of 6 months during 1995/1996. In the first paper, the discovery of the chromospheric evaporation process at radio wavelengths is described. In the second paper, the radio detection is used to quantify electron densities in the upflowing heated plasma in flare loops, which is then compared with independent other density measurements from soft X-rays, or the plasma frequency of electron beams originating in the acceleration region. In the third paper, the diagnostic results of the chromospheric evaporation process are embedded into a broader picture of a standard flare scenario. Abstracts of these three papers are attached.

  20. Imaging performance and tests of soft x-ray telescopes

    SciTech Connect

    Spiller, E.; McCorkle, R.; Wilczynski, J. . Thomas J. Watson Research Center); Golub, L.; Nystrom, G. ); Takacz, P.Z. ); Welch, C. )

    1990-08-01

    Photos obtained during 5 min. of observation time from the flight of our 10 in. normal incidence soft x-ray ({lambda} = 63.5{Angstrom}) telescope on September 11, 1989 are analyzed and the data are compared to the results expected from tests of the mirror surfaces. These tests cover a range of spatial periods from 25 cm to 1{Angstrom}. The photos demonstrate a reduction in the scattering of the multilayer mirror compared to a single surface for scattering angles above 1 arcmin, corresponding to surface irregularities with spatial periods below 10 {mu}m. Our results are used to predict the possible performance of future flights. Sounding rocket observations might be able to reach a resolution around 0.1 arcsec. Higher resolutions will require flights of longer durations and improvements in mirror testing for the largest spatial periods. 21 refs., 7 figs., 1 tab.

  1. Early Results from the YOHKOH Soft X-ray Telescope

    NASA Astrophysics Data System (ADS)

    Bruner, M. E.; Acton, L. W.; Lemen, J.; Hirayama, T.; Tsuneta, S.

    1992-05-01

    The The Soft X-ray Telescope on the Yohkoh satellite, launched by Japan on August 30, 1992, has proved to be a resounding success. It is providing a wealth of new information and many surprises, both on flares and on the behavior of the solar corona. Performance of the telescope has met or exceed our most optimistic expectations and it appears to be in perfect focus. Unlike the Skylab instruments, the Yohkoh telescope is not limited by a finite supply of film, permitting long sequences of images to be made with relatively high time resolution. Repetition rates for a given exposure / filter combination are typically a few seconds per frame to a few minutes per frame, depending on the selected field size. Movies assembled from long exposure sequences have shown the corona to be even more dynamic than expected. Major re-structuring, involving large fractions of the visible corona, can take place in an hour or two. Smaller regions are even more dynamic, changing almost continuously. Movies, created from long exposure sequences, have demonstrated the fundamental importance of large-scale coronal loops in connecting widely separated regions such that activity in one region quickly affects the physical conditions at remote sites. The images also show that the majority of the loops have nearly constant cross sections along their lengths, rather than one that increases with height. Several X-class flares have been observed; the surprising result is that they do not appear to be very dynamic in soft X-rays. The flare kernels seem to consist of compact loop structures that brighten and then fade without changing size or shape. Bright points are not as prominent as in the Skylab images; a result of using a CCD (a linear detector) rather than film which has a logarithmic response. The other instruments on Yohkoh are producing equally exciting results; it seems clear that the Yohkoh mission will produce many major advances in our knowledge of the flare mechanism.

  2. Implementation of soft x-ray microscopy with several tens nanometers spatial resolution at NSRL

    NASA Astrophysics Data System (ADS)

    Jiang, Shiping; Chen, Liang

    2009-09-01

    A transmission soft x-ray microscope (TXM), which is similar to the full-field x-ray microscopes installed on other synchrotron radiation sources in the world, was developed at National Synchrotron Radiation Laboratory (NSRL) in Hefei. An x-ray image taken with the microscope was acquired and its spatial resolution was estimated to be better than 70nm.

  3. Surface layering and melting in an ionic liquid studied by resonant soft X-ray reflectivity

    PubMed Central

    Mezger, Markus; Ocko, Benjamin M.; Reichert, Harald; Deutsch, Moshe

    2013-01-01

    The molecular-scale structure of the ionic liquid [C18mim]+[FAP]− near its free surface was studied by complementary methods. X-ray absorption spectroscopy and resonant soft X-ray reflectivity revealed a depth-decaying near-surface layering. Element-specific interfacial profiles were extracted with submolecular resolution from energy-dependent soft X-ray reflectivity data. Temperature-dependent hard X-ray reflectivity, small- and wide-angle X-ray scattering, and infrared spectroscopy uncovered an intriguing melting mechanism for the layered region, where alkyl chain melting drove a negative thermal expansion of the surface layer spacing. PMID:23431181

  4. EUV and Soft X-Ray Emissions From Comets

    NASA Astrophysics Data System (ADS)

    Krasnopolsky, V. A.

    2001-05-01

    We analyzed 8 observations of comets with the Extreme Ultraviolet Explorer (EUVE). A soft X-ray camera in the range of 97-165 eV FWHM with a peak effective area of 28 cm2 and three spectrometers at 80-180, 170-360, and 300-720 Å with peak effective areas of 2.1, 0.5, and 0.8 cm2, respectively, were used for those observations. The detection limit of the X-ray camera corresponds to the X-ray luminosity of 1.9x 1014 Δ 2 erg s-1 for photon energy ɛ > 100 eV. (Δ is the geocentric distance in AU.) Five comets were detected with the X-ray camera: Hyakutake, Borrelly, d'Arrest, pre- and postperihelion Hale-Bopp. Their images reveal a crescent-like structure with peak brightness offsets from the nuclei between the sunward and comet orbital velocity directions. X-ray luminosities and their spatial distributions were determined from the observations. The measured luminosities are in excellent correlation with gas production rates in comets, resulting in the efficiency of (6.4 +/- 0.9)x 10-5 AU3/2 in the range of 97-165 eV. Correlation with dust production rates is poor, and this favor a gas-related excitation process. The peak brightnesses scaled to r2 are constant and equal to 26+/- 9 millirayleighs. This means that comae are optically or collisionally thick near the brightness centers. Of a few suggested excitation mechanisms, only charge exchange between solar wind heavy ions and cometary neutrals agrees with both these facts. The EUVE spectra of comets Hale-Bopp and Hyakutake have been analyzed. Due to the close flyby of Hyakutake at 0.1 AU, its spectra are of exceptionally high quality and exceed the currently published spectra of comets by a factor of 3 in resolving power and by two orders of magnitude in photon statistics. The spectra reveal for the first time the emission lines of multiple charged ions which are brought to the comet by the solar wind and excited in charge exchange with cometary neutral species. The most prominent lines are O4+ 215 Å, C4+ 249

  5. TiO2 Nanoparticles as a Soft X-ray Molecular Probe

    SciTech Connect

    Larabell, Carolyn; Ashcroft, Jared M.; Gu, Weiwei; Zhang, Tierui; Hughes, Steven M.; Hartman, Keith B.; Hofmann, Cristina; Kanaras, Antonios G.; Kilcoyne, David A.; Le Gros, Mark; Yin, Yadong; Alivisatos, A. Paul; Larabell, Carolyn A.

    2007-06-30

    With the emergence of soft x-ray techniques for imaging cells, there is a pressing need to develop protein localization probes that can be unambiguously identified within the region of x-ray spectrum used for imaging. TiO2 nanocrystal colloids, which have a strong absorption cross-section within the "water-window" region of x-rays, areideally suited as soft x-ray microscopy probes. To demonstrate their efficacy, TiO2-streptavidin nanoconjugates were prepared and subsequently labeled microtubules polymerized from biotinylated tubulin. The microtubules were imaged using scanning transmission x-ray microscopy (STXM), and the TiO2 nanoparticle tags were specifically identified using x-ray absorption near edge spectroscopy (XANES). These experiments demonstrate that TiO2 nanoparticles are potential probes for protein localization analyses using soft x-ray microscopy.

  6. ON THE X-RAY OUTBURSTS OF TRANSIENT ANOMALOUS X-RAY PULSARS AND SOFT GAMMA-RAY REPEATERS

    SciTech Connect

    Cal Latin-Small-Letter-Dotless-I skan, Sirin; Ertan, Uenal

    2012-10-20

    We show that the X-ray outburst light curves of four transient anomalous X-ray pulsars (AXPs) and soft gamma-ray repeaters (SGRs), namely, XTE J1810-197, SGR 0501+4516, SGR 1627-41, and CXOU J164710.2-455216, can be produced by the fallback disk model that was also applied to the outburst light curves of persistent AXPs and SGRs in our earlier work. The model solves the diffusion equation for the relaxation of a disk that has been pushed back by a soft gamma-ray burst. The sets of main disk parameters used for these transient sources are very similar to each other and to those employed in our earlier models of persistent AXPs and SGRs. There is a characteristic difference between the X-ray outburst light curves of transient and persistent sources. This can be explained by the differences in the disk surface density profiles of the transient and persistent sources in quiescence indicated by their quiescent X-ray luminosities. Our results imply that a viscous disk instability operating at a critical temperature in the range of {approx}1300-2800 K is a common property of all fallback disks around AXPs and SGRs. The effect of the instability is more pronounced and starts earlier for the sources with lower quiescent luminosities, which leads to the observable differences in the X-ray enhancement light curves of transient and persistent sources. A single active disk model with the same basic disk parameters can account for the enhancement phases of both transient and persistent AXPs and SGRs. We also present a detailed parameter study to show the effects of disk parameters on the evolution of the X-ray luminosity of AXPs and SGRs in the X-ray enhancement phases.

  7. Inelastic x-ray scattering studies on dynamic structure factor of polymeric liquid Se under pressure

    SciTech Connect

    Inui, Masanori; Kajihara, Yukio; Kimura, Koji; Matsuda, Kazuhiro; Ohara, Koji; Tsutsui, Satoshi; Ishikawa, Daisuke

    2015-08-17

    Inelastic X-ray scattering measurements at 25 MPa using synchrotron radiation were carried out for semiconducting liquid Se at high temperatures up to 1673 K. The excitation energy of the acoustic mode disperses approximately 10-50 % faster than the ultrasonic sound velocity in the observed temperature range while the ultrasonic sound rapidly slows down with increasing temperature. We carried out X-ray scattering measurements and found that the average coordination number at 1673 K is 1.3, indicating that the high temperature liquid consists of short chain molecules. These results suggest that weakening of the interatomic interaction is correlated with breaking of polymeric chain molecules.

  8. Acoustic phonons in chrysotile asbestos probed by high-resolution inelastic x-ray scattering

    SciTech Connect

    Mamontov, Eugene; Vakhrushev, S. B.; Kumzerov, Yu. A,; Alatas, A.

    2009-01-01

    Acoustic phonons in an individual, oriented fiber of chrysotile asbestos (chemical formula Mg{sub 3}Si{sub 2}O{sub 5}(OH){sub 4}) were observed at room temperature in the inelastic x-ray measurement with a very high (meV) resolution. The x-ray scattering vector was aligned along [1 0 0] direction of the reciprocal lattice, nearly parallel to the long axis of the fiber. The latter coincides with [1 0 0] direction of the direct lattice and the axes of the nano-channels. The data were analyzed using a damped harmonic oscillator model. Analysis of the phonon dispersion in the first Brillouin zone yielded the longitudinal sound velocity of (9200 {+-} 600) m/s.

  9. Chemically selective soft x-ray patterning of polymers

    SciTech Connect

    Wang, J.; Stover, H.D.; Hitchcock, A.P.; Tyliszczak, T.

    2007-06-19

    The chemically selective modification of polymer mixtures by monochromated soft X-rays has been explored using the high-brightness fine-focused 50 nm beam of a scanning transmission X-ray microscope. Four different polymer systems were examined: a polymethylmethacrylate (PMMA) polyacrylonitrile (PAN) bilayer film; a PMMA-blend-PAN microphase-separated film; a poly(MMA-co-AN) copolymer film; and a poly(ethyl cyanoacrylate) homopolymer film. A high level of chemically selective modification was achieved for the PMMA/PAN bilayer; in particular, irradiation at 288.45 eV selectively removed the carbonyl group from PMMA while irradiation at 286.80 eV selectively reduced the nitrile group of PAN, even when these irradiations were carried out at the same (x,y) position of the sample. In the last two homogeneous polymer systems, similar amounts of damage to the nitrile and carbonyl groups occurred during irradiation at either 286.80 or 288.45 eV. This is attributed to damage transfer between the C=N and C=O groups mediated by primary electrons, secondary electrons or radical/ionic processes, aided by their close spatial proximity. Although the overall thickness of the bilayer sample at 70 nm is smaller than the lateral line spreading of 100 nm, the interface between the layers appears to effectively block the transport of energy, and hence damage, between the two layers. The origins of the line spreading in homogeneous phases and possible origins of the damage blocking effect of the interface are discussed. To demonstrate chemically selective patterning, high-resolution multi-wavelength patterns were created in the PMMA/PAN bilayer system.

  10. Toward the development of a soft x-ray reflection imaging microscope in the Schwarzschild configuration using a soft x-ray laser at 18. 2 nm

    SciTech Connect

    Dicicco, D.; Rosser, R. ); Kim, D.; Suckewer, S. . Plasma Physics Lab.)

    1991-12-01

    We present the recent results obtained from a soft X-ray reflection imaging microscope in the Schwarzschild configuration. The microscope demonstrated a spatial resolution of 0.7 {mu}m with a magnification of 16 at 18.2 nm. The soft X-ray laser at 18.2 nm was used as an X-ray source. Mo/Si multilayers were coated on the Schwarzschild optics and the normal incidence reflectivity at 18.2 nm per surface was measured to be {approximately} 20 %. 18 refs., 6 figs.

  11. Resonant inelastic x-ray scattering studies of the organic semiconductor copper phthalocyanine

    SciTech Connect

    Kodituwakku, C. N.; Burns, C. A.; Said, A. H.; Sinn, H.; Wang, X.; Gog, T.; Casa, D. M.; Tuel, M.; Western Michigan Univ.; DESY, Hasylab

    2008-01-01

    We report resonant inelastic x-ray scattering (RIXS) measurements on polycrystalline and single crystal samples of the organic semiconductor {beta}-copper phthalocyanine (CuPc) as well as time dependent density functional theory calculations of the electronic properties of the CuPc molecule. Resonant and nonresonant excitations were measured along the three crystal axes with 120 meV resolution. We observe molecular excitations as well as charge-transfer excitons along certain crystal directions and compare our data with the calculations. Our results demonstrate that RIXS is a powerful tool for studying excitons and other electronic excitations in organic semiconductors.

  12. Hydration structures near finite-sized nanoscopic objects reconstructed using inelastic x-ray scattering measurements.

    PubMed

    Coridan, Robert H; Schmidt, Nathan W; Lai, Ghee Hwee; Wong, Gerard C L

    2009-10-21

    Recent work has shown that it is possible to use high resolution dynamical structure factor S(q,ω) data measured with inelastic x-ray scattering to reconstruct the Green's function of water, which describes its dynamical density response to a point charge. Here, we generalize this approach and describe a strategy for reconstructing hydration behavior near simple charge distributions with excluded volumes, with the long term goal of engaging hydration processes in complex molecular systems. We use this Green's function based imaging of dynamics method to generate hydration structures and show that they are consistent with those of well-studied model systems.

  13. Elastic modulus of supercooled liquid and hot solid silicon measured by inelastic X-ray scattering

    SciTech Connect

    Alatas, A.; Said, A. H.; Sinn, H.; Alp, E. E.; Kodituwakku, C. N.; Reinhart, B.; Saboungi, M. -L.; Price, D. L.

    2005-12-01

    We measured the dynamical structure factors of supercooled-liquid and hot-solid silicon by inelastic X-ray scattering at the same temperature, 1620 K. Two significant changes in the averaged longitudinal sound velocities and in the longitudinal modulus are observed. We, first observe a different longitudinal modulus in the polycrystalline hot-solid silicon compared to the extrapolated value obtained from the single-crystal measurement. Furthermore, this reduction of the modulus may be a precursor of the semiconductor-to-metal transition. Second, the increase in the longitudinal modulus in the liquid upon supercooling is consistent with an increase in the degree of the directional bonding.

  14. A pressure cell for nonresonant inelastic x-ray scattering studies of gas phases

    SciTech Connect

    Minzer, M.; Bradley, J. A.; Musgrave, R.; Seidler, G. T.; Skilton, A.

    2008-08-15

    We report the design and performance of a gas-phase sample cell for measurements of momentum transfer (q) dependent nonresonant inelastic x-ray scattering (NRIXS). NRIXS measurements from He gas at 2 MPa (20 bars) readily demonstrate dipole-allowed and dipole-forbidden final states for two-electron excitations. Direct comparison of gas-phase NRIXS measurements with the corresponding nonresonant electron energy loss spectroscopy results (EELS) will be a valuable method for characterizing systematic errors in either technique for studies that require absolute normalization of the double differential cross section.

  15. Inelastic X-ray scattering experiments on B[subscript 4]C under high static pressures

    SciTech Connect

    Kumar, Ravhi S.; Dandekar, Dattatraya; Leithe-Jasper, Andres; Tanaka, Takaho; Xiao, Yuming; Chow, Paul; Nicol, Malcolm F.; Cornelius, Andrew L.

    2010-05-04

    Boron K-edge inelastic X-ray scattering experiments were performed on clean B{sub 4}C and shock impact recovered boron carbide up to 30 GPa and at ambient temperature to understand the pressure induced bonding changes. The spectral features corresponding to the boron site in the interlinking chain remained unchanged up to 30 GPa. The results of our experiments indicate that pressure induces less distortion to the boron sites and the local amorphization observed in the previous reports are due to the rearrangement of carbon atoms under extreme conditions without affecting the boron environment.

  16. Novel rhenium gasket design for nuclear resonant inelastic x-ray scattering at high pressure

    SciTech Connect

    Tanis, Elizabeth A.; Giefers, Hubertus; Nicol, Malcolm F.

    2008-02-15

    For the first time, a highly absorbing element, rhenium, has been proven to be a strong, reliable, and safe gasket material for achieving high pressure in nuclear resonant inelastic x-ray scattering (NRIXS) experiments. Rhenium foil was cut into rectangular slices and in order to reduce absorption, the elevated imprint due to preindenting of the gasket is removed using electrical discharge machining. By utilizing this novel gasket design, transmission losses were mitigated while performing NRIXS experiments conducted on the {sup 119}Sn and {sup 57}Fe Moessbauer isotopes.

  17. X-ray/UV variability and the origin of soft X-ray excess emission from II Zw 177

    NASA Astrophysics Data System (ADS)

    Pal, Main; Dewangan, Gulab C.; Misra, Ranjeev; Pawar, Pramod K.

    2016-03-01

    We study X-ray and UV emission from the narrow-line Seyfert 1 galaxy II Zw 177 using a 137 ks long and another 13 ks short XMM-Newton observation performed in 2012 and 2001, respectively. Both observations show soft X-ray excess emission contributing 76.9 ± 4.9 per cent in 2012 and 58.8 ± 10.2 per cent in 2001 in the 0.3-2 keV band. We find that both blurred reflection from an ionized disc and Comptonized disc emission describe the observed soft excess well. Time-resolved spectroscopy on scales of ˜20 ks reveals strong correlation between the soft excess and the power-law components. The fractional variability amplitude Fvar derived from EPIC-pn light curves at different energy bands is nearly constant (Fvar ˜ 20 per cent). This is in contrast to other active galactic nuclei where the lack of short term variation in soft X-ray excess emission has been attributed to intense light bending in the framework of the `lamppost' model. Thus, the variations in power-law emission are most likely intrinsic to corona rather than just due to the changes of height of compact corona. The variable UV emission (Fvar ˜ 1 per cent) is uncorrelated to any of the X-ray components on short time-scales suggesting that the UV emission is not dominated by the reprocessed emission. The gradual observed decline in the UV emission in 2012 may be related to the secular decline due to the changes in the accretion rate. In this case, the short term X-ray variability is not due to the changes in the seed photons but intrinsic to the hot corona.

  18. Multilayer on-chip stacked Fresnel zone plates: Hard x-ray fabrication and soft x-ray simulations

    SciTech Connect

    Li, Kenan; Wojcik, Michael J.; Ocola, Leonidas E.; Divan, Ralu; Jacobsen, Chris

    2015-11-01

    Fresnel zone plates are widely used as x-ray nanofocusing optics. To achieve high spatial resolution combined with good focusing efficiency, high aspect ratio nanolithography is required, and one way to achieve that is through multiple e-beam lithography writing steps to achieve on-chip stacking. A two-step writing process producing 50 nm finest zone width at a zone thickness of 1.14 µm for possible hard x-ray applications is shown here. The authors also consider in simulations the case of soft x-ray focusing where the zone thickness might exceed the depth of focus. In this case, the authors compare on-chip stacking with, and without, adjustment of zone positions and show that the offset zones lead to improved focusing efficiency. The simulations were carried out using a multislice propagation method employing Hankel transforms.

  19. Resonant Inelastic X-Ray Scattering Response of the Kitaev Honeycomb Model

    NASA Astrophysics Data System (ADS)

    Halász, Gábor B.; Perkins, Natalia B.; van den Brink, Jeroen

    2016-09-01

    We calculate the resonant inelastic X-ray scattering (RIXS) response of the Kitaev honeycomb model, an exactly solvable quantum-spin-liquid model with fractionalized Majorana and flux excitations. We find that the fundamental RIXS channels, the spin-conserving (SC) and the non-spin-conserving (NSC) ones, do not interfere and give completely different responses. SC-RIXS picks up exclusively the Majorana sector with a pronounced momentum dispersion, whereas NSC-RIXS also creates immobile fluxes, thereby rendering the response only weakly momentum dependent, as in the spin structure factor measured by inelastic neutron scattering. RIXS can therefore pick up the fractionalized excitations of the Kitaev spin liquid separately, making it a sensitive probe to detect spin-liquid character in potential material incarnations of the Kitaev honeycomb model.

  20. The GALAXIES beamline at the SOLEIL synchrotron: inelastic X-ray scattering and photoelectron spectroscopy in the hard X-ray range.

    PubMed

    Rueff, J P; Ablett, J M; Céolin, D; Prieur, D; Moreno, Th; Balédent, V; Lassalle-Kaiser, B; Rault, J E; Simon, M; Shukla, A

    2015-01-01

    The GALAXIES beamline at the SOLEIL synchrotron is dedicated to inelastic X-ray scattering (IXS) and photoelectron spectroscopy (HAXPES) in the 2.3-12 keV hard X-ray range. These two techniques offer powerful complementary methods of characterization of materials with bulk sensitivity, chemical and orbital selectivity, resonant enhancement and high resolving power. After a description of the beamline components and endstations, the beamline capabilities are demonstrated through a selection of recent works both in the solid and gas phases and using either IXS or HAXPES approaches. Prospects for studies on liquids are discussed.

  1. The GALAXIES beamline at the SOLEIL synchrotron: inelastic X-ray scattering and photoelectron spectroscopy in the hard X-ray range.

    PubMed

    Rueff, J P; Ablett, J M; Céolin, D; Prieur, D; Moreno, Th; Balédent, V; Lassalle-Kaiser, B; Rault, J E; Simon, M; Shukla, A

    2015-01-01

    The GALAXIES beamline at the SOLEIL synchrotron is dedicated to inelastic X-ray scattering (IXS) and photoelectron spectroscopy (HAXPES) in the 2.3-12 keV hard X-ray range. These two techniques offer powerful complementary methods of characterization of materials with bulk sensitivity, chemical and orbital selectivity, resonant enhancement and high resolving power. After a description of the beamline components and endstations, the beamline capabilities are demonstrated through a selection of recent works both in the solid and gas phases and using either IXS or HAXPES approaches. Prospects for studies on liquids are discussed. PMID:25537606

  2. Real space soft x-ray imaging at 10 nm spatial resolution

    SciTech Connect

    Chao, Weilun; Fischer, Peter; Tyliszczak, T.; Rekawa, Senajith; Anderson, Erik; Naulleau, Patrick

    2011-04-24

    Using Fresnel zone plates made with our robust nanofabrication processes, we have successfully achieved 10 nm spatial resolution with soft x-ray microscopy. The result, obtained with both a conventional full-field and scanning soft x-ray microscope, marks a significant step forward in extending the microscopy to truly nanoscale studies.

  3. Toward a soft x-ray Fourier-transform spectrometer

    SciTech Connect

    Howells, M.R.; Frank, K.; Hussain, Z.; Moler, E.J.; Reich, T. |; Moeller, D.; Shirley, D.A.

    1993-10-29

    The use of Fourier transform spectroscopy (FTS) in the soft x-ray region is advocated as a possible route to spectral resolution superior to that attainable with a grating system. A technical plan is described for applying FTS to the study of the absorption spectrum of helium in the region of double ionization around 60--80 eV. The proposed scheme includes a Mach-Zehnder interferometer deformed into a rhombus shape to provide grazing incidence reflections. The path difference between the interfering beams is to be tuned by translation of a table carrying four mirrors over a range {+-}1 cm which, in the absence of errors generating relative tilts of the wave fronts, would provide a resolving power equal to the number of waves of path difference: half a million at 65 eV, for example. The signal-to-noise ratio of the spectrum is analyzed and for operation on an Advanced Light Source bending magnet beam line should be about 330.

  4. Soft X Ray Telescope (SXT) focus error analysis

    NASA Technical Reports Server (NTRS)

    Ahmad, Anees

    1991-01-01

    The analysis performed on the soft x-ray telescope (SXT) to determine the correct thickness of the spacer to position the CCD camera at the best focus of the telescope and to determine the maximum uncertainty in this focus position due to a number of metrology and experimental errors, and thermal, and humidity effects is presented. This type of analysis has been performed by the SXT prime contractor, Lockheed Palo Alto Research Lab (LPARL). The SXT project office at MSFC formed an independent team of experts to review the LPARL work, and verify the analysis performed by them. Based on the recommendation of this team, the project office will make a decision if an end to end focus test is required for the SXT prior to launch. The metrology and experimental data, and the spreadsheets provided by LPARL are used at the basis of the analysis presented. The data entries in these spreadsheets have been verified as far as feasible, and the format of the spreadsheets has been improved to make these easier to understand. The results obtained from this analysis are very close to the results obtained by LPARL. However, due to the lack of organized documentation the analysis uncovered a few areas of possibly erroneous metrology data, which may affect the results obtained by this analytical approach.

  5. White dwarfs as the maximal soft x-ray scatterers

    SciTech Connect

    Akbari-Moghanjoughi, M.

    2013-09-15

    In this paper, we explore the effect of density on the structure formation and the electromagnetic wave (EMw) elastic scattering on quantum plasmas, using the generalized quantum hydrodynamic model valid for a wide range of the plasma density and relativistic degeneracy. It is found that the electron quantum diffraction effect caused by the Bohm potential has a fundamental effect on the ion correlations in a degenerate electron fluid and crystallization in quantum plasmas in the solid-density regime and beyond. The ion correlations and structure formation are shown to be fundamentally affected by the plasma density and the relativistic degeneracy parameters. Moreover, distinct behavior is shown to exist between the non-relativistic and relativistic matter density regimes, regarding the normalized EMw elastic scattering cross-sections. It is theoretically discovered that the maximal Thomson scattering coincides with the average density of a typical white dwarf corresponding to the soft X-ray wavelength regime. Current research can be very useful in plasma optical diagnostic methods for a wide range of electron number-density from warm dense matter and inertial confinement fusion to the astrophysical compact objects.

  6. Plasma Emission Profile Recreation using Soft X-Ray Tomography

    NASA Astrophysics Data System (ADS)

    Page, J. W.; Mauel, M. E.; Levesque, J. P.

    2015-11-01

    With sufficient views from multiple diode arrays, soft X-ray tomography is an invaluable plasma diagnostic because it is a non-perturbing method to reconstruct the emission within the interior of the plasma. In preparation for the installation of new SXR arrays in HBT-EP, we compute high-resolution tomographic reconstructions of discharges having kink-like structures that rotate nearly rigidly. By assuming a uniform angular mapping from the kink mode rotation, Δϕ ~ ωΔ t, a temporal sequence from a single 16-diode fan array represents as many as 16 x 100 independent views. We follow the procedure described by Wang and Granetz and use Bessel basis functions to take the inverse Radon transform. This transform is fit to our data using a least-squares method to estimate the internal SXR emissivity as a sum of polar functions. By varying different parameters of the transformation, we optimize the quality of our recreation of the emission profile and quantify how the reconstruction changes with the azimuthal order of the transform. Supported by U.S. DOE Grant DE-FG02-86ER53222.

  7. TOPICAL REVIEW: Human soft tissue analysis using x-ray or gamma-ray techniques

    NASA Astrophysics Data System (ADS)

    Theodorakou, C.; Farquharson, M. J.

    2008-06-01

    This topical review is intended to describe the x-ray techniques used for human soft tissue analysis. X-ray techniques have been applied to human soft tissue characterization and interesting results have been presented over the last few decades. The motivation behind such studies is to provide improved patient outcome by using the data obtained to better understand a disease process and improve diagnosis. An overview of theoretical background as well as a complete set of references is presented. For each study, a brief summary of the methodology and results is given. The x-ray techniques include x-ray diffraction, x-ray fluorescence, Compton scattering, Compton to coherent scattering ratio and attenuation measurements. The soft tissues that have been classified using x-rays or gamma rays include brain, breast, colon, fat, kidney, liver, lung, muscle, prostate, skin, thyroid and uterus.

  8. The stellar contribution to the galactic soft X-ray background

    NASA Technical Reports Server (NTRS)

    Rosner, R.; Avni, Y.; Bookbinder, J.; Giacconi, R.; Golub, L.; Harnden, F. R., Jr.; Maxson, C. W.; Topka, K.; Vaiana, G. S.

    1981-01-01

    Log N-log S relations for stars are constructed based on median X-ray luminosities for dF, dG, and dK stars previously reported for the Einstein Observatory/Center for Astrophysics stellar survey and on a detailed X-ray luminosity function derived here for dM stars, and the stellar contribution to the diffuse soft X-ray background is investigated. The principal results are that stars provide approximately 20% of the soft X-ray background in the 0.28-1.0 keV passband and therefore contribute significantly to the soft X-ray background in this energy range (with dM stars constituting the dominant contributing class), and that the stellar contribution to the diffuse X-ray background in the 0.15-0.28 keV passband is less than approximately 3%.

  9. Observation of soft X-rays from extended sources. [such as Perseus star cluster

    NASA Technical Reports Server (NTRS)

    Catura, R. C.; Acton, L. W.

    1974-01-01

    Efforts were directed toward surveying several supernova remnants for the emission of soft X-rays. Rather than attempt to detect such faint X-ray emission, the program was redirected to observe the spectrum and angular structure of the extended X-ray source in the Perseus cluster of galaxies and the super-nova remnant Puppis A. An attempt was made to detect X-ray line emission from Puppis A with a Bragg crystal spectrometer. Observations provide evidence for the presence of X-ray line emission in the spectrum of Puppis A near .65 keV.

  10. High-resolution, high-transmission soft x-ray spectrometer for the study of biological samples

    NASA Astrophysics Data System (ADS)

    Fuchs, O.; Weinhardt, L.; Blum, M.; Weigand, M.; Umbach, E.; Bär, M.; Heske, C.; Denlinger, J.; Chuang, Y.-D.; McKinney, W.; Hussain, Z.; Gullikson, E.; Jones, M.; Batson, P.; Nelles, B.; Follath, R.

    2009-06-01

    We present a variable line-space grating spectrometer for soft x-rays that covers the photon energy range between 130 and 650 eV. The optical design is based on the Hettrick-Underwood principle and tailored to synchrotron-based studies of radiation-sensitive biological samples. The spectrometer is able to record the entire spectral range in one shot, i.e., without any mechanical motion, at a resolving power of 1200 or better. Despite its slitless design, such a resolving power can be achieved for a source spot as large as (30×3000) μm2, which is important for keeping beam damage effects in radiation-sensitive samples low. The high spectrometer efficiency allows recording of comprehensive two-dimensional resonant inelastic soft x-ray scattering (RIXS) maps with good statistics within several minutes. This is exemplarily demonstrated for a RIXS map of highly oriented pyrolytic graphite, which was taken within 10 min.

  11. High-resolution, high-transmission soft x-ray spectrometer for the study of biological samples

    SciTech Connect

    Fuchs, Oliver; Weinhardt, L.; Blum, M.; Weigand, M.; Umbach, E.; Bar, M.; Heske, Clemens; Denlinger, Jonathan; Chuang, Y.-D.; McKinney, Wayne; Hussain, Zahid; Gullikson, Eric; Jones, M.; Batson, Phil; Nelles, B.; Follath, R.

    2009-03-09

    We present a variable line-space grating spectrometer for soft x-rays that covers the photon energy range between 130 and 650 eV. The optical design is based on the Hettrick-Underwood principle and tailored to synchrotron-based studies of radiation-sensitive biological samples. The spectrometer is able to record the entire spectral range in one shot, i.e., without any mechanical motion, at a resolving power of 1200 or better. Despite its slitless design, such a resolving power can be achieved for a source spot as large as 30x3000 mu m2, which is important for keeping beam damage effects in radiation-sensitive samples low. The high spectrometer efficiency allows recording of comprehensive two-dimensional resonant inelastic soft x-ray scattering (RIXS) maps with good statistics within several minutes. This is exemplarily demonstrated for a RIXS map of highly oriented pyrolytic graphite, which was taken within 10 min.

  12. Particle-hole cumulant approach for inelastic losses in x-ray spectra

    NASA Astrophysics Data System (ADS)

    Kas, J. J.; Rehr, J. J.; Curtis, J. B.

    2016-07-01

    Inelastic losses in core level x-ray spectra arise from many-body excitations, leading to broadening and damping as well as satellite peaks in x-ray photoemission (XPS) and x-ray absorption (XAS) spectra. Here we present a practical approach for calculating these losses based on a cumulant representation of the particle-hole Green's function, a quasiboson approximation, and a partition of the cumulant into extrinsic, intrinsic, and interference terms. The intrinsic losses are calculated using real-time time-dependent density functional theory while the extrinsic losses are obtained from the G W approximation of the photoelectron self-energy and the interference terms are approximated. These effects are included in the spectra using a convolution with an energy dependent particle-hole spectral function. The approach elucidates the nature of the spectral functions in XPS and XAS and explains the significant cancellation between extrinsic and intrinsic losses. Edge-singularity effects in metals are also accounted for. Illustrative results are presented for the XPS and XAS of both weakly and more correlated systems.

  13. Ground-based x-ray calibration of the Astro-H soft x-ray telescopes

    NASA Astrophysics Data System (ADS)

    Iizuka, Ryo; Hayashi, Takayuki; Maeda, Yoshitomo; Ishida, Manabu; Tomikawa, Kazuki; Sato, Toshiki; Kikuchi, Naomichi; Okajima, Takashi; Soong, Yang; Serlemitsos, Peter J.; Mori, Hideyuki; Izumiya, Takanori; Minami, Sari

    2014-07-01

    The X-ray astronomy satellite Astro-H, planned to be launched in 2015, will have several instruments for covering a wide energy band from a few hundreds eV to 600 keV. There are four X-ray telescopes, and two of them are soft X-ray telescopes (SXTs) covering up to about 15 keV. One is for an X-ray micro-calorimeter detector (SXS) and the other is for an X-ray CCD detector (SXI). The design of the SXTs is a conical approximation of the Wolter Type-I optics, which is also adopted for the telescopes on the previous mission Suzaku launched in 2005. It consists 203 thin-foil reflectors coated with gold monolayer (2000 Å) on the aluminum substrate (101.6 mm length) with the thickness of 0.15, 0.23 and 0.31 mm. These are nested confocally within the radius of 58 to 225 mm. The focal length of SXTs is 5.6 m. The weight is as light as ~ 43 kg per telescope. We present the current status of the calibration activity of two SXTs (SXT-1 and SXT-2). The developments of two SXTs were completed by NASA's Goddard Space Flight Center (GSFC). First X-ray measurements with a diverging beam at the GSFC 100m beamline found an angular resolution at 8.0 keV to be 1.1 and 1.0 arcmin (HPD) for SXT-1 and SXT-2, respectively. The full characterization of the X-ray performance has been now continuously calibrated with the 30m X-ray beamline facility at the Institute of Space and Astronautical Science (ISAS) of Japan Aerospace eXploration Agency (JAXA) in Japan. We adopted a raster scan method with a narrow X-ray pencil beam with the divergence of ~ 15". X-ray characterization of the two SXTs has been measured from May and December 2013, respectively. In the case of SXT-1, the on-axis effective area was approximately 580, 445, 370, 270, 185 and 90 cm2 at energies of 1.5, 4.5, 8.0, 9.4, 11.1 and 12.9 keV respectively. The effective area of SXT-2 is 2% larger than that of SXT-1 irrespective to X-ray energy. The on-axis angular resolution of SXT-1 was evaluated as 1.3 - 1.5 arcmin (HPD) in the 1

  14. Soft X-Ray Observations of a Complete Sample of X-Ray--selected BL Lacertae Objects

    NASA Astrophysics Data System (ADS)

    Perlman, Eric S.; Stocke, John T.; Wang, Q. Daniel; Morris, Simon L.

    1996-01-01

    We present the results of ROSAT PSPC observations of the X-ray selected BL Lacertae objects (XBLs) in the complete Einstein Extended Medium Sensitivity Survey (EM MS) sample. None of the objects is resolved in their respective PSPC images, but all are easily detected. All BL Lac objects in this sample are well-fitted by single power laws. Their X-ray spectra exhibit a variety of spectral slopes, with best-fit energy power-law spectral indices between α = 0.5-2.3. The PSPC spectra of this sample are slightly steeper than those typical of flat ratio-spectrum quasars. Because almost all of the individual PSPC spectral indices are equal to or slightly steeper than the overall optical to X-ray spectral indices for these same objects, we infer that BL Lac soft X-ray continua are dominated by steep-spectrum synchrotron radiation from a broad X-ray jet, rather than flat-spectrum inverse Compton radiation linked to the narrower radio/millimeter jet. The softness of the X-ray spectra of these XBLs revives the possibility proposed by Guilbert, Fabian, & McCray (1983) that BL Lac objects are lineless because the circumnuclear gas cannot be heated sufficiently to permit two stable gas phases, the cooler of which would comprise the broad emission-line clouds. Because unified schemes predict that hard self-Compton radiation is beamed only into a small solid angle in BL Lac objects, the steep-spectrum synchrotron tail controls the temperature of the circumnuclear gas at r ≤ 1018 cm and prevents broad-line cloud formation. We use these new ROSAT data to recalculate the X-ray luminosity function and cosmological evolution of the complete EMSS sample by determining accurate K-corrections for the sample and estimating the effects of variability and the possibility of incompleteness in the sample. Our analysis confirms that XBLs are evolving "negatively," opposite in sense to quasars, with Ve/Va = 0.331±0.060. The statistically significant difference between the values for

  15. Soft-x-ray hollow fiber optics with inner metal coating

    SciTech Connect

    Matsuura, Yuji; Oyama, Tadaaki; Miyagi, Mitsunobu

    2005-10-10

    A glass capillary with an inner metal coating is proposed to be used as soft-x-ray fiber optics in medical applications. Based on the results of theoretical calculations, nickel was chosen as the coating material for x rays radiated from a conventional x-ray tube. A nickel-coated capillary was fabricated by electroless deposition, and focusing and collimating effects were observed from measurements of the transmission efficiency of soft x rays. The transmission of a nickel-coated capillary with an inner diameter of 0.53 mm and a length of 300 mm was 10%, which is approximately double that of an uncoated glass capillary.

  16. Design and performance of AERHA, a high acceptance high resolution soft x-ray spectrometer

    NASA Astrophysics Data System (ADS)

    Chiuzbǎian, Sorin G.; Hague, Coryn F.; Avila, Antoine; Delaunay, Renaud; Jaouen, Nicolas; Sacchi, Maurizio; Polack, François; Thomasset, Muriel; Lagarde, Bruno; Nicolaou, Alessandro; Brignolo, Stefania; Baumier, Cédric; Lüning, Jan; Mariot, Jean-Michel

    2014-04-01

    A soft x-ray spectrometer based on the use of an elliptical focusing mirror and a plane varied line spacing grating is described. It achieves both high resolution and high overall efficiency while remaining relatively compact. The instrument is dedicated to resonant inelastic x-ray scattering studies. We set out how this optical arrangement was judged best able to guarantee performance for the 50 - 1000 eV range within achievable fabrication targets. The AERHA (adjustable energy resolution high acceptance) spectrometer operates with an effective angular acceptance between 100 and 250 μsr (energy dependent) and a resolving power well in excess of 5000 according to the Rayleigh criterion. The high angular acceptance is obtained by means of a collecting pre-mirror. Three scattering geometries are available to enable momentum dependent measurements with 135°, 90°, and 50° scattering angles. The instrument operates on the Synchrotron SOLEIL SEXTANTS beamline which serves as a high photon flux 2 × 200 μm2 focal spot source with full polarization control.

  17. Plane-grating flat-field soft x-ray spectrometer

    NASA Astrophysics Data System (ADS)

    Hague, C. F.; Underwood, J. H.; Avila, A.; Delaunay, R.; Ringuenet, H.; Marsi, M.; Sacchi, M.

    2005-02-01

    We describe a soft x-ray spectrometer covering the 120-800 eV range. It is intended for resonant inelastic x-ray scattering experiments performed at third generation synchrotron radiation (SR) facilities and has been developed with SOLEIL, the future French national SR source in mind. The Hettrick-Underwood principle is at the heart of the design using a combination of varied line-spacing plane grating and spherical-mirror to provide a flat-field image. It is slitless for optimum acceptance. This means the source size determines the resolving power. A spot size of ⩽5μm is planned at SOLEIL which, according to simulations, should ensure a resolving power ⩾1000 over the whole energy range. A 1024×1024 pixel charge-coupled device (CCD) with a 13μm×13μm pixel size is used. This is an improvement on the use of microchannel-plate detectors, both as concerns efficiency and spatial resolution. Additionally spectral line curvature is avoided by the use of a horizontal focusing mirror concentrating the beam in the nondispersing direction. It allows for readout using a binning mode to reduce the intrinsically large CCD readout noise. Preliminary results taken at beamlines at Elettra (Trieste) and at BESSY (Berlin) are presented.

  18. Design and performance of AERHA, a high acceptance high resolution soft x-ray spectrometer.

    PubMed

    Chiuzbăian, Sorin G; Hague, Coryn F; Avila, Antoine; Delaunay, Renaud; Jaouen, Nicolas; Sacchi, Maurizio; Polack, François; Thomasset, Muriel; Lagarde, Bruno; Nicolaou, Alessandro; Brignolo, Stefania; Baumier, Cédric; Lüning, Jan; Mariot, Jean-Michel

    2014-04-01

    A soft x-ray spectrometer based on the use of an elliptical focusing mirror and a plane varied line spacing grating is described. It achieves both high resolution and high overall efficiency while remaining relatively compact. The instrument is dedicated to resonant inelastic x-ray scattering studies. We set out how this optical arrangement was judged best able to guarantee performance for the 50 - 1000 eV range within achievable fabrication targets. The AERHA (adjustable energy resolution high acceptance) spectrometer operates with an effective angular acceptance between 100 and 250 μsr (energy dependent) and a resolving power well in excess of 5000 according to the Rayleigh criterion. The high angular acceptance is obtained by means of a collecting pre-mirror. Three scattering geometries are available to enable momentum dependent measurements with 135°, 90°, and 50° scattering angles. The instrument operates on the Synchrotron SOLEIL SEXTANTS beamline which serves as a high photon flux 2 × 200 μm(2) focal spot source with full polarization control.

  19. Design and performance of AERHA, a high acceptance high resolution soft x-ray spectrometer

    SciTech Connect

    Chiuzbăian, Sorin G. Hague, Coryn F.; Brignolo, Stefania; Baumier, Cédric; Lüning, Jan; Avila, Antoine; Delaunay, Renaud; Mariot, Jean-Michel; Jaouen, Nicolas; Polack, François; Thomasset, Muriel; Lagarde, Bruno; Nicolaou, Alessandro; Sacchi, Maurizio

    2014-04-15

    A soft x-ray spectrometer based on the use of an elliptical focusing mirror and a plane varied line spacing grating is described. It achieves both high resolution and high overall efficiency while remaining relatively compact. The instrument is dedicated to resonant inelastic x-ray scattering studies. We set out how this optical arrangement was judged best able to guarantee performance for the 50 − 1000 eV range within achievable fabrication targets. The AERHA (adjustable energy resolution high acceptance) spectrometer operates with an effective angular acceptance between 100 and 250 μsr (energy dependent) and a resolving power well in excess of 5000 according to the Rayleigh criterion. The high angular acceptance is obtained by means of a collecting pre-mirror. Three scattering geometries are available to enable momentum dependent measurements with 135°, 90°, and 50° scattering angles. The instrument operates on the Synchrotron SOLEIL SEXTANTS beamline which serves as a high photon flux 2 × 200 μm{sup 2} focal spot source with full polarization control.

  20. Soft X-ray spectral observations of quasars and high X-ray luminosity Seyfert galaxies

    NASA Technical Reports Server (NTRS)

    Petre, R.; Mushotzky, R. F.; Krolik, J. H.; Holt, S. S.

