Molecular dynamics simulation of shock wave and spallation phenomena in metal foils irradiated by femtosecond laser pulse

NASA Astrophysics Data System (ADS)

Zhakhovsky, Vasily; Demaske, Brian; Inogamov, Nail; Oleynik, Ivan

2010-03-01

Femtosecond laser irradiation of metals is an effective technique to create a high-pressure frontal layer of 100-200 nm thickness. The associated ablation and spallation phenomena can be studied in the laser pump-probe experiments. We present results of a large-scale MD simulation of ablation and spallation dynamics developing in 1,2,3μm thick Al and Au foils irradiated by a femtosecond laser pulse. Atomic-scale mechanisms of laser energy deposition, transition from pressure wave to shock, reflection of the shock from the rear-side of the foil, and the nucleation of cracks in the reflected tensile wave, having a very high strain rate, were all studied. To achieve a realistic description of the complex phenomena induced by strong compression and rarefaction waves, we developed new embedded atom potentials for Al and Au based on cold pressure curves. MD simulations revealed the complex interplay between spallation and ablation processes: dynamics of spallation depends on the pressure profile formed in the ablated zone at the early stage of laser energy absorption. It is shown that the essential information such as material properties at high strain rate and spall strength can be extracted from the simulated rear-side surface velocity as a function of time.

Moisture-Induced Spallation and Interfacial Hydrogen Embrittlement of Alumina Scales

NASA Technical Reports Server (NTRS)

Smialek, James L.

2005-01-01

Thermal expansion mismatch stresses and interfacial sulfur activity are the major factors producing primary Al2O3 scale spallation on high temperature alloys. However, moisture-induced delayed spallation appears as a secondary, but often dramatic, illustration of an additional mechanistic detail. A historical review of delayed failure of alumina scales and TBC s on superalloys is presented herein. Similarities with metallic phenomena suggest that hydrogen embrittlement from ambient humidity, resulting from the reaction Al+3H2O=Al(OH)3+3H(+)+3e(-), is the operative mechanism. This proposal was tested by standard cathodic hydrogen charging in 1N H2SO4, applied to Rene N5 pre-oxidized at 1150 C for 1000 1-hr cycles, and monitored by weight change, induced current, and microstructure. Here cathodic polarization at -2.0 V abruptly stripped mature Al2O3 scales at the oxide-metal interface. Anodic polarization at +2.0 V, however, produced alloy dissolution. Finally, with no applied voltage, the electrolyte alone produced neither scale spallation nor alloy dissolution. These experiments thus highlight the detrimental effects of hydrogen charging on alumina scale adhesion. It is proposed that interfacial hydrogen embrittlement is produced by moist air and is the root cause of both moisture-induced, delayed scale spallation and desktop TBC failures.

European Neutrons form Parasitic Research to Global Strategy: Realizing Plans for a Transnational European Spallation Source in the Wake of the Cold War

NASA Astrophysics Data System (ADS)

Kaiserfeld, Thomas

2016-03-01

Studies of Big Science have early on focused on instrumentation and scientific co-operation in large organizations, later on to take into account symbolic values and specific research styles while more recently also involving the relevance of commercial interests and economic development as well as the assimilation of research traditions. In accordance with these transformed practices, this presentation will analyze how an organization with the purpose of realizing a Big-Science facility, The European Spallation Source, has successfully managed to present the project as relevant to different national and international policy-makers, to the community of European neutron researchers as well as to different industrial interests. All this has been achieved in a research-policy environment, which has been the subject to drastic transformations, from calls to engage researchers from the former eastern bloc in the early 1990s via competition with American and Asian researchers at the turn of the century 2000 to intensified demands on business applications. During this process, there has also been fierce competition between different potential sites in the U.K., Germany, Spain, Hungary and Sweden, not once, but twice. The project has in addition been plagued by withdrawals of key actors as well as challenging problems in the field of spallation-source construction. Nevertheless, the European Spallation Source has survived from the early 1990s until today, now initiating the construction process at Lund in southern Sweden. In this presentation, the different measures taken and arguments raised by the European Spallation Source project in order to realize the facility will be analysed. Especially the different designs of the European Spallation Source will be analysed as responses to external demands and threats.

Radionuclide production and dose rate estimation during the commissioning of the W-Ta spallation target

NASA Astrophysics Data System (ADS)

Yu, Q. Z.; Liang, T. J.

2018-06-01

China Spallation Neutron Source (CSNS) is intended to begin operation in 2018. CSNS is an accelerator-base multidisciplinary user facility. The pulsed neutrons are produced by a 1.6GeV short-pulsed proton beam impinging on a W-Ta spallation target, at a beam power of100 kW and a repetition rate of 25 Hz. 20 neutron beam lines are extracted for the neutron scattering and neutron irradiation research. During the commissioning and maintenance scenarios, the gamma rays induced from the W-Ta target can cause the dose threat to the personal and the environment. In this paper, the gamma dose rate distributions for the W-Ta spallation are calculated, based on the engineering model of the target-moderator-reflector system. The shipping cask is analyzed to satisfy the dose rate limit that less than 2 mSv/h at the surface of the shipping cask. All calculations are performed by the Monte carlo code MCNPX2.5 and the activation code CINDER’90.

GRAIN-SCALE FAILURE IN THERMAL SPALLATION DRILLING

DOE Office of Scientific and Technical Information (OSTI.GOV)

Walsh, S C; Lomov, I; Roberts, J J

2012-01-19

Geothermal power promises clean, renewable, reliable and potentially widely-available energy, but is limited by high initial capital costs. New drilling technologies are required to make geothermal power financially competitive with other energy sources. One potential solution is offered by Thermal Spallation Drilling (TSD) - a novel drilling technique in which small particles (spalls) are released from the rock surface by rapid heating. While TSD has the potential to improve drilling rates of brittle granitic rocks, the coupled thermomechanical processes involved in TSD are poorly described, making system control and optimization difficult for this drilling technology. In this paper, we discussmore » results from a new modeling effort investigating thermal spallation drilling. In particular, we describe an explicit model that simulates the grain-scale mechanics of thermal spallation and use this model to examine existing theories concerning spalling mechanisms. We will report how borehole conditions influence spall production, and discuss implications for macro-scale models of drilling systems.« less

Design specification for the European Spallation Source neutron generating target element

NASA Astrophysics Data System (ADS)

Aguilar, A.; Sordo, F.; Mora, T.; Mena, L.; Mancisidor, M.; Aguilar, J.; Bakedano, G.; Herranz, I.; Luna, P.; Magan, M.; Vivanco, R.; Jimenez-Villacorta, F.; Sjogreen, K.; Oden, U.; Perlado, J. M.; Martinez, J. L.; Bermejo, F. J.

2017-06-01

The paper addresses some of the most relevant issues concerning the thermal hydraulics and radiation damage of the neutron generation target to be built at the European Spallation Source as recently approved after a critical design review. The target unit consists of a set of Tungsten blocks placed inside a wheel of 2.5 m diameter which rotates at some 0.5 Hz in order to distribute the heat generated from incoming protons which reach the target in the radial direction. The spallation material elements are composed of an array of Tungsten pieces which rest on a rotating steel support (the cassette) and are distributed in a cross-flow configuration. The thermal, mechanical and radiation effects resulting from the impact of a 2 GeV proton pulse are analysed in detail as well as an evaluation of the inventory of spallation products. The current design is found to conform to specifications and found to be robust enough to deal with several accident scenarios.

Detection of supernova neutrinos at spallation neutron sources

NASA Astrophysics Data System (ADS)

Huang, Ming-Yang; Guo, Xin-Heng; Young, Bing-Lin

2016-07-01

After considering supernova shock effects, Mikheyev-Smirnov-Wolfenstein effects, neutrino collective effects, and Earth matter effects, the detection of supernova neutrinos at the China Spallation Neutron Source is studied and the expected numbers of different flavor supernova neutrinos observed through various reaction channels are calculated with the neutrino energy spectra described by the Fermi-Dirac distribution and the “beta fit” distribution respectively. Furthermore, the numerical calculation method of supernova neutrino detection on Earth is applied to some other spallation neutron sources, and the total expected numbers of supernova neutrinos observed through different reactions channels are given. Supported by National Natural Science Foundation of China (11205185, 11175020, 11275025, 11575023)

Multimaterial lamination as a means of retarding penetration and spallation failures in plates

NASA Technical Reports Server (NTRS)

Dibattista, J. D.; Humes, D. H.

1972-01-01

Experimental data are presented which show that hypervelocity impact spallation and penetration failures of a single solid aluminum plate and of a solid aluminum plate spaced a distance behind a Whipple meteor bumper may be retarded by replacing the solid aluminum plate with a laminated plate. Four sets of experiments were conducted. The first set of experiments was conducted with projectile mass and velocity held constant and with polycarbonate cylinders impacted into single plates of different construction. The second set of experiments was done with single plates of various construction and aluminum spherical projectiles of similar mass but different velocities. These two experiments showed that a laminated plate of aluminum and polycarbonate or aluminum and methyl methacrylate could prevent spallation and penetration failures with a lower areal density than either an all-aluminum laminated plate or a solid aluminum plate. The aluminum laminated plate was in turn superior to the solid aluminum plate in resisting spallation and penetration failures. In addition, through an example of 6061-T6 aluminum and methyl methacrylate, it is shown that a laminated structure ballistically superior to its parent materials may be built. The last two sets of experiments were conducted using bumper-protected main walls of solid aluminum and of laminated aluminum and polycarbonate. Again, under hypervelocity impact conditions, the laminated main walls were superior to the solid aluminum main walls in retarding spallation and penetration failures.

Behind the Scenes of the Spallation Neutron Source – The Linear Accelerator

ScienceCinema

Galambos, John

2018-06-25

The Spallation Neutron Source at Oak Ridge National Laboratory is a one-of-a-kind research facility that provides the most intense pulsed neutron beams in the world for scientific research and industrial development. Take a look inside the facility's linear accelerator.

Spallation reaction study for fission products in nuclear waste: Cross section measurements for 137Cs, 90Sr and 107Pd on proton and deuteron

NASA Astrophysics Data System (ADS)

Wang, He; Otsu, Hideaki; Sakurai, Hiroyoshi; Ahn, DeukSoon; Aikawa, Masayuki; Ando, Takashi; Araki, Shouhei; Chen, Sidong; Chiga, Nobuyuki; Doornenbal, Pieter; Fukuda, Naoki; Isobe, Tadaaki; Kawakami, Shunsuke; Kawase, Shoichiro; Kin, Tadahiro; Kondo, Yosuke; Koyama, Shupei; Kubono, Shigeru; Maeda, Yukie; Makinaga, Ayano; Matsushita, Masafumi; Matsuzaki, Teiichiro; Michimasa, Shinichiro; Momiyama, Satoru; Nagamine, Shunsuke; Nakamura, Takashi; Nakano, Keita; Niikura, Megumi; Ozaki, Tomoyuki; Saito, Atsumi; Saito, Takeshi; Shiga, Yoshiaki; Shikata, Mizuki; Shimizu, Yohei; Shimoura, Susumu; Sumikama, Toshiyuki; Söderström, Pär-Anders; Suzuki, Hiroshi; Takeda, Hiroyuki; Takeuchi, Satoshi; Taniuchi, Ryo; Togano, Yasuhiro; Tsubota, Junichi; Uesaka, Meiko; Watanabe, Yasushi; Watanabe, Yukinobu; Wimmer, Kathrin; Yamamoto, Tatsuya; Yoshida, Koichi

2017-09-01

Spallation reactions for the long-lived fission products 137Cs, 90Sr and 107Pd have been studied for the purpose of nuclear waste transmutation. The cross sections on the proton- and deuteron-induced spallation were obtained in inverse kinematics at the RIKEN Radioactive Isotope Beam Factory. Both the target and energy dependences of cross sections have been investigated systematically. and the cross-section differences between the proton and deuteron are found to be larger for lighter fragments. The experimental data are compared with the SPACS semi-empirical parameterization and the PHITS calculations including both the intra-nuclear cascade and evaporation processes.

Moisture-Induced Delayed Alumina Scale Spallation on a Ni(Pt)Al Coating

NASA Technical Reports Server (NTRS)

Smialek, James L.

2009-01-01

Delayed interfacial scale failure takes place after cooling for samples of a Ni(Pt)Al-coated CMSX4 single crystal superalloy, cycled at 1150 C for up to 2000 hr. One sample exhibited premature coating grain boundary wrinkling, alumina scale spallation to bare metal, and a final weight loss of 3.3 mg/cm2 . Spallation under ambient conditions was monitored with time after cooldown and was found to continue for 24 hr. This produced up to 0.05 mg/cm2 additional loss for each hold, accumulating 0.7 mg/cm 2 (20 percent of the total) over the course of the test. After test termination, water immersion produced an additional 0.15 mg/cm2 loss. (A duplicate sample produced much less wrinkling and time dependent spalling, maintaining a net weight gain.) The results are consistent with the general phenomena of moisture-induced delayed spallation (MIDS) of mature, distressed alumina scales formed on oxidation resistant M-Al alloys. Relative ambient humidity is discussed as the factor controlling adsorbed moisture, reaction with the substrate, and hydrogen effects on interface strength.

Universal odd-even staggering in isotopic fragmentation and spallation cross sections of neutron-rich fragments

NASA Astrophysics Data System (ADS)

Mei, B.; Tu, X. L.; Wang, M.

2018-04-01

An evident odd-even staggering (OES) in fragment cross sections has been experimentally observed in many fragmentation and spallation reactions. However, quantitative comparisons of this OES effect in different reaction systems are still scarce for neutron-rich nuclei near the neutron drip line. By employing a third-order difference formula, the magnitudes of this OES in extensive experimental cross sections are systematically investigated for many neutron-rich nuclei with (N -Z ) from 1 to 23 over a broad range of atomic numbers (Z ≈3 -50 ). A comparison of these magnitude values extracted from fragment cross sections measured in different fragmentation and spallation reactions with a large variety of projectile-target combinations over a wide energy range reveals that the OES magnitude is almost independent of the projectile-target combinations and the projectile energy. The weighted average of these OES magnitudes derived from cross sections accurately measured in different reaction systems is adopted as the evaluation value of the OES magnitude. These evaluated OES magnitudes are recommended to be used in fragmentation and spallation models to improve their predictions for fragment cross sections.

Numerical Simulations of Thermo-Mechanical Processes during Thermal Spallation Drilling for Geothermal Reservoirs

NASA Astrophysics Data System (ADS)

Vogler, D.; Walsh, S. D. C.; Rudolf von Rohr, P.; Saar, M. O.

2017-12-01

Drilling expenses constitute a significant share of the upfront capital costs and thereby the associated risks of geothermal energy production. This is especially true for deep boreholes, as drilling costs per meter increase significantly with depth. Thermal spallation drilling is a relatively new drilling technique, particularly suited to the hard crystalline (e.g., basement) rocks in which many deep geothermal resources are located. The method uses a hot jet-flame to rapidly heat the rock surface, which leads to large temperature gradients in the rock. These temperature gradients cause localized thermal stresses that, in combination with the in situ stress field, lead to the formation and ejection of spalls. These spalls are then transported out of the borehole with the drilling mud. Thermal spallation not only in principle enables much faster rates of penetration than traditional rotary drilling, but is also contact-less, which significantly reduces the long tripping times associated with conventional rotary head drilling. We present numerical simulations investigating the influence of rock heterogeneities on the thermal spallation process. Special emphasis is put on different mineral compositions, stress regimes, and heat sources.

Material issues relating to high power spallation neutron sources

NASA Astrophysics Data System (ADS)

Futakawa, M.

2015-02-01

Innovative researches using neutrons are being performed at the Materials and Life Science Experimental Facility (MLF) at the Japan Proton Accelerator Research Complex (J-PARC), in which a mercury target system is installed for MW-class pulse spallation neutron sources. In order to produce neutrons by the spallation reaction, proton beams are injected into the mercury target. At the moment, when the intense proton beam hits the target, pressure waves are generated in mercury because of the abrupt heat deposition. The pressure waves interact with the target vessel, leading to negative pressure that may cause cavitation along the vessel wall, i.e. on the interface between liquid and solid metals. On the other hand, the structural materials are subjected to irradiation damage due to protons and neutrons, very high cycle fatigue damages and so-called "liquid metal embrittlement". That is, the structural materials must be said to be exposed to the extremely severe environments. In the paper, research and development relating to the material issues in the high power spallation neutron sources that has been performed so far at J-PARC is summarized.

Ductility recovery in structural materials for spallation targets by post-irradiation annealing

NASA Astrophysics Data System (ADS)

Chen, J.; Jung, P.; Rödig, M.; Ullmaier, H.; Bauer, G. S.

2005-08-01

Low temperature irradiation embrittlement is one of the major criteria to determine the lifetime of spallation targets. Embrittlement is especially high at low service temperatures, e.g. 250 °C in liquid-mercury sources. It was the aim of the present study to investigate the effect of post-irradiation annealing on the mechanical properties of irradiated structural materials. The specimens used were obtained from spent target components of operating spallation facilities (Los Alamos Neutron Science Center, LANSCE, and the Spallation Neutron Source at Rutherford-Appleton Laboratory, ISIS). The investigated materials include a nickel-based alloy (IN718), an austenitic stainless steel (AISI 304L), a martensitic stainless steel (DIN 1.4926) and a refractory metal (Ta) which experienced 800 MeV proton irradiation to fluences of several 10 25 p/m 2. The specimens were annealed from 300 °C to 700 °C for 1 to 10 h, respectively, and their mechanical property changes were subsequently investigated at room temperature and 250 °C by tensile testing and fracture surface analysis conducted by scanning electron microscopy (SEM). The results showed that the ductility recovered to a large degree in 304L and DIN 1.4926 materials while their strength remained almost unchanged. Especially for DIN 1.4926, the ductility recovery is remarkable already at 400 °C. Together with its favorable thermo-mechanical properties, this makes martensitic steel a candidate for structural materials of spallation targets.

Thermal barrier coating life prediction model development, phase 2

NASA Technical Reports Server (NTRS)

Meier, Susan Manning; Sheffler, Keith D.; Nissley, David M.

1991-01-01

The objective of this program was to generate a life prediction model for electron-beam-physical vapor deposited (EB-PVD) zirconia thermal barrier coating (TBC) on gas turbine engine components. Specific activities involved in development of the EB-PVD life prediction model included measurement of EB-PVD ceramic physical and mechanical properties and adherence strength, measurement of the thermally grown oxide (TGO) growth kinetics, generation of quantitative cyclic thermal spallation life data, and development of a spallation life prediction model. Life data useful for model development was obtained by exposing instrumented, EB-PVD ceramic coated cylindrical specimens in a jet fueled burner rig. Monotonic compression and tensile mechanical tests and physical property tests were conducted to obtain the EB-PVD ceramic behavior required for burner rig specimen analysis. As part of that effort, a nonlinear constitutive model was developed for the EB-PVD ceramic. Spallation failure of the EB-PVD TBC system consistently occurred at the TGO-metal interface. Calculated out-of-plane stresses were a small fraction of that required to statically fail the TGO. Thus, EB-PVD spallation was attributed to the interfacial cracking caused by in-plane TGO strains. Since TGO mechanical properties were not measured in this program, calculation of the burner rig specimen TGO in-plane strains was performed by using alumina properties. A life model based on maximum in-plane TGO tensile mechanical strain and TGO thickness correlated the burner rig specimen EB-PVD ceramic spallation lives within a factor of about plus or minus 2X.

Radiation effects in structural materials of spallation targets

NASA Astrophysics Data System (ADS)

Jung, P.

2002-02-01

Effects of radiation damage by protons and neutrons in structural materials of spallation neutron sources are reviewed. Effects of atomic displacements, defect mobility and transmutation products, especially hydrogen and helium, on physical and mechanical properties are discussed. The most promising candidate materials (austenitic stainless steels, ferritic/martensitic steels and refractory alloys) are compared, and needed investigations are identified.

Linac design for the European spallation source

DOE Office of Scientific and Technical Information (OSTI.GOV)

Klein, H.

1995-10-01

A study group has started to develop a conceptual design for a European Spallation Source (ESS). This pulsed 5 MW source presently consists of a 1.334 GeV linac and two compressor rings. In the following mainly the high intensity linac part will be discussed, which has some features of interest for accelerators for transmutation of radioactive waste too.

High power neutron production targets

DOE Office of Scientific and Technical Information (OSTI.GOV)

Wender, S.

1996-06-01

The author describes issues of concern in the design of targets and associated systems for high power neutron production facilities. The facilities include uses for neutron scattering, accelerator driven transmutation, accelerator production of tritium, short pulse spallation sources, and long pulse spallation sources. Each of these applications requires a source with different design needs and consequently different implementation in practise.

Toward high-efficiency and detailed Monte Carlo simulation study of the granular flow spallation target

NASA Astrophysics Data System (ADS)

Cai, Han-Jie; Zhang, Zhi-Lei; Fu, Fen; Li, Jian-Yang; Zhang, Xun-Chao; Zhang, Ya-Ling; Yan, Xue-Song; Lin, Ping; Xv, Jian-Ya; Yang, Lei

2018-02-01

The dense granular flow spallation target is a new target concept chosen for the Accelerator-Driven Subcritical (ADS) project in China. For the R&D of this kind of target concept, a dedicated Monte Carlo (MC) program named GMT was developed to perform the simulation study of the beam-target interaction. Owing to the complexities of the target geometry, the computational cost of the MC simulation of particle tracks is highly expensive. Thus, improvement of computational efficiency will be essential for the detailed MC simulation studies of the dense granular target. Here we present the special design of the GMT program and its high efficiency performance. In addition, the speedup potential of the GPU-accelerated spallation models is discussed.

Determination of neutron multiplication coefficients for fuel elements irradiated by spallation neutrons

DOE Office of Scientific and Technical Information (OSTI.GOV)

Bhatia, Chitra; Kumar, V.

2010-02-15

A neutron multiplication coefficient, k{sub eff}, has been estimated for spallation neutron flux using the data of spectrum average cross sections of all absorption, fission, and nonelastic reaction channels of {sup 232}Th, {sup 238}U, {sup 235}U, and {sup 233}U fuel elements. It has been revealed that in spallation neutron flux (i) nonfission, nonabsorption reactions play an important role in the calculation of k{sub eff}, (ii) one can obtain a high value of k{sub eff} even for fertile {sup 232}Th fuel, which is hardly possible in a conventional fast reactor, and (iii) spectrum average absorption cross sections of neutron poisons ofmore » a conventional reactor are relatively very small.« less

Helium (3) Rich Solar Flares

DOE R&D Accomplishments Database

Colgate, S. A.; Audouze, J.; Fowler, W. A.

1977-05-03

The extreme enrichment of {sup 3} He {sup 4} He greater than or equal to 1 in some solar flares as due to spallation and the subsequent confinement of the products in a high temperature, kT approx. = 200 keV, high density, n{sub e} approx. = 3 x 10{sup 15} cm {sup -3} plasma associated with the magnetic instability producing the flare is interpreted. The pinch or filament is a current of high energy protons that creates the spallation and maintains the temperature that produces the high energy x-ray spectrum and depletes other isotopes D, Li, Be, and B as observed. Finally the high temperature plasma is a uniquely efficient spallation target that is powered by the interaction of stellar convection and self generated magnetic field.

Benchmarking shielding simulations for an accelerator-driven spallation neutron source

DOE PAGES

Cherkashyna, Nataliia; Di Julio, Douglas D.; Panzner, Tobias; ...

2015-08-09

The shielding at an accelerator-driven spallation neutron facility plays a critical role in the performance of the neutron scattering instruments, the overall safety, and the total cost of the facility. Accurate simulation of shielding components is thus key for the design of upcoming facilities, such as the European Spallation Source (ESS), currently in construction in Lund, Sweden. In this paper, we present a comparative study between the measured and the simulated neutron background at the Swiss Spallation Neutron Source (SINQ), at the Paul Scherrer Institute (PSI), Villigen, Switzerland. The measurements were carried out at several positions along the SINQ monolithmore » wall with the neutron dosimeter WENDI-2, which has a well-characterized response up to 5 GeV. The simulations were performed using the Monte-Carlo radiation transport code Geant4, and include a complete transport from the proton beam to the measurement locations in a single calculation. An agreement between measurements and simulations is about a factor of 2 for the points where the measured radiation dose is above the background level, which is a satisfactory result for such simulations spanning many energy regimes, different physics processes and transport through several meters of shielding materials. The neutrons contributing to the radiation field emanating from the monolith were confirmed to originate from neutrons with energies above 1 MeV in the target region. The current work validates Geant4 as being well suited for deep-shielding calculations at accelerator-based spallation sources. We also extrapolate what the simulated flux levels might imply for short (several tens of meters) instruments at ESS.« less

Moisture-Induced Alumina Scale Spallation: The Hydrogen Factor

NASA Technical Reports Server (NTRS)

Smialek, James L.

2010-01-01

For some time the oxidation community has been concerned with interfacial spallation of protective alumina scales, not just upon immediate cool down, but as a time-delayed phenomenon. Moisture-induced delayed spallation (MIDS) and desktop spallation (DTS) of thermal barrier coatings (TBCs) refer to this process. It is most apparent for relatively adherent alumina scales that have survived initial cool down in a dry environment, have built up considerable thickness and strain energy, and have been somewhat damaged, such as by cyclic oxidation cracking. Indeed, a "sensitive zone" can be described that maximizes the observed effect as a function of all the relevant factors. Moisture has been postulated to serve as a source of interfacial hydrogen embrittlement. Hydrogen is derived from reaction with aluminum in the alloy at an exposed interface. The purpose of this monograph is to trace the close analogy of this phenomenon to other hydrogen-induced effects, such as embrittlement of aluminides and blistering of alloys and anodic alumina films. A formalized, top-down, logic-tree structure is presented as a guide to this discussion. A theoretical basis for interfacial weakening by hydrogen is first cited, as are demonstrations of hydrogen detection as a reaction product or interfacial species. Further support is provided by critical experiments that recreate the moisture effect, but by isolating hydrogen from other potential causative factors. These experiments include tests in H 2-containing atmospheres or cathodic hydrogen charging. Accordingly, they strongly indicate that interfacial hydrogen, derived from moisture, is the key chemical species accounting for delayed alumina scale spallation.

Spallation-induced roughness promoting high spatial frequency nanostructure formation on Cr

NASA Astrophysics Data System (ADS)

Abou-Saleh, A.; Karim, E. T.; Maurice, C.; Reynaud, S.; Pigeon, F.; Garrelie, F.; Zhigilei, L. V.; Colombier, J. P.

2018-04-01

Interaction of ultrafast laser pulses with metal surfaces in the spallation regime can result in the formation of anisotropic nanoscale surface morphology commonly referred to as laser-induced periodic surface structures (LIPSS) or ripples. The surface structures generated by a single pulse irradiation of monocrystalline Cr samples are investigated experimentally and computationally for laser fluences that produce high spatial frequency nanostructures in the multi-pulse irradiation regime. Electron microscopy reveals distinct response of samples with different crystallographic surface orientations, with (100) surfaces exhibiting the formation of more refined nanostructure by a single pulse irradiation and a more pronounced LIPSS after two laser pulses as compared to (110) surfaces. A large-scale molecular dynamics simulation of laser interaction with a (100) Cr target provides detailed information on processes responsible for spallation of a liquid layer, redistribution of molten material, and rapid resolidification of the target. The nanoscale roughness of the resolidified surface predicted in the simulation features elongated frozen nanospikes, nanorims and nanocavities with dimensions and surface density similar to those in the surface morphology observed for (100) Cr target with atomic force microscopy. The results of the simulation suggest that the types, sizes and dimensions of the nanoscale surface features are defined by the competition between the evolution of transient liquid structures generated in the spallation process and the rapid resolidification of the surface region of the target. The spallation-induced roughness is likely to play a key role in triggering the generation of high-frequency LIPSS upon irradiation by multiple laser pulses.

Spallation backgrounds in Super-Kamiokande are made in muon-induced showers

NASA Astrophysics Data System (ADS)

Li, Shirley Weishi; Beacom, John F.

2015-05-01

Crucial questions about solar and supernova neutrinos remain unanswered. Super-Kamiokande has the exposure needed for progress, but detector backgrounds are a limiting factor. A leading component is the beta decays of isotopes produced by cosmic-ray muons and their secondaries, which initiate nuclear spallation reactions. Cuts of events after and surrounding muon tracks reduce this spallation decay background by ≃ 90 % (at a cost of ≃ 20 % deadtime), but its rate at 6-18 MeV is still dominant. A better way to cut this background was suggested in a Super-Kamiokande paper by Bays et al. [Phys. Rev. D 85, 052007 (2012)] on a search for the diffuse supernova neutrino background. They found that spallation decays above 16 MeV were preceded near the same location by a peak in the apparent Cherenkov light profile from the muon; a more aggressive cut was applied to a limited section of the muon track, leading to decreased background without increased deadtime. We put their empirical discovery on a firm theoretical foundation. We show that almost all spallation decay isotopes are produced by muon-induced showers and that these showers are rare enough and energetic enough to be identifiable. This is the first such demonstration for any detector. We detail how the physics of showers explains the peak in the muon Cherenkov light profile and other Super-K observations. Our results provide a physical basis for practical improvements in background rejection that will benefit multiple studies. For solar neutrinos, in particular, it should be possible to dramatically reduce backgrounds at energies as low as 6 MeV.

Determination of the Secondary Neutron Flux at the Massive Natural Uranium Spallation Target

NASA Astrophysics Data System (ADS)

Zeman, M.; Adam, J.; Baldin, A. A.; Furman, W. I.; Gustov, S. A.; Katovsky, K.; Khushvaktov, J.; Mar`in, I. I.; Novotny, F.; Solnyshkin, A. A.; Tichy, P.; Tsoupko-Sitnikov, V. M.; Tyutyunnikov, S. I.; Vespalec, R.; Vrzalova, J.; Wagner, V.; Zavorka, L.

The flux of secondary neutrons generated in collisions of the 660 MeV proton beam with the massive natural uranium spallation target was investigated using a set of monoisotopic threshold activation detectors. Sandwiches made of thin high-purity Al, Co, Au, and Bi metal foils were installed in different positions across the whole spallation target. The gamma-ray activity of products of (n,xn) and other studied reactions was measured offline with germanium semiconductor detectors. Reaction yields of radionuclides with half-life exceeding 100 min and with effective neutron energy thresholds between 3.6 MeV and 186 MeV provided us with information about the spectrum of spallation neutrons in this energy region and beyond. The experimental neutron flux was determined using the measured reaction yields and cross-sections calculated with the TALYS 1.8 nuclear reaction program and INCL4-ABLA event generator of MCNP6. Neutron spectra in the region of activation sandwiches were also modeled with the radiation transport code MCNPX 2.7. Neutron flux based on excitation functions from TALYS provides a reasonable description of the neutron spectrum inside the spallation target and is in good agreement with Monte-Carlo predictions. The experimental flux that uses INCL4 cross-sections rather underestimates the modeled spectrum in the whole region of interest, but the agreement within few standard deviations was reached as well. The paper summarizes basic principles of the method for determining the spectrum of high-energy neutrons without employing the spectral adjustment routines and points out to the need for model improvements and precise cross-section measurements.

Pairing-energy coefficients of neutron-rich fragments in spallation reactions

NASA Astrophysics Data System (ADS)

Niu, Fei; Ma, Chun-Wang

2018-02-01

The ratio of pairing-energy coefficient to temperature (a p/T) of neutron-rich fragments produced in spallation reactions has been investigated by adopting an isobaric yield ratio method deduced in the framework of a modified Fisher model. A series of spallation reactions, 0.5A and 1A GeV 208Pb + p, 1A GeV 238U + p, 0.5A GeV 136Xe + d, 0.2A, 0.5A and 1A GeV 136Xe + p, and 56Fe + p with incident energy ranging from 0.3A to 1.5A GeV, has been analysed. An obvious odd-even staggering is shown in the fragments with small neutron excess (I ≡ N-Z), and in the relatively small-A fragments which have large I. The values of a p/T for the fragments, with I from 0 to 36, have been found to be in a range from -4 to 4, and most values of a p/T fall in the range from -1 to 1. It is suggested that a small pairing-energy coefficient should be considered in predicting the cross sections of fragments in spallation reactions. It is also concluded that the method proposed in this article is not good for fragments with A/A s > 85% (where A s is the mass number of the spallation system). Supported by National Natural Science Foundation of China (U1732135), Natural Science Foundation of Henan Province (162300410179) and Henan Normal University for the Excellent Youth (154100510007)

Delayed Alumina Scale Spallation on Rene'n5+y: Moisture Effects and Acoustic Emission

NASA Technical Reports Server (NTRS)

Smialek, James L.; Morscher, Gregory N.

2001-01-01

The single crystal superalloy Rene'N5 (with or without Y-doping and hydrogen annealing) was cyclically oxidized at 1150 C for 1000 hours. After considerable scale growth (>= 500 hours), even the adherent alumina scales formed on Y-doped samples exhibited delayed interfacial spallation during subsequent water immersion tests, performed up to one year after oxidation. Spallation was characterized by weight loss, the amount of spalled area, and acoustic emission response. Hydrogen annealing (prior to oxidation) reduced spallation both before and after immersion, but without measurably reducing the bulk sulfur content of the Y-doped alloys. The duration and frequency of sequential, co-located acoustic emission events implied an interfacial crack growth rate at least 10(exp -3) m/s, but possibly higher than 10(exp 2) m/s. This is much greater than classic moisture-assisted slow crack growth rates in bulk alumina (10(exp -6) to 10(exp -3) m/s), which may still have occurred undetected by acoustic emission. An alternative failure sequence is proposed: an incubation process for preferential moisture ingress leads to a local decrease in interfacial toughness, thus allowing fast fracture driven by stored strain energy.

Kinetics of Cyclic Oxidation and Cracking and Finite Element Analysis of MA956 and Sapphire/MA956 Composite System

NASA Technical Reports Server (NTRS)

Lee, Kang N.; Arya, Vinod K.; Halford, Gary R.; Barrett, Charles A.