    1983-01-01

    Results of the analysis of 28 Einstein SSS observations of 15 high X-ray luminosity (L(x) 10 to the 435 power erg/s) quasars and Seyfert type 1 nuclei are presented. The 0.75-4.5 keV spectra are in general well fit by a simple model consisting of a power law plus absorption by cold gas. The averager spectral index alpha is 0.66 + or - .36, consistent with alpha for the spectrum of these objects above 2 keV. In all but one case, no evidence was found for intrinsic absorption, with an upper limit of 2 x 10 to the 21st power/sq cm. Neither was evidence found for partial covering of the active nucleus by dense, cold matter (N(H) 10 to the 22nd power/sq cm; the average upper limit on the partial covering fraction is 0.5. There is no obvious correlation between spectral index and 0175-4.5 keV X-ray luminosity (which ranges from 3 x 10 to the 43rd to 47th powers erg/s or with other source properties. The lack of intrinsic X-ray absorption allows us to place constraints on the density and temperature of the broad-line emission region, and narrow line emission region, and the intergalactic medium.

  1. Small scale H I structure and the soft X-ray background

    NASA Technical Reports Server (NTRS)

    Jahoda, K.; Mccammon, D.; Lockman, F. J.

    1986-01-01

    The observed anticorrelation between diffuse soft X-ray flux and H I column density has been explained as absorption of soft X-rays produced in a hot galactic halo, assuming that the neutral interstellar material is sufficiently clumped to reduce the soft X-ray absorption cross section by a factor of two to three. A 21 cm emission line study of H I column density variations at intermediate and high galactic latitudes to 10' spatial resolution has been done. The results confirm conclusions from preliminary work at coarser resolution, and in combination with other data appear to rule out the hypothesis that clumping of neutral interstellar matter on any angular scale significantly reduces X-ray absorption cross sections in the 0.13 - 0.28 keV energy range. It is concluded therefore that the observed anticorrelation is not primarily a consequence of absorption of soft X-rays produced in a hot galactic halo.

  2. Molecular Orbital Simulations of Metal 1s2p Resonant Inelastic X-ray Scattering.

    PubMed

    Guo, Meiyuan; Källman, Erik; Sørensen, Lasse Kragh; Delcey, Mickaël G; Pinjari, Rahul V; Lundberg, Marcus

    2016-07-28

    For first-row transition metals, high-resolution 3d electronic structure information can be obtained using resonant inelastic X-ray scattering (RIXS). In the hard X-ray region, a K pre-edge (1s→3d) excitation can be followed by monitoring the dipole-allowed Kα (2p→1s) or Kβ (3p→1s) emission, processes labeled 1s2p or 1s3p RIXS. Here the restricted active space (RAS) approach, which is a molecular orbital method, is used for the first time to study hard X-ray RIXS processes. This is achieved by including the two sets of core orbitals in different partitions of the active space. Transition intensities are calculated using both first- and second-order expansions of the wave vector, including, but not limited to, electric dipoles and quadrupoles. The accuracy of the approach is tested for 1s2p RIXS of iron hexacyanides [Fe(CN)6](n-) in ferrous and ferric oxidation states. RAS simulations accurately describe the multiplet structures and the role of 2p and 3d spin-orbit coupling on energies and selection rules. Compared to experiment, relative energies of the two [Fe(CN)6](3-) resonances deviate by 0.2 eV in both incident energy and energy transfer directions, and multiplet splittings in [Fe(CN)6](4-) are reproduced within 0.1 eV. These values are similar to what can be expected for valence excitations. The development opens the modeling of hard X-ray scattering processes for both solution catalysts and enzymatic systems. PMID:27398775

  3. The Soft X-Ray Spectrometer (SXS) for the ISAS/JAXA New Exploration X-Ray Telescope

    NASA Astrophysics Data System (ADS)

    Kelley, Richard L.; Kilbourne, C. A.; McCammon, D.; Mushotzky, R. F.; Okajima, T.; Petre, R.; Porter, F. S.; Serlemitsos, P. J.; Smith, R. K.; Soong, Y.; Szymkowiak, A. E.; Mitsuda, K.; Ohashi, T.; Ishisaki, Y.; Ezoe, Y.; Yamasaki, N. Y.; Shinozaki, K.; Fujimoto, R.; Kawaharada, M.

    2008-03-01

    The ISAS/JAXA New Exploration X-Ray Telescope (NEXT) is now under development for launch in 2013. The observatory is designed to provide extremely high spectral resolution with large collecting area below 10 keV using an x-ray calorimeter, and a very large band pass (up to 300 keV) with extraordinary sensitivity over the range 10-80 keV using focusing x-ray optics. In this talk we will discuss plans for the Soft X-Ray Spectrometer (SXS), which uses an x-ray calorimeter array to provide the high spectral resolution. The SXS is a joint effort between ISAS and NASA and recently proposed to NASA as a Mission of Opportunity for the US participation. The SXS incorporates a 6x6 calorimeter array that has strong heritage in the Suzaku program and better than 7 eV energy resolution, with 4-5 eV expected based on recent laboratory tests. The cryogenic system will be a hybrid design with both liquid helium and mechanical coolers to provide a robust, redundant system with long life (> 3 years). The x-ray optical system (6 m focal length) uses thin-foil conical optics to provide at least 220 square cm at 6 keV. The SXS will enable a wide variety of interesting science topics to be pursued, including testing theories of structure formation using velocity measurements of clusters of galaxies and inferring the energy output from the jets and winds of active galaxies. The SXS will accurately measure metal abundances in the oldest galaxies, providing unique information on the origin of the elements, and observe matter in extreme gravitational fields, enabling time-resolved spectra from material approaching the event horizon of a black hole. Along with providing the instrument, we have proposed a well supported guest investigator program that will enable full US participation.

  4. The dynamical signature of the ISM in soft X-rays. I. Diffuse soft X-rays from galaxies

    NASA Astrophysics Data System (ADS)

    Breitschwerdt, Dieter; Schmutzler, Thomas

    1999-07-01

    We present the first dynamically and thermally self-consistent calculations of fast adiabatically expanding gas flows from the Galactic disk into the halo. It is shown that in a hot plasma (T >= 10(6) K) with a high overpressure with respect to the ambient medium, the dynamical time scale is much shorter than the intrinsic time scales (e.g. for recombination, collisional excitation and ionization etc.). Therefore dynamical models that use collisional ionization equilibrium (CIE) cooling functions for the evolution of the plasma are in general not correct. In particular, the emission spectra obtained from non-equilibrium calculations are radically different. We describe a method to obtain self-consistent solutions using an iterative procedure. It is demonstrated that soft X-ray background emission between 0.3 and 1.5 keV can be well explained by a superposition of line emission and delayed recombination of an initially hot plasma streaming away from the Galactic disk (outflow and/or winds). In addition to these local winds we also present calculations on global winds from spiral galaxies, which originate from a hot and quiescent galactic corona. We also emphasize that it is dangerous to derive plasma temperatures merely from line ratios of ionized species, such as N v/O vi, unless the dynamical and thermal history of the plasma is known.

  5. SASE3: soft x-ray beamline at European XFEL

    NASA Astrophysics Data System (ADS)

    La Civita, Daniele; Gerasimova, Natalia; Sinn, Harald; Vannoni, Maurizio

    2014-09-01

    The European XFEL in Hamburg will be comprised of a linear accelerator and three Free-Electron-Laser beamlines (SASE1, SASE2 and SASE3) covering the energy range from 250 eV to 24 keV. It will provide up to 2700 pulses in trains of 600 microsecond duration at a repetition rate of 10 Hz. SASE3 beamline is the soft X-ray beamline (0.25 - 3 keV) and delivers photon pulses to SQS (Small Quantum System) and SCS (Spectroscopy & Coherent Scattering) experiments. The beamline is able to operate in both monochromatic and non-monochromatic mode. The latter provides the inherent FEL bandwidth at higher intensities. The beamline from photon source to experimental station is about 450 m long. The length of the beamline is related to the optics single-shotdamage issue. The almost diffraction-limited beam is propagated along the beamline with very long (up to 800 mm clear aperture), cooled (with eutectic bath) and super-polished (50 nrad RMS slope error and less than 3 nm PV residual height error) mirrors. The VLS-PG (variable line spacing - plane grating) monochromator covers the entire beamline energy range and its optical design is guided by the optimization of the energy resolving power, the minimization of the pulse broadening and the maximization of optics damage tolerance. Grating substrates are 530 mm long, eutectic cooled and present outstanding surface quality. The VLS parameters of the blazed profile are also a real challenge under manufacturing and measuring point of view. Adaptive optics in the horizontal (the second offset mirror) and vertical (monochromator premirror) plane are foreseen in the optical layout to increase the beamline tunability and to preserve the highly coherent beam properties. Beamline optical design, expected performance and also mechanical aspects of main beamline components are reported.

  6. Deconstructing the Spectrum of the Soft X-ray Background

    NASA Technical Reports Server (NTRS)

    Kuntz, K. D.; Snowden, S. L.

    2000-01-01

    The soft X-ray background in the 0.1-1.0 keV band is known to be produced by at least three sources; the Local Hot Bubble (LHB), the extragalactic power law (EPL), and a seemingly galactic component that lies outside the bulk of the absorption that is due to the ISM of the galactic disk. This last component, which we call the Trans-Absorption Emission (TAE), has been modeled by a number of groups who have derived disparate measures of its temperature. The differences have arisen from differing assumptions about the structure of the emitting gas and unrecognized methodological difficulties. In particular, spectral fitting methods do not uniquely separate the TAE from the foreground emission that is due the LHB. This "degeneracy" can be resolved using the angular variation of the absorption of the TAE. We show that the TAE cannot be characterized by a single thermal component; no single-component model can be consistent with both the spectral energy distribution of the TAE emission and the angular variation due to absorption by the galactic disk. We use the angular anticorrelation of the ROSAT All-Sky Survey with the galactic absorption to separate local from distant emission components, and to fit the spectral energy distribution of the resulting distant emission. We find that the emission is best described by a two-thermal-component model with logT(sub S) = 6.06(sup +0.14, sub -0.12) and log T(sub H) = 6.42(sup +0.14, sub -0.12). This two-thermal-component TAE fits the ROSAT spectral energy distribution significantly better than single-component models, and is consistent with both angular variation and spectral constraints.

  7. The Soft X-ray Spectrum of the High Mass X-Ray Binary V0332+53 in Quiescence

    NASA Astrophysics Data System (ADS)

    Elshamouty, Khaled G.; Heinke, Craig O.; Chouinard, Rhys

    2016-08-01

    The behaviour of neutron stars in high mass X-ray binaries (HMXBs) during periods of low mass transfer is of great interest. Indications of spectral softening in systems at low mass transfer rates suggest that some HMXBs are undergoing fundamental changes in their accretion regime, but the nature of the quiescent X-ray emission is not clear. We performed a 39 ks XMM-Newton observation of the transient HMXB V0332+53, finding it at a very low X-ray luminosity (Lx ˜ 4 × 1032 erg s-1). A power-law spectral fit requires an unusually soft spectral index (4.4^{+0.9}_{-0.6}), while a magnetized neutron star atmosphere model, with temperature LogTeff 6.7±0.2 K and inferred emitting radius of ˜0.2 - 0.3 km, gives a good fit. We suggest that the quiescent X-ray emission from V0332+53 is mainly from a hot spot on the surface of the neutron star. No conclusions on the presence of pulsations could be drawn due to the low count rate. Due to the high absorption column, thermal emission from the rest of the neutron star could be only weakly constrained, to LogTeff <6.14^{+0.05}_{-6.14} K, or <3 × 1033 erg s-1.

  8. Soft-x-ray damage to p-terphenyl coatings for detectors.

    PubMed

    Benitez, E L; Dark, M L; Husk, D E; Schnatterly, S E; Tarrio, C

    1994-04-01

    The organic phosphor p-terphenyl is used as a wavelength-converter coating in some soft-x-ray detectors. We have measured the absolute photoluminescent efficiency of p-terphenyl as a function of incident photon energy from 36 to 191 eV. We have also measured changes in the efficiency caused by soft-x-ray fluence (total photons absorbed per unit area) at several photon energies in this range. We find that efficiency drops rapidly as a function of fluence, with the rate of decrease increasing with higher soft x-ray energies.

  9. High-average-power water window soft X-rays from an Ar laser plasma

    NASA Astrophysics Data System (ADS)

    Amano, Sho

    2016-07-01

    A high average power of 140 mW and high conversion efficiency of 14% were demonstrated in “water window” soft X-rays generated using a laser plasma source developed in-house, when a solid Ar target was irradiated by a commercial Nd:YAG Q-switched laser with an energy of 1 J at a repetition rate of 1 Hz. This soft X-ray power compared favorably with that produced using a synchrotron radiation source, and the developed laser plasma source can be used in various applications, such as soft X-ray microscopy, in place of synchrotron facilities.

  10. Tunable thin film polarizer for the vacuum ultraviolet and soft x-ray spectral regions

    SciTech Connect

    Yang, Minghong; Cobet, Christoph; Esser, Norbert

    2007-03-01

    A low pass polarizer that suppresses higher-order diffraction light from vacuum ultraviolet and soft x-ray monochromators is presented in this paper. This vacuum ultraviolet and soft x-ray polarizer is based on a concept of sandwiched metal-dielectric-metal triple reflection configuration. By appropriate optimization of material and angle of incidence, the proposed Au-SiC-Au polarizer demonstrates the capability of matching to desired cutoff edge of photon energy. Furthermore, the optimized soft x-ray polarizer shows the possibility to tune cutoff photon energy in a broadband spectral region ranging from 80 down to down to 20 eV.

  11. A CATALOG OF SOLAR X-RAY PLASMA EJECTIONS OBSERVED BY THE SOFT X-RAY TELESCOPE ON BOARD YOHKOH

    SciTech Connect

    Tomczak, M.; Chmielewska, E. E-mail: chmielewska@astro.uni.wroc.pl

    2012-03-01

    A catalog of X-ray plasma ejections (XPEs) observed by the Soft X-ray Telescope on board the Yohkoh satellite has been recently developed in the Astronomical Institute of University of Wroclaw. The catalog contains records of 368 events observed in years 1991-2001 including movies and cross-references to associated events like flares and coronal mass ejections (CMEs). One hundred sixty-three XPEs out of 368 in the catalog were not reported until now. A new classification scheme of XPEs is proposed in which morphology, kinematics, and recurrence are considered. The relation between individual subclasses of XPEs and the associated events was investigated. The results confirm that XPEs are strongly inhomogeneous, responding to different processes that occur in the solar corona. A subclass of erupting loop-like XPEs is a promising candidate to be a high-temperature precursor of CMEs.

  12. Nuclear resonant inelastic X-ray scattering at high pressure and low temperature

    DOE PAGES

    Bi, Wenli; Zhao, Jiyong; Lin, Jung -Fu; Jia, Quanjie; Hu, Michael Y.; Jin, Changqing; Ferry, Richard; Yang, Wenge; Struzhkin, Viktor; Alp, E. Ercan

    2015-01-01

    In this study, a new synchrotron radiation experimental capability of coupling nuclear resonant inelastic X-ray scattering with the cryogenically cooled high-pressure diamond anvil cell technique is presented. The new technique permits measurements of phonon density of states at low temperature and high pressure simultaneously, and can be applied to studies of phonon contribution to pressure- and temperature-induced magnetic, superconducting and metal–insulator transitions in resonant isotope-bearing materials. In this report, a pnictide sample, EuFe2As2, is used as an example to demonstrate this new capability at beamline 3-ID of the Advanced Photon Source, Argonne National Laboratory. A detailed description of the technicalmore » development is given. The Fe-specific phonon density of states and magnetism from the Fe sublattice in Eu57Fe2As2 at high pressure and low temperature were derived by using this new capability.« less

  13. Implications of resonant inelastic x-ray scattering data for theoretical models of cuprates

    NASA Astrophysics Data System (ADS)

    Chen, Wei; Sushkov, Oleg P.

    2013-11-01

    There are two commonly discussed points of view in theoretical description of cuprate superconductors: (i) Cuprates can be described by the modified t-J model; (ii) overdoped cuprates are close to the regime of normal Fermi liquid (NFL). We argue that recent resonant inelastic x-ray scattering data challenge both points. While the modified t-J model describes well the strongly underdoped regime, it fails to describe high energy magnetic excitations when approaching optimal doping. This probably indicates failure of the Zhang-Rice singlet picture. In the overdoped regime the momentum-integrated spin structure factor S(ω) has the same intensity and energy distribution as that in an undoped parent compound. This implies that the entire spin spectral sum rule is saturated at ω≈2J, while in an NFL the spectral weight should saturate only at the total bandwidth which is much larger than 2J.

  14. Inelastic x-ray scattering measurements of phonon dynamics in URu2Si2

    DOE PAGES

    Gardner, D. R.; Bonnoit, C. J.; Chisnell, R.; Said, A. H.; Leu, B. M.; Williams, Travis J.; Luke, G. M.; Lee, Y. S.

    2016-02-11

    In this paper, we study high-resolution inelastic x-ray scattering measurements of the acoustic phonons of URu2Si2. At all temperatures, the longitudinal acoustic phonon linewidths are anomalously broad at small wave vectors revealing a previously unknown anharmonicity. The phonon modes do not change significantly upon cooling into the hidden order phase. In addition, our data suggest that the increase in thermal conductivity in the hidden order phase cannot be driven by a change in phonon dispersions or lifetimes. Hence, the phonon contribution to the thermal conductivity is likely much less significant compared to that of the magnetic excitations in the lowmore » temperature phase.« less

  15. Kohn anomaly in MgB2 by inelastic X-ray scattering.

    PubMed

    Baron, A Q R; Uchiyama, H; Tanaka, Y; Tsutsui, S; Ishikawa, D; Lee, S; Heid, R; Bohnen, K-P; Tajima, S; Ishikawa, T

    2004-05-14

    We study phonons in MgB2 using inelastic x-ray scattering (1.6 and 6 meV resolution). We clearly observe the softening and broadening of the crucial E(2g) mode through the Kohn anomaly along GammaM, in excellent agreement with ab initio calculations. Low temperature measurements (just above and below T(c)) show negligible changes for the momentum transfers investigated and no change in the E(2g) mode at A between room temperature and 16 K. We report the presence of a longitudinal mode along GammaA near in energy to the E(2g) mode that is not predicted by theory.

  16. Resonant inelastic hard x-ray scattering with diced analyzer crystals and position-sensitive detectors

    SciTech Connect

    Huotari, S.; Albergamo, F.; Vanko, Gy.; Verbeni, R.; Monaco, G.

    2006-05-15

    A novel design of a high-resolution spectrometer is proposed for emission spectroscopy and resonant inelastic hard x-ray scattering applications. The spectrometer is based on a Rowland circle geometry with a diced analyzer crystal and a position-sensitive detector. The individual flat crystallites of the diced analyzer introduce a well-defined linear position-energy relationship within the analyzer focus. This effect can be exploited to measure emission spectra with an unprecedented resolution. For demonstration, a spectrometer was constructed using a diced Si(553) analyzer working at the Cu K edge with an intrinsic resolution of 60 meV. With the proposed design, spectrometers operating at the K edges of 3d transition metals can have intrinsic resolutions below 100 meV even with analyzer crystals not working in Bragg-backscattering conditions.

  17. Collective dynamics in fully hydrated phospholipid bilayers studied by inelastic x-ray scattering.

    PubMed

    Chen, S H; Liao, C Y; Huang, H W; Weiss, T M; Bellisent-Funel, M C; Sette, F

    2001-01-22

    The short wavelength density fluctuation of DLPC (dilaurylphosphatidylcholine) bilayers close to full hydration has been studied by the inelastic x-ray scattering technique below and above the main transition temperature. The analysis based on a generalized three effective eigenmode theory allows us to construct the dispersion relation of the high frequency sound mode for the first time. The marked softening of the excitation near k = 14 nm(-1), corresponding to the lipid chain-chain correlation peak in the structure factor, in the L(alpha) phase implies prevalent occurrences of short-wavelength in-plane motions of lipid chains that might be of importance for transportation of small molecules across membranes. PMID:11177926

  18. The correlation timescale of the X-ray flux during the outbursts of soft X-ray transients

    NASA Astrophysics Data System (ADS)

    Wu, Yuxiang; Yu, Wenfei; Li, Tipei

    2010-01-01

    Recent studies of black hole and neutron star low mass X-ray binaries (LMXBs) show a positive correlation between the X-ray flux at which the low/hard(LH)-to-high/soft(HS) state transition occurs and the peak flux of the following HS state. By analyzing the data from the All Sky Monitor (ASM) onboard the Rossi X-ray Timing Explorer (RXTE), we show that the HS state flux after the source reaches its HS flux peak still correlates with the transition flux during soft X-ray transient (SXT) outbursts. By studying large outbursts or flares of GX 339-4, Aql X-1 and 4U 1705-44, we have found that the correlation holds up to 250, 40, and 50 d after the LH-to-HS state transition, respectively. These time scales correspond to the viscous time scale in a standard accretion disk around a stellar mass black hole or a neutron star at a radius of ˜104-5 R g, indicating that the mass accretion rates in the accretion flow either correlate over a large range of radii at a given time or correlate over a long period of time at a given radius. If the accretion geometry is a two-flow geometry composed of a sub-Keplerian inflow or outflow and a disk flow in the LH state, the disk flow with a radius up to ˜105 R g would have contributed to the nearly instantaneous non-thermal radiation directly or indirectly, and therefore affects the time when the state transition occurs.

  19. Partially coherent wavefront propagation simulations for inelastic x-ray scattering beamline including crystal optics

    NASA Astrophysics Data System (ADS)

    Suvorov, Alexey; Cai, Yong Q.; Sutter, John P.; Chubar, Oleg

    2014-09-01

    Up to now simulation of perfect crystal optics in the "Synchrotron Radiation Workshop" (SRW) wave-optics computer code was not available, thus hindering the accurate modelling of synchrotron radiation beamlines containing optical components with multiple-crystal arrangements, such as double-crystal monochromators and high-energy-resolution monochromators. A new module has been developed for SRW for calculating dynamical diffraction from a perfect crystal in the Bragg case. We demonstrate its successful application to the modelling of partially-coherent undulator radiation propagating through the Inelastic X-ray Scattering (IXS) beamline of the National Synchrotron Light Source II (NSLS-II) at Brookhaven National Laboratory. The IXS beamline contains a double-crystal and a multiple-crystal highenergy- resolution monochromator, as well as complex optics such as compound refractive lenses and Kirkpatrick-Baez mirrors for the X-ray beam transport and shaping, which makes it an excellent case for benchmarking the new functionalities of the updated SRW codes. As a photon-hungry experimental technique, this case study for the IXS beamline is particularly valuable as it provides an accurate evaluation of the photon flux at the sample position, using the most advanced simulation methods and taking into account parameters of the electron beam, details of undulator source, and the crystal optics.

  20. Inelastic x-ray scattering in vicinity of xenon L{sub 3} edge

    SciTech Connect

    Zitnik, M.; Kavcic, M.; Bucar, K.; Mihelic, A.; Stuhec, M.; Kokalj, J.; Szlachetko, J.

    2007-09-15

    A series of x-ray emission spectra of xenon in the region of L{sub 3}M{sub 5,4}(L{alpha}{sub 1,2}) and L{sub 3}N{sub 5,4}(L{beta}{sub 2,15}) lines were recorded along the polarization direction of the incoming photons with energies ranging from 4779.4 to 4804.4 eV. A combination of monochromatic photon beam and high resolution x-ray spectrometer resulted in the experimental broadening of 1 eV allowing the observation of resonantly enhanced and narrowed emission lines from the decay of [2p{sub 3/2}]nd,ns states. The measured spectra are decomposed into the continuum and resonant contributions to determine their relative emission strengths and the energies of the lowest resonant excitations converging to the L{sub 3} edge. The calculated differential cross section for inelastically scattered photons is compared to the measured data. Each of the resonant states is described by a single relativistic configuration in the frame of the Dirac-Fock model, and the continuum contribution to the scattered light is evaluated within the Caldwell-Zare approach, which neglects anisotropic interaction of the ejected electron with the ion.

  1. Incident-energy-dependent spectral weight of resonant inelastic x-ray scattering in doped cuprates

    NASA Astrophysics Data System (ADS)

    Tsutsui, Kenji; Tohyama, Takami

    2016-08-01

    We theoretically investigate the incident-photon energy ωi dependence of resonant inelastic x-ray scattering (RIXS) tuned for the Cu L edge in cuprate superconductors by using the exact diagonalization technique for a single-band Hubbard model. Depending on the value of core-hole Coulomb interaction in the intermediate state, RIXS for non-spin-flip channel shows either a ωi-dependent fluorescencelike or ωi-independent Raman-like behavior for hole doping. An analysis of x-ray absorption suggests that the core-hole Coulomb interaction is larger than on-site Coulomb interaction in the Hubbard model, resulting in a fluorescencelike behavior in RIXS consistent with recent RIXS experiments. A shift on the high-energy side of the center of spectral distribution is also predicted for electron-doped systems though spectral weight is small. Main structures in the spin-flip channel exhibit a Raman-like behavior as expected, accompanied with a fluorescencelike behavior with small intensity.

  2. Real-time cumulant approach for inelastic losses in x-ray spectra

    NASA Astrophysics Data System (ADS)

    Kas, J. J.; Rehr, J. J.; Curtis, J. B.

    Intrinsic inelastic losses in core level x-ray absorption (XAS), emission (XES), and x-ray photo-emission spectra (XPS), arise from excitations of the system due to the sudden creation or annihilation of a deep core hole. Additional extrinsic losses arise during the propagation of the photoelectron, and interference processes are also important. These excitations are reflected in the satellite peaks observed in XPS. Formally the distribution of these excitations are described in terms of the core-hole spectral function, which can be calculated in terms of the core-hole Green's function represented in exponential form. Here we discuss an approach for calculating the exponent, or cumulant in terms of local density fluctuations via real-space, real-time time-dependent density functional theory. The role of extrinsic and interference terms is also discussed. Our method is illustrated in calculations of XAS and XPS for number of systems, including weakly correlated as well as d- and f-electron materials. Supported by DOE BES Grant DE-FG03-97ER45623.

  3. Grazing-incidence cylindric mirror with multiple reflection for the soft X-ray spectral range

    NASA Astrophysics Data System (ADS)

    Alexandrov, Yu. M.; Fedin, D. A.; Fedorchuk, R. V.; Koshevoi, M. O.; Kozhevnikov, I. V.; Murashova, V. A.; Pisarzyk, T.; Rupasov, A. A.; Shikanov, A. S.; Yakimenko, M. N.; Vinogradov, A. V.

    1991-10-01

    New possibilities of the SR beam control are opened with the use of grazing incidence elements based on the "whispering gallery" effect. Experimental investigations of such an X-ray optical element have been performed on the S-60 synchrotron at the Lebedev Institute. By using the absolute spectral characteristics of the X-ray photofilm RAR 2497 (Kodak) and the SR spectral shape we have determined the output-angle integral spectral coefficient of reflection of the studied mirror. A high value of the reflection coefficient makes it possible to use such an X-ray optical element as the effective reflector for soft X-ray beams.

  4. Biological imaging by soft x-ray diffraction microscopy

    SciTech Connect

    Shapiro, D.; Thibault, P.; Beetz, T.; Elser, V.; Howells, M.; Jacobsen, C.; Kirz, J.; Lima, E.; Miao, H.; Neiman, A. M.; Sayre, D.

    2005-10-25

    We have used the method of x-ray diffraction microscopy to image the complex-valued exit wave of an intact and unstained yeast cell. The images of the freeze-dried cell, obtained by using 750-eV x-rays from different angular orientations, portray several of the cell's major internal components to 30-nm resolution. The good agreement among the independently recovered structures demonstrates the accuracy of the imaging technique. To obtain the best possible reconstructions, we have implemented procedures for handling noisy and incomplete diffraction data, and we propose a method for determining the reconstructed resolution. This work represents a previously uncharacterized application of x-ray diffraction microscopy to a specimen of this complexity and provides confidence in the feasibility of the ultimate goal of imaging biological specimens at 10-nm resolution in three dimensions.

  5. Biological imaging by soft x-ray diffraction microscopy

    DOE PAGES

    Shapiro, D.; Thibault, P.; Beetz, T.; Elser, V.; Howells, M.; Jacobsen, C.; Kirz, J.; Lima, E.; Miao, H.; Neiman, A. M.; et al

    2005-10-25

    We have used the method of x-ray diffraction microscopy to image the complex-valued exit wave of an intact and unstained yeast cell. The images of the freeze-dried cell, obtained by using 750-eV x-rays from different angular orientations, portray several of the cell's major internal components to 30-nm resolution. The good agreement among the independently recovered structures demonstrates the accuracy of the imaging technique. To obtain the best possible reconstructions, we have implemented procedures for handling noisy and incomplete diffraction data, and we propose a method for determining the reconstructed resolution. This work represents a previously uncharacterized application of x-ray diffractionmore » microscopy to a specimen of this complexity and provides confidence in the feasibility of the ultimate goal of imaging biological specimens at 10-nm resolution in three dimensions.« less

  6. Imaging cochlear soft tissue displacement with coherent x-rays

    NASA Astrophysics Data System (ADS)

    Rau, Christoph; Richter, Claus-Peter

    2015-10-01

    At present, imaging of cochlear mechanics at mid-cochlear turns has not been accomplished. Although challenging, this appears possible with partially coherent hard x-rays. The present study shows results from stroboscopic x-ray imaging of a test object at audio frequencies. The vibration amplitudes were quantified. In a different set of experiments, an intact and calcified gerbil temporal bone was used to determine displacements of the reticular lamina, tectorial membrane, and Reissner’s membrane with the Lucas and Kanade video flow algorithm. The experiments validated high frequency x-ray imaging and imaging in a calcified cochlea. The present work is key for future imaging of cochlear micromechanics at a high spatial resolution.

  7. A new soft x-ray pulse height analysis array in the HL-2A tokamak

    SciTech Connect

    Zhang, Y. P.; Liu Yi; Yang, J. W.; Song, X. Y.; Liao, M.; Li, X.; Yuan, G. L.; Yang, Q. W.; Duan, X. R.; Pan, C. H.

    2009-12-15

    A new soft x-ray pulse height analysis (PHA) array including nine independent subsystems, on basis of a nonconventional software multichannel analysis system and a silicon drift detector (SDD) linear array consisting of nine high performance SDD detectors, has been developed in the HL-2A tokamak. The use of SDD has greatly improved the measurement accuracy and the spatiotemporal resolutions of the soft x-ray PHA system. Since the ratio of peak to background counts obtained from the SDD PHA system is very high, p/b{>=}3000, the soft x-ray spectra measured by the SDD PHA system can approximatively be regarded as electron velocity distribution. The electron velocity distribution can be well derived in the pure ohmic and auxiliary heating discharges. The performance of the new soft x-ray PHA array and the first experimental results with some discussions are presented.

  8. Homogeneous focusing with a transient soft X-ray laser for irradiation experiments

    NASA Astrophysics Data System (ADS)

    Kazamias, S.; Cassou, K.; Guilbaud, O.; Klisnick, A.; Ros, D.; Plé, F.; Jamelot, G.; Rus, B.; Koslová, M.; Stupka, M.; Mocek, T.; Douillet, D.; Zeitoun, Ph.; Joyeux, D.; Phalippou, D.

    2006-07-01

    We report the work done on a transient soft X-ray laser (SXRL) beam to deliver a proper extreme UV irradiation source for applications. The same optical tool was first demonstrated on a quasi stationnary state (QSS) soft X-Ray laser at the PALS Institute in Prague. The problem set by the transient soft X-Ray laser developed by the LIXAM at the LULI installation in Palaiseau is more crucial, first because the beam spatial profile is more irregular secondly because high repetition rate soft X-ray laser facilities in the future are based on this SXRL type. The spots obtained show a 20 micron average diameter and a rather homogeneous and smooth profile that make them a realistic irradiation source to interact with targets requiring relatively high fluence (near 1 J/cm 2) or intensity (near 10 11 W/cm 2) in the extreme UV domain.

  9. Bright High Average Power Table-top Soft X-Ray Lasers

    SciTech Connect

    Rocca, Jorge; Reagan, Brendon; Wernsing, Keith; Luther, Brad; Curtis, Alden; Nichols,, Anthony; Wang, Yong; Alessi, David; Martz, Dale; Yin, Liang; Wang, Shoujun; Berrill, Mark A; Furch, Federico; Woolston, Mark; Patel, Dinesh; Marconi, Mario; Menoni, Carmen

    2012-01-01

    We have demonstrated the generation of bright soft x-ray laser pulses with record-high average power from compact plasma amplifiers excited by ultrafast solid state lasers. These lasers have numerous applications in nanoscience and nanotechnology.

  10. Investigation of the amorphous to crystalline phase transition of chemical solution deposited Pb(Zr30Ti70)O3 thin films by soft x-ray absorption and soft x-ray emission spectroscopy

    SciTech Connect

    Schneller, T.; Schneller, T.; Kohlstedt, H.; Petraru, A.; Waser, R.; Guo, J.; Denlinger, J.; Learmonth, T.; Glans, Per-Andres; Smith, K. E.

    2008-08-01

    Chemical solution deposited (CSD) complex oxide thin films attract considerable interest in various emerging fields as for example, fuel cells, ferroelectric random access memories or coated conductors. In the present paper the results of soft-x-ray spectroscopy between 100 eV and 500 eV on the amorphous to crystalline phase transition of ferroelectric PbZr{sub 0.3}Ti{sub 0.7}O{sub 3} (PZT) thin films are presented. Five CSD samples derived from the same wafer coated with a PZT film pyrolyzed at 350 C were heat treated at different temperatures between 400 C and 700 C. At first the sample were morphologically and electrically characterized. Subsequently the soft-x-ray absorption and emission experiments were performed at the undulator beamline 8.0 of the Advanced Light Source of the Lawrence Berkeley National Laboratory. Soft-x-ray absorption spectra were acquired for the Ti L{sub 2,3-}, O K-, and C K-edge thresholds by using simultaneously the total electron yield (TEY) and total fluorescence yield (TFY) detection methods. For two samples, annealed at 400 C and 700 C, respectively, the resonant inelastic soft-x-ray spectroscopy (RIXS) was applied for various excitation energies near the Ti L-, O K-edges. We observed clear evidence of a rutile phase at untypically low temperatures. This rutile phase transforms into the perovskite phase upon increasing annealing temperature. These results are discussed in the framework of current microscopic models of the PZT (111) texture selection.

  11. Absolutely calibrated soft-x-ray streak camera for laser-fusion applications

    SciTech Connect

    Kauffman, R.L.; Medecki, H.; Stradling, G.

    1982-01-01

    The intensity output of a soft-x-ray streak camera was calibrated (SXRSC) in order to make absolute flux measurements of x rays emitted from laser-produced plasmas. The SXRSC developed at LLNL is used to time-resolve x-ray pulses to better than 20 ps. The SXRSC uses a Au photocathode on a thin carbon substrate which is sensitive to x rays from 100 eV to greater than 10 keV. Calibrations are done in the dynamic mode using a small laser-produced x-ray source. The SXRSC is calibrated by comparing its integrated signal to the output of calibrated x-ray diodes monitoring the source strength. The measured SXRSC response is linear over greater than two orders of magnitude. Using these calibrations, absolute intensities can be measured to an accuracy of +-30%.

  12. Introduction of Soft X-Ray Spectromicroscopy as an Advanced Technique for Plant Biopolymers Research

    PubMed Central

    Karunakaran, Chithra; Christensen, Colleen R.; Gaillard, Cedric; Lahlali, Rachid; Blair, Lisa M.; Perumal, Vijayan; Miller, Shea S.; Hitchcock, Adam P.

    2015-01-01

    Soft X-ray absorption spectroscopy coupled with nano-scale microscopy has been widely used in material science, environmental science, and physical sciences. In this work, the advantages of soft X-ray absorption spectromicroscopy for plant biopolymer research were demonstrated by determining the chemical sensitivity of the technique to identify common plant biopolymers and to map the distributions of biopolymers in plant samples. The chemical sensitivity of soft X-ray spectroscopy to study biopolymers was determined by recording the spectra of common plant biopolymers using soft X-ray and Fourier Transform mid Infrared (FT-IR) spectroscopy techniques. The soft X-ray spectra of lignin, cellulose, and polygalacturonic acid have distinct spectral features. However, there were no distinct differences between cellulose and hemicellulose spectra. Mid infrared spectra of all biopolymers were unique and there were differences between the spectra of water soluble and insoluble xylans. The advantage of nano-scale spatial resolution exploited using soft X-ray spectromicroscopy for plant biopolymer research was demonstrated by mapping plant cell wall biopolymers in a lentil stem section and compared with the FT-IR spectromicroscopy data from the same sample. The soft X-ray spectromicroscopy enables mapping of biopolymers at the sub-cellular (~30 nm) resolution whereas, the limited spatial resolution in the micron scale range in the FT-IR spectromicroscopy made it difficult to identify the localized distribution of biopolymers. The advantages and limitations of soft X-ray and FT-IR spectromicroscopy techniques for biopolymer research are also discussed. PMID:25811457

  13. The possible effect of solar soft X rays on thermospheric nitric oxide

    NASA Astrophysics Data System (ADS)

    Siskind, D. E.; Barth, C. A.; Cleary, D. D.

    1990-04-01

    A rocket observation of nitric oxide in the lower thermosphere during a time of high solar activity is compared to the results of calculations from a one-dimensional photochemical model. A solar soft X-ray flux of 0.75 erg/sq cm/s is needed to explain the observed NO densities. This result supports the theory that the variation in the low-latitude thermospheric NO is caused by variation in solar soft X-rays.

  14. Introduction of soft X-ray spectromicroscopy as an advanced technique for plant biopolymers research.

    PubMed

    Karunakaran, Chithra; Christensen, Colleen R; Gaillard, Cedric; Lahlali, Rachid; Blair, Lisa M; Perumal, Vijayan; Miller, Shea S; Hitchcock, Adam P

    2015-01-01

    Soft X-ray absorption spectroscopy coupled with nano-scale microscopy has been widely used in material science, environmental science, and physical sciences. In this work, the advantages of soft X-ray absorption spectromicroscopy for plant biopolymer research were demonstrated by determining the chemical sensitivity of the technique to identify common plant biopolymers and to map the distributions of biopolymers in plant samples. The chemical sensitivity of soft X-ray spectroscopy to study biopolymers was determined by recording the spectra of common plant biopolymers using soft X-ray and Fourier Transform mid Infrared (FT-IR) spectroscopy techniques. The soft X-ray spectra of lignin, cellulose, and polygalacturonic acid have distinct spectral features. However, there were no distinct differences between cellulose and hemicellulose spectra. Mid infrared spectra of all biopolymers were unique and there were differences between the spectra of water soluble and insoluble xylans. The advantage of nano-scale spatial resolution exploited using soft X-ray spectromicroscopy for plant biopolymer research was demonstrated by mapping plant cell wall biopolymers in a lentil stem section and compared with the FT-IR spectromicroscopy data from the same sample. The soft X-ray spectromicroscopy enables mapping of biopolymers at the sub-cellular (~30 nm) resolution whereas, the limited spatial resolution in the micron scale range in the FT-IR spectromicroscopy made it difficult to identify the localized distribution of biopolymers. The advantages and limitations of soft X-ray and FT-IR spectromicroscopy techniques for biopolymer research are also discussed.

  15. Running Shanghai Soft x-ray FEL with the EEHG scheme

    SciTech Connect

    Xiang, D; Stupakov, G.; /SLAC

    2008-12-18

    With the nominal beam parameters (beam energy: 0.84 GeV, slice energy spread: 168 keV, peak current: 600 A, normalized emittance: 2 mm mrad) of the Shanghai soft X-ray Free Electron Laser (SXFEL) project, we show that using the echo-enabled harmonic generation (EEHG) scheme, 9 nm coherent soft x-ray with peak power exceeding 400 MW can be generated directly from the 270 nm seeding laser.

  16. Inelastic X-ray scattering from 6H-SiC

    SciTech Connect

    Macrander, A.T.; Blasdell, B.; Montano, P.A. |; Kao, C.C.

    1995-07-01

    The authors have studied electronic excitations in 6H-SiC using inelastic x-ray scattering. Inelastic scattering spectra were measured at momentum transfers ranging from 0.47 {angstrom}{sup {minus}1} to 2.00 {angstrom}{sup {minus}1} along the c-axis in the hexagonal lattice, i.e. , along [00{center_dot}1], and from 0.67 {angstrom}{sup {minus}1} to 2.00 {angstrom}{sup {minus}1} along the a-axis, i.e., alone, [10{center_dot}0]. Comparison of the two sets of data reveals an orientation dependence of the spectra, except for a characteristic peak at 22--23 eV that occurs for both directions at low Q. This peak has also been observed in electron energy loss spectroscopy studies and is identified as a bulk plasmon. The orientation dependence of the other spectral features is indicative of band structure effects. These data were obtained using a Ge(444) analyzer in a near backscattering geometry.

  17. Crystal Dynamics of (delta) fcc Pu-Ga by High Resolution Inelastic X-Ray Scattering

    SciTech Connect

    Wong, J; Krisch, M; Farber, D; Occelli, F; Xu, R; Chiang, T C; Clatterbuck, D; Schwartz, A J; Wall, M; Boro, C

    2004-09-28

    We have used a microbeam on large grain sample concept to carry out an inelastic x-ray scattering experiment to map the full phonon dispersion curves of an fcc {delta}-phase Pu-Ga alloy. This approach obviates experimental difficulties with conventional inelastic neutron scattering due to the high absorption cross section of the common {sup 239}Pu isotope and the non-availability of large (mm size) single crystal materials for Pu and its alloys. A classical Born von-Karman force constant model was used to model the experimental results, and no less than 4th nearest neighbor interactions had to be included to account for the observation. Several unusual features including, a large elastic anisotropy, a small shear elastic modulus, (C{sub 11}-C{sub 12})/2, a Kohn-like anomaly in the T{sub 1}[011] branch, and a pronounced softening of the T[111] branch towards the L point in the Brillouin are found. These features can be related to the phase transitions of plutonium and to strong coupling between the crystal structure and the 5f valence instabilities. Our results represent the first full phonon dispersions ever obtained for any Pu-bearing material, thus ending a 40-year quest for this fundamental data. The phonon data also provide a critical test for theoretical treatments of highly correlated 5f electron systems as exemplified by recent dynamical mean field theory (DMFT) calculations for {delta}-plutonium.

  18. Observation of soft X-ray emission from the supernova remnant HB9

    NASA Technical Reports Server (NTRS)

    Tuohy, I. R.; Clark, D. H.; Garmire, G. P.

    1979-01-01

    The number of known X-ray emitting supernova remnants in our galaxy has significantly grown as a result of the soft X-ray survey by the HEAO-1 spacecraft. The HEAO-1 A-2 experiment has observed soft X-ray emission from the old supernova remnant HB9 which lies close to the previously identified X-ray source, Capella. Spectral data and the low optical obscuration in the direction of the remnant suggest that HB9 is a good candidate for detecting Fe XIV coronal forbidden-line emission. Mapping of the coronal line emission in association with the imaging X-ray data expected from HEAO-2 would allow the temperature profile of the emitting shell to be determined in a manner similar to that used by Tuohy, Nousek, and Garmire (1979) for the Cygnus Loop, which is in a similar evolutionary phase to HB9.

  19. The X-ray eclipse geometry of the super-soft X-ray source CAL 87

    SciTech Connect

    Ribeiro, T.; Lopes de Oliveira, R.

    2014-09-01

    We explore XMM-Newton observations of the eclipsing super-soft X-ray source CAL 87 in order to map the accretion structures of the system. Indirect imaging techniques were applied in X-ray light curves to provide eclipse maps. The surface brightness distribution exhibits an extended and symmetric emission, and a feature is revealed from the hardest X-rays that is likely due to a bright spot. A rate of P-dot =(+6±2)×10{sup −10} for changes in the orbital period of the system was derived from the eclipses. There is no significant variation of the emission lines even during eclipses, arguing that the lines are formed in an extended region. The continuum emission dominates the decrease in flux that is observed during eclipses. The O VIII Lyα line reveals a broadening velocity that is estimated to be 365{sub −69}{sup +65} km s{sup –1} (at 1σ), marginal evidence for asymmetry in its profile, and sometimes shows evidence of double-peaked emission. Together, the results support that the wind-driven mass transfer scenario is running in CAL 87.

  20. Development of Multilayer Optics in EUV, Soft X-Ray and X-Ray Range at IPOE

    NASA Astrophysics Data System (ADS)

    Wang, Zhanshan; Zhu, Jingtao; Zhang, Zhong; Cheng, Xinbin; Xu, Jing; Wang, Fengli; Wang, Xiaoqiang; Chen, Lingyan

    Multilayer coatings are key optical components in the EUV, soft X-ray and X-ray range. At Institute of Precision Optical Engineering (IPOE), the development of multilayer optics has been impelled for their wide applications in X-ray laser, plasma diagnostics, astronomical observation and synchrotron radiation. The paper presents our recent results of periodic multilayers of Mo/Si, Cr/C, Cr/Sc, La/B4C, Mo/B4C, Si/C, Si/SiC, Mg/SiC Mo/Y and Ru/Y. To improve the reflectivity of Ru/Y multilayer mirrors, Mo layers were inserted between Ru and Y layer. The Mo barrier layers suppress intermixing between Ru and Y, thereby increasing the reflectivity of Ru/Y multilayer. We also discuss the application of Mo/Si, Mo/Y, Mo/B4C, La/B4C non-periodic multilayers in EUV broadband polarization measurement.

  1. Progress and prospects in soft x-ray holographic microscopy

    SciTech Connect

    Howells, M.R.; Jacobsen, C.; Kirz, J.; McQuaid, K.; Rothman, S.S.

    1987-12-01

    We report some of the latest developments in x-ray holography experiments and make some speculations about the limits of performance of the approaches currently in use. We also make some suggestions about where the technique can (and cannot) go in the future. 32 refs., 5 figs., 1 tab.

  2. Soft X-ray astronomy using grazing incidence optics

    NASA Technical Reports Server (NTRS)

    Davis, John M.

    1989-01-01

    The instrumental background of X-ray astronomy with an emphasis on high resolution imagery is outlined. Optical and system performance, in terms of resolution, are compared and methods for improving the latter in finite length instruments described. The method of analysis of broadband images to obtain diagnostic information is described and is applied to the analysis of coronal structures.

  3. A hard X-ray view of the soft excess in AGN

    NASA Astrophysics Data System (ADS)

    Boissay, Rozenn; Ricci, Claudio; Paltani, Stéphane

    2016-04-01

    An excess of X-ray emission below 1 keV, called soft excess, is detected in a large fraction of Seyfert 1-1.5s. The origin of this feature remains debated, as several models have been suggested to explain it, including warm Comptonization and blurred ionized reflection. In order to constrain the origin of this component, we exploit the different behaviors of these models above 10 keV. Ionized reflection covers a broad energy range, from the soft X-rays to the hard X-rays, while Comptonization drops very quickly in the soft X-rays. We present here the results of a study done on 102 Seyfert 1s (Sy 1.0, 1.2, 1.5 and NLSy1) from the Swift BAT 70-Month Hard X-ray Survey catalog. The joint spectral analysis of Swift/BAT and XMM-Newton data allows a hard X-ray view of the soft excess that is present in about 80% of the objects of our sample. We discuss how the soft-excess strength is linked to the reflection at high energy, to the photon index of the primary continuum and to the Eddington ratio. In particular, we find a positive dependence of the soft excess intensity on the Eddington ratio. We compare our results to simulations of blurred ionized-reflection models and show that they are in contradiction. By stacking both XMM-Newton and Swift/BAT spectra per soft-excess strength, we see that the shape of reflection at hard X-rays stays constant when the soft excess varies, showing an absence of link between reflection and soft excess. We conclude that the ionized-reflection model as the origin of the soft excess is disadvantaged in favor of the warm Comptonization model in our sample of Seyfert 1s.

  4. A von Hamos x-ray spectrometer based on a segmented-type diffraction crystal for single-shot x-ray emission spectroscopy and time-resolved resonant inelastic x-ray scattering studies

    SciTech Connect

    Szlachetko, J.; Nachtegaal, M.; Boni, E. de; Willimann, M.; Safonova, O.; Sa, J.; Smolentsev, G.; Szlachetko, M.; Bergamaschi, A.; Schmitt, B.; David, C.; Luecke, A.; Bokhoven, J. A. van; Dousse, J.-Cl.; Hoszowska, J.; Kayser, Y.; Jagodzinski, P.

    2012-10-15

    We report on the design and performance of a wavelength-dispersive type spectrometer based on the von Hamos geometry. The spectrometer is equipped with a segmented-type crystal for x-ray diffraction and provides an energy resolution in the order of 0.25 eV and 1 eV over an energy range of 8000 eV-9600 eV. The use of a segmented crystal results in a simple and straightforward crystal preparation that allows to preserve the spectrometer resolution and spectrometer efficiency. Application of the spectrometer for time-resolved resonant inelastic x-ray scattering and single-shot x-ray emission spectroscopy is demonstrated.

  5. A von Hamos x-ray spectrometer based on a segmented-type diffraction crystal for single-shot x-ray emission spectroscopy and time-resolved resonant inelastic x-ray scattering studies.

    PubMed

    Szlachetko, J; Nachtegaal, M; de Boni, E; Willimann, M; Safonova, O; Sa, J; Smolentsev, G; Szlachetko, M; van Bokhoven, J A; Dousse, J-Cl; Hoszowska, J; Kayser, Y; Jagodzinski, P; Bergamaschi, A; Schmitt, B; David, C; Lücke, A

    2012-10-01

    We report on the design and performance of a wavelength-dispersive type spectrometer based on the von Hamos geometry. The spectrometer is equipped with a segmented-type crystal for x-ray diffraction and provides an energy resolution in the order of 0.25 eV and 1 eV over an energy range of 8000 eV-9600 eV. The use of a segmented crystal results in a simple and straightforward crystal preparation that allows to preserve the spectrometer resolution and spectrometer efficiency. Application of the spectrometer for time-resolved resonant inelastic x-ray scattering and single-shot x-ray emission spectroscopy is demonstrated.

  6. Soft X-ray induced damage in PVA-based membranes in water environment monitored by X-ray absorption spectroscopy

    NASA Astrophysics Data System (ADS)

    Tzvetkov, George; Späth, Andreas; Fink, Rainer H.

    2014-10-01

    The effect of synchrotron X-ray flux in a soft X-ray scanning-transmission microspectroscope (STXM) instrument on the chemical structure of air-filled poly(vinyl alcohol) (PVA) based microbubbles and their stabilizing shell has been examined. Prolonged soft X-ray illumination of the particles in aqueous suspension leads to the breaking of the microbubbles' protective polymer shell and substantial chemical changes. The latter were clarified via a micro-spot C K-edge near-edge X-ray absorption fine structure (NEXAFS) spectroscopy with further respect to the absorbed X-ray doses. Our results revealed a continuous degradation of the PVA network associated with formation of carbonyl- and carboxyl-containing species as well as an increased content of unsaturated bonds. The observed effects must be taken into account in studies of micro- and nanostructured polymer materials utilizing X-rays.

  7. A table-top femtosecond time-resolved soft x-ray transient absorption spectrometer

    SciTech Connect

    Leone, Stephen; Loh, Zhi-Heng; Khalil, Munira; Correa, Raoul E.; Leone, Stephen R.

    2008-05-21

    A laser-based, table-top instrument is constructed to perform femtosecond soft x-ray transient absorption spectroscopy. Ultrashort soft x-ray pulses produced via high-order harmonic generation of the amplified output of a femtosecond Ti:sapphire laser system are used to probe atomic core-level transient absorptions in atoms and molecules. The results provide chemically specific, time-resolved dynamics with sub-50-fs time resolution. In this setup, high-order harmonics generated in a Ne-filled capillary waveguide are refocused by a gold-coated toroidal mirror into the sample gas cell, where the soft x-ray light intersects with an optical pump pulse. The transmitted high-order harmonics are spectrally dispersed with a home-built soft x-ray spectrometer, which consists of a gold-coated toroidal mirror, a uniform-line spaced plane grating, and a soft x-ray CCD camera. The optical layout of the instrument, design of the soft x-ray spectrometer, and spatial and temporal characterization of the high-order harmonics are described. Examples of static and time-resolved photoabsorption spectra collected on this apparatus are presented.

  8. Ground Laboratory Soft X-Ray Durability Evaluation of Aluminized Teflon FEP Thermal Control Insulation. Revised

    NASA Technical Reports Server (NTRS)

    Banks, Bruce A.; deGroh, Kim K.; Stueber, Thomas J.; Sechkar, Edward A.; Hall, Rachelle L.

    1998-01-01

    Metallized Teflon fluorinated ethylene propylene (FEP) thermal control insulation is mechanically degraded if exposed to a sufficient fluence of soft x-ray radiation. Soft x-ray photons (4-8 A in wavelength or 1.55 - 3.2 keV) emitted during solar flares have been proposed as a cause of mechanical properties degradation of aluminized Teflon FEP thermal control insulation on the Hubble Space Telescope (HST). Such degradation can be characterized by a reduction in elongation-to-failure of the Teflon FEP. Ground laboratory soft x-ray exposure tests of aluminized Teflon FEP were conducted to assess the degree of elongation degradation which would occur as a result of exposure to soft x-rays in the range of 3-10 keV. Tests results indicate that soft x-ray exposure in the 3-10 keV range, at mission fluence levels, does not alone cause the observed reduction in elongation of flight retrieved samples. The soft x-ray exposure facility design, mechanical properties degradation results and implications will be presented.

  9. Ground Laboratory Soft X-Ray Durability Evaluation of Aluminized Teflon FEP Thermal Control Insulation

    NASA Technical Reports Server (NTRS)

    Banks, Bruce A.; deGroh, Kim K.; Stueber, Thomas J.; Sechkar, Edward A.

    1998-01-01

    Metallized Teflon fluorinated ethylene propylene (FEP) thermal control insulation is mechanically degraded if exposed to a sufficient fluence of soft x-ray radiation. Soft x-ray photons (4-8 A in wavelength or 1.55 - 3.2 keV) emitted during solar flares have been proposed as a cause of mechanical properties degradation of aluminized Teflon FEP thermal control insulation on the Hubble Space Telescope (HST). Such degradation can be characterized by a reduction in elongation-to-failure of the Teflon FER Ground laboratory soft x-ray exposure tests of aluminized Teflon FEP were conducted to assess the degree of elongation degradation which would occur as a result of exposure to soft x-rays in the range of 3-10 keV. Tests results indicate that soft x-ray exposure in the 3-10 keV range, at mission fluence levels, does not alone cause the observed reduction in elongation of flight retrieved samples. The soft x-ray exposure facility design, mechanical properties degradation results and implications will be presented.

  10. [Experimental investigation of laser plasma soft X-ray source with gas target].

    PubMed

    Ni, Qi-liang; Gong, Yan; Lin, Jing-quan; Chen, Bo; Cao, Jian-lin

    2003-02-01

    This paper describes a debris-free laser plasma soft X-ray source with a gas target, which has high operating frequency and can produce strong soft X-ray radiation. The valve of this light source is drived by a piezoelectrical ceramic whose operating frequency is up to 400 Hz. In comparison with laser plasma soft X-ray sources using metal target, the light source is debris-free. And it has higher operating frequency than gas target soft X-ray sources whose nozzle is controlled by a solenoid valve. A channel electron multiplier (CEM) operating in analog mode is used to detect the soft X-ray generated by the laser plasma source, and the CEM's output is fed to to a charge-sensitive preamplifier for further amplification purpose. Output charges from the CEM are proportional to the amplitude of the preamplifier's output voltage. Spectra of CO2, Xe and Kr at 8-14 nm wavelength which can be used for soft X-ray projection lithography are measured. The spectrum for CO2 consists of separate spectral lines originate mainly from the transitions in Li-like and Be-like ions. The Xe spectrum originating mainly from 4d-5f, 4d-4f, 4d-6p and 4d-5p transitions in multiply charged xenon ions. The spectrum for Kr consists of separate spectral lines and continuous broad spectra originating mainly from the transitions in Cu-, Ni-, Co- and Fe-like ions.

  11. Omega Dante soft x-ray power diagnostic component calibration at the National Synchrotron Light Source

    NASA Astrophysics Data System (ADS)

    Campbell, K. M.; Weber, F. A.; Dewald, E. L.; Glenzer, S. H.; Landen, O. L.; Turner, R. E.; Waide, P. A.

    2004-10-01

    The Dante soft x-ray spectrometer, installed on the Omega laser facility at the Laboratory for Laser Energetics, University of Rochester, is a 12-channel filter-edge defined soft x-ray power diagnostic. It is used to measure the spectrally resolved, absolute flux from direct drive, indirect drive (hohlraums) and other plasma sources. Dante component calibration efforts using two beam lines, U3C (50 eV-1 keV) and X8A (1-6 keV) at the National Synchrotron Light Source have been implemented to improve the accuracy of these measurements. We have calibrated metallic vacuum x-ray diodes, mirrors and filters.

  12. Studying Nanoscale Magnetism and its Dynamics with Soft X-ray Microscopy

    SciTech Connect

    Mccall, Monnikue M; Fischer, Peter

    2008-05-01

    Magnetic soft X-ray microscopy allows for imaging magnetic structures at a spatial resolution down to 15nm and a time resolution in the sub-100ps regime. Inherent elemental specificity can be used to image the magnetic response of individual components such as layers in multilayered systems. This review highlights current achievements and discusses the future potential of magnetic soft X-ray microscopy at fsec X-ray sources where snapshot images of ultrafast spin dynamics with a spatial resolution below 10nm will become feasible.

  13. Is the DA white dwarf 1910 + 047 a soft X-ray source?

    NASA Technical Reports Server (NTRS)

    Vennes, Stephane

    1990-01-01

    The possibility that the recently discovered DA white dwarf WD 1910 + 047 might be an Einstein soft X-ray source is studied, applying a complete model atmosphere analyis to both the optical and the soft X-ray data. It is found that the X-ray source in question is at least one order of magnitude too strong to be compatible with the estimated atmospheric parameters of the possible optical counterpart. The spatial coincidence between the two, however, remains extremely intriguing and has left us with the dilemma of accepting the relatively improbable coincidence of two unrelated objects or rejoicing over the discovery of a highly unusual one.

  14. Pushing the Boundaries of Suborbital Soft X-ray Spectroscopy

    NASA Astrophysics Data System (ADS)

    McEntaffer, Randall

    There are two primary objectives for this investigation. First, we propose to launch a preexisting payload to perform scientific investigations. Second, we propose to build a new payload which will integrate and demonstrate key technologies vital to future X-ray observatories. These efforts will train graduate students and prepare junior researchers to be major contributors to the next suite of NASA missions. We propose to increase the ability of gratings to obtain high resolution at energies below 1 keV. The concept that will be developed in this proposed investigation will be capable of meeting the requirements of future X-ray observatories. In addition, the design could be utilized effectively on smaller, Explorer class missions as pathfinders to the larger observatories while providing important scientific insights along the way. For this investigation, we propose to fly two separate, but related, rocket payloads. The first payload, christened OGRESS, has already been constructed and successfully flown three times. OGRESS is optimized to observe diffuse X-ray sources with a wire-grid collimating optic, parallel groove sinusoidal gratings, and Gaseous Electron Multiplier (GEM) detectors and is capable of attaining high resolution of E/dE ~ 25-80 in the 1/4 keV band. OGRESS will take high resolution spectra of the Vela Supernova Remnant (SNR) in the 1/4 keV band. This flight will provide the highest resolution spectra yet taken of Vela in this band and will produce a PhD thesis. The second payload, OGRE, will demonstrate key technologies necessary for the next X-ray observatory and provide even higher resolution of E/dE ~ 1000-2000 between 0.2 1.0 keV. To improve upon the resolution of OGRESS, OGRE will integrate several key technologies which have already been developed in a laboratory setting, but have not been flight proven. OGRE will use a modified Wolter telescope made from slumped glass to provide a smaller focus and increase throughput. Slumped glass

  15. Soft X-ray characterisation of the long-term properties of supergiant fast X-ray transients

    NASA Astrophysics Data System (ADS)

    Romano, P.; Ducci, L.; Mangano, V.; Esposito, P.; Bozzo, E.; Vercellone, S.

    2014-08-01

    Context. Supergiant fast X-ray transients (SFXTs) are high mass X-ray binaries (HMXBs) that are characterised by a hard X-ray (≥ 15 keV) flaring behaviour. These flares reach peak luminosities of 1036-1037 erg s-1 and last a few hours in the hard X-rays. Aims: We investigate the long-term properties of SFXTs by examining the soft (0.3-10 keV) X-ray emission of the three least active SFXTs in the hard X-ray and by comparing them with the remainder of the SFXT sample. Methods: We performed the first high-sensitivity soft X-ray long-term monitoring with Swift/XRT of three relatively unexplored SFXTs, IGR J08408-4503, IGR J16328-4726, and IGR J16465-4507, whose hard X-ray duty cycles are the lowest measured among the SFXT sample. We assessed how long each source spends in each flux state and compared their properties with those of the prototypical SFXTs. Results: The behaviour of IGR J08408-4503 and IGR J16328-4726 resembles that of other SFXTs, and it is characterised by a relatively high inactivity duty cycle (IDC) and pronounced dynamic range (DR) in the X-ray luminosity. We found DR ~ 7400, IDC ~ 67% for IGR J08408-4503, and DR ~ 750, IDC ~ 61% for IGR J16328-4726 (in all cases the IDC is given with respect to the limiting flux sensitivity of XRT, that is 1-3 × 10-12 erg cm-2 s-1). In common with all the most extreme SFXT prototypes (IGR J17544-2619, XTE J1739-302, and IGR J16479-4514), IGR J08408-4503 shows two distinct flare populations. The first one is associated with the brightest outbursts (X-ray luminosity LX ≳ 1035 - 36 erg s-1), while the second comprises dimmer events with typical luminosities of LX ≲ 1035 erg s-1. This double-peaked distribution of the flares as a function of the X-ray luminosity seems to be a ubiquitous feature of the extreme SFXTs. The lower DR of IGR J16328-4726 suggests that this is an intermediate SFXT. IGR J16465-4507 is characterised by a low IDC ~ 5% and a relatively narrow DR ~ 40, reminiscent of classical supergiant

  16. Time-resolved near-edge x-ray absorption fine structure spectroscopy on photo-induced phase transitions using a tabletop soft-x-ray spectrometer

    NASA Astrophysics Data System (ADS)

    Grossmann, P.; Rajkovic, I.; Moré, R.; Norpoth, J.; Techert, S.; Jooss, C.; Mann, Klaus

    2012-05-01

    We present a table-top soft-x-ray spectrometer for the wavelength range λ = 1-5 nm based on a stable laser-driven x-ray source, making use of a gas-puff target. With this setup, optical light-pump/soft-x-ray probe near-edge x-ray absorption fine structure (NEXAFS) experiments with a temporal resolution of about 230 ps are feasible. Pump-probe NEXAFS measurements were carried out in the "water-window" region (2.28 nm-4.36 nm) on the manganite Pr0.7Ca0.3MnO3, investigating diminutive changes of the oxygen K edge that derive from an optically induced phase transition. The results show the practicability of the table-top soft-x-ray spectrometer on demanding investigations so far exclusively conducted at synchrotron radiation sources.

  17. Development of a Time-resolved Soft X-ray Spectrometer for Laser Produced Plasma Experiments

    SciTech Connect

    Cone, K V; Dunn, J; Schneider, M B; Baldis, H A; Brown, G V; Emig, J; James, D L; May, M J; Park, J; Shepherd, R; Widmann, K

    2010-05-12

    A 2400 line/mm variable spaced grating spectrometer (VSG) has been used to measure soft x-ray emission (8-22 {angstrom}) from laser-produced plasma experiments at Lawrence Livermore National Laboratory's Compact Multipulse Terrawatt (COMET) Laser Facility. The spectrometer was coupled to a Kentech x-ray streak camera to study the temporal evolution of soft x-rays emitted from the back of mylar and copper foils irradiated at 10{sup 15} W/cm{sup 2}. The instrument demonstrated a resolving power of {approx} 120 at 19 {angstrom} with a time resolution of 31 ps. The time-resolved copper emission spectrum was consistent with a photodiode monitoring the laser temporal pulse shape and indicated that the soft x-ray emission follows the laser heating of the target. The time and spectral resolution of this diagnostic make it useful for studies of high temperature plasmas.

  18. Ultrastructural and elemental imaging of biological specimens by soft x-ray contact microscopy

    SciTech Connect

    Panessa, B.J.; Hoffman, P. . Dept. of Orthopedics); Warren, J.B. ); Feder, R.; Sayre, D. . Thomas J. Watson Research Center)

    1980-01-01

    Soft X-ray contact microscopy offers a means of visualizing unstained as well as stained biological materials at better than 6 nm resolution. Soft X-ray imaging depends on differential absorption of incident soft (1--10nm wavelength) X-rays by the endogenous elements within a specimen. The advantages of using soft X-rays for imaging are: (1) reduced specimen damage during exposure; (2) ability to image hydrated specimens at atmospheric pressure; (3) ability to image specimens ranging in thickness from less than 40 nm to as much as 10{mu}m; and (4) ability to map the elemental composition of the specimen through observation of the differential absorption of properly chosen incident x-ray wavelengths. This paper explains the principles of image formation and demonstrates the use of soft X-ray contact microscopy with biological samples which could not readily be imaged in their natural form using conventional electron microscopy methods. Data are also presented on the recognition of compositional features in histochemically treated articular joint tissues. 30 refs., 15 figs.

  19. Noninterferometric quantitative phase imaging with soft x rays.

    PubMed

    Allman, B E; McMahon, P J; Tiller, J B; Nugent, K A; Paganin, D; Barty, A

    2000-10-01

    We demonstrate quantitative noninterferometric x-ray phase-amplitude measurement. We present results from two experimental geometries. The first geometry uses x rays diverging from a point source to produce high-resolution holograms of submicrometer-sized objects. The measured phase of the projected image agrees with the geometrically determined phase to within +/-7%. The second geometry uses a direct imaging microscope setup that allows the formation of a magnified image with a zone-plate lens. Here a direct measure of the object phase is made and agrees with that of the magnified object to better than +/-10%. In both cases the accuracy of the phase is limited by the pixel resolution.

  20. The Columbia University proton-induced soft x-ray microbeam.

    PubMed

    Harken, Andrew D; Randers-Pehrson, Gerhard; Johnson, Gary W; Brenner, David J

    2011-09-15

    A soft x-ray microbeam using proton-induced x-ray emission (PIXE) of characteristic titanium (K(α) 4.5 keV) as the x-ray source has been developed at the Radiological Research Accelerator Facility (RARAF) at Columbia University. The proton beam is focused to a 120 μm × 50 μm spot on the titanium target using an electrostatic quadrupole quadruplet previously used for the charged particle microbeam studies at RARAF. The proton induced x-rays from this spot project a 50 μm round x-ray generation spot into the vertical direction. The x-rays are focused to a spot size of 5 μm in diameter using a Fresnel zone plate. The x-rays have an attenuation length of (1/e length of ~145 μm) allowing more consistent dose delivery across the depth of a single cell layer and penetration into tissue samples than previous ultra soft x-ray systems. The irradiation end station is based on our previous design to allow quick comparison to charged particle experiments and for mixed irradiation experiments.

  1. OSO-8 soft X-ray experiment (Wisconsin)

    NASA Technical Reports Server (NTRS)

    1975-01-01

    Information for operating and reducing data from the experiment which was designed to map low energy X-ray background emissions from 130 eV to 35 keV is presented. The detectors, counters, data system, and the gas system are discussed along with the functional operation of the subsystems. A command list indicating preconditions and resulting telemetry response for each command is included.

  2. Design considerations for soft X-ray television imaging detectors

    NASA Technical Reports Server (NTRS)

    Kalata, Kenneth; Golub, Leon

    1988-01-01

    Television sensors for X-rays can be coupled to converters and image intensifiers to obtain active areas, high flux capabilities, quantum efficiency, high time resolution, or ease of construction and operation that may not be obtained with a directly illuminated sensor. A general purpose system which makes use of these capabilities for a number of applications is decribed. Some of the performance characteristics of this type of system are examined, and the expected future developments for such systems are briefly addressed.

  3. Correlative Analysis of hard and Soft X-rays in Solar Flares using CGRO/BATSE and YOHKOH

    NASA Technical Reports Server (NTRS)

    Zarro, Dominic M.

    1996-01-01

    The objective of this work is to study different mechanisms of solar flare heating by comparing their predictions with simultaneous hard and soft X-ray observations. The datasets used in this work consist of hard X-ray observations from the Bragg Crystal Spectrometer (BCS) and Soft X-ray telescope (SXT) on the Japanese Yohkoh spacecraft.

  4. In-situ observations of catalytic surface reactions with soft x-rays under working conditions

    NASA Astrophysics Data System (ADS)

    Toyoshima, Ryo; Kondoh, Hiroshi

    2015-03-01

    Catalytic chemical reactions proceeding on solid surfaces are an important topic in fundamental science and industrial technologies such as energy conversion, pollution control and chemical synthesis. Complete understanding of the heterogeneous catalysis and improving its efficiency to an ultimate level are the eventual goals for many surface scientists. Soft x-ray is one of the prime probes to observe electronic and structural information of the target materials. Most studies in surface science using soft x-rays have been performed under ultra-high vacuum conditions due to the technical limitation, though the practical catalytic reactions proceed under ambient pressure conditions. However, recent developments of soft x-ray based techniques operating under ambient pressure conditions have opened a door to the in-situ observation of materials under realistic environments. The near-ambient-pressure x-ray photoelectron spectroscopy (NAP-XPS) using synchrotron radiation enables us to observe the chemical states of surfaces of condensed matters under the presence of gas(es) at elevated pressures, which has been hardly conducted with the conventional XPS technique. Furthermore, not only the NAP-XPS but also ambient-pressure compatible soft x-ray core-level spectroscopies, such as near-edge absorption fine structure (NEXAFS) and x-ray emission spectroscopy (XES), have been significantly contributing to the in-situ observations. In this review, first we introduce recent developments of in-situ observations using soft x-ray techniques and current status. Then we present recent new findings on catalytically active surfaces using soft x-ray techniques, particularly focusing on the NAP-XPS technique. Finally we give a perspective on the future direction of this emerging technique.

  5. SWIFT X-RAY OBSERVATIONS OF CLASSICAL NOVAE. II. THE SUPER SOFT SOURCE SAMPLE

    SciTech Connect

    Schwarz, Greg J.; Ness, Jan-Uwe; Osborne, J. P.; Page, K. L.; Evans, P. A.; Beardmore, A. P.; Walter, Frederick M.; Andrew Helton, L.; Woodward, Charles E.; Bode, Mike; Starrfield, Sumner; Drake, Jeremy J.

    2011-12-01

    The Swift gamma-ray burst satellite is an excellent facility for studying novae. Its rapid response time and sensitive X-ray detector provides an unparalleled opportunity to investigate the previously poorly sampled evolution of novae in the X-ray regime. This paper presents Swift observations of 52 Galactic/Magellanic Cloud novae. We included the X-Ray Telescope (0.3-10 keV) instrument count rates and the UltraViolet and Optical Telescope (1700-8000 A) filter photometry. Also included in the analysis are the publicly available pointed observations of 10 additional novae the X-ray archives. This is the largest X-ray sample of Galactic/Magellanic Cloud novae yet assembled and consists of 26 novae with Super Soft X-ray emission, 19 from Swift observations. The data set shows that the faster novae have an early hard X-ray phase that is usually missing in slower novae. The Super Soft X-ray phase occurs earlier and does not last as long in fast novae compared to slower novae. All the Swift novae with sufficient observations show that novae are highly variable with rapid variability and different periodicities. In the majority of cases, nuclear burning ceases less than three years after the outburst begins. Previous relationships, such as the nuclear burning duration versus t{sub 2} or the expansion velocity of the eject and nuclear burning duration versus the orbital period, are shown to be poorly correlated with the full sample indicating that additional factors beyond the white dwarf mass and binary separation play important roles in the evolution of a nova outburst. Finally, we confirm two optical phenomena that are correlated with strong, soft X-ray emission which can be used to further increase the efficiency of X-ray campaigns.

  6. Resonant inelastic scattering in dilute magnetic semiconductors by x-ray fluorescence spectroscopy

    SciTech Connect

    Lawniczak-Jablonska, K. |; Jia, J.J.; Underwood, J.H.

    1997-04-01

    As modern, technologically important materials have become more complex, element specific techniques have become invaluable in studying the electronic structure of individual components from the system. Soft x-ray fluorescence (SXF) and absorption (SXA) spectroscopies provide a unique means of measuring element and angular momentum density of electron states, respectively, for the valence and conducting bands in complex materials. X-ray absorption and the decay through x-ray emission are generally assumed to be two independent one-photon processes. Recent studies, however have demonstrated that SXF excited near the absorption threshold generate an array of spectral features that depend on nature of materials, particularly on the localization of excited states in s and d-band solids and that these two processes can no be longer treated as independent. Resonant SXF offers thus the new way to study the dynamics of the distribution of electronic valence states in the presence of a hole which is bound to the electron low lying in the conduction band. This process can simulate the interaction between hole-electron pair in wide gap semiconductors. Therefore such studies can help in understanding of transport and optics phenomena in the wide gap semiconductors. The authors report the result of Mn and S L-resonant emission in Zn{sub 1{minus}x}Mn{sub x}S (with x=0.2 and 0.3) and MnS as the energy of exciting radiation is tuned across the Mn and S L{sub 3,2} absorption edge, along with the resonant excited spectra from elemental Mn as a reference.

  7. Soft X-Ray Measurements of Z-Pinch-Driven Vacuum Hohlraums

    SciTech Connect

    Baker, K.L.; Porter, J.L.; Ruggles, L.E.; Chandler, G.A.; Deeney, Chris; Varas, M.; Moats, Ann; Struve, Ken; Torres, J.; McGurn, J.; Simpson, W.W.; Fehl, D.L.; Chrien, R.E.; Matuska, W.; Idzorek, G.C.

    1999-07-21

    This article reports the experimental characterization of a z-pinch driven-vacuum hohlraum. The authors have measured soft x-ray fluxes of 5 x 10{sup 12} W/cm{sup 2} radiating from the walls of hohlraums which are 2.4--2.5 cm in diameter by 1 cm tall. The x-ray source used to drive these hohlraums was a z-pinch consisting of a 300 wire tungsten array driven by a 2 MA, 100 ns current pulse. In this hohlraum geometry, the z-pinch x-ray source can produce energies in excess of 800 kJ and powers in excess of 100 TW to drive these hohlraums. The x-rays released in these hohlraums represent greater than a factor of 25 in energy and more than a factor of three in x-ray power over previous laboratory-driven hohlraums.

  8. Ultra-high-resolution inelastic X-ray scattering at high-repetition-rate self-seeded X-ray free-electron lasers.

    PubMed

    Chubar, Oleg; Geloni, Gianluca; Kocharyan, Vitali; Madsen, Anders; Saldin, Evgeni; Serkez, Svitozar; Shvyd'ko, Yuri; Sutter, John

    2016-03-01

    Inelastic X-ray scattering (IXS) is an important tool for studies of equilibrium dynamics in condensed matter. A new spectrometer recently proposed for ultra-high-resolution IXS (UHRIX) has achieved 0.6 meV and 0.25 nm(-1) spectral and momentum-transfer resolutions, respectively. However, further improvements down to 0.1 meV and 0.02 nm(-1) are required to close the gap in energy-momentum space between high- and low-frequency probes. It is shown that this goal can be achieved by further optimizing the X-ray optics and by increasing the spectral flux of the incident X-ray pulses. UHRIX performs best at energies from 5 to 10 keV, where a combination of self-seeding and undulator tapering at the SASE-2 beamline of the European XFEL promises up to a 100-fold increase in average spectral flux compared with nominal SASE pulses at saturation, or three orders of magnitude more than what is possible with storage-ring-based radiation sources. Wave-optics calculations show that about 7 × 10(12) photons s(-1) in a 90 µeV bandwidth can be achieved on the sample. This will provide unique new possibilities for dynamics studies by IXS. PMID:26917127

  9. Ultra-high-resolution inelastic X-ray scattering at high-repetition-rate self-seeded X-ray free-electron lasers.

    PubMed

    Chubar, Oleg; Geloni, Gianluca; Kocharyan, Vitali; Madsen, Anders; Saldin, Evgeni; Serkez, Svitozar; Shvyd'ko, Yuri; Sutter, John

    2016-03-01

    Inelastic X-ray scattering (IXS) is an important tool for studies of equilibrium dynamics in condensed matter. A new spectrometer recently proposed for ultra-high-resolution IXS (UHRIX) has achieved 0.6 meV and 0.25 nm(-1) spectral and momentum-transfer resolutions, respectively. However, further improvements down to 0.1 meV and 0.02 nm(-1) are required to close the gap in energy-momentum space between high- and low-frequency probes. It is shown that this goal can be achieved by further optimizing the X-ray optics and by increasing the spectral flux of the incident X-ray pulses. UHRIX performs best at energies from 5 to 10 keV, where a combination of self-seeding and undulator tapering at the SASE-2 beamline of the European XFEL promises up to a 100-fold increase in average spectral flux compared with nominal SASE pulses at saturation, or three orders of magnitude more than what is possible with storage-ring-based radiation sources. Wave-optics calculations show that about 7 × 10(12) photons s(-1) in a 90 µeV bandwidth can be achieved on the sample. This will provide unique new possibilities for dynamics studies by IXS.

  10. Ultra-high-resolution inelastic X-ray scattering at high-repetition-rate self-seeded X-ray free-electron lasers

    PubMed Central

    Chubar, Oleg; Geloni, Gianluca; Kocharyan, Vitali; Madsen, Anders; Saldin, Evgeni; Serkez, Svitozar; Shvyd’ko, Yuri; Sutter, John

    2016-01-01

    Inelastic X-ray scattering (IXS) is an important tool for studies of equilibrium dynamics in condensed matter. A new spectrometer recently proposed for ultra-high-resolution IXS (UHRIX) has achieved 0.6 meV and 0.25 nm−1 spectral and momentum-transfer resolutions, respectively. However, further improvements down to 0.1 meV and 0.02 nm−1 are required to close the gap in energy–momentum space between high- and low-frequency probes. It is shown that this goal can be achieved by further optimizing the X-ray optics and by increasing the spectral flux of the incident X-ray pulses. UHRIX performs best at energies from 5 to 10 keV, where a combination of self-seeding and undulator tapering at the SASE-2 beamline of the European XFEL promises up to a 100-fold increase in average spectral flux compared with nominal SASE pulses at saturation, or three orders of magnitude more than what is possible with storage-ring-based radiation sources. Wave-optics calculations show that about 7 × 1012 photons s−1 in a 90 µeV bandwidth can be achieved on the sample. This will provide unique new possibilities for dynamics studies by IXS. PMID:26917127

  11. Ultra-high-resolution inelastic X-ray scattering at high-repetition-rate self-seeded X-ray free-electron lasers

    DOE PAGES

    Chubar, Oleg; Geloni, Gianluca; Kocharyan, Vitali; Madsen, Anders; Saldin, Evgeni; Serkez, Svitozar; Shvyd'ko, Yuri; Sutter, John

    2016-02-12

    Inelastic X-ray scattering (IXS) is an important tool for studies of equilibrium dynamics in condensed matter. A new spectrometer recently proposed for ultra-high-resolution IXS (UHRIX) has achieved 0.6 meV and 0.25 nm₋1spectral and momentum-transfer resolutions, respectively. However, further improvements down to 0.1 meV and 0.02 nm₋1are required to close the gap in energy–momentum space between high- and low-frequency probes. It is shown that this goal can be achieved by further optimizing the X-ray optics and by increasing the spectral flux of the incident X-ray pulses. UHRIX performs best at energies from 5 to 10 keV, where a combination of self-seedingmore » and undulator tapering at the SASE-2 beamline of the European XFEL promises up to a 100-fold increase in average spectral flux compared with nominal SASE pulses at saturation, or three orders of magnitude more than what is possible with storage-ring-based radiation sources. Wave-optics calculations show that about 7 × 1012 photons s₋1in a 90 µeV bandwidth can be achieved on the sample. Ultimately, this will provide unique new possibilities for dynamics studies by IXS.« less

  12. Inelastic x-ray study of plasmons in oriented single and multi-walled carbon nanotubes.

    SciTech Connect

    Casa, D. M.; Upton, M. H.; Gog, T.; Misewich, J.; Hill, J.P.; Lowndes, D.; Eres, G.; BNL; ORNL

    2006-01-01

    Carbon nanotubes (CNT) have a wide variety of interesting properties and a large number of potential aplications in electronic and optical devices. In this study we concentrate on one important aspect of their electronic stucture: the plasmon dispersions in both single- and multi-wall CNTs and their relation to those in graphite. For the first time inelastic X-ray scattering is used to study these collective electronic excitations in oriented CNT samples. The experiments were performed on the IXS instrument at beamline 9ID CMC-XOR, APS, ANL. The incident energy was defined by a Si(333) monochromator, a spherically bent Ge(733) diced analyzer at the end of a 1-m arm focused the incident radiation onto a solid-state detector. The overall resolution was {approx}300 meV FWHM. The incident photons were linearly polarized perpendicular to the scattering plane. Energy loss scans were taken by varying the incident energy while keeping the exit energy fixed at 8.9805 keV. The momentum transfer was kept along the nanotubes axis. Spectra were taken at room temperature. The samples were oriented CNTs (both single- and multi-wall) grown on a Si substrate. The samples referred to as 'single-wall' were in fact a few walls at most (1-5) while the multi-walled ones had {approx}12 walls. Fig. 1. shows the inelastic spectra for the single-, multi-wall, and highly oriented pyrolithic graphite (HOPG) from top to bottom. Momentum transfer was Q = 0.79 {angstrom}{sup -1} in all cases, its direction was along the tubes for the first two samples or parallel to the sheets for graphite. The peaks at {approx}10 and {approx}30 eV are known as the {pi} and {sigma} + {pi} plasmons respectively. Fig. 2. shows the complete dispersion curves for both plasmon modes as a function of momentum transfer for all three samples.

  13. Atomic-scale roughness of Li metal surface evident in soft X-ray absorption spectroscopy

    NASA Astrophysics Data System (ADS)

    Prendergast, David; Wan, Liwen; Liang, Yufeng; Chuang, Yi-De; Qiao, Ruimin; Yan, Shishen; Yang, Wanli

    2015-03-01

    Realizing Li metal electrodes depends on fundamental understanding and efficient control of surface properties, which requires reliable characterization of the Li metal surface. Controlled experiments of Li K-edge soft X-ray absorption spectroscopy (XAS) reveal evidence of steady oxidation of the Li metal surface even under ultrahigh vacuum (UHV) conditions. The XAS of the short-lived Li metal surface, prepared by in-situ scratching, exhibits a prominent peak at 55.6 eV, more intense and at a slightly higher energy than the first peak expected for bulk Li metal at 55 eV. First-principles XAS calculations explain the origin of both the increased intensity and energy shift. This required the use of surface structural models with under-coordinated Li atoms and an estimated 4 Åinelastic mean-free-path for Auger electrons, implying extreme surface sensitivity of the measurements to the first 2-3 atomic layers. This work provides a benchmark on both experiment and theory for further studies of Li and other reactive metal surfaces, which are currently under scrutiny for next-generation energy storage devices. DP, LW, and YL acknowledge support from the Joint Center for Energy Storage Research, an Energy Innovation Hub funded by the US Dept. of Energy, Office of Science, Basic Energy Sciences.

  14. Soft x-ray laser experiments at Novette Laser Facility

    SciTech Connect

    Matthews, D.; Hagelstein, P.; Rosen, M.; Kauffman, R.; Lee, R.; Wang, C.; Medecki, H.; Campbell, M.; Ceglio, N.; Leipelt, G.

    1984-03-05

    We discuss the results of and future plans for experiments to study the possibility of producing an x-ray laser. The schemes we have investigated are all pumped by the Novette Laser, operated at short pulse (tau/sub L/ approx. 100 psec) and an incident wavelength of lambda /sub L/ approx. 0.53 ..mu..m. We have studied the possibility of lasing at 53.6, 68.0 to 72.0, 119.0, and 153.0 eV, using the inversion methods of resonant photo-excitation, collisional excitation, and three-body recombination.

  15. The soft X-ray excess in Einstein quasar spectra

    NASA Technical Reports Server (NTRS)

    Masnou, J. L.; Wilkes, B. J.; Elvis, M.; Mcdowell, J. C.; Arnaud, K. A.

    1992-01-01

    An SNR-limited subsample of 14 quasars from the Wilkes and Elvis (1987) sample is presently investigated for low-energy excess above a high-energy power law in the X-ray spectra obtained by the Einstein Imaging Proportional Counter. A significant excess that is 1-6 times as strong as the high-energy component at 0.2 keV is noted in eight of the 14 objects. In the case of 3C273, multiple observations show the excess to be variable.

  16. Chemical Contrast in Soft X-Ray Ptychography

    NASA Astrophysics Data System (ADS)

    Beckers, Mike; Senkbeil, Tobias; Gorniak, Thomas; Reese, Michael; Giewekemeyer, Klaus; Gleber, Sophie-Charlotte; Salditt, Tim; Rosenhahn, Axel

    2011-11-01

    The unique strengths of x-ray microscopy are high penetration depth and near-edge resonances that provide chemical information. We use ptychography, a coherent diffractive imaging technique that disposes of the requirement for isolated specimens, and demonstrate resonant imaging by exploiting resonances near the oxygen K edge to differentiate between two oxygen-containing materials. To highlight a biological system where resonant ptychography might be used for chemical mapping of unsliced cells, reconstructions of freeze-dried Deinococcus radiodurans cells at an energy of 517 eV are shown.

  17. Current research activities in the field of multilayer for EUV, soft x-ray and x-rays in IPOE

    NASA Astrophysics Data System (ADS)

    Wang, Zhanshan; Wang, Fengli; Zhang, Zhong; Wang, Hongchang; Wu, Wenjuan; Zhang, Shumin; Gu, Zhongxiang; Cheng, Xinbin; Wang, Bei; Qin, Shuji; Chen, Lingyan

    2006-01-01

    The present status of studies on EUV, soft x-ray and x-ray multilayer in the Institute of Precision Optical Engineering (IPOE) is briefly reviewed. With the aim of realizing a Mach-Zender interferometer working at 13.9nm, we have developed a semitransparent beam splitter with multilayer deposited on the back side of a silicon nitride membrane. On the basis of the experimental optical properties of the beam splitter, design has been performed to define the multilayer structure that provides the highest product of reflectivity and transmission. Optimized Mo/Si multilayer has been successfully deposited on the back side of a silicon nitride membrane by use of the magnetron sputtering. Measurements by means of a reflectometer in Beijing Synchrotron Radiation Facility at 13.9nm and at an angle of 7.2° provide a reflectivity of 20% and a transmission of 22%. Such a beam splitter has been used for X-ray Mach-Zender interferometer at 13.9nm. The broadband multilayer analyzer in the range between 12.4nm and 20nm is designed, and made which can deviate the Quasi-Brewster's angle several degree and show very high polarization. The main feature of our design approach is the use of an analytical solution as a starting point for direct computer search, and the desired results can be given in a reasonable time. The method can be applied in different spectral range for suitable material combination. Supermirrors with broad angular band working at different wavelength such as Cu Kα line are designed, manufactured and measured. The results show that the performance of the supermirrors is in agreement with designed data.

  18. Evaluating the quality of images produced by soft X-ray units.

    PubMed

    Bradley, D A; Wong, C S; Ng, K H

    2000-01-01

    For broad-beam soft X-ray sources, assessment of the quality of image produced by such units is made complex by the low penetration capabilities of the radiation. In the present study we have tested the utility of several types of test tool, some of which have been fabricated by us, as part of an effort to evaluate several key image defining parameters. These include the film characteristic, focal-spot size, image resolution and detail detectability. The two sources of X-rays used in present studies were the University of Malaya flash X-ray device (UMFX1) and a more conventional soft X-ray tube (Softex, Tokyo), the latter operating at peak accelerating potentials of 20 kVp. We have established, for thin objects, that both systems produce images of comparable quality and, in particular, objects can be resolved down to better than 45 microm. PMID:11003508

  19. Wide-field MAXI: soft x-ray transient monitor on the ISS

    NASA Astrophysics Data System (ADS)

    Kawai, Nobuyuki; Tomida, Hiroshi; Yatsu, Yoichi; Mihara, Tatehiro; Ueno, Shiro; Kimura, Masashi; Arimoto, Makoto; Serino, Motoko; Sakamoto, Takanori; Tsunemi, Hiroshi; Kohmura, Takayoshi; Negoro, Hitoshi; Ueda, Yoshihiro; Morii, Mikio; Tsuboi, Yoko; Ebisawa, Ken; Yoshida, Atsumasa

    2014-07-01

    WF-MAXI is a soft X-ray transient monitor proposed for the ISS/JEM. Unlike MAXI, it will always cover a large field of view (20 % of the entire sky) to detect short transients more efficiently. In addition to the various transient sources seen by MAXI, we hope to localize X-ray counterparts of gravitational wave events, expected to be directly detected by Advanced-LIGO, Virgo and KAGRA in late 2010's. The main instrument, the Soft X-ray Large Solid Angle Cameras (SLC) is sensitive in the 0.7-12 keV band with a localization accuracy of ~ 0:1°. The Hard X-ray Monitor (HXM) covers the same sky field in the 20 keV-1 MeV band.

  20. Interrelation of soft and hard X-ray emissions during solar flares. I - Observations

    NASA Technical Reports Server (NTRS)

    Winglee, R. M.; Kiplinger, A. L.; Zarro, D. M.; Dulk, G. A.; Lemen, J. R.

    1991-01-01

    The interrelation between the acceleration and heating of electrons and ions during impulsive solar flares is determined on the basis of simulataneous observations of hard and soft X-ray emission from the Solar Maximum Mission at high time resolution (6 s). For all the flares, the hard X-rays are found to have a power-law spectrum which breaks down during the rise phase and beginning of the decay phase. After that, the spectrum changes to either a single power law or a power law that breaks up at high energies. The characteristics of the soft X-ray are found to depend on the flare position. It is suggested that small-scale quasi-static electric fields are important for determining the acceleration of the X-ray-producing electrons and the outflowing chromospheric ions.