1996-01-01

Sapphire fiber-reinforced MA956 composites hold promise for significant weight savings and increased high-temperature structural capability, as compared to unreinforced MA956. As part of an overall assessment of the high-temperature characteristics of this material system, cyclic oxidation behavior was studied at 1093 C and 1204 C. Initially, both sets of coupons exhibited parabolic oxidation kinetics. Later, monolithic MA956 exhibited spallation and a linear weight loss, whereas the composite showed a linear weight gain without spallation. Weight loss of the monolithic MA956 resulted from the linking of a multiplicity of randomly oriented and closely spaced surface cracks that facilitated ready spallation. By contrast, cracking of the composite's oxide layer was nonintersecting and aligned nominally parallel with the orientation of the subsurface reinforcing fibers. Oxidative lifetime of monolithic MA956 was projected from the observed oxidation kinetics. Linear elastic, finite element continuum, and micromechanics analyses were performed on coupons of the monolithic and composite materials. Results of the analyses qualitatively agreed well with the observed oxide cracking and spallation behavior of both the MA956 and the Sapphire/MA956 composite coupons.

Analysis of a Neutronic Experiment on a Simulated Mercury Spallation Neutron Target Assembly Bombarded by Giga-Electron-Volt Protons

DOE Office of Scientific and Technical Information (OSTI.GOV)

Maekawa, Fujio; Meigo, Shin-ichiro; Kasugai, Yoshimi

2005-05-15

A neutronic benchmark experiment on a simulated spallation neutron target assembly was conducted by using the Alternating Gradient Synchrotron at Brookhaven National Laboratory and was analyzed to investigate the prediction capability of Monte Carlo simulation codes used in neutronic designs of spallation neutron sources. The target assembly consisting of a mercury target, a light water moderator, and a lead reflector was bombarded by 1.94-, 12-, and 24-GeV protons, and the fast neutron flux distributions around the target and the spectra of thermal neutrons leaking from the moderator were measured in the experiment. In this study, the Monte Carlo particle transportmore » simulation codes NMTC/JAM, MCNPX, and MCNP-4A with associated cross-section data in JENDL and LA-150 were verified based on benchmark analysis of the experiment. As a result, all the calculations predicted the measured quantities adequately; calculated integral fluxes of fast and thermal neutrons agreed approximately within {+-}40% with the experiments although the overall energy range encompassed more than 12 orders of magnitude. Accordingly, it was concluded that these simulation codes and cross-section data were adequate for neutronics designs of spallation neutron sources.« less

The US Spallation Neutron Source Project

NASA Astrophysics Data System (ADS)

Olsen, David K.

1997-10-01

Slow neutrons, with wavelengths between a few tenths to a few tens of angstroms, are an important probe for condensed-matter physics and are produced with either fission reactors or accelerator-based spallation sources. The Spallation Neutron Source (SNS) is a collaborative project between DOE National Laboratories including LBNL, LANL, BNL, ANL and ORNL to build the next research neutron source in the US. This source will be sited at ORNL and is being designed to serve the needs of the neutron science community well into the next century. The SNS consists of a 1.1-mA H- front end and a 1.0-GeV high-intensity pulsed proton linac. The 1-ms pulses from the linac will be compressed in a 221-m-circumference accumulator ring to produce 600-ns pulses at a 60-Hz rate. This accelerator system will produce spallation neutrons from a 1.0-MW liquid Hg target for a broad spectrum of neutron scattering research with an initial target hall containing 18 instruments. The baseline conceptual design, critical issues, upgrade possibilities, and the collaborative arrangement will be discussed. It is expected that SNS construction will commence in FY99 and, following a seven year project, start operation in 2006.

Generation of negative pressures and spallation phenomena in diamond exposed to a picosecond laser pulse

NASA Astrophysics Data System (ADS)

Abrosimov, S. A.; Bazhulin, A. P.; Bol'shakov, A. P.; Konov, V. I.; Krasyuk, I. K.; Pashinin, P. P.; Ral'chenko, V. G.; Semenov, A. Yu; Sovyk, D. N.; Stuchebryukhov, I. A.; Fortov, V. E.; Khishchenko, K. V.; Khomich, A. A.

2014-06-01

The spallation phenomena in poly- and single-crystal synthetic diamonds have been experimentally investigated. A shockwave impact on a target was implemented using a 70-ps laser pulse in the Kamerton-T facility. The ablation pressure of 0.66 TPa on the front target surface was formed by pulsed radiation of a neodymium phosphate glass laser (second harmonic λ = 0.527 mm, pulse energy 2.5 J) with an intensity as high as 2 × 1013 W cm-2. The maximum diamond spall strength σ* ≈ 16.5 GPa is found to be 24% of the theoretical ultimate strength. Raman scattering data indicate that a small amount of crystalline diamond in the spallation region on the rear side of the target is graphitised.

Hydrocode modeling of the spallation process during hypervelocity impacts: Implications for the ejection of Martian meteorites

NASA Astrophysics Data System (ADS)

Kurosawa, Kosuke; Okamoto, Takaya; Genda, Hidenori

2018-02-01

Hypervelocity ejection of material by impact spallation is considered a plausible mechanism for material exchange between two planetary bodies. We have modeled the spallation process during vertical impacts over a range of impact velocities from 6 to 21 km/s using both grid- and particle-based hydrocode models. The Tillotson equations of state, which are able to treat the nonlinear dependence of density on pressure and thermal pressure in strongly shocked matter, were used to study the hydrodynamic-thermodynamic response after impacts. The effects of material strength and gravitational acceleration were not considered. A two-dimensional time-dependent pressure field within a 1.5-fold projectile radius from the impact point was investigated in cylindrical coordinates to address the generation of spalled material. A resolution test was also performed to reject ejected materials with peak pressures that were too low due to artificial viscosity. The relationship between ejection velocity veject and peak pressure Ppeak was also derived. Our approach shows that "late-stage acceleration" in an ejecta curtain occurs due to the compressible nature of the ejecta, resulting in an ejection velocity that can be higher than the ideal maximum of the resultant particle velocity after passage of a shock wave. We also calculate the ejecta mass that can escape from a planet like Mars (i.e., veject > 5 km/s) that matches the petrographic constraints from Martian meteorites, and which occurs when Ppeak = 30-50 GPa. Although the mass of such ejecta is limited to 0.1-1 wt% of the projectile mass in vertical impacts, this is sufficient for spallation to have been a plausible mechanism for the ejection of Martian meteorites. Finally, we propose that impact spallation is a plausible mechanism for the generation of tektites.

Process technology and effects of spallation products: Circuit components, maintenance, and handling

DOE Office of Scientific and Technical Information (OSTI.GOV)

Sigg, B.; Haines, S.J.; Dressler, R.

1996-06-01

Working Session D included an assessment of the status of the technology and components required to: (1) remove impurities from the liquid metal (mercury or Pb-Bi) target flow loop including the effects of spallation products, (2) provide the flow parameters necessary for target operations, and (3) maintain the target system. A series of brief presentations were made to focus the discussion on these issues. The subjects of these presentations, and presenters were: (1) Spallation products and solubilities - R. Dressler; (2) Spallation products for Pb-Bi - Y. Orlov; (3) Clean/up/impurity removal components - B. Sigg; (4) {open_quotes}Road-Map{close_quotes} and remote handlingmore » needs - T. McManamy; (5) Remote handling issues and development - M. Holding. The overall conclusion of this session was that, with the exception of (i) spallation product related processing issues, (ii) helium injection and clean-up, and (iii) specialized remote handling equipment, the technology for all other circuit components (excluding the target itself) exists. Operating systems at the Institute of Physics in Riga, Latvia (O. Lielausis) and at Ben-Gurion University in Beer Shiva, Israel (S. Lesin) have demonstrated that other liquid metal circuit components including pumps, heat exchangers, valves, seals, and piping are readily available and have been reliably used for many years. In the three areas listed above, the designs and analysis are not judged to be mature enough to determine whether and what types of technology development are required. Further design and analysis of the liquid metal target system is therefore needed to define flow circuit processing and remote handling equipment requirements and thereby identify any development needs.« less

The possible use of a spallation neutron source for neutron capture therapy with epithermal neutrons.

PubMed

Grusell, E; Condé, H; Larsson, B; Rönnqvist, T; Sornsuntisook, O; Crawford, J; Reist, H; Dahl, B; Sjöstrand, N G; Russel, G

1990-01-01

Spallation is induced in a heavy material by 72-MeV protons. The resulting neutrons can be characterized by an evaporation spectrum with a peak energy of less than 2 MeV. The neutrons are moderated in two steps: first in iron and then in carbon. Results from neutron fluence measurements in a perspex phantom placed close to the moderator are presented. Monte Carlo calculations of neutron fluence in a water phantom are also presented under some chosen configurations of spallation source and moderator. The calculations and measurements are in good agreement and show that, for proton currents of less than 0.5 mA, useful thermal-neutron fluences are attainable in the depth of the brain. However, the dose contribution from the unavoidable gamma background component has not been included in the present investigation.

Negative pressure and spallation in graphite targets under nano- and picosecond laser irradiation

DOE Office of Scientific and Technical Information (OSTI.GOV)

Belikov, R S; Khishchenko, K V; Krasyuk, I K

We present the results of experiments on the spallation phenomena in graphite targets under shock-wave nano- and picosecond irradiation, which have been performed on Kamerton-T (GPI, Moscow, Russia) and PHELIX (GSI, Darmstadt, Germany) laser facilities. In the range of the strain rates of 10{sup 6} – 10{sup 7} s{sup -1}, the data on the dynamic mechanical strength of the material at rapure (spallation) have been for the first time obtained. With a maximal strain rate of 1.4 × 10{sup 7} s{sup -1}, the spall strength of 2.1 GPa is obtained, which constitutes 64% of the theoretical ultimate tensile strength ofmore » graphite. The effect of spallation is observed not only on the rear side of the target, but also on its irradiated (front) surface. With the use of optical and scanning electron microscopes, the morphology of the front and rear surfaces of the targets is studied. By means of Raman scattering of light, the graphite structure both on the target front surface under laser exposure and on its rear side in the spall zone is investigated. A comparison of the dynamic strength of graphite and synthetic diamond is performed. (extreme light fields and their applications)« less

Editorial

NASA Astrophysics Data System (ADS)

Mansur, Louis K.

2018-08-01

The Thirteenth International Workshop on Spallation Materials Technology (IWSMT-13) was held at Chattanooga, Tennessee, October 30 to November 4, 2016. The meeting was organized by Oak Ridge National Laboratory, with participation from the Belgian Nuclear Research Centre, Chinese Academy of Sciences, European Spallation Source, Japan Atomic Energy Agency, Los Alamos National Laboratory, Paul Scherrer Institut, Rutherford Appleton Laboratory and other institutes. The meeting included 52 presentations, of which 9 peer-reviewed full papers are published in this special issue.

Spallation and fracture resulting from reflected and intersecting stress waves.

NASA Technical Reports Server (NTRS)

Kinslow, R.

1973-01-01

Discussion of the effects of stress waves produced in solid by explosions or high-velocity impacts. These waves rebound from free surfaces in the form of tensile waves that are capable of causing internal fractures or spallation of the material. The high-speed framing camera is shown to be an important tool for observing the stress waves and fracture in transparent targets, and its photographs provide valuable information on the mechanics of fracture.

The thermal triple-axis-spectrometer EIGER at the continuous spallation source SINQ

NASA Astrophysics Data System (ADS)

Stuhr, U.; Roessli, B.; Gvasaliya, S.; Rønnow, H. M.; Filges, U.; Graf, D.; Bollhalder, A.; Hohl, D.; Bürge, R.; Schild, M.; Holitzner, L.; Kaegi, C.,; Keller, P.; Mühlebach, T.

2017-05-01

EIGER is the new thermal triple-axis-spectrometer at the continuous spallation SINQ at PSI. The shielding of the monochromator consists only of non- or low magnetizable materials, which allows the use of strong magnetic fields with the instrument. This shielding reduces the high energy neutron contamination to a comparable level of thermal spectrometers at reactor sources. The instrument design, the performance and first results of the spectrometer are presented.

Probing light sterile neutrino signatures at reactor and Spallation Neutron Source neutrino experiments

NASA Astrophysics Data System (ADS)

Kosmas, T. S.; Papoulias, D. K.; Tórtola, M.; Valle, J. W. F.

2017-09-01

We investigate the impact of a fourth sterile neutrino at reactor and Spallation Neutron Source neutrino detectors. Specifically, we explore the discovery potential of the TEXONO and COHERENT experiments to subleading sterile neutrino effects through the measurement of the coherent elastic neutrino-nucleus scattering event rate. Our dedicated χ2-sensitivity analysis employs realistic nuclear structure calculations adequate for high purity sub-keV threshold Germanium detectors.

Negative pressures and spallation in water drops subjected to nanosecond shock waves

DOE PAGES

Stan, Claudiu A.; Willmott, Philip R.; Stone, Howard A.; ...

2016-05-16

Most experimental studies of cavitation in liquid water at negative pressures reported cavitation at tensions significantly smaller than those expected for homogeneous nucleation, suggesting that achievable tensions are limited by heterogeneous cavitation. We generated tension pulses with nanosecond rise times in water by reflecting cylindrical shock waves, produced by X-ray laser pulses, at the internal surface of drops of water. Depending on the X-ray pulse energy, a range of cavitation phenomena occurred, including the rupture and detachment, or spallation, of thin liquid layers at the surface of the drop. When spallation occurred, we evaluated that negative pressures below –100 MPamore » were reached in the drops. As a result, we model the negative pressures from shock reflection experiments using a nucleation-and-growth model that explains how rapid decompression could outrun heterogeneous cavitation in water, and enable the study of stretched water close to homogeneous cavitation pressures.« less

Systematic neutron guide misalignment for an accelerator-driven spallation neutron source

NASA Astrophysics Data System (ADS)

Zendler, C.; Bentley, P. M.

2016-08-01

The European Spallation Source (ESS) is a long pulse spallation neutron source that is currently under construction in Lund, Sweden. A considerable fraction of the 22 planned instruments extend as far as 75-150 m from the source. In such long beam lines, misalignment between neutron guide segments can decrease the neutron transmission significantly. In addition to a random misalignment from installation tolerances, the ground on which ESS is built can be expected to sink with time, and thus shift the neutron guide segments further away from the ideal alignment axis in a systematic way. These systematic errors are correlated to the ground structure, position of buildings and shielding installation. Since the largest deformation is expected close to the target, even short instruments might be noticeably affected. In this study, the effect of this systematic misalignment on short and long ESS beam lines is analyzed, and a possible mitigation by overillumination of subsequent guide sections investigated.

Microstructural probing of ferritic/martensitic steels using internal transmutation-based positron source

NASA Astrophysics Data System (ADS)

Krsjak, Vladimir; Dai, Yong

2015-10-01

This paper presents the use of an internal 44Ti/44Sc radioisotope source for a direct microstructural characterization of ferritic/martensitic (f/m) steels after irradiation in targets of spallation neutron sources. Gamma spectroscopy measurements show a production of ∼1MBq of 44Ti per 1 g of f/m steels irradiated at 1 dpa (displaced per atom) in the mixed proton-neutron spectrum at the Swiss spallation neutron source (SINQ). In the decay chain 44Ti → 44Sc → 44Ca, positrons are produced together with prompt gamma rays which enable the application of different positron annihilation spectroscopy (PAS) analyses, including lifetime and Doppler broadening spectroscopy. Due to the high production yield, long half-life and relatively high energy of positrons of 44Ti, this methodology opens up new potential for simple, effective and inexpensive characterization of radiation induced defects in f/m steels irradiated in a spallation target.

Spallation processes and nuclear interaction products of cosmic rays.

PubMed

Silberberg, R; Tsao, C H

1990-08-01

Most cosmic-ray nuclei heavier than helium have suffered nuclear collisions in the interstellar gas, with transformation of nuclear composition. The isotopic and elemental composition at the sources has to be inferred from the observed composition near the Earth. The source composition permits tests of current ideas on sites of origin, nucleosynthesis in stars, evolution of stars, the mixing and composition of the interstellar medium and injection processes prior to acceleration. The effects of nuclear spallation, production of radioactive nuclides and the time dependence of their decay provide valuable information on the acceleration and propagation of cosmic rays, their nuclear transformations, and their confinement time in the Galaxy. The formation of spallation products that only decay by electron capture and are relatively long-lived permits an investigation of the nature and density fluctuations (like clouds) of the interstellar medium. Since nuclear collisions yield positrons, antiprotons, gamma rays and neutrinos, we shall discuss these topics briefly.

Simulation of spallation life of metals in relation to operating stresses in the nanosecond loading time range

NASA Astrophysics Data System (ADS)

Makarov, P. V.; Bakeev, R. A.

2015-10-01

Spall fracture of materials is still the only means for investigation of the material life and mechanisms of its fracture in the micro-, nano-, and picosecond time ranges of tensile loading. The phenomenological model based on the concepts of multiscale fracture of materials as nonlinear dynamic systems is shown to satisfactorily describe their life in the given range. The model is employed for the calculation of spallation life.

The Macromolecular Neutron Diffractometer MaNDi at the Spallation Neutron Source

DOE PAGES

Coates, Leighton; Cuneo, Matthew J.; Frost, Matthew J.; ...

2015-07-18

The Macromolecular Neutron Diffractometer (MaNDi) is located on beamline 11B of the Spallation Neutron Source at Oak Ridge National Laboratory. Moreover, the instrument is a neutron time-of-flight wavelength-resolved Laue diffractometer optimized to collect diffraction data from single crystals. Finally, the instrument has been designed to provide flexibility in several instrumental parameters, such as beam divergence and wavelength bandwidth, to allow data collection from a range of macromolecular systems.

Fundamental neutron physics beamline at the spallation neutron source at ORNL

DOE PAGES

Fomin, N.; Greene, G. L.; Allen, R. R.; ...

2014-11-04

In this paper, we describe the Fundamental Neutron Physics Beamline (FnPB) facility located at the Spallation Neutron Source at Oak Ridge National Laboratory. The FnPB was designed for the conduct of experiments that investigate scientific issues in nuclear physics, particle physics, astrophysics and cosmology using a pulsed slow neutron beam. Finally, we present a detailed description of the design philosophy, beamline components, and measured fluxes of the polychromatic and monochromatic beams.

Chemical isolation of .sup.82 Sr from proton-irradiated Mo targets

DOEpatents

Grant, Patrick M.; Kahn, Milton; O'Brien, Jr., Harold A.

1976-01-01

Spallation reactions are induced in Mo targets with 200-800 MeV protons to produce microcurie to millicurie amounts of a variety of radionuclides. A six-step radiochemical procedure, incorporating precipitation, solvent extractions, and ion exchange techniques, has been developed for the separation and purification of Sr radioactivities from other spallation products and the bulk target material. Radiostrontium can be quantitatively recovered in a sufficiently decontaminated state for use in biomedical generator development.

Observation of galactic cosmic ray spallation events from the SoHO mission 20-yr operation of LASCO

NASA Astrophysics Data System (ADS)

Koutchmy, S.; Tavabi, E.; Urtado, O.

2018-07-01

A shower of secondary cosmic ray (CR) particles is produced at high altitudes in the Earth's atmosphere, so the primordial galactic cosmic rays (GCRs) are never directly measured outside the Earth magnetosphere and atmosphere. They approach the Earth and other planets in the complex pattern of rigidity's dependence, generally excluded by the magnetosphere. GCRs revealed by images of single nuclear reactions also called spallation events are described here. Such an event was seen on 2015 November 29 using a unique Large Angle and Spectrometric Coronagraphs C3 space coronagraph routine image taken during the Solar and Heliospheric Observatory (SoHO) mission observing uninterruptedly at the Lagrangian L1 point. The spallation signature of a GCR identified well outside the Earth's magnetosphere is obtained for the first time. The resulting image includes different diverging linear `tracks' of varying intensity, leading to a single pixel; this frame identifies the site on the silicon CCD chip of the coronagraph camera. There was no solar flare reported at that time, nor coronal mass ejection and no evidence of optical debris around the spacecraft. More examples of smaller CR events have been discovered through the 20 yr of continuous observations from SoHO. This is the first spallation event from a CR, recorded outside the Earth's magnetosphere. We evaluate the probable energy of these events suggesting a plausible galactic source.

Observation of galactic cosmic ray spallation events from the SoHO mission 20-Year operation of LASCO

NASA Astrophysics Data System (ADS)

Koutchmy, S.; Tavabi, E.; Urtado, O.

2018-05-01

A shower of secondary Cosmic Ray (CR) particles is produced at high altitudes in the Earth's atmosphere, so the primordial Galactic Cosmic Rays (GCRs) are never directly measured outside the Earth magnetosphere and atmosphere. They approach the Earth and other planets in the complex pattern of rigidity's dependence, generally excluded by the magnetosphere. GCRs revealed by images of single nuclear reactions also called spallation events are described here. Such an event was seen on Nov. 29, 2015 using a unique LASCO C3 space coronagraph routine image taken during the Solar and Heliospheric Observatory (SoHO) mission observing uninterruptedly at the Lagrangian L1 point. The spallation signature of a GCR identified well outside the Earth's magnetosphere is obtained for the 1st time. The resulting image includes different diverging linear "tracks" of varying intensity, leading to a single pixel; this frame identifies the site on the silicon CCD chip of the coronagraph camera. There was no solar flare reported at that time, nor Coronal Mass Ejection (CME) and no evidence of optical debris around the spacecraft. More examples of smaller CR events have been discovered through the 20 years of continuous observations from SoHO. This is the first spallation event from a CR, recorded outside the Earth's magnetosphere. We evaluate the probable energy of these events suggesting a plausible galactic source.

Moisture-Induced Alumina Scale Spallation: The Hydrogen Factor

NASA Technical Reports Server (NTRS)

Smialek, James L.

2009-01-01

For some time our community has been concerned with interfacial spallation of protective alumina scales, not just upon immediate cooldown, but as a time-delayed phenomenon. Moisture-induced delayed spallation (MIDS) and desktop spallation (DTS) of TBC's refer to this process. It is most apparent for relatively adherent alumina scales that have survived cool down in a dry environment, built up considerable thickness and strain energy, and have been somewhat damaged, such as by cyclic oxidation cracking. Indeed, a "sweet zone" can be defined that maximizes the observed effect as a function of all the relevant factors. Moisture has been postulated to serve as a source of interfacial hydrogen embrittlement derived from reaction with aluminum in the alloy at an exposed interface. The purpose of this monograph is to trace the close analogy of this phenomenon to other hydrogen effects, such as embrittlement of aluminides and blistering of alloys and anodic alumina films. A formalized, top-down, logic tree structure is presented as a guide to this discussion. A theoretical basis for interfacial weakening by hydrogen is first cited, as are demonstrations of hydrogen as a reaction product or detected interfacial species. Further support is provided by critical experiments that produce the same moisture effect, but by isolating hydrogen from other potential causative factors. These experiments include tests in H2-containing atmospheres or cathodic hydrogen charging.

Decommissioning and PIE of the MEGAPIE spallation target

DOE Office of Scientific and Technical Information (OSTI.GOV)

Latge, C.; Henry, J.; Wohlmuther, M.

2013-07-01

A key experiment in the Accelerated Driven Systems roadmap, the MEGAwatt PIlot Experiment (MEGAPIE) (1 MW) was initiated in 1999 in order to design and build a liquid lead-bismuth spallation target, then to operate it into the Swiss spallation neutron facility SINQ at Paul Scherrer Institute. The target has been designed, manufactured, and tested during integral tests, before irradiation carried out end of 2006. During irradiation, neutron and thermo hydraulic measurements were performed allowing deep interpretation of the experiment and validation of the models used during design phase. The decommissioning, Post Irradiation Examinations and waste management phases were defined properly.more » The phases dedicated to cutting, sampling, cleaning, waste management, samples preparation and shipping to various laboratories were performed by PSI teams: all these phases constitute a huge work, which allows now to perform post-irradiation examination (PIE) of structural material, irradiated in relevant conditions. Preliminary results are presented in the paper, they concern chemical characterization. The following radio-nuclides have been identified by γ-spectrometry: {sup 60}Co, {sup 101}Rh, {sup 102}Rh, {sup 108m}Ag, {sup 110m}Ag, {sup 133}Ba, {sup 172}Hf/Lu, {sup 173}Lu, {sup 194}Hg/Au, {sup 195}Au, {sup 207}Bi. For some of these nuclides the activities can be easily evaluated from γ-spectrometry results ({sup 207}Bi, {sup 194}Hg/Au), while other nuclides can only be determined after chemical separations ({sup 108m}Ag, {sup 110m}Ag, {sup 195}Au, {sup 129}I, {sup 36}Cl and α-emitting {sup 208-210}Po). The concentration of {sup 129}I is lower than expected. The chemical analysis already performed on spallation and corrosion products in the lead-bismuth eutectic (LBE) are very relevant for further applications of LBE as a spallation media and more generally as a coolant.« less

Windows(Registered Trademark)-Based Software Models Cyclic Oxidation Behavior

NASA Technical Reports Server (NTRS)

Smialek, J. L.; Auping, J. V.

2004-01-01

Oxidation of high-temperature aerospace materials is a universal issue for combustion-path components in turbine or rocket engines. In addition to the question of the consumption of material due to growth of protective scale at use temperatures, there is also the question of cyclic effects and spallation of scale on cooldown. The spallation results in the removal of part of the protective oxide in a discontinuous step and thereby opens the way for more rapid oxidation upon reheating. In experiments, cyclic oxidation behavior is most commonly characterized by measuring changes in weight during extended time intervals that include hundreds or thousands of heating and cooling cycles. Weight gains occurring during isothermal scale-growth processes have been well characterized as being parabolic or nearly parabolic functions of time because diffusion controls reaction rates. In contrast, the net weight change in cyclic oxidation is the sum of the effects of the growth and spallation of scale. Typically, the net weight gain in cyclic oxidation is determined only empirically (that is, by measurement), with no unique or straightforward mathematical connection to either the rate of growth or the amount of metal consumed. Thus, there is a need for mathematical modeling to infer spallation mechanisms. COSP is a computer program that models the growth and spallation processes of cyclic oxidation on the basis of a few elementary assumptions that were discussed in COSP: A Computer Model of Cyclic Oxidation, Oxidation of Metals, vol. 36, numbers 1 and 2, 1991, pages 81-112. Inputs to the model include the selection of an oxidation-growth law and a spalling geometry, plus oxide-phase, growth-rate, cycle-duration, and spall-constant parameters. (The spalling fraction is often shown to be a constant factor times the existing amount of scale.) The output of COSP includes the net change in weight, the amounts of retained and spalled oxide, the total amounts of oxygen and metal consumed, and the terminal rates of weight loss and metal consumption.

Spallation radiation effects in materials

DOE Office of Scientific and Technical Information (OSTI.GOV)

Mansur, L.K.; Farrell, K.; Wechsler, M.S.

1996-06-01

Spallation refers to the process whereby particles (chiefly neutrons) are ejected from nuclei upon bombardment by high-energy protons. Spallation neutron sources (SNS`s) use these neutrons for neutron scattering and diffraction research, and SNS`s are proposed as the basis for systems for tritium production and transmutation of nuclear waste. Materials in SNS`s are exposed to the incident proton beam (energies typically about 1000 MeV) and to the spallation neutrons (spectrum of energies extending up to about 1000 MeV). By contrast the fission neutrons in nuclear reactors have an average energy of only about 2 MeV, and the neutrons in fusion reactorsmore » would have energies below about 14 MeV. Furthermore, the protons and neutrons in SNS`s for scattering and diffraction research are pulsed at frequencies of about 10 to 60 Hz, from which significant changes in the kinetics of point and extended defects may be expected. In addition, much higher transmutation rates occur in SNS-irradiated materials, On the whole, then, significant differences in microstructural development and macroscopic properties may result upon exposure in SNS systems, as compared with fission and fusion irradiations. In a more general sense, subjecting materials to new radiation environments has almost routinely led to new discoveries. To the extent that data are avaiable, however, the spallation environment appears to increase the degree of damage without introducing totally new effects. The first part of this presentation is an overview of radiation effects in materials, outlining essential concepts and property changes and their physical bases. This background is followed by a description of SNS irradiation environments and the effects on materials of exposure to these environments. A special discussion is given of the selection of target (e.g., liquid mercury), container (e.g., austenitic stainless steel or ferritic/martensitic steel), and structural materials in SNS systems.« less

Longitudinal space charge compensation at PSR

NASA Astrophysics Data System (ADS)

Neri, Filippo

1998-11-01

The longitudinal space-charge force in neutron spallation source compressor ring or other high intensity proton storage rings can be compensated by introducing an insert in the ring. The effect of the inductor is to cancel all or part of the space charge potential, because it is capacitive. The Proton Storage Ring at Los Alamos National Laboratory is a compressor ring used to produce short pulses of spallation neutrons. Inductive inserts design for space charge compensation at the Los Alamos Proton Storage Ring is described.

Incineration of nuclear waste by accelerator

NASA Astrophysics Data System (ADS)

Martino, J.; Fioni, G.; Leray, S.

1998-10-01

An important international effort is devoted to find a suitable solution to incinerate radioactive nuclear waste issued from conventional power plants and from nuclear disarmament. Practically all innovative projects consist of a sub critical system driven by an external neutron source obtained by spallation induced by a high intensity proton accelerator irradiating a heavy target. New nuclear data measurements are necessary for the realization of these systems, in particular a good knowledge of the spallation process and of the neutron cross sections for transuranic elements are essential.

X-ray microtomography study of the spallation response in Ta-W

NASA Astrophysics Data System (ADS)

McDonald, Samuel; Cotton, Matthew; Millett, Jeremy; Bourne, Neil; Withers, Philip

2013-06-01

The response of metallic materials to high strain-rate (impact) loading is of interest to a number of communities. Traditionally, the largest driver has been the military, in its need to understand armour and resistance to ballistic attack. More recently, industries such as aerospace (foreign object damage, bird strike, etc.), automotive (crash-worthiness) and satellite protection (orbital debris) have all appreciated the necessity of such information. It is therefore important to understand the dynamic tensile or spallation response, and in particular to be able to observe in three-dimensions, and in a non-invasive manner, the physical damage present in the spalled region post-impact. The current study presents plate impact experiments investigating the spallation damage response of recovered targets of the tantalum alloy Ta-2.5%W. Using X-ray microtomography the damage resulting from differing impact conditions (impact velocity/stress, pulse duration) is compared and characterised in 3-D. Combined with free surface velocity measurements, the tensile failure mechanisms during dynamic loading have been identified.

Influence of deposited nanoparticles on the spall strength of metals under the action of picosecond pulses of shock compression

NASA Astrophysics Data System (ADS)

Ebel, A. A.; Mayer, A. E.

2018-01-01

Molecular dynamic simulations of the generation and propagation of shock pulses of picosecond duration initiated by nanoscale impactors, and their interaction with the rear surface is carried out for aluminum and copper. It is shown that the presence of deposited nanoparticles on the rear surface increases the threshold value of the impact intensity leading to the rear spallation. The interaction of a shock wave with nanoparticles leads to severe plastic deformation in the surface layer of the metal including nanoparticles. A part of the compression pulse energy is expended on the plastic deformation, which suppresses the spall fracture. Spallation threshold substantially increases at large diameters of deposited nanoparticles, but instability develops on the rear surface of the target, which is accompanied by ejection of droplets. The instability disrupts the integrity of the rear surface, though the loss of integrity occurs through the ejection of mass, rather than a spallation.

Studies on cosmogenic nuclides in meteorites with regard to an application as potential depth indicators

NASA Technical Reports Server (NTRS)

Sarafin, R.; Herpers, U.; Englert, P.; Wieler, R.; Signer, P.; Bonani, G.; Hofmann, H. J.; Morenzoni, E.; Nessi, M.; Suter, M.

1986-01-01

Measurements of stable and radioactive spallation products in meteorites allow to investigate their histories, especially with respect to the exposure to galactic cosmic ray particles and the pre-atmospheric size of the object. While the concentrations of spallation products lead to the determination of exposure and terrestrial ages, production rate ratios are characteristic for the location of the sample in the meteorite. So, one of the aims of this investigation on meteorites is to obtain depth indicators from suitable pairs of cosmogenic nuclides. Because of the different depth profiles for nuclide productions it is necessary to determine the concentrations of a larger number of spallation products in aliquots of a single small sample. Such same sample measurements of Be-10 and light noble gases were performed on 15 ordinary chondrites (7 H- and 8 L-chondrites. Be-10 was determined by accelerator mass spectrometry and the noble gases were measured by static mass spectrometry. The results are summarized and discussed.

Initial observations of cavitation-induced erosion of liquid metal spallation target vessels at the Spallation Neutron Source

DOE Office of Scientific and Technical Information (OSTI.GOV)

McClintock, David A; Riemer, Bernie; Ferguson, Phillip D

2012-01-01

During operation of the Spallation Neutron Source (SNS) at Oak Ridge National Laboratory the mechanical properties of the AISI 316L target module are altered by high-energy neutron and proton radiation. The interior surfaces of the target vessel are also damaged by cavitation-induced erosion, which results from repetitive rapid heating of the liquid mercury by high-energy proton beam pulses. Until recently no observations of cavitation-induced erosion were possible for conditions prototypical to the SNS. Post irradiation examination (PIE) of the first and second operational SNS targets was performed to gain insight into the radiation-induced changes in mechanical properties of the 316Lmore » target material and the extent of cavitation-induced erosion to the target vessel inner surfaces. Observations of cavitation-induced erosion of the first and second operational SNS target modules are presented here, including images of the target vessel interiors and specimens removed from the target beam-entrance regions.« less

Energy deposition calculated by PHITS code in Pb spallation target

NASA Astrophysics Data System (ADS)

Yu, Quanzhi

2016-01-01

Energy deposition in a Pb spallation target irradiated by high energetic protons was calculated by PHITS2.52 code. The validation of the energy deposition and neutron production calculated by PHITS code was performed. Results show good agreements between the simulation results and the experimental data. Detailed comparison shows that for the total energy deposition, PHITS simulation result was about 15% overestimation than that of the experimental data. For the energy deposition along the length of the Pb target, the discrepancy mainly presented at the front part of the Pb target. Calculation indicates that most of the energy deposition comes from the ionizations of the primary protons and the produced secondary particles. With the event generator mode of PHITS, the deposit energy distribution for the particles and the light nulclei is presented for the first time. It indicates that the primary protons with energy more than 100 MeV are the most contributors to the total energy deposition. The energy depositions peaking at 10 MeV and 0.1 MeV, are mainly caused by the electrons, pions, d, t, 3He and also α particles during the cascade process and the evaporation process, respectively. The energy deposition density caused by different proton beam profiles are also calculated and compared. Such calculation and analyses are much helpful for better understanding the physical mechanism of energy deposition in the spallation target, and greatly useful for the thermal hydraulic design of the spallation target.

Opportunities for Neutrino Physics at the Spallation Neutron Source: A White Paper

DOE Office of Scientific and Technical Information (OSTI.GOV)

Bolozdynya, A.; Cavanna, F.; Efremenko, Y.

2012-11-01

The Spallation Neutron Source (SNS) at Oak Ridge National Laboratory, Tennessee, provides an intense flux of neutrinos in the few tens-of-MeV range, with a sharply-pulsed timing structure that is beneficial for background rejection. In this document, the product of a workshop at the SNS in May 2012, we describe this free, high-quality stopped-pion neutrino source and outline various physics that could be done using it. We describe without prioritization some specific experimental configurations that could address these physics topics.

Surface modification to prevent oxide scale spallation

DOEpatents

Stephens, Elizabeth V; Sun, Xin; Liu, Wenning; Stevenson, Jeffry W; Surdoval, Wayne; Khaleel, Mohammad A

2013-07-16

A surface modification to prevent oxide scale spallation is disclosed. The surface modification includes a ferritic stainless steel substrate having a modified surface. A cross-section of the modified surface exhibits a periodic morphology. The periodic morphology does not exceed a critical buckling length, which is equivalent to the length of a wave attribute observed in the cross section periodic morphology. The modified surface can be created using at least one of the following processes: shot peening, surface blasting and surface grinding. A coating can be applied to the modified surface.

Influence of sweeping detonation-wave loading on damage evolution during spallation loading of tantalum in both a planar and curved geometry

DOE Office of Scientific and Technical Information (OSTI.GOV)

Gray, George Thompson III; Hull, Lawrence Mark; Livescu, Veronica

Widespread research over the past five decades has provided a wealth of experimental data and insight concerning the shock hardening, damage evolution, and the spallation response of materials subjected to square-topped shock-wave loading profiles. However, fewer quantitative studies have been conducted on the effect of direct, in-contact, high explosive (HE)-driven Taylor wave (unsupported shocks) loading on the shock hardening, damage evolution, or spallation response of materials. Systematic studies quantifying the effect of sweeping-detonation wave loading are yet sparser. In this study, the damage evolution and spallation response of Ta is shown to be critically dependent on the peak shock stress,more » the geometry of the sample (flat or curved plate geometry), and the shock obliquity during sweeping-detonation-wave shock loading. Sweepingwave loading in the flat-plate geometry is observed to: a) yield a lower spall strength than previously documented for 1-D supported-shock-wave loading, b) exhibit increased shock hardening as a function of increasing obliquity, and c) lead to an increased incidence of deformation twin formation with increasing shock obliquity. Sweeping-wave loading of a 10 cm radius curved Ta plate is observed to: a) lead to an increase in the shear stress as a function of increasing obliquity, b) display a more developed level of damage evolution, extensive voids and coalescence, and lower spall strength with obliquity in the curved plate than seen in the flat-plate sweeping-detonation wave loading for an equivalent HE loading, and c) no increased propensity for deformation twin formation with increasing obliquity as seen in the flat-plate geometry. The overall observations comparing and contrasting the flat versus curved sweeping-wave spall experiments with 1D loaded spallation behavior suggests a coupled influence of obliquity and geometry on dynamic shock-induced damage evolution and spall strength. Coupled experimental and modeling research to quantify the combined effects of sweeping-wave loading with increasingly complex sample geometries on the shockwave response of materials is clearly crucial to providing the basis for developing and thereafter validation of predictive modeling capability.« less

Bacterial spores in granite survive hypervelocity launch by spallation: implications for lithopanspermia.

PubMed

Fajardo-Cavazos, Patricia; Langenhorst, Falko; Melosh, H Jay; Nicholson, Wayne L

2009-09-01

Bacterial spores are considered good candidates for endolithic life-forms that could survive interplanetary transport by natural impact processes, i.e., lithopanspermia. Organisms within rock can only embark on an interplanetary journey if they survive ejection from the surface of the donor planet and the associated extremes of compressional shock, heating, and acceleration. Previous simulation experiments have measured each of these three stresses more or less in isolation of one another, and results to date indicate that spores of the model organism Bacillus subtilis can survive each stress applied singly. Few simulations, however, have combined all three stresses simultaneously. Because considerable experimental and theoretical evidence supports a spallation mechanism for launch, we devised an experimental simulation of launch by spallation using the Ames Vertical Gun Range (AVGR). B. subtilis spores were applied to the surface of a granite target that was impacted from above by an aluminum projectile fired at 5.4 km/s. Granite spall fragments were captured in a foam recovery fixture and then recovered and assayed for shock damage by transmission electron microscopy and for spore survival by viability assays. Peak shock pressure at the impact site was calculated to be 57.1 GPa, though recovered spall fragments were only very lightly shocked at pressures of 5-7 GPa. Spore survival was calculated to be on the order of 10(-5), which is in agreement with results of previous static compressional shock experiments. These results demonstrate that endolithic spores can survive launch by spallation from a hypervelocity impact, which lends further evidence in favor of lithopanspermia theory.

Principles for timing at spallation neutron sources based on developments at LANSCE

DOE Office of Scientific and Technical Information (OSTI.GOV)

Nelson, R. O.; Merl, R. B.; Rose, C. R.

2001-01-01

Due to AC-power-grid frequency fluctuations, the designers for accelerator-based spallation-neutron facilities have worked to optimize the conflicting demands of accelerator and neutron chopper performance. For the first time, we are able to quantitatively access the tradeoffs between these two constraints and design or upgrade a facility to optimize total system performance using powerful new simulation techniques. We have modeled timing systems that integrate chopper controllers and chopper hardware and built new systems. Thus, at LANSCE, we now operate multiple chopper systems and the accelerator as simple slaves to a single master-timing-reference generator. Based on this experience we recommend that spallationmore » neutron sources adhere to three principles. First, timing for pulsed sources should be planned starting with extraction at a fixed phase and working backwards toward the leading edge of the beam pulse. Second, accelerator triggers and storage ring extraction commands from neutron choppers offer only marginal benefits to accelerator-based spallation sources. Third, the storage-ring RF should be phase synchronized with neutron choppers to provide extraction without the one orbit timing uncertainty.« less

Fracture Mechanics Analyses of Subsurface Defects in Reinforced Carbon-Carbon Joggles Subjected to Thermo-Mechanical Loads

NASA Technical Reports Server (NTRS)

Knight, Norman F., Jr.; Raju, Ivatury S.; Song, Kyongchan

2011-01-01

Coating spallation events have been observed along the slip-side joggle region of the Space Shuttle Orbiter wing-leading-edge panels. One potential contributor to the spallation event is a pressure build up within subsurface voids or defects due to volatiles or water vapor entrapped during fabrication, refurbishment, or normal operational use. The influence of entrapped pressure on the thermo-mechanical fracture-mechanics response of reinforced carbon-carbon with subsurface defects is studied. Plane-strain simulations with embedded subsurface defects are performed to characterize the fracture mechanics response for a given defect length when subjected to combined elevated-temperature and subsurface-defect pressure loadings to simulate the unvented defect condition. Various subsurface defect locations of a fixed-length substrate defect are examined for elevated temperature conditions. Fracture mechanics results suggest that entrapped pressure combined with local elevated temperatures have the potential to cause subsurface defect growth and possibly contribute to further material separation or even spallation. For this anomaly to occur, several unusual circumstances would be required making such an outcome unlikely but plausible.

New generation high performance in situ polarized 3He system for time-of-flight beam at spallation sources.

PubMed

Jiang, C Y; Tong, X; Brown, D R; Glavic, A; Ambaye, H; Goyette, R; Hoffmann, M; Parizzi, A A; Robertson, L; Lauter, V

2017-02-01

Modern spallation neutron sources generate high intensity neutron beams with a broad wavelength band applied to exploring new nano- and meso-scale materials from a few atomic monolayers thick to complicated prototype device-like systems with multiple buried interfaces. The availability of high performance neutron polarizers and analyzers in neutron scattering experiments is vital for understanding magnetism in systems with novel functionalities. We report the development of a new generation of the in situ polarized 3 He neutron polarization analyzer for the Magnetism Reflectometer at the Spallation Neutron Source at Oak Ridge National Laboratory. With a new optical layout and laser system, the 3 He polarization reached and maintained 84% as compared to 76% in the first-generation system. The polarization improvement allows achieving the transmission function varying from 50% to 15% for the polarized neutron beam with the wavelength band of 2-9 Angstroms. This achievement brings a new class of experiments with optimal performance in sensitivity to very small magnetic moments in nano systems and opens up the horizon for its applications.

Mercury Cavitation Phenomenon in Pulsed Spallation Neutron Sources

DOE Office of Scientific and Technical Information (OSTI.GOV)

Futakawa, Masatoshi; Naoe, Takashi; Kawai, Masayoshi

2008-06-24

Innovative researches will be performed at Materials and Life Science Experimental Facility in J-PARC, in which a mercury target system will be installed as MW-class pulse spallation neutron sources. Proton beams will be injected into mercury target to induce the spallation reaction. At the moment the intense proton beam hits the target, pressure waves are generated in the mercury because of the abrupt heat deposition. The pressure waves interact with the target vessel leading to negative pressure that may cause cavitation along the vessel wall. Localized impacts by micro-jets and/or shock waves which are caused by cavitation bubble collapse imposemore » pitting damage on the vessel wall. The pitting damage which degrades the structural integrity of target vessels is a crucial issue for high power mercury targets. Micro-gas-bubbles injection into mercury may be useful to mitigate the pressure wave and the pitting damage. The visualization of cavitation-bubble and gas-bubble collapse behaviors was carried out by using a high-speed video camera. The differences between them are recognized.« less

Production of radioactive isotopes through cosmic muon spallation in KamLAND

DOE Office of Scientific and Technical Information (OSTI.GOV)

Abe, S.; Furuno, K.; Gando, Y.

2010-02-15

Radioactive isotopes produced through cosmic muon spallation are a background for rare-event detection in nu detectors, double-beta-decay experiments, and dark-matter searches. Understanding the nature of cosmogenic backgrounds is particularly important for future experiments aiming to determine the pep and CNO solar neutrino fluxes, for which the background is dominated by the spallation production of {sup 11}C. Data from the Kamioka liquid-scintillator antineutrino detector (KamLAND) provides valuable information for better understanding these backgrounds, especially in liquid scintillators, and for checking estimates from current simulations based upon MUSIC, FLUKA, and GEANT4. Using the time correlation between detected muons and neutron captures, themore » neutron production yield in the KamLAND liquid scintillator is measured to be Y{sub n}=(2.8+-0.3)x10{sup -4} mu{sup -1} g{sup -1} cm{sup 2}. For other isotopes, the production yield is determined from the observed time correlation related to known isotope lifetimes. We find some yields are inconsistent with extrapolations based on an accelerator muon beam experiment.« less

Study of the Production of Radioactive Isotopes through Cosmic Muon Spallation in KamLAND

DOE Office of Scientific and Technical Information (OSTI.GOV)

KamLAND Collaboration; Abe, S.; Enomoto, S.

2009-06-30

Radioactive isotopes produced through cosmic muon spallation are a background for rare event detection in {nu} detectors, double-beta-decay experiments, and dark-matter searches. Understanding the nature of cosmogenic backgrounds is particularly important for future experiments aiming to determine the pep and CNO solar neutrino fluxes, for which the background is dominated by the spallation production of {sup 11}C. Data from the Kamioka Liquid scintillator Anti-Neutrino Detector (KamLAND) provides valuable information for better understanding these backgrounds, especially in liquid scintillator, and for checking estimates from current simulations based upon MUSIC, FLUKA, and Geant4. Using the time correlation between detected muons and neutronmore » captures, the neutron production yield in the KamLAND liquid scintillator is measured to be (2.8 {+-} 0.3) x 10{sup -4} n/({mu} {center_dot} (g/cm{sup 2})). For other isotopes, the production yield is determined from the observed time correlation related to known isotope lifetimes. We find some yields are inconsistent with extrapolations based on an accelerator muon beam experiment.« less

The National Spallation Neutron Source (NSNS) Project

NASA Astrophysics Data System (ADS)

Appleton, Bill R.

1997-05-01

The need and justification for new sources and instrumentation in neutron science have been firmly established by numerous assessments since the early 1970s by the scientific community and the Department of Energy (DOE). In their 1996 budget, the DOE Office of Energy Research asked ORNL to lead the R&D and conceptual design effort for a next-generation spallation neutron source to be used for neutron scattering. To accomplish this, the NSNS collaboration involving five national laboratories (ANL, BNL, LANL, LBNL, and ORNL) has been formed. The NSNS reference design is for a 1-GeV linac and accumulator ring that delivers 1-MW proton beams in microsend pulses to a mercuty target; neutrons are produced by the spallation reaction, moderated, and guided into an experimental hall for neutron scattering. The design includes the necessary flexibility to upgrade the source in stages to significantly higher powers in the future and to expand the experimental capabilities. This talk will describe the origins at NSNS, the current funding status, progress on the technical design, user community input and the intended uses, and future prospects.

Study of 232Th(n, γ) and 232Th(n,f) reaction rates in a graphite moderated spallation neutron field produced by 1.6 GeV deuterons on lead target

NASA Astrophysics Data System (ADS)

Asquith, N. L.; Hashemi-Nezhad, S. R.; Westmeier, W.; Zhuk, I.; Tyutyunnikov, S.; Adam, J.

2015-02-01

The Gamma-3 assembly of the Joint Institute for Nuclear Research (JINR), Dubna, Russia is designed to emulate the neutron spectrum of a thermal Accelerator Driven System (ADS). It consists of a lead spallation target surrounded by reactor grade graphite. The target was irradiated with 1.6 GeV deuterons from the Nuclotron accelerator and the neutron capture and fission rate of 232Th in several locations within the assembly were experimentally measured. 232Th is a proposed fuel for envisaged Accelerator Driven Systems and these two reactions are fundamental to the performance and feasibility of 232Th in an ADS. The irradiation of the Gamma-3 assembly was also simulated using MCNPX 2.7 with the INCL4 intra-nuclear cascade and ABLA fission/evaporation models. Good agreement between the experimentally measured and calculated reaction rates was found. This serves as a good validation for the computational models and cross section data used to simulate neutron production and transport of spallation neutrons within a thermal ADS.

Oak Ridge Spallation Neutron Source (ORSNS) target station design integration

DOE Office of Scientific and Technical Information (OSTI.GOV)

McManamy, T.; Booth, R.; Cleaves, J.

1996-06-01

The conceptual design for a 1- to 3-MW short pulse spallation source with a liquid mercury target has been started recently. The design tools and methods being developed to define requirements, integrate the work, and provide early cost guidance will be presented with a summary of the current target station design status. The initial design point was selected with performance and cost estimate projections by a systems code. This code was developed recently using cost estimates from the Brookhaven Pulsed Spallation Neutron Source study and experience from the Advanced Neutron Source Project`s conceptual design. It will be updated and improvedmore » as the design develops. Performance was characterized by a simplified figure of merit based on a ratio of neutron production to costs. A work breakdown structure was developed, with simplified systems diagrams used to define interfaces and system responsibilities. A risk assessment method was used to identify potential problems, to identify required research and development (R&D), and to aid contingency development. Preliminary 3-D models of the target station are being used to develop remote maintenance concepts and to estimate costs.« less

Mining Archived HYSPEC User Data to Analyze the Prompt Pulse at the SNS

DOE Office of Scientific and Technical Information (OSTI.GOV)

Smith, Michael B.; Iverson, Erik B.; Gallmeier, Franz X.

The Hybrid-Spectrometer (HYSPEC) is one of 17 instruments currently operated at the Spallation Neutron Source (SNS) at Oak Ridge National Laboratories (ORNL). The secondary spectrometer of this instrument is located inside an out-building off the north side of the SNS instrument hall. HYSPEC has experienced a larger background feature than similar inelastic instruments since its commissioning in 2011. This background feature is caused by a phenomenon known as the “prompt pulse” which is an essential part of neutron production in a pulsed spallation source but comes with unfortunate side effects.

Observations of Space Charge effects in the Spallation Neutron Source Accumulator Ring

DOE Office of Scientific and Technical Information (OSTI.GOV)

Potts III, Robert E; Cousineau, Sarah M; Holmes, Jeffrey A

2012-01-01

The Spallation Neutron Source accumulator ring was designed to allow independent control of the transverse beam distribution in each plane. However, at high beam intensities, nonlinear space charge forces can strongly influence the final beam distribution and compromise our ability to independently control the transverse distributions. In this study we investigate the evolution of the beam at intensities of up to ~8x10^13 ppp through both simulation and experiment. Specifically, we analyze the evolution of the beam distribution for beams with different transverse aspect ratios and tune splits. We present preliminary results of simulations of our experiments.

Comparison between experimental data and Monte-Carlo simulations of neutron production in spallation reactions of 0.7-1.5 GeV protons on a thick, lead target

NASA Astrophysics Data System (ADS)

Krása, A.; Majerle, M.; Krízek, F.; Wagner, V.; Kugler, A.; Svoboda, O.; Henzl, V.; Henzlová, D.; Adam, J.; Caloun, P.; Kalinnikov, V. G.; Krivopustov, M. I.; Stegailov, V. I.; Tsoupko-Sitnikov, V. M.

2006-05-01

Relativistic protons with energies 0.7-1.5 GeV interacting with a thick, cylindrical, lead target, surrounded by a uranium blanket and a polyethylene moderator, produced spallation neutrons. The spatial and energetic distributions of the produced neutron field were measured by the Activation Analysis Method using Al, Au, Bi, and Co radio-chemical sensors. The experimental yields of isotopes induced in the sensors were compared with Monte-Carlo calculations performed with the MCNPX 2.4.0 code.

Characterization of γ-ray background at IMAT beamline of ISIS Spallation Neutron Source

NASA Astrophysics Data System (ADS)

Festa, G.; Andreani, C.; Arcidiacono, L.; Burca, G.; Kockelmann, W.; Minniti, T.; Senesi, R.

2017-08-01

The environmental γ -ray background on the IMAT beamline at ISIS Spallation Neutron Source, Target Station 2, is characterized via γ spectroscopy. The measurements include gamma exposure at the imaging detector position, along with the gamma background inside the beamline. Present results are discussed and compared with previous measurements recorded at INES and VESUVIO beamlines operating at Target Station 1. They provide new outcome for expanding and optimizing the PGAA experimental capability at the ISIS neutron source for the investigation of materials, engineering components and cultural heritage objects at the ISIS neutron source.

Double differential cross section calculations for 16O and 90Zr elements

NASA Astrophysics Data System (ADS)

Demirkol, İ.

2018-04-01

Double differential cross sections in proton induced reactions on 90Zr and O2 (inert matrix fuel) is calculated at the bombarding energies between 29 and 300 MeV. The proton-induced nuclear reaction cross section data can be used in technical applications such as the isotope production alternatives, spallation reactions for production of neutrons in spallation neutron source, etc. In this study, the cascade excition model including the effect of preequilibrium is used to calculate the differential cross section. Then, the obtained results are discussed and compared with available experimental data.

Moisture-Induced TBC Spallation on Turbine Blade Samples

NASA Technical Reports Server (NTRS)

Smialek, James

2011-01-01

Delayed failure of TBCs is a widely observed laboratory phenomenon, although many of the early observations went unreported. The weekend effect or DeskTop Spallation (DTS) is characterized by initial survival of a TBC after accelerated laboratory thermal cycling, then failure by exposure to ambient humidity or water. Once initiated, failure can occur quite dramatically in less than a second. To this end, the water drop test and digital video recordings have become useful techniques in studies at NASA (Smialek, Zhu, Cuy), DECHMA (Rudolphi, Renusch, Schuetze), and CNRS Toulouse/SNECMA (Deneux, Cadoret, Hervier, Monceau). In the present study the results for a commercial turbine blade, with a standard EB-PVD 7YSZ TBC top coat and Pt-aluminide diffusion bond coat are reported. Cut sections were intermittently oxidized at 1100, 1150, and 1200 C and monitored by weight change and visual appearance. Failures were distributed widely over a 5-100 hr time range, depending on temperature. At some opportune times, failure was captured by video recording, documenting the appearance and speed of the moisture-induced spallation process. Failure interfaces exhibited alumina scale grains, decorated with Ta-rich oxide particles, and alumina inclusions as islands and streamers. The phenomenon is thus rooted in moisture-induced delayed spallation (MIDS) of the alumina scale formed on the bond coat. In that regard, many studies show the susceptibility of alumina scales to moisture, as long as high strain energy and a partially exposed interface exist. The latter conditions result from severe cyclic oxidation conditions, which produce a highly stressed and partially damaged scale. In one model, it has been proposed that moisture reacts with aluminum in the bond coat to release hydrogen atoms that embrittle the interface. A negative synergistic effect with interfacial sulfur is also invoked.

Moisture-Induced TBC Spallation on Turbine Blade Samples

NASA Technical Reports Server (NTRS)

Smialek, James L.

2011-01-01

Delayed failure of TBCs is a widely observed laboratory phenomenon, although many of the early observations went unreported. "The weekend effect" or "DeskTop Spallation" (DTS) is characterized by initial survival of a TBC after accelerated laboratory thermal cycling, then failure by exposure to ambient humidity or water. Once initiated, failure can occur quite dramatically in less than a second. To this end, the water drop test and digital video recordings have become useful techniques in studies at NASA (Smialek, Zhu, Cuy), DECHMA (Rudolphi, Renusch, Schuetze), and CNRS Toulouse/SNECMA (Deneux, Cadoret, Hervier, Monceau). In the present study the results for a commercial turbine blade, with a standard EB-PVD 7YSZ TBC top coat and Pt-aluminide diffusion bond monitored by weight change and visual appearance. Failures were distributed widely over a 5-100 hr time range, depending on temperature. At some opportune times, failure was captured by video recording, documenting the appearance and speed of the moisture-induced spallation process. Failure interfaces exhibited alumina scale grains, decorated with Ta-rich oxide particles, and alumina inclusions as islands and streamers. The phenomenon is thus rooted in moisture-induced delayed spallation (MIDS) of the alumina scale formed on the bond coat. In that regard, many studies show the susceptibility of alumina scales to moisture, as long as high strain energy and a partially exposed interface exist. The latter conditions result from severe cyclic oxidation conditions, which produce a highly stressed and partially damaged scale. In one model, it has been proposed that moisture reacts with aluminum in the bond coat to release hydrogen atoms that 'embrittle' the interface. A negative synergistic effect with interfacial sulfur is also invoked.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Anderson, David E.

The JEMA modulator was originally developed for the European Spallation Source (ESS) when Spain was under consideration as a location for the ESS facility. Discussions ensued and the Spallation Neutron Source Research Accelerator Division agreed to form a collaboration with ESS-Bilbao (ESS-B) consortium to provide services for specifying the requirements for a version of the modulator capable of operating twelve 550 kW klystrons, monitoring the technical progress on the contract with JEMA, installing and commissioning the modulator at SNS, and performing a 30 day full power test. This work was recently completed, and this report discusses those activities with primarymore » emphasis on the installation and testing activities.« less

Specific features of single-pulse femtosecond laser micron and submicron ablation of a thin silver film coated with a micron-thick photoresist layer

DOE Office of Scientific and Technical Information (OSTI.GOV)

Zayarnyi, D A; Ionin, A A; Kudryashov, S I

Specific features of ablation of a thin silver film with a 1-μm-thick layer of a highly transparent photoresist and the same film without a photoresist layer under single tightly focused femtosecond laser pulses in the visible range (515 nm) are experimentally investigated. Interference effects of internal modification of the photoresist layer, its spallation ablation from the film surface and formation of through hollow submicron channels in the resist without its spallation but with ablation of the silver film lying under the resist are found and discussed. (extreme light fields and their applications)

Deformation dynamics and spallation strength of aluminium under a single-pulse action of a femtosecond laser

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ashitkov, Sergei I; Komarov, P S; Ovchinnikov, A V

An interferometric method is developed and realised using a frequency-modulated pulse for diagnosing a dynamics of fast deformations with a spatial and temporal resolution under the action of a single laser pulse. The dynamics of a free surface of a submicron-thick aluminium film is studied under an action of the ultrashort compression pulse with the amplitude of up to 14 GPa, excited by a femtosecond laser heating of the target surface layer. The spallation strength of aluminium was determined at a record high deformation rate of 3 Multiplication-Sign 10{sup 9} s{sup -1}. (extreme light fields and their applications)

Rare gases and Ca, Sr, and Ba in Apollo 17 drill-core fines

NASA Technical Reports Server (NTRS)

Pepin, R. O.; Dragon, J. C.; Johnson, N. L.; Bates, A.; Coscio, M. R., Jr.; Murthy, V. R.

1975-01-01

Trapped gas isotopic compositions and spallation gas concentrations as functions of depth in the Apollo 17 drill core were determined from mass spectrometer studies by means of correlation techniques. The distribution of He, Ne, Ar, Kr, and Xe as well as Ca, Sr, and Ba was investigated, and rare-gas spallation and neutron capture profiles are compared with attention to proposed depositional models for the Taurus-Littrow regolith. The data exclude a sedimentation pattern similar to that found at the Apollo 15 site but are possibly compatible with long-term continuous accretion models or models of very recent rapid accumulation of regolith.

Practical in-situ determination of ortho-para hydrogen ratios via fiber-optic based Raman spectroscopy

DOE PAGES

Sutherland, Liese -Marie; Knudson, James N.; Mocko, Michal; ...

2015-12-17

An experiment was designed and developed to prototype a fiber-optic-based laser system, which measures the ratio of ortho-hydrogen to para-hydrogen in an operating neutron moderator system at the Los Alamos Neutron Science Center (LANSCE) spallation neutron source. Preliminary measurements resulted in an ortho to para ratio of 3.06:1, which is within acceptable agreement with the previously published ratio. As a result, the successful demonstration of Raman Spectroscopy for this measurement is expected to lead to a practical method that can be applied for similar in-situ measurements at operating neutron spallation sources.

Practical in-situ determination of ortho-para hydrogen ratios via fiber-optic based Raman spectroscopy

DOE Office of Scientific and Technical Information (OSTI.GOV)

Sutherland, Liese -Marie; Knudson, James N.; Mocko, Michal

An experiment was designed and developed to prototype a fiber-optic-based laser system, which measures the ratio of ortho-hydrogen to para-hydrogen in an operating neutron moderator system at the Los Alamos Neutron Science Center (LANSCE) spallation neutron source. Preliminary measurements resulted in an ortho to para ratio of 3.06:1, which is within acceptable agreement with the previously published ratio. As a result, the successful demonstration of Raman Spectroscopy for this measurement is expected to lead to a practical method that can be applied for similar in-situ measurements at operating neutron spallation sources.

Penny-shaped crack propagation in spallation of Zr-BMGs

NASA Astrophysics Data System (ADS)

Ling, Z.; Huang, X.; Dai, L. H.

2015-09-01

Typical penny-shaped microcracks at their propagating in spallation of Zr-based bulk metallic glass (Zr-BMG) samples were captured by a specially designed plate impact technique. Based on the morphology and stress environment of the microcrack, a damaged zone or propagation zone around the crack tips, similar to the cohesive zone in classical fracture theories, is applied. Especially the scale of such a damaged zone represents a scale of the crack propagation. Its fast propagation would quickly bring a longer crack or cause cracks coalesce to form another longer one. The estimated propagation scales of microcracks are reasonable compared with what occurred in the Zr-BMG samples.

Chemical Vapor Deposition of Turbine Thermal Barrier Coatings

NASA Technical Reports Server (NTRS)

Haven, Victor E.

1999-01-01

Ceramic thermal barrier coatings extend the operating temperature range of actively cooled gas turbine components, therefore increasing thermal efficiency. Performance and lifetime of existing ceram ic coatings are limited by spallation during heating and cooling cycles. Spallation of the ceramic is a function of its microstructure, which is determined by the deposition method. This research is investigating metalorganic chemical vapor deposition (MOCVD) of yttria stabilized zirconia to improve performance and reduce costs relative to electron beam physical vapor deposition. Coatings are deposited in an induction-heated, low-pressure reactor at 10 microns per hour. The coating's composition, structure, and response to the turbine environment will be characterized.

The Spallation Neutron Source (SNS) project accelerator systems

NASA Astrophysics Data System (ADS)

Holmes, Jeffrey A.; Alonso, Jose R.

1999-06-01

The SNS will be the world's leading accelerator-based neutron-scattering research facility when it begins operation in 2005. By delivering 1-MW of beam power to a heavy-metal target in short (<1 μs) bursts of 1-GeV protons, the SNS will provide intense neutron beams with flux levels at least a factor of five over present spallation sources. A multi-laboratory (LBNL, LANL, BNL, ANL and ORNL) collaboration, led by Oak Ridge National Laboratory, has developed a reference design that addresses the challenging technology issues associated with this project. This paper discusses the requirements, issues, and constraints that led to the present design choices.

Oxidation behavior of FeAl+Hf,Zr,B

NASA Technical Reports Server (NTRS)

Smialek, James L.; Doychak, Joseph

1988-01-01

The oxidation behavior of Fe-40Al-1Hf, Fe-40Al-1Hf-0.4B, and Fe-40Al-0.1Zr-0.4B (at. percent) alloys was characterized after 900, 1000, and 100 C exposures. Isothermal tests revealed parabolic kinetics after a period of transitional theta-alumina scale growth. The parabolic growth rates for the subsequent alpha-alumina scales were about five times higher than those for NiAl+0.1Zr alloys. The isothermally grown scales showed a propensity toward massive scale spallation due to both extensive rumpling from growth stresses and to an inner layer of HfO2. Cyclic oxidation for 200 1-hr cycles produced little degradation at 900 or 1000 C, but caused significant spallation at 1100 C in the form of small segments of the outer scale. The major difference in the cyclic oxidation of the three FeAl alloys was increased initial spallation for FeAl+Zr,B. Although these FeAl alloys showed many similarities to NiAl alloys, they were generally less oxidation resistant. It is believed that this resulted from nonoptimal levels of dopants and larger thermal expansion mismatch stresses.

Evolution in boron-based GEM detectors for diffraction measurements: from planar to 3D converters

NASA Astrophysics Data System (ADS)

Albani, Giorgia; Perelli Cippo, Enrico; Croci, Gabriele; Muraro, Andrea; Schooneveld, Erik; Scherillo, Antonella; Hall-Wilton, Richard; Kanaki, Kalliopi; Höglund, Carina; Hultman, Lars; Birch, Jens; Claps, Gerardo; Murtas, Fabrizio; Rebai, Marica; Tardocchi, Marco; Gorini, Giuseppe

2016-11-01

The so-called ‘3He-crisis’ has motivated the neutron detector community to undertake an intense R&D programme in order to develop technologies alternative to standard 3He tubes and suitable for neutron detection systems in future spallation sources such as the European spallation source (ESS). Boron-based GEM (gas electron multiplier) detectors are a promising ‘3He-free’ technology for thermal neutron detection in neutron scattering experiments. In this paper the evolution of boron-based GEM detectors from planar to 3D converters with an application in diffraction measurements is presented. The use of 3D converters coupled with GEMs allows for an optimization of the detector performances. Three different detectors were used for diffraction measurements on the INES instrument at the ISIS spallation source. The performances of the GEM-detectors are compared with those of conventional 3He tubes installed on the INES instrument. The conceptual detector with the 3D converter used in this paper reached a count rate per unit area of about 25% relative to the currently installed 3He tube. Its timing resolution is similar and the signal-to-background ratio (S/B) is 2 times lower.

Cavitation damage prediction for spallation target vessels by assessment of acoustic vibration

DOE Office of Scientific and Technical Information (OSTI.GOV)

Futakawa, Masatoshi; Kogawa, Hiroyuki; Hasegawa, Shoichi

2008-01-01

Liquid-mercury target systems for MW-class spallation neutron sources are being developed around the world. Proton beams are used to induce the spallation reaction. At the moment the proton beam hits the target, pressure waves are generated in the mercury because of the abrupt heat deposition. The pressure waves interact with the target vessel leading to negative pressure that may cause cavitation along the vessel wall. In order to estimate the cavitation erosion, i.e. the pitting damage formed by the collapse of cavitation bubbles, off-beam tests were performed by using an electric magnetic impact testing machine (MIMTM), which can impose equivalentmore » pressure pulses in mercury. The damage potential was defined based on the relationship between the pitting damage and the time-integrated acoustic vibration induced by impact due to the bubble collapses. Additionally, the damage potential was measured in on-beam tests carried out by using the proton beam at WNR (Weapons Neutron Research) facility in Los Alamos Neutron Science Center (LANSCE). In this paper, the concept of the damage potential, the relationship between the pitting damage formation and the damage potential both in off-beam and on-beam tests is shown.« less

Assessment of the neutron cross section database for mercury for the ORNL spallation source

DOE Office of Scientific and Technical Information (OSTI.GOV)

Leal, L.C.; Spencer, R.R.; Ingersoll, D.T.