  1. Soft x-ray imager (SXI) onboard ASTRO-H

    NASA Astrophysics Data System (ADS)

    Tsunemi, Hiroshi; Hayashida, Kiyoshi; Tsuru, Takeshi Go; Dotani, Tadayasu; Hiraga, Junko S.; Anabuki, Naohisa; Bamba, Aya; Hatsukade, Isamu; Kohmura, Takayoshi; Mori, Koji; Murakami, Hiroshi; Nakajima, Hiroshi; Ozaki, Masanobu; Uchida, Hiroyuki; Yamauchi, Makoto

    2010-07-01

    We are designing an X-ray CCD camera (SXI) for ASTRO-H, including many new items. We have developed the CCD, CCD-NeXT4, that is a P-channel type CCD. It has a thick depletion layer of 200μm with an imaging area of 30mm square. Since it is back-illuminated, it has a good low energy response and is robust against the impact of micro-meteorites. We will employ 4 chips to cover the area of 60mm square. A mechanical rather than peltier cooler will be employed so that we can cool the CCD to -120°C. We will also introduce an analog ASIC that is placed very close to the CCD. It performs well, having a similar noise level to that assembled by using individual parts used on SUZAKU. We also employ a modulated X-ray source (MXS), that improves the accuracy of the calibration. The SXI will have one of the largest SΩ among various satellites.

  2. Development of near atomically perfect diffraction gratings for EUV and soft x-rays with very high efficiency and resolving power

    NASA Astrophysics Data System (ADS)

    Voronov, D. L.; Anderson, E. H.; Cambie, R.; Gawlitza, P.; Goray, L. I.; Gullikson, E. M.; Salmassi, F.; Warwick, T.; Yashchuk, V. V.; Padmore, H. A.

    2013-03-01

    Multilayer-coated Blazed Gratings (MBG) can offer high diffraction efficiency in a very high diffraction order and are therefore of great interest for high-resolution EUV and soft x-ray spectroscopy techniques such as Resonance Inelastic X-ray Scattering. However, realization of the MBG concept requires nano-scale precision in fabrication of a saw-tooth substrate with atomically smooth facets, and reproduction of the blazed groove profile in the course of conformal growth of a multilayer coating. We report on recent progress achieved in the development, fabrication, and characterization of ultra-dense MBGs for EUV and soft x-rays. As a result of thorough optimization of all steps of the fabrication process, an absolute diffraction efficiency as high as 44% and 12.7% was achieved for a 5250 l/mm grating in the EUV and soft x-ray regions respectively. This work now shows a direct route to achieving high diffraction efficiency in high order at wavelengths throughout the soft x-ray energy range with revolutionary applications in synchrotron science.

  3. Time-resolved Soft X-Ray Imaging (SXRI) diagnostic for use at the NIF and OMEGA lasers (version 2)

    SciTech Connect

    Schneider, M B; Holder, J P; James, D L; Bruns, H C; Celeste, J R; Compton, S; Costa, R L; Ellis, A D; Emig, J A; Hargrove, D; Kalantar, D H; MacGowan, B J; Power, G D; Sorce, C; Rekow, V; Widmann, K; Young, B K; Young, P E; Garcia, O F; McKenney, J; Haugh, M; Goldin, F; MacNeil, L P; Cone, K

    2006-07-21

    The soft x-ray imager (SXRI) built for the first experiments at the National Ignition Facility (NIF) has four soft x-ray channels and one hard x-ray channel. The SXRI is a snout that mounts to a four strip gated imager. This produces four soft x-ray images per strip, which can be separated in time by {approx}60psec. Each soft x-ray channel consists of a mirror plus a filter. The diagnostic was used to study x-ray burnthrough of hot hohlraum targets at the NIF and OMEGA lasers. The SXRI snout design and issues involved in selecting the desired soft x-ray channels are discussed.

  4. Dynamics of confined water reconstructed from inelastic x-ray scattering measurements of bulk response functions

    NASA Astrophysics Data System (ADS)

    Coridan, Robert H.; Schmidt, Nathan W.; Lai, Ghee Hwee; Abbamonte, Peter; Wong, Gerard C. L.

    2012-03-01

    Nanoconfined water and surface-structured water impacts a broad range of fields. For water confined between hydrophilic surfaces, measurements and simulations have shown conflicting results ranging from “liquidlike” to “solidlike” behavior, from bulklike water viscosity to viscosity orders of magnitude higher. Here, we investigate how a homogeneous fluid behaves under nanoconfinement using its bulk response function: The Green's function of water extracted from a library of S(q,ω) inelastic x-ray scattering data is used to make femtosecond movies of nanoconfined water. Between two confining surfaces, the structure undergoes drastic changes as a function of surface separation. For surface separations of ≈9 Å, although the surface-associated hydration layers are highly deformed, they are separated by a layer of bulklike water. For separations of ≈6 Å, the two surface-associated hydration layers are forced to reconstruct into a single layer that modulates between localized “frozen’ and delocalized “melted” structures due to interference of density fields. These results potentially reconcile recent conflicting experiments. Importantly, we find a different delocalized wetting regime for nanoconfined water between surfaces with high spatial frequency charge densities, where water is organized into delocalized hydration layers instead of localized hydration shells, and are strongly resistant to `freezing' down to molecular distances (<6 Å).

  5. Inelastic x-ray scattering of dense solid oxygen: Evidence for intermolecular bonding

    SciTech Connect

    Meng, Yue; Eng, Peter J.; Tse, John S.; Shaw, Dawn M.; Hu, Michael Y.; Shu, Jinfu; Gramsch, Stephen A.; Kao, Chichang; Hemley, Russell J.; Mao, Ho-kwang

    2008-08-14

    The detailing of the intermolecular interactions in dense solid oxygen is essential for an understanding of the rich polymorphism and remarkable properties of this element at high pressure. Synchrotron inelastic x-ray scattering measurements of oxygen K-edge excitations to 38 GPa reveal changes in electronic structure and bonding on compression of the molecular solid. The measurements show that O{sub 2} molecules interact predominantly through the half-filled 1{pi}{sub g}* orbital <10 GPa. Enhanced intermolecular interactions develop because of increasing overlap of the 1{pi}{sub g}* orbital in the low-pressure phases, leading to electron delocalization and ultimately intermolecular bonding between O{sub 2} molecules at the transition to the {epsilon}-phase. The {epsilon}-phase, which consists of (O{sub 2}){sub 4} clusters, displays the bonding characteristics of a closed-shell system. Increasing interactions between (O{sub 2}){sub 4} clusters develop upon compression of the {epsilon}-phase, and provide a potential mechanism for intercluster bonding in still higher-pressure phases.

  6. Resonant inelastic x-ray scattering as a band structure probe of high-temperature superconductors

    NASA Astrophysics Data System (ADS)

    Kanasz-Nagy, Marton; Shi, Yifei; Klich, Israel; Demler, Eugene

    I will analyze recent resonant inelastic x-ray scattering (RIXS) experimental data on YBa2Cu3O6 + x [Minola et al., Phys. Rev. Lett. 114, 217003 (2015)] within quasi-particle theory. This measurement has been performed with the incoming photon energy detuned at several values from the resonance maximum, and, surprisingly, the data shows much weaker dependence on detuning than expected from recent measurements on a different cuprate superconductor, Bi2Sr2CuO6 + x [Guarise et al., Nat. Commun. 5, 5760 (2014)]. I will demonstrate, that this discrepancy, originally attributed to collective magnetic excitations, can be understood in terms of the differences between the band structures of these materials. We found good agreement between theory and experiment over a large range of dopings [M. Kanasz-Nagy et al., arXiv:1508.06639]. Moreover, I will demonstrate that the RIXS signal depends sensitively on excitations at energies well above the Fermi surface, that are inaccessible to traditionally used band structure probes, such as angle-resolved photoemission spectroscopy. This makes RIXS a powerful probe of band structure, not suffering from surface preparation problems and small sample sizes, making it potentially applicable to a wide range of materials. The work of M. K.-N. was supported by the Harvard-MIT CUA, NSF Grant No. DMR-1308435, AFOSR Quantum Simulation MURI, the ARO-MURI on Atomtronics, and ARO MURI Quism program.

  7. Nuclear resonant inelastic x-ray scattering: Methodology and extraction of vibrational properties of minerals

    NASA Astrophysics Data System (ADS)

    Hu, M. Y.; Alp, E. E.; Bi, W.; Sturhahn, W.; Toellner, T. S.; Zhao, J.

    2013-12-01

    Nuclear resonant inelastic x-ray scattering (NRIXS) is a synchrotron radiation based experimental method [1]. Since its introduction almost 20 years ago [2], NRIXS has found an expanding range of applications of studying lattice dynamics in condensed matter physics, materials science, high-pressure research, geosciences, and biophysics. After the first high pressure application in geophysics of measuring sound velocity of iron up to 153 GPa [3], it has become a widely used method to investigate deep earth compositions through sound velocity measurements [4,5]. Thermodynamic properties are also explored, in particular Grueneisen parameters [6]. Later, it was realized that isotope fractionaton factors can be derived from NRIXS measurements [7,8]. Sum rules and moments of NRIXS is a critical part of this methodology [9,10]. We will discuss this and in general the data analysis of NRIXS which enables the above mentioned applications. [1] Alp et al. Hyperfine Interactions 144/145, 3 (2002) [2] Sturhahn et al., PRL 74, 3832 (1995) [3] Mao et al., Science 292, 914 (2001) [4] Hu et al., PRB 67, 094304 (2003) [5] Sturhahn & Jackson, GSA special paper 421 (2007) [6] Murphy et al., Geophys. Res. Lett. 38, L24306 (2011) [7] Polyakov, Science 323, 912 (2009) [8] Dauphas et al., Geochimica et Cosmochimica Acta 94, 254 (2012) [9] Lipkin, PRB 52, 10073 (1995) [10] Hu et al., PRB 87, 064301 (2013)

  8. A new method to derive electronegativity from resonant inelastic x-ray scattering

    SciTech Connect

    Carniato, S.; Journel, L.; Guillemin, R.; Piancastelli, M. N.; Simon, M.; Stolte, W. C.; Lindle, D. W.

    2012-10-14

    Electronegativity is a well-known property of atoms and substituent groups. Because there is no direct way to measure it, establishing a useful scale for electronegativity often entails correlating it to another chemical parameter; a wide variety of methods have been proposed over the past 80 years to do just that. This work reports a new approach that connects electronegativity to a spectroscopic parameter derived from resonant inelastic x-ray scattering. The new method is demonstrated using a series of chlorine-containing compounds, focusing on the Cl 2p{sup -1}LUMO{sup 1} electronic states reached after Cl 1s{yields} LUMO core excitation and subsequent KL radiative decay. Based on an electron-density analysis of the LUMOs, the relative weights of the Cl 2p{sub z} atomic orbital contributing to the Cl 2p{sub 3/2} molecular spin-orbit components are shown to yield a linear electronegativity scale consistent with previous approaches.

  9. Structural and dynamical properties of chlorinated hydrocarbons studied with resonant inelastic x-ray scattering

    NASA Astrophysics Data System (ADS)

    Bohinc, R.; Žitnik, M.; Bučar, K.; Kavčič, M.; Carniato, S.; Journel, L.; Guillemin, R.; Marchenko, T.; Kawerk, E.; Simon, M.; Cao, W.

    2016-04-01

    We present a theoretical and experimental study of resonant inelastic x-ray scattering on a large group of chlorinated hydrocarbons: CH3Cl, CH2Cl2, CHCl3, CCl4, CH3CH2Cl, ClCH2CH2Cl, CH3CHCl2, CH3CCl3, C2H2Cl2-iso, C2H2Cl2-cis, C2H2Cl2-trans, and C6H5Cl. Differences in structural and dynamical properties of the molecules generated by diverse chemical environments are observed in the measured Cl(Kα) spectral maps as well as in the Cl(K) total fluorescence yield spectra. The energy position, relative intensity, and the width of the Franck-Condon distribution of low-lying σ∗ and π∗ resonances are extracted by a fitting procedure taking into account the experimental broadening. The theoretical values obtained with the transition potential and Δ Kohn-Sham methods are in good agreement with the experimental parameters indicating subtle differences due to variations in the molecular structure.

  10. Nuclear resonant inelastic X-ray scattering at high pressure and low temperature

    SciTech Connect

    Bi, Wenli; Zhao, Jiyong; Lin, Jung -Fu; Jia, Quanjie; Hu, Michael Y.; Jin, Changqing; Ferry, Richard; Yang, Wenge; Struzhkin, Viktor; Alp, E. Ercan

    2015-01-01

    In this study, a new synchrotron radiation experimental capability of coupling nuclear resonant inelastic X-ray scattering with the cryogenically cooled high-pressure diamond anvil cell technique is presented. The new technique permits measurements of phonon density of states at low temperature and high pressure simultaneously, and can be applied to studies of phonon contribution to pressure- and temperature-induced magnetic, superconducting and metal–insulator transitions in resonant isotope-bearing materials. In this report, a pnictide sample, EuFe2As2, is used as an example to demonstrate this new capability at beamline 3-ID of the Advanced Photon Source, Argonne National Laboratory. A detailed description of the technical development is given. The Fe-specific phonon density of states and magnetism from the Fe sublattice in Eu57Fe2As2 at high pressure and low temperature were derived by using this new capability.

  11. Raman and fluorescence characteristics of resonant inelastic X-ray scattering from doped superconducting cuprates

    DOE PAGES

    Huang, H. Y.; Jia, C. J.; Chen, Z. Y.; Wohlfeld, K.; Moritz, B.; Devereaux, T. P.; Wu, W. B.; Okamoto, J.; Lee, W. S.; Hashimoto, M.; et al

    2016-01-22

    Measurements of spin excitations are essential for an understanding of spin-mediated pairing for superconductivity; and resonant inelastic X-ray scattering (RIXS) provides a considerable opportunity to probe high-energy spin excitations. However, whether RIXS correctly measures the collective spin excitations of doped superconducting cuprates remains under debate. Here we demonstrate distinct Raman- and fluorescence-like RIXS excitations of Bi1.5Pb0.6Sr1.54CaCu2O8+δ. Combining photon-energy and momentum dependent RIXS measurements with theoretical calculations using exact diagonalization provides conclusive evidence that the Raman-like RIXS excitations correspond to collective spin excitations, which are magnons in the undoped Mott insulators and evolve into paramagnons in doped superconducting compounds. In contrast,more » the fluorescence-like shifts are due primarily to the continuum of particle-hole excitations in the charge channel. Our results show that under the proper experimental conditions RIXS indeed can be used to probe paramagnons in doped high-Tc cuprate superconductors.« less

  12. Signatures of strong correlation effects in resonant inelastic x-ray scattering studies on cuprates

    NASA Astrophysics Data System (ADS)

    Li, Wan-Ju; Lin, Cheng-Ju; Lee, Ting-Kuo

    2016-08-01

    Recently, spin excitations in doped cuprates have been measured using resonant inelastic x-ray scattering. The paramagnon dispersions show the large hardening effect in the electron-doped systems and seemingly doping independence in the hole-doped systems, with the energy scales comparable to that of the antiferromagnetic (AFM) magnons. This anomalous hardening effect and the lack of softening were partially explained by using the strong-coupling t -J model but with a three-site term [Nat. Commun. 5, 3314 (2014), 10.1038/ncomms4314], although the hardening effect is already present even without the latter. By considering the t -t'-t''-J model and using the slave-boson mean-field theory, we obtain, via the spin-spin susceptibility, the spin excitations in qualitative agreement with the experiments. The doping-dependent bandwidth due to the strong correlation physics is the origin of the hardening effect. We also show that dispersions in the AFM regime, different from those in the paramagnetic (PM) regime, hardly vary with dopant density. These excitations are mainly collective in nature instead of particle-hole-like. We further discuss the interplay and different contributions of these two kinds of excitations in the PM phase and show that the dominance of the collective excitation increases with decreasing dopant concentrations.

  13. Collective dynamics of hydrated β-lactoglobulin by inelastic x-ray scattering.

    PubMed

    Yoshida, Koji; Hosokawa, Shinya; Baron, Alfred Q R; Yamaguchi, Toshio

    2010-10-01

    Inelastic x-ray scattering measurements of hydrated β-lactoglobulin (β-lg) were performed to investigate the collective dynamics of hydration water and hydrated protein on a picosecond time scale. Samples with different hydration levels h [=mass of water (g)/mass of protein (g)] of 0 (dry), 0.5, and 1.0 were measured at ambient temperature. The observed dynamical structure factor S(Q,ω)/S(Q) was analyzed by a model composed of a Lorentzian for the central peak and a damped harmonic oscillator (DHO) for the side peak. The dispersion relation between the excitation energy in the DHO model and the momentum transfer Q was obtained for the hydrated β-lg at both hydration levels, but no DHO excitation was found for the dry β-lg. The high-frequency sound velocity was similar to that previously observed in pure water. The ratio of the high-frequency sound velocity of hydrated β-lg to the adiabatic one of hydrated lysozyme (h=0.41) was estimated as ∼1.6 for h=0.5. The value is significantly smaller than that (∼2) of pure water that has the tetrahedral network structure. The present finding thus suggests that the tetrahedral network structure of water around the β-lg is partially disrupted by the perturbation from protein surface. These results are consistent with those reported from Brillouin neutron spectroscopy and molecular dynamics simulation studies of hydrated ribonuclease A. PMID:20942540

  14. Stelllar wind induced soft X-ray emission from close-in exoplanets

    NASA Astrophysics Data System (ADS)

    Kislyakova, Kristina; Fossati, Luca; Johnstone, Colin P.; Holmström, Mats; Zaitsev, Valery V.; Lammer, Helmut

    2016-04-01

    We estimate the X-ray emission from close-in exoplanets. We show that the Solar/Stellar Wind Charge Exchange Mechanism (SWCX) which produces soft X-ray radiation is very effective for hot Jupiters. In this mechanism, X-ray photons are produces by charge exchange between heavy ions in the solar wind and the atmospheric neutral particles. This mechanism is know to generate X-ray emission of comets in the Solar system. It has also been shown to operate in the heliosphere, in the terrestrial magnetosheath, and on Mars, Venus and Moon. Since the number of emitted photons is proportional to the solar wind mass flux, this mechanism is not effective for the Solar system giants. We present a simple estimate of the X-ray emission intensity that can be produced by close-in extrasolar Hot Jupiters due to charge exchange with the heavy ions of the stellar wind. Using the example of HD 209458b, we show that this mechanism alone can be responsible for an X-ray emission of ≈ 1022 erg s-1, which is 106 times stronger than the emission from the Jovian aurora. We discuss the possibility to observe the predicted soft X-ray flux of hot Jupiters and show that despite high emission intensities they are unobservable with current facilities.

  15. STELLAR WIND INDUCED SOFT X-RAY EMISSION FROM CLOSE-IN EXOPLANETS

    SciTech Connect

    Kislyakova, K. G.; Lammer, H.; Fossati, L.; Johnstone, C. P.; Holmström, M.; Zaitsev, V. V.

    2015-01-30

    In this Letter, we estimate the X-ray emission from close-in exoplanets. We show that the Solar/Stellar Wind Charge Exchange Mechanism (SWCX), which produces soft X-ray emission, is very effective for hot Jupiters. In this mechanism, X-ray photons are emitted as a result of the charge exchange between heavy ions in the solar wind and the atmospheric neutral particles. In the solar system, comets produce X-rays mostly through the SWCX mechanism, but it has also been shown to operate in the heliosphere, in the terrestrial magnetosheath, and on Mars, Venus, and the Moon. Since the number of emitted photons is proportional to the solar wind mass flux, this mechanism is not very effective for the solar system giants. Here we present a simple estimate of the X-ray emission intensity that can be produced by close-in extrasolar giant planets due to charge exchange with the heavy ions of the stellar wind. Using the example of HD 209458b, we show that this mechanism alone can be responsible for an X-ray emission of ≈10{sup 22} erg s{sup –1}, which is 10{sup 6} times stronger than the emission from the Jovian aurora. We discuss also the possibility of observing the predicted soft X-ray flux of hot Jupiters and show that despite high emission intensities they are unobservable with current facilities.

  16. Stelllar wind induced soft X-ray emission from close-in exoplanets

    NASA Astrophysics Data System (ADS)

    Kislyakova, Kristina; Fossati, Luca; Johnstone, Colin P.; Holmström, Mats; Zaitsev, Valery V.; Lammer, Helmut

    2016-04-01

    We estimate the X-ray emission from close-in exoplanets. We show that the Solar/Stellar Wind Charge Exchange Mechanism (SWCX) which produces soft X-ray radiation is very effective for hot Jupiters. In this mechanism, X-ray photons are produces by charge exchange between heavy ions in the solar wind and the atmospheric neutral particles. This mechanism is know to generate X-ray emission of comets in the Solar system. It has also been shown to operate in the heliosphere, in the terrestrial magnetosheath, and on Mars, Venus and Moon. Since the number of emitted photons is proportional to the solar wind mass flux, this mechanism is not effective for the Solar system giants. We present a simple estimate of the X-ray emission intensity that can be produced by close-in extrasolar Hot Jupiters due to charge exchange with the heavy ions of the stellar wind. Using the example of HD 209458b, we show that this mechanism alone can be responsible for an X-ray emission of ≈ 1022 erg s‑1, which is 106 times stronger than the emission from the Jovian aurora. We discuss the possibility to observe the predicted soft X-ray flux of hot Jupiters and show that despite high emission intensities they are unobservable with current facilities.

  17. The soft x-ray instrument for materials studies at the linac coherent light source x-ray free-electron laser

    SciTech Connect

    Schlotter, W. F.; Turner, J. J.; Rowen, M.; Holmes, M.; Messerschmidt, M.; Moeller, S.; Krzywinski, J.; Lee, S.; Coffee, R.; Hays, G.; Heimann, P.; Krupin, O.; Soufli, R.; Fernandez-Perea, M.; Hau-Riege, S.; Kelez, N.; Beye, M.; Gerken, N.; Sorgenfrei, F.; Wurth, W.; and others

    2012-04-15

    The soft x-ray materials science instrument is the second operational beamline at the linac coherent light source x-ray free electron laser. The instrument operates with a photon energy range of 480-2000 eV and features a grating monochromator as well as bendable refocusing mirrors. A broad range of experimental stations may be installed to study diverse scientific topics such as: ultrafast chemistry, surface science, highly correlated electron systems, matter under extreme conditions, and laboratory astrophysics. Preliminary commissioning results are presented including the first soft x-ray single-shot energy spectrum from a free electron laser.

  18. Calibration of a high resolution grating soft x-ray spectrometer

    SciTech Connect

    Magee, E. W.; Dunn, J.; Brown, G. V.; Beiersdorfer, P.; Cone, K. V.; Park, J.; Porter, F. S.; Kilbourne, C. A.; Kelley, R. L.

    2010-10-15

    The calibration of the soft x-ray spectral response of a large radius of curvature, high resolution grating spectrometer (HRGS) with a back-illuminated charge-coupled device detector is reported. The instrument is cross-calibrated for the 10-50 A waveband at the Lawrence Livermore National Laboratory electron beam ion trap (EBIT) x-ray source with the EBIT calorimeter spectrometer. The HRGS instrument is designed for laser-produced plasma experiments and is important for making high dynamic range measurements of line intensities, line shapes, and x-ray sources.

  19. Calibration of a high resolution grating soft x-ray spectrometer.

    PubMed

    Magee, E W; Dunn, J; Brown, G V; Cone, K V; Park, J; Porter, F S; Kilbourne, C A; Kelley, R L; Beiersdorfer, P

    2010-10-01

    The calibration of the soft x-ray spectral response of a large radius of curvature, high resolution grating spectrometer (HRGS) with a back-illuminated charge-coupled device detector is reported. The instrument is cross-calibrated for the 10-50 Å waveband at the Lawrence Livermore National Laboratory electron beam ion trap (EBIT) x-ray source with the EBIT calorimeter spectrometer. The HRGS instrument is designed for laser-produced plasma experiments and is important for making high dynamic range measurements of line intensities, line shapes, and x-ray sources. PMID:21034013

  20. Ultra soft X-ray Microbeam: optical analysis and intensity measurements

    NASA Astrophysics Data System (ADS)

    Emilio, M. Di Paolo; Palladino, L.; Del Grande, F.

    2016-06-01

    In this work, optical analysis and intensity measurements of the Ultra Soft x-ray microbeam (100 eV–1 keV) are presented. X-ray emission at 500 eV are generated from a plasma produced by focusing Nd-YAG laser beam on the Yttrium target. In particular, we will report the study of x-ray intensity and the measurement of focal spot dimension. Moreover, the software/hardware control of sample holder position and the alignment of biological sample to the microbeam will be described.

  1. Imaging of lateral spin valves with soft x-ray microscopy

    SciTech Connect

    Mosendz, O.; Mihajlovic, G.; Pearson, J. E.; Fischer, P.; Im, M.-Y.; Bader, S. D.; Hoffmann, A.

    2009-05-01

    We investigated Co/Cu lateral spin valves by means of high-resolution transmission soft x-ray microscopy with magnetic contrast that utilizes x-ray magnetic circular dichroism (XMCD). No magnetic XMCD contrast was observed at the Cu L{sub 3} absorption edge, which should directly image the spin accumulation in Cu. Although electrical transport measurements in a non-local geometry clearly detected the spin accumulation in Cu, which remained unchanged during illumination with circular polarized x-rays at the Co and Cu L{sub 3} absorption edges.

  2. A Sealed, UHV Compatible, Soft X-ray Detector Utilizing Gas Electron Multipliers

    SciTech Connect

    Schaknowski, N.A.; Smith, G.

    2009-10-25

    An advanced soft X-ray detector has been designed and fabricated for use in synchrotron experiments that utilize X-ray absorption spectroscopy in the study a wide range of materials properties. Fluorescence X-rays, in particular C{sub K} at 277eV, are converted in a low pressure gas medium, and charge multiplication occurs in two gas electron multipliers, fabricated in-house from glass reinforced laminate, to enable single photon counting. The detector satisfies a number of demanding characteristics often required in synchrotron environments, such as UHV compatibility compactness, long-term stability, and energy resolving capability.

  3. Anti-contamination device for cryogenic soft X-ray diffraction microscopy

    DOE PAGES

    Huang, Xiaojing; Miao, Huijie; Nelson, Johanna; Turner, Joshua; Steinbrener, Jan; Shapiro, David; Kirz, Janos; Jacobsen, Chris

    2011-05-01

    Cryogenic microscopy allows one to view frozen hydrated biological and soft matter specimens with good structural preservation and a high degree of stability against radiation damage. We describe a liquid nitrogen-cooled anti-contamination device for cryogenic X-ray diffraction microscopy. The anti-contaminator greatly reduces the buildup of ice layers on the specimen due to condensation of residual water vapor in the experimental vacuum chamber. We show by coherent X-ray diffraction measurements that this leads to fivefold reduction of background scattering, which is important for far-field X-ray diffraction microscopy of biological specimens.

  4. Omega Dante Soft X-Ray Power Diagnostic Component Calibration at the National Synchrotron Light Source

    SciTech Connect

    Campbell, K; Weber, F; Dewald, E; Glenzer, S; Landen, O; Turner, R; Waide, P

    2004-04-15

    The Dante soft x-ray spectrometer installed on the Omega laser facility at the Laboratory for Laser Energetics, University of Rochester is a twelve-channel filter-edge defined x-ray power diagnostic. It is used to measure the absolute flux from direct drive, indirect drive (hohlraums) and other plasma sources. Calibration efforts using two beam lines, U3C (50eV-1keV) and X8A (1keV-6keV) at the National Synchrotron Light Source (NSLS) have been implemented to insure the accuracy of these measurements. We have calibrated vacuum x-ray diodes, mirrors and filters.

  5. X-ray dense cellular inclusions in the cells of the green alga Chlamydomonas reinhardtii as seen by soft-x-ray microscopy

    SciTech Connect

    Stead, A.D.; Ford, T.W.; Page, A.M.; Brown, J.T.; Meyer-Ilse, W.

    1997-04-01

    Soft x-rays, having a greater ability to penetrate biological material than electrons, have the potential for producing images of intact, living cells. In addition, by using the so-called {open_quotes}water window{close_quotes} area of the soft x-ray spectrum, a degree of natural contrast is introduced into the image due to differential absorption of the wavelengths by compounds with a high carbon content compared to those with a greater oxygen content. The variation in carbon concentration throughout a cell therefore generates an image which is dependent upon the carbon density within the specimen. Using soft x-ray contact microscopy the authors have previously examined the green alga Chlamydomonas reinhardtii, and the most prominent feature of the cells are the numerous x-ray absorbing spheres, But they were not seen by conventional transmission electron microscopy. Similar structures have also been reported by the Goettingen group using their cryo transmission x-ray microscope at BESSY. Despite the fact that these spheres appear to occupy up to 20% or more of the cell volume when seen by x-ray microscopy, they are not visible by transmission electron microscopy. Given the difficulties and criticisms associated with soft x-ray contact microscopy, the present study was aimed at confirming the existence of these cellular inclusions and learning more of their possible chemical composition.

  6. Emission Line Spectra in the Soft X-ray Region 20 - 75 Angstroms

    NASA Technical Reports Server (NTRS)

    Lepson, J. K.; Beiersdorfer, P.; Chen, H.; Behar, E.; Kahn, S. M.

    2002-01-01

    As part of a project to complete a comprehensive catalogue of astrophysically relevant emission lines in support of new-generation X-ray observatories using the Lawrence Livermore electron beam ion traps EBIT-I and EDIT-II, emission lines of argon and sulfur in the soft X-ray and extreme ultraviolet region were studied. Observations of Ar IX through Ar XVI and S VII through S XIV between 20 and 75 Angstrom are presented to illustrate our work.

  7. The Soft X-ray research instrument at the Linac Coherent Light Source

    DOE PAGES

    Dakovski, Georgi L.; Heimann, Philip; Holmes, Michael; Krupin, Oleg; European XFEL, Hamburg; Minitti, Michael P.; Mitra, Ankush; Moeller, Stefan; Rowen, Michael; Schlotter, William F.; et al

    2015-04-02

    The Soft X-ray Research instrument provides intense ultrashort X-ray pulses in the energy range 280–2000 eV. A diverse set of experimental stations may be installed to investigate a broad range of scientific topics such as ultrafast chemistry, highly correlated materials, magnetism, surface science, and matter under extreme conditions. A brief description of the main instrument components will be given, followed by some selected scientific highlights.

  8. Soft X-ray imaging techniques for calculating the Earth's dayside boundaries

    NASA Astrophysics Data System (ADS)

    Connor, Hyunju; Kuntz, Kip; Sibeck, David; Collier, Michael; Aryan, Homayon; Branduardi-Raymont, Graziella; Collado-Vega, Yaireska; Porter, Frederick; Purucker, Michael; Snowden, Steven; Raeder, Joachim; Thomas, Nicholas; Walsh, Brian

    2016-04-01

    Charged particles and neutral atoms exchange electrons in many space plasma venues. Soft X-rays are emitted when highly charged solar wind ions, such as C6+. O7+, and Fe13+, interact with Hydrogen and Helium atoms. Soft X-ray images can be a powerful technique to remotely probe the plasma and neutral density structures created when the solar wind interacts with planetary exospheres, such as those at the Earth, Moon, Mars, Venus, and comets. The recently selected ESA-China joint spacecraft mission, "Solar wind - Magnetosphere - Ionosphere Link Explorer (SMILE)" will have a soft X-ray imager on board and provide pictures of the Earth's dayside system after its launch in 2021. In preparation for this future mission, we simulate soft X-ray images of the Earth's dayside system, using the OpenGGCM global magnetosphere MHD model and the Hodges model of the Earth's exosphere. Then, we discuss techniques to determine the location of the Earth's dayside boundaries (bow shock and magnetopause) from the soft X-ray images.

  9. Laser Plasma Soft X-Ray Contact Microscopy of Polymer Composites

    NASA Astrophysics Data System (ADS)

    Azuma, Hirozumi; Takeichi, Akihiro; Noda, Shoji

    1994-08-01

    Microstructures of polymer composites are observed with a good contrast and with a submicron spatial resolution by contact soft X-ray microscopy with a laser plasma as a soft X-ray source. An iron target was irradiated by a YAG laser ( 2ω=532 nm, 0.4 J) at laser power density of 2.5×1012 W/cm2 and the emitted soft X-rays were filtered with a thin aluminum foil. For a 0.1-µ m-thick poly acrylonitrile-butadiene-styrene specimen, poly-butadiene or copolymer of butadiene spheres of about 500 nm diameter, which are selectively stained with osmium, is observed with soft X-rays in the wavelength region between 17 and 20 nm. For a 4-µ m-thick polyvinyl chloride film specimen formed by polymer powder compaction, peripheral areas of holes, grain boundaries, and areas probably degraded by HCl reduction are observed with soft X-rays in the wavelength region mainly around 2 nm.

  10. High-resolution, high-transmission soft x-ray spectrometer for the study of biological samples

    SciTech Connect

    Fuchs, Oliver; Weinhardt, L.; Blum, M.; Welgand, M.; Umbach, E.; Bar, M.; Heske, C.; Denlinger, J.; Chuang, Y.-D.; McKinney, W.; Hussain, Z.; Gullikson, E.; Jones, M.; Batson, P.; Nelles, B.; Follath, R.

    2009-06-11

    We present a variable line-space grating spectrometer for soft s-rays that coverst the photon energy range between 130 and 650 eV. The optical design is based on the Hettrick-Underwood principle and tailored to synchrotron-based studies of radiation-sensitive biological samples. The spectrometer is able to record the entire spectral range in one shot, i.e., without any mechanical motion, at a resolving power of 1200 or better. Despite is slitless design, such a resolving power can be achieved for a source spot as large as (30 x 3000) micrometers squared, which is important for keeping beam damage effects in radiation-sensitive samples low. The high spectrometer efficiency allows recording of comprehensive two-dimensional resonant inelastic soft x-ray scatters (RIXS) maps with good statistics within several minutes. This is exemplarily demonstrated for a RIXS map of highly oriented pyrolytic graphite, which was taken with 10 min.

  11. Electron-multiplying CCDs for future soft X-ray spectrometers

    NASA Astrophysics Data System (ADS)

    Tutt, J. H.; Holland, A. D.; Murray, N. J.; Harriss, R. D.; Hall, D. J.; Soman, M.

    2012-02-01

    CCDs have been used in several high resolution soft X-ray spectrometers for both space and terrestrial applications such as the Reflection Grating Spectrometer on XMM-Newton and the Super Advanced X-ray Emission Spectrometer at the Paul Scherrer Institut in Switzerland. However, with their ability to use multiplication gain to amplify signal and suppress readout noise, EM-CCDs are being considered instead of CCDs for future soft X-ray spectrometers. When detecting low energy X-rays, EM-CCDs are able to increase the Signal-to-Noise ratio of the device, making the X-rays much easier to detect. If the signal is also significantly split between neighbouring pixels, the increase in the size of the signal will make complete charge collection and techniques such as centroiding easier to accomplish. However, multiplication gain from an EM-CCD does cause a degradation of the energy resolution of the device and there are questions about how the high field region in an EM-CCD will behave over time in high radiation environments. This paper analyses the possible advantages and disadvantages of using EM-CCDs for high resolution soft X-ray spectroscopy and suggests in which situations using them would not only be possible, but also beneficial to the instrument.

  12. Soft x-ray ionization induced fragmentation of glycine

    SciTech Connect

    Itälä, E.; Kooser, K.; Rachlew, E.; Huels, M. A.; Kukk, E.

    2014-06-21

    X-ray absorption commonly involves dissociative core ionization producing not only momentum correlated charged fragments but also low- and high-energy electrons capable of inducing damage in living tissue. This gives a natural motivation for studying the core ionization induced fragmentation processes in biologically important molecules such as amino acids. Here the fragmentation of amino acid glycine following carbon 1s core ionization has been studied. Using photoelectron-photoion-photoion coincidence technique, a detailed analysis on fragmentation of the sample molecule into pairs of momentum correlated cations has been carried out. The main characteristics of core ionization induced fragmentation of glycine were found to be the rupture of the C–C{sub α} bond and the presence of the CNH{sub 2}{sup +} fragment.

  13. Constraining the redshifted 21-cm signal with the unresolved soft X-ray background

    NASA Astrophysics Data System (ADS)

    Fialkov, Anastasia; Cohen, Aviad; Barkana, Rennan; Silk, Joseph

    2016-10-01

    We use the observed unresolved cosmic X-ray background (CXRB) in the 0.5 - 2 keV band and existing upper limits on the 21-cm power spectrum to constrain the high-redshift population of X-ray sources, focusing on their effect on the thermal history of the Universe and the cosmic 21-cm signal. Because the properties of these sources are poorly constrained, we consider hot gas, X-ray binaries and mini-quasars (i.e., sources with soft or hard X-ray spectra) as possible candidates. We find that (1) the soft-band CXRB sets an upper limit on the X-ray efficiency of sources that existed before the end of reionization, which is one-to-two orders of magnitude higher than typically assumed efficiencies, (2) hard sources are more effective in generating the CXRB than the soft ones, (3) the commonly-assumed limit of saturated heating is not valid during the first half of reionization in the case of hard sources, with any allowed value of X-ray efficiency, (4) the maximal allowed X-ray efficiency sets a lower limit on the depth of the absorption trough in the global 21-cm signal and an upper limit on the height of the emission peak, while in the 21-cm power spectrum it sets a minimum amplitude and frequency for the high-redshift peaks, and (5) the existing upper limit on the 21-cm power spectrum sets a lower limit on the X-ray efficiency for each model. When combined with the 21-cm global signal, the CXRB will be useful for breaking degeneracies and helping constrain the nature of high-redshift heating sources.

  14. An alternative scheme of angular-dispersion analyzers for high-resolution medium-energy inelastic X-ray scattering.

    PubMed

    Huang, Xian Rong

    2011-11-01

    The development of medium-energy inelastic X-ray scattering optics with meV and sub-meV resolution has attracted considerable efforts in recent years. Meanwhile, there are also concerns or debates about the fundamental and feasibility of the involved schemes. Here the central optical component, the back-reflection angular-dispersion monochromator or analyzer, is analyzed. The results show that the multiple-beam diffraction effect together with transmission-induced absorption can noticeably reduce the diffraction efficiency, although it may not be a fatal threat. In order to improve the efficiency, a simple four-bounce analyzer is proposed that completely avoids these two adverse effects. The new scheme is illustrated to be a feasible alternative approach for developing meV- to sub-meV-resolution inelastic X-ray scattering spectroscopy.

  15. High-resolution inelastic x-ray scattering to study the high-frequency atomic dynamics of disordered systems

    NASA Astrophysics Data System (ADS)

    Monaco, Giulio

    2008-06-01

    The use of momentum-resolved inelastic x-ray scattering with meV energy resolution to study the high-frequency atomic dynamics in disordered systems is here reviewed. The typical realization of this experiment is described together with some common models used to interpret the measured spectra and to extract parameters of interest for the investigation of disordered systems. With the help of some selected examples, the present status of the field is discussed. Particular attention is given to those results which are still open for discussion or controversial, and which will require further development of the technique to be fully solved. Such an instrumental development seems nowadays possible at the light of recently proposed schemes for advanced inelastic x-ray scattering spectrometers. To cite this article: G. Monaco, C. R. Physique 9 (2008).

  16. Continuous high-repetition-rate operation of collisional soft-x-ray lasers with solid targets.

    PubMed

    Weith, A; Larotonda, M A; Wang, Y; Luther, B M; Alessi, D; Marconi, M C; Rocca, J J; Dunn, J

    2006-07-01

    We have generated a laser average output power of 2 microW at a wavelength of 13.9 nm by operating a tabletop laser-pumped Ni-like Ag laser at a 5 Hz repetition rate, using a solid helicoidal target that is continuously rotated and advanced to renew the target surface between shots. More than 2 x 10(4) soft-x-ray laser shots were obtained by using a single target. Similar results were obtained at 13.2 nm in Ni-like Cd with a Cd-coated target. This scheme will allow uninterrupted operation of laser-pumped tabletop collisional soft-x-ray lasers at a repetition rate of 10 Hz for a period of hours, enabling the generation of continuous high average soft-x-ray powers for applications. PMID:16770410

  17. Wide field-of-view soft X-ray imaging for solar wind-magnetosphere interactions

    NASA Astrophysics Data System (ADS)

    Walsh, B. M.; Collier, M. R.; Kuntz, K. D.; Porter, F. S.; Sibeck, D. G.; Snowden, S. L.; Carter, J. A.; Collado-Vega, Y.; Connor, H. K.; Cravens, T. E.; Read, A. M.; Sembay, S.; Thomas, N. E.

    2016-04-01

    Soft X-ray imagers can be used to study the mesoscale and macroscale density structures that occur whenever and wherever the solar wind encounters neutral atoms at comets, the Moon, and both magnetized and unmagnetized planets. Charge exchange between high charge state solar wind ions and exospheric neutrals results in the isotropic emission of soft X-ray photons with energies from 0.1 to 2.0 keV. At Earth, this process occurs primarily within the magnetosheath and cusps. Through providing a global view, wide field-of-view imaging can determine the significance of the various proposed solar wind-magnetosphere interaction mechanisms by evaluating their global extent and occurrence patterns. A summary of wide field-of-view (several to tens of degrees) soft X-ray imaging is provided including slumped micropore microchannel reflectors, simulated images, and recent flight results.

  18. ALP conversion and the soft X-ray excess in the outskirts of the Coma cluster

    SciTech Connect

    Kraljic, David; Rummel, Markus; Conlon, Joseph P. E-mail: Markus.Rummel@physics.ox.ac.uk

    2015-01-01

    It was recently found that the soft X-ray excess in the center of the Coma cluster can be fitted by conversion of axion-like-particles (ALPs) of a cosmic axion background (CAB) to photons. We extend this analysis to the outskirts of Coma, including regions up to 5 Mpc from the center of the cluster. We extract the excess soft X-ray flux from ROSAT All-Sky Survey data and compare it to the expected flux from ALP to photon conversion of a CAB. The soft X-ray excess both in the center and the outskirts of Coma can be simultaneously fitted by ALP to photon conversion of a CAB. Given the uncertainties of the cluster magnetic field in the outskirts we constrain the parameter space of the CAB. In particular, an upper limit on the CAB mean energy and a range of allowed ALP-photon couplings are derived.

  19. Initial Operation of the NSTX Fast Tangential Soft X-Ray Camera

    SciTech Connect

    B.C. Stratton; R. Feder; S. von Goeler; G.F. Renda; J.L. Lowrance; V.J. Mastrocola

    2004-05-11

    Fast, two-dimensional, soft x-ray imaging is a powerful technique for the study of MHD instabilities in tokamak plasmas. We have constructed an ultra-fast frame rate soft x-ray camera for the National Spherical Torus Experiment. It is based on a recently developed 64 x 64 pixel CCD camera capable of capturing 300 frames at up to 500,000 frames per second. A pinhole aperture images the plasma soft x-ray emission (0.2-10 keV) onto a P47 scintillator deposited on a fiber-optic faceplate; the scintillator visible light output is detected and amplified by a demagnifying image intensifier and lens-coupled to the CCD chip. A selection of beryllium foils provides discrimination of low-energy emission. The system is installed on NSTX with a wide-angle tangential view of the plasma. Initial plasma data and an assessment of the system performance are presented.

  20. 3D simulation of the image formation in soft x-ray microscopes.

    PubMed

    Selin, Mårten; Fogelqvist, Emelie; Holmberg, Anders; Guttmann, Peter; Vogt, Ulrich; Hertz, Hans M

    2014-12-15

    In water-window soft x-ray microscopy the studied object is typically larger than the depth of focus and the sample illumination is often partially coherent. This blurs out-of-focus features and may introduce considerable fringing. Understanding the influence of these phenomena on the image formation is therefore important when interpreting experimental data. Here we present a wave-propagation model operating in 3D for simulating the image formation of thick objects in partially coherent soft x-ray microscopes. The model is compared with present simulation methods as well as with experiments. The results show that our model predicts the image formation of transmission soft x-ray microscopes more accurately than previous models.

  1. Heating of low-density CHO-foam layers by means of soft X-rays

    NASA Astrophysics Data System (ADS)

    Rosmej, O. N.; Bagnoud, V.; Eisenbarth, U.; Vatulin, V.; Zhidkov, N.; Suslov, N.; Kunin, A.; Pinegin, A.; Schäfer, D.; Nisius, Th.; Wilhein, Th.; Rienecker, T.; Wiechula, J.; Jacoby, J.; Zhao, Y.; Vergunova, G.; Borisenko, N.; Orlov, N.

    2011-10-01

    Interaction of soft X-ray thermal radiation with polymer foam layers has been studied experimentally. Indirectly heated CHO-foams were used to create a plasma target for applications in combined heavy ion beam-laser experiments that are aimed at investigation of the heavy ion energy loss in ionized matter. In this work, we report experimental results on heating of low Z foams by means of the Planckian radiation generated in gold hohlraums. The experimental goal was to study the hohlraum radiation field, duration of the soft X-ray pulse, the conversion efficiency of the laser energy into soft X-rays, measurements of the absorption properties of foam layers and parameters of the foam targets heated by the Plankian radiation.