1996-06-01

Neutron source generation based on a high energy particle accelerator has been considered as an alternative to the canceled Advanced Neutron Source project at Oak Ridge National Laboratory. The proposed technique consists of a spallation neutron source in which neutrons are produced via the interaction of high-energy charged particles in a heavy metal target. Preliminary studies indicate that liquid mercury bombarded with GeV protons provides an excellent neutron source. Accordingly, a survey has been made of the available neutron cross-section data. Since it is expected that spectral modifiers, specifically moderators, will also be incorporated into the source design, the surveymore » included thermal energy, resonance region, and high energy data. It was found that data of individual isotopes were almost non-existent and that the only evaluation found for the natural element had regions of missing data or discrepant data. Therefore, it appears that to achieve the desired degree of accuracy in the spallation source design it is necessary to re-evaluate the mercury database including making new measurements. During the presentation the currently available data will be presented and experiments proposed which can lead to design quality cross sections.« less

Overview of ten-year operation of the superconducting linear accelerator at the Spallation Neutron Source

NASA Astrophysics Data System (ADS)

Kim, S.-H.; Afanador, R.; Barnhart, D. L.; Crofford, M.; Degraff, B. D.; Doleans, M.; Galambos, J.; Gold, S. W.; Howell, M. P.; Mammosser, J.; McMahan, C. J.; Neustadt, T. S.; Peters, C.; Saunders, J. W.; Strong, W. H.; Vandygriff, D. J.; Vandygriff, D. M.

2017-04-01

The Spallation Neutron Source (SNS) has acquired extensive operational experience of a pulsed proton superconducting linear accelerator (SCL) as a user facility. Numerous lessons have been learned in its first 10 years operation to achieve a stable and reliable operation of the SCL. In this paper, an overview of the SNS SCL design, qualification of superconducting radio frequency (SRF) cavities and ancillary subsystems, an overview of the SNS cryogenic system, the SCL operation including SCL output energy history and downtime statistics, performance stability of the SRF cavities, efforts for SRF cavity performance recovery and improvement at the SNS, and maintenance activities for cryomodules are introduced.

Low-energy beam transport studies supporting the spallation neutron source 1-MW beam operation.

PubMed

Han, B X; Kalvas, T; Tarvainen, O; Welton, R F; Murray, S N; Pennisi, T R; Santana, M; Stockli, M P

2012-02-01

The H(-) injector consisting of a cesium enhanced RF-driven ion source and a 2-lens electrostatic low-energy beam transport (LEBT) system supports the spallation neutron source 1 MW beam operation with ∼38 mA beam current in the linac at 60 Hz with a pulse length of up to ∼1.0 ms. In this work, two important issues associated with the low-energy beam transport are discussed: (1) inconsistent dependence of the post-radio frequency quadrupole accelerator beam current on the ion source tilt angle and (2) high power beam losses on the LEBT electrodes under some off-nominal conditions compromising their reliability.

Interpretation of various radiation backgrounds observed in the gamma-ray spectrometer experiments carried on the Apollo missions and implications for diffuse gamma-ray measurements

NASA Technical Reports Server (NTRS)

Dyer, C. S.; Trombka, J. I.; Metzger, A. E.; Seltzer, S. M.; Bielefeld, M. J.; Evans, L. G.

1975-01-01

Since the report of a preliminary analysis of cosmic gamma-ray measurements made during the Apollo 15 mission, an improved calculation of the spallation activation contribution has been made including the effects of short-lived spallation fragments, which can extend the correction to 15 MeV. In addition, a difference between Apollo 15 and 16 data enables an electron bremsstrahlung contribution to be calculated. A high level of activation observed in a crystal returned on Apollo 17 indicates a background contribution from secondary neutrons. These calculations and observations enable an improved extraction of spurious components and suggest important improvements for future detectors.

Overview of ten-year operation of the superconducting linear accelerator at the Spallation Neutron Source

DOE PAGES

Kim, Sang-Ho; Afanador, Ralph; Barnhart, Debra L.; ...

2017-02-04

The Spallation Neutron Source (SNS) has acquired extensive operational experience of a pulsed proton superconducting linear accelerator (SCL) as a user facility. Numerous lessons have been learned in its first 10 years operation to achieve a stable and reliable operation of the SCL. In this paper, an overview of the SNS SCL design, qualification of superconducting radio frequency (SRF) cavities and ancillary subsystems, an overview of the SNS cryogenic system, the SCL operation including SCL output energy history and downtime statistics, performance stability of the SRF cavities, efforts for SRF cavity performance recovery and improvement at the SNS, and maintenancemore » activities for cryomodules are introduced.« less

Overview of ten-year operation of the superconducting linear accelerator at the Spallation Neutron Source

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kim, Sang-Ho; Afanador, Ralph; Barnhart, Debra L.

The Spallation Neutron Source (SNS) has acquired extensive operational experience of a pulsed proton superconducting linear accelerator (SCL) as a user facility. Numerous lessons have been learned in its first 10 years operation to achieve a stable and reliable operation of the SCL. In this paper, an overview of the SNS SCL design, qualification of superconducting radio frequency (SRF) cavities and ancillary subsystems, an overview of the SNS cryogenic system, the SCL operation including SCL output energy history and downtime statistics, performance stability of the SRF cavities, efforts for SRF cavity performance recovery and improvement at the SNS, and maintenancemore » activities for cryomodules are introduced.« less

Study on induced radioactivity of China Spallation Neutron Source

NASA Astrophysics Data System (ADS)

Wu, Qing-Biao; Wang, Qing-Bin; Wu, Jing-Min; Ma, Zhong-Jian

2011-06-01

China Spallation Neutron Source (CSNS) is the first High Energy Intense Proton Accelerator planned to be constructed in China during the State Eleventh Five-Year Plan period, whose induced radioactivity is very important for occupational disease hazard assessment and environmental impact assessment. Adopting the FLUKA code, the authors have constructed a cylinder-tunnel geometric model and a line-source sampling physical model, deduced proper formulas to calculate air activation, and analyzed various issues with regard to the activation of different tunnel parts. The results show that the environmental impact resulting from induced activation is negligible, whereas the residual radiation in the tunnels has a great influence on maintenance personnel, so strict measures should be adopted.

Preliminary Numerical and Experimental Analysis of the Spallation Phenomenon

NASA Technical Reports Server (NTRS)

Martin, Alexandre; Bailey, Sean C. C.; Panerai, Francesco; Davuluri, Raghava S. C.; Vazsonyi, Alexander R.; Zhang, Huaibao; Lippay, Zachary S.; Mansour, Nagi N.; Inman, Jennifer A.; Bathel, Brett F.;

Evaluation of the 3-GeV proton beam profile at the spallation target of the JSNS

NASA Astrophysics Data System (ADS)

Meigo, Shin-ichiro; Noda, Fumiaki; Ishikura, Syuichi; Futakawa, Masatoshi; Sakamoto, Shinichi; Ikeda, Yujiro

2006-06-01

At JSNS, 3-GeV protons beam is delivered from rapid cycling synchrotron (RCS) to the spallation neutron target. In order to reduce the damage of pitting on the target container, the peak current density should be kept as small as possible. In this study, the beam profile at spallation neutron target is evaluated. The phase-space distribution, including the space-charge effect, is calculated with SIMPSONS code. The beam profile on the target is obtained with the transfer matrix from exit of RCS to the target. As for injection to RCS, two methods of correlated and anti-correlated painting are considered. By using anti-correlated painting for injection of beam at RCS, it is found the shape of beam becomes flatter than the distribution by using correlated painting. As other aspect for the study of target, in order to carry out target performance test especially for the study of pitting issue, it is better to have the beam profile variety from the beginning of facility. The adjustable range for the beam profile at the beginning is also studied. Although the beam shape is narrow and the duty is very low, the strong enough peak density is achievable equivalent as 1 MW.

Spallation studies on shock loaded uranium

DOE Office of Scientific and Technical Information (OSTI.GOV)

Tonks, D.L.; Hixson, R.; Gustavsen, R.L.

1997-12-31

Uranium samples at two different purity levels were used for spall strength measurements at three different stress levels. A 50 mm single-stage gas-gun was used to produce planar impact conditions using Z-cut quartz impactors. Samples of depleted uranium were taken from very high purity material and from material that had 300 ppm of carbon added. A pair of shots was done for each impact strength, one member of the pair with VISAR diagnostics and the second with soft recovery for metallographical examination. A series of increasing final stress states were chosen to effectively freeze the microstructural damage at three placesmore » in the development to full spall separation. This allowed determination of the dependence of spall mechanisms on stress level and sample purity. This report will discuss both the results of the metallurgical examination of soft recovered samples and the modeling of the free surface VISAR data. The micrographs taken from the recovered samples show brittle cracking as the spallation failure mechanism. Deformation induced twins are plentiful and obviously play a role in the spallation process. The twins are produced in the initial shock loading and, so, are present already before the fracture process begins. The 1 d characteristics code CHARADE has been used to model the free surface VISAR data.« less

Universal Responses of Cyclic-Oxidation Models Studied

NASA Technical Reports Server (NTRS)

Smialek, James L.

2003-01-01

Oxidation is an important degradation process for materials operating in the high-temperature air or oxygen environments typical of jet turbine or rocket engines. Reaction of the combustion gases with the component material forms surface layer scales during these oxidative exposures. Typically, the instantaneous rate of reaction is inversely proportional to the existing scale thickness, giving rise to parabolic kinetics. However, more realistic applications entail periodic startup and shutdown. Some scale spallation may occur upon cooling, resulting in loss of the protective diffusion barrier provided by a fully intact scale. Upon reheating, the component will experience accelerated oxidation due to this spallation. Cyclic-oxidation testing has, therefore, been a mainstay of characterization and performance ranking for high-temperature materials. Models simulate this process by calculating how a scale spalls upon cooling and regrows upon heating (refs. 1 to 3). Recently released NASA software (COSP for Windows) allows researchers to specify a uniform layer or discrete segments of spallation (ref. 4). Families of model curves exhibit consistent regularity and trends with input parameters, and characteristic features have been empirically described in terms of these parameters. Although much insight has been gained from experimental and model curves, no equation has been derived that can describe this behavior explicitly as functions of the key oxidation parameters.

Study of neutron shielding collimators for curved beamlines at the European Spallation Source

NASA Astrophysics Data System (ADS)

Santoro, V.; DiJulio, D. D.; Ansell, S.; Cherkashyna, N.; Muhrer, G.; Bentley, P. M.

2018-06-01

The European Spallation Source is being constructed in Lund, Sweden and is planned to be the world’s brightest pulsed spallation neutron source for cold and thermal neutron beams (≤ 1 eV). The facility uses a 2 GeV proton beam to produce neutrons from a tungsten target. The neutrons are then moderated in a moderator assembly consisting of both liquid hydrogen and water compartments. Surrounding the moderator are 22 beamports, which view the moderator’s outside surfaces. The beamports are connected to long neutron guides that transport the moderated neutrons to the sample position via reflections. As well as the desired moderated neutrons, fast neutrons coming directly from the target can find their way down the beamlines. These can create unwanted sources of background for the instruments. To mitigate such a kind of background, several instruments will use curved guides to lose direct line-of-sight (LoS) to the moderator and the target. In addition instruments can also use shielding collimators to reduce the amount of fast neutrons further traveling down the guide due to albedo reflections or streaming. Several different materials have been proposed for this purpose. We present the results of a study of different options for collimators and identify the optimal choices that balance cost, background and activation levels.

Coupled Ablation, Heat Conduction, Pyrolysis, Shape Change and Spallation of the Galileo Probe

NASA Technical Reports Server (NTRS)

Milos, Frank S.; Chen, Y.-K.; Rasky, Daniel J. (Technical Monitor)

1995-01-01

The Galileo probe enters the atmosphere of Jupiter in December 1995. This paper presents numerical methodology and detailed results of our final pre-impact calculations for the heat shield response. The calculations are performed using a highly modified version of a viscous shock layer code with massive radiation coupled with a surface thermochemical ablation and spallation model and with the transient in-depth thermal response of the charring and ablating heat shield. The flowfield is quasi-steady along the trajectory, but the heat shield thermal response is dynamic. Each surface node of the VSL grid is coupled with a one-dimensional thermal response calculation. The thermal solver includes heat conduction, pyrolysis, and grid movement owing to surface recession. Initial conditions for the heat shield temperature and density were obtained from the high altitude rarefied-flow calculations of Haas and Milos. Galileo probe surface temperature, shape, mass flux, and element flux are all determined as functions of time along the trajectory with spallation varied parametrically. The calculations also estimate the in-depth density and temperature profiles for the heat shield. All this information is required to determine the time-dependent vehicle mass and drag coefficient which are necessary inputs for the atmospheric reconstruction experiment on board the probe.

SINQ layout, operation, applications and R&D to high power

NASA Astrophysics Data System (ADS)

Bauer, G. S.; Dai, Y.; Wagner, W.

2002-09-01

Since 1997, the Paul Scherrer Institut (PSI) is operating a 1 MW class research spallation neutron source, named SINQ. SINQ is driven by a cascade of three accelerators, the final stage being a 590 MeV isochronous ring cyclotron which delivers a beam current of 1.8 mA at an rf-frequency of 51 MHz. Since for neutron production this is essentially a dc-device, SINQ is a continuous neutron source and is optimized in its design for high time average neutron flux. This makes the facility similar to a research reactor in terms of utilization, but, in terms of beam power, it is, by a large margin, the most powerful spallation neutron source currently in operation world wide. As a consequence, target load levels prevail in SINQ which are beyond the realm of existing experience, demanding a careful approach to the design and operation of a high power target. While the best neutronic performance of the source is expected for a liquid lead-bismuth eutectic target, no experience with such systems exists. For this reason a staged approach has been embarked upon, starting with a heavy water cooled rod target of Zircaloy-2 and proceeding via steel clad lead rods towards the final goal of a target optimised in both, neutronic performance and service life time. Experience currently accruing with a test target containing sample rods with different materials specimens will help to select the proper structural material and make dependable life time estimates accounting for the real operating conditions that prevail in the facility. In parallel, both theoretical and experimental work is going on within the MEGAPIE (MEGAwatt Pilot Experiment) project, a joint initiative by six European research institutions and JAERI (Japan), DOE (USA) and KAERI (Korea), to design, build, operate and explore a liquid lead-bismuth spallation target for 1MW of beam power, taking advantage of the existing spallation neutron facility SINQ.

Self-healing effect of spallation damageability

NASA Astrophysics Data System (ADS)

Buravova, S. N.

2017-10-01

The self-healing effect has been found in a study of the microstructure of the bands of localized deformation. It has been shown that interstitial elements (O, C) and the particles of a doping phase migrate to the zone of growing spallation damageability from the matrix material. When considering the wave pattern of the process of localization, it has been ascertained that the formation of bands of localized deformation is accompanied by the process of reverberation which is characterized by the formation of periodically repeated compression-extension cycles. A weak attenuation of the reverberation has led to an increase in the duration of the deformation pulse of the sample by two to three orders of magnitude compared with the time of the initial compression pulse.

Detection of spallation neutrons and protons using the (nat)Cd activation technique in transmutation experiments at Dubna.

PubMed

Manolopoulou, M; Stoulos, S; Fragopoulou, M; Brandt, R; Westmeier, W; Krivopustov, M; Sosnin, A; Zamani, M

2006-07-01

Various spallation sources have been used to transmute long-lived radioactive waste, mostly making use of the wide energy neutron fluence. In addition to neutrons, a large number of protons and gamma rays are also emitted from these sources. In this paper (nat)Cd is proved to be a useful activation detector for determining both thermal-epithermal neutron as well as secondary proton fluences. The fluences measured with (nat)Cd compared with other experimental data and calculations of DCM-DEM code were found to be in reasonable agreement. An accumulation of thermal-epithermal neutrons around the center of the target (i.e. after approx. 10 cm) and of secondary protons towards the end of the target is observed.

Transmutation of 129I and 237Np using spallation neutrons produced by 1.5, 3.7 and 7.4 GeV protons

NASA Astrophysics Data System (ADS)

Wan, J.-S.; Schmidt, Th.; Langrock, E.-J.; Vater, P.; Brandt, R.; Adam, J.; Bradnova, V.; Bamblevski, V. P.; Gelovani, L.; Gridnev, T. D.; Kalinnikov, V. G.; Krivopustov, M. I.; Kulakov, B. A.; Sosnin, A. N.; Perelygin, V. P.; Pronskikh, V. S.; Stegailov, V. I.; Tsoupko-Sitnikov, V. M.; Modolo, G.; Odoj, R.; Phlippen, P.-W.; Zamani-Valassiadou, M.; Adloff, J. C.; Debeauvais, M.; Hashemi-Nezhad, S. R.; Guo, S.-L.; Li, L.; Wang, Y.-L.; Dwivedi, K. K.; Zhuk, I. V.; Boulyga, S. F.; Lomonossova, E. M.; Kievitskaja, A. F.; Rakhno, I. L.; Chigrinov, S. E.; Wilson, W. B.

2001-05-01

Small samples of 129I and 237Np, two long-lived radwaste nuclides, were exposed to spallation neutron fluences from relatively small metal targets of lead and uranium, that were surrounded with a 6 cm thick paraffin moderator, and irradiated with 1.5, 3.7 and 7.4 GeV protons. The (n,γ) transmutation rates were determined for these nuclides. Conventional radiochemical La- and U-sensors and a variety of solid-state nuclear track detectors were irradiated simultaneously with secondary neutrons. Compared with results from calculations with well-known cascade codes (LAHET from Los Alamos and DCM/CEM from Dubna), the observed secondary neutron fluences are larger.

Generic guide concepts for the European Spallation Source

NASA Astrophysics Data System (ADS)

Zendler, C.; Martin Rodriguez, D.; Bentley, P. M.

2015-12-01

The construction of the European Spallation Source (ESS) faces many challenges from the neutron beam transport point of view: the spallation source is specified as being driven by a 5 MW beam of protons, each with 2 GeV energy, and yet the requirements in instrument background suppression relative to measured signal vary between 10-6 and 10-8. The energetic particles, particularly above 20 MeV, which are expected to be produced in abundance in the target, have to be filtered in order to make the beamlines safe, operational and provide good quality measurements with low background. We present generic neutron guides of short and medium length instruments which are optimised for good performance at minimal cost. Direct line of sight to the source is avoided twice, with either the first point out of line of sight or both being inside the bunker (20 m) to minimise shielding costs. These guide geometries are regarded as a baseline to define standards for instruments to be constructed at ESS. They are used to find commonalities and develop principles and solutions for common problems. Lastly, we report the impact of employing the over-illumination concept to mitigate losses from random misalignment passively, and that over-illumination should be used sparingly in key locations to be effective. For more widespread alignment issues, a more direct, active approach is likely to be needed.

Validation of PHITS Spallation Models from the Perspective of the Shielding Design of Transmutation Experimental Facility

NASA Astrophysics Data System (ADS)

Iwamoto, Hiroki; Meigo, Shin-ichiro

2017-09-01

The impact of different spallation models implemented in the particle transport code PHITS on the shielding design of Transmutation Experimental Facility is investigated. For 400-MeV proton incident on a lead-bismuth eutectic target, an effective dose rate at the end of a thick radiation shield (3-m-thick iron and 3-m-thick concrete) calculated by the Liège intranuclear cascade (INC) model version 4.6 (INCL4.6) coupled with the GEMcode (INCL4.6/GEM) yields about twice as high as the Bertini INC model (Bertini/GEM). A comparison with experimental data for 500-MeV proton incident on a thick lead target suggest that the prediction accuracy of INCL4.6/GEM would be better than that of Bertini/GEM. In contrast, it is found that the dose rates in beam ducts in front of targets calculated by the INCL4.6/GEMare lower than those by the Bertini/GEM. Since both models underestimate the experimental results for neutron-production doubledifferential cross sections at 180° for 140-MeV proton incident on carbon, iron, and gold targets, it is concluded that it is necessary to allow a margin for uncertainty caused by the spallation models, which is a factor of two, in estimating the dose rate induced by neutron streaming through a beam duct.

In situ measurement of atmospheric krypton and xenon on Mars with Mars Science Laboratory

DOE PAGES

Conrad, P. G.; Malespin, C. A.; Franz, H. B.; ...

2016-11-01

Mars Science Laboratory's Sample Analysis at Mars (SAM) investigation has measured all of the stable isotopes of the heavy noble gases krypton and xenon in the martian atmosphere, in situ, from the Curiosity Rover at Gale Crater, Mars. Previous knowledge of martian atmospheric krypton and xenon isotope ratios has been based upon a combination of the Viking mission's krypton and xenon detections and measurements of noble gas isotope ratios in martian meteorites. But, the meteorite measurements reveal an impure mixture of atmospheric, mantle, and spallation contributions. The xenon and krypton isotopic measurements reported here include the complete set of stablemore » isotopes, unmeasured by Viking. Our new results generally agree with Mars meteorite measurements but also provide a unique opportunity to identify various non-atmospheric heavy noble gas components in the meteorites. Kr isotopic measurements define a solar-like atmospheric composition, but deviating from the solar wind pattern at 80Kr and 82Kr in a manner consistent with contributions originating from neutron capture in Br. The Xe measurements suggest an intriguing possibility that isotopes lighter than 132Xe have been enriched to varying degrees by spallation and neutron capture products degassed to the atmosphere from the regolith, and a model is constructed to explore this possibility. Such a spallation component, but, is not apparent in atmospheric Xe trapped in the glassy phases of martian meteorites.« less

In situ measurement of atmospheric krypton and xenon on Mars with Mars Science Laboratory

NASA Astrophysics Data System (ADS)

Conrad, P. G.; Malespin, C. A.; Franz, H. B.; Pepin, R. O.; Trainer, M. G.; Schwenzer, S. P.; Atreya, S. K.; Freissinet, C.; Jones, J. H.; Manning, H.; Owen, T.; Pavlov, A. A.; Wiens, R. C.; Wong, M. H.; Mahaffy, P. R.

2016-11-01

Mars Science Laboratory's Sample Analysis at Mars (SAM) investigation has measured all of the stable isotopes of the heavy noble gases krypton and xenon in the martian atmosphere, in situ, from the Curiosity Rover at Gale Crater, Mars. Previous knowledge of martian atmospheric krypton and xenon isotope ratios has been based upon a combination of the Viking mission's krypton and xenon detections and measurements of noble gas isotope ratios in martian meteorites. However, the meteorite measurements reveal an impure mixture of atmospheric, mantle, and spallation contributions. The xenon and krypton isotopic measurements reported here include the complete set of stable isotopes, unmeasured by Viking. The new results generally agree with Mars meteorite measurements but also provide a unique opportunity to identify various non-atmospheric heavy noble gas components in the meteorites. Kr isotopic measurements define a solar-like atmospheric composition, but deviating from the solar wind pattern at 80Kr and 82Kr in a manner consistent with contributions originating from neutron capture in Br. The Xe measurements suggest an intriguing possibility that isotopes lighter than 132Xe have been enriched to varying degrees by spallation and neutron capture products degassed to the atmosphere from the regolith, and a model is constructed to explore this possibility. Such a spallation component, however, is not apparent in atmospheric Xe trapped in the glassy phases of martian meteorites.

Overview of the Conceptual Design of the Future VENUS Neutron Imaging Beam Line at the Spallation Neutron Source

NASA Astrophysics Data System (ADS)

Bilheux, Hassina; Herwig, Ken; Keener, Scott; Davis, Larry

VENUS (Versatile Neutron Imaging Beam line at the Spallation Neutron Source) will be a world-class neutron-imaging instrument that will uniquely utilize the Spallation Neutron Source (SNS) time-of-flight (TOF) capabilities to measure and characterize objects across several length scales (mm to μm). When completed, VENUS will provide academia, industry and government laboratories with the opportunity to advance scientific research in areas such as energy, materials, additive manufacturing, geosciences, transportation, engineering, plant physiology, biology, etc. It is anticipated that a good portion of the VENUS user community will have a strong engineering/industrial research focus. Installed at Beam line 10 (BL10), VENUS will be a 25-m neutron imaging facility with the capability to fully illuminate (i.e., umbra illumination) a 20 cm x 20 cm detector area. The design allows for a 28 cm x 28 cm field of view when using the penumbra to 80% of the full illumination flux. A sample position at 20 m will be implemented for magnification measurements. The optical components are comprised of a series of selected apertures, T0 and bandwidth choppers, beam scrapers, a fast shutter to limit sample activation, and flight tubes filled with Helium. Techniques such as energy selective, Bragg edge and epithermal imaging will be available at VENUS.

In Situ Measurement of Atmospheric Krypton and Xenon on Mars with Mars Science Laboratory

NASA Technical Reports Server (NTRS)

Conrad, P. G.; Malespin, C. A.; Franz, H. B.; Pepin, R. O.; Trainer, M. G.; Schwenzer, S. P.; Atreya, S. K.; Freissinet, C.; Jones, J. H.; Manning, H.;

In situ measurement of atmospheric krypton and xenon on Mars with Mars Science Laboratory

DOE Office of Scientific and Technical Information (OSTI.GOV)

Conrad, P. G.; Malespin, C. A.; Franz, H. B.

Mars Science Laboratory's Sample Analysis at Mars (SAM) investigation has measured all of the stable isotopes of the heavy noble gases krypton and xenon in the martian atmosphere, in situ, from the Curiosity Rover at Gale Crater, Mars. Previous knowledge of martian atmospheric krypton and xenon isotope ratios has been based upon a combination of the Viking mission's krypton and xenon detections and measurements of noble gas isotope ratios in martian meteorites. But, the meteorite measurements reveal an impure mixture of atmospheric, mantle, and spallation contributions. The xenon and krypton isotopic measurements reported here include the complete set of stablemore » isotopes, unmeasured by Viking. Our new results generally agree with Mars meteorite measurements but also provide a unique opportunity to identify various non-atmospheric heavy noble gas components in the meteorites. Kr isotopic measurements define a solar-like atmospheric composition, but deviating from the solar wind pattern at 80Kr and 82Kr in a manner consistent with contributions originating from neutron capture in Br. The Xe measurements suggest an intriguing possibility that isotopes lighter than 132Xe have been enriched to varying degrees by spallation and neutron capture products degassed to the atmosphere from the regolith, and a model is constructed to explore this possibility. Such a spallation component, but, is not apparent in atmospheric Xe trapped in the glassy phases of martian meteorites.« less

Calculation Package: Derivation of Facility-Specific Derived Air Concentration (DAC) Values in Support of Spallation Neutron Source Operations

DOE Office of Scientific and Technical Information (OSTI.GOV)

McLaughlin, David A

Derived air concentration (DAC) values for 175 radionuclides* produced at the Oak Ridge National Laboratory (ORNL) Spallation Neutron Source (SNS), but not listed in Appendix A of 10 CFR 835 (01/01/2009 version), are presented. The proposed DAC values, ranging between 1 E-07 {micro}Ci/mL and 2 E-03 {micro}Ci/mL, were calculated in accordance with the recommendations of the International Commission on Radiological Protection (ICRP), and are intended to support an exemption request seeking regulatory relief from the 10 CFR 835, Appendix A, requirement to apply restrictive DACs of 2E-13 {micro}Ci/mL and 4E-11 {micro}Ci/mL and for non-listed alpha and non-alpha-emitting radionuclides, respectively.

On the empirical determination of positron trapping coefficient at nano-scale helium bubbles in steels irradiated in spallation target

NASA Astrophysics Data System (ADS)

Krsjak, Vladimir; Kuriplach, Jan; Vieh, Christiane; Peng, Lei; Dai, Yong

2018-06-01

In the present work, the specific positron trapping rate of small helium bubbles was empirically derived from positron annihilation lifetime spectroscopy (PALS) and transmission electron microscopy (TEM) studies of Fe9Cr martensitic steels. Both techniques are well known to be sensitive to nanometer-sized helium-filled cavities induced during irradiation in a mixed proton-neutron spectrum of spallation target. Complementary TEM and PALS studies show that positrons are being trapped to these defects at a rate of 1.2 ± 0.8 × 10-14 m3s-1. This suggests that helium bubbles in ferritic/martensitic steels are attractive traps for positrons comparable to mono-vacancies and quantitative analysis of the bubbles by PALS technique is plausible.

Beam commission of the high intensity proton source developed at INFN-LNS for the European Spallation Source

NASA Astrophysics Data System (ADS)

Neri, L.; Celona, L.; Gammino, S.; Miraglia, A.; Leonardi, O.; Castro, G.; Torrisi, G.; Mascali, D.; Mazzaglia, M.; Allegra, L.; Amato, A.; Calabrese, G.; Caruso, A.; Chines, F.; Gallo, G.; Longhitano, A.; Manno, G.; Marletta, S.; Maugeri, A.; Passarello, S.; Pastore, G.; Seminara, A.; Spartà, A.; Vinciguerra, S.

2017-07-01

At the Istituto Nazionale di Fisica Nucleare - Laboratori Nazionali del Sud (INFN-LNS) the beam commissioning of the high intensity Proton Source for the European Spallation Source (PS-ESS) started in November 2016. Beam stability at high current intensity is one of the most important parameter for the first steps of the ongoing commissioning. Promising results were obtained since the first source start with a 6 mm diameter extraction hole. The increase of the extraction hole to 8 mm allowed improving PS-ESS performances and obtaining the values required by the ESS accelerator. In this work, extracted beam current characteristics together with Doppler shift and emittance measurements are presented, as well as the description of the next phases before the installation at ESS in Lund.

HYSPEC : A CRYSTAL TIME OF FLIGHT HYBRID SPECTROMETER FOR THE SPALLATION NEUTRON SOURCE.

DOE Office of Scientific and Technical Information (OSTI.GOV)

SHAPIRO,S.M.; ZALIZNYAK,I.A.

2002-12-30

This document lays out a proposal by the Instrument Development Team (IDT) composed of scientists from leading Universities and National Laboratories to design and build a conceptually new high-flux inelastic neutron spectrometer at the pulsed Spallation Neutron Source (SNS) at Oak Ridge. This instrument is intended to supply users of the SNS and scientific community, of which the IDT is an integral part, with a platform for ground-breaking investigations of the low-energy atomic-scale dynamical properties of crystalline solids. It is also planned that the proposed instrument will be equipped with a polarization analysis capability, therefore becoming the first polarized beammore » inelastic spectrometer in the SNS instrument suite, and the first successful polarized beam inelastic instrument at a pulsed spallation source worldwide. The proposed instrument is designed primarily for inelastic and elastic neutron spectroscopy of single crystals. In fact, the most informative neutron scattering studies of the dynamical properties of solids nearly always require single crystal samples, and they are almost invariably flux-limited. In addition, in measurements with polarization analysis the available flux is reduced through selection of the particular neutron polarization, which puts even more stringent limits on the feasibility of a particular experiment. To date, these investigations have mostly been carried out on crystal spectrometers at high-flux reactors, which usually employ focusing Bragg optics to concentrate the neutron beam on a typically small sample. Construction at Oak Ridge of the high-luminosity spallation neutron source, which will provide intense pulsed neutron beams with time-averaged fluxes equal to those at medium-flux reactors, opens entirely new opportunities for single crystal neutron spectroscopy. Drawing upon experience acquired during decades of studies with both crystal and time-of-flight (TOF) spectrometers, the IDT has developed a conceptual design for a focused-beam, hybrid time-of-flight instrument with a crystal monochromator for the SNS called HYSPEC (an acronym for hybrid spectrometer). The proposed instrument has a potential to collect data more than an order of magnitude faster than existing steady-source spectrometers over a wide range of energy transfer ({h_bar}{omega}) and momentum transfer (Q) space, and will transform the way that data in elastic and inelastic single-crystal spectroscopy are collected. HYSPEC is optimized to provide the highest neutron flux on sample in the thermal and epithermal neutron energy ranges at a good-to-moderate energy resolution. By providing a flux on sample several times higher than other inelastic instruments currently planned for the SNS, the proposed instrument will indeed allow unique ground-breaking measurements, and will ultimately make polarized beam studies at a pulsed spallation source a realistic possibility.« less

Characterization of Depleted-Uranium Strength and Damage Behavior

DOE Office of Scientific and Technical Information (OSTI.GOV)

Gray, III, George T.; Chen, Shuh-Rong; Bronkhorst, Curt A.

2012-12-17

The intent of this report is to document the status of our knowledge of the mechanical and damage behavior of Depleted Uranium(DU hereafter). This report briefly summaries the motivation of the experimental and modeling research conducted at Los Alamos National Laboratory(LANL) on DU since the early 1980’s and thereafter the current experimental data quantifying the strength and damage behavior of DU as a function of a number of experimental variables including processing, strain rate, temperature, stress state, and shock prestraining. The effect of shock prestraining on the structure-property response of DU is described and the effect on post-shock mechanical behaviormore » of DU is discussed. The constitutive experimental data utilized to support the derivation of two constitutive strength (plasticity) models, the Preston-Tonks-Wallace (PTW) and Mechanical Threshold Stress (MTS) models, for both annealed and shock prestrained DU are detailed and the Taylor cylinder validation tests and finite-element modeling (FEM) utilized to validate these strength models is discussed. The similarities and differences in the PTW and MTS model descriptions for DU are discussed for both the annealed and shock prestrained conditions. Quasi-static tensile data as a function of triaxial constraint and spallation test data are described. An appendix additionally briefly describes low-pressure equation-of-state data for DU utilized to support the spallation experiments. The constitutive behavior of DU screw/bolt material is presented. The response of DU subjected to dynamic tensile extrusion testing as a function of temperature is also described. This integrated experimental technique is planned to provide an additional validation test in the future. The damage data as a function of triaxiality, tensile and spallation data, is thereafter utilized to support derivation of the Tensile Plasticity (TEPLA) damage model and simulations for comparison to the DU spallation data are presented. Finally, a discussion of future needs in the area of needed DU strength and damage research at LANL is presented to support the development of physically-based predictive strength and damage modeling capability.« less

Gadolinium-148 and other spallation production cross section measurements for accelerator target facilities

NASA Astrophysics Data System (ADS)

Kelley, Karen Corzine

At the Los Alamos Neutron Science Center accelerator complex, protons are accelerated to 800 MeV and directed to two tungsten targets, Target 4 at the Weapons Neutron Research facility and the 1L target at the Lujan Center. The Department of Energy requires hazard classification analyses to be performed on these targets and places limits on certain radionuclide inventories in the targets to avoid characterizing the facilities as "nuclear facilities." Gadolinium-148 is a radionuclide created from the spallation of tungsten. Allowed isotopic inventories are particularly low for this isotope because it is an alpha-particle emitter with a 75-year half-life. The activity level of Gadolinium-148 is low, but it encompasses almost two-thirds of the total dose burden for the two tungsten targets based on present yield estimates. From a hazard classification standpoint, this severely limits the lifetime of these tungsten targets. The cross section is not well-established experimentally and this is the motivation for measuring the Gadolinium-148 production cross section from tungsten. In a series of experiments at the Weapons Neutron Research facility, Gadolinium-148 production was measured for 600- and 800-MeV protons on tungsten, tantalum, and gold. These experiments used 3 mum thin tungsten, tantalum, and gold foils and 10 mum thin aluminum activation foils. In addition, spallation yields were determined for many short-lived and long-lived spallation products with these foils using gamma and alpha spectroscopy and compared with predictions of the Los Alamos National Laboratory codes CEM2k+GEM2 and MCNPX. The cumulative Gadolinium-148 production cross section measured from tantalum, tungsten, and gold for incident 600-MeV protons were 15.2 +/- 4.0, 8.31 +/- 0.92, and 0.591 +/- 0.155, respectively. The average production cross sections measured at 800 MeV were 28.6 +/- 3.5, 19.4 +/- 1.8, and 3.69 +/- 0.50 for tantalum, tungsten, and gold, respectively. These cumulative measurements compared best with Bertini and were within a factor of two to three of CEM2k+GEM2.

Student Tutorials II

NASA Astrophysics Data System (ADS)

Student Tutorials

2006-05-01

(Open to all conferees) Lunch followed by a tour of the Spallation Neutron Source and Center for Nanophase Materials at of Oak Ridge National Laboratory. Buses leave from the University of Tenessee-Knoxville Nielsen Physics Building.

Design of the low energy beam transport line for the China spallation neutron source

NASA Astrophysics Data System (ADS)

Li, Jin-Hai; Ouyang, Hua-Fu; Fu, Shi-Nian; Zhang, Hua-Shun; He, Wei

2008-03-01

The design of the China Spallation Neutron Source (CSNS) low-energy beam transport (LEBT) line, which locates between the ion source and the radio-frequency quadrupole (RFQ), has been completed with the TRACE3D code. The design aims at perfect matching, primary chopping, a small emittance growth and sufficient space for beam diagnostics. The line consists of three solenoids, three vacuum chambers, two steering magnets and a pre-chopper. The total length of LEBT is about 1.74 m. This LEBT is designed to transfer 20 mA of H-pulsed beam from the ion source to the RFQ. An induction cavity is adopted as the pre-chopper. The electrostatic octupole steerer is discussed as a candidate. A four-quadrant aperture for beam scraping and beam position monitoring is designed.

Cross section measurement of residues produced in proton- and deuteron-induced spallation reactions on 93Zr at 105 MeV/u using the inverse kinematics method

NASA Astrophysics Data System (ADS)

Kawase, Shoichiro; Watanabe, Yukinobu; Wang, He; Otsu, Hideaki; Sakurai, Hiroyoshi; Takeuchi, Satoshi; Togano, Yasuhiro; Nakamura, Takashi; Maeda, Yukie; Ahn, Deuk Soon; Aikawa, Masayuki; Araki, Shouhei; Chen, Sidong; Chiga, Nobuyuki; Doornenbal, Pieter; Fukuda, Naoki; Ichihara, Takashi; Isobe, Tadaaki; Kawakami, Shunsuke; Kin, Tadahiro; Kondo, Yosuke; Koyama, Shunpei; Kubo, Toshiyuki; Kubono, Shigeru; Kurokawa, Meiko; Makinaga, Ayano; Matsushita, Masafumi; Matsuzaki, Teiichiro; Michimasa, Shin'ichiro; Momiyama, Satoru; Nagamine, Shunsuke; Nakano, Keita; Niikura, Megumi; Ozaki, Tomoyuki; Saito, Atsumi; Saito, Takeshi; Shiga, Yoshiaki; Shikata, Mizuki; Shimizu, Yohei; Shimoura, Susumu; Sumikama, Toshiyuki; Söderström, Pär-Anders; Suzuki, Hiroshi; Takeda, Hiroyuki; Taniuchi, Ryo; Tsubota, Jun'ichi; Watanabe, Yasushi; Wimmer, Kathrin; Yamamoto, Tatsuya; Yoshida, Koichi

2017-09-01

Isotopic production cross sections in the proton- and deuteron-induced spallation reactions on 93Zr at an energy of 105 MeV/u were measured in inverse kinematics conditions for the development of realistic nuclear transmutation processes for long-lived fission products (LLFPs) with neutron and light-ion beams. The experimental results were compared to the PHITS calculations describing the intra-nuclear cascade and evaporation processes. Although an overall agreement was obtained, a large overestimation of the production cross sections for the removal of a few nucleons was seen. A clear shell effect associated with the neutron magic number N = 50 was observed in the measured isotopic production yields of Zr and Y isotopes, which can be reproduced reasonably by the PHITS calculation.

Spallation as a dominant source of pusher-fuel and hot-spot mix in inertial confinement fusion capsules

DOE PAGES

Orth, Charles D.

2016-02-23

We suggest that a potentially dominant but previously neglected source of pusher-fuel and hot-spot “mix” may have been the main degradation mechanism for fusion energy yields of modern inertial confinement fusion (ICF) capsules designed and fielded to achieve high yields — not hydrodynamic instabilities. This potentially dominant mix source is the spallation of small chunks or “grains” of pusher material into the fuel regions whenever (1) the solid material adjacent to the fuel changes its phase by nucleation, and (2) this solid material spalls under shock loading and sudden decompression. Finally, we describe this mix mechanism, support it with simulationsmore » and experimental evidence, and explain how to eliminate it and thereby allow higher yields for ICF capsules and possibly ignition at the National Ignition Facility.« less

VSI@ESS: Case study for a vibrational spectroscopy instrument at the european spallation source

NASA Astrophysics Data System (ADS)

Zoppi, Marco; Fedrigo, Anna; Celli, Milva; Colognesi, Daniele

2015-01-01

Neutron Vibrational Spectroscopy is a well-established experimental technique where elementary excitations at relatively high frequency are detected via inelastic neutron scattering. This technique attracts a high interest in a large fraction of the scientific community in the fields of chemistry, materials science, physics, and biology, since one of its main applications exploits the large incoherent scattering cross section of the proton with respect to all the other elements, whose dynamics can be spectroscopically detected, even if dissolved in very low concentration in materials composed of much heavier atoms. We have proposed a feasibility study for a Vibrational Spectroscopy Instrument (VSI) at the European Spallation Source ESS. Here, we will summarize the preliminary design calculations and the corresponding McStas simulation results for a possible ToF, Inverted Geometry, VSI beamline.

Determination of the ¹⁴C content in activated steel components from a neutron spallation source and a nuclear power plant.

PubMed

Schumann, Dorothea; Stowasser, Tanja; Volmert, Benjamin; Günther-Leopold, Ines; Linder, Hanspeter; Wieland, Erich

2014-06-03

The (14)C content in activated steel components from the Swiss Nuclear Power Plant (NPP) Gösgen and the Spallation Neutron Source SINQ at the Paul Scherrer Institute is determined using a wet chemistry digestion technique and liquid scintillation counting for (14)C activity measurements. The (14)C activity of an activated fuel assembly steel nut from the NPP is further compared with theoretical predictions made on the basis of a Monte Carlo reactor model for this NPP. Knowledge of the (14)C inventory in these activated steel materials is important in conjunction with future corrosion studies on these materials aimed at identifying the (14)C containing organic compounds possibly formed in the cement-based near field of a repository for radioactive waste.

Radiological Hazard of Spallation Products in Accelerator-Driven System

DOE Office of Scientific and Technical Information (OSTI.GOV)

Saito, M.; Stankovskii, A.; Artisyuk, V.

The central issue underlying this paper is related to elucidating the hazard of radioactive spallation products that might be an important factor affecting the design option of accelerator-driven systems (ADSs). Hazard analysis based on the concept of Annual Limit on Intake identifies alpha-emitting isotopes of rare earths (REs) (dysprosium, gadolinium, and samarium) as the dominant contributors to the overall toxicity of traditional (W, Pb, Pb-Bi) targets. The matter is addressed from several points of view: code validation to simulate their yields, choice of material for the neutron producing targets, and challenging the beam type. The paper quantitatively determines the domainmore » in which the toxicity of REs exceeds that of polonium activation products broadly discussed now in connection with advertising lead-bismuth technology for the needs of ADSs.« less

Thermal-barrier-coated turbine blade study

NASA Technical Reports Server (NTRS)

Siemers, P. A.; Hillig, W. B.

1981-01-01

The effects of coating TBC on a CF6-50 stage 2 high-pressure turbine blade were analyzed with respect to changes in the mean bulk temperature, cooling air requirements, and high-cycle fatigue. Localized spallation was found to have a possible deleterious effect on low-cycle fatigue life. New blade design concepts were developed to take optimum advantage of TBCs. Process and material development work and rig evaluations were undertaken which identified the most promising combination as ZrO2 containing 8 w/o Y2O3 applied by air plasma spray onto a Ni22Cr-10Al-1Y bond layer. The bond layer was applied by a low-pressure, high-velocity plasma spray process onto the base alloy. During the initial startup cycles the blades experienced localized leading edge spallation caused by foreign objects.

New developments in the McStas neutron instrument simulation package

NASA Astrophysics Data System (ADS)

Willendrup, P. K.; Knudsen, E. B.; Klinkby, E.; Nielsen, T.; Farhi, E.; Filges, U.; Lefmann, K.

2014-07-01

The McStas neutron ray-tracing software package is a versatile tool for building accurate simulators of neutron scattering instruments at reactors, short- and long-pulsed spallation sources such as the European Spallation Source. McStas is extensively used for design and optimization of instruments, virtual experiments, data analysis and user training. McStas was founded as a scientific, open-source collaborative code in 1997. This contribution presents the project at its current state and gives an overview of the main new developments in McStas 2.0 (December 2012) and McStas 2.1 (expected fall 2013), including many new components, component parameter uniformisation, partial loss of backward compatibility, updated source brilliance descriptions, developments toward new tools and user interfaces, web interfaces and a new method for estimating beam losses and background from neutron optics.

Strain rate effects for spallation of concrete

NASA Astrophysics Data System (ADS)

Häussler-Combe, Ulrich; Panteki, Evmorfia; Kühn, Tino

2015-09-01

Appropriate triaxial constitutive laws are the key for a realistic simulation of high speed dynamics of concrete. The strain rate effect is still an open issue within this context. In particular the question whether it is a material property - which can be covered by rate dependent stress strain relations - or mainly an effect of inertia is still under discussion. Experimental and theoretical investigations of spallation of concrete specimen in a Hopkinson Bar setup may bring some evidence into this question. For this purpose the paper describes the VERD model, a newly developed constitutive law for concrete based on a damage approach with included strain rate effects [1]. In contrast to other approaches the dynamic strength increase is not directly coupled to strain rate values but related to physical mechanisms like the retarded movement of water in capillary systems and delayed microcracking. The constitutive law is fully triaxial and implemented into explicit finite element codes for the investigation of a wide range of concrete structures exposed to impact and explosions. The current setup models spallation experiments with concrete specimen [2]. The results of such experiments are mainly related to the dynamic tensile strength and the crack energy of concrete which may be derived from, e.g., the velocity of spalled concrete fragments. The experimental results are compared to the VERD model and two further constitutive laws implemented in LS-Dyna. The results indicate that both viscosity and retarded damage are required for a realistic description of the material behaviour of concrete exposed to high strain effects [3].

Comparison of different target material options for the European Spallation Source based on certain aspects related to the final disposal

NASA Astrophysics Data System (ADS)

Kókai, Zsófia; Török, Szabina; Zagyvai, Péter; Kiselev, Daniela; Moormann, Rainer; Börcsök, Endre; Zanini, Luca; Takibayev, Alan; Muhrer, Günter; Bevilacqua, Riccardo; Janik, József

2018-02-01

Different target options have been examined for the European Spallation Source, which is under construction in Lund, Sweden. During the design update phase, parameters and characteristics for the target design have been optimized not only for neutronics but also with respect to the waste characteristics related to the final disposal of the target. A rotating, solid tungsten target was eventually selected as baseline concept; the other options considered included mercury and lead-bismuth (LBE) targets suitable for a pulsed source. Since the licensee is obliged to present a decommissioning plan even before the construction phase starts, the radioactive waste category of the target after full operation time is of crucial importance. The results obtained from a small survey among project partners of 7th Framework Program granted by EU 202247 contract have been used. Waste characteristics of different potential spallation target materials were compared. Based on waste index, the tungsten target is the best alternative and the second one is the mercury target. However, all alternatives have HLW category after a 10 year cooling. Based on heat generation alone all of the options would be below the HLW limit after this cooling period. The LBE is the least advantageous alternative based on waste index and heat generation comparison. These results can be useful in compiling the licensing documents of the ESS facility as the target alternatives can be compared from various aspects related to their disposal.

Plume-Surface Interaction Modeling for a Human-Scale Mars Lander

NASA Technical Reports Server (NTRS)

Hart, Kenneth

2017-01-01

Landing vehicles impart thermal and strain energy onto the landing site from the retrorocket exhaust. Depending on the design of the vehicle, the energy may be great enough to cause spallation at the landing site. This damage may be minor and repairable in the case of landing on a terrestrial landing pad. For missions to other planetary bodies, the spallation may cause the landing site to become uneven and unstable, as well as damage. Simulating this phenomenon in a laboratory or computationally would require a significant amount of time and other resources. These resources typically are not available during the design phase of a mission. This paper presents a computationally-efficient model for the temperature and stress distributions that arise during landing. These quantities can be used along with existing failure criteria, such as the Hoek-Brown criterion for geological materials, to quickly determine whether spallation will occur. The stress and temperature distributions at the landing site are inherently 3D; however, there is a plane of symmetry and in that plane the distributions are 2D. Both quantities are modeled using series solutions to their governing partial differential equations (PDEs). The stress is modeled using the Airy stress potential function and its governing PDE is the biharmonic equation. The temperature is governed by Fourier's law. The models assume that stress due to gravity can be neglected, the points in the plane do not accelerate, and that the material properties are constant.

Spallation neutron production and the current intra-nuclear cascade and transport codes

NASA Astrophysics Data System (ADS)

Filges, D.; Goldenbaum, F.; Enke, M.; Galin, J.; Herbach, C.-M.; Hilscher, D.; Jahnke, U.; Letourneau, A.; Lott, B.; Neef, R.-D.; Nünighoff, K.; Paul, N.; Péghaire, A.; Pienkowski, L.; Schaal, H.; Schröder, U.; Sterzenbach, G.; Tietze, A.; Tishchenko, V.; Toke, J.; Wohlmuther, M.

A recent renascent interest in energetic proton-induced production of neutrons originates largely from the inception of projects for target stations of intense spallation neutron sources, like the planned European Spallation Source (ESS), accelerator-driven nuclear reactors, nuclear waste transmutation, and also from the application for radioactive beams. In the framework of such a neutron production, of major importance is the search for ways for the most efficient conversion of the primary beam energy into neutron production. Although the issue has been quite successfully addressed experimentally by varying the incident proton energy for various target materials and by covering a huge collection of different target geometries --providing an exhaustive matrix of benchmark data-- the ultimate challenge is to increase the predictive power of transport codes currently on the market. To scrutinize these codes, calculations of reaction cross-sections, hadronic interaction lengths, average neutron multiplicities, neutron multiplicity and energy distributions, and the development of hadronic showers are confronted with recent experimental data of the NESSI collaboration. Program packages like HERMES, LCS or MCNPX master the prevision of reaction cross-sections, hadronic interaction lengths, averaged neutron multiplicities and neutron multiplicity distributions in thick and thin targets for a wide spectrum of incident proton energies, geometrical shapes and materials of the target generally within less than 10% deviation, while production cross-section measurements for light charged particles on thin targets point out that appreciable distinctions exist within these models.

Deformation and Spallation of Explosive Welded Steels under Gas Gun Shock Loading

NASA Astrophysics Data System (ADS)

Yu, Ying; Li, Chao; Ma, Hong-Hao; Qi, Mei-Lan; Luo, Sheng-Nian

2018-01-01

Not Available Supported by the National Basic Research Program of China under Grant No 2014CB845904, and the National Natural Science Foundation of China under Grant Nos 11627901, 11372113 and 11672110.

Enigmatic Moisture Effects on Al2O3 Scale and TBC Adhesion

NASA Technical Reports Server (NTRS)

Smialek, James L.

2008-01-01

Alumina scale adhesion to high temperature alloys is known to be affected primarily by sulfur segregation and reactive element additions. However, adherent scales can become partially compromised by excessive strain energy and cyclic cracking. With time, exposure of such scales to moisture can lead to spontaneous interfacial decohesion, occurring while the samples are maintained at ambient conditions. Examples of this Moisture-Induced Delayed Spallation (MIDS) are presented for NiCrAl and single crystal superalloys, becoming more severe with sulfur level and cyclic exposure conditions. Similarly, delayed failure or Desk Top Spallation (DTS) results are reviewed for thermal barrier coatings (TBCs), culminating in the water drop failure test. Both phenomena are discussed in terms of moisture effects on bulk alumina and bulk aluminides. A mechanism is proposed based on hydrogen embrittlement and is supported by a cathodic hydrogen charging experiment. Hydroxylation of aluminum from the alloy interface appears to be the relevant basic reaction.

Enigmatic Moisture Effects on Al2O3 Scale and TBC Adhesion

NASA Technical Reports Server (NTRS)

Smialek, James L.

2008-01-01

Alumina scale adhesion to high temperature alloys is known to be affected primarily by sulfur segregation and reactive element additions. However adherent scales can become partially compromised by excessive strain energy and cyclic cracking. With time, exposure of such scales to moisture can lead to spontaneous interfacial decohesion, occurring while the samples are maintained at ambient conditions. Examples of this Moisture-Induced Delayed Spallation (MIDS) are presented for NiCrAl and single crystal superalloys, becoming more severe with sulfur level and cyclic exposure conditions. Similarly, delayed failure or Desk Top Spallation (DTS) results are reviewed for TBC s, culminating in the water drop failure test. Both phenomena are discussed in terms of moisture effects on bulk alumina and bulk aluminides. A mechanism is proposed based on hydrogen embrittlement and is supported by a cathodic hydrogen charging experiment. Hydroxylation of aluminum from the alloy interface appears to be the relevant basic reaction.

Impedance measurements of the extraction kicker system for the rapid cycling synchrotron of China Spallation Neutron Source

NASA Astrophysics Data System (ADS)

Huang, Liang-Sheng; Wang, Sheng; Liu, Yu-Dong; Li, Yong; Liu, Ren-Hong; Xiao, Ou-Zheng

2016-04-01

The fast extraction kicker system is one of the most important accelerator components and the main source of impedance in the Rapid Cycling Synchrotron of the China Spallation Neutron Source. It is necessary to understand the kicker impedance before its installation into the tunnel. Conventional and improved wire methods are employed in the impedance measurement. The experimental results for the kicker impedance are explained by comparison with simulation using CST PARTICLE STUDIO. The simulation and measurement results confirm that the window-frame ferrite geometry and the end plate are the important structures causing coupling impedance. It is proved in the measurements that the mismatching from the power form network to the kicker leads to a serious oscillation sideband of the longitudinal and vertical impedance and the oscillation can be reduced by ferrite absorbing material. Supported by National Natural Science Foundation of China (11175193, 11275221)

Radiation damage calculations for the SINQ Target 5

NASA Astrophysics Data System (ADS)

Wechsler, Monroe S.; Lu, Wei; Dai, Yong

2003-03-01

Calculations are underway of radiation damage (production of displacements, helium, and hydrogen) at Target 5 of the SINQ spallation neutron source at the Paul Scherrer Institute in Switzerland. The target is bombarded by 575-MeV protons, and the spallation-neutron-producing target material is liquid lead. The calculations employ the Monte Carlo code MCNPX (version 2.3.0). The peak proton and neutron fluxes at the aluminum-alloy entrance window are determined to be about 1.9E14 protons/cm2s per mA of incident proton current and 2.4E13 neutrons/cm2s per mA. For a beam exposure of 10 Ahr, the peak damage sustained at the entrance window due to protons and neutrons combined is calculated to be 7.8 dpa, 2000 appmHe, and 4000 appmH. The significance of the damage results for the entrance window and components within Target 5 will be discussed.

Simulations towards optimization of a neutron/anti-neutron oscillation experiment at the European Spallation Source

NASA Astrophysics Data System (ADS)

Frost, Matthew; Kamyshkov, Yuri; Castellanos, Luis; Klinkby, Esben; US NNbar Collaboration

2015-04-01

The observation of Neutron/Anti-neutron oscillation would prove the existence of Baryon Number Violation (BNV), and thus an explanation for the dominance of matter over anti-matter in the universe. The latest experiments have shown the oscillation time to be greater than 8.6 x 107 seconds, whereas current theoretical predictions suggest times on the order of 108 to 109 seconds. A neutron oscillation experiment proposed at the European Spallation Source (ESS) would provide sensitivity of more than 1000 times previous experiments performed, thus providing a result well-suited to confirm or deny current theory. A conceptual design of the proposed experiment will be presented, as well as the optimization of key experiment components using Monte-Carlo simulation methods, including the McStas neutron ray-trace simulation package. This work is supported by the Organized Research Units Program funded by The University of Tennessee, Knoxville Office of Research and Engagement.

International workshop on cold neutron sources

DOE Office of Scientific and Technical Information (OSTI.GOV)

Russell, G.J.; West, C.D.

1991-08-01

The first meeting devoted to cold neutron sources was held at the Los Alamos National Laboratory on March 5--8, 1990. Cosponsored by Los Alamos and Oak Ridge National Laboratories, the meeting was organized as an International Workshop on Cold Neutron Sources and brought together experts in the field of cold-neutron-source design for reactors and spallation sources. Eighty-four people from seven countries attended. Because the meeting was the first of its kind in over forty years, much time was spent acquainting participants with past and planned activities at reactor and spallation facilities worldwide. As a result, the meeting had more ofmore » a conference flavor than one of a workshop. The general topics covered at the workshop included: Criteria for cold source design; neutronic predictions and performance; energy deposition and removal; engineering design, fabrication, and operation; material properties; radiation damage; instrumentation; safety; existing cold sources; and future cold sources.« less

The Fundamental Neutron Physics Beamline at the Spallation Neutron Source.

PubMed

Greene, Geoffrey; Cianciolo, Vince; Koehler, Paul; Allen, Richard; Snow, William Michael; Huffman, Paul; Gould, Chris; Bowman, David; Cooper, Martin; Doyle, John

2005-01-01

The Spallation Neutron Source (SNS), currently under construction at Oak Ridge National Laboratory with an anticipated start-up in early 2006, will provide the most intense pulsed beams of cold neutrons in the world. At a projected power of 1.4 MW, the time averaged fluxes and fluences of the SNS will approach those of high flux reactors. One of the flight paths on the cold, coupled moderator will be devoted to fundamental neutron physics. The fundamental neutron physics beamline is anticipated to include two beam-lines; a broad band cold beam, and a monochromatic beam of 0.89 nm neutrons for ultracold neutron (UCN) experiments. The fundamental neutron physics beamline will be operated as a user facility with experiment selection based on a peer reviewed proposal process. An initial program of five experiments in neutron decay, hadronic weak interaction and time reversal symmetry violation have been proposed.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Stan, Claudiu A.; Willmott, Philip R.; Stone, Howard A.

Most experimental studies of cavitation in liquid water at negative pressures reported cavitation at tensions significantly smaller than those expected for homogeneous nucleation, suggesting that achievable tensions are limited by heterogeneous cavitation. We generated tension pulses with nanosecond rise times in water by reflecting cylindrical shock waves, produced by X-ray laser pulses, at the internal surface of drops of water. Depending on the X-ray pulse energy, a range of cavitation phenomena occurred, including the rupture and detachment, or spallation, of thin liquid layers at the surface of the drop. When spallation occurred, we evaluated that negative pressures below –100 MPamore » were reached in the drops. As a result, we model the negative pressures from shock reflection experiments using a nucleation-and-growth model that explains how rapid decompression could outrun heterogeneous cavitation in water, and enable the study of stretched water close to homogeneous cavitation pressures.« less

Low-level rf control of Spallation Neutron Source: System and characterization

NASA Astrophysics Data System (ADS)

Ma, Hengjie; Champion, Mark; Crofford, Mark; Kasemir, Kay-Uwe; Piller, Maurice; Doolittle, Lawrence; Ratti, Alex

2006-03-01

The low-level rf control system currently commissioned throughout the Spallation Neutron Source (SNS) LINAC evolved from three design iterations over 1 yr intensive research and development. Its digital hardware implementation is efficient, and has succeeded in achieving a minimum latency of less than 150 ns which is the key for accomplishing an all-digital feedback control for the full bandwidth. The control bandwidth is analyzed in frequency domain and characterized by testing its transient response. The hardware implementation also includes the provision of a time-shared input channel for a superior phase differential measurement between the cavity field and the reference. A companion cosimulation system for the digital hardware was developed to ensure a reliable long-term supportability. A large effort has also been made in the operation software development for the practical issues such as the process automations, cavity filling, beam loading compensation, and the cavity mechanical resonance suppression.

γ-Ray background sources in the VESUVIO spectrometer at ISIS spallation neutron source

NASA Astrophysics Data System (ADS)

Pietropaolo, A.; Perelli Cippo, E.; Gorini, G.; Tardocchi, M.; Schooneveld, E. M.; Andreani, C.; Senesi, R.

2009-09-01

An investigation of the gamma background was carried out in the VESUVIO spectrometer at the ISIS spallation neutron source. This study, performed with a yttrium-aluminum-perovskite (YAP) scintillator, follows high resolution pulse height measurements of the gamma background carried out on the same instrument with the use of a high-purity germanium detector. In this experimental work, a mapping of the gamma background was attempted, trying to find the spatial distribution and degree of directionality of the different contributions identified in the previous study. It is found that the gamma background at low times is highly directional and mostly due to the gamma rays generated in the moderator-decoupler system. The other contributions, consistently to the findings of a previous experiment, are identified as a nearly isotropic one due to neutron absorption in the walls of the experimental hall, and a directional one coming from the beam dump.

Core Vessel Insert Handling Robot for the Spallation Neutron Source

DOE Office of Scientific and Technical Information (OSTI.GOV)

Graves, Van B; Dayton, Michael J

2011-01-01

The Spallation Neutron Source provides the world's most intense pulsed neutron beams for scientific research and industrial development. Its eighteen neutron beam lines will eventually support up to twenty-four simultaneous experiments. Each beam line consists of various optical components which guide the neutrons to a particular instrument. The optical components nearest the neutron moderators are the core vessel inserts. Located approximately 9 m below the high bay floor, these inserts are bolted to the core vessel chamber and are part of the vacuum boundary. They are in a highly radioactive environment and must periodically be replaced. During initial SNS construction,more » four of the beam lines received Core Vessel Insert plugs rather than functional inserts. Remote replacement of the first Core Vessel Insert plug was recently completed using several pieces of custom-designed tooling, including a highly complicated Core Vessel Insert Robot. The design of this tool are discussed.« less

AC magnetic field measurement using a small flip coil system for rapid cycling AC magnets at the China Spallation Neutron Source (CSNS)

NASA Astrophysics Data System (ADS)

Zhou, Jianxin; Kang, Wen; Li, Shuai; Liu, Yudong; Liu, Yiqin; Xu, Shouyan; Guo, Xiaoling; Wu, Xi; Deng, Changdong; Li, Li; Wu, Yuwen; Wang, Sheng

2018-02-01

The China Spallation Neutron Source (CSNS) has two major accelerator systems, a linear accelerator and a rapid cycling synchrotron (RCS). The RCS accelerator is used to accumulate and accelerate protons from the energy of 80 MeV to the design energy of 1.6 GeV at the repetition rate of 25 Hz, and extract the high energy beam to the target. The main magnets of the RCS accelerator are excited by AC current with DC bias. The magnetic field quality is very important for the RCS accelerator operation, since it should guarantee and focus a circulating beam. In order to characterize the AC magnets, a small flip coil measurement system has been developed and one of each type of AC magnets has been studied. The measurement system and selected measurement results are presented in this paper.

Feasibility and applications of the spin-echo modulation option for a small angle neutron scattering instrument at the European Spallation Source

NASA Astrophysics Data System (ADS)

Kusmin, A.; Bouwman, W. G.; van Well, A. A.; Pappas, C.

2017-06-01

We describe theoretical and practical aspects of spin-echo modulated small-angle neutron scattering (SEMSANS) as well as the potential combination with SANS. Based on the preliminary technical designs of SKADI (a SANS instrument proposed for the European Spallation Source) and a SEMSANS add-on, we assess the practicability, feasibility and scientific merit of a combined SANS and SEMSANS setup by calculating tentative SANS and SEMSANS results for soft matter, geology and advanced material samples that have been previously studied by scattering methods. We conclude that lengths from 1 nm up to 0.01 mm can be observed simultaneously in a single measurement. Thus, the combination of SANS and SEMSANS instrument is suited for the simultaneous observation of a wide range of length scales, e.g. for time-resolved studies of kinetic processes in complex multiscale systems.

Fast neutron irradiation tests of flash memories used in space environment at the ISIS spallation neutron source

NASA Astrophysics Data System (ADS)

Andreani, C.; Senesi, R.; Paccagnella, A.; Bagatin, M.; Gerardin, S.; Cazzaniga, C.; Frost, C. D.; Picozza, P.; Gorini, G.; Mancini, R.; Sarno, M.

2018-02-01

This paper presents a neutron accelerated study of soft errors in advanced electronic devices used in space missions, i.e. Flash memories performed at the ChipIr and VESUVIO beam lines at the ISIS spallation neutron source. The two neutron beam lines are set up to mimic the space environment spectra and allow neutron irradiation tests on Flash memories in the neutron energy range above 10 MeV and up to 800 MeV. The ISIS neutron energy spectrum is similar to the one occurring in the atmospheric as well as in space and planetary environments, with intensity enhancements varying in the range 108- 10 9 and 106- 10 7 respectively. Such conditions are suitable for the characterization of the atmospheric, space and planetary neutron radiation environments, and are directly applicable for accelerated tests of electronic components as demonstrated here in benchmark measurements performed on flash memories.

On the spectrum of stable secondary nuclei in cosmic rays

NASA Astrophysics Data System (ADS)

Blasi, P.

2017-10-01

The ratio of the fluxes of secondary and primary nuclei in cosmic rays has long been used as an indicator of the grammage traversed in the journey of cosmic ray particles throughout the Galaxy. The basic idea is that primary particles are accelerated in astrophysical sources, such as supernova remnant shocks and eventually propagate in the Galactic volume, occasionally interacting with gas, mainly in the disc of the Galaxy, and there they produce secondary nuclei through spallation. At sufficiently high energy, typically ≳100 GeV/n, the ratio of fluxes of the secondary nucleus to that of the main primary nucleus is found to scale as Ek^{-δ }, where Ek is the energy per nucleon (a conserved quantity in spallation reactions) and δ identifies the energy dependence of the diffusion coefficient. The same shock waves that may be responsible for cosmic ray acceleration in the first place also pick up any other charged particle in the upstream, provided being above threshold for injection. The secondary nuclei produced by spallation in the interstellar medium are no exception, hence they also get accelerated. This effect is unavoidable, only its strength may be subject of debate. We compute the spectrum of secondary elements such as boron and lithium taking into account shock reacceleration and compare our predictions with the recent observations of the B/C ratio and preliminary measurements of the boron and lithium flux. Both these sets of data seem to confirm that reacceleration of secondary nuclei indeed plays an important role, thereby affecting the validity of those scaling rules that are often used in cosmic ray physics.

Cavitation instability in bulk metallic glasses

NASA Astrophysics Data System (ADS)

Dai, L. H.; Huang, X.; Ling, Z.

2015-09-01

Recent experiments have shown that fracture surfaces of bulk metallic glasses (BMGs) usually exhibit an intriguing nanoscale corrugation like fractographic feature mediated by nanoscale void formation. We attribute the onset of this nanoscale corrugation to TTZs (tension transformation zones) mediated cavitation. In our recent study, the spall experiments of Zr-based BMG using a single-stage light gas gun were performed. To uncover the mechanisms of the spallation damage nucleation and evolution, the samples were designed to be subjected to dynamic tensile loadings of identical amplitude but with different durations by making use of the multi-stress pulse and the double-flyer techniques. It is clearly revealed that the macroscopic spall fracture in BMGs originates from the nucleation, growth and coalescence of micro-voids. Then, a microvoid nucleation model of BMGs based on free volume theory is proposed, which indicates that the nucleation of microvoids at the early stage of spallation in BMGs is resulted from diffusion and coalescence of free volume. Furthermore, a theoretical model of void growth in BMGs undergoing remote dynamic hydrostatic tension is developed. The critical condition of cavitation instability is obtained. It is found that dynamic void growth in BMGs can be well controlled by a dimensionless inertial number characterizing the competition between intrinsic and extrinsic time scales. To unveil the atomic-level mechanism of cavitation, a systematic molecular dynamics (MD) simulation of spallation behaviour of a binary metallic glass with different impact velocities was performed. It is found that micro-void nucleation is determined TTZs while the growth is controlled by shear transformation zones (STZs) at atomic scale.

Cosmic-Ray Nucleosynthesis of p-nuclei: Yields and Routes

NASA Astrophysics Data System (ADS)

Kusakabe, Motohiko; Mathews, Grant J.