  2. The coolest DA white dwarfs detected at soft X-ray wavelengths

    NASA Technical Reports Server (NTRS)

    Kidder, K. M.; Holberg, J. B.; Barstow, M. A.; Tweedy, R. W.; Wesemael, F.

    1992-01-01

    New soft X-ray/EUV photometric observations of the DA white dwarfs KPD 0631 + 1043 = WD 0631 + 107 and PG 1113 + 413 = WD 1113 + 413 are analyzed. Previously reported soft X-ray detections of three other DAs and the failure to detect a fourth DA in deep Exosat observations are investigated. New ground-based spectra are presented for all of the objects, with IUE Ly-alpha spectra for some. These data are used to constrain the effective temperatures and surface gravities. The improved estimates of these parameters are employed to refer a photospheric He abundance for the hotter objects and to elucidate an effective observational low-temperature threshold for the detection of pure hydrogen DA white dwarfs at soft X-ray wavelengths.

  3. Electronic Raman scattering with excitation between localized states observed in the zinc M{sub 2,3} soft x-ray spectra of ZnS

    SciTech Connect

    Zhou, L.; Callcott, T.A.; Jia, J.J.

    1997-04-01

    Zn M{sub 2,3} soft x-ray fluorescence (SXF) spectra of ZnS and ZnS{sub .5}Se{sub .5} excited near threshold show strong inelastic scattering effects that can be explained using a simple model and an inelastic scattering theory based on second order perturbation theory. This scattering is often called electronic resonance Raman scattering. Tulkki and Aberg have developed this theory in detail for atomic systems, but their treatment can be applied to solid systems by utilizing electronic states characteristic of solids rather than of atomic systems.

  4. Dynamics of electron-phonon scattering: crystal- and angular-momentum transfer probed by resonant inelastic x-ray scattering.

    PubMed

    Beye, M; Hennies, F; Deppe, M; Suljoti, E; Nagasono, M; Wurth, W; Föhlisch, A

    2009-12-01

    Experimentally, we observe angular-momentum transfer in electron-phonon scattering, although it is commonly agreed that phonons transfer mostly linear momentum. Therefore, the incorporation of angular momentum to describe phonons is necessary already for simple semiconductors and bears significant implications for the formation of new quasiparticles in correlated functional materials. Separation of linear and angular-momentum transfer in electron-phonon scattering is achieved by highly selective excitations on the femtosecond time scale of resonant inelastic x-ray scattering.

  5. Soft X-ray observations of pre-main sequence stars in the chamaeleon dark cloud

    NASA Technical Reports Server (NTRS)

    Feigelson, Eric D.; Kriss, Gerard A.

    1987-01-01

    Einstein IPC observations of the nearby Chamaeleon I star forming cloud show 22 well-resolved soft X-ray sources in a 1x2 deg region. Twelve are associated with H-alpha emission line pre-main sequence (PMS) stars, and four with optically selected PMS stars. Several X-ray sources have two or more PMS stars in their error circles. Optical spectra were obtained at CTIO of possible stellar counterparts of the remaining X-ray sources. They reveal 5 probable new cloud members, K7-MO stars with weak or absent emission lines. These naked X-ray selected PMS stars are similar to those found in the Taurus-Auriga cloud. The spatial distributions and H-R diagrams of the X-ray and optically selected PMS stars in the cloud are very similar. Luminosity functions indicate the Chamaeleon stars are on average approximately 5 times more X-ray luminous than Pleiad dwarfs. A significant correlation between L sub x and optical magnitude suggests this trend may continue within the PMS phase of stellar evolution. The relation of increasing X-ray luminosity with decreasing stellar ages is thus extended to stellar ages as young as 1 million years.

  6. Electronic structure of alkali-intercalated graphite studied by soft-x-ray emission spectroscopy

    NASA Astrophysics Data System (ADS)

    Mansour, A.; Schnatterly, S. E.; Ritsko, J. J.

    1987-02-01

    Carbon K soft-x-ray emission spectra of LiC6, KC8, and CsC8 are presented. An absolute value for the charge transfer from the alkali metal to the carbon π band is obtained. A model fit to the data reveals similar effects on both spectral shape and threshold energy, independent of the choice of the alkali-metal intercalant, and provides a measure of departures from the rigid-band approximation. An enhancement of the soft-x-ray emission spectrum near EF is reported.

  7. Multilayer films with sharp, stable interfaces for use in EUV and soft X-ray application

    DOEpatents

    Barbee, Jr., Troy W.; Bajt, Sasa

    2002-01-01

    The reflectivity and thermal stability of Mo/Si (molybdenum/silicon) multilayer films, used in soft x-ray and extreme ultraviolet region, is enhanced by deposition of a thin layer of boron carbide (e.g., B.sub.4 C) between alternating layers of Mo and Si. The invention is useful for reflective coatings for soft X-ray and extreme ultraviolet optics, multilayer for masks, coatings for other wavelengths and multilayers for masks that are more thermally stable than pure Mo/Si multilayers

  8. Experimental demonstration of a soft x-ray self-seeded free-electron laser

    DOE PAGES

    Ratner, D.; Abela, R.; Amann, J.; Behrens, C.; Bohler, D.; Bouchard, G.; Bostedt, C.; Boyes, M.; Chow, K.; Cocco, D.; et al

    2015-02-06

    The Linac Coherent Light Source has added self-seeding capability to the soft x-ray range using a grating monochromator system. We report demonstration of soft x-ray self-seeding with a measured resolving power of 2000-5000, wavelength stability of 10-4, and an increase in peak brightness by a factor of 2-5 across the photon energy range of 500-1000 eV. By avoiding the need for a monochromator at the experimental station, the self-seeded beam can deliver as much as 50 fold higher brightness to users.

  9. Numerical Experiments on Oxygen Plasma Focus: Scaling Laws of Soft X-Ray Yields

    NASA Astrophysics Data System (ADS)

    Akel, M.

    2013-08-01

    Numerical experiments have been investigated on UNU/ICTP PFF low energy plasma focus device with oxygen filling gas. In these numerical experiments, the temperature window of 119-260 eV has been used as a suitable temperature range for generating oxygen soft X-rays. The Lee model was applied to characterize the UNU/ICTP PFF plasma focus. The optimum soft X-ray yield (Ysxr) was found to be 0.75 J, with the corresponding efficiency of about 0.03 % at pressure of 2.36 Torr and the end axial speed was va = 5 cm/μs. The practical optimum combination of p0, z0 and `a' for oxygen Ysxr was found to be 0.69 Torr, 4.8 cm and 2.366 cm respectively, with the outer radius b = 3.2 cm. This combination gives Ysxr ~ 5 J, with the corresponding efficiency of about 0.16 %. Thus we expect to increase the oxygen Ysxr of UNU/ICTP PFF, without changing the capacitor bank, merely by changing the electrode configuration and operating pressure. Scaling laws on oxygen soft X-ray yield, in terms of storage energies E0, peak discharge current Ipeak and focus pinch current Ipinch were found over the range from 1 kJ to 1 MJ. It was found that the oxygen soft X-ray yields scale well with and for the low inductance (L0 = 30 nH) (where yields are in J and currents in kA). While the soft X-ray yield scaling laws in terms of storage energies were found to be as (E0 in kJ and Ysxr in J) with the scaling showing gradual deterioration as E0 rises over the range. The oxygen soft X-ray yield emitted from plasma focus is found to be about 8.7 kJ for storage energy of 1 MJ. The optimum efficiency for soft X-ray yield (1.1 %) is with capacitor bank energy of 120 kJ. This indicates that oxygen plasma focus is a good soft X-ray source when properly designed.

  10. Intracellular nanoparticles mass quantification by near-edge absorption soft X-ray nanotomography

    PubMed Central

    Conesa, Jose Javier; Otón, Joaquín; Chiappi, Michele; Carazo, Jose María; Pereiro, Eva; Chichón, Francisco Javier; Carrascosa, José L.

    2016-01-01

    We used soft X-ray three-dimensional imaging to quantify the mass of superparamagnetic iron oxide nanoparticles (SPION) within whole cells, by exploiting the iron oxide differential absorption contrast. Near-edge absorption soft X-ray nanotomography (NEASXT) combines whole-cell 3D structure determination at 50 nm resolution, with 3D elemental mapping and high throughput. We detected three-dimensional distribution of SPIONs within cells with 0.3 g/cm3 sensitivity, sufficient for detecting the density corresponding to a single nanoparticle. PMID:26960695

  11. Experimental demonstration of a soft x-ray self-seeded free-electron laser

    SciTech Connect

    Ratner, D.; Abela, R.; Amann, J.; Behrens, C.; Bohler, D.; Bouchard, G.; Bostedt, C.; Boyes, M.; Chow, K.; Cocco, D.; Decker, F. J.; Ding, Y.; Eckman, C.; Emma, P.; Fairley, D.; Feng, Y.; Field, C.; Flechsig, U.; Gassner, G.; Hastings, J.; Heimann, P.; Huang, Z.; Kelez, N.; Krzywinski, J.; Loos, H.; Lutman, A.; Marinelli, A.; Marcus, G.; Maxwell, T.; Moeller, S.; Morton, D.; Nuhn, H. D.; Rodes, N.; Schlotter, W.; Serkez, S.; Stevens, T.; Turner, J.; Walz, D.; Welch, J.; Wu, J.

    2015-02-06

    The Linac Coherent Light Source has added self-seeding capability to the soft x-ray range using a grating monochromator system. We report demonstration of soft x-ray self-seeding with a measured resolving power of 2000-5000, wavelength stability of 10-4, and an increase in peak brightness by a factor of 2-5 across the photon energy range of 500-1000 eV. By avoiding the need for a monochromator at the experimental station, the self-seeded beam can deliver as much as 50 fold higher brightness to users.

  12. Soft x-ray resonant magnetic scattering from an imprinted magnetic domain pattern

    SciTech Connect

    Kinane,C.; Suszka, A.; Marrows, C.; Hickey, B.; Arena, D.; Dvorak, J.; Charlton, T.; Langridge, S.

    2006-01-01

    The authors report on the use of a Co/Pt multilayer, which exhibits strong perpendicular magnetic anisotropy, to magnetostatically imprint a domain pattern onto a 50 Angstroms thick Permalloy layer. Element specific soft x-ray magnetic scattering experiments were then performed so as to be sensitive to the magnetic structure of the Permalloy only. Off-specular magnetic satellite peaks, corresponding to a periodic domain stripe width of 270 nm, were observed, confirmed by magnetic force microscopy and micromagnetic modeling. Thus the authors have exploited the element specificity of soft x-ray scattering to discern the purely magnetic correlations in a structurally flat Permalloy film.

  13. Soft X-ray emission in kink-unstable coronal loops

    NASA Astrophysics Data System (ADS)

    Pinto, Rui; Vilmer, Nicole; Brun, Allan Sacha

    Solar flares are associated with intense soft X-ray emission generated by the hot flaring plasma in coronal magnetic loops. We investigate the temporal, spectral and spatial evolution of the properties of the thermal X-ray emission produced in simulated kink-unstable magnetic flux-ropes. The numerical setup used consists of a highly twisted loop embedded in a region of uniform and untwisted background coronal magnetic field. The magnetic flux-rope reconnects with the background flux after the triggering of the kink instability and is then allowed to relax to a lower energy state. Strong ohmic heating leads to strong and quick heating (up to more than 15 MK), to a strong peak of X-ray emission and to the hardening of the thermal X-ray spectrum. The emission pattern is often filamentary and the amount of twist deduced from the X-ray emission alone is considerably lower than the maximum twist in the simulated flux-ropes. The flux-rope plasma becomes strongly multi-thermal during the flaring episode. The emission measure evolves into a bi-modal distribution as a function of temperature during the saturation phase, and later converges to the power-law distribution mathrm{EM}~ T(-4.2) (during the relaxation/cooling) phase. These soft X-ray emission properties are maintained for a large range of coronal magnetic field strength, plasma density and flux-rope twist values.

  14. Nanostructured diffractive optical devices for soft X-ray microscopes

    NASA Astrophysics Data System (ADS)

    Hambach, D.; Peuker, M.; Schneider, G.

    2001-07-01

    The new transmission X-ray microscope (TXM) installed at the BESSY II electron storage ring uses an off-axis transmission zone plate (OTZ) as diffractive and focusing element of the condenser-monochromator setup. A high resolution micro-zone plate (MZP) forms a magnified image on a CCD-detector. Both, the OTZ with an active area of up to 24 mm2 and the MZP with zone widths as small as 25 nm are generated by a process including electron beam lithography (EBL), dry etching and subsequent electroplating of nickel on top of silicon membrane substrates with about 100- 150 nm thickness. The combination of a larger zone width and the usage of nickel zone structures allows to increase the diffraction efficiency of the condenser element at least by a factor of 3 compared to the earlier used KZP7 condenser zone plate in the TXM at BESSY I. Groove diffraction efficiencies of 21.6% and 14.7% were measured for MZP objectives with 40 and 25 nm outermost zone width, respectively.

  15. The ISM From the Soft X-ray Background Perspective

    NASA Technical Reports Server (NTRS)

    Snowden, S. L.

    2003-01-01

    In the past few years progress in understanding the local and Galactic ISM in terms of the diffuse X-ray background has been as much about what hasn't been seen as it has been about detections. High resolution spectra of the local SXRB have been observed, but are inconsistent with current thermal emission models. An excess over the extrapolation of the high-energy (most clearly visible at E greater than 1.5 keV) extragalactic power law down to 3/4 keV has been observed but only at the level consistent with cosmological models, implying the absence of at least a bright hot Galactic halo. A very recent FUSE result indicates that O VI emission from the Local Hot Bubble is insignificant, if it exists at all, a result which is also inconsistent with current thermal emission models. A short review of the current status of our (well, at least my) understanding of the Galactic SXRB and ISM is presented here.

  16. A linear motion machine for soft x-ray interferometry

    SciTech Connect

    Duarte, R.; Howells, M.R.; Hussain, Z.; Lauritzen, T.; McGill, R.

    1997-07-01

    A Fourier Transform X-ray Spectrometer has been designed and built for use at the Advanced light source at Lawrence Berkeley National Laboratory. The design requires a total rectilinear motion of 15 mm with a maximum pitch error of the stage below {+-}0.4 {mu}radians, to achieve this the authors chose to build the entire machine as a single monolithic flexure. A hydraulic driver with sliding O-ring seals was developed with the intention to provide motion with a stick-slip position error of less than 0.8 nm at a uniform velocity of 20 {mu}m/sec. The machine is comprised of two pairs of nested linear motion flexures, all explained by means of a theory published earlier by Hathaway. Certain manufacturing errors were successfully corrected by an extra weak-link feature in the monolith frame. The engineering details of all the subsystems of the linear motion machine are described and measured performance reported.

  17. Analysis of inelastic x-ray scattering spectra of low-temperature water

    PubMed

    Liao; Chen; Sette

    2000-02-01

    We analyze a set of high-resolution inelastic x-ray scattering (IXS) spectra from H2O measured at T=259, 273, and 294 K using two different phenomenological models. Model I, called the "dynamic cage model," combines the short time in-cage dynamics described by a generalized Enskog kinetic theory with a long-time cage relaxation dynamics described by an alpha relaxation. This model is appropriate for supercooled water where the cage effect is dominant and the existence of an alpha relaxation is evident from molecular-dynamics (MD) simulation data of extended simple point charge (SPC/E) model water. Model II is essentially a generalized hydrodynamic theory called the "three effective eigenmode theory" by de Schepper et al. 11. This model is appropriate for normal liquid water where the cage effect is less prominent and there is no evidence of the alpha relaxation from the MD data. We use the model I to analyze IXS data at T=259 K (supercooled water). We successfully extract the Debye-Waller factor, the cage relaxation time from the long-time dynamics, and the dispersion relation of high-frequency sound from the short time dynamics. We then use the model II to analyze IXS data at all three temperatures, from which we are able to extract the relaxation rate of the central mode and the damping of the sound mode as well as the dispersion relation for the high-frequency sound. It turns out that the dispersion relations extracted from the two models at their respective temperatures agree with each other giving the high-frequency sound speed of 2900+/-300 m/s. This is to be compared with a slightly higher value reported previously, 3200+/-320 m/s, by analyzing similar IXS data with a phenomenological-damped harmonic oscillator model 22. This latter model has traditionally been used exclusively for the analysis of inelastic scattering spectra of water. The k-dependent sound damping and central mode relaxation rate extracted from our model analyses are compared with the known

  18. Single-shot calibration of soft x-ray mirrors using a sinusoidal transmission grating.

    PubMed

    Shpilman, Z; Ehrlich, Y; Maman, S; Levy, I; Shussman, T; Oren, G; Zakosky Nueberger, I; Hurvitz, G

    2014-11-01

    Calibration of soft x-ray diagnostics is a challenge due to the lack of laboratory-size calibrated sources. An in situ calibration method for newly developed x-ray mirrors, is presented. The x-ray source is produced by laser-matter interaction, and twin transmission gratings which create two identical dispersion lines. The gratings have a sinusoidal transmission function, which produces a highly precise high-orders free spectrum. An x-ray mirror interacts with one of the dispersion lines, and the mirror efficiency curve as a function of wavelength is extracted. Mirror efficiency shows good agreement with the literature, and evidence of water layer may justify the need of in situ calibration.

  19. Versatile soft X-ray-optical cross-correlator for ultrafast applications

    PubMed Central

    Schick, Daniel; Eckert, Sebastian; Pontius, Niko; Mitzner, Rolf; Föhlisch, Alexander; Holldack, Karsten; Sorgenfrei, Florian

    2016-01-01

    We present an X-ray-optical cross-correlator for the soft (>150 eV) up to the hard X-ray regime based on a molybdenum-silicon superlattice. The cross-correlation is done by probing intensity and position changes of superlattice Bragg peaks caused by photoexcitation of coherent phonons. This approach is applicable for a wide range of X-ray photon energies as well as for a broad range of excitation wavelengths and requires no external fields or changes of temperature. Moreover, the cross-correlator can be employed on a 10 ps or 100 fs time scale featuring up to 50% total X-ray reflectivity and transient signal changes of more than 20%. PMID:27795974

  20. Prototype high resolution multienergy soft x-ray array for NSTX

    SciTech Connect

    Tritz, K.; Stutman, D.; Finkenthal, M.; Delgado-Aparicio, L.; Kaita, R.; Roquemore, L.

    2010-10-15

    A novel diagnostic design seeks to enhance the capability of multienergy soft x-ray (SXR) detection by using an image intensifier to amplify the signals from a larger set of filtered x-ray profiles. The increased number of profiles and simplified detection system provides a compact diagnostic device for measuring T{sub e} in addition to contributions from density and impurities. A single-energy prototype system has been implemented on NSTX, comprised of a filtered x-ray pinhole camera, which converts the x-rays to visible light using a CsI:Tl phosphor. SXR profiles have been measured in high performance plasmas at frame rates of up to 10 kHz, and comparisons to the toroidally displaced tangential multi-energy SXR have been made.

  1. The photoelectric effect from CsI by polarized soft X-rays

    NASA Technical Reports Server (NTRS)

    Shaw, Ping S.; Church, Eric D.; Hanany, Shaul; Liu, Yee; Fleischman, Judith; Kaaret, Philip; Novick, Robert; Manzo, Giuseppe

    1991-01-01

    Studies of the polarization dependence of the photoelectric effect produced by soft X-rays from CsI indicate that the geometrical effects in these experiments can often mimic the polarization signature. This paper presents a detailed calculation of these geometrical effects that are produced when the X-ray beam is not precisely aligned on a rotatable plane photocathode. The experimentally observed geometrical effects were used to precisely determine the realignment of the incident beam of polarized X-rays on a rotatable photocathode. The results allow determinations of the true polarization dependence of the photoemission from CsI. It is shown that the photoelectric effect in CsI depends on the polarization state of the X-rays.

  2. Developing a CCD camera with high spatial resolution for RIXS in the soft X-ray range

    NASA Astrophysics Data System (ADS)

    Soman, M. R.; Hall, D. J.; Tutt, J. H.; Murray, N. J.; Holland, A. D.; Schmitt, T.; Raabe, J.; Schmitt, B.

    2013-12-01

    The Super Advanced X-ray Emission Spectrometer (SAXES) at the Swiss Light Source contains a high resolution Charge-Coupled Device (CCD) camera used for Resonant Inelastic X-ray Scattering (RIXS). Using the current CCD-based camera system, the energy-dispersive spectrometer has an energy resolution (E/ΔE) of approximately 12,000 at 930 eV. A recent study predicted that through an upgrade to the grating and camera system, the energy resolution could be improved by a factor of 2. In order to achieve this goal in the spectral domain, the spatial resolution of the CCD must be improved to better than 5 μm from the current 24 μm spatial resolution (FWHM). The 400 eV-1600 eV energy X-rays detected by this spectrometer primarily interact within the field free region of the CCD, producing electron clouds which will diffuse isotropically until they reach the depleted region and buried channel. This diffusion of the charge leads to events which are split across several pixels. Through the analysis of the charge distribution across the pixels, various centroiding techniques can be used to pinpoint the spatial location of the X-ray interaction to the sub-pixel level, greatly improving the spatial resolution achieved. Using the PolLux soft X-ray microspectroscopy endstation at the Swiss Light Source, a beam of X-rays of energies from 200 eV to 1400 eV can be focused down to a spot size of approximately 20 nm. Scanning this spot across the 16 μm square pixels allows the sub-pixel response to be investigated. Previous work has demonstrated the potential improvement in spatial resolution achievable by centroiding events in a standard CCD. An Electron-Multiplying CCD (EM-CCD) has been used to improve the signal to effective readout noise ratio achieved resulting in a worst-case spatial resolution measurement of 4.5±0.2 μm and 3.9±0.1 μm at 530 eV and 680 eV respectively. A method is described that allows the contribution of the X-ray spot size to be deconvolved from these

  3. A study of X-ray emission from galactic and extragalactic sources with emphasis on soft and ultra-soft wavelengths

    NASA Technical Reports Server (NTRS)

    Bowyer, C. S.; Lampton, M.; Cruddace, R. G.; Paresce, F.

    1974-01-01

    A Black Brant VC rocket was used to scan the Coma and Virgo clusters in order to measure structure in the X-ray sources. The rocket also made measurements of soft X-ray spectra, soft X-ray background flux during a 50 deg scan of the sky, soft X-rays from De Voucoulers 50, set limits to the energy dependence of soft X-ray background spectra, and the flux of solar 584 A radiation resonantly scattered by interstellar He flowing through the solar system.

  4. Analysis of the operation and plasma dynamics of extreme- ultraviolet and soft x-ray lasers

    NASA Astrophysics Data System (ADS)

    Bender, Howard Albert, III

    Extending lasing action into the extreme ultraviolet and soft x-ray regions of the electromagnetic spectrum has been a natural progression in the continuing development of short wavelength radiation sources. However fundamental difficulties with the media used to produce short wavelength lasers has in general hindered the widespread development and use of such lasers in applications. Up to now all EUV and soft x-ray lasers have operated with plasmas as the gain medium to support lasing. This is a general requirement imposed by (1) the characteristics of short wavelength radiation as it originates from highly energetic atomic transitions and (2) the fundamental aspects of lasing at these wavelengths. Thus the plasma environment has been the defining characteristic in achieving lasing in the EUV and soft x-ray spectral regions. This thesis presents investigations into two types of EUV/Soft x-ray lasers that describe the operation and associated plasma dynamics of these devices. The first is a numerical investigation into a recombination pumped x-ray laser at 13.5 nm operating in a Li plasma. Using a collisional-radiative model of the atomic system, simulations were performed to determine the plasma conditions necessary to produce gain that were observed in reported experiments. The second investigation is the experimental development and operation of a capillary discharge driven laser operating at 46.9 nm in Ar. This device is a new generation of EUV/Soft X-ray laser based on a small scale driver system. The first interferometric probing experiments of this device will be discussed and related to the plasma dynamics of the capillary discharge.

  5. Diagnosing the accretion flow in ultraluminous X-ray sources using soft X-ray atomic features

    NASA Astrophysics Data System (ADS)

    Middleton, Matthew J.; Walton, Dominic J.; Fabian, Andrew; Roberts, Timothy P.; Heil, Lucy; Pinto, Ciro; Anderson, Gemma; Sutton, Andrew

    2015-12-01

    The lack of unambiguous detections of atomic features in the X-ray spectra of ultraluminous X-ray sources (ULXs) has proven a hindrance in diagnosing the nature of the accretion flow. The possible association of spectral residuals at soft energies with atomic features seen in absorption and/or emission and potentially broadened by velocity dispersion could therefore hold the key to understanding much about these enigmatic sources. Here we show for the first time that such residuals are seen in several sources and appear extremely similar in shape, implying a common origin. Via simple arguments we assert that emission from extreme colliding winds, absorption in a shell of material associated with the ULX nebula and thermal plasma emission associated with star formation are all highly unlikely to provide an origin. Whilst CCD spectra lack the energy resolution necessary to directly determine the nature of the features (i.e. formed of a complex of narrow lines or intrinsically broad lines), studying the evolution of the residuals with underlying spectral shape allows for an important, indirect test for their origin. The ULX NGC 1313 X-1 provides the best opportunity to perform such a test due to the dynamic range in spectral hardness provided by archival observations. We show through highly simplified spectral modelling that the strength of the features (in either absorption or emission) appears to anticorrelate with spectral hardness, which would rule out an origin via reflection of a primary continuum and instead supports a picture of atomic transitions in a wind or nearby material associated with such an outflow.

  6. Soft X-ray Luminosity and Photospheric Magnetic Field in Quiet Sun.

    NASA Astrophysics Data System (ADS)

    Pevtsov, A. A.; Acton, L. W.

    2000-05-01

    We are using full disk soft X-ray data from Yohkoh and Kitt Peak daily magnetograms to study the coronal luminosity and photospheric magnetic field in the quiet Sun between 1991 November and 1998 December. For every image of our data set we extract three areas 4 by 4 solar degrees in size centered at 00N00W, 50N00W and 50S00W and compute X-ray luminosity and unsigned magnetic flux for each of these areas. Between 1991 (active Sun) and 1996 (quiet Sun) the X-ray luminosity at the heliographic center decreases by more than a factor of 7...while the magnetic flux decreases by only a factor of 2. A similar tendency is observed for our high latitude samples. Apart from the cycle-related variations, all three areas of quiet Sun exhibit significant non-periodic changes in X-ray luminosity. These variations occur on 9-12 month intervals and clearly correlate with increase/decrease in sunspot activity. Similar variations are present in the total X-ray irradiance averaged over the solar disk. On the contrary, the magnetic fluxes from the same areas of quiet Sun show no corresponding variations on this time scale. In our opinion, coronal heating models based on the reconnection of quiet sun magnetic elements (variously called chromospheric network, "magnetic carpet" or "salt and pepper" field) can not explain the million degree corona observed by the Yohkoh soft X-ray telescope. We conclude that the X-ray luminosity in the quiet Sun (at least in the Yohkoh temperature range, >2 MK) is primarily associated with the strong magnetic fields of active regions, not with weak photospheric fields. To further support this conclusion, we show one example of a dramatic change in X-ray luminosity over the entire visible corona that was associated with the emergence of a single small active region.

  7. Soft x-ray studies of plasma-focus pinch structures in PF-1000U experiments

    NASA Astrophysics Data System (ADS)

    Sadowski, M. J.; Paduch, M.; Skladnik-Sadowska, E.; Surala, W.; Zaloga, D.; Miklaszewski, R.; Zielinska, E.; Tomaszewski, K.

    2015-10-01

    This work reports on recent experiments performed at the modernized PF-1000U plasma-focus facility. In contrast to earlier studies the main attention was focussed on measurements of the soft x-ray emission. Detailed time-integrated x-ray measurements, carried out using filtered pinhole cameras with sensitive x-ray films, are presented and analysed. The fine structure of the collapsing current sheath and dense pinch column is investigated. Observations of ‘plasma filaments’ are discussed and compared with those from the old POSEIDON facility. New results are time-integrated x-ray images of PF-1000U discharges with additional gas puffing, which in many cases show distinct plasma filaments and/or ‘hot spots’ formed inside the dense pinch column. The formation of such ‘hot-spots’ is explained by necking and breaking of the plasma filaments. Results of time-resolved x-ray measurements, performed outside the experimental chamber by means of scintillation probes, and inside with PIN-diodes placed behind pinholes and absorption filters, are also presented Time-resolved measurements, carried out using an old XUV framing-camera and a new soft x-ray four-frame camera (SXRFFC), are also presented and discussed. Correlations of the time-integrated x-ray images (of plasma filaments and hot spots) with time-resolved x-ray signals are discussed. The hypothesis that plasma-current filaments appear in almost all PF-type discharges is supported by pictures of radial erosion tracks on the anode front-plate after many discharges.

  8. Resolving the Origin of the Diffuse Soft X-ray Background

    NASA Technical Reports Server (NTRS)

    Smith, Randall K.; Foster, Adam R.; Edgar, Ricard J.; Brickhouse, Nancy S.; Sanders, Wilton T.

    2012-01-01

    In January 1993, the Diffuse X-ray Spectrometer (DXS) measured the first high-resolution spectrum of the diffuse soft X-ray background between 44-80A. A line-dominated spectrum characteristic of a 10(exp 6)K collisionally ionized plasma' was expected but while the observed spectrum was clearly line-dominated, no model would fit. Then in 2003 the Cosmic Hot Interstellar Plasma Spectrometer (CHIPS) launched and observed the diffuse extreme-ultraviolet (EUV) spectrum between 90- 265A. Although many emission lines were again expected; only Fe IX at 171.1A was detected. The discovery of X-rays from comets led to the realization that heavy ions (Z=6-28) in the solar wind will emit soft X-rays as the ions interact via charge exchange with neutral atoms in the heliosphere and geocorona. Using a new model for solar wind charge exchange (SWCX) emission, we show that the diffuse soft X-ray background can be understood as a combination of emission from charge exchange onto the slow and fast solar wind together with a more distant and diffuse hot (10(exp 6)K) plasma.

  9. A Soft X-Ray Transient in the M31 Bulge

    NASA Astrophysics Data System (ADS)

    Williams, Benjamin F.; Garcia, Michael R.; McClintock, Jeffrey E.; Primini, Frank A.; Murray, Stephen S.

    2006-01-01

    We have examined a probable soft X-ray transient source in the M31 bulge at R.A.=0h42m41.814s+/-0.08", decl.=41deg16'35.86"+/-0.07". On the three occasions we observed the source, its spectrum was soft (kTin~1 keV). The brightest detection of the source was on 2004 July 17, with a 0.3-7 keV luminosity of ~5×1037 ergs s-1. The only previous detection of the source was in 1979 by the Einstein observatory. The multiple detections over 25 years suggest that the duty cycle of the source is in the range 0.02-0.06. Coordinated HST ACS imaging before, during, and after the outburst revealed no variable optical source within the position errors of the X-ray source. The optical data place a firm upper limit on the brightness of the counterpart of the X-ray outburst of B>24.7, suggesting that the binary has a period <~5.2 days. The X-ray spectrum and lack of bright stars at the source location indicate that the source was a soft transient event occurring in a low-mass X-ray binary, making this source a good black hole candidate in M31.

  10. X-Ray Scatter Correction on Soft Tissue Images for Portable Cone Beam CT

    PubMed Central

    Aootaphao, Sorapong; Thongvigitmanee, Saowapak S.; Rajruangrabin, Jartuwat; Thanasupsombat, Chalinee; Srivongsa, Tanapon; Thajchayapong, Pairash

    2016-01-01

    Soft tissue images from portable cone beam computed tomography (CBCT) scanners can be used for diagnosis and detection of tumor, cancer, intracerebral hemorrhage, and so forth. Due to large field of view, X-ray scattering which is the main cause of artifacts degrades image quality, such as cupping artifacts, CT number inaccuracy, and low contrast, especially on soft tissue images. In this work, we propose the X-ray scatter correction method for improving soft tissue images. The X-ray scatter correction scheme to estimate X-ray scatter signals is based on the deconvolution technique using the maximum likelihood estimation maximization (MLEM) method. The scatter kernels are obtained by simulating the PMMA sheet on the Monte Carlo simulation (MCS) software. In the experiment, we used the QRM phantom to quantitatively compare with fan-beam CT (FBCT) data in terms of CT number values, contrast to noise ratio, cupping artifacts, and low contrast detectability. Moreover, the PH3 angiography phantom was also used to mimic human soft tissues in the brain. The reconstructed images with our proposed scatter correction show significant improvement on image quality. Thus the proposed scatter correction technique has high potential to detect soft tissues in the brain. PMID:27022608

  11. X-Ray Scatter Correction on Soft Tissue Images for Portable Cone Beam CT.

    PubMed

    Aootaphao, Sorapong; Thongvigitmanee, Saowapak S; Rajruangrabin, Jartuwat; Thanasupsombat, Chalinee; Srivongsa, Tanapon; Thajchayapong, Pairash

    2016-01-01

    Soft tissue images from portable cone beam computed tomography (CBCT) scanners can be used for diagnosis and detection of tumor, cancer, intracerebral hemorrhage, and so forth. Due to large field of view, X-ray scattering which is the main cause of artifacts degrades image quality, such as cupping artifacts, CT number inaccuracy, and low contrast, especially on soft tissue images. In this work, we propose the X-ray scatter correction method for improving soft tissue images. The X-ray scatter correction scheme to estimate X-ray scatter signals is based on the deconvolution technique using the maximum likelihood estimation maximization (MLEM) method. The scatter kernels are obtained by simulating the PMMA sheet on the Monte Carlo simulation (MCS) software. In the experiment, we used the QRM phantom to quantitatively compare with fan-beam CT (FBCT) data in terms of CT number values, contrast to noise ratio, cupping artifacts, and low contrast detectability. Moreover, the PH3 angiography phantom was also used to mimic human soft tissues in the brain. The reconstructed images with our proposed scatter correction show significant improvement on image quality. Thus the proposed scatter correction technique has high potential to detect soft tissues in the brain. PMID:27022608

  12. The high-field magnet endstation for X-ray magnetic dichroism experiments at ESRF soft X-ray beamline ID32.

    PubMed

    Kummer, K; Fondacaro, A; Jimenez, E; Velez-Fort, E; Amorese, A; Aspbury, M; Yakhou-Harris, F; van der Linden, P; Brookes, N B

    2016-03-01

    A new high-field magnet endstation for X-ray magnetic dichroism experiments has been installed and commissioned at the ESRF soft X-ray beamline ID32. The magnet consists of two split-pairs of superconducting coils which can generate up to 9 T along the beam and up to 4 T orthogonal to the beam. It is connected to a cluster of ultra-high-vacuum chambers that offer a comprehensive set of surface preparation and characterization techniques. The endstation and the beam properties have been designed to provide optimum experimental conditions for X-ray magnetic linear and circular dichroism experiments in the soft X-ray range between 400 and 1600 eV photon energy. User operation started in November 2014. PMID:26917134

  13. Performance of the ASTRO-H Soft X-ray Telescope (SXT-1)

    NASA Astrophysics Data System (ADS)

    Okajima, Takashi; Serlemitsos, P. J.; Soong, Y.

    2013-04-01

    The X-ray astronomy satellite, ASTRO-H, being developed under the collaboration among JAXA, NASA's GSFC and ESA, will have two Soft X-ray Telescopes (SXTs), among other instruments onboard, with a sensitive energy band up to 15 keV. One is for an X-ray micro-calorimeter detector and the other for an X-ray CCD detector. The SXT uses a conically approximated Wolter I grazing incidence optic implemented by thin aluminum foil substrates with thickness of 0.152, 0.229, and 0.305 mm. X-ray reflecting surface is a gold thin layer (2000A) transferred from a smooth glass mandrel to the substrate by a replication method using an epoxy buffer layer (12 um). It is similar to the Suzaku X-ray telescope, but with larger diameter (45 cm) and longer focal length (5.6 m). Recently we have completed the first flight SXT (SXT-1). X-ray measurments with a diverging beam at the Goddard 100-m beamline found an angular resolution to be 1.13 arcmin (HPD) at 4.5 keV. Since we also found that this performance has radial dependence, the angular resolution will be different for a parallel beam, i.e. in orbit. It will be measured by the full performance characterization at ISAS/JAXA, Japan, later this year. SXT-1 has successfully gone through environmental testing (vibration and thermal) and the performance ramains same. In this paper, we will report X-ray test results obtained at the Goddard X-ray beamline.

  14. Efficient alignment scheme for zone-plates-based transmission soft X-ray microscope

    NASA Astrophysics Data System (ADS)

    Lim, Jun; Shin, Hyun-Joon; Hong, Chung Ki

    2010-12-01

    Alignment and operation of a zone-plate (ZP)-based transmission soft X-ray microscope (TXM) is difficult and time consuming, especially when the TXM has no dedicated X-ray source. We introduce here an efficient TXM alignment scheme. The TXM employed is a simple in-situ-experiment-capable setup. It includes ultrahigh-vacuum (UHV)-compatible conflat flanges and is mountable in tandem with any soft X-ray synchrotron radiation beamlines. Obtaining zeroth- and first-order diffracted (condenser-zone-plate [CZP]-focused) beams simultaneously by means of the objective zone plate (OZP) is the most essential step in the alignment scheme. We were able to acquire, in one hour at a radiation wavelength of 2.49 nm, an image of 50 nm spatial resolution.

  15. Resolving the origin of the diffuse soft X-ray background

    SciTech Connect

    Smith, Randall K.; Foster, Adam R.; Edgar, Richard J.; Brickhouse, Nancy S.

    2014-05-20

    The ubiquitous diffuse soft (1/4 keV) X-ray background was one of the earliest discoveries of X-ray astronomy. At least some of the emission may arise from charge exchange between solar wind ions and neutral atoms in the heliosphere, but no detailed models have been fit to the available data. Here, we report on a new model for charge exchange in the solar wind, which, when combined with a diffuse hot plasma component, filling the Local Cavity provides a good fit to the only available high-resolution soft X-ray and extreme ultraviolet spectra using plausible parameters for the solar wind. The implied hot plasma component is in pressure equilibrium with the local cloud that surrounds the solar system, creating for the first time a self-consistent picture of the local interstellar medium.

  16. Ultra-soft x-ray absorption spectroscopy: A bulk and surface probe of materials

    SciTech Connect

    Fischer, D.A. ); Mitchell, G.E.; Dekoven, B.M. ); Yeh, A.T.; Gland, J.L. ); Moodenbaugh, A.R. )

    1993-01-01

    Direct comparisons between surface and bulk of diverse materials can be made by simultaneous electron yield (5 nm depth sensitivity) and fluorescence yield (200 nm) ultra soft x-ray absorption spectroscopy measurements utilizing a rapid sample interchange apparatus. For example the orientations of functional groups have been characterized at and near the surface of a series of model polymeric materials highlighting the chemical and molecular sensitivity of ultra soft x-ray absorption spectroscopy. In addition we discuss a bulk sensitive use of fluorescence yield to non destructively study a buried metal polymer interface. A second bulk sensitive example is the use of fluorescence yield oxygen K near edge x-ray spectroscopy as a method to determine the hole state density of high Tc materials.

  17. Ultra-soft x-ray absorption spectroscopy: A bulk and surface probe of materials

    SciTech Connect

    Fischer, D.A.; Mitchell, G.E.; Dekoven, B.M.; Yeh, A.T.; Gland, J.L.; Moodenbaugh, A.R.

    1993-06-01

    Direct comparisons between surface and bulk of diverse materials can be made by simultaneous electron yield (5 nm depth sensitivity) and fluorescence yield (200 nm) ultra soft x-ray absorption spectroscopy measurements utilizing a rapid sample interchange apparatus. For example the orientations of functional groups have been characterized at and near the surface of a series of model polymeric materials highlighting the chemical and molecular sensitivity of ultra soft x-ray absorption spectroscopy. In addition we discuss a bulk sensitive use of fluorescence yield to non destructively study a buried metal polymer interface. A second bulk sensitive example is the use of fluorescence yield oxygen K near edge x-ray spectroscopy as a method to determine the hole state density of high Tc materials.

  18. Compact high-resolution differential interference contrast soft x-ray microscopy

    SciTech Connect

    Bertilson, Michael C.; Hofsten, Olov von; Lindblom, Magnus; Hertz, Hans M.; Vogt, Ulrich

    2008-02-11

    We demonstrate high-resolution x-ray differential interference contrast (DIC) in a compact soft x-ray microscope. Phase contrast imaging is enabled by the use of a diffractive optical element objective which is matched to the coherence conditions in the microscope setup. The performance of the diffractive optical element objective is evaluated in comparison with a normal zone plate by imaging of a nickel siemens star pattern and linear grating test objects. Images obtained with the DIC optic exhibit typical DIC enhancement in addition to the normal absorption contrast. Contrast transfer functions based on modulation measurements in the obtained images show that the DIC optic gives a significant increase in contrast without reducing the spatial resolution. The phase contrast operation mode now available for our compact soft x-ray microscope will be a useful tool for future studies of samples with low absorption contrast.

  19. Spatial and spectral features of soft diffuse X ray background seen by the Einstein observatory

    NASA Technical Reports Server (NTRS)

    Micela, G.; Harnden, F. R.; Rosner, R., Jr.; Sciortino, S.; Vaiana, G. S.

    1989-01-01

    A survey of the diffuse soft X-ray background as seen directly by the Einstein Observatory Imaging Proportional Counter (IPC) is presented. A source free region of the detector 1 by 1 degree field is used. The background in the 0.16 to 3.5 keV spectral region is viewed. The data covers roughly 5 percent of the sky, with some bias in coverage towards the galactic plane. The moderate energy resolution of the IPC enables the characterization and the production of maps of the background as a function of energy within the Einstein passband. The results are compared with previous observations of the diffuse X-ray background. The implications for galactic structure and for the soft component of the extragalactic X-ray background are discussed.

  20. XAFS Measurements under Atmospheric Pressure in the Soft X-ray Region

    SciTech Connect

    Nakanishi, Koji; Ohta, Toshiaki; Yagi, Shinya

    2010-06-23

    We have developed a compact experimental set-up for X-ray absorption fine structure (XAFS) measurements in He at atmospheric pressure (AP) in the soft X-ray region and used it for Mg and Cl K-edge XAFS measurements of MgCl{sub 2} and MgCl{sub 2{center_dot}}6H{sub 2}O. The spectra of MgCl{sub 2{center_dot}}6H{sub 2}O measured in He at AP were significantly different from those measured in vacuum. This suggests the importance of performing soft X-ray XAFS experiments under AP to obtain reliable spectra from hydrated compounds.

  1. Tomographic reconstruction in soft x-ray microscopy using focus-stack back-projection.

    PubMed

    Selin, Mårten; Fogelqvist, Emelie; Werner, Stephan; Hertz, Hans M

    2015-05-15

    Tomographic reconstruction in soft x-ray microscopy is a powerful technique for obtaining high-resolution 3D images of biological samples. However, the depth of focus of such zone-plate-based microscopes is typically shorter than the thickness of many relevant biological objects, challenging the validity of the projection assumption used in conventional reconstruction algorithms. In order to make full use of the soft x-ray microscopes' high resolution, the tomographic reconstruction needs to take the depth of focus into account. Here we present a method to achieve high resolution in the full sample when the depth of focus is short compared to the sample thickness. The method relies on the back-projection of focus-stacked image data from x-ray microscopy. We demonstrate the method on theoretical and experimental data. PMID:26393699

  2. Investigation on Soft X-Ray Lasers with a Picosecond-Laser-Irradiated Gas Puff Target

    SciTech Connect

    Fiedorowiez, H; Bartnik, A; Jarocki, R; Rakowski, R; Dunn, J; Smith, R F; Hunter, J; Hilsen, J; Shlyaptsev, V N

    2002-10-09

    We present results of experimental studies on transient gain soft x-ray lasers with a picosecond-laser-irradiated gas puff target. The target in a form of an elongated gas sheet is formed by pulsed injection of gas through a slit nozzle using a high-pressure electromagnetic valve developed and characterized at the Institute of Optoelectronics. The x-ray laser experiments were performed at the Lawrence Livermore National Laboratory using the tabletop Compact Multipulse Terawatt (COMET) laser to irradiate argon, krypton or xenon gas puff targets. Soft x-ray lasing in neon-like argon on the 3p-3s transition at 46.9 nm and the 3d-3p transition at 45.1 nm have been demonstrated, however, no amplification for nickel-like krypton or xenon was observed. Results of the experiments are presented and discussed.

  3. Soft X-Ray Irradiation of Silicates: Implications for Dust Evolution in Protoplanetary Disks

    NASA Astrophysics Data System (ADS)

    Ciaravella, A.; Cecchi-Pestellini, C.; Chen, Y.-J.; Muñoz Caro, G. M.; Huang, C.-H.; Jiménez-Escobar, A.; Venezia, A. M.

    2016-09-01

    The processing of energetic photons on bare silicate grains was simulated experimentally on silicate films submitted to soft X-rays of energies up to 1.25 keV. The silicate material was prepared by means of a microwave assisted sol-gel technique. Its chemical composition reflects the Mg2SiO4 stoichiometry with residual impurities due to the synthesis method. The experiments were performed using the spherical grating monochromator beamline at the National Synchrotron Radiation Research Center in Taiwan. We found that soft X-ray irradiation induces structural changes that can be interpreted as an amorphization of the processed silicate material. The present results may have relevant implications in the evolution of silicate materials in X-ray-irradiated protoplanetary disks.