2018-02-01

We investigate the cosmic-ray nucleosynthesis (CRN) of proton-rich stable nuclides (p-nuclides). We calculate the cosmic-ray (CR) energy spectra of heavy nuclides with mass number A=[74,209], taking into account the detailed nuclear spallation, decay, energy loss, and escape from the Galaxy during the CR propagation. We adopt the latest semiempirical formula SPACS for the spallation cross sections and the latest data on nuclear decay. Effective electron-capture decay rates are calculated using the proper cross sections for recombination and ionization in the whole CR energy region. Calculated CR spectral shapes vary for different nuclides. Abundances of proton-rich unstable nuclides increase in CRs with increasing energy relative to those of other nuclides. Yields of the primary and secondary spallation processes and differential yields from respective seed nuclides are calculated. We find that the CR energy region of ≤slant { \\mathcal O }(100) MeV/nucleon predominantly contributes to the total yields. The atomic cross sections in the low-energy range adopted in this study are then necessary. Effects of CRN on the Galactic chemical evolution of p-nuclides are calculated. Important seed nuclides are identified for respective p-nuclides. The contribution of CRN is significant for 180m Ta, accounting for about 20% of the solar abundance. About 87% of the 180m Ta CRN yield can be attributed to the primary process. The most important production routes are reactions of 181Ta, 180Hf, and 182W. CRN yields of other p-nuclides are typically about { \\mathcal O }(10‑4–10‑2) of solar abundances.

Simulation of a beam rotation system for a spallation source

NASA Astrophysics Data System (ADS)

Reiss, Tibor; Reggiani, Davide; Seidel, Mike; Talanov, Vadim; Wohlmuther, Michael

2015-04-01

With a nominal beam power of nearly 1 MW on target, the Swiss Spallation Neutron Source (SINQ), ranks among the world's most powerful spallation neutron sources. The proton beam transport to the SINQ target is carried out exclusively by means of linear magnetic elements. In the transport line to SINQ the beam is scattered in two meson production targets and as a consequence, at the SINQ target entrance the beam shape can be described by Gaussian distributions in transverse x and y directions with tails cut short by collimators. This leads to a highly nonuniform power distribution inside the SINQ target, giving rise to thermal and mechanical stresses. In view of a future proton beam intensity upgrade, the possibility of homogenizing the beam distribution by means of a fast beam rotation system is currently under investigation. Important aspects which need to be studied are the impact of a rotating proton beam on the resulting neutron spectra, spatial flux distributions and additional—previously not present—proton losses causing unwanted activation of accelerator components. Hence a new source description method was developed for the radiation transport code MCNPX. This new feature makes direct use of the results from the proton beam optics code TURTLE. Its advantage to existing MCNPX source options is that all phase space information and correlations of each primary beam particle computed with TURTLE are preserved and transferred to MCNPX. Simulations of the different beam distributions together with their consequences in terms of neutron production are presented in this publication. Additionally, a detailed description of the coupling method between TURTLE and MCNPX is provided.

Spallation reactions in shock waves at supernova explosions and related problems

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ustinova, G. K., E-mail: ustinova@dubna.net.ru

2013-05-15

The isotopic anomalies of some extinct radionuclides testify to the outburst of a nearby supernova just before the collapse of the protosolar nebula, and to the fact that the supernova was Sn Ia, i.e. the carbon-detonation supernova. A key role of spallation reactions in the formation of isotopic anomalies in the primordial matter of the Solar System is revealed. It is conditioned by the diffusive acceleration of particles in the explosive shock waves, which leads to the amplification of rigidity of the energy spectrum of particles and its enrichment with heavier ions. The quantitative calculations of such isotopic anomalies ofmore » many elements are presented. It is well-grounded that the anomalous Xe-HL in meteoritic nanodiamonds was formed simultaneously with nanodiamonds themselves during the shock wave propagation at the Sn Ia explosion. The possible effects of shock wave fractionation of noble gases in the atmosphere of planets are considered. The origin of light elements Li, Be and B in spallation reactions, predicted by Fowler in the middle of the last century, is argued. All the investigated isotopic anomalies give the evidence for the extremely high magnetohydrodynamics (MHD) conditions at the initial stage of free expansion of the explosive shock wave from Sn Ia, which can be essential in solution of the problem of origin of cosmic rays. The specific iron-enriched matter of Sn Ia and its MHD-separation in turbulent processes must be taking into account in the models of origin of the Solar System.« less

Experimental impact crater morphology

NASA Astrophysics Data System (ADS)

Dufresne, A.; Poelchau, M. H.; Hoerth, T.; Schaefer, F.; Thoma, K.; Deutsch, A.; Kenkmann, T.

2012-04-01

The research group MEMIN (Multidisciplinary Experimental and Impact Modelling Research Network) is conducting impact experiments into porous sandstones, examining, among other parameters, the influence of target pore-space saturation with water, and projectile velocity, density and mass, on the cratering process. The high-velocity (2.5-7.8 km/s) impact experiments were carried out at the two-stage light-gas gun facilities of the Fraunhofer Institute EMI (Germany) using steel, iron meteorite (Campo del Cielo IAB), and aluminium projectiles with Seeberg Sandstone as targets. The primary objectives of this study within MEMIN are to provide detailed morphometric data of the experimental craters, and to identify trends and characteristics specific to a given impact parameter. Generally, all craters, regardless of impact conditions, have an inner depression within a highly fragile, white-coloured centre, an outer spallation (i.e. tensile failure) zone, and areas of arrested spallation (i.e. spall fragments that were not completely dislodged from the target) at the crater rim. Within this general morphological framework, distinct trends and differences in crater dimensions and morphological characteristics are identified. With increasing impact velocity, the volume of craters in dry targets increases by a factor of ~4 when doubling velocity. At identical impact conditions (steel projectiles, ~5km/s), craters in dry and wet sandstone targets differ significantly in that "wet" craters are up to 76% larger in volume, have depth-diameter ratios generally below 0.19 (whereas dry craters are almost consistently above this value) at significantly larger diameters, and their spallation zone morphologies show very different characteristics. In dry craters, the spall zone surfaces dip evenly at 10-20° towards the crater centre. In wet craters, on the other hand, they consist of slightly convex slopes of 10-35° adjacent to the inner depression, and of sub-horizontal tensile failure planes ("terraces") in the outer, near-surface region of the crater. We suggest that these differences are due to a reduction in tensile strength in pore-space saturated sandstone. Linking morphological characteristics to impact conditions might provide a tool to help reconstruct impact conditions in small, more strength- than gravity-dominated impact craters in nature. Findings in small-scale experiments can aid the identification of particular structures in the field, such as spallation induced uplift of strata outside of the crater margins.

Assessment of Laser-Driven Pulsed Neutron Sources for Poolside Neutron-based Advanced NDE – A Pathway to LANSCE-like Characterization at INL

DOE Office of Scientific and Technical Information (OSTI.GOV)

Roth, Markus; Vogel, Sven C.; Bourke, Mark Andrew M.

A variety of opportunities for characterization of fresh nuclear fuels using thermal (~25meV) and epithermal (~10eV) neutrons have been documented at Los Alamos National Laboratory. They include spatially resolved non-destructive characterization of features, isotopic enrichment, chemical heterogeneity and stoichiometry. The LANSCE spallation neutron source is well suited in neutron fluence and temporal characteristics for studies of fuels. However, recent advances in high power short pulse lasers suggest that compact neutron sources might, over the next decade, become viable at a price point that would permit their consideration for poolside characterization on site at irradiation facilities. In a laser-driven neutron sourcemore » the laser is used to accelerate deuterium ions into a beryllium target where neutrons are produced. At this time, the technology is new and their total neutron production is approximately four orders of magnitude less than a facility like LANSCE. However, recent measurements on a sub-optimized system demonstrated >10 10 neutrons in sub-nanosecond pulses in predominantly forward direction. The compactness of the target system compared to a spallation target may allow exchanging the target during a measurement to e.g. characterize a highly radioactive sample with thermal, epithermal, and fast neutrons as well as hard X-rays, thus avoiding sample handling. At this time several groups are working on laser-driven neutron production and are advancing concepts for lasers, laser targets, and optimized neutron target/moderator systems. Advances in performance sufficient to enable poolside fuels characterization with LANSCE-like fluence on sample within a decade may be possible. This report describes the underlying physics and state-of-the-art of the laser-driven neutron production process from the perspective of the DOE/NE mission. It also discusses the development and understanding that will be necessary to provide customized capability for characterization of irradiated fuels. Potential operational advantages compared to a spallation neutron source include reduced shielding complexity, reduced energy requirements, and a production target free of fission products. Contributors to this report include experts in laser-driven neutron production (Roth, Fernandez), laser design (Haefner, Siders, Leemans), laser target design (Glenzer), spallation target/moderator design (Mocko), neutron instrumentation and characterization applications (Vogel, Bourke).« less

Cosmogenic 180W variations in meteorites and re-assessment of a possible 184Os-180W decay system

NASA Astrophysics Data System (ADS)

Cook, David L.; Kruijer, Thomas S.; Leya, Ingo; Kleine, Thorsten

2014-09-01

We measured tungsten (W) isotopes in 23 iron meteorites and the metal phase of the CB chondrite Gujba in order to ascertain if there is evidence for a large-scale nucleosynthetic heterogeneity in the p-process isotope 180W in the solar nebula as recently suggested by Schulz et al. (2013). We observed large excesses in 180W (up to ≈ 6 ε) in some irons. However, significant within-group variations in magmatic IIAB and IVB irons are not consistent with a nucleosynthetic origin, and the collateral effects on 180W from an s-deficit in IVB irons cannot explain the total variation. We present a new model for the combined effects of spallation and neutron capture reactions on 180W in iron meteorites and show that at least some of the observed within-group variability is explained by cosmic ray effects. Neutron capture causes burnout of 180W, whereas spallation reactions lead to positive shifts in 180W. These effects depend on the target composition and cosmic-ray exposure duration; spallation effects increase with Re/W and Os/W ratios in the target and with exposure age. The correlation of 180W/184W with Os/W ratios in iron meteorites results in part from spallogenic production of 180W rather than from 184Os decay, contrary to a recent study by Peters et al. (2014). Residual ε180W excesses after correction for an s-deficit and for cosmic ray effects may be due to ingrowth of 180W from 184Os decay, but the magnitude of this ingrowth is at least a factor of ≈2 smaller than previously suggested. These much smaller effects strongly limit the applicability of the putative 184Os-180W system to investigate geological problems.

New Insights into the Explosion Source from SPE

NASA Astrophysics Data System (ADS)

Patton, H. J.

2015-12-01

Phase I of the Source Physics Experiments (SPE) is a series of chemical explosions at varying depths and yields detonated in the same emplacement hole on Climax stock, a granitic pluton located on the Nevada National Security Site. To date, four of the seven planned tests have been conducted, the last in May 2015, called SPE-4P, with a scaled depth of burial of 1549 m/kt1/3 in order to localize the source in time and space. Surface ground motions validated that the source medium did not undergo spallation, and a key experimental objective was achieved where SPE-4P is the closest of all tests in the series to a pure monopole source and will serve as an empirical Green's function for analysis against other SPE tests. A scientific objective of SPE is to understand mechanisms of rock damage for generating seismic waves, particularly surface and S waves, including prompt damage under compressive stresses and "late-time" damage under tensile stresses. Studies have shown that prompt damage can explain ~75% of the seismic moment for some SPE tests. Spallation is a form of late-time damage and a facilitator of damage mechanisms under tensile stresses including inelastic brittle deformation and shear dilatancy on pre-existing faults or joints. As an empirical Green's function, SPE-4P allows the study of late-time damage mechanisms on other SPE tests that induce spallation and late-time damage, and I'll discuss these studies. The importance for nuclear monitoring cannot be overstated because new research shows that damage mechanisms can affect surface wave magnitude Ms more than tectonic release, and are a likely factor related to anomalous mb-Ms behavior for North Korean tests.

Predicting oxidation-limited lifetime of thin-walled components of NiCrW alloy 230

DOE PAGES

Duan, R.; Jalowicka, Aleksandra; Unocic, Kinga A.; ...

2016-10-18

Using alloy 230 as an example, a generalized oxidation lifetime model for chromia-forming Ni-base wrought alloys is proposed, which captures the most important damaging oxidation effects relevant for component design: wall thickness loss, scale spallation, and the occurrence of breakaway oxidation. For deriving input parameters and for verification of the model approach, alloy 230 specimens with different thicknesses were exposed for different times at temperatures in the range 950–1050 °C in static air. The studies focused on thin specimens (0.2–0.5 mm) to obtain data for critical subscale depletion processes resulting in breakaway oxidation within reasonably achievable test times up tomore » 3000 h. The oxidation kinetics and oxidation-induced subscale microstructural changes were determined by combining gravimetric data with results from scanning electron microscopy with energy dispersive X-ray spectroscopy. The modeling of the scale spallation and re-formation was based on the NASA cyclic oxidation spallation program, while a new model was developed to describe accelerated oxidation occurring after longer exposure times in the thinnest specimens. The calculated oxidation data were combined with the reservoir model equation, by means of which the relation between the consumption and the remaining concentration of Cr in the alloy was established as a function of temperature and specimen thickness. Based on this approach, a generalized lifetime diagram is proposed, in which wall thickness loss is plotted as a function of time, initial specimen thickness, and temperature. As a result, the time to reach a critical Cr level at the scale/alloy interface of 10 wt% is also indicated in the diagrams.« less

APT radionuclide production experiment

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ullmann, J.L.; Gavron, A.; King, J.D.

1994-07-02

Tritium ({sup 3}H, a heavy isotope of hydrogen) is produced by low energy neutron-induced reactions on various elements. One such reaction is n+{sup 3}He {yields}>{sup 3}H+{sup 1}H in which {sup 3}He is transmuted to tritium. Another reaction, which has been used in reactor production of tritium, is the n+{sup 6}Li {yields}> {sup 3}H+{sup 4}He reaction. Accelerator Production of Tritium relies on a high-energy proton beam to produce these neutrons using the spallation reaction, in which high-energy proton beam to produce these neutrons using the spallation reaction, in which high-energy protons reacting with a heavy nucleus produce a shower of low-energymore » neutrons and a lower-mass residual nucleus. It is important to quantify the residual radionuclides produced in the spallation target for two reasons. From an engineering point of view, one must understand short-lived isotopes that may contribute to decay heat. From a safety viewpoint, one must understand what nuclei and decay gammas are produced in order to design adequate shielding, to estimate ultimate waste disposal problems, and to predict possible effects due to accidental dispersion during operation. The authors have performed an experiment to measure the production of radioisotopes in stopping-length W and Pb targets irradiated by a 800 MeV proton beam, and are comparing the results to values obtained from calculations using LAHET and MCNP. The experiment was designed to pay particular attention to the short half-life radionuclides, which have not been previously measured. In the following, they present details of the experiment, explain how they analyzed the data and obtain the results, how they perform the calculations, and finally, how the experimental data agree with the calculations.« less

Influence of the nuclear level density on the odd-even staggering in 56Fe+p spallation at energies from 300 to 1500 MeV/nucleon

NASA Astrophysics Data System (ADS)

Su, Jun; Zhu, Long; Guo, Chenchen

2018-05-01

Background: Special attention has been paid to study the shell effect and odd-even staggering (OES) in the nuclear spallation. Purpose: In this paper, we investigate the influence of the nuclear level density on the OES in the 56Fe+p spallations at energies from 300 to 1500 MeV/nucleon. Method: The isospin-dependent quantum molecular dynamics (IQMD) model is applied to produce the highly excited and equilibrium remnants, which is then de-excited using the statistical model gemini. The excitation energy of the heaviest hot fragments is applied to match the IQMD model with the gemini model. In the gemini model, the statistical description of the evaporation are based on the Hauser-Feshbach formalism, in which level density prescriptions are applied. Results: By investigating the OES of the excited pre-fragments, it is found that the OES originates at the end of the decay process when the excitation energy is close to the nucleon-emission threshold energy, i.e., the smaller value of the neutron separation energy and proton separation energy. The strong influence of level density on the OES is noticed. Two types of the nuclear level densities, the discrepancy of which is only about 7% near the nucleon emission threshold energy, are used in the model. However, the calculated values of the OES differ by the factor of 3 for the relevant nuclei. Conclusions: It is suggested that, although the particle-separation energies play a key role in determining the OES, the level density at excitation energy lower than the particle-separation energies should be taken into consideration

Jet formation in spallation of metal film from substrate under action of femtosecond laser pulse

DOE Office of Scientific and Technical Information (OSTI.GOV)

Inogamov, N. A., E-mail: nailinogamov@googlemail.com; Zhakhovskii, V. V.; Khokhlov, V. A.

2015-01-15

It is well known that during ablation by an ultrashort laser pulse, the main contribution to ablation of the substance is determined not by evaporation, but by the thermomechanical spallation of the substance. For identical metals and pulse parameters, the type of spallation is determined by film thickness d{sub f}. An important gauge is metal heating depth d{sub T} at the two-temperature stage, at which electron temperature is higher than ion temperature. We compare cases with d{sub f} < d{sub T} (thin film) and d{sub f} ≫ d{sub T} (bulk target). Radius R{sub L} of the spot of heating bymore » an optical laser is the next (after d{sub f}) important geometrical parameter. The morphology of film bulging in cases where d{sub f} < d{sub T} on the substrate (blistering) changes upon a change in radius R{sub L} in the range from diffraction limit R{sub L} ∼ λ to high values of R{sub L} ≫ λ, where λ ∼ 1 μm is the wavelength of optical laser radiation. When d{sub f} < d{sub T}, R{sub L} ∼ λ, and F{sub abs} > F{sub m}, gold film deposited on the glass target acquires a cupola-shaped blister with a miniature frozen nanojet in the form of a tip on the circular top of the cupola (F{sub abs} and F{sub m} are the absorbed energy and the melting threshold of the film per unit surface area of the film). A new physical mechanism leading to the formation of the nanojet is proposed.« less

Predicting oxidation-limited lifetime of thin-walled components of NiCrW alloy 230

DOE Office of Scientific and Technical Information (OSTI.GOV)

Duan, R.; Jalowicka, Aleksandra; Unocic, Kinga A.

Using alloy 230 as an example, a generalized oxidation lifetime model for chromia-forming Ni-base wrought alloys is proposed, which captures the most important damaging oxidation effects relevant for component design: wall thickness loss, scale spallation, and the occurrence of breakaway oxidation. For deriving input parameters and for verification of the model approach, alloy 230 specimens with different thicknesses were exposed for different times at temperatures in the range 950–1050 °C in static air. The studies focused on thin specimens (0.2–0.5 mm) to obtain data for critical subscale depletion processes resulting in breakaway oxidation within reasonably achievable test times up tomore » 3000 h. The oxidation kinetics and oxidation-induced subscale microstructural changes were determined by combining gravimetric data with results from scanning electron microscopy with energy dispersive X-ray spectroscopy. The modeling of the scale spallation and re-formation was based on the NASA cyclic oxidation spallation program, while a new model was developed to describe accelerated oxidation occurring after longer exposure times in the thinnest specimens. The calculated oxidation data were combined with the reservoir model equation, by means of which the relation between the consumption and the remaining concentration of Cr in the alloy was established as a function of temperature and specimen thickness. Based on this approach, a generalized lifetime diagram is proposed, in which wall thickness loss is plotted as a function of time, initial specimen thickness, and temperature. As a result, the time to reach a critical Cr level at the scale/alloy interface of 10 wt% is also indicated in the diagrams.« less

The European scene regarding spallation neutron sources

DOE Office of Scientific and Technical Information (OSTI.GOV)

Bauer, G.S.

1996-06-01

In Europe, a short pulse spallation neutron source, ISIS, has been operating for over 10 years, working its way up to a beam power level of 200 kW. A continuous source, SINQ, designed for a beam power of up to 1 MW, is scheduled to start operating at the end of 1996, and a detailed feasibility study has been completed for a 410 kW short pulse source, AUSTRON. Each of these sources seems to have settled for a target concept which is at or near the limits of its feasibility: The ISIS depleted uranium plate targets, heavy water cooled andmore » Zircaloy clad, have so far not shown satisfactory service time and operation is likely to continue with a Ta-plate target, which, in the past has been used successfully for the equivalent of one full-beam-year before it was taken out of service due to degrading thermal properties. SINQ will initially use a rod target, made of Zircaloy only, but plans exist to move on to clad lead rods as quickly as possible. Apart from the not yet explored effect of hydrogen and helium production, there are also concerns about the generation of 7-Be in the cooling water from the spallation of oxygen, which might result in undesirably high radioactivity in the cooling plant room. A Liquid metal target, also under investigation for SINQ, would not only reduce this problem to a level of about 10 %, but would also minimize the risk of radiolytic corrosion in the beam interaction zone. Base on similar arguments, AUSTRON has been designed for edge cooled targets, but thermal and stress analyses show, that this concept is not feasible at higher power levels.« less

Preface

NASA Astrophysics Data System (ADS)

Gorse, D.; Boutard, J.-L.

2002-09-01

The Symposium on “Structural materials for Hybrid systems: A challenge in metallurgy" was held during the “Journées d'Automne 2001" of the “Société Française de Métallurgie et de Matériaux", Paris from October 29 through 31, 2001. The editors of this volume, D. Gorse and J.-L. Boutard, would like to acknowledge GDR GEDEON, CEA - Direction de l'énergie Nucléaire, CNRS - Département des Sciences Chimiques, et Centre d'études de Chimie Métallurgique for sponsoring this symposium. This symposium was divided into three sessions dealing with i) thermodynamics, intergranular penetration and liquid metal embrittlement, ii) irradiation effects in structural materials and iii) compatibility of structural materials with lead alloys in relation with R& D studies for MEGAPIE. The intent of this symposium was to provide a forum for discussing the most recent results obtained in the frame of the materials research program of the “Groupement De Recherche (GDR) GEDEON". Special emphasis was given to all factors susceptible to affect the durability of structural materials for spallation targets, like irradiation effects under proton and neutron mixed spectrum, Liquid Metal Corrosion (LMC) and Embrittlement (LME). The material research program of GEDEON is a joint CEA-CNRS venture. In 1997, the GDR GEDEON gave opportunity to metallurgists and nuclear physicists of both organizations to collaborate for validating the concept of Pb-Bi spallation targets as a key component for Accelerator-Driven Systems (ADS). Historically, since 1995, GDR GEDEON has promoted ADS, also called Hybrid System, as an option for waste management. The starting point of the material program was the 1st GEDEON Workshop on “Materials For Hybrid Systems" held in Paris in 1997, where reference materials of the 9-12 Cr martensitic steels series were selected: EM10 (9Cr-1Mo) and the modified 9Cr-1Mo, T91 (9Cr-1Mo-V-Nb). However, besides their specific concern for ADS, our studies are also of interest for the next generation of LM spallation targets in EU, U.S.A. and Japan. These proceedings contain manuscripts from 90% of the presented papers. The organizers would like to thank all their Colleagues who presented papers, contributed with manuscripts and attended the sessions at the symposium. For sake of clarity, this volume is divided into five sections: 1) general R& D for spallation targets, 2) irradiation effects in liquid metal spallation targets, 3) oxygen control: thermodynamics and monitoring, 4) resistance to liquid metal corrosion and embrittlement of structural materials for spallation targets and 5) basic studies of intergranular penetration and liquid metal embrittlement. Section 1 begins with a description of the spallation neutron source facility SINQ and of ongoing R& D programs at PSI (Switzerland), including MEGAPIE, the joint initiative by six European research institutions and JAERI (Japan), DOE (USA) and KAERI (Korea) to design, build, operate and assess the performance of a liquid lead-bismuth spallation target for 1MW of beam power (G. Bauer et al.). The materials aspects related to the MEGAPIE target and to the LiSoR (Liquid Solid Reactions under irradiation) experiment are reviewed by T. Auger et al. The advantages and drawbacks of solid tungsten spallation targets, compared to liquid Pb-Bi eutectic spallation targets are examined by R. Enderlé et al., presenting the CEA point of view. Section 2 is dedicated to irradiation effects in Liquid Metal (LM) spallation targets structure, a crucial problem for the feasibility of ADS. P. Jung is pointing out the specificity of the irradiation conditions in LM targets by comparison with fast neutron fission and fusion reactors, and the metallurgical consequences like irradiation and helium-induced embrittlement. The author emphasizes the importance of spallation residues whose deleterious effects on in-service properties of target container and window are largely unknown. Until recently, say 1997, only predictions of spallation residues production were available. This motivated the GEDEON workshop on “Nuclear Data for materials studies in the frame of hybrid systems" held in 1999 in Vichy (France). The paper presented by C. Villagrasa et al. highlights the progress achieved during the past five years, promoted by GDR GEDEON. The reverse kinematics experiments performed during that period allowed to obtaining reliable values for production cross sections of residual nuclei produced by spallation reactions. The authors also mention improvements on the computation codes. The case of the target window, thin target simply made of iron from the nuclear physics point of view, is thoroughly investigated. The authors also treat the production of residues in heavy metals, like lead. The experimental data reported below results from the cooperation of CEA, CNRS and Forschungszentrum Jülich within the program SPIRE of the 5th European Framework Program. From the metallurgists point of view, O. Danylova et al. reported an interesting attempt to simulate by doping production of three spallation residues, namely phosphorus, sulfur and titanium, certainly detrimental regarding the mechanical properties (fracture toughness...) of the 9% Cr martensitic steels pre-selected for the target window and container. The authors describe the inherent difficulties encountered for obtaining the microstructure and modified steel composition expected under irradiation. In all cases, production of hydrogen and helium is expected very high, ~90 000 appm/year for hydrogen and ~5000 appm/year for helium, corresponding to a damage level of ~100 dpa/year in the target window. These estimated values are just mentioned to show the importance of the metallurgical problem to be faced. These data motivated studies of helium implantation effects by J. Henry et al. in two 9Cr-1Mo (EM10) and modified 9Cr-1Mo-V-Nb (T91) pre-selected martensitic steels. Homogeneous implantation of 5000 appm He in T91 and EM10 thin foils followed by TEM examination and tensile testing revealed an important hardening and embrittlement at 250 °C. At 500 °C both materials exhibit far less hardening and retain significant ductility. In the latter case, those findings were correlated with the appearance of helium bubbles detected in Transmission Electron Microscopy (TEM) examination. At 250 °C, no He bubble is detected by TEM. Conversely, Small Angle Neutron Scattering (SANS) allows to identify a high density of objects ~1-2 nm, most probably tiny He bubbles. The low temperature He embrittlement is most probably due to the conjunction of grain hardening and decrease of the cohesive energy of prior austenitic grain boundaries due to He segregation. Besides hydrogen and helium, significant quantities of other spallation residues will be also accumulated in the target window during one year of operation. About 1000 appm of calcium form after one year of irradiation with 1 GeV protons. This exemplary insoluble spallation residue could also contribute to embrittle the window. G. Amiri et al. studied the implantation of both calcium and sulfur (up to 1-2 at% corresponding to a 20 dpa damage level) at 500 °C, assumed to be the highest temperature of the target window in service conditions. P. Pareige et al. detected the formation of Ca nanoclusters using the 3D atomic probe. Neither calcium sulfides nor carbides were detectable whatever the temperature (300 °C or 500 °C) and damage levels. E. Cadel, P. Pareige and M.O. Ruault showed how powerful is the 3D atom probe to characterize both chemical and structural evolution of irradiated steel specimens, at a nanometric scale allowing for interpretation of radiation damages “from first principles". Section 3 is dedicated to oxygen control, including thermodynamic aspects and monitoring. The GDR GEDEON material program promoted the development of oxygen sensors in liquid metals. V. Ghetta et al. studied carefully the possibilities, limitations of existing sensors and proposed new developments allowing to interpret e.m.f measurements at temperatures well below 450 °C. Intercomparisons between oxygen sensors, using various static facilities (BIP, JACOMEX and COLIMESTA) were carried out by J.-L. Courouau et al. This study is now going on including our EU partners in the closely related TECLA program granted by the 5th framework program. C. Lesueur et al. developed original methods for measuring wettability, permitting to determine the stability of native oxides (on Al, Fe, Ni and also T91 steel) in contact with molten lead. A. Maitre et al. presented a preliminary thermodynamic study of the quinary Bi-Fe-Hg-O-Pb system, beginning with the Bi-Hg-Pb system. No solid ternary phase was found in Pb-Bi eutectic in the temperature range expected for the spallation target. Then the authors focused on the possible formation of oxygenated compounds of low melting point either at the T91 steel/Pb or at the T91 steel/Pb-Bi eutectic interface. Section 4 concerns the resistance to LMC and LME of structural materials pre-selected for the spallation target of ADS, with special emphasis on the liquid Pb-Bi eutectic target concept. The compatibility of 9% Cr martensitic steels (like EM10 or T91...) with liquid Pb and Pb-Bi eutectic was examined. Qualification of the T91 steel/LBE system is required to build the liquid Pb-Bi target in PSI in 2005 and for further applications. A comparative study of the long-term corrosion behaviour of various martensitic and austenitic steels in forced circulation loop was carried out by F. Balbaud-Celerier et al. allowing to vary the temperature and oxygen content in LBE covering the range 10-8wt% -10-6wt.% . This work results from a fruitful collaboration with IPPE (Obninsk, Russia). The two following papers of Section 4 deal with the tensile behaviour of T91 steel in contact with lead and its alloys. The most severe metallurgical (J.-B. Vogt et al.) and environmental (J.-L. Pastol et al.) conditions are considered in order to estimate the risk of LME for the target window in service. J.-B. Vogt et al. observed a transgranular (TG) brittle fracture after hardening heat treatment of T91 steel after tensile testing of notched specimens at 350 °C in oxygen-saturated lead. Note that cases of TG-LME are rather scarcely observed. On the other hand, J.-L. Pastol et al. obtained an embrittling effect on notched specimens by optimizing the environmental parameters (in LBE at 350 °C under He-4% H2 cover gas...) and tensile testing conditions. F. Gamaoun et al. showed that a few days exposure of T91 steel in lead under either reducing or oxidizing conditions gives rise to a significant porosity in the steel. This could justify the increased stress relaxation kinetics of specimens submitted to 4-point bending tests under the same conditions. Besides the R& D research related to the spallation target for ADS, a non-negligible part of the GEDEON material research program was dedicated to intergranular penetration and LME. Some exemplary LME studies are reported in Section 5 of this volume, illustrating various aspects of this very old, tricky and exotic problem in metallurgy. One can find in this volume studies involving various Solid Metal/Liquid Metal (SM/LM) couples, going from high purity metal couples (Ni/Pb, Ni/Bi...) to industrial metallic alloys put in contact with liquid metals or alloys of varying purity. LME is a multi scale phenomenon that cannot be explained on the sole basis of either thermodynamics, metallurgical or kinetics criteria. In this section, the role of the stress-strain state is emphasized. The importance of the microstructure of the grains boundaries (facetting...) on LM penetration is also pointed out. This aspect of the problem can now be dealt with thanks to Atomic Force Microscopy (AFM), High Resolution Transmission Electron Microscopy (HRTEM), Electron Energy Loss Spectroscopy (EELS) and Auger Electron Spectroscopy (AES) techniques. Crack propagation kinetics can now be followed at ESRF (Grenoble) using synchrotron radiation imaging techniques. It is now possible to follow the propagation, structure and chemistry of the embrittling phase in the crack, at microscopic and at nanometric scale. It is also possible, in principle, to take into account the role of defects in grain-boundaries (GB) on the penetration of the embrittling species and conversely to investigate the role of the defects produced by wetting on the GB microstructure. We do hope that these techniques open a new and attractive field of research to improve the understanding of LME. The HRTEM study carried out by A. Charai et al. enlightens the importance of crystallography on wetting. Two exemplary couples are thoroughly investigated: the Mo/Ni couple giving rise to an interfacial nanometer thick interface for one type of Mo bicrystal wetted by nickel and the Ni/Pb couple pointing out the role of the GB plane on wetting. Y. Brechet et al. investigated not only the microstructure effects on “LM" penetration into cracks (cracks kinetics and morphologies), but also the plasticity effects ahead of the crack tip, studying a variant of the mythic Al/Ga couple, say the 7010 Aluminum alloy in contact with Gallium, allowing for modifications of the precipitation state at the GBs by applying various heat treatments. Y. Brechet et al. conclude in favour of a step by step penetration process, quasi at atomic scale and give an estimate of crack propagation velocity, of the order of a few micrometers per second, in good agreement with experimental observations. The author stresses the importance of defects in the GBs (precipitates...) at different scales which can explain discrepancies between the experimental crack velocity and the one calculated using a continuum elastic model. The paper presented by W. Ludwig et al. concentrates on two synchrotron radiation imaging techniques (X-ray micro-radiography and micro-fluorescence) available at ESRF (Grenoble) in order to characterize the penetration kinetics of embrittling species in the crack. Beside the Al/Ga couple, it is shown that those techniques are suitable to follow intergranular propagation of cracks in the Ni/Bi system, even when the embrittling layer becomes nanometric. Structuration of liquid Al in contact with Cu(100) and Cu(111) surfaces of a bulk Cu crystal was studied by P. Geysermans et al. using Molecular Dynamics simulations. The authors showed an epitaxial relationship, whatever the density of the solid and contacting liquid phases. This feature is of importance to understand the structure of the wetting layers in GBs. J. Bernardini et al. emphasize the role of macroscopic defects like facets in GBs on “LM" penetration and propose a model allowing to describe the real shape of the cracks they observed with Ni annealed in contact with pure lead, inconsistent with Mullins grooving theory. Cu/Bi, Cu/LBE (Lead-Bismuth Eutectic) and Ni/LBE systems were studied by K. Wolski et al. using AES semi-quantitative analysis of fractured specimens under vacuum within an Auger Electron spectrometer, enlightening the embrittling role of the nanometer-thick wetting layer in the crack tip area. In summary, during the past five years close cooperation between researchers within the material research program of GEDEON co-sponsored by the 5th EU Framework program allowed to make significant progress. Research dedicated to radiation damage in structural materials for ADS and spallation targets was very active and a number of impressive results were obtained. The low temperature He embrittlement is certainly a matter of concern. The controlling mechanisms and their dependence with temperature, He and dpa production rate has to be clarified. Likewise, compatibility studies of structural materials with lead and lead alloys, particularly LBE, gave rise to a number of remarkable results. One can mention here specifically the progress made with oxygen sensors. Significant is also the renewal of interest for LME during the past five years. Promising results on LME and intergranular penetration are already obtained and should be obtained in this attractive field of research. Of course, a great deal of work remains to be done in order to validate the concept of Pb-Bi spallation target for ADS. Especially, the effect of spallation elements production in structural materials and in LBE has to be assessed as well as LMC and LME under irradiation.