  4. Tomographic reconstruction in soft x-ray microscopy using focus-stack back-projection.

    PubMed

    Selin, Mårten; Fogelqvist, Emelie; Werner, Stephan; Hertz, Hans M

    2015-05-15

    Tomographic reconstruction in soft x-ray microscopy is a powerful technique for obtaining high-resolution 3D images of biological samples. However, the depth of focus of such zone-plate-based microscopes is typically shorter than the thickness of many relevant biological objects, challenging the validity of the projection assumption used in conventional reconstruction algorithms. In order to make full use of the soft x-ray microscopes' high resolution, the tomographic reconstruction needs to take the depth of focus into account. Here we present a method to achieve high resolution in the full sample when the depth of focus is short compared to the sample thickness. The method relies on the back-projection of focus-stacked image data from x-ray microscopy. We demonstrate the method on theoretical and experimental data.

  5. Soft X-Ray Imaging of spin dynamics at high spatial and temporalresolution

    SciTech Connect

    Mesler, Brooke L.; Fischer, Peter; Chao, Weilun; Anderson, Erik H.

    2007-06-01

    Soft X-ray microscopy provides element specific magnetic imaging with a spatial resolution down to 15nm. At XM-1, the full-field soft X-ray microscope at the Advanced Light Source in Berkeley, a stroboscopic pump and probe setup has been developed to study fast magnetization dynamics in ferromagnetic elements with a time resolution of 70ps which is set by the width of the X-ray pulses from the synchrotron. Results obtained with a 2 {micro}m x 4 {micro}m x 45nm rectangular permalloy sample exhibiting a seven domain Landau pattern reveal dynamics up to several nsec after the exciting magnetic field pulse. Domain wall motion, a gyrotropic vortex motion, and a coupling between vortices in the rectangular geometry are observed.

  6. Soft X-Ray Irradiation of Silicates: Implications for Dust Evolution in Protoplanetary Disks

    NASA Astrophysics Data System (ADS)

    Ciaravella, A.; Cecchi-Pestellini, C.; Chen, Y.-J.; Muñoz Caro, G. M.; Huang, C.-H.; Jiménez-Escobar, A.; Venezia, A. M.

    2016-09-01

    The processing of energetic photons on bare silicate grains was simulated experimentally on silicate films submitted to soft X-rays of energies up to 1.25 keV. The silicate material was prepared by means of a microwave assisted sol–gel technique. Its chemical composition reflects the Mg2SiO4 stoichiometry with residual impurities due to the synthesis method. The experiments were performed using the spherical grating monochromator beamline at the National Synchrotron Radiation Research Center in Taiwan. We found that soft X-ray irradiation induces structural changes that can be interpreted as an amorphization of the processed silicate material. The present results may have relevant implications in the evolution of silicate materials in X-ray-irradiated protoplanetary disks.

  7. State transition in soft X-ray transients: "To be or not to be"

    NASA Astrophysics Data System (ADS)

    Maitra, Dipankar

    2006-02-01

    One of the most intriguing challenges in high-energy astrophysics has been understanding the dynamics of accretion flow onto compact objects. X-ray binaries exhibit many different patterns of accretion flow, manifested as "X- ray states". Various states show dramatically different spectral energy distributions and temporal behavior. In particular, two canonical states are seen in most X-ray binaries---a "soft" state characterized by strong thermal emission and low variability in the light curve, and a "hard" state characterized by nonthermal power law emission and high variability. Besides these canonical states, a variety of intermediate and extreme states are also seen often. A complete understanding of these X-ray states is essential not only to understand the physical mechanisms associated with the different types of accretion flows, but also in enabling one to test physics in the regime of strong-field general relativity. While it is generally known that the mass accretion rate onto the compact object influences a transition from one state to another, recent observations have shown that there are additional factors that determine the state of a source. In this dissertation, I have used X-ray spectral and temporal information from neutron star and black hole systems to explore the factors that might be contributing towards a state transition. The X-ray data were obtained using the Rossi X-ray Timing Explorer (RXTE) satellite, triggered by our optical/near-IR monitoring of X-ray binaries using the CTIO 1.3m telescope operated by SMARTS consortium. I have also used data from our long-term (~ 8 years) optical/near-IR monitoring of the neutron star system Aql X-1 to show that the outer accretion disk heats up like a simple blackbody during the course of evolution of an outburst. Optical data, along with soft-X-ray data from the All Sky Monitor aboard RXTE, demonstrated that besides the canonical "fast-rise and exponential-decay" (FRED) lightcurve morphology seen

  8. Specular and diffuse reflection of soft x-rays from mirrors

    SciTech Connect

    Hogrefe, H.; Haelbich, R.P.; Kunz, C.

    1985-08-01

    Measurements of surface scattering from plane mirrors with different degrees of roughness using soft x-rays are reported. Angle resolved distributions of s-polarized light, scattered in the plane of incidence, were obtained with a precise reflectometer for various angles of incidence and different wavelengths. The influence of the sample preparation and the optical constants on the scattering properties is shown.

  9. A Laboratory-Scale Coaxial Fluorescence and Soft X-ray Microscope for Biological Observation

    NASA Astrophysics Data System (ADS)

    Takaba, K.; Aoki, S.

    2011-09-01

    A laboratory-scale coaxial fluorescence and soft x-ray microscope for biological observation was developed. The characteristic features of a fluorescence microscope were introduced to the conventional soft x-ray microscope, which was developed in our previous study, where the specimens can be set in air. One of the technical difficulties in detecting visible fluorescence is the chromatic aberration. This was overcome by applying a reflective optics, Wolter mirror, to the coaxial optical system. The coaxial optical system offers experimental simplicity and makes it possible to obtain soft x-ray images and fluorescence images of an identical specimen, which can be more informative than applying either imaging modality alone. Therefore, the newly developed optical system offers high-quality structural and morphological details of biological specimens with the ability to localize specific cells and other important sub-cellular targets. Soft x-ray images and fluorescence images of an identical DNA, which were derived from redfish testes and stained with DAPI (4', 6-diamidino-2-phenylindole), were obtained by the newly developed coaxial optical system.

  10. Soft-x-ray projection lithography experiments using Schwarzschild imaging optics

    SciTech Connect

    Tichenor, D.A.; Kubiak, G.D.; Malinowski, M.E.; Stulen, R.H.; Haney, S.J.; Berger, K.W.; Brown, L.A. ); Sweatt, W.C. ); Bjorkholm, J.E.; Freeman, R.R.; Himel, M.D.; MacDowell, A.A.; Tennant, D.M.; Wood II, O.R. ); Bokor, J.; Jewell, T.E.; Mansfield, W.M.; Waskiewicz, W.K.; White, D.L.; Windt, D.L. )

    1993-12-01

    Soft-x-ray projection imaging is demonstrated by the use of 14-nm radiation from a laser plasma source and a single-surface multilayer-coated ellipsoidal condenser. Aberrations in the condenser and the Schwarzschild imaging objective are characterized and correlated with imaging performance. A new Schwarzschild housing, designed for improved alignment stability, is described.

  11. Soft X-ray spectrum of laser-produced aluminum plasma

    SciTech Connect

    Vergunova, G. A.; Grushin, A. S.; Kologrivov, A. A.; Novikov, V. G.; Osipov, M. V.; Puzyrev, V. N. Rozanov, V. B. Starodub, A. N. Yakushev, O. F.

    2015-05-15

    Soft X-ray spectra (30–70 Å) of aluminum plasma have been measured in experiments carried out at the Kanal-2 laser facility at laser intensities of (1–7) × 10{sup 13} W/cm{sup 2}. It is shown that the measured spectra satisfactory agree with those calculated using the RADIAN numerical code.

  12. A soft x-ray undulator for the U5 beamline at NSLS

    SciTech Connect

    Viccaro, P.J.; Shenoy, G.K.; Kim, S.H.; Bader, S.D.

    1988-10-01

    The magnetic structure and spectral properties of a 7.5-cm, 30-period hybrid undulator are described. The device will be installed at the U5 port of the VUV storage ring at Brookhaven National Laboratory and will be a tunable source of very high brilliance soft x-ray radiation over the range of 13 from approximately 150 eV.

  13. Utilizing ablation of solids to characterize a focused soft X-ray laser beam

    NASA Astrophysics Data System (ADS)

    Chalupský, J.; Juha, L.; Kuba, J.; Hájková, V.; Cihelka, J.; Homer, P.; Kozlová, M.; Mocek, T.; Polan, J.; Rus, B.; Krzywinsky, J.; Sobierajski, R.; Wabnitz, H.; Feldhaus, J.; Tiedtke, K.; the, And

    2007-05-01

    An advanced time integrated method has been developed for soft X-ray pulsed laser beam characterization. A technique based on poly (methyl methacrylate) - PMMA laser induced ablation has been used for beam investigations of soft X-ray laser sources like FLASH (Free-electron LASer in Hamburg; formerly known as VUV FEL and/or TTF2 FEL) and plasma-based Ne-like Zn laser performed at PALS (Prague Asterix Laser System). For the interaction experiments reported here, the FLASH system provided ultra-short pulses (~10-fs) of 21.7-nm radiation. The PMMA ablation was also induced by plasma-based Ne-like Zn soft X-ray laser pumped by NIR beams at the PALS facility. This quasi-steady-state (QSS) soft X-ray laser provides 100-ps pulses of 21.2-nm radiation, i.e. at a wavelength very close to that of FLASH but with about 5,000 times longer pulses. In both cases, the PMMA samples were irradiated by a single shot with a focused beam under normal incidence conditions. Characteristics of ablated craters obtained with AFM (Atomic Force Microscope) and Nomarski microscopes were utilized for profile reconstruction and diameter determination of the focused laser beams ablating the PMMA surface.

  14. Soft Gamma Repeaters and Anomalous X-ray Pulsars: Magnetar Candidates

    NASA Technical Reports Server (NTRS)

    Woods, P. M.; Thompson, C.

    2005-01-01

    This article is a review of Soft Gamma Repeaters and Anomalous X-ray Pulsars. It contains a brief historical record of the emergence of these classes of neutron stars, a thorough overview of the observational data, a succinct summary of the magnetar model, and suggested directions for future research in this field.

  15. Generation of intense coherent soft x-ray with electron microbunches induced and frozen by lasers

    SciTech Connect

    Yu. L.H.

    1983-01-01

    We describe a new improved version of Transverse Optical Klystron Harmonic Generator that uses three lasers to replace the undulators in the modulator and radiator and freeze the electron microbunching. We show that intense soft x-rays can be generated.

  16. A surface recombination model applied to large features in inorganic phosphor efficiency measurements in the soft x-ray region

    NASA Astrophysics Data System (ADS)

    Benitez, E. L.; Husk, D. E.; Schnatterly, S. E.; Tarrio, C.

    1991-09-01

    The photoluminescent quantum efficiencies of the inorganic phosphors Y2O2S:Eu, Y2O3:Eu, La2O2S:Tm, Gd2O2S:Tb, and Sr5Cl(PO4)3:Eu have been measured in the range 17 to 450 eV. The optical properties of these phosphors from 2 to 160 eV have been determined from inelastic electron scattering measurements. Using a model which involves nonradiative recombination at the surface of the material, we relate photoluminescent efficiency to optical absorption properties, and find that surface recombination is the predominant source of efficiency loss for these materials in the soft x-ray range. From the model, we obtain values for the diffusion length, surface recombination velocity, and bulk quantum efficiency of these materials.

  17. Soft X-ray spectromicroscopy for speciation, quantitation and nano-eco-toxicology of nanomaterials.

    PubMed

    Lawrence, J R; Swerhone, G D W; Dynes, J J; Korber, D R; Hitchcock, A P

    2016-02-01

    There is a critical need for methods that provide simultaneous detection, identification, quantitation and visualization of nanomaterials at their interface with biological and environmental systems. The approach should allow speciation as well as elemental analysis. Using the intrinsic X-ray absorption properties, soft X-ray scanning transmission X-ray spectromicroscopy (STXM) allows characterization and imaging of a broad range of nanomaterials, including metals, oxides and organic materials, and at the same time is able to provide detailed mapping of biological components. Thus, STXM offers considerable potential for application to research on nanomaterials in biology and the environment. The potential and limitations of STXM in this context are discussed using a range of examples, focusing on the interaction of nanomaterials with microbial cells, biofilms and extracellular polymers. The studies outlined include speciation and mapping of metal-containing nanomaterials (Ti, Ni, Cu) and carbon-based nanomaterials (multiwalled carbon nanotubes, C60 fullerene). The benefits of X-ray fluorescence detection in soft X-ray STXM are illustrated with a study of low levels of Ni in a natural river biofilm.

  18. Overview of nanoscale NEXAFS performed with soft X-ray microscopes

    PubMed Central

    Bittencourt, Carla

    2015-01-01

    Summary Today, in material science nanoscale structures are becoming more and more important. Not only for the further miniaturization of semiconductor devices like carbon nanotube based transistors, but also for newly developed efficient energy storage devices, gas sensors or catalytic systems nanoscale and functionalized materials have to be analysed. Therefore, analytical tools like near-edge X-ray absorption fine structure (NEXAFS) spectroscopy has to be applied on single nanostructures. Scanning transmission X-ray microscopes (STXM) as well as full-field transmission X-ray microscopes (TXM) allow the required spatial resolution to study individual nanostructures. In the soft X-ray energy range only STXM was used so far for NEXAFS studies. Due to its unique setup, the TXM operated by the Helmholtz-Zentrum Berlin (HZB) at the electron storage ring BESSY II is the first one in the soft X-ray range which can be used for NEXAFS spectroscopy studies which will be shown in this review. Here we will give an overview of the different microscopes used for NEXAFS studies and describe their advantages and disadvantages for different samples. PMID:25821700

  19. Overview of nanoscale NEXAFS performed with soft X-ray microscopes.

    PubMed

    Guttmann, Peter; Bittencourt, Carla

    2015-01-01

    Today, in material science nanoscale structures are becoming more and more important. Not only for the further miniaturization of semiconductor devices like carbon nanotube based transistors, but also for newly developed efficient energy storage devices, gas sensors or catalytic systems nanoscale and functionalized materials have to be analysed. Therefore, analytical tools like near-edge X-ray absorption fine structure (NEXAFS) spectroscopy has to be applied on single nanostructures. Scanning transmission X-ray microscopes (STXM) as well as full-field transmission X-ray microscopes (TXM) allow the required spatial resolution to study individual nanostructures. In the soft X-ray energy range only STXM was used so far for NEXAFS studies. Due to its unique setup, the TXM operated by the Helmholtz-Zentrum Berlin (HZB) at the electron storage ring BESSY II is the first one in the soft X-ray range which can be used for NEXAFS spectroscopy studies which will be shown in this review. Here we will give an overview of the different microscopes used for NEXAFS studies and describe their advantages and disadvantages for different samples. PMID:25821700

  20. A new streaked soft x-ray imager for the National Ignition Facility

    DOE PAGES

    Benstead, J.; Moore, A. S.; Ahmed, M. F.; Morton, J.; Guymer, T. M.; Pardini, T.; Soufli, R.; Hibbard, R. L.; Bailey, C. G.; Bell, P. M.; et al

    2016-05-27

    Here, a new streaked soft x-ray imager has been designed for use on high energy-density (HED) physics experiments at the National Ignition Facility based at the Lawrence Livermore National Laboratory. This streaked imager uses a slit aperture, single shallow angle reflection from a nickel mirror, and soft x-ray filtering to, when coupled to one of the NIF’s x-ray streak cameras, record a 4× magnification, one-dimensional image of an x-ray source with a spatial resolution of less than 90 μm. The energy band pass produced depends upon the filter material used; for the first qualification shots, vanadium and silver-on-titanium filters weremore » used to gate on photon energy ranges of approximately 300–510 eV and 200–400 eV, respectively. A two-channel version of the snout is available for x-ray sources up to 1 mm and a single-channel is available for larger sources up to 3 mm. Both the one and two-channel variants have been qualified on quartz wire and HED physics target shots.« less

  1. A new streaked soft x-ray imager for the National Ignition Facility.

    PubMed

    Benstead, J; Moore, A S; Ahmed, M F; Morton, J; Guymer, T M; Soufli, R; Pardini, T; Hibbard, R L; Bailey, C G; Bell, P M; Hau-Riege, S; Bedzyk, M; Shoup, M J; Reagan, S; Agliata, T; Jungquist, R; Schmidt, D W; Kot, L B; Garbett, W J; Rubery, M S; Skidmore, J W; Gullikson, E; Salmassi, F

    2016-05-01

    A new streaked soft x-ray imager has been designed for use on high energy-density (HED) physics experiments at the National Ignition Facility based at the Lawrence Livermore National Laboratory. This streaked imager uses a slit aperture, single shallow angle reflection from a nickel mirror, and soft x-ray filtering to, when coupled to one of the NIF's x-ray streak cameras, record a 4× magnification, one-dimensional image of an x-ray source with a spatial resolution of less than 90 μm. The energy band pass produced depends upon the filter material used; for the first qualification shots, vanadium and silver-on-titanium filters were used to gate on photon energy ranges of approximately 300-510 eV and 200-400 eV, respectively. A two-channel version of the snout is available for x-ray sources up to 1 mm and a single-channel is available for larger sources up to 3 mm. Both the one and two-channel variants have been qualified on quartz wire and HED physics target shots. PMID:27250473

  2. iWF-MAXI: Soft X-ray Transient Monitor on the ISS

    NASA Astrophysics Data System (ADS)

    Kawai, Nobuyuki; Tomida, Hiroshi; Ueno, Shiro; Kimura, Masashi; Ebisawa, Ken; Yatsu, Yoichi; Arimoto, Makoto; Mihara, Tatehiro; Serino, Motoko; Tsunemi, Hiroshi; Kohmura, Takayoshi; Sakamoto, Takanori; Negoro, Hitoshi; Ueda, Yoshihiro; Tsuboi, Yohko; Yoshida, Atsumasa

    2015-08-01

    iWF-MAXI is an X-ray transient monitor mission proposed for the ISS/JEM, starting in 2018-2019.It has four main scientific goals:(1) To find and localize the X-ray counterparts of gravitational wave events, which are expected to be detected by the next generation gravitational wave detectors such as Advance LIGO and KAGRA in late 2010's.(2) To detect short soft X-ray transients such as stellar flares, nova ignitions, and supernova shock breakouts, and promptly notify the world.(3) To trigger on short high-energy transients such as gamma-ray bursts and tidal disruption events, and promptly disseminate their locations to the community.(4) To detect the onset of activities from black hole binaries, neutron star binaries, and active galactic nuclei (AGN), and issue alerts to the astronomical community of the world.Its main scientific instrument is the Soft X-ray Large Solid Angle Camera (SLC). It is sensitive in the energy range of 0.7--10 keV with a localization accuracy of 0.1 degres. It will detect short transient events like GRBs with durations from a fraction of a second to minutes that occur in its large large field of view (>10% of the entire sky) .With the orbital revolution of the ISS, iWF-MAXI scans much larger sky area in 90 minutes, and looks for slower events such as outbursts of X-ray binaries.

  3. Dissociation of the benzene molecule by ultraviolet and soft X-rays in circumstellar environment

    NASA Astrophysics Data System (ADS)

    Boechat-Roberty, H. M.; Neves, R.; Pilling, S.; Lago, A. F.; de Souza, G. G. B.

    2009-04-01

    Benzene molecules, present in the proto-planetary nebula CRL 618, are ionized and dissociated by ultraviolet (UV) and X-ray photons originated from the hot central star and by its fast wind. Ionic species and free radicals produced by these processes can lead to the formation of new organic molecules. The aim of this work is to study the photoionization and photodissociation processes of the benzene molecule, using synchrotron radiation and time-of-flight mass spectrometry. Mass spectra were recorded at different energies corresponding to the vacuum UV (21.21 eV) and soft X-ray (282-310 eV) spectral regions. The production of ions from the benzene dissociative photoionization is here quantified, indicating that C6H6 is more efficiently fragmented by soft X-ray than UV radiation, where 50 per cent of the ionized benzene molecules survive to UV dissociation while only about 4 per cent resist to X-rays. Partial ion yields of H+ and small hydrocarbons, such as C2H+2, C3H+3, C4H+2, are determined as a function of photon energy. Absolute photoionization and dissociative photoionization cross-sections have also been determined. From these values, half-life of benzene molecule due to UV and X-ray photon fluxes in CRL 618 was obtained.

  4. Overview of nanoscale NEXAFS performed with soft X-ray microscopes.

    PubMed

    Guttmann, Peter; Bittencourt, Carla

    2015-01-01

    Today, in material science nanoscale structures are becoming more and more important. Not only for the further miniaturization of semiconductor devices like carbon nanotube based transistors, but also for newly developed efficient energy storage devices, gas sensors or catalytic systems nanoscale and functionalized materials have to be analysed. Therefore, analytical tools like near-edge X-ray absorption fine structure (NEXAFS) spectroscopy has to be applied on single nanostructures. Scanning transmission X-ray microscopes (STXM) as well as full-field transmission X-ray microscopes (TXM) allow the required spatial resolution to study individual nanostructures. In the soft X-ray energy range only STXM was used so far for NEXAFS studies. Due to its unique setup, the TXM operated by the Helmholtz-Zentrum Berlin (HZB) at the electron storage ring BESSY II is the first one in the soft X-ray range which can be used for NEXAFS spectroscopy studies which will be shown in this review. Here we will give an overview of the different microscopes used for NEXAFS studies and describe their advantages and disadvantages for different samples.

  5. A new streaked soft x-ray imager for the National Ignition Facility.

    PubMed

    Benstead, J; Moore, A S; Ahmed, M F; Morton, J; Guymer, T M; Soufli, R; Pardini, T; Hibbard, R L; Bailey, C G; Bell, P M; Hau-Riege, S; Bedzyk, M; Shoup, M J; Reagan, S; Agliata, T; Jungquist, R; Schmidt, D W; Kot, L B; Garbett, W J; Rubery, M S; Skidmore, J W; Gullikson, E; Salmassi, F

    2016-05-01

    A new streaked soft x-ray imager has been designed for use on high energy-density (HED) physics experiments at the National Ignition Facility based at the Lawrence Livermore National Laboratory. This streaked imager uses a slit aperture, single shallow angle reflection from a nickel mirror, and soft x-ray filtering to, when coupled to one of the NIF's x-ray streak cameras, record a 4× magnification, one-dimensional image of an x-ray source with a spatial resolution of less than 90 μm. The energy band pass produced depends upon the filter material used; for the first qualification shots, vanadium and silver-on-titanium filters were used to gate on photon energy ranges of approximately 300-510 eV and 200-400 eV, respectively. A two-channel version of the snout is available for x-ray sources up to 1 mm and a single-channel is available for larger sources up to 3 mm. Both the one and two-channel variants have been qualified on quartz wire and HED physics target shots.

  6. A compact soft X-ray microscope using an electrode-less Z-pinch source

    NASA Astrophysics Data System (ADS)

    Horne, S. F.; Silterra, J.; Holber, W.

    2009-09-01

    Soft X-rays (< 1Kev) are of medical interest both for imaging and microdosimetry applications. X-ray sources at this low energy present a technological challenge. Synchrotrons, while very powerful and flexible, are enormously expensive national research facilities. Conventional X-ray sources based on electron bombardment can be compact and inexpensive, but low x-ray production efficiencies at low electron energies restrict this approach to very low power applications. Laser-based sources tend to be expensive and unreliable. Energetiq Technology, Inc. (Woburn, MA, USA) markets a 92 eV, 10W(2pi sr) electrode-less Z-pinch source developed for advanced semiconductor lithography. A modified version of this commercial product has produced 400 mW at 430 eV (2pi sr), appropriate for water window soft X-ray microscopy. The US NIH has funded Energetiq to design and construct a demonstration microscope using this source, coupled to a condenser optic, as the illumination system. The design of the condenser optic matches the unique characteristics of the source to the illumination requirements of the microscope, which is otherwise a conventional design. A separate program is underway to develop a microbeam system, in conjunction with the RARAF facility at Columbia University, NY, USA. The objective is to develop a focused, sub-micron beam capable of delivering > 1 Gy/second to the nucleus of a living cell. While most facilities of this type are coupled to a large and expensive particle accelerator, the Z-pinch X-ray source enables a compact, stand-alone design suitable to a small laboratory. The major technical issues in this system involve development of suitable focusing X-ray optics. Current status of these programs will be reported. (Supported by NIH grants 5R44RR022488-03 and 5R44RR023753-03)

  7. Soft x-ray generation in gases with an ultrashort pulse laser

    SciTech Connect

    Ditmire, T R

    1996-01-08

    An experimental investigation of soft x-ray production resulting from the interaction of intense near infra-red laser radiation with gases is presented in this thesis. Specifically, soft x-ray generation through high order harmonic generation or exploiting intense inverse bremsstrahlung heating is examined. Most of these studies are conducted with femtosecond, terawatt class Cr:LiSrAlF{sub 6} (LiSAF) laser, though results derived from studies with other laser systems are presented as well. The majority of this work is devoted to experimental investigations, however, theoretical and computational models are developed to interpret the data. These studies are motivated by the possibility of utilizing the physics of intense laser/matter interactions as a potential compact source of bright x-rays. Consequently, the thrust of many of the experiments conducted is aimed at characterizing the x-rays produced for possible use in applications. In general, the studies of this manuscript fall into three categories. First, a unique 130 fs, 8 TW laser that is based on chirped pulse amplification, is described, and its performance is evaluated. The generation of x-rays through high order harmonics is then discussed with emphasis on characterizing and optimizing harmonic generation. Finally, the generation of strong, incoherent x-ray radiation by the intense irradiation of large (>1,000 atom) clusters in gas jets, is explored. The physics of laser energy absorption by clusters illuminated with intensities of 10{sup 15} to 10{sup 17} W/cm{sup 2} is considered in detail. X-ray spectroscopy of the hot plasmas that result from the irradiation of the clusters is conducted, and energy transport and kinetics issues in these plasmas are discussed.

  8. Development of the ASTRO-H Soft X-ray Telescope (SXT): Engineering Model Performance

    NASA Astrophysics Data System (ADS)

    Okajima, Takashi; Serlemitsos, P. J.; Soong, Y.

    2011-09-01

    The X-ray astronomy satellite, ASTRO-H, being developed under the collaboration among JAXA, NASA's GSFC and ESA, will have two Soft X-ray Telescopes (SXTs), among other instruments onboard, with a sensitive energy band up to 15 keV. One is for an X-ray micro-calorimeter detector and the other for an X-ray CCD detector. The SXT uses a conically approximated Wolter I grazing incidence optic implemented by thin aluminum foil substrates with thickness of 0.152, 0.229, and 0.305 mm. X-ray reflecting surface is a gold thin layer ( 2000A) transferred from a smooth glass mandrel to the substrate by a replication method using an epoxy buffer layer (12 um). It is similar to the Suzaku XRT, but with larger diameter (45 cm) and longer focal length (5.6 m). Goals of angular resolution and effective area are 1 arcmin and 390 cm2 at 6 keV, respectively. We made several improvements from Suzaku to ASTRO-H, such as thicker substrates, more forming mandrels, thinner epoxy layer for replication, stiffer housings, precise alignment bars, etc. With all these changes, we have fabricated the engineering test unit of the SXT. In this paper, we will discuss all the changes made, their effects, and report X-ray performance of the SXT test unit. An angular resolution of the test unit was measured at new Goddard X-ray calibration facility (100 m X-ray beamline) and was found to be 65 arcsec at 4.5 keV. We will also discuss further improvements toward the flight unit to be delivered to JAXA in 2012.

  9. Soft X-ray study of solar wind charge exchange from the Earth's magnetosphere : Suzaku observations and a future X-ray imaging mission concept

    NASA Astrophysics Data System (ADS)

    Ezoe, Y.; Ishisaki, Y.; Ohashi, T.; Ishikawa, K.; Miyoshi, Y.; Fujimoto, R.; Terada, N.; Kasahara, S.; Fujimoto, M.; Mitsuda, K.; Nishijo, K.; Noda, A.

    2013-12-01

    Soft X-ray observations of solar wind charge exchange (SWCX) emission from the Earth's magnetosphere using the Japanese X-ray astronomy satellite Suzaku are shown, together with our X-ray imaging mission concept to characterize the solar wind interaction with the magnetosphere. In recent years, the SWCX emission from the Earth's magnetosphere, originally discovered as unexplained noise during the soft X-ray all sky survey (Snowden et al. 1994), is receiving increased attention on studying geospace. The SWCX is a reaction between neutrals in exosphere and highly charged ions in the magnetosphere originated from solar wind. Robertson et al. (2005) modeled the SWCX emission as seen from an observation point 50 Re from Earth. In the resulting X-ray intensities, the magnetopause, bow shock and cusp were clearly visible. High sensitivity soft X-ray observation with CCDs onboard recent X-ray astronomy satellites enables us to resolve SWCX emission lines and investigate time correlation with solar wind as observed with ACE and WIND more accurately. Suzaku is the 5th Japanese X-ray astronomy satellite launched in 2005. The line of sight direction through cusp is observable, while constraints on Earth limb avoidance angle of other satellites often limits observable regions. Suzaku firstly detected the SWCX emission while pointing in the direction of the north ecliptic pole (Fujimoto et al. 2007). Using the Tsyganenko 1996 magnetic field model, the distance to the nearest SWCX region was estimated as 2-8 Re, implying that the line of sight direction can be through magnetospheric cusp. Ezoe et al. (2010) reported SWCX events toward the sub-solar side of the magnetosheath. These cusp and sub-solar side magnetosheath regions are predicted to show high SWCX fluxes by Robertson et al. (2005). On the other hand, Ishikawa et al. (2013) discovered a similarly strong SWCX event when the line of sight direction did not transverse these two regions. Motivated by these detections

  10. Soft X-Ray Luminosity and Photospheric Magnetic Field in Quiet Sun

    NASA Astrophysics Data System (ADS)

    Pevtsov, Alexei A.; Acton, Loren W.

    2001-06-01

    We use full-disk soft X-ray data from Yohkoh and Kitt Peak daily magnetograms to study the coronal irradiance and photospheric magnetic field remote from active regions between 1991 November and 1998 December. For every image of our data set we extract three areas 4°×4° in size centered at N00° W00°, N50° W00°, and S50° W00° and compute X-ray irradiance and unsigned magnetic flux for each of these areas. Between 1991 (active Sun) and 1996 (quiet Sun) the X-ray irradiance at the heliographic center decreased by more than a factor of 7, while the magnetic flux decreased by only a factor of 2. A similar tendency is observed for our high-latitude samples. Apart from the cycle-related variations, all three areas of quiet Sun exhibit significant nonperiodic changes in X-ray irradiance. These variations occur on 9-12 month intervals and clearly correlate with changes in sunspot activity. Similar variations are present in the total X-ray irradiance averaged over the solar disk. By contrast, the magnetic fluxes from the photosphere beneath these same areas show no corresponding variations on this time scale. In our opinion, coronal heating models based on the reconnection of quiet-Sun magnetic elements (variously called chromospheric network, ``magnetic carpet,'' or ``salt and pepper'' field) can at best account for a minimal contribution to heating the million-degree corona observed by the Yohkoh soft X-ray telescope. We conclude that the X-ray irradiance in the quiet Sun (at least in the Yohkoh temperature range, >2 MK) is primarily associated with the strong magnetic fields of active regions, not with weak photospheric fields. The association, however, is not direct. We interpret the enhanced X-ray irradiance above the quiet Sun not as a result of the coronal ``canopy'' formed by the active-region magnetic field above the quiet-Sun areas, but as the large-scale relaxation process in the corona triggered by the evolution of active regions. To further support this

  11. Low energy excitations in iridates studied with Resonant Inelastic X-ray Scattering

    NASA Astrophysics Data System (ADS)

    Liu, Xuerong

    2013-03-01

    In the iridium oxides, the strong spin-orbit coupling (SOC) of the 5d iridium electrons entangles the orbital and spin degrees of freedom, providing opportunities for exotic magnetic states with highly anisotropic exchange interactions. At the same time, the spatially extended 5d electrons are expected to have much stronger hybridization with the oxygen 2p orbitals, comparing with that in 3d transition element compounds. Both factors make crystal symmetry and local environment crucial in determining the electronic and magnetic properties of the iridates. We present here our resonant inelastic X-ray scattering (RIXS) studies of a number of octahedrally coordinated iridates with special structures, exploring these effects. In particular, for the 1-D spin 1/2 chain compound, Sr3CuIrO6, the wavefunction of the hole in the t2g manifold was reconstructed based on the RIXS spectra. Our results show that it is significantly modified from the isotropic shape expected for Jeff = 1 / 2 states in the strong SOC limit, due to the distortion of the oxygen octahedral cage. This distortion is comparable to, or smaller than, that present in most iridates and thus this work emphasizes the importance of local symmetry for the iridate families. Further, the magnetic excitations of this material were also measured. A large gap of ~30 meV, was found, comparable to the magnetic dispersion bandwidth. This is in contrast to the gapless dispersion expected for linear chain with isotropic Heisenberg exchange interaction. We also studied Na4Ir3O8 which has a hyperkagome lattice, and is a candidate quantum spin liquid. Here, a low energy continuum is observed below the d-d excitations. Optical conductivity measurements performed on the same sample and polarization dependence of the RIXS signal suggest that these excitations are magnetic in origin, agreeing with the spin-liquid state prediction. The work at Brookhaven was supported by the U.S. Department of Energy, Division of Materials Science

  12. A sample of active galactic nuclei with strong soft X-ray variabilities

    NASA Astrophysics Data System (ADS)

    Bi, Da; Liu, Teng; Wang, JunXian

    2015-04-01

    Large-amplitude X-ray variation is a special feature of AGN, reflecting possible extreme change in the central engine or the absorption along the line of sight. Till now there are only a few relevant studies on individual sources or rather small samples. In this work we aim to perform a systematic study of AGNs with strong soft X-ray variations at timescale of ≳ 10 years. To build the sample, we compare the soft X-ray fluxes of AGNs measured in ROSAT All-Sky Survey (RASS) during 1990-1991 with those measured by XMM-Newton during 2000-2009. This investigation bings forth to a sample of 13 AGNs, which appeared bright in RASS era, and went into low states (flux dropped by a factor of ≳ 10) when they were caught by XMM-Newton. Most of the 13 sources are type I Seyfert galaxies. 5 of them are noticed to have strong X-ray variation for the first time. We study the nature of their variations through performing XMM-Newton spectral analyses and by collecting reports from the existing literature. We find the sample could be divided into three categories according to the possible causes of the strong X-ray variations. The variations in MRK 0478 and 1H 0419-557 are consistent with strong light-bending effect, i.e., the observed X-ray flux drops significantly as the X-ray emitting corona gets much closer to the central black hole. The variations in ESO 140-G043 and NGC 7158 are caused by absorption changes along the line of sight. For one special case MRK 0335, the variation can be explained by either light-bending or absorption variation. In the rest 8 sources (˜ 60%), the strong soft X-ray variations are likely to exist due to intrinsic changes in the activities of the corona, although in some of them without high quality X-ray spectra we are unable to rule out alternative models. This sample provides good targets for future monitoring campaigns with more extensive studies.

  13. Soft x-ray-controlled dose deposition in yeast cells: techniques, model, and biological assessment

    NASA Astrophysics Data System (ADS)

    Milani, Marziale; Batani, Dimitri; Conti, Aldo; Masini, Alessandra; Costato, Michele; Pozzi, Achille; Turcu, I. C. Edmond

    1996-12-01

    A procedure is presented to release soft x-rays onto yeast cell membrane allegedly damaging the resident enzymatic processes connected with fermentation. The damage is expected to be restricted to regulating fermentation processes without interference with respiration. By this technique fermentation is followed leading to CO2 production, and respiration resulting in global pressure measurements. A solid state pressure sensor system has been developed linked to a data acquisition system. Yeast cells cultures have been investigated at different concentrations and with different nutrients. A non-monotone response in CO2 production as a function of the delivered x-ray dose is observed.

  14. Soft-x-ray emission spectroscopy study of the electronic structure of nonstoichiometric silicon nitride

    NASA Astrophysics Data System (ADS)

    Nithianandam, V. Jeyasingh; Schnatterly, S. E.

    1987-07-01

    Soft-x-ray emission spectroscopy was used to investigate the electronic structure of nonstoichiometric silicon nitride samples of different compositions. The Si L23 x-ray emission spectra from these samples are presented and interpreted using a two-phase linear superposition model for the valence-band region. We assumed a model for the valence-band edge and for the emission in the gap region due to trap states and the Si 2p core exciton. The results obtained from these fits are compared with relevant models and other experiments.

  15. Demonstration of 12 nm resolution Fresnel zone plate lens based soft x-ray microscopy

    SciTech Connect

    Chao, W.; Kim, J.; Rekawa, S.; Fischer, P.; Anderson, E. H.

    2009-06-05

    To extend soft x-ray microscopy to a resolution of order 10 nm or better, we developed a new nanofabrication process for Fresnel zone plate lenses. The new process, based on the double patterning technique, has enabled us to fabricate high quality gold zone plates with 12 nm outer zones. Testing of the zone plate with the full-field transmission x-ray microscope, XM-1, in Berkeley, showed that the lens clearly resolved 12 nm lines and spaces. This result represents a significant step towards 10 nm resolution and beyond.

  16. Iridium/Iridium Silicide as an Oxidation Resistant Capping Layer for Soft X-ray Mirrors

    SciTech Connect

    Prisbrey, S; Vernon, S

    2004-04-05

    Rust on a sword, tarnish on the silverware, and a loss in reflectivity for soft x-ray mirrors are all caused by oxidation that changes the desired characteristics of a material. Methods to prevent the oxidation have varied over the centuries with the default method of a protective coating being the most common. The protective coating for x-ray mirrors is usually a self-limiting oxidized layer on the surface of the material that stops further oxidation of the material by limiting the diffusion of oxygen to the material underneath.

  17. Optically Triggered RXTE Observations of Soft X-Ray Transients (core Program)

    NASA Astrophysics Data System (ADS)

    We propose to use optical/infra-red observations from the SMARTS consortium to trigger RXTE observations of transient soft X-ray binaries. We will trigger on two kinds of events: 1) a rise from quiescence; 2) state transitions during an outburst. These RXTE data, together with data from our already approved Swift program, radio ATCA observations and the SMARTS data themselves, will provide broad-band coverage in optical/IR and X-ray bandpasses, which will be used to study accretion processes and jets in black holes and neutron stars.

  18. Design of an imaging microscope for soft X-ray applications

    NASA Technical Reports Server (NTRS)

    Hoover, Richard B.; Shealy, David L.; Gabardi, David R.; Walker, Arthur B. C., Jr.; Lindblom, Joakim F.

    1988-01-01

    An imaging soft X-ray microscope with a spatial resolution of 0.1 micron and normal incidence multilayer optics is discussed. The microscope has a Schwarzschild configuration, which consists of two concentric spherical mirrors with radii of curvature which minimize third-order spherical aberration, coma, and astigmatism. The performance of the Stanford/MSFC Cassegrain X-ray telescope and its relevance to the present microscope are addressed. A ray tracing analysis of the optical system indicates that diffraction-limited performance can be expected for an object height of 0.2 mm.

  19. Soft X-ray emission from the Lupus Loop and Sn 1006 supernova remnants

    NASA Technical Reports Server (NTRS)

    Winkler, P. F., Jr.; Hearn, D. R.; Richardson, J. A.; Behnken, J. M.

    1979-01-01

    X-ray maps of the Lupus region have been obtained in a raster scan observation from SAS 3. These show the Lupus Loop to be a faint extended source of soft X-rays with a temperature about 2.5 million K. The most prominent feature of the region is the A.D. 1006 supernova remnant, which is unexpectedly bright at 0.2-1.0 keV. One speculative interpretation of the low-energy flux from SN 1006 is as blackbody radiation from a hot neutron star.

  20. Standing-wave excited soft x-ray photoemission microscopy: application to Co microdot magnetic arrays

    SciTech Connect

    Gray, Alexander; Kronast, Florian; Papp, Christian; Yang, See-Hun; Cramm, Stefan; Krug, Ingo P.; Salmassi, Farhad; Gullikson, Eric M.; Hilken, Dawn L.; Anderson, Erik H.; Fischer, Peter; Durr, Hermann A.; Schneider, Claus M.; Fadley, Charles S.

    2010-10-29

    We demonstrate the addition of depth resolution to the usual two-dimensional images in photoelectron emission microscopy (PEEM), with application to a square array of circular magnetic Co microdots. The method is based on excitation with soft x-ray standing-waves generated by Bragg reflection from a multilayer mirror substrate. Standing wave is moved vertically through sample simply by varying the photon energy around the Bragg condition. Depth-resolved PEEM images were obtained for all of the observed elements. Photoemission intensities as functions of photon energy were compared to x-ray optical calculations in order to quantitatively derive the depth-resolved film structure of the sample.

  1. Aplanatic Three-Mirror Objective for High-Magnification Soft X-Ray Microscopy

    SciTech Connect

    Toyoda, M.; Jinno, T.; Yanagihara, M.

    2011-09-09

    An innovative solution for high-magnification microscopy, based on attaching afocal optics for focal length reduction, is proposed. The solution, consisting of three spherical mirrors, allows one to enhance a magnification of a laboratory based soft x-ray microscope over 1000x, where movies with diffraction-limited resolution can be observed with an x-ray CCD. The design example, having a numerical aperture of 0.25, was successfully demonstrated both a high magnification and a large field of view.

  2. High-resolution multiwire proportional soft x-ray diagnostic measurements on TCV

    SciTech Connect

    Sushkov, A.; Andreev, V.; Camenen, Y.; Pochelon, A.; Klimanov, I.; Scarabosio, A.; Weisen, H.

    2008-02-15

    A multiwire proportional x-ray (MPX) detector is used on the TCV tokamak (Tokamak a configuration variable) as a high spatial and temporal resolution soft x-ray emissivity imaging diagnostic. The MPX system consists of 64 vertically viewing channels and has been designed to complement the existing TCV soft x-ray tomography system by enhancing the spatial resolution. The MPX detector is suitable for the measurement of fast and localized phenomena and can be used, for instance, for the observation of magnetohydrodynamic activity, for the characterization of transport barriers or for an improved determination of the electron cyclotron heating power deposition profile. The MPX detector operates in continuous-current mode and measures the plasma soft x-ray emission in the 3-30 keV range with a radial resolution of about 5 mm - 1% of plasma diameter - and a frequency bandwidth of 50 kHz. A detailed description of the MPX detector construction and the principle of its operation are given. The properties of the detector in photon-counting and continuous-current operation modes are studied. The implementation of the system on TCV and experimental results illustrating the potential of the diagnostic are also presented.

  3. Study of NbC thin films for soft X-ray multilayer applications

    SciTech Connect

    Singh, Amol E-mail: rrcat.amol@gmail.com; Modi, Mohammed H.; Lodha, G. S.; Rajput, Parasmani; Jha, S. N.

    2015-06-24

    Compound materials are being used in soft x-ray and Extreme ultraviolet (EUV) optics applications. Structural properties of compound materials changes drastically when ultrathin films are formed from bulk material. Structural properties need to be investigated to determine the suitability of compound materials in soft x-ray multilayer applications. In the present study Niobium carbide (NbC) thin films were deposited using ion beam sputtering of an NbC target on Si (100) substrate. Thickness roughness and film mass density was determined from the X-ray reflectivity (XRR) data. XRR data revealed that the film mass density was increasing with increase in film thickness. For 500Ǻ thick film, mass density of 6.85 g/cm{sup 3}, close to bulk density was found. Rms roughness for all the films was less than 10Å. Local structure of NbC thin films was determined from EXAFS measurements. The EXAFS data showed an increase in Nb-C and Nb-(C)-Nb peak ratio approaches towards bulk NbC with increasing thickness of NbC. From the present study, NbC thin films were found suitable for actual use in soft x-ray multilayer applications.

  4. Imaging interfacial micro- and nano-bubbles by scanning transmission soft X-ray microscopy.

    PubMed

    Zhang, Lijuan; Zhao, Binyu; Xue, Lian; Guo, Zhi; Dong, Yaming; Fang, Haiping; Tai, Renzhong; Hu, Jun

    2013-05-01

    Synchrotron-based scanning transmission soft X-ray microscopy (STXM) with nanometer resolution was used to investigate the existence and behavior of interfacial gas nanobubbles confined between two silicon nitride windows. The observed nanobubbles of SF6 and Ne with diameters smaller than 2.5 µm were quite stable. However, larger bubbles became unstable and grew during the soft X-ray imaging, indicating that stable nanobubbles may have a length scale, which is consistent with a previous report using atomic force microscopy [Zhang et al. (2010), Soft Matter, 6, 4515-4519]. Here, it is shown that STXM is a promising technique for studying the aggregation of gases near the solid/water interfaces at the nanometer scale.

  5. Probing single magnon excitations in Sr₂IrO₄ using O K-edge resonant inelastic x-ray scattering

    DOE PAGES

    Liu, X.; Dean, M. P. M.; Liu, J.; Chiuzbaian, S. G.; Jaouen, N.; Nicolaou, A.; Yin, W. G.; Rayan Serrao, C.; Ramesh, R.; Ding, H.; et al

    2015-04-28

    Resonant inelastic X-ray scattering (RIXS) at the L-edge of transition metal elements is now commonly used to probe single magnon excitations. Here we show that single magnon excitations can also be measured with RIXS at the K-edge of the surrounding ligand atoms when the center heavy metal elements have strong spin-orbit coupling. This is demonstrated with oxygen K-edge RIXS experiments on the perovskite Sr₂IrO₄, where low energy peaks from single magnon excitations were observed. This new application of RIXS has excellent potential to be applied to a wide range of magnetic systems based on heavy elements, for which the L-edgemore » RIXS energy resolutions in the hard X-ray region is usually poor.« less

  6. Probing single magnon excitations in Sr₂IrO₄ using O K-edge resonant inelastic x-ray scattering

    SciTech Connect

    Liu, X.; Dean, M. P. M.; Liu, J.; Chiuzbaian, S. G.; Jaouen, N.; Nicolaou, A.; Yin, W. G.; Rayan Serrao, C.; Ramesh, R.; Ding, H.; Hill, J. P.

    2015-04-28

    Resonant inelastic X-ray scattering (RIXS) at the L-edge of transition metal elements is now commonly used to probe single magnon excitations. Here we show that single magnon excitations can also be measured with RIXS at the K-edge of the surrounding ligand atoms when the center heavy metal elements have strong spin-orbit coupling. This is demonstrated with oxygen K-edge RIXS experiments on the perovskite Sr₂IrO₄, where low energy peaks from single magnon excitations were observed. This new application of RIXS has excellent potential to be applied to a wide range of magnetic systems based on heavy elements, for which the L-edge RIXS energy resolutions in the hard X-ray region is usually poor.

  7. Recent results in capillary discharge soft x-ray laser research

    NASA Astrophysics Data System (ADS)

    Rocca, Jorge J.; Marconi, Mario C.; Wang, Yong; Luther, Bradley M.; Pedacci, Francesco; Grisham, Michael; Vaschenko, Georgiy; Menoni, Carmen S.; Filevich, Jorge; Juha, Libor; Pershin, Yu. P.; Zubarev, E. N.; Voronov, D. L.; Sevryukova, V. A.; Kondratenko, V. V.; Shlyaptsev, Vyacheslav V.; Vinogradov, Alexander; Artioukov, Igor

    2003-12-01

    We report results of the development of capillary discharge driven metal-vapor plasma waveguides for the development of efficient laser-pumped soft x-ray lasers; and of the use of a previously developed capillary discharge Ne-like Ar 46.9 nm laser in study of the interaction of intense soft x-ray laser with materials. The guiding of a laser beam in a dense capillary discharge plasma channel containing a large density of Ag ions is reported. In term of applications we have conducted studies of materials modification and ablation with focalized 46.9 nm laser radiation at fluences between 0.1 and 100 J cm-2. The experiments demonstrated that the combined high repetition rate and high energy per pulse of the capillary discharge laser allows for the first time the processing of large surface areas with intense soft x-ray laser radiation. The damage threshold and damage mechanism of extreme ultraviolet Sc/Si multilayer mirror coatings was studied . Damage threshold fluences of ~ 0.08 J/cm2 were determined for coatings deposited on both borosilicate glass and Si substrates. Scanning and transmission electron microscopy, and small-angle X-ray diffraction techniques revealed the thermal nature of the damage mechanism. These results provide a benchmark for the use of Sc/Si multilayer mirrors in high fluence applications, and for the development of higher damage threshold mirrors. Soft x-ray laser ablation studies were also conducted for silicon and several plastic materials, including PMMA, Polyamide and PTFE.

  8. Multi-tens of GW peak power plasma-based soft x-ray laser

    NASA Astrophysics Data System (ADS)

    Oliva, E.; Fajardo, M.; Li, L.; Le, T. T. T.; Ros, D.; Sebban, S.; Velarde, P.; Zeitoun, P.

    2013-09-01

    Ultra-intense X-ray sources have opened new avenues by creating new states of matter or probing and imaging living or inert matter. Free-electron lasers have a strong leadership by delivering pulses combining femtosecond duration and 10s of microJoules to milliJoule energy. However, these sources remain highly expensive limiting their number to a few worldwide. In parallel, laser-pumped soft X-ray lasers hold outstanding promises having demonstrated the most energetic monochromatic soft x-ray pulse and being intrinsically fully synchronized with any secondary source of the pump laser. Since the first successful demonstration of amplification of a high harmonic pulse in a plasma from gas in 2003 and from solid in 2008, we have developed an extensive numerical study. 2D hydrodynamic simulations showed that optimized Transient Collisional Excitation plasma amplifiers, may store up to 0.4 mJ in the population inversion. If carefully seeded, pulses of 80 fs and 20 μJ might be generated with table-top lasers (10J). As the energy extracted is far from the milliJoule requirements of most exciting applications, we studied the seminal experiment of Ditmire et al who seeded a plasma emitting milliJoules in the form of Amplified Spontaneous Emission (ASE).We retrieved and explained for the first time the experimental result (ASE 1,000 times stronger than amplified seed). We thus proposed and fully modeled the transposition of the so-called Chirped Pulse Amplification (CPA) in the soft X-ray range, showing that 6 mJ, 200 fs, fully coherent soft X-ray pulse is accessible with compact pump lasers.

  9. Generation of bright isolated attosecond soft X-ray pulses driven by multicycle midinfrared lasers.

    PubMed

    Chen, Ming-Chang; Mancuso, Christopher; Hernández-García, Carlos; Dollar, Franklin; Galloway, Ben; Popmintchev, Dimitar; Huang, Pei-Chi; Walker, Barry; Plaja, Luis; Jaroń-Becker, Agnieszka A; Becker, Andreas; Murnane, Margaret M; Kapteyn, Henry C; Popmintchev, Tenio

    2014-06-10

    High harmonic generation driven by femtosecond lasers makes it possible to capture the fastest dynamics in molecules and materials. However, to date the shortest subfemtosecond (attosecond, 10(-18) s) pulses have been produced only in the extreme UV region of the spectrum below 100 eV, which limits the range of materials and molecular systems that can be explored. Here we experimentally demonstrate a remarkable convergence of physics: when midinfrared lasers are used to drive high harmonic generation, the conditions for optimal bright, soft X-ray generation naturally coincide with the generation of isolated attosecond pulses. The temporal window over which phase matching occurs shrinks rapidly with increasing driving laser wavelength, to the extent that bright isolated attosecond pulses are the norm for 2-µm driving lasers. Harnessing this realization, we experimentally demonstrate the generation of isolated soft X-ray attosecond pulses at photon energies up to 180 eV for the first time, to our knowledge, with a transform limit of 35 attoseconds (as), and a predicted linear chirp of 300 as. Most surprisingly, advanced theory shows that in contrast with as pulse generation in the extreme UV, long-duration, 10-cycle, driving laser pulses are required to generate isolated soft X-ray bursts efficiently, to mitigate group velocity walk-off between the laser and the X-ray fields that otherwise limit the conversion efficiency. Our work demonstrates a clear and straightforward approach for robustly generating bright isolated attosecond pulses of electromagnetic radiation throughout the soft X-ray region of the spectrum.

  10. Generation of bright isolated attosecond soft X-ray pulses driven by multicycle midinfrared lasers

    PubMed Central

    Chen, Ming-Chang; Mancuso, Christopher; Hernández-García, Carlos; Dollar, Franklin; Galloway, Ben; Popmintchev, Dimitar; Huang, Pei-Chi; Walker, Barry; Plaja, Luis; Jaroń-Becker, Agnieszka A.; Becker, Andreas; Murnane, Margaret M.; Kapteyn, Henry C.; Popmintchev, Tenio

    2014-01-01

    High harmonic generation driven by femtosecond lasers makes it possible to capture the fastest dynamics in molecules and materials. However, to date the shortest subfemtosecond (attosecond, 10−18 s) pulses have been produced only in the extreme UV region of the spectrum below 100 eV, which limits the range of materials and molecular systems that can be explored. Here we experimentally demonstrate a remarkable convergence of physics: when midinfrared lasers are used to drive high harmonic generation, the conditions for optimal bright, soft X-ray generation naturally coincide with the generation of isolated attosecond pulses. The temporal window over which phase matching occurs shrinks rapidly with increasing driving laser wavelength, to the extent that bright isolated attosecond pulses are the norm for 2-µm driving lasers. Harnessing this realization, we experimentally demonstrate the generation of isolated soft X-ray attosecond pulses at photon energies up to 180 eV for the first time, to our knowledge, with a transform limit of 35 attoseconds (as), and a predicted linear chirp of 300 as. Most surprisingly, advanced theory shows that in contrast with as pulse generation in the extreme UV, long-duration, 10-cycle, driving laser pulses are required to generate isolated soft X-ray bursts efficiently, to mitigate group velocity walk-off between the laser and the X-ray fields that otherwise limit the conversion efficiency. Our work demonstrates a clear and straightforward approach for robustly generating bright isolated attosecond pulses of electromagnetic radiation throughout the soft X-ray region of the spectrum. PMID:24850866

  11. Ionized Absorbers in Active Galactic Nuclei and Very Steap Soft X-Ray Quasars

    NASA Technical Reports Server (NTRS)

    Fiore, Fabrizio; White, Nicholas (Technical Monitor)

    2000-01-01

    Steep soft X-ray (0.1-2 keV) quasars share several unusual properties: narrow Balmer lines, strong Fe II emission, large and fast X-ray variability, and a rather steep 2-10 keV spectrum. These intriguing objects have been suggested to be the analogues of Galactic black hole candidates in the high, soft state. We present here results from ASCA observations for two of these quasars: NAB 0205 + 024 and PG 1244 + 026. Both objects show similar variations (factor of approximately 2 in 10 ks), despite a factor of approximately 10 difference in the 0.5-10 keV luminosity (7.3 x 10(exp 43) erg/s for PG 1244 + 026 and 6.4 x 10(exp 44) erg/s for NAB 0205 + 024, assuming isotropic emission, H(sub 0) = 50.0 and q(sub 0) = 0.0). The X-ray continuum of the two quasars flattens by 0.5-1 going from the 0.1-2 keV band towards higher energies, strengthening recent results on another half-dozen steep soft X-ray active galactic nuclei. PG 1244 + 026 shows a significant feature in the '1-keV' region, which can be described either as a broad emission line centered at 0.95 keV (quasar frame) or as edge or line absorption at 1.17 (1.22) keV. The line emission could be a result of reflection from a highly ionized accretion disc, in line with the view that steep soft X-ray quasars are emitting close to the Eddington luminosity. Photoelectric edge absorption or resonant line absorption could be produced by gas outflowing at a large velocity (0.3-0.6 c).

  12. A CANDIDATE ACTIVE GALACTIC NUCLEUS WITH A PURE SOFT THERMAL X-RAY SPECTRUM

    SciTech Connect

    Terashima, Yuichi; Kamizasa, Naoya; Awaki, Hisamitsu; Kubota, Aya; Ueda, Yoshihiro

    2012-06-20

    We report the discovery of a candidate active galactic nucleus (AGN), 2XMM J123103.2+110648 at z = 0.13, with an X-ray spectrum represented purely by soft thermal emission reminiscent of Galactic black hole (BH) binaries in the disk-dominated state. This object was found in the second XMM-Newton serendipitous source catalog as a highly variable X-ray source. In three separate observations, its X-ray spectrum can be represented either by a multicolor disk blackbody model with an inner temperature of kT{sub in} Almost-Equal-To 0.16-0.21 keV or a Wien spectrum Comptonized by an optically thick plasma with kT Almost-Equal-To 0.14-0.18 keV. The soft X-ray luminosity in the 0.5-2 keV band is estimated to be (1.6-3.8) Multiplication-Sign 10{sup 42} erg s{sup -1}. Hard emission above {approx}2 keV is not detected. The ratio of the soft to hard emission is the strongest among AGNs observed thus far. Spectra selected in high/low-flux time intervals are examined in order to study spectral variability. In the second observation with the highest signal-to-noise ratio, the low-energy (below 0.7 keV) spectral regime flattens when the flux is high, while the shape of the high-energy part (1-1.7 keV) remains unchanged. This behavior is qualitatively consistent with being caused by strong Comptonization. Both the strong soft excess and spectral change consistent with Comptonization in the X-ray spectrum imply that the Eddington ratio is large, which requires a small BH mass (smaller than {approx}10{sup 5} M{sub Sun }).

  13. Electronic structure of La{sub 5/3}Sr{sub 1/3}NiO{sub 4} by x-ray emission spectroscopy and resonant inelastic x-ray scattering

    SciTech Connect

    Simonelli, L.; Huotari, S.; Monaco, G.; Saini, N. L.; Giordano, V. M.

    2012-06-01

    Here, we report a study of the electronic structure of La{sub 5/3}Sr{sub 1/3}NiO{sub 4} by x-ray emission spectroscopy (XES) and resonant inelastic x-ray scattering (RIXS). The combination of these techniques has permitted us to reveal a complete picture of the occupied and unoccupied states, and to identify various charge transfer transitions appearing as inelastic features in the RIXS spectra. The results add further information on the electronic excitations in this system, and show how the combination of XES and RIXS can be an important experimental tool to address basic physics of complex systems.

  14. Fabrication of compound refractive lens using soft and deep X-ray lithography beamline on Indus-2

    SciTech Connect

    Dhamgaye, V. P.; Lodha, G. S.

    2012-06-05

    X-ray compound refractive lenses (CRL) have been fabricated using Soft and Deep X-ray lithography (SDXRL) beamline on Indus-2. Upto 50 parabolic lenses are fabricated in PMMA using 1X X-ray mask. The mask contains of 20 micron thick gold absorbing pattern on polyimide membrane. The lens fabrication is done by exposing 500 {mu}m thick PMMA sheets to 5-12keV X-rays from Indus-2. The fabricated CRL will be suitable for generating focused X-ray beam of Indus-2 bending magnet source.

  15. Influence of the soft X-ray plasma focus radiation on live microorganisms

    NASA Astrophysics Data System (ADS)

    Zapryanov, S.; Goltsev, V.; Galutsov, B.; Gelev, M.; Blagoev, A.

    2012-04-01

    A 3 kJ plasma focus device was used to study the influence of the soft X-ray on live microorganisms. When Saccharomyces cerevisiae - (yeast) was treated with a dose of 65 mSv of the X-ray radiation (14 shots), no difference in the fertility activity between the control probe and the sample was observed. Also no change in the survival enzyme activity was found after irradiation through a 100 μm Al foil of another type of yeast - Kluyveromyces marxiamus. The irradiation of the Chlamydomonas reinhardtii samples by the PF-X-ray emission through 20 μm Al foil with a dose of 11 mSv produces a considerable change of the photosynthesis parameters. This result is similar to the results of previous studies with plasma focus radiation where strong effects were derived with low doses but with a high dose power.

  16. Time-resolved soft x-ray spectra from laser-produced Cu plasma

    SciTech Connect

    Cone, K. V.; Baldis, H. A.; Dunn, J.; May, M. J.; Schneider, M. B.; Scott, H. A.; Purvis, M. A.

    2012-10-15

    The volumetric heating of a thin copper target has been studied with time resolved x-ray spectroscopy. The copper target was heated by a plasma produced using the Lawrence Livermore National Laboratory's Compact Multipulse Terawatt (COMET) laser. A variable spaced grating spectrometer coupled to an x-ray streak camera measured soft x-ray emission (800-1550 eV) from the back of the copper target to characterize the bulk heating of the target. Radiation hydrodynamic simulations were modeled in two-dimensions using the HYDRA code. The target conditions calculated by HYDRA were post-processed with the atomic kinetics code CRETIN to generate synthetic emission spectra. A comparison between the experimental and simulated spectra indicates the presence of specific ionization states of copper and the corresponding electron temperatures and ion densities throughout the laser-heated copper target.

  17. Time-resolved soft x-ray spectra from laser-produced Cu plasma.

    PubMed

    Cone, K V; Baldis, H A; Dunn, J; May, M J; Purvis, M A; Schneider, M B; Scott, H A

    2012-10-01

    The volumetric heating of a thin copper target has been studied with time resolved x-ray spectroscopy. The copper target was heated by a plasma produced using the Lawrence Livermore National Laboratory's Compact Multipulse Terawatt (COMET) laser. A variable spaced grating spectrometer coupled to an x-ray streak camera measured soft x-ray emission (800-1550 eV) from the back of the copper target to characterize the bulk heating of the target. Radiation hydrodynamic simulations were modeled in two-dimensions using the HYDRA code. The target conditions calculated by HYDRA were post-processed with the atomic kinetics code CRETIN to generate synthetic emission spectra. A comparison between the experimental and simulated spectra indicates the presence of specific ionization states of copper and the corresponding electron temperatures and ion densities throughout the laser-heated copper target.

  18. Characterization and possible repair of defects in Soft X-ray Projection Lithography masks

    SciTech Connect

    Hawryluk, A.M.

    1993-07-01

    Soft X-ray Projection Lithography (SXPL) is one promising technique for the mass production of integrated circuits with minimum features sizes below 100 nm. Mask fabrication, inspection and repair processes are critically important to all forms of lithography, including SXPL which requires a reflection mask (a substrate coated with a x-ray multilayer coating and patterned with thin metallization layer). Processes for the repair of defects in the metallization patterns have been developed, but at present, there exist no processes for the repair of defects in the multilayer coatings deposited in LLNL`s magnetron sputter deposition facility, which produces state of the art x-ray multilayer mirrors. We also propose one possible process for the repair of defects in these multilayer coatings.

  19. Time-resolved soft x-ray spectra from laser-produced Cu plasma

    SciTech Connect

    Cone, K V; Dunn, J; Baldis, H A; May, M J; Purvis, M A; Scott, H A; Schneider, M B

    2012-05-02

    The volumetric heating of a thin copper target has been studied with time resolved x-ray spectroscopy. The copper target was heated from a plasma produced using the Lawrence Livermore National Laboratory's Compact Multipulse Terrawatt (COMET) laser. A variable spaced grating spectrometer coupled to an x-ray streak camera measured soft x-ray emission (800-1550 eV) from the back of the copper target to characterize the bulk heating of the target. Radiation hydrodynamic simulations were modeled in 2-dimensions using the HYDRA code. The target conditions calculated by HYDRA were post-processed with the atomic kinetics code CRETIN to generate synthetic emission spectra. A comparison between the experimental and simulated spectra indicates the presence of specific ionization states of copper and the corresponding electron temperatures and ion densities throughout the laser-heated copper target.

  20. Characterization of surface carbon films on weathered Japaneseroof tiles by soft x-ray spectroscopy

    SciTech Connect

    Muramatsu, Y.; Yamashita, M.; Motoyama, M.; Hirose, M.; Denlinger, J.D.; Gullikson, E.M.; Perera, R.C.

    2004-07-15

    The effects of weathering on carbon films deposited onJapanese smoked roof tileswere investigated by soft x-ray absorption andemission spectroscopy using synchrotron radiation. X-ray absorptionmeasurements revealed that weathering oxidizes the carbon films and thatpartial carboxy chemical bonding occurs. Incident angle-dependent x-rayabsorption spectra in the C K region confirmed that the degree of theorientation at the surface of the oxidized carbon films decreases withweathering. However, the take-off angle-dependent C K x-ray emissionspectra showed that the orientation of the layered carbon structure ismaintained in the bulk portion when weathered. Therefore, it is confirmedthat oxidation proceeds from the surface of the carbon films. Weatheringdegrades and oxidizes the surface carbon films, which causes the metallicsilver color to change to darker gray.

  1. Compact 'diode-based' multi-energy soft x-ray diagnostic for NSTX

    SciTech Connect

    Tritz, K.; Clayton, D. J.; Stutman, D.; Finkenthal, M.

    2012-10-15

    A novel and compact, diode-based, multi-energy soft x-ray (ME-SXR) diagnostic has been developed for the National Spherical Tokamak Experiment. The new edge ME-SXR system tested on NSTX consists of a set of vertically stacked diode arrays, each viewing the plasma tangentially through independent pinholes and filters providing an overlapping view of the plasma midplane which allows simultaneous SXR measurements with coarse sub-sampling of the x-ray spectrum. Using computed x-ray spectral emission data, combinations of filters can provide fast (>10 kHz) measurements of changes in the electron temperature and density profiles providing a method to 'fill-in' the gaps of the multi-point Thomson scattering system.

  2. SolpeX: the soft X-ray flare polarimeter-spectrometer for the ISS

    NASA Astrophysics Data System (ADS)

    Sylwester, Janusz; Płocieniak, Stefan; Bakała, Jarosław; Szaforz, Żaneta; Stȩślicki, Marek; Ścisłowski, Daniel; Kowaliński, Mirosław; Podgórski, Piotr; Hernandez, Jose; Shestov, Sergey

    2015-10-01

    We present the innovative soft X-ray spectro-polarimeter, SolpeX. This instrument consists of three functionally independent blocks. They are to be included into the Russian instrument KORTES, to be mounted onboard the ISS. The three SolpeX units are: a simple pin-hole X-ray spectral imager, a polarimeter, and a fast-rotating drum multiple-flat-crystal Bragg spectrometer. Such a combination of measuring blocks will offer a new opportunity to reliably measure possible X-ray polarization and spectra of solar flares, in particular during the impulsive phase. Polarized Bremsstrahlung and line emission due to the presence of directed particle beams will be detected, and measurements of the velocities of evaporated hot plasma will be made. In this paper we discuss the details of the construction of the SolpeX units. The delivery of KORTES with SolpeX to the ISS is expected to happen in 2017/2018.

  3. Hot bubbles in a magnetic interstellar medium - Another look at the soft X-ray background

    NASA Technical Reports Server (NTRS)

    Edgar, Richard J.; Cox, Donald P.

    1993-01-01

    An attempt is made to understand the origin and properties of an isolated local bubble of hot gas using models of explosive events in a magnetic interstellar medium which mimic the local bubble in terms of the C band X-ray surface brightness and radius. The residual bubble of hot gas reaches a maximum size with an internal pressure below ambient, and then shrinks to smaller volume and a pressure nearly equal to ambient. The X-ray brightness reaches its minimum at the time of maximum radius and rises thereafter. It is found that the bubble growth must have been confined by a probably unacceptably large external pressure in order for the hot gas in the maximally extended cavity to radiate at a rate like that observed in the soft X-ray background.

  4. Superconducting Detector System for High-Resolution Energy-Dispersive Soft X-Ray Spectroscopy

    SciTech Connect

    Friedrich, S; Niedermayr, T; Drury, O; Funk, T; Frank, M; Labov, S E; Cramer, S

    2001-02-21

    Synchrotron-based soft x-ray spectroscopy is often limited by detector performance. Grating spectrometers have the resolution, but lack the efficiency for the analysis of dilute samples. Semiconducting Si(Li) or Ge detectors are efficient, but often lack the resolution to separate weak signals from strong nearby lines in multi-element samples. Superconducting tunnel junctions (STJs) operated at temperatures below 1 K can be used as high-resolution high-efficiency x-ray detectors. They combine high energy resolution around 10 eV FWHM with the broad band efficiency of energy-dispersive detectors. We have designed a two-stage adiabatic demagnetization refrigerator (ADR) to operate STJ detectors in x-ray fluorescence measurements at beam line 4 of the ALS. We demonstrate the capabilities of such a detector system for fluorescence analysis of dilute metal sites in proteins and inorganic model compounds.

  5. Soft X-ray observations of Centaurus X-3 from Copernicus

    NASA Technical Reports Server (NTRS)

    Margon, B.; Mason, K. O.; Hawkins, F. J.; Sanford, P. W.

    1975-01-01

    We have detected soft X-ray emission from Centaurus X-3 in the 0.6-1.9 keV band, using the focusing telescope aboard OAO Copernicus. The flux is compatible with an extrapolation of the harder X-ray spectrum, attenuated by (3-4) times 10 to the 22nd atoms per sq cm of interstellar and/or circumstellar matter. The data are consistent with the distance estimate of 5-10 kpc derived from the spectroscopic modulus of the optical component, and obviate the need to postulate the primary to be an anomalously subluminous hot star. There is currently no compelling evidence that such models must be invoked to explain any of the observed compact X-ray sources.

  6. Octupole Magnet For Soft X Ray Magnetic Dichroism Experiments: Design and Performance

    SciTech Connect

    Arenholz, Elke; Prestemon, Soren O.

    2004-05-12

    An octupole magnet endstation for soft x ray magnetic dichroism measurements has been developed at the Advanced Light Source. The system consists of an eight pole electromagnet that surrounds a small vacuum chamber. The magnet provides fields up to 0.9 T that can be applied in any direction relative to the incoming x ray beam. High precision magnetic circular and linear dichroism spectra can be obtained reversing the magnetic field for each photon energy in an energy scan. Moreover, the field dependence of all components of the magnetization vector can be studied in detail by choosing various angles of x ray incidence while keeping the relative orientation of magnetic field and sample fixed.

  7. Gas cell for in situ soft X-ray transmission-absorption spectroscopy of materials

    SciTech Connect

    Drisdell, W. S.; Kortright, J. B.

    2014-07-15

    A simple gas cell design, constructed primarily from commercially available components, enables in situ soft X-ray transmission-absorption spectroscopy of materials in contact with gas at ambient temperature. The cell has a minimum X-ray path length of 1 mm and can hold gas pressures up to ∼300 Torr, and could support higher pressures with simple modifications. The design enables cycling between vacuum and gas environments without interrupting the X-ray beam, and can be fully sealed to allow for measurements of air-sensitive samples. The cell can attach to the downstream port of any appropriate synchrotron beamline, and offers a robust and versatile method for in situ measurements of certain materials. The construction and operation of the cell are discussed, as well as sample preparation and proper spectral analysis, illustrated by examples of spectral measurements. Potential areas for improvement and modification for specialized applications are also mentioned.

  8. Single particle imaging with soft x-rays at the Linac Coherent Light Source

    NASA Astrophysics Data System (ADS)

    Martin, Andrew V.; Andreasson, Jakob; Aquila, Andrew; Bajt, Saša; Barends, Thomas R. M.; Barthelmess, Miriam; Barty, Anton; Benner, W. Henry; Bostedt, Christoph; Bozek, John D.; Bucksbaum, Phillip; Caleman, Carl; Coppola, Nicola; DePonte, Daniel P.; Ekeberg, Tomas; Epp, Sascha W.; Erk, Benjamin; Farquar, George R.; Fleckenstein, Holger; Foucar, Lutz; Frank, Matthias; Gumprecht, Lars; Hampton, Christina Y.; Hantke, Max; Hartmann, Andreas; Hartmann, Elisabeth; Hartmann, Robert; Hau-Riege, Stephan P.; Hauser, Günther; Holl, Peter; Hoemke, André; Jönsson, Olof; Kassemeyer, Stephan; Kimmel, Nils; Kiskinova, Maya; Krasniqi, Faton; Krzywinski, Jacek; Liang, Mengning; Loh, Ne-Te Duane; Lomb, Lukas; Maia, Filipe R. N. C.; Marchesini, Stefano; Messerschmidt, Marc; Nass, Karol; Odic, Duško; Pedersoli, Emanuele; Reich, Christian; Rolles, Daniel; Rudek, Benedikt; Rudenko, Artem; Schmidt, Carlo; Schultz, Joachim; Seibert, M. Marvin; Shoeman, Robert L.; Sierra, Raymond G.; Soltau, Heike; Starodub, Dmitri; Steinbrener, Jan; Stellato, Francesco; Strüder, Lothar; Svenda, Martin; Tobias, Herbert; Ullrich, Joachim; Weidenspointner, Georg; Westphal, Daniel; White, Thomas A.; Williams, Garth; Hajdu, Janos; Schlichting, Ilme; Bogan, Michael J.; Chapman, Henry N.

    2011-06-01

    Results of coherent diffractive imaging experiments performed with soft X-rays (1-2 keV) at the Linac Coherent Light Source are presented. Both organic and inorganic nano-sized objects were injected into the XFEL beam as an aerosol focused with an aerodynamic lens. The high intensity and femtosecond duration of X-ray pulses produced by the Linac Coherent Light Source allow structural information to be recorded by X-ray diffraction before the particle is destroyed. Images were formed by using iterative methods to phase single shot diffraction patterns. Strategies for improving the reconstruction methods have been developed. This technique opens up exciting opportunities for biological imaging, allowing structure determination without freezing, staining or crystallization.

  9. Installation of soft X-ray array diagnostics and its application to tomography reconstruction using synthetic KSTAR X-ray images

    SciTech Connect

    Lee, Seung Hun; Jang, Juhyeok; Hong, Joohwan; Jang, Siwon; Choe, Wonho; Pacella, D.; Romano, A.; Gabellieri, L.; Kim, Junghee

    2014-11-15

    Four-array system of soft X-ray diagnostics was installed on KSTAR tokamak. Each array has 32 viewing chords of two photo-diode array detectors with spatial resolution of 2 cm. To estimate signals from the soft X-ray radiation power, typical n{sub e}, T{sub e}, and argon impurity line radiation profiles in KSTAR are chosen. The photo-diodes were absolutely calibrated as a function of the incident photon energy in 2–40 keV range with a portable X-ray tube. Two-dimensional T{sub e} image properties by multi-energy method were simulated and visualized with six combinations of beryllium filter sets within the dynamic range of signal ratio.

  10. Wavelength dispersing devices for soft and ultrasoft x-ray spectrometers

    SciTech Connect

    Arai, Tomoya; Ryon, R.W.; Shoji, Takashi

    1984-01-01

    Monochromatization combining total reflection by a selected mirror and an appropriate filter offered an alternative approach in order to increase measurable intensity with reasonable spectral resolution. Recently, the use of synthetic multilayers, which are prepared by sputter/evaporation techniques, has been introduced for the detection of soft and ultrasoft x-rays. Studies on the use of these new wavelength dispersing devices have been conducted and it has been found that the reflectivity of these devices is very high compared with single crystals and soap multilayers and that their resolving power is fairly good. This report makes comparisons regarding efficiency of reflection, resolving power and x-ray analytical problems for practical applications among long spacing single crystals, soap multilayers, total reflection combined with a selected mirror and filtering and synthetic multilayers. The x-ray analytical capablities are shown based upon a standard x-ray fluorescence spectrometer equipped with a sealed-off x-ray tube and a gas flow proportional counter with thin film detector window.

  11. Yeast cell metabolism investigated by CO{_2} production and soft X-ray irradiation

    NASA Astrophysics Data System (ADS)

    Masini, A.; Batani, D.; Previdi, F.; Milani, M.; Pozzi, A.; Turcu, E.; Huntington, S.; Takeyasu, H.

    1999-01-01

    Results obtained using a new technique for studying cell metabolism are presented. The technique, consisting in CO2 production monitoring, has been applied to Saccharomyces cerevisiae yeast cells. Also the cells were irradiated using the soft X-ray laser-plasma source at Rutherford Appleton Laboratory with the aim of producing a damage of metabolic processes at the wall level, responsible for fermentation, without great interference with respiration, taking place in mitochondria, and DNA activity. The source was calibrated with PIN diodes and X-ray spectrometers and used Teflon stripes as target, emitting X-rays at about 0.9 keV, with a very low penetration in biological material. X-ray doses delivered to the different cell compartments were calculated following a Lambert-Bouguet-Beer law. Immediately after irradiation, the damage to metabolic activity was measured again by monitoring CO2 production. Results showed a general reduction in gas production by irradiated samples, together with non-linear and non-monotone response to dose. There was also evidence of oscillations in cell metabolic activity and of X-ray induced changes in oscillation frequency.

  12. Soft x-ray images of the Laser Entrance Hole of NIC Hohlraums (paper, HTPD2012)

    SciTech Connect

    Schneider, M B; Meezan, N B

    2012-04-30

    Hohlraums at the National Ignition Facility convert laser energy into a thermal x-radiation drive, which implodes the capsule, thus compressing the fuel. The x-radiation drive is measured with a low resolution, time-resolved x-ray spectrometer that views the hohlraum's laser entrance hole (LEH) at 37{sup o} to the hohlraum axis. This measurement has no spatial resolution. To convert this to the drive inside the hohlraum, the area and fraction of the measured x-radiation which comes from the region inside the hohlraum must be known. The size of the LEH is measured with the time integrated Static X-ray Imager (SXI) which view the LEH at 18{sup o} to the hohlraum axis. A soft x-ray image has been added to the SXI to measure the fraction of x-radiation inside the LEH's Clear Aperture in order to correct the measured radiation. A multilayer mirror plus filter selects an x-ray band centered at 870 eV, near the x-ray energy peak of a 300 eV blackbody. Results from this channel and corrections to the x-radiation drive are discussed.

  13. Soft x-ray images of the laser entrance hole of ignition hohlraums.

    PubMed

    Schneider, M B; Meezan, N B; Alvarez, S S; Alameda, J; Baker, S; Bell, P M; Bradley, D K; Callahan, D A; Celeste, J R; Dewald, E L; Dixit, S N; Döppner, T; Eder, D C; Edwards, M J; Fernandez-Perea, M; Gullikson, E; Haugh, M J; Hau-Riege, S; Hsing, W; Izumi, N; Jones, O S; Kalantar, D H; Kilkenny, J D; Kline, J L; Kyrala, G A; Landen, O L; London, R A; MacGowan, B J; MacKinnon, A J; McCarville, T J; Milovich, J L; Mirkarimi, P; Moody, J D; Moore, A S; Myers, M D; Palma, E A; Palmer, N; Pivovaroff, M J; Ralph, J E; Robinson, J; Soufli, R; Suter, L J; Teruya, A T; Thomas, C A; Town, R P; Vernon, S P; Widmann, K; Young, B K

    2012-10-01

    Hohlraums are employed at the national ignition facility to convert laser energy into a thermal x-radiation drive, which implodes a fusion capsule, thus compressing the fuel. The x-radiation drive is measured with a low spectral resolution, time-resolved x-ray spectrometer, which views the region around the hohlraum's laser entrance hole. This measurement has no spatial resolution. To convert this to the drive inside the hohlraum, the size of the hohlraum's opening ("clear aperture") and fraction of the measured x-radiation, which comes from this opening, must be known. The size of the clear aperture is measured with the time integrated static x-ray imager (SXI). A soft x-ray imaging channel has been added to the SXI to measure the fraction of x-radiation emitted from inside the clear aperture. A multilayer mirror plus filter selects an x-ray band centered at 870 eV, near the peak of the x-ray spectrum of a 300 eV blackbody. Results from this channel and corrections to the x-radiation drive are discussed. PMID:23127032

  14. Soft-x-ray fluorescence study of buried silicides in antiferromagnetically coupled Fe/Si multilayers

    SciTech Connect

    Carlisle, J.A.; Chaiken, A.; Michel, R.P.

    1997-04-01

    Multilayer films made by alternate deposition of two materials play an important role in electronic and optical devices such as quantum-well lasers and x-ray mirrors. In addition, novel phenomena like giant magnetoresistance and dimensional crossover in superconductors have emerged from studies of multilayers. While sophisticated x-ray techniques are widely used to study the morphology of multilayer films, progress in studying the electronic structure has been slower. The short mean-free path of low-energy electrons severely limits the usefulness of photoemission and related electron free path of low-energy electrons severely limit spectroscopies for multilayer studies. Soft x-ray fluorescence (SXF) is a bulk-sensitive photon-in, photon-out method to study valence band electronic states. Near-edge x-ray absorption fine-structure spectroscopy (NEXAFS) measured with partial photon yield can give complementary bulk-sensitive information about unoccupied states. Both these methods are element-specific since the incident x-ray photons excite electrons from core levels. By combining NEXAFS and SXF measurements on buried layers in multilayers and comparing these spectra to data on appropriate reference compounds, it is possible to obtain a detailed picture of the electronic structure. Results are presented for a study of a Fe/Si multilayer system.

  15. Single-band model of resonant inelastic x-ray scattering by quasiparticles in high-T(c) cuprate superconductors.

    PubMed

    Benjamin, David; Klich, Israel; Demler, Eugene

    2014-06-20

    We show that a simple model of noninteracting quasiparticles accurately describes resonant inelastic x-ray scattering (RIXS) experiments in the hole-doped cuprate superconductors. Band structure alone yields signatures previously attributed to collective magnetic modes, such as the dispersing peaks and nontrivial polarization dependence found in several experiments. We conclude that RIXS data can be explained without positing the existence of magnetic excitations that persist with increasing doping. In so doing we develop a formalism for RIXS in itinerant electron systems that accounts for the positively charged core hole exactly and discover a mechanism by which the core hole produces polarization dependence mimicking that of a magnetic system. PMID:24996103

  16. The single particle dynamics of iodine in the Sachs-Teller regime: An inelastic x-ray scattering study

    SciTech Connect

    Izzo, M. G.; Bencivenga, F.; Di Fonzo, S.; Cunsolo, A.; Verbeni, R.; De Lorenzo, R. Gimenez

    2010-09-28

    The high frequency dynamics of liquid iodine has been investigated by deep inelastic x-ray scattering at exchanged wave-vectors (q) ranging from 2.5 to 15 A{sup -1}. The experimental data have been analyzed in the frame of the Sachs-Teller theory of the molecular spectrum while accounting for final state corrections to the lineshape. The performed data analysis carries insights on physical quantities as relevant as the mean rototranslational kinetic energy and the mean square Laplacian of the intermolecular potential. In both cases the measured values are consistent with corresponding theoretical expectations.

  17. Influence of magnetism on phonons in CaFe2As2 as seen via inelastic x-ray scattering

    SciTech Connect

    Hahn, S.E.; Lee, Y.; Ni, N.; Canfield, P.C.; Goldman, A.I.; McQueeney, R.J.; Harmon, B.N.; Alatas, A.; Leu, B.M.; Alp, E.E.; Chung, D.Y.; Todorov, I.S.; Kanatzidis, M.G.

    2009-06-19

    In the iron pnictides, the strong sensitivity of the iron magnetic moment to the arsenic position suggests a significant relationship between phonons and magnetism. We measured the phonon dispersion of several branches in the high-temperature tetragonal phase of CaFe{sub 2}As{sub 2} using inelastic x-ray scattering on single-crystal samples. These measurements were compared to ab initio calculations of the phonons. Spin-polarized calculations imposing the antiferromagnetic order present in the low-temperature orthorhombic phase dramatically improve agreement between theory and experiment. This is discussed in terms of the strong antiferromagnetic correlations that are known to persist in the tetragonal phase.

  18. Resonant inelastic X-ray scattering spectrometer with 25 meV resolution at the Cu K-edge.

    PubMed

    Ketenoglu, Didem; Harder, Manuel; Klementiev, Konstantin; Upton, Mary; Taherkhani, Mehran; Spiwek, Manfred; Dill, Frank Uwe; Wille, Hans Christian; Yavaş, Hasan

    2015-07-01

    An unparalleled resolution is reported with an inelastic X-ray scattering instrument at the Cu K-edge. Based on a segmented concave analyzer, featuring single-crystal quartz (SiO₂) pixels, the spectrometer delivers a resolution near 25 meV (FWHM) at 8981 eV. Besides the quartz analyzer, the performance of the spectrometer relies on a four-bounce Si(553) high-resolution monochromator and focusing Kirkpatrick-Baez optics. The measured resolution agrees with the ray-tracing simulation of an ideal spectrometer. The performance of the spectrometer is demonstrated by reproducing the phonon dispersion curve of a beryllium single-crystal.

  19. Resonant inelastic X-ray scattering spectrometer with 25meV resolution at the Cu K -edge

    DOE PAGES

    Ketenoglu, Didem; Harder, Manuel; Klementiev, Konstantin; Upton, Mary; Taherkhani, Mehran; Spiwek, Manfred; Dill, Frank-Uwe; Wille, Hans-Christian; Yavaş, Hasan

    2015-06-27

    An unparalleled resolution is reported with an inelastic X-ray scattering instrument at the CuK-edge. Based on a segmented concave analyzer, featuring single-crystal quartz (SiO2) pixels, the spectrometer delivers a resolution near 25meV (FWHM) at 8981eV. Besides the quartz analyzer, the performance of the spectrometer relies on a four-bounce Si(553) high-resolution monochromator and focusing Kirkpatrick–Baez optics. The measured resolution agrees with the ray-tracing simulation of an ideal spectrometer. The performance of the spectrometer is demonstrated by reproducing the phonon dispersion curve of a beryllium single-crystal.

  20. EUV and soft x-ray excess emission from clusters of galaxies

    NASA Astrophysics Data System (ADS)

    Bonamente, Massimiliano

    2000-08-01

    Extreme ultra-violet and soft X-ray radiation (~60-400 eV) from extragalactic sources suffers from severe Galactic absorption losses, rendering the detection of radiation at these energies a complicated task. Clusters are well known to be X-ray emitters; some EUV and soft X-rays are therefore expected as the low- energy `tail' of this emission. The first detection of excess EUV emission, i.e., above that expected fro the X-ray emitting gas, was achieved only very recently (1996), nearly thirty years after cluster X-rays were detected. Basic dynamic and energetic properties of clusters of galaxies are reviewed in Chapter 2. Clusters analyzed in this Dissertation (A2199, A1795, Coma and Virgo) all lie along directions of low line-of-sight Galactic HI column density (NH <= 1-2 × 1020 cm-2), and diffuse excess EUV emission from them was detected in the 60-200 eV band by the Extreme Ultraviolet Explorer (EUVE). Instrumental issues concerning the Deep Survey detector aboard EUVE are therefore scrutinised in Chapter 3 in order to devise a correct method of data analysis. Relevant issues to the ROSAT Position-sensitive Proportional Counter (PSPC) detector, used for its soft X-ray sensitivity, are also considered. The EUV and soft X-ray excess emission (the cluster soft excess phenomenon, CSE) is found for all four clusters in the sample (Chapter 4). Some of the clusters show a peculiar trend of the CSE emission, resulting in the increase of the relative importance of the CSE emission with radial distance (the soft-excess radial trend, SERT). Two alternative explanations of the CSE emission are explored: non-thermal radiation due to Inverse Compton (IC) scattering of relativistic electrons and radiation from a warm (~106 K) gas. A detailed treatment of IC scattering (off the microwave background field, the MWB) in the cluster environment is described in Chapter 5, where cluster spectra are fitted to IC models. It is initially shown that the soft excess of some clusters (e

  1. Band gap states in nanocrystalline WO3 thin films studied by soft x-ray spectroscopy and optical spectrophotometry.

    PubMed

    Johansson, M B; Kristiansen, P T; Duda, L; Niklasson, G A; Österlund, L

    2016-11-30

    Nanocrystalline tungsten trioxide (WO3) thin films prepared by DC magnetron sputtering have been studied using soft x-ray spectroscopy and optical spectrophotometry. Resonant inelastic x-ray scattering (RIXS) measurements reveal band gap states in sub-stoichiometric γ-WO3-x with x  =  0.001-0.005. The energy positions of these states are in good agreement with recently reported density functional calculations. The results were compared with optical absorption measurements in the near infrared spectral region. An optical absorption peak at 0.74 eV is assigned to intervalence transfer of polarons between W sites. A less prominent peak at energies between 0.96 and 1.16 eV is assigned to electron excitation of oxygen vacancies. The latter results are supported by RIXS measurements, where an energy loss in this energy range was observed, and this suggests that electron transfer processes involving transitions from oxygen vacancy states can be observed in RIXS. Our results have implications for the interpretation of optical properties of WO3, and the optical transitions close to the band gap, which are important in photocatalytic and photoelectrochemical applications. PMID:27660919

  2. Band gap states in nanocrystalline WO3 thin films studied by soft x-ray spectroscopy and optical spectrophotometry

    NASA Astrophysics Data System (ADS)

    Johansson, M. B.; Kristiansen, P. T.; Duda, L.; Niklasson, G. A.; Österlund, L.

    2016-11-01

    Nanocrystalline tungsten trioxide (WO3) thin films prepared by DC magnetron sputtering have been studied using soft x-ray spectroscopy and optical spectrophotometry. Resonant inelastic x-ray scattering (RIXS) measurements reveal band gap states in sub-stoichiometric γ-WO3-x with x  =  0.001-0.005. The energy positions of these states are in good agreement with recently reported density functional calculations. The results were compared with optical absorption measurements in the near infrared spectral region. An optical absorption peak at 0.74 eV is assigned to intervalence transfer of polarons between W sites. A less prominent peak at energies between 0.96 and 1.16 eV is assigned to electron excitation of oxygen vacancies. The latter results are supported by RIXS measurements, where an energy loss in this energy range was observed, and this suggests that electron transfer processes involving transitions from oxygen vacancy states can be observed in RIXS. Our results have implications for the interpretation of optical properties of WO3, and the optical transitions close to the band gap, which are important in photocatalytic and photoelectrochemical applications.

  3. Band gap states in nanocrystalline WO3 thin films studied by soft x-ray spectroscopy and optical spectrophotometry.

    PubMed

    Johansson, M B; Kristiansen, P T; Duda, L; Niklasson, G A; Österlund, L

    2016-11-30

    Nanocrystalline tungsten trioxide (WO3) thin films prepared by DC magnetron sputtering have been studied using soft x-ray spectroscopy and optical spectrophotometry. Resonant inelastic x-ray scattering (RIXS) measurements reveal band gap states in sub-stoichiometric γ-WO3-x with x  =  0.001-0.005. The energy positions of these states are in good agreement with recently reported density functional calculations. The results were compared with optical absorption measurements in the near infrared spectral region. An optical absorption peak at 0.74 eV is assigned to intervalence transfer of polarons between W sites. A less prominent peak at energies between 0.96 and 1.16 eV is assigned to electron excitation of oxygen vacancies. The latter results are supported by RIXS measurements, where an energy loss in this energy range was observed, and this suggests that electron transfer processes involving transitions from oxygen vacancy states can be observed in RIXS. Our results have implications for the interpretation of optical properties of WO3, and the optical transitions close to the band gap, which are important in photocatalytic and photoelectrochemical applications.