Neutron Scattering Facilities

Science.gov Websites

Low Energy Neutron Source (LENS), Indiana University Cyclotron Facility, USA McMaster Nuclear Reactor Research, Gaithersburg, Maryland, USA Peruvian Institute of Nuclear Energy (IPEN), Lima, Peru Spallation Nuclear Science and Technology Organisation, Lucas Heights, Australia High-flux Advanced Neutron

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ene, D.; Andersson, K.; Jensen, M.

The European Spallation Source (ESS) will produce tritium via spallation and activation processes during operational activities. Within the location of ESS facility in Lund, Sweden site it is mandatory to demonstrate that the management strategy of the produced tritium ensures the compliance with the country regulation criteria. The aim of this paper is to give an overview of the different aspects of the tritium management in ESS facility. Besides the design parameter study of the helium coolant purification system of the target the consequences of the tritium releasing into the environment were also analyzed. Calculations show that the annual releasemore » of tritium during the normal operations represents a small fraction from the estimated total dose. However, more refined calculations of migration of activated-groundwater should be performed for higher hydraulic conductivities, with the availability of the results on soil examinations. With the assumption of 100% release of tritium to the atmosphere during the occurring of the extreme accidents, it was found as well that the total dose complies with the constraint. (authors)« less

Improvements to the internal and external antenna H(-) ion sources at the Spallation Neutron Source.

PubMed

Welton, R F; Dudnikov, V G; Han, B X; Murray, S N; Pennisi, T R; Pillar, C; Santana, M; Stockli, M P; Turvey, M W

2014-02-01

The Spallation Neutron Source (SNS), a large scale neutron production facility, routinely operates with 30-40 mA peak current in the linac. Recent measurements have shown that our RF-driven internal antenna, Cs-enhanced, multi-cusp ion sources injects ∼55 mA of H(-) beam current (∼1 ms, 60 Hz) at 65-kV into a Radio Frequency Quadrupole (RFQ) accelerator through a closely coupled electrostatic Low-Energy Beam Transport system. Over the last several years a decrease in RFQ transmission and issues with internal antennas has stimulated source development at the SNS both for the internal and external antenna ion sources. This report discusses progress in improving internal antenna reliability, H(-) yield improvements which resulted from modifications to the outlet aperture assembly (applicable to both internal and external antenna sources) and studies made of the long standing problem of beam persistence with the external antenna source. The current status of the external antenna ion source will also be presented.

Cosmic ray models for early galactic lithium, beryllium, and boron production

NASA Technical Reports Server (NTRS)

Fields, Brian D.; Olive, Keith A.; Schramm, David N.

1994-01-01

To better understand the early galactic production of Li, Be, and B by cosmic ray spallation and fusion reactions, the dependence of these production rates on cosmic ray models and model parameters is examined. The sensitivity of elemental and isotropic production to the cosmic ray pathlength magnitude and energy dependence, source spectrum spallation kinematics, and cross section uncertainties is studied. Changes in these model features, particularly those features related to confinement, are shown to alter the Be- and B-versus-Fe slopes from a naive quadratic relation. The implications of our results for the diffuse gamma-ray background are examined, and the role of chemical evolution and its relation to our results is noted. It is also noted that the unmeasured high energy behavior of alpha + alpha fusion can lead to effects as large as a factor of 2 in the resultant yields. Future data should enable Population II Li, Be, and B abundances to constrain cosmic ray models for the early Galaxy.

The cold neutron chopper spectrometer at the Spallation Neutron Source—A review of the first 8 years of operation

DOE PAGES

Ehlers, G.; Podlesnyak, A. A.; Kolesnikov, A. I.

2016-09-13

The first eight years of operation of the Cold Neutron Chopper Spectrometer (CNCS) at the Spallation Neutron Source in Oak Ridge is being reviewed. The instrument has been part of the facility user program since 2009, and more than 250 individual user experiments have been performed to date. CNCS is an extremely powerful and versatile instrument and offers leading edge performance in terms of beam intensity, energy resolution, and flexibility to trade one for another. In addition, experiments are being routinely performed with the sample at extreme conditions: T ≲ 0.05 K, p ≳ 2 GPa, and B = 8more » T can be achieved individually or in combination. In particular, CNCS is in a position to advance the state of the art with inelastic neutron scattering under pressure, and some of the recent accomplishments in this area will be presented in more detail.« less

Spallative nucleosynthesis in supernova remnants. II. Time-dependent numerical results

NASA Astrophysics Data System (ADS)

Parizot, Etienne; Drury, Luke

1999-06-01

We calculate the spallative production of light elements associated with the explosion of an isolated supernova in the interstellar medium, using a time-dependent model taking into account the dilution of the ejected enriched material and the adiabatic energy losses. We first derive the injection function of energetic particles (EPs) accelerated at both the forward and the reverse shock, as a function of time. Then we calculate the Be yields obtained in both cases and compare them to the value implied by the observational data for metal-poor stars in the halo of our Galaxy, using both O and Fe data. We find that none of the processes investigated here can account for the amount of Be found in these stars, which confirms the analytical results of Parizot & Drury (1999). We finally analyze the consequences of these results for Galactic chemical evolution, and suggest that a model involving superbubbles might alleviate the energetics problem in a quite natural way.

Interfacial characteristics and determination of cohesive and adhesive strength of plasma-coated hydroxyapatite via nanoindentation and microscratch techniques.

PubMed

McManamon, Colm; de Silva, Johann P; Power, John; Ramirez-Garcia, Sonia; Morris, Michael A; Cross, Graham L W

2014-09-30

We investigate the chemical composition and mechanical properties of plasma-deposited hydroxyapatite on grit-blasted Ti-6Al-4V coupons as models of typical prosthetic hip implants. Nanoindentation is used to extract the mechanical properties of the hydroxyapatite (HA) coating and to evaluate the behavior of the material as a function of distance from the interface. A microscratch technique was used to determine parameters of cohesive and adhesive failure of the material that are critical in determining the functionality of these biomedical devices. This delamination method has not been studied in detail before and is usually considered to be unsuitable because of the thickness of the HA and the roughness of the substrate. However, through cross-section analysis of the scratch test, we can determine the point at which the HA delaminates from the substrate. It was concluded that spallation occurs locally, and there is no evidence of gross spallation, indicating that the coating is well adhered to the substrate.

The Spallation Neutron Source accelerator system design

NASA Astrophysics Data System (ADS)

Henderson, S.; Abraham, W.; Aleksandrov, A.; Allen, C.; Alonso, J.; Anderson, D.; Arenius, D.; Arthur, T.; Assadi, S.; Ayers, J.; Bach, P.; Badea, V.; Battle, R.; Beebe-Wang, J.; Bergmann, B.; Bernardin, J.; Bhatia, T.; Billen, J.; Birke, T.; Bjorklund, E.; Blaskiewicz, M.; Blind, B.; Blokland, W.; Bookwalter, V.; Borovina, D.; Bowling, S.; Bradley, J.; Brantley, C.; Brennan, J.; Brodowski, J.; Brown, S.; Brown, R.; Bruce, D.; Bultman, N.; Cameron, P.; Campisi, I.; Casagrande, F.; Catalan-Lasheras, N.; Champion, M.; Champion, M.; Chen, Z.; Cheng, D.; Cho, Y.; Christensen, K.; Chu, C.; Cleaves, J.; Connolly, R.; Cote, T.; Cousineau, S.; Crandall, K.; Creel, J.; Crofford, M.; Cull, P.; Cutler, R.; Dabney, R.; Dalesio, L.; Daly, E.; Damm, R.; Danilov, V.; Davino, D.; Davis, K.; Dawson, C.; Day, L.; Deibele, C.; Delayen, J.; DeLong, J.; Demello, A.; DeVan, W.; Digennaro, R.; Dixon, K.; Dodson, G.; Doleans, M.; Doolittle, L.; Doss, J.; Drury, M.; Elliot, T.; Ellis, S.; Error, J.; Fazekas, J.; Fedotov, A.; Feng, P.; Fischer, J.; Fox, W.; Fuja, R.; Funk, W.; Galambos, J.; Ganni, V.; Garnett, R.; Geng, X.; Gentzlinger, R.; Giannella, M.; Gibson, P.; Gillis, R.; Gioia, J.; Gordon, J.; Gough, R.; Greer, J.; Gregory, W.; Gribble, R.; Grice, W.; Gurd, D.; Gurd, P.; Guthrie, A.; Hahn, H.; Hardek, T.; Hardekopf, R.; Harrison, J.; Hatfield, D.; He, P.; Hechler, M.; Heistermann, F.; Helus, S.; Hiatt, T.; Hicks, S.; Hill, J.; Hill, J.; Hoff, L.; Hoff, M.; Hogan, J.; Holding, M.; Holik, P.; Holmes, J.; Holtkamp, N.; Hovater, C.; Howell, M.; Hseuh, H.; Huhn, A.; Hunter, T.; Ilg, T.; Jackson, J.; Jain, A.; Jason, A.; Jeon, D.; Johnson, G.; Jones, A.; Joseph, S.; Justice, A.; Kang, Y.; Kasemir, K.; Keller, R.; Kersevan, R.; Kerstiens, D.; Kesselman, M.; Kim, S.; Kneisel, P.; Kravchuk, L.; Kuneli, T.; Kurennoy, S.; Kustom, R.; Kwon, S.; Ladd, P.; Lambiase, R.; Lee, Y. Y.; Leitner, M.; Leung, K.-N.; Lewis, S.; Liaw, C.; Lionberger, C.; Lo, C. C.; Long, C.; Ludewig, H.; Ludvig, J.; Luft, P.; Lynch, M.; Ma, H.; MacGill, R.; Macha, K.; Madre, B.; Mahler, G.; Mahoney, K.; Maines, J.; Mammosser, J.; Mann, T.; Marneris, I.; Marroquin, P.; Martineau, R.; Matsumoto, K.; McCarthy, M.; McChesney, C.; McGahern, W.; McGehee, P.; Meng, W.; Merz, B.; Meyer, R.; Meyer, R.; Miller, B.; Mitchell, R.; Mize, J.; Monroy, M.; Munro, J.; Murdoch, G.; Musson, J.; Nath, S.; Nelson, R.; Nelson, R.; O`Hara, J.; Olsen, D.; Oren, W.; Oshatz, D.; Owens, T.; Pai, C.; Papaphilippou, I.; Patterson, N.; Patterson, J.; Pearson, C.; Pelaia, T.; Pieck, M.; Piller, C.; Plawski, T.; Plum, M.; Pogge, J.; Power, J.; Powers, T.; Preble, J.; Prokop, M.; Pruyn, J.; Purcell, D.; Rank, J.; Raparia, D.; Ratti, A.; Reass, W.; Reece, K.; Rees, D.; Regan, A.; Regis, M.; Reijonen, J.; Rej, D.; Richards, D.; Richied, D.; Rode, C.; Rodriguez, W.; Rodriguez, M.; Rohlev, A.; Rose, C.; Roseberry, T.; Rowton, L.; Roybal, W.; Rust, K.; Salazer, G.; Sandberg, J.; Saunders, J.; Schenkel, T.; Schneider, W.; Schrage, D.; Schubert, J.; Severino, F.; Shafer, R.; Shea, T.; Shishlo, A.; Shoaee, H.; Sibley, C.; Sims, J.; Smee, S.; Smith, J.; Smith, K.; Spitz, R.; Staples, J.; Stein, P.; Stettler, M.; Stirbet, M.; Stockli, M.; Stone, W.; Stout, D.; Stovall, J.; Strelo, W.; Strong, H.; Sundelin, R.; Syversrud, D.; Szajbler, M.; Takeda, H.; Tallerico, P.; Tang, J.; Tanke, E.; Tepikian, S.; Thomae, R.; Thompson, D.; Thomson, D.; Thuot, M.; Treml, C.; Tsoupas, N.; Tuozzolo, J.; Tuzel, W.; Vassioutchenko, A.; Virostek, S.; Wallig, J.; Wanderer, P.; Wang, Y.; Wang, J. G.; Wangler, T.; Warren, D.; Wei, J.; Weiss, D.; Welton, R.; Weng, J.; Weng, W.-T.; Wezensky, M.; White, M.; Whitlatch, T.; Williams, D.; Williams, E.; Wilson, K.; Wiseman, M.; Wood, R.; Wright, P.; Wu, A.; Ybarrolaza, N.; Young, K.; Young, L.; Yourd, R.; Zachoszcz, A.; Zaltsman, A.; Zhang, S.; Zhang, W.; Zhang, Y.; Zhukov, A.

2014-11-01

The Spallation Neutron Source (SNS) was designed and constructed by a collaboration of six U.S. Department of Energy national laboratories. The SNS accelerator system consists of a 1 GeV linear accelerator and an accumulator ring providing 1.4 MW of proton beam power in microsecond-long beam pulses to a liquid mercury target for neutron production. The accelerator complex consists of a front-end negative hydrogen-ion injector system, an 87 MeV drift tube linear accelerator, a 186 MeV side-coupled linear accelerator, a 1 GeV superconducting linear accelerator, a 248-m circumference accumulator ring and associated beam transport lines. The accelerator complex is supported by ~100 high-power RF power systems, a 2 K cryogenic plant, ~400 DC and pulsed power supply systems, ~400 beam diagnostic devices and a distributed control system handling ~100,000 I/O signals. The beam dynamics design of the SNS accelerator is presented, as is the engineering design of the major accelerator subsystems.

Measurement of Recoil Losses and Ranges for Spallation Products Produced in Proton Interactions with Al, Si, Mg at 200 and 500 MeV

NASA Technical Reports Server (NTRS)

Sisterson, J. M.

2005-01-01

Cosmic rays interact with extraterrestrial materials to produce a variety of spallation products. If these cosmogenic nuclides are produced within an inclusion in such material, then an important consideration is the loss of the product nuclei, which recoil out of the inclusion. Of course, at the same time, some atoms of the product nuclei under study may be knocked into the inclusion from the surrounding material, which is likely to have a different composition to that of the inclusion [1]. For example, Ne-21 would be produced in presolar grains, such as SiC, when irradiated in interstellar space. However, to calculate a presolar age, one needs to know how much 21Ne is retained in the grain. For small grains, the recoil losses might be large [2, 3] To study this effect under laboratory conditions, recoil measurements were made using protons with energies from 66 - 1600 MeV on Si, Al and Ba targets [3, 4, 5].

New controller for high voltage converter modulator at spallation neutron source

DOE Office of Scientific and Technical Information (OSTI.GOV)

Wezensky, Mark W; Brown, David L; Lee, Sung-Woo

2017-01-01

The Spallation Neutron Source (SNS) has developed a new control system for the High Voltage Convertor Modulator (HVCM) at the SNS to replace the original control system which is approaching obsolescence. The original system was based on controllers for similar high voltage systems that were already in use [1]. The new controller, based on National Instruments PXI/FlexRIO Field Programmable Gate Array (FPGA) platform, offers enhancements such as modular construction, flexibility and non-proprietary software. The new controller also provides new capabilities like various methods for modulator pulse flattening, waveform capture, and first fault detection. This paper will discuss the design ofmore » the system, including the human machine interface, based on lessons learned at the SNS and other projects. It will also discuss performance and other issues related to its operation in an accelerator facility which requires high availability. To date, 73% of the operational HVCMs have been upgraded to with the new controller, and the remainder are scheduled for completion by mid-2017.« less

Cosmic-ray models for early Galactic Lithium, Beryllium, and Boron production

NASA Technical Reports Server (NTRS)

Fields, Brian D.; Olive, Keith A.; Schramm, David N.

1994-01-01

To understand better the early Galactic production of Li, Be, and B by comsmic-ray spallation and fusion reactions, the dependence of these production rates on cosmic-ray models and model parameters is examined. The sensitivity of elemental and isotopic production to the cosmic-ray path length magnitude and energy dependence, source spectrum, spallation kinematics, and cross section uncertainties is studied. Changes in these model features, particularly those features related to confinement, are shown to alter the Be- and B- versus-Fe slopes from a naive quadratic relation. The implications of our results for the diffuse gamma-ray background are examined, and the role of chemical evolution and its relation to our results is noted. It is also noted that the unmeasured high-energy behavior of alpha + alpha fusion can lead to effects as large as a factor of 2 in the resultant yields. Future data should enable Population II Li, Be, and B abundances to constrain cosmic-ray models for the early Galaxy.

The boron-to-beryllium ratio in halo stars - A signature of cosmic-ray nucleosynthesis in the early Galaxy

NASA Technical Reports Server (NTRS)

Walker, T. P.; Steigman, G.; Schramm, D. N.; Olive, K. A.; Fields, B.

1993-01-01

We discuss Galactic cosmic-ray (GCR) spallation production of Li, Be, and B in the early Galaxy with particular attention to the uncertainties in the predictions of this model. The observed correlation between the Be abundance and the metallicity in metal-poor Population II stars requires that Be was synthesized in the early Galaxy. We show that the observations and such Population II GCR synthesis of Be are quantitatively consistent with the big bang nucleosynthesis production of Li-7. We find that there is a nearly model independent lower bound to B/Be of about 7 for GCR synthesis. Recent measurements of B/Be about 10 in HD 140283 are in excellent agreement with the predictions of Population II GCR nucleosynthesis. Measurements of the boron abundance in additional metal-poor halo stars is a key diagnostic of the GCR spallation mechanism. We also show that Population II GCR synthesis can produce amounts of Li-6 which may be observed in the hottest halo stars.

Possible Contribution of Nuclear Fragmentation Induced by High Energy Cosmic Protons to Single Effects Transients in Modern 3D Technology On-Board Devices

NASA Astrophysics Data System (ADS)

Chechenin, Nikolay; Chumanov, Vladimir; Kadmenskii, Anatolii

There is a tendency in modern integrated circuits manufacturing technology that in line with the growth of the density of transistors, the volume occupied by isolated conductive metallic layers on-chip also increases with copper and tungsten more frequently used instead of aluminum. Spallation reaction of 10 MeV to 1 GeV and above protons with tungsten and copper nuclei leads to formation of a large number of isotopes of elements from O to Ta. Experimental data on the cross sections of nuclear spallation reactions and average speed of residual nuclear fragments in inverse kinematics have been published in the last decade. In our report, we analyze the published data and evaluate ionization effects of the fragments from the reaction W (p, X) in the sensitive areas of transistors in microcircuit made by 3DIC technology with interlayer coupling by tungsten conductive pins (or vias), and metallic in-layer interconnection paths.

The CENNS-10 liquid argon detector to measure CEvNS at the Spallation Neutron Source

NASA Astrophysics Data System (ADS)

Tayloe, R.

2018-04-01

The COHERENT collaboration is deploying a suite of low-energy detectors in a low-background corridor of the ORNL Spallation Neutron Source (SNS) to measure coherent elastic neutrino-nucleus scattering (CEvNS) on an array of nuclear targets employing different detector technologies. A measurement of CEvNS on different nuclei will test the N2-dependence of the CEvNS cross section and further the physics reach of the COHERENT effort. The first step of this program has been realized recently with the observation of CEvNS in a 14.6 kg CsI detector. Operation and deployment of Ge and NaI detectors are also underway. A 22 kg, single-phase, liquid argon detector (CENNS-10) started data-taking in Dec. 2016 and will provide results on CEvNS from a lighter nucleus. Initial results indicate that light output, pulse-shape discrimination, and background suppression are sufficient for a measurement of CEvNS on argon.

Single-shot femtosecond laser ablation of gold surface in air and isopropyl alcohol

NASA Astrophysics Data System (ADS)

Kudryashov, S. I.; Saraeva, I. N.; Lednev, V. N.; Pershin, S. M.; Rudenko, A. A.; Ionin, A. A.

2018-05-01

Single-shot IR femtosecond-laser ablation of gold surfaces in ambient air and liquid isopropyl alcohol was studied by scanning electron microscopy characterization of crater topographies and time-resolved optical emission spectroscopy of ablative plumes in regimes, typical for non-filamentary and non-fragmentation laser production of nanoparticle sols. Despite one order of magnitude shorter (few nanoseconds) lifetimes and almost two orders of magnitude lower intensities of the quenched ablative plume emission in the alcohol ambient at the same peak laser fluence, craters for the dry and wet conditions appeared with rather similar nanofoam-like spallative topographies and the same thresholds. These facts envision the underlying surface spallation as one of the basic ablation mechanisms relevant for both dry and wet advanced femtosecond laser surface nano/micro-machining and texturing, as well as for high-throughput femtosecond laser ablative production of colloidal nanoparticles by MHz laser-pulse trains via their direct nanoscale jetting from the nanofoam in air and fluid environments.

A target development program for beamhole spallation neutron sources in the megawatt range

DOE Office of Scientific and Technical Information (OSTI.GOV)

Bauer, G.S.; Atchison, F.

1995-10-01

Spallation sources as an alternative to fission neutron sources have been operating successfully up to 160 kW of beam power. With the next generation of these facilities aiming at the medium power range between 0.5 and 5 MW, loads on the targets will be high enough to make present experience of little relevance. With the 0.6 MW continuous facility SINQ under construction, and a 5 MW pulsed facility (ESS) under study in Europe, a research and development program is about to be started which aimes at assessing the limits of stationary and moving solid targets and the feasibility and potentialmore » benefits of flowing liquid metal targets. Apart from theoretical work and examination of existing irradiated material, including used targets from ISIS, it is intended to take advantage of the SINQ solid rod target design to improve the relevant data base by building the target in such a way that individual rods can be equipped as irradiation capsules.« less

Spin exchange optical pumping based polarized 3He filling station for the Hybrid Spectrometer at the Spallation Neutron Source.

PubMed

Jiang, C Y; Tong, X; Brown, D R; Culbertson, H; Graves-Brook, M K; Hagen, M E; Kadron, B; Lee, W T; Robertson, J L; Winn, B

2013-06-01

The Hybrid Spectrometer (HYSPEC) is a new direct geometry spectrometer at the Spallation Neutron Source at the Oak Ridge National Laboratory. This instrument is equipped with polarization analysis capability with 60° horizontal and 15° vertical detector coverages. In order to provide wide angle polarization analysis for this instrument, we have designed and built a novel polarized (3)He filling station based on the spin exchange optical pumping method. It is designed to supply polarized (3)He gas to HYSPEC as a neutron polarization analyzer. In addition, the station can optimize the (3)He pressure with respect to the scattered neutron energies. The depolarized (3)He gas in the analyzer can be transferred back to the station to be repolarized. We have constructed the prototype filling station. Preliminary tests have been carried out demonstrating the feasibility of the filling station. Here, we report on the design, construction, and the preliminary results of the prototype filling station.

Experiment Automation with a Robot Arm using the Liquids Reflectometer Instrument at the Spallation Neutron Source

DOE Office of Scientific and Technical Information (OSTI.GOV)

Zolnierczuk, Piotr A; Vacaliuc, Bogdan; Sundaram, Madhan

The Liquids Reflectometer instrument installed at the Spallation Neutron Source (SNS) enables observations of chemical kinetics, solid-state reactions and phase-transitions of thin film materials at both solid and liquid surfaces. Effective measurement of these behaviors requires each sample to be calibrated dynamically using the neutron beam and the data acquisition system in a feedback loop. Since the SNS is an intense neutron source, the time needed to perform the measurement can be the same as the alignment process, leading to a labor-intensive operation that is exhausting to users. An update to the instrument control system, completed in March 2013, implementedmore » the key features of automated sample alignment and robot-driven sample management, allowing for unattended operation over extended periods, lasting as long as 20 hours. We present a case study of the effort, detailing the mechanical, electrical and software modifications that were made as well as the lessons learned during the integration, verification and testing process.« less

Testing Single Phase IGBT H-Bridge Switch Plates for the High Voltage Converter Modulator at the Spallation Neutron Source

DOE Office of Scientific and Technical Information (OSTI.GOV)

Peplov, Vladimir V; Anderson, David E; Solley, Dennis J

2014-01-01

Three IGBT H-bridge switching networks are used in each High Voltage Converter Modulator (HVCM) system at the Spallation Neutron Source (SNS) to generate drive currents to three boost transformer primaries switching between positive and negative bus voltages at 20 kHz. Every switch plate assembly is tested before installing it into an operational HVCM. A Single Phase Test Stand has been built for this purpose, and it is used for adjustment, measurement and testing of different configurations of switch plates. This paper will present a description of the Test Stand configuration and discuss the results of testing switch plates with twomore » different types of IGBT gate drivers currently in use on the HVCM systems. Comparison of timing characteristics of the original and new drivers and the resulting performance reinforces the necessity to replace the original H-bridge network drivers with the upgraded units.« less

800-MeV proton irradiation of thorium and depleted uranium targets

DOE Office of Scientific and Technical Information (OSTI.GOV)

Russell, G.J.; Brun, T.O.; Pitcher, E.J.

As part of the Los Alamos Fertile-to-Fissile-Conversion (FERFICON) program in the late 1980`s, thick targets of the fertile materials thorium and depleted uranium were bombarded by 800-MeV protons to produce the fissile materials {sup 233}U and {sup 239}Pu, respectively. The amount of {sup 233}U made was determined by measuring the {sup 233}Pa activity, and the yield of {sup 239}Pu was deduced by measuring the activity of {sup 239}Np. For the thorium target, 4 spallation products and 34 fission products were also measured. For the depleted uranium target, 3 spallation products and 16 fission products were also measured. The number ofmore » fissions in each target was deduced from fission product mass-yield curves. In actuality, axial distributions of the products were measured, and the distributions were then integrated over the target volume to obtain the total number of products for each reaction.« less

Neutron production for 250 MeV protons bombarding on thick grain-made tungsten target

NASA Astrophysics Data System (ADS)

Zhang, Xueying; Zhang, Yanbin; Ma, Fei; Ju, Yongqin; Chen, Liang; Zhang, Hongbin; Li, Yanyan; Wan, Bo; Wang, Jianguo; Ge, Honglin

2015-08-01

Neutron yield for 250 MeV protons incident on a tungsten target has been measured using the water bath method. The target was made of many randomly placed tungsten grains. Through analyzing the activity of Au foils, the neutron flux distribution in water was obtained. The neutrons slowing down process shows that the neutrons from tungsten have an average energy lower than neutrons from the lead target. The neutron yield was experimentally determined to be 2.02 ± 0.15 neutron/proton. Detailed simulation was also performed with the Geant4 toolkit. Comparison has been made with the experimentally derived neutron yield. It was found that, around 250 MeV, experimental results were described satisfactorily with a combination of high-energy spallation, low-energy neutron reaction and scattering. It was shown that the grain-packed target does not affect much the main neutronic properties, which are of crucial importance for the design of the spallation target.

Design and implementation of a multiaxial loading capability during heating on an engineering neutron diffractometer

DOE PAGES

Benafan, O.; Padula, S. A.; Skorpenske, H. D.; ...

2014-10-02

Here we discuss a gripping capability that was designed, implemented, and tested for in situ neutron diffraction measurements during multiaxial loading and heating on the VULCAN engineering materials diffractometer at the spallation neutron source at Oak Ridge National Laboratory.

RADIATION-RESISTANT FIBER OPTIC STRAIN SENSORS FOR SNS TARGET INSTRUMENTATION

DOE Office of Scientific and Technical Information (OSTI.GOV)

Blokland, Willem; Bryan, Jeff; Riemer, Bernie

2016-01-01

Measurement of stresses and strains in the mercury tar-get vessel of the Spallation Neutron Source (SNS) is important to understand the structural dynamics of the target. This work reports the development of radiation-resistant fiber optic strain sensors for the SNS target in-strumentation.

The Interstellar 7Li/6Li Ratio in the Diffuse Gas Near IC 443

NASA Astrophysics Data System (ADS)

Ritchey, A. M.; Taylor, C. J.; Federman, S. R.; Lambert, D. L.

2010-11-01

Supernova remnants are believed to be the primary acceleration sites of Galactic cosmic rays (GCR), which are essential to gas-phase interstellar chemistry since they are a major source of ionization in both diffuse and dense environments. The interaction of accelerated particles with interstellar gas will also synthesize isotopes of the light elements Li, Be, and B through the spallation of CNO nuclei (producing all stable LiBeB isotopes) and through α+α fusion (yielding 6Li and 7Li, only). Type II supernovae may provide an additional source of 7Li and 11B during core collapse through neutrino-induced spallation in the He and C shells of the progenitor star (the ν-process). However, direct observational evidence for light element synthesis resulting from cosmic-ray or neutrino-induced spallation is rare. Here, we examine 7Li/6Li isotope ratios along four lines of sight through the supernova remnant IC 443 using observations of the Li I λ6707 doublet made with the Hobby-Eberly Telescope (HET) at McDonald Observatory. The 7Li/6Li ratio in the general interstellar medium is expected to be similar to the ratio of ~12 that characterizes solar system material. A local enhancement in the cosmic-ray flux will act to lower 7Li/6Li, yielding a ratio of ~2 when cosmic rays dominate Li synthesis. Gamma-ray emission from IC 443 provides strong evidence for the interaction of cosmic rays accelerated by the remnant with the ambient atomic and molecular gas. Yet this material has also been contaminated by the ejecta of a Type II supernova, which should be enriched in 7Li. We are seeking 7Li/6Li ratios that are either higher than the solar system ratio as a result of the ν-process or lower due to cosmic-ray spallation. Since the fine structure separation of the Li I doublet is comparable to the isotope shift (~7 km s-1) and each fine structure line is further split into hyperfine components, the velocity structure along the line of sight must be carefully constrained if meaningful 7Li/6Li ratios are to be determined. In our analysis, the strongest components seen in K I and CH are used to synthesize the complex Li I profiles. We will discuss the implications of our results on 7Li/6Li (and Li/K) ratios in the context of Li production by Type II supernovae.

Los Alamos high-power proton linac designs

DOE Office of Scientific and Technical Information (OSTI.GOV)

Lawrence, G.P.

1995-10-01

Medium-energy high-power proton linear accelerators have been studied at Los Alamos as drivers for spallation neutron applications requiring large amounts of beam power. Reference designs for such accelerators are discussed, important design factors are reviewed, and issues and concern specific to this unprecedented power regime are discussed.

MW Spallation Neutron Sources for Fusion Materials Testing

ScienceCinema

Dr. Donald Rej

2018-04-18

Dr. Donald Rej of Los Alamos National Laboratory presents an overview of issues, needs, and performance gaps related to materials testing and how they are being addressed at their facility. Current projects such as the Los Alamos Neutron Science Center (LANSCE) and Matter-Radiation Interactions in Extremes (MaRIE) are also discussed.

Method and apparatus for measuring on-line failure of turbine thermal barrier coatings

DOEpatents

Zombo, Paul J.; Lemieux, Dennis; Diatzikis, Evangelos

2010-04-06

A method of remotely monitoring the radiant energy (6) emitted from a turbine component such as a turbine blade (1) having a low-reflective surface coating (3) which may be undergoing potential degradation is used to determine whether erosion, spallation, delamination, or the like, of the coating (3) is occurring.

America COMPETES Act and the FY2010 Budget

DTIC Science & Technology

2009-06-15

Outstanding Junior Investigator, Nuclear Physics Outstanding Junior Investigator, Fusion Energy Sciences Plasma Physics Junior Faculty Development...Spallation Neutron Source Instrumentation Fellowships, and the Fusion Energy Sciences Graduate Fellowships.2 If members of Congress agree with this...Nuclear Physics Outstanding Junior Investigator, Fusion Energy Sciences Plasma Physics Junior Faculty Development; Advanced Scientific Computing

Lorentz force detuning analysis of the Spallation Neutron Source (SNS) accelerating cavities.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Mitchell, R.R.; Matsumoto, K. Y.; Ciovati, G.

2001-01-01

The Spallation Neutron Source (SNS) project incorporates a superconducting radio-frequency (SRF) accelerator for the final section of the pulsed mode linac. Cavities with geometrical {beta} values of {beta}=0.61 and {beta}=0.81 are utilized in the SRF section, and are constructed out of thin-walled niobium with stiffener rings welded between the cells near the iris. The welded titanium helium vessel and tuner assembly restrains the cavity beam tubes. Cavities with {beta} values less than one have relatively steep and flat side-walls making the cavities susceptible to Lorentz force detuning. In addition, the pulsed RF induces cyclic Lorentz pressures that mechanically excite themore » cavities, producing a dynamic Lorentz force detuning different from a continuous RF system. The amplitude of the dynamic detuning for a given cavity design is a function of the mechanical damping, stiffness of the tuner/helium vessel assembly, RF pulse profile, and the RF pulse rate. This paper presents analysis and testing results to date, and indicates areas where more investigation is required.« less

HEKATE-A novel grazing incidence neutron scattering concept for the European Spallation Source.

PubMed

Glavic, Artur; Stahn, Jochen

2018-03-01

Structure and magnetism at surfaces and buried interfaces on the nanoscale can only be accessed by few techniques, one of which is grazing incidence neutron scattering. While the technique has its strongest limitation in a low signal and large background, due to the low scattering probability and need for high resolution, it can be expected that the high intensity of the European Spallation Source in Lund, Sweden, will make many more such studies possible, warranting a dedicated beamline for this technique. We present an instrument concept, Highly Extended K range And Tunable Experiment (HEKATE), for surface scattering that combines the advantages of two Selene neutron guides with unique capabilities of spatially separated distinct wavelength frames. With this combination, it is not only possible to measure large specular reflectometry ranges, even on free liquid surfaces, but also to use two independent incident beams with tunable sizes and resolutions that can be optimized for the specifics of the investigated samples. Further the instrument guide geometry is tuned for reduction of high energy particle background and only uses low to moderate supermirror coatings for high reliability and affordable cost.

HEKATE—A novel grazing incidence neutron scattering concept for the European Spallation Source

NASA Astrophysics Data System (ADS)

Glavic, Artur; Stahn, Jochen

2018-03-01

Structure and magnetism at surfaces and buried interfaces on the nanoscale can only be accessed by few techniques, one of which is grazing incidence neutron scattering. While the technique has its strongest limitation in a low signal and large background, due to the low scattering probability and need for high resolution, it can be expected that the high intensity of the European Spallation Source in Lund, Sweden, will make many more such studies possible, warranting a dedicated beamline for this technique. We present an instrument concept, Highly Extended K range And Tunable Experiment (HEKATE), for surface scattering that combines the advantages of two Selene neutron guides with unique capabilities of spatially separated distinct wavelength frames. With this combination, it is not only possible to measure large specular reflectometry ranges, even on free liquid surfaces, but also to use two independent incident beams with tunable sizes and resolutions that can be optimized for the specifics of the investigated samples. Further the instrument guide geometry is tuned for reduction of high energy particle background and only uses low to moderate supermirror coatings for high reliability and affordable cost.

Advancing Materials Science using Neutrons at Oak Ridge National Laboratory

ScienceCinema

Carpenter, John

2018-02-14

Jack Carpenter, pioneer of accelerator-based pulsed spallation neutron sources, talks about neutron science at Oak Ridge National Laboratory (ORNL) and a need for a second target station at the Spallation Neutron Source (SNS). ORNL is the Department of Energy's largest multiprogram science and energy laboratory, and is home to two scientific user facilities serving the neutron science research community: the High Flux Isotope Reactor (HFIR) and SNS. HFIR and SNS provide researchers with unmatched capabilities for understanding the structure and properties of materials, macromolecular and biological systems, and the fundamental physics of the neutron. Neutrons provide a window through which to view materials at a microscopic level that allow researchers to develop better materials and better products. Neutrons enable us to understand materials we use in everyday life. Carpenter explains the need for another station to produce long wavelength neutrons, or cold neutrons, to answer questions that are addressed only with cold neutrons. The second target station is optimized for that purpose. Modern technology depends more and more upon intimate atomic knowledge of materials, and neutrons are an ideal probe.

Candidate molten salt investigation for an accelerator driven subcritical core

NASA Astrophysics Data System (ADS)

Sooby, E.; Baty, A.; Beneš, O.; McIntyre, P.; Pogue, N.; Salanne, M.; Sattarov, A.

2013-09-01

We report a design for accelerator-driven subcritical fission in a molten salt core (ADSMS) that utilizes a fuel salt composed of NaCl and transuranic (TRU) chlorides. The ADSMS core is designed for fast neutronics (28% of neutrons >1 MeV) to optimize TRU destruction. The choice of a NaCl-based salt offers benefits for corrosion, operating temperature, and actinide solubility as compared with LiF-based fuel salts. A molecular dynamics (MD) code has been used to estimate properties of the molten salt system which are important for ADSMS design but have never been measured experimentally. Results from the MD studies are reported. Experimental measurements of fuel salt properties and studies of corrosion and radiation damage on candidate metals for the core vessel are anticipated. A special thanks is due to Prof. Paul Madden for introducing the ADSMS group to the concept of using the molten salt as the spallation target, rather than a conventional heavy metal spallation target. This feature helps to optimize this core as a Pu/TRU burner.

HIGH POWER BEAM DUMP AND TARGET / ACCELERATOR INTERFACE PROCEDURES

DOE Office of Scientific and Technical Information (OSTI.GOV)

Blokland, Willem; Plum, Michael A; Peters, Charles C

Satisfying operational procedures and limits for the beam target interface is a critical concern for high power operation at spallation neutron sources. At the Oak Ridge Spallation Neutron Source (SNS) a number of protective measures are instituted to ensure that the beam position, beam size and peak intensity are within acceptable limits at the target and high power Ring Injection Dump (RID). The high power beam dump typically handles up to 50 100 kW of beam power and its setup is complicated by the fact that there are two separate beam components simultaneously directed to the dump. The beam onmore » target is typically in the 800-1000 kW average power level, delivered in sub- s 60 Hz pulses. Setup techniques using beam measurements to quantify the beam parameters at the target and dump will be described. However, not all the instrumentation used for the setup and initial qualification is available during high power operation. Additional techniques are used to monitor the beam during high power operation to ensure the setup conditions are maintained, and these are also described.« less

Improved design of proton source and low energy beam transport line for European Spallation Source

DOE Office of Scientific and Technical Information (OSTI.GOV)

Neri, L., E-mail: neri@lns.infn.it; Celona, L.; Gammino, S.

2014-02-15

The design update of the European Spallation Source (ESS) accelerator is almost complete and the construction of the prototype of the microwave discharge ion source able to provide a proton beam current larger than 70 mA to the 3.6 MeV Radio Frequency Quadrupole (RFQ) started. The source named PS-ESS (Proton Source for ESS) was designed with a flexible magnetic system and an extraction system able to merge conservative solutions with significant advances. The ESS injector has taken advantage of recent theoretical updates and new plasma diagnostics tools developed at INFN-LNS (Laboratori Nazionali del Sud, Istituto Nazionale di Fisica Nucleare). Themore » design strategy considers the PS-ESS and the low energy beam transport line as a whole, where the proton beam behaves like an almost neutralized non-thermalized plasma. Innovative solutions have been used as hereinafter described. Thermo-mechanical optimization has been performed to withstand the chopped beam and the misaligned focused beam over the RFQ input collimator; the results are reported here.« less

Thermal barrier coating life prediction model development

NASA Technical Reports Server (NTRS)

Sheffler, K. D.; Demasi, J. T.

1985-01-01

A methodology was established to predict thermal barrier coating life in an environment simulative of that experienced by gas turbine airfoils. Specifically, work is being conducted to determine failure modes of thermal barrier coatings in the aircraft engine environment. Analytical studies coupled with appropriate physical and mechanical property determinations are being employed to derive coating life prediction model(s) on the important failure mode(s). An initial review of experimental and flight service components indicates that the predominant mode of TBC failure involves thermomechanical spallation of the ceramic coating layer. This ceramic spallation involves the formation of a dominant crack in the ceramic coating parallel to and closely adjacent to the metal-ceramic interface. Initial results from a laboratory test program designed to study the influence of various driving forces such as temperature, thermal cycle frequency, environment, and coating thickness, on ceramic coating spalling life suggest that bond coat oxidation damage at the metal-ceramic interface contributes significantly to thermomechanical cracking in the ceramic layer. Low cycle rate furnace testing in air and in argon clearly shows a dramatic increase of spalling life in the non-oxidizing environments.

Simulation of a suite of generic long-pulse neutron instruments to optimize the time structure of the European Spallation Source.

PubMed

Lefmann, Kim; Klenø, Kaspar H; Birk, Jonas Okkels; Hansen, Britt R; Holm, Sonja L; Knudsen, Erik; Lieutenant, Klaus; von Moos, Lars; Sales, Morten; Willendrup, Peter K; Andersen, Ken H

2013-05-01

We here describe the result of simulations of 15 generic neutron instruments for the long-pulsed European Spallation Source. All instruments have been simulated for 20 different settings of the source time structure, corresponding to pulse lengths between 1 ms and 2 ms; and repetition frequencies between 10 Hz and 25 Hz. The relative change in performance with time structure is given for each instrument, and an unweighted average is calculated. The performance of the instrument suite is proportional to (a) the peak flux and (b) the duty cycle to a power of approximately 0.3. This information is an important input to determining the best accelerator parameters. In addition, we find that in our simple guide systems, most neutrons reaching the sample originate from the central 3-5 cm of the moderator. This result can be used as an input in later optimization of the moderator design. We discuss the relevance and validity of defining a single figure-of-merit for a full facility and compare with evaluations of the individual instrument classes.

rf improvements for Spallation Neutron Source H- ion sourcea)

NASA Astrophysics Data System (ADS)

Kang, Y. W.; Fuja, R.; Goulding, R. H.; Hardek, T.; Lee, S.-W.; McCarthy, M. P.; Piller, M. C.; Shin, K.; Stockli, M. P.; Welton, R. F.

2010-02-01

The Spallation Neutron Source at Oak Ridge National Laboratory is ramping up the accelerated proton beam power to 1.4 MW and just reached 1 MW. The rf-driven multicusp ion source that originates from the Lawrence Berkeley National Laboratory has been delivering ˜38 mA H- beam in the linac at 60 Hz, 0.9 ms. To improve availability, a rf-driven external antenna multicusp ion source with a water-cooled ceramic aluminum nitride (AlN) plasma chamber is developed. Computer modeling and simulations have been made to analyze and optimize the rf performance of the new ion source. Operational statistics and test runs with up to 56 mA medium energy beam transport beam current identify the 2 MHz rf system as a limiting factor in the system availability and beam production. Plasma ignition system is under development by using a separate 13 MHz system. To improve the availability of the rf power system with easier maintenance, we tested a 70 kV isolation transformer for the 80 kW, 6% duty cycle 2 MHz amplifier to power the ion source from a grounded solid-state amplifier.

rf improvements for Spallation Neutron Source H- ion source.

PubMed

Kang, Y W; Fuja, R; Goulding, R H; Hardek, T; Lee, S-W; McCarthy, M P; Piller, M C; Shin, K; Stockli, M P; Welton, R F

2010-02-01

The Spallation Neutron Source at Oak Ridge National Laboratory is ramping up the accelerated proton beam power to 1.4 MW and just reached 1 MW. The rf-driven multicusp ion source that originates from the Lawrence Berkeley National Laboratory has been delivering approximately 38 mA H(-) beam in the linac at 60 Hz, 0.9 ms. To improve availability, a rf-driven external antenna multicusp ion source with a water-cooled ceramic aluminum nitride (AlN) plasma chamber is developed. Computer modeling and simulations have been made to analyze and optimize the rf performance of the new ion source. Operational statistics and test runs with up to 56 mA medium energy beam transport beam current identify the 2 MHz rf system as a limiting factor in the system availability and beam production. Plasma ignition system is under development by using a separate 13 MHz system. To improve the availability of the rf power system with easier maintenance, we tested a 70 kV isolation transformer for the 80 kW, 6% duty cycle 2 MHz amplifier to power the ion source from a grounded solid-state amplifier.

Effects of displacement damage and helium production rates on the nucleation and growth of helium bubbles - Positron annihilation spectroscopy aspects

NASA Astrophysics Data System (ADS)

Krsjak, Vladimir; Degmova, Jarmila; Sojak, Stanislav; Slugen, Vladimir

2018-02-01

Fe-12 wt% Cr model alloy samples were implanted by 250 keV He2+ ions to three different fluencies (3 × 1017, 9 × 1017 and 1.5 × 1018 cm-2) at T < 100 °C. In a depth profile manner, the implantation impact according to defined peak profile was investigated using variable energy slow positrons, with the primary focus on the 2-13 dpa region. The obtained data were compared to published data on Optifer IX steel samples [1] irradiated in the frame of a two-years irradiation program of the Swiss Spallation Neutron Source. Bi-modal defect distribution represented by two defect components in positron lifetime spectrum reveals two distinct helium bubbles growth mechanisms. While at the lower helium production rate of the spallation environment, the bubbles grow primarily by migration and coalescence, at the high production rates of helium in the implanted samples, the results indicate this growth is driven by Ostwald ripening mechanism. A competitive growth process via emission of interstitial atoms (clusters) is discussed in terms of low-temperature He implantations.

Stripper foil failure modes and cures at the Spallation Neutron Source

DOE Office of Scientific and Technical Information (OSTI.GOV)

Cousineau, Sarah M; Galambos, John D; Kim, Sang-Ho

2011-01-01

The Spallation Neutron Source comprises a 1 GeV, 1.4 MW linear accelerator followed by an accumulator ring and a liquid mercury target. To manage the beam loss caused by the $H^0$ excited states created during the $H^-$ charge exchange injection into the accumulator ring, the stripper foil is located inside one of the chicane dipoles. This has some interesting consequences that were not fully appreciated until the beam power reached about 840 kW. One consequence was sudden failure of the stripper foil system due to convoy electrons stripped from the incoming $H^-$ beam, which circled around to strike the foilmore » bracket and cause bracket failure. Another consequence is that convoy electrons can reflect back up from the electron catcher and strike the foil and bracket. An additional contributor to foil system failure is vacuum breakdown due to the charge developed on the foil by secondary electron emission. In this paper we detail these and other interesting failure mechanisms and describe the improvements we have made to mitigate them.« less

Stripper foil failure modes and cures at the Oak Rdige Spallation Neutron Source

DOE Office of Scientific and Technical Information (OSTI.GOV)

Plum, M.A.; Raparia, D.; Cousineau, S.M.

2011-03-28

The Oak Ridge Spallation Neutron Source comprises a 1 GeV, 1.5 MW linear accelerator followed by an accumulator ring and a liquid mercury target. To manage the beam loss caused by the H{sup 0} excited states created during the H{sup -} charge-exchange injection into the accumulator ring, the stripper foil is located inside one of the chicane dipoles. This has some interesting consequences that were not fully appreciated until the beam power reached about 840 kW. One consequence was sudden failure of the stripper foil system due to convoy electrons stripped from the incoming H{sup -} beam, which circled aroundmore » to strike the foil bracket and cause bracket failure. Another consequence is that convoy electrons can reflect back up from the electron catcher and strike the foil and bracket. An additional contributor to foil system failure is vacuum breakdown due to the charge developed on the foil by secondary electron emission. In this paper we detail these and other interesting failure mechanisms and describe the improvements we have made to mitigate them.« less

Spallation Neutron Source Second Target Station Integrated Systems Update

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ankner, John Francis; An, Ke; Blokland, Willem

The Spallation Neutron Source (SNS) was designed from the beginning to accommodate both an accelerator upgrade to increase the proton power and a second target station (STS). Four workshops were organized in 2013 and 2014 to identify key science areas and challenges where neutrons will play a vital role [1-4]. Participants concluded that the addition of STS to the existing ORNL neutron sources was needed to complement the strengths of High Flux Isotope Reactor (HFIR) and the SNS first target station (FTS). To address the capability gaps identified in the workshops, a study was undertaken to identify instrument concepts thatmore » could provide the required new science capabilities. The study outlined 22 instrument concepts and presented an initial science case for STS [5]. These instrument concepts formed the basis of a planning suite of instruments whose requirements determined an initial site layout and moderator selection. An STS Technical Design Report (TDR) documented the STS concept based on those choices [6]. Since issue of the TDR, the STS concept has significantly matured as described in this document.« less

The continued development of the Spallation Neutron Source external antenna H- ion sourcea)

NASA Astrophysics Data System (ADS)

Welton, R. F.; Carmichael, J.; Desai, N. J.; Fuga, R.; Goulding, R. H.; Han, B.; Kang, Y.; Lee, S. W.; Murray, S. N.; Pennisi, T.; Potter, K. G.; Santana, M.; Stockli, M. P.

2010-02-01

The U.S. Spallation Neutron Source (SNS) is an accelerator-based, pulsed neutron-scattering facility, currently in the process of ramping up neutron production. In order to ensure that the SNS will meet its operational commitments as well as provide for future facility upgrades with high reliability, we are developing a rf-driven, H- ion source based on a water-cooled, ceramic aluminum nitride (AlN) plasma chamber. To date, early versions of this source have delivered up to 42 mA to the SNS front end and unanalyzed beam currents up to ˜100 mA (60 Hz, 1 ms) to the ion source test stand. This source was operated on the SNS accelerator from February to April 2009 and produced ˜35 mA (beam current required by the ramp up plan) with availability of ˜97%. During this run several ion source failures identified reliability issues, which must be addressed before the source re-enters production: plasma ignition, antenna lifetime, magnet cooling, and cooling jacket integrity. This report discusses these issues, details proposed engineering solutions, and notes progress to date.

Recent UCN source developments at Los Alamos

DOE Office of Scientific and Technical Information (OSTI.GOV)

Seestrom, S.J.; Anaya, J.M.; Bowles, T.J.

The most intense sources of ultra cold neutrons (UCN) have bee built at reactors where the high average thermal neutron flux can overcome the low UCN production rate to achieve usable densities of UCN. At spallation neutron sources the average flux available is much lower than at a reactor, though the peak flux can be comparable or higher. The authors have built a UCN source that attempts to take advantage of the high peak flux available at the short pulse spallation neutron source at the Los Alamos Neutron Science Center (LANSCE) to generate a useful number of UCN. In themore » source UCN are produced by Doppler-shifted Bragg scattering of neutrons to convert 400-m/s neutrons down into the UCN regime. This source was initially tested in 1996 and various improvements were made based on the results of the 1996 running. These improvements were implemented and tested in 1997. In sections 2 and 3 they discuss the improvements that have been made and the resulting source performance. Recently an even more interesting concept was put forward by Serebrov et al. This involves combining a solid Deuterium UCN source, previously studied by Serebrov et al., with a pulsed spallation source to achieve world record UCN densities. They have initiated a program of calculations and measurements aimed at verifying the solid Deuterium UCN source concept. The approach has been to develop an analytical capability, combine with Monte Carlo calculations of neutron production, and perform benchmark experiments to verify the validity of the calculations. Based on the calculations and measurements they plan to test a modified version of the Serebrov UCN factory. They estimate that they could produce over 1,000 UCN/cc in a 15 liter volume, using 1 {micro}amp of 800 MeV protons for two seconds every 500 seconds. They will discuss the result UCN production measurements in section 4.« less

Proceedings of the international workshop on the technology and thermal hydraulics of heavy liquid metals (Hg, Pb, Bi, and their eutectics)

DOE Office of Scientific and Technical Information (OSTI.GOV)

Appleton, B.R.; Bauer, G.S.

1996-06-01

The International Workshop on the Technology and Thermal Hydraulics of Heavy Liquid Metals (Schruns Workshop) was organized to assess the R&D and technology problems associated with designing and building a heavy liquid metal target for a spallation neutron source. The European scientific community is completing a feasibility study for a future, accelerator-based, pulsed spallation neutron source that would deliver a beam power of 5 megawatts (MW) to a target. They have concluded that a liquid metal target is preferable to conventional solid targets for handling the extreme radiation environments, high heat loads, and pulsed power. Similarly, the ORNL has beenmore » funded by the DOE to design a high-power, pulsed spallation neutron source that would begin operation at about 1 MW but that could be upgraded to significantly higher powers in the future. Again, the most feasible target design appears to be a liquid metal target. Since the expertise needed to consider these problems resides in a number of disparate disciplines not normally covered by existing conferences, this workshop was organized to bring a small number of scientists and engineers together to assess the opportunities for building such a target. The objectives and goals of the Schruns Workshop were to: review and share existing information on the science and technology of heavy liquid metal systems. Evaluate the opportunities and limitations of materials compatibility, thermal hydraulics and heat transfer, chemical reactions, corrosion, radiation effects, liquid-gas mixtures, systems designs, and circuit components for a heavy liquid metal target. Establish the critical R & D and technology that is necessary to construct a liquid metal target. Explore opportunities for cooperative R & D among members of the international community that could expedite results, and share expertise and resources. Selected papers are indexed separately for inclusion in the Energy Science and Technology Database.« less

Thermal-hydraulic simulation of mercury target concepts for a pulsed spallation neutron source

DOE Office of Scientific and Technical Information (OSTI.GOV)

Siman-Tov, M.; Wendel, M.; Haines, J.

1996-06-01

The Oak Ridge Spallation Neutron Source (ORSNS) is a high-power, accelerator-based pulsed spallation neutron source being designed by a multi-laboratory team led by Oak Ridge National Laboratory to achieve very high fluxes of neutrons for scientific experiments. The ORSNS is projected to have a 1 MW proton beam upgradable to 5 MW. About 60% of the beam power (1-5 MW, 17-83 kJ/pulse in 0.5 microsec at 60 cps) is deposited in the liquid metal (mercury) target having the dimensions of 65x30x10 cm (about 19.5 liter). Peak steady state power density is about 150 and 785 MW/m{sup 3} for 1 MWmore » and 5 MW beam respectively, whereas peak pulsed power density is as high as 5.2 and 26.1 GW/m{sup 3}, respectively. The peak pulse temperature rise rate is 14 million C/s (for 5 MW beam) whereas the total pulse temperature rise is only 7 C. In addition to thermal shock and materials compatibility, key feasibility issues for the target are related to its thermal-hydraulic performance. This includes proper flow distribution, flow reversals, possible {open_quotes}hot spots{close_quotes} and the challenge of mitigating the effects of thermal shock through possible injection of helium bubbles throughout the mercury volume or other concepts. The general computational fluid dynamics (CFD) code CFDS-FLOW3D was used to simulate the thermal and flow distribution in three preliminary concepts of the mercury target. Very initial CFD simulation of He bubbles injection demonstrates some potential for simulating behavior of He bubbles in flowing mercury. Much study and development will be required to be able to `predict`, even in a crude way, such a complex phenomena. Future direction in both design and R&D is outlined.« less

Neutron Collar Evolution and Fresh PWR Assembly Measurements with a New Fast Neutron Passive Collar

DOE Office of Scientific and Technical Information (OSTI.GOV)

Menlove, Howard Olsen; Geist, William H.; Root, Margaret A.

The passive neutron collar approach removes the effect of poison rods when using a 1mm Gd liner. This project sets out to solve the following challenges: BWR fuel assemblies have less mass and less neutron multiplication than PWR; and effective removal of cosmic ray spallation neutron bursts needed via QC tests.

Corrigendum to "Fundamental neutron physics beamline at the spallation neutron source at ORNL" [Nucl. Instrum. Methods Phys. Res. A 773 (2015) 45-51

NASA Astrophysics Data System (ADS)

Fomin, N.; Greene, G. L.; Allen, R. R.; Cianciolo, V.; Crawford, C.; Ito, T. M.; Huffman, P. R.; Iverson, E. B.; Mahurin, R.; Snow, W. M.

2015-07-01

The authors regret that there was an error in the author list of the original publication. The name of author Dr. Ito was misspelled. The correct author list is as above. The authors would like to apologise for any inconvenience caused.

Preface

NASA Astrophysics Data System (ADS)

Dai, Yong

2016-01-01

The Twelfth International Workshop on Spallation Materials Technology (IWSMT-12) was held on October 20 to 23, 2014, in Bregenz, Austria. The meeting was organized by the Paul Scherrer Institute (Switzerland), in cooperation with the Belgian Nuclear Research Centre, the Institute of High Energy Physics of Chinese Academy of Sciences, Japan Atomic Energy Agency, Los Alamos National Laboratory (USA) and Oak Ridge National Laboratory (USA).

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kashiwa, Bryan Andrew; Hull, Lawrence Mark

Highlights of recent phenomenological studies of metal failure are given. Failure leading to spallation and fragmentation are typically of interest. The current ‘best model’ includes the following; a full history stress in tension; nucleation initiating dynamic relaxation; toward a tensile yield function; failure dependent on strain, strain rate, and temperature; a mean-preserving ‘macrodefect’ is introduced when failure occurs in tension; and multifield theoretical refinements

DOE Office of Scientific and Technical Information (OSTI.GOV)

Abudureyimu, Reheman; Huang, Chunning; Liu, Yun

We report on a first experimental demonstration of locking a doubly-resonant Fabry-Perot cavity to burst-mode picosecond ultraviolet (UV) pulses by using a temperature controlled dispersion compensation method. This technique will eventually enable the intra cavity power enhancement of burst-mode 402.5MHz/50ps UV laser pulses with a MW level peak power required for the laser assisted H- beam stripping experiment at the Spallation Neutron Source.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Hurd, Alan J; Rhyne, James J; Lewis, Paul S

This two-day workshop will engage the international neutron scattering community to vet and improve the Lujan Center Strategic Plan 2007-2013 (SP07). Sponsored by the LANL SC Program Office and the University of California, the workshop will be hosted by LANSCE Professor Sunny Sinha (UCSD). Endorsement by the Spallation Neutron Source will be requested. The discussion will focus on the role that the Lujan Center will play in the national neutron scattering landscape assuming full utilization of beamlines, a refurbished LANSCE, and a 1.4-MW SNS. Because the Lujan Strategic Plan is intended to set the stage for the Signature Facility eramore » at LANSCE, there will be some discussion of the long-pulse spallation source at Los Alamos. Breakout groups will cover several new instrument concepts, upgrades to present instruments, expanded sample environment capabilities, and a look to the future. The workshop is in keeping with a request by BES to update the Lujan strategic plan in coordination with the SNS and the broader neutron community. Workshop invitees will be drawn from the LANSCE User Group and a broad cross section of the US, European, and Pacific Rim neutron scattering research communities.« less

Assessment of In Situ Time Resolved Shock Experiments at Synchrotron Light Sources*

NASA Astrophysics Data System (ADS)

Belak, J.; Ilavsky, J.; Hessler, J. P.

2005-07-01

Prior to fielding in situ time resolved experiments of shock wave loading at the Advanced Photon Source, we have performed feasibility experiments assessing a single photon bunch. Using single and poly-crystal Al, Ti, V and Cu shock to incipient spallation on the gas gun, samples were prepared from slices normal to the spall plane of thickness 100-500 microns. In addition, single crystal Al of thickness 500 microns was shocked to incipient spallation and soft recovered using the LLNL e-gun mini-flyer system. The e-gun mini-flyer impacts the sample target producing a 10's ns flat-top shock transient. Here, we present results for imaging, small-angle scattering (SAS), and diffraction. In particular, there is little SAS away from the spall plane and significant SAS at the spall plane, demonstrating the presence of sub-micron voids. * Use of the Advanced Photon Source was supported by the U. S. Department of Energy, Office of Science, Office of Basic Energy Sciences, under Contract No. W-31-109-Eng-38 and work performed under the auspices of the U.S. Department of Energy by University of California, Lawrence Livermore National Laboratory under Contract W-7405-Eng-48.

Characterization of irradiated AISI 316L stainless steel disks removed from the Spallation Neutron Source

DOE Office of Scientific and Technical Information (OSTI.GOV)

Vevera, Bradley J; Hyres, James W; McClintock, David A

2014-01-01

Irradiated AISI 316L stainless steel disks were removed from the Spallation Neutron Source (SNS) for post-irradiation examination (PIE) to assess mechanical property changes due to radiation damage and erosion of the target vessel. Topics reviewed include high-resolution photography of the disk specimens, cleaning to remove mercury (Hg) residue and surface oxides, profile mapping of cavitation pits using high frequency ultrasonic testing (UT), high-resolution surface replication, and machining of test specimens using wire electrical discharge machining (EDM), tensile testing, Rockwell Superficial hardness testing, Vickers microhardness testing, scanning electron microscopy (SEM), and energy dispersive spectroscopy (EDS). The effectiveness of the cleaning proceduremore » was evident in the pre- and post-cleaning photography and permitted accurate placement of the test specimens on the disks. Due to the limited amount of material available and the unique geometry of the disks, machine fixturing and test specimen design were critical aspects of this work. Multiple designs were considered and refined during mock-up test runs on unirradiated disks. The techniques used to successfully machine and test the various specimens will be presented along with a summary of important findings from the laboratory examinations.« less

Aerial Neutron Detection of Cosmic-Ray Interactions with the Earth's Surface

DOE Office of Scientific and Technical Information (OSTI.GOV)

Richard Maurer

2008-09-18

We have demonstrated the ability to measure the neutron flux produced by the cosmic-ray interaction with nuclei in the ground surface using aerial neutron detection. High energy cosmic-rays (primarily muons with GeV energies) interact with the nuclei in the ground surface and produce energetic neutrons via spallation. At the air-surface interface, the neutrons produced by spallation will either scatter within the surface material, become thermalized and reabsorbed, or be emitted into the air. The mean free path of energetic neutrons in air can be hundreds of feet as opposed to a few feet in dense materials. As such, the fluxmore » of neutrons escaping into the air provides a measure of the surface nuclei composition. It has been demonstrated that this effect can be measured at long range using neutron detectors on low flying helicopters. Radiological survey measurements conducted at Government Wash in Las Vegas, Nevada, have shown that the neutron background from the cosmic-soil interactions is repeatable and directly correlated to the geological data. Government Wash has a very unique geology, spanning a wide variety of nuclide mixtures and formations. The results of the preliminary measurements are presented.« less

The characteristics of void distribution in spalled high purity copper cylinder under sweeping detonation

NASA Astrophysics Data System (ADS)

Yang, Yang; Jiang, Zhi; Chen, Jixinog; Guo, Zhaoliang; Tang, Tiegang; Hu, Haibo

2018-03-01

The effects of different peak compression stresses (2-5 GPa) on the spallation behaviour of high purity copper cylinder during sweeping detonation were examined by Electron Backscatter Diffraction Microscopy, Doppler Pins System and Optical Microscopy techniques. The velocity history of inner surface and the characteristics of void distributions in spalled copper cylinder were investigated. The results indicated that the spall strength of copper in these experiments was less than that revealed in previous reports concerning plate impact loading. The geometry of cylindrical copper and the obliquity of incident shock during sweeping detonation may be the main reasons. Different loading stresses seemed to be responsible for the characteristics of the resultant damage fields, and the maximum damage degree increased with increasing shock stress. Spall planes in different cross-sections of sample loaded with the same shock stress of 3.29 GPa were found, and the distance from the initiation end has little effect on the maximum damage degree (the maximum damage range from 12 to 14%), which means that the spallation behaviour was stable along the direction parallel to the detonation propagation direction under the same shock stress.

Thermal barrier coating life prediction model development

NASA Technical Reports Server (NTRS)

Demasi, J. T.

1986-01-01

A methodology is established to predict thermal barrier coating life in a environment similar to that experienced by gas turbine airfoils. Experiments were conducted to determine failure modes of the thermal barrier coating. Analytical studies were employed to derive a life prediction model. A review of experimental and flight service components as well as laboratory post evaluations indicates that the predominant mode of TBC failure involves thermomechanical spallation of the ceramic coating layer. This ceramic spallation involves the formation of a dominant crack in the ceramic coating parallel to and closely adjacent to the topologically complex metal ceramic interface. This mechanical failure mode clearly is influenced by thermal exposure effects as shown in experiments conducted to study thermal pre-exposure and thermal cycle-rate effects. The preliminary life prediction model developed focuses on the two major damage modes identified in the critical experiments tasks. The first of these involves a mechanical driving force, resulting from cyclic strains and stresses caused by thermally induced and externally imposed mechanical loads. The second is an environmental driving force based on experimental results, and is believed to be related to bond coat oxidation. It is also believed that the growth of this oxide scale influences the intensity of the mechanical driving force.

Spallation Neutron Source Materials Studies

NASA Astrophysics Data System (ADS)

Sommer, W. F.

1998-04-01

Operation of accelerator facilities such as Los Alamos Neutron Science Center (LANSCE), ISIS at Rutherford Appleton Laboratory, the Swiss Institute Neutron Source (SINQ) at Paul Scherrer Institute, and others has provided valuable information on materials performance in high energy particle beams and high energy neutron environments. The Accelerator Production of Tritium (APT) project is sponsoring an extensive series of tests on the effect of spallation neutron source environments to physical and mechanical properties of candidate materials such as nickel-based alloys, stainless steel alloys, aluminum alloys and solid target materials such as tungsten. Measurements of corrosion rates of these candidate materials during irradiation and while in contact with flowing coolant water are being made. The APT tests use the irradiation facility in the beam stop area of the LANSCE accelerator using 800 MeV protons as well as the neutron flux-spectrum generated as these protons interact with targets. The initial irradiations were completed in summer 1997, exposing materials to a fluence approaching 4-6 x 10^21 protons/cm^2. Sample retrieval is now underway. Mechanical properties measurements are being conducted at several laboratories. Studies on components used in service have also been initiated.

Electrical Engineering in Los Alamos Neutron Science Center Accelerator

DOE Office of Scientific and Technical Information (OSTI.GOV)

Silva, Michael James

The field of electrical engineering plays a significant role in particle accelerator design and operations. Los Alamos National Laboratories LANSCE facility utilizes the electrical energy concepts of power distribution, plasma generation, radio frequency energy, electrostatic acceleration, signals and diagnostics. The culmination of these fields produces a machine of incredible potential with uses such as isotope production, neutron spallation, neutron imaging and particle analysis. The key isotope produced in LANSCE isotope production facility is Strontium-82 which is utilized for medical uses such as cancer treatment and positron emission tomography also known as PET scans. Neutron spallation is one of the verymore » few methods used to produce neutrons for scientific research the other methods are natural decay of transuranic elements from nuclear reactors. Accelerator produce neutrons by accelerating charged particles into neutron dense elements such as tungsten imparting a neutral particle with kinetic energy, this has the benefit of producing a large number of neutrons as well as minimizing the waste generated. Utilizing the accelerator scientist can gain an understanding of how various particles behave and interact with matter to better understand the natural laws of physics and the universe around us.« less

Mechanochemical mechanism for reaction of aluminium nano- and micrometre-scale particles.

PubMed

Levitas, Valery I

2013-11-28

A recently suggested melt-dispersion mechanism (MDM) for fast reaction of aluminium (Al) nano- and a few micrometre-scale particles during fast heating is reviewed. Volume expansion of 6% during Al melting produces pressure of several GPa in a core and tensile hoop stresses of 10 GPa in an oxide shell. Such stresses cause dynamic fracture and spallation of the shell. After spallation, an unloading wave propagates to the centre of the particle and creates a tensile pressure of 3-8 GPa. Such a tensile pressure exceeds the cavitation strength of liquid Al and disperses the melt into small, bare clusters (fragments) that fly at a high velocity. Reaction of the clusters is not limited by diffusion through a pre-existing oxide shell. Some theoretical and experimental results related to the MDM are presented. Various theoretical predictions based on the MDM are in good qualitative and quantitative agreement with experiments, which resolves some basic puzzles in combustion of Al particles. Methods to control and improve reactivity of Al particles are formulated, which are exactly opposite to the current trends based on diffusion mechanism. Some of these suggestions have experimental confirmation.

New sources and instrumentation for neutron science

NASA Astrophysics Data System (ADS)

Gil, Alina

2011-04-01

Neutron-scattering research has a lot to do with our everyday lives. Things like medicine, food, electronics, cars and airplanes have all been improved by neutron-scattering research. Neutron research also helps scientists improve materials used in a multitude of different products, such as high-temperature superconductors, powerful lightweight magnets, stronger, lighter plastic products etc. Neutron scattering is one of the most effective ways to obtain information on both, the structure and the dynamics of condensed matter. Most of the world's neutron sources were built decades ago, and although the uses and demand for neutrons have increased throughout the years, few new sources have been built. The new construction, accelerator-based neutron source, the spallation source will provide the most intense pulsed neutron beams in the world for scientific research and industrial development. In this paper it will be described what neutrons are and what unique properties