  4. Spectrally-resolved Soft X-ray Observations and the Temperature Structure of the Solar Corona

    NASA Astrophysics Data System (ADS)

    Caspi, Amir; Warren, Harry; McTiernan, James; Woods, Thomas N.

    2015-04-01

    Solar X-ray observations provide important diagnostics of plasma heating and particle acceleration, during solar flares and quiescent periods. How the corona is heated to its ~1-3 MK nominal temperature remains one of the fundamental unanswered questions of solar physics; heating of plasma to tens of MK during solar flares -- particularly to the hottest observed temperatures of up to ~50 MK -- is also still poorly understood. Soft X-ray emission (~0.1-10 keV; or ~0.1-10 nm) is particularly sensitive to hot coronal plasma and serves as a probe of the thermal processes driving coronal plasma heating. Spectrally- and temporally-resolved measurements are crucial for understanding these energetic processes, but there have historically been very few such observations. We present new solar soft X-ray spectra from the Amptek X123-SDD, measuring quiescent solar X-ray emission from ~0.5 to ~30 keV with ~0.15 keV FWHM resolution from two SDO/EVE calibration sounding rocket underflights in 2012 and 2013. Combined with observations from RHESSI, GOES/XRS, SDO/EVE, and SDO/AIA, the temperature distribution derived from these data suggest significant hot (5-10 MK) emission from active regions, and the 2013 spectra suggest a low-FIP enhancement of only ~1.6 relative to the photosphere, 40% of the usually-observed value from quiescent coronal plasma. We explore the implications of these findings on coronal heating. We discuss future missions for spectrally-resolved soft X-ray observations using the X123-SDD, including the upcoming MinXSS 3U CubeSat using the X123-SDD and scheduled for deployment in mid-2015, and the CubIXSS 6U CubeSat mission concept.

  5. 3D nanoscale imaging of biological samples with laboratory-based soft X-ray sources

    NASA Astrophysics Data System (ADS)

    Dehlinger, Aurélie; Blechschmidt, Anne; Grötzsch, Daniel; Jung, Robert; Kanngießer, Birgit; Seim, Christian; Stiel, Holger

    2015-09-01

    In microscopy, where the theoretical resolution limit depends on the wavelength of the probing light, radiation in the soft X-ray regime can be used to analyze samples that cannot be resolved with visible light microscopes. In the case of soft X-ray microscopy in the water-window, the energy range of the radiation lies between the absorption edges of carbon (at 284 eV, 4.36 nm) and oxygen (543 eV, 2.34 nm). As a result, carbon-based structures, such as biological samples, posses a strong absorption, whereas e.g. water is more transparent to this radiation. Microscopy in the water-window, therefore, allows the structural investigation of aqueous samples with resolutions of a few tens of nanometers and a penetration depth of up to 10μm. The development of highly brilliant laser-produced plasma-sources has enabled the transfer of Xray microscopy, that was formerly bound to synchrotron sources, to the laboratory, which opens the access of this method to a broader scientific community. The Laboratory Transmission X-ray Microscope at the Berlin Laboratory for innovative X-ray technologies (BLiX) runs with a laser produced nitrogen plasma that emits radiation in the soft X-ray regime. The mentioned high penetration depth can be exploited to analyze biological samples in their natural state and with several projection angles. The obtained tomogram is the key to a more precise and global analysis of samples originating from various fields of life science.

  6. The Soft X-Ray Emission in a Large Sample of Galaxy Clusters with ROSAT PSPC

    NASA Technical Reports Server (NTRS)

    Bonamente, Massimiliano; Lieu, Richard; Joy, Marshall K.; Nevalainen, Jukka H.; Six, N. Frank (Technical Monitor)

    2002-01-01

    The study of soft X-ray emission of 38 X-ray selected galaxy clusters observed by ROSAT PSPC indicates that the soft excess phenomenon may be a common occurrence in galaxy clusters. Excess soft X-ray radiation, above the contribution from the hot intra-cluster medium, is evident in a large fraction of sources, and is clearly detected with large statistical significance in the deepest observations. The investigation relies on new, high resolution 21 cm HI observations. The sample selection also features analysis of infrared images, to further ensure reliability of results with respect to the characteristics of Galactic absorption. The possibility of background or calibration effects as cause of the excess emission is likewise investigated; a detailed analysis of the distribution of the excess emission with respect to detector position and Galactic HI column density shows that the excess emission is a genuine celestial phenomenon. We find evidence for a preferential distribution of the soft excess emission at distances larger than approx. 150-200 kpc from the centers of clusters; this behavior may be naturally explained in the context of a non-thermal Inverse-Compton scenario. Alternatively, we propose that the phenomenon maybe caused by thermal emission of very large-scale 'warm' filaments seen in recent hydrodynamic simulations. This new interpretation relieves the very demanding requirements of either the traditional intra-cluster 'warm' gas and the non-thermal scenarios. We also investigate the possibility of the soft excess originating from unresolved, X-ray faint cluster galaxies.

  7. Dante soft x-ray power diagnostic for National Ignition Facility

    NASA Astrophysics Data System (ADS)

    Dewald, E. L.; Campbell, K. M.; Turner, R. E.; Holder, J. P.; Landen, O. L.; Glenzer, S. H.; Kauffman, R. L.; Suter, L. J.; Landon, M.; Rhodes, M.; Lee, D.

    2004-10-01

    Soft x-ray power diagnostics are essential for measuring the total x-ray flux, radiation temperature, conversion efficiency, and albedo that define the energetics in indirect and direct drive, as well as other types of high temperature laser plasma experiments. A key diagnostic for absolute radiation flux and radiation temperature in hohlraum experiments is the Dante broadband soft x-ray spectrometer. For the extended range of x-ray fluxes predicted for National Ignition Facility (NIF) compared to Omega or Nova hohlraums, the Dante spectrometer for NIF will include more high energy (<2 keV) edge filter band-pass channels and access to an increased dynamic range using grids and signal division. This will allow measurements of radiation fluxes of between 0.01 to 100 TW/sr, for hohlraum radiation temperatures between 50 eV and 1 keV. The NIF Dante will include a central four-channel imaging line-of-sight to verify the source size, alignment as well as checking for any radiation contributions from unconverted laser light plasmas.

  8. Multiphoton Ionization of Atoms and Molecules with Soft and Hard X-rays

    NASA Astrophysics Data System (ADS)

    Rolles, Daniel

    2015-05-01

    We have recently extended our previous investigations of the multiphoton ionization of heavy atoms, such as Kr and Xe, and of high-Z atom containing molecules from the soft into the hard X-ray range as well as into the XUV regime. Using the 100-nm focus environment at LCLS, we were able to reach peak intensities up to 1019W/cm2 at photon energies between 5 to 9 keV. This allows studying atomic and molecular ionization processes under unprecedented X-ray intensities and, in particular, under the identical conditions where typical coherent diffractive imaging experiments are performed. Our results are thus important benchmarks for calculating radiation damage effects in FEL-based X-ray imaging experiments. Using new micro-focusing capabilities at FLASH, we also extended our studies into the XUV range between 70 and 200 eV photon energy and observed significantly higher charge states than previously reported. I will present the results from our recent measurements at LCLS and FLASH and discuss the different multiphoton ionization mechanisms that play a role in the XUV, soft, and hard X-ray range.

  9. Analysis of neon soft x-ray spectra from short-pulse laser-produced plasmas

    SciTech Connect

    Abare, A.C.; Keane, C.J.; Crane, J.K.; DaSilva, L.B.; Lee, R.W.; Perry, M.D.; Falcone, R.W.

    1993-04-01

    We report preliminary results from the analysis of streaked soft x-ray neon spectra obtained from the interaction of a picosecond Nd:glass laser with a gas jet target. In these experiments streaked spectra show prompt harmonic emission followed by longer time duration soft x-ray line emission. The majority of the line emission observed was found to originate from Li- and Be-like Ne and the major transitions in the observed spectra have been identified. Li-like emission lines were observed to decay faster in time than Be-like transitions, suggesting that recombination is taking place. Line ratios of n=4-2 and n=3-2 transitions supported the view that these lines were optically thin and thick, respectively. The time history of Li-like Ne 2p-4d and 2p-3d lines is in good agreement with a simple adiabatic expansion model coupled to a time dependent collisional-radiative code. Further x-ray spectroscopic analysis is underway which is aimed at diagnosing plasma conditions and assessing the potential of this recombining neon plasma as a quasi-steady-state recombination x-ray laser medium.

  10. Absolute pulse energy measurements of soft x-rays at the Linac Coherent Light Source.

    PubMed

    Tiedtke, K; Sorokin, A A; Jastrow, U; Juranić, P; Kreis, S; Gerken, N; Richter, M; Arp, U; Feng, Y; Nordlund, D; Soufli, R; Fernández-Perea, M; Juha, L; Heimann, P; Nagler, B; Lee, H J; Mack, S; Cammarata, M; Krupin, O; Messerschmidt, M; Holmes, M; Rowen, M; Schlotter, W; Moeller, S; Turner, J J

    2014-09-01

    This paper reports novel measurements of x-ray optical radiation on an absolute scale from the intense and ultra-short radiation generated in the soft x-ray regime of a free electron laser. We give a brief description of the detection principle for radiation measurements which was specifically adapted for this photon energy range. We present data characterizing the soft x-ray instrument at the Linac Coherent Light Source (LCLS) with respect to the radiant power output and transmission by using an absolute detector temporarily placed at the downstream end of the instrument. This provides an estimation of the reflectivity of all x-ray optical elements in the beamline and provides the absolute photon number per bandwidth per pulse. This parameter is important for many experiments that need to understand the trade-offs between high energy resolution and high flux, such as experiments focused on studying materials via resonant processes. Furthermore, the results are compared with the LCLS diagnostic gas detectors to test the limits of linearity, and observations are reported on radiation contamination from spontaneous undulator radiation and higher harmonic content. PMID:25321502

  11. Analysis of neon soft x-ray spectra from short-pulse laser-produced plasmas

    NASA Astrophysics Data System (ADS)

    Abare, Amber C.; Keane, Christopher J.; Crane, John K.; Da Silva, Luiz B.; Lee, Richard W.; Perry, Michael D.; Falcone, Roger W.

    1993-07-01

    We report preliminary results from the analysis of streaked soft x-ray neon spectra obtained from the interaction of a picosecond Nd:glass laser with a gas jet target. In these experiments streaked spectra show prompt harmonic emission followed by longer time duration soft x-ray line emission. The majority of the line emission observed was found to originate from Li- and Be-like Ne and the major transitions in the observed spectra have been identified. Li-like emission lines were observed to decay faster in time than Be-like transitions, suggesting that recombination is taking place. Line ratios of n equals 4 - 2 and n equals 3 - 2 transitions supported the view that these lines were optically thin and thick, respectively. The time history of Li-like Ne 2p-4d and 2p-3d lines is in good agreement with a simple adiabatic expansion model coupled to a time dependent collisional-radiative code. Further x-ray spectroscopic analysis is underway which is aimed at diagnosing plasma conditions and assessing the potential of this recombining neon plasma as a quasi-steady-state recombination x-ray laser medium.

  12. The Ultraviolet Surprise. Efficient Soft X-Ray High Harmonic Generation in Multiply-Ionized Plasmas

    SciTech Connect

    Popmintchev, Dimitar; Hernandez-Garcia, Carlos; Dollar, Franklin; Mancuso, Christopher; Perez-Hernandez, Jose A.; Chen, Ming-Chang; Hankla, Amelia; Gao, Xiaohui; Shim, Bonggu; Gaeta, Alexander L.; Tarazkar, Maryam; Romanov, Dmitri A.; Levis, Robert J.; Gaffney, Jim A.; Foord, Mark; Libby, Stephen B.; Jaron-Becker, Agnieskzka; Becker, Andreas; Plaja, Luis; Muranane, Margaret M.; Kapteyn, Henry C.; Popmintchev, Tenio

    2015-12-04

    High-harmonic generation is a universal response of matter to strong femtosecond laser fields, coherently upconverting light to much shorter wavelengths. Optimizing the conversion of laser light into soft x-rays typically demands a trade-off between two competing factors. Reduced quantum diffusion of the radiating electron wave function results in emission from each species which is highest when a short-wavelength ultraviolet driving laser is used. But, phase matching—the constructive addition of x-ray waves from a large number of atoms—favors longer-wavelength mid-infrared lasers. We identified a regime of high-harmonic generation driven by 40-cycle ultraviolet lasers in waveguides that can generate bright beams in the soft x-ray region of the spectrum, up to photon energies of 280 electron volts. Surprisingly, the high ultraviolet refractive indices of both neutral atoms and ions enabled effective phase matching, even in a multiply ionized plasma. We observed harmonics with very narrow linewidths, while calculations show that the x-rays emerge as nearly time-bandwidth–limited pulse trains of ~100 attoseconds.

  13. The Ultraviolet Surprise. Efficient Soft X-Ray High Harmonic Generation in Multiply-Ionized Plasmas

    DOE PAGES

    Popmintchev, Dimitar; Hernandez-Garcia, Carlos; Dollar, Franklin; Mancuso, Christopher; Perez-Hernandez, Jose A.; Chen, Ming-Chang; Hankla, Amelia; Gao, Xiaohui; Shim, Bonggu; Gaeta, Alexander L.; et al

    2015-12-04

    High-harmonic generation is a universal response of matter to strong femtosecond laser fields, coherently upconverting light to much shorter wavelengths. Optimizing the conversion of laser light into soft x-rays typically demands a trade-off between two competing factors. Reduced quantum diffusion of the radiating electron wave function results in emission from each species which is highest when a short-wavelength ultraviolet driving laser is used. But, phase matching—the constructive addition of x-ray waves from a large number of atoms—favors longer-wavelength mid-infrared lasers. We identified a regime of high-harmonic generation driven by 40-cycle ultraviolet lasers in waveguides that can generate bright beams inmore » the soft x-ray region of the spectrum, up to photon energies of 280 electron volts. Surprisingly, the high ultraviolet refractive indices of both neutral atoms and ions enabled effective phase matching, even in a multiply ionized plasma. We observed harmonics with very narrow linewidths, while calculations show that the x-rays emerge as nearly time-bandwidth–limited pulse trains of ~100 attoseconds.« less

  14. Broad-band soft x-ray diagnostic instruments at the LLNL Novette laser facility

    SciTech Connect

    Tirsell, K.G.; Lee, P.H.Y.; Nilson, D.G.; Medecki, H.

    1983-09-15

    Complementary broad-band instruments have been developed to measure time dependent, absolute soft x-ray spectra at the Lawrence Livermore National Laboratory (LLNL) Nd glass laser irradiation facilities. Absolute flux measurements of x rays emitted from laser-produced plasmas are important for understanding laser absorption and energy transport. We will describe two new 10-channel XRD systems that have been installed at the LLNL Novette facility for use in the 0.15- to 1.5-keV range. Since XRD channel time response is limited by available oscilloscope performance to 120 ps, a soft x-ray streak camera has been developed for better time resolution (20 ps) and greater dynamic range (approx.10/sup 3/) in the same x-ray energy region. Using suitable filters, grazing incidence mirrors, and a gold or cesium-iodide transmission cathode, this streak camera instrument has been installed at Novette to provide one broad and four relatively narrow channels. It can also be used in a single channel, spatially discriminating mode by means of pinhole imaging. The complementary nature of these instruments has been enhanced by locating them in close proximity and matching their channel energy responses. As an example of the use of these instruments, we present results from Novette 2..omega..(0.53 ..mu..m) gold disk irradiations at 1 ns and 10/sup 14/ to 10/sup 15/ W/cm/sup 2/.

  15. Discovery of an Extraordinary Luminous And Soft X-ray Transient MAXI J0158-744

    NASA Astrophysics Data System (ADS)

    Morii, Mikio; Tomida, Hiroshi; Kimura, Masaki; Suwa, Fumitoshi; Negoro, Hitoshi; Serino, Motoko; Kennea, Jamie A.; Page, Kim L.; Curran, Peter A.; Walter, Frederick M.; Kuin, N. Paul. M.; Pritchard, Tyler; Nakahira, Satoshi; Hiroi, Kazuo; Usui, Ryuichi; Kawai, Nobuyuki; Osborne, Julian P.; Mihara, Tatehiro; Burrows, David N.; Gehrels, Neil; Kohama, Mitsuhiro; Matsuoka, Masaru; Nakajima, Motoki; Roming, Peter W. A.; Sugimori, Kousuke; Sugizaki, Mutsumi; Tsuboi, Yohko; Tsunemi, Hiroshi; Ueda, Yoshihiro; Ueno, Shiro; Yoshida, Atsumasa

    Monitor of All-sky X-ray Image (MAXI) is an X-ray all-sky monitor in operation now. MAXI GSC and SSC are sensitive in the 2-30 and 0.5-12 keV bands, respectively. On November 11, 2011 (UT), MAXI GSC discovered an unusually luminous and soft X-ray transient, MAXI J0158-744, on the outskirts of the Small Magellanic Cloud (SMC). The outburst lasted for no more than three hours and the luminosity peaked at ˜1040 erg s-1. By the Swift follow-up observation and the optical spectroscopy, we find that the transient was a kind of the nova explosion on a white dwarf in a binary paired with a Be star. We discuss that the outburst can be explained as shock-induced emission caused by a nova explosion in a dense circumstellar medium around a Be star or a photospheric emission on an ignition of a nova explosion. Its fast optical decay (t2 = 1.9 ± 0.2 days) and extremely early turn-on (<0.44 days) of the super-soft X-ray phase suggest that the white dwarf is very massive.

  16. Transverse dynamics of water across the melting point: A parallel neutron and x-ray inelastic scattering study

    SciTech Connect

    Cunsolo A.; Kodituwakku C.; Bencivenga, F.; Frontzek, M.; Leu, b.M.; Said, A.H.

    2012-05-29

    Joint inelastic neutron and x-ray scattering measurements have been performed on heavy water across the melting point. The spectra bear clear evidence of low- and high-frequency inelastic shoulders related to transverse and longitudinal modes, respectively. Upon increasing the momentum transfer, the spectral shape evolves from a viscoelastic regime, where the low-frequency mode is clearly over-damped, toward an elastic one where its propagation becomes instead allowed. The crossover between the two regimes occurs whenever both the characteristic frequency and the linewidth of the low-frequency mode match the inverse of the structural relaxation time. Furthermore, we observe that the frequency of the transverse mode undergoes a discontinuity across the melting, whose extent reduces upon increasing the exchanged momentum.

  17. Resonant Soft X-Ray Contrast Variation Methods as Composition-Specific Probes of Thin Polymer Film Structure

    SciTech Connect

    Welch, Cynthia; Welch, Cynthia F.; Hjelm, Rex P.; Mang, Joseph T.; Hawley, Marilyn E.; Wrobleski, Debra A.; Orler, E. Bruce; Kortright, Jeffrey B

    2008-04-04

    We have developed complementary soft x-ray scattering and reflectometry techniques that allow for the morphological analysis of thin polymer films without resorting to chemical modification or isotopic 2 labeling. With these techniques, we achieve significant, x-ray energy-dependent contrast between carbon atoms in different chemical environments using soft x-ray resonance at the carbon edge. Because carbon-containing samples absorb strongly in this region, the scattering length density depends on both the real and imaginary parts of the atomic scattering factors. Using a model polymer film of poly(styrene-b-methyl methacrylate), we show that the soft x-ray reflectivity data is much more sensitive to these atomic scattering factors than the soft x-ray scattering data. Nevertheless, fits to both types of data yield useful morphological details on the polymer?slamellar structure that are consistent with each other and with literature values.

  18. Inelastic x-ray scattering study of supercooled liquid and solid silicon.

    SciTech Connect

    Alatas, A.; Said, A.; Sinn, H.; Alp, E.E.; Kodituwakku, C.N.; Saboungi, M.L.; Price, D.L.; X-Ray Science Division; Western Michigan Univ.; Purdue Univ.; CRMD-CNRS; CRMHT-CNRS

    2006-01-01

    Momentum-resolved inelastic x-ray scattering (IXS) technique is one of the powerful methods for the study of dynamical properties of a given system even in extreme conditions like high temperature and high pressure. At the same time, experimental studies of physical and structural properties of liquids have multiplied in recent years with the advent of containerless techniques. These methods reduce the possibility of contamination of specimens and remove external nucleation sites. Therefore, by combining the IXS method with the levitation method, the dynamical properties of stable liquids up to 3000 K and supercooled phase of liquids can be studied. Silicon is a basic material in the semiconductor industry and has been the subject of a large amount of experimental and theoretical studies over a long time. In the crystalline phase at ambient conditions, silicon is a diamond-structured semiconductor, but upon melting it undergoes a semiconductor-to-metal transition accompanied by significant changes in the structure and density. The coordination number increases from 4 in the solid to about 6.5 in the liquid, and liquid density is increased by about 10%. The principal purpose of the present study was to determine silicon's elastic modulus from the measurement of averaged sound speed determined from IXS. The experiments were carried out at the Advanced Photon Source (APS) beamline 3-ID with a high-resolution monochromator consisting of two nested channel-cut crystals and four backscattering analyzer setups in the horizontal scattering plane 6 m from the sample. The requirements for very high energy resolution and the basic principles of such instrumentation are discussed elsewhere as referenced. The levitation apparatus was enclosed in a bell jar specially designed for backscattering geometry with a separation of 10 cm between the sample and the detector. Silicon spheres of 2 to 3 mm in diameter were suspended in an argon gas jet and heated with a 270 W CO{sub 2

  19. X-Ray Point Sources in the Sombrero Galaxy: Very Soft Sources, the Globular Cluster/Low-Mass X-Ray Binary Connection, and an Overview

    NASA Astrophysics Data System (ADS)

    Di Stefano, R.; Kong, A. K. H.; VanDalfsen, M. L.; Harris, W. E.; Murray, S. S.; Delain, K. M.

    2003-12-01

    We report on the population of point sources discovered during an 18.5 ks Chandra ACIS-S observation of the Sombrero galaxy. We present the luminosity function and the spectra of the six brightest sources, consider correlations with globular clusters (GCs) and with planetary nebulae, and study the galaxy's population of very soft sources. We detected 122 sources. Twenty-two sources are identified as very soft; of these, five appear to be classical luminous supersoft X-ray sources (SSSs), while 17 may belong to the slightly harder class referred to as quasi-soft (QSSs). There is an overdensity of very soft sources within 2 kpc of the nucleus, which is itself the brightest X-ray source. Very soft sources are also found in the disk and halo, with one QSS in a globular cluster (GC). This source is somewhat harder than most SSSs; the energy distribution of its photons is consistent with what is expected from an accreting intermediate-mass black hole. Several sources in the Sombrero's halo are good candidates for SSS models in which the accretor is a nuclear-burning white dwarf. In total, 32 X-ray sources are associated with GCs. The majority of sources with luminosity greater than 1038 ergs s-1 are in GCs. These results for M104, an Sa galaxy, are similar to what has been found for elliptical galaxies and for the late-type spiral M31. We find that those optically bright GCs with X-ray sources house only the brightest X-ray sources. We find that, in common with other galaxies, there appears to be a positive connection between young (metal-rich) GCs and X-ray sources but that the brightest X-ray sources are equally likely to be in metal-poor GCs. The luminosity function of X-ray sources in GCs has a cut-off near the Eddington luminosity for a 1.4 Msolar object. We propose a model that can explain the trends seen in the data sets from the Sombrero and other galaxies. Thermal timescale mass transfer can occur in some of the younger clusters in which the turnoff mass is

  20. Improving the spatial resolution of soft X-ray detection using an Electron-Multiplying Charge-Coupled Device

    NASA Astrophysics Data System (ADS)

    Soman, M. R.; Hall, D. J.; Tutt, J. H.; Murray, N. J.; Holland, A. D.; Schmitt, T.; Raabe, J.; Schmitt, B.

    2013-01-01

    The Super Advanced X-ray Emission Spectrometer (SAXES) is an instrument at the Swiss Light Source designed for Resonant Inelastic X-ray Scattering with an energy resolution (E/ΔE) better than 12000 at 930 eV. Improvements to the instrument have been predicted that could allow the energy resolution to be improved by a factor of two. To achieve this, the spatial resolution of the detector (currently a Charge-Coupled Device, CCD) over which the energy spectrum is dispersed would have to be improved to better than 5 μm. X-ray photons with energies between a few hundred to a few thousand electron volts primarily interact within the field-free region of back-illuminated CCDs, where each photon forms an electron cloud that diffuses isotropically before reaching the depleted region close to the electrodes. Each photon's electron cloud is likely to be detected as an event with signal split across multiple pixels. Analysing these split events using centroiding techniques allows the photon's interaction position to be determined to a sub-pixel level. PolLux is a soft X-ray microspectroscopy endstation at the Swiss Light Source that can focus 200 eV to 1200 eV X-rays to a spot size of approximately 20 nm. Previous studies using data taken with a linear scan across the centre of a pixel in 3 μm steps predicted an improved resolution by applying centroiding techniques and using an Electron-Multiplying CCD (EM-CCD). In this study, a full 2D map of the centroiding accuracy in the pixel is presented, formed by rastering in two dimensions across the image plane in single micron steps. The improved spatial resolution from centroiding events in the EM-CCD in all areas of the pixel over the standard CCD is attributed to the improved signal to noise ratio provided by the multiplication register even at high pixel readout speeds (tens of MHz).

  1. 0.5-keV Soft X-ray attosecond continua

    PubMed Central

    Teichmann, S. M.; Silva, F.; Cousin, S. L.; Hemmer, M.; Biegert, J.

    2016-01-01

    Attosecond light pulses in the extreme ultraviolet have drawn a great deal of attention due to their ability to interrogate electronic dynamics in real time. Nevertheless, to follow charge dynamics and excitations in materials, element selectivity is a prerequisite, which demands such pulses in the soft X-ray region, above 200 eV, to simultaneously cover several fundamental absorption edges of the constituents of the materials. Here, we experimentally demonstrate the exploitation of a transient phase matching regime to generate carrier envelope controlled soft X-ray supercontinua with pulse energies up to 2.9±0.1 pJ and a flux of (7.3±0.1) × 107 photons per second across the entire water window and attosecond pulses with 13 as transform limit. Our results herald attosecond science at the fundamental absorption edges of matter by bridging the gap between ultrafast temporal resolution and element specific probing. PMID:27167525

  2. Soft x-ray camera for internal shape and current density measurements on a noncircular tokamak

    SciTech Connect

    Fonck, R.J.; Jaehnig, K.P.; Powell, E.T.; Reusch, M.; Roney, P.; Simon, M.P.

    1988-05-01

    Soft x-ray measurements of the internal plasma flux surface shaped in principle allow a determination of the plasma current density distribution, and provide a necessary monitor of the degree of internal elongation of tokamak plasmas with a noncircular cross section. A two-dimensional, tangentially viewing, soft x-ray pinhole camera has been fabricated to provide internal shape measurements on the PBX-M tokamak. It consists of a scintillator at the focal plane of a foil-filtered pinhole camera, which is, in turn, fiber optically coupled to an intensified framing video camera (/DELTA/t />=/ 3 msec). Automated data acquisition is performed on a stand-alone image-processing system, and data archiving and retrieval takes place on an optical disk video recorder. The entire diagnostic is controlled via a PDP-11/73 microcomputer. The derivation of the polodial emission distribution from the measured image is done by fitting to model profiles. 10 refs., 4 figs.

  3. High average power, highly brilliant laser-produced plasma source for soft X-ray spectroscopy.

    PubMed

    Mantouvalou, Ioanna; Witte, Katharina; Grötzsch, Daniel; Neitzel, Michael; Günther, Sabrina; Baumann, Jonas; Jung, Robert; Stiel, Holger; Kanngiesser, Birgit; Sandner, Wolfgang

    2015-03-01

    In this work, a novel laser-produced plasma source is presented which delivers pulsed broadband soft X-radiation in the range between 100 and 1200 eV. The source was designed in view of long operating hours, high stability, and cost effectiveness. It relies on a rotating and translating metal target and achieves high stability through an on-line monitoring device using a four quadrant extreme ultraviolet diode in a pinhole camera arrangement. The source can be operated with three different laser pulse durations and various target materials and is equipped with two beamlines for simultaneous experiments. Characterization measurements are presented with special emphasis on the source position and emission stability of the source. As a first application, a near edge X-ray absorption fine structure measurement on a thin polyimide foil shows the potential of the source for soft X-ray spectroscopy. PMID:25832284

  4. Soft X-Ray Absorption Spectroscopy of High-Abrasion-Furnace Carbon Black

    SciTech Connect

    Muramatsu, Yasuji; Harada, Ryusuke; Gullikson, Eric M.

    2007-02-02

    The soft x-ray absorption spectra of high-abrasion-furnace carbon black were measured to obtain local-structure/chemical-states information of the primary particles and/or crystallites. The soft x-ray absorption spectral features of carbon black represent broader {pi}* and {sigma}* peak structures compared to highly oriented pyrolytic graphite (HOPG). The subtracted spectra between the carbon black and HOPG, (carbon black) - (HOPG), show double-peak structures on both sides of the {pi}* peak. The lower-energy peak, denoted as the 'pre-peak', in the subtracted spectra and the {pi}*/{sigma}* peak intensity ratio in the absorption spectra clearly depend on the specific surface area by nitrogen adsorption (NSA). Therefore, it is concluded that the pre-peak intensity and the {pi}*/{sigma}* ratio reflect the local graphitic structure of carbon black.

  5. An extended soft X-ray source in Delphinus - H2027+19

    NASA Technical Reports Server (NTRS)

    Stern, R. A.; Walker, A. B. C.; Charles, P. A.; Nugent, J. J.; Garmire, G. P.

    1980-01-01

    A new extended soft X-ray source has been observed with the HEAO 1 A-2 experiment. The source, H2027+19, emits primarily in the 0.16-0.4 keV band with a total flux in this band of 2 x 10 to the -11th erg/sq cm s. It is found that both simple continuum and coronal plasma models provide good fits to the observed pulse-height spectrum. The most likely physical models are either that the source is an old supernova remnant or that it is a region of enhanced soft X-ray emission surrounding an H I cloud imbedded in a coronal plasma, as suggested by Hayakawa et al. (1979) for the Lupus Loop.

  6. Optics Design for a Soft X-ray FEL at the SLAC A-Line

    SciTech Connect

    Geng, H; Ding, Y.; Emma, P.; Huang, Z.; Nosochkov, Y.; Woodley, M.; /SLAC

    2009-05-15

    LCLS capabilities can be significantly extended with a second undulator aiming at the soft x-ray spectrum (1-5 nm). To allow for simultaneous hard and soft x-ray operations, 14 GeV beams at the end of the LCLS accelerator can be intermittently switched into the SLAC A-line (the beam transport line to End Station A) where the second undulator may be located. In this paper, we discuss the A-line optics design for transporting the high-brightness LCLS beams using the existing tunnel. To preserve the high brightness of the LCLS beams, special attention is paid to effects of incoherent and coherent synchrotron radiation. Start-to-end simulations using realistic LCLS beam distributions are carried out.

  7. Resolving new ultrastructural features of cytokinetic abscission with soft-X-ray cryo-tomography

    PubMed Central

    Sherman, Shachar; Kirchenbuechler, David; Nachmias, Dikla; Tamir, Adi; Werner, Stephan; Elbaum, Michael; Elia, Natalie

    2016-01-01

    Mammalian cytokinetic abscission is mediated by the ESCRT membrane fission machinery. While much has been clarified on the topology and kinetics of abscission through high-resolution microscopy, key questions regarding the mechanism of abscission remain open. Here we apply cryogenic soft-X-ray tomography to elucidate new ultrastructural details in the intercellular membrane bridge connecting cells undergoing abscission. In particular, we resolve defined ring-like structures inside the midbody dark zone that have been inaccessible to EM, and identify membrane extrusions at the abscission sites. In cells at late stages of abscission we resolve a complex array of helical spirals, extending the structural information obtained by EM. Our results highlight the advantages of soft-X-ray tomography and emphasize the importance of using complementary approaches for characterizing cellular structures. Notably, by providing new structural data from intact cells we present a realistic view on the topology of abscission and suggest new mechanistic models for ESCRT mediated abscission. PMID:27282220

  8. Molecular bond selective x-ray scattering for nanoscale analysisof soft matter

    SciTech Connect

    Mitchell, G.E.; Koprinarov, I.; Landes, B.G.; Lyons, J.; Kern,B.J.; Devon, M.J.; Gullikson, E.M.; Kortright, J.B.

    2005-05-26

    We introduce a new technique using resonant soft x-ray scattering for characterizing heterogeneous chemical structure at nanometer length scales in polymers, biological material, and other soft matter. Resonant enhancements bring new contrast mechanisms and increased sensitivity to bridge a gap between bond-specific contrast in chemical sensitive imaging and the higher spatial resolution of traditional small-angle scattering techniques. We illustrate sensitivity to chemical bonding with the resonant scattering near the carbon K edge from latex spheres of differing chemistry and sizes. By tuning to x-ray absorption resonances associated with particular carbon-carbon or carbon-oxygen bonds we can isolate the scattering from different phases in a 2-phase mixture. We then illustrate this increased scattering contrast with a study of the templating process to form nanometer scale pores in 100 nm thick polymer films.

  9. Resolving new ultrastructural features of cytokinetic abscission with soft-X-ray cryo-tomography.

    PubMed

    Sherman, Shachar; Kirchenbuechler, David; Nachmias, Dikla; Tamir, Adi; Werner, Stephan; Elbaum, Michael; Elia, Natalie

    2016-01-01

    Mammalian cytokinetic abscission is mediated by the ESCRT membrane fission machinery. While much has been clarified on the topology and kinetics of abscission through high-resolution microscopy, key questions regarding the mechanism of abscission remain open. Here we apply cryogenic soft-X-ray tomography to elucidate new ultrastructural details in the intercellular membrane bridge connecting cells undergoing abscission. In particular, we resolve defined ring-like structures inside the midbody dark zone that have been inaccessible to EM, and identify membrane extrusions at the abscission sites. In cells at late stages of abscission we resolve a complex array of helical spirals, extending the structural information obtained by EM. Our results highlight the advantages of soft-X-ray tomography and emphasize the importance of using complementary approaches for characterizing cellular structures. Notably, by providing new structural data from intact cells we present a realistic view on the topology of abscission and suggest new mechanistic models for ESCRT mediated abscission. PMID:27282220

  10. A multi-frame soft x-ray pinhole imaging diagnostic for single-shot applications.

    PubMed

    Wurden, G A; Coffey, S K

    2012-10-01

    For high energy density magnetized target fusion experiments at the Air Force Research Laboratory FRCHX machine, obtaining multi-frame soft x-ray images of the field reversed configuration (FRC) plasma as it is being compressed will provide useful dynamics and symmetry information. However, vacuum hardware will be destroyed during the implosion. We have designed a simple in-vacuum pinhole nosecone attachment, fitting onto a Conflat window, coated with 3.2 mg∕cm(2) of P-47 phosphor, and covered with a thin 50-nm aluminum reflective overcoat, lens-coupled to a multi-frame Hadland Ultra intensified digital camera. We compare visible and soft x-ray axial images of translating (~200 eV) plasmas in the FRX-L and FRCHX machines in Los Alamos and Albuquerque.

  11. High average power, highly brilliant laser-produced plasma source for soft X-ray spectroscopy

    SciTech Connect

    Mantouvalou, Ioanna; Grötzsch, Daniel; Neitzel, Michael; Günther, Sabrina; Baumann, Jonas; Kanngießer, Birgit; Witte, Katharina; Jung, Robert; Stiel, Holger; Sandner, Wolfgang

    2015-03-15

    In this work, a novel laser-produced plasma source is presented which delivers pulsed broadband soft X-radiation in the range between 100 and 1200 eV. The source was designed in view of long operating hours, high stability, and cost effectiveness. It relies on a rotating and translating metal target and achieves high stability through an on-line monitoring device using a four quadrant extreme ultraviolet diode in a pinhole camera arrangement. The source can be operated with three different laser pulse durations and various target materials and is equipped with two beamlines for simultaneous experiments. Characterization measurements are presented with special emphasis on the source position and emission stability of the source. As a first application, a near edge X-ray absorption fine structure measurement on a thin polyimide foil shows the potential of the source for soft X-ray spectroscopy.

  12. A multi-frame soft x-ray pinhole imaging diagnostic for single-shot applications

    SciTech Connect

    Wurden, G. A.; Coffey, S. K.

    2012-10-15

    For high energy density magnetized target fusion experiments at the Air Force Research Laboratory FRCHX machine, obtaining multi-frame soft x-ray images of the field reversed configuration (FRC) plasma as it is being compressed will provide useful dynamics and symmetry information. However, vacuum hardware will be destroyed during the implosion. We have designed a simple in-vacuum pinhole nosecone attachment, fitting onto a Conflat window, coated with 3.2 mg/cm{sup 2} of P-47 phosphor, and covered with a thin 50-nm aluminum reflective overcoat, lens-coupled to a multi-frame Hadland Ultra intensified digital camera. We compare visible and soft x-ray axial images of translating ({approx}200 eV) plasmas in the FRX-L and FRCHX machines in Los Alamos and Albuquerque.

  13. Ablation gas dynamics of low-Z materials illuminated by soft x-rays

    SciTech Connect

    Hatchett, S.P.

    1991-09-06

    Though many of our results will have much greater generality, the main purpose of this paper is to provide a simple, accurate, physical theory of what happens when a Planckian spectrum of soft x-rays is incident on one side of the slab of initially cold, dense material, of small nuclear charge Z. Our approach will be to consider in some detail the idealized situation. A semi-infinite (x {le} 0) slab of initially cold (T < 300 K), dense ({rho} {approximately} 1 {minus} 10 g/cc), low-Z (Z < 5) material is suddenly subjected at time t = 0 and thereafter to radiation incoming from x = +{infinity} with a specific intensity in directions toward the slab that is Planckian, characterized by a black-body temperature, T{sub R} in the soft x-ray region.

  14. Soft x-ray magneto-optic Kerr rotation and element-specific hysteresis measurement

    SciTech Connect

    Kortright, J.B.; Rice, M.

    1996-03-01

    Soft x-ray magneto-optic Kerr rotation has been measured using a continuously tunable multilayer linear polarizer in the beam reflected form samples in applied magnetic fields. Like magnetic circular dichroism, Kerr rotation in the soft x-ray can be element - specific and much larger than in the visible spectral range when the photon energy is tuned near atomic core resonances. Thus sensitive element-specific hysteresis measurements are possible with this technique. Examples showing large Kerr rotation from an Fe film and element-specific hysteresis loops of the Fe and Cr in an Fe/Cr multilayer demonstrate these new capabilities. Some consequences of the strong anomalous dispersion near the FeL{sub 2,3} edges to the Kerr rotation are discussed.

  15. New soft X-ray beamline BL07LSU at SPring-8

    PubMed Central

    Yamamoto, Susumu; Senba, Yasunori; Tanaka, Takashi; Ohashi, Haruhiko; Hirono, Toko; Kimura, Hiroaki; Fujisawa, Masami; Miyawaki, Jun; Harasawa, Ayumi; Seike, Takamitsu; Takahashi, Sunao; Nariyama, Nobuteru; Matsushita, Tomohiro; Takeuchi, Masao; Ohata, Toru; Furukawa, Yukito; Takeshita, Kunikazu; Goto, Shunji; Harada, Yoshihisa; Shin, Shik; Kitamura, Hideo; Kakizaki, Akito; Oshima, Masaharu; Matsuda, Iwao

    2014-01-01

    A new soft X-ray beamline, BL07LSU, has been constructed at SPring-8 to perform advanced soft X-ray spectroscopy for materials science. The beamline is designed to achieve high energy resolution (E/ΔE> 10000) and high photon flux [>1012 photons s−1 (0.01% bandwidth)−1] in the photon energy range 250–2000 eV with controllable polarization. To realise this state-of-the-art performance, a novel segmented cross undulator was developed and adopted as a light source. The details of the undulator light source and beamline monochromator design are described. The achieved performance of the beamline, such as the photon flux, energy resolution and the state of polarization, is reported. PMID:24562556

  16. Soft x-ray spectroscopy undulator beamline at the Advanced Photon Source

    SciTech Connect

    Randall, K.J.; Xu, Z.; Moore, J.F.; Gluskin, E.

    1997-09-01

    Construction of the high-resolution soft x ray spectroscopy undulator beamline, 2ID-C, at the Advanced Photon Source (APS) has been completed. The beamline, one of two soft x ray beamlines at the APS, will cover the photon energy range from 500 to 3,000 eV, with a maximum resolving power between 7,000 and 14,000. The optical design is based on a spherical grating monochromator (SGM) giving both high resolution and high flux throughput. Photon flux is calculated to be approximately 10{sup 12}--10{sup 13} photons per second with a beam size of approximately 1 x 1 mm{sup 2} at the sample.

  17. High average power, highly brilliant laser-produced plasma source for soft X-ray spectroscopy

    NASA Astrophysics Data System (ADS)

    Mantouvalou, Ioanna; Witte, Katharina; Grötzsch, Daniel; Neitzel, Michael; Günther, Sabrina; Baumann, Jonas; Jung, Robert; Stiel, Holger; Kanngießer, Birgit; Sandner, Wolfgang

    2015-03-01

    In this work, a novel laser-produced plasma source is presented which delivers pulsed broadband soft X-radiation in the range between 100 and 1200 eV. The source was designed in view of long operating hours, high stability, and cost effectiveness. It relies on a rotating and translating metal target and achieves high stability through an on-line monitoring device using a four quadrant extreme ultraviolet diode in a pinhole camera arrangement. The source can be operated with three different laser pulse durations and various target materials and is equipped with two beamlines for simultaneous experiments. Characterization measurements are presented with special emphasis on the source position and emission stability of the source. As a first application, a near edge X-ray absorption fine structure measurement on a thin polyimide foil shows the potential of the source for soft X-ray spectroscopy.

  18. Soft x-ray power diagnostic improvements at the Omega Laser Facility

    SciTech Connect

    Sorce, C.; Schein, J.; Weber, F.; Widmann, K.; Campbell, K.; Dewald, E.; Turner, R.; Landen, O.; Jacoby, K.; Torres, P.; Pellinen, D.

    2006-10-15

    Soft x-ray power diagnostics are essential for evaluating high temperature laser plasma experiments. The Dante soft x-ray spectrometer, a core diagnostic for radiation flux and temperature measurements of Hohlraums, installed on the Omega Laser Facility at the Laboratory for Laser Energetics has recently undergone a series of upgrades. Work performed at Brookhaven National Laboratory for the development of the National Ignition Facility (NIF) Dante spectrometer enables the Omega Dante to offer a total of 18 absolutely calibrated channels in the energy range from 50 eV to 20 keV. This feature provides Dante with the capability to measure higher, NIF relevant, radiation temperatures with increased accuracy including a differentiation of higher energy radiation such as the Au M and L bands. Diagnostic monitoring using experimental data from directly driven Au spherical shots is discussed.

  19. Generation of subterawatt-attosecond pulses in a soft x-ray free-electron laser

    NASA Astrophysics Data System (ADS)

    Huang, Senlin; Ding, Yuantao; Huang, Zhirong; Marcus, Gabriel

    2016-08-01

    We propose a novel scheme to generate attosecond soft x rays in a self-seeded free-electron laser (FEL) suitable for enabling attosecond spectroscopic investigations. A time-energy chirped electron bunch with additional sinusoidal energy modulation is adopted to produce a short seed pulse through a self-seeding monochromator. This short seed pulse, together with high electron current spikes and a cascaded delay setup, enables a high-efficiency FEL with a fresh bunch scheme. Simulations show that using the Linac Coherent Light Source (LCLS) parameters, soft x-ray pulses with a FWHM of 260 attoseconds and a peak power of 0.5 TW can be obtained. This scheme also has the feature of providing a stable central wavelength determined by the self-seeding monochromator.

  20. Elimination of higher-order diffraction using zigzag transmission grating in soft x-ray region

    SciTech Connect

    Zang, H. P.; Wang, C. K.; Gao, Y. L.; Zhou, W. M.; Kuang, L. Y.; Wei, L.; Fan, W.; Zhang, W. H.; Zhao, Z. Q.; Cao, L. F.; Gu, Y. Q.; Zhang, B. H.; Jiang, G.; Zhu, X. L.; Xie, C. Q.; Zhao, Y. D.; Cui, M. Q.

    2012-03-12

    We present a realization of the sinusoidal transmission function using a series of zigzag-profiled strips where the transmission takes on the binary values 0 and 1 in a two-dimensional distribution. A zigzag transmission grating of 1000 line/mm has been fabricated and demonstrated on the soft x-ray beam of synchrotron radiation. The axial single-order diffraction indicates that the zigzag transmission grating is adequate for spectroscopic application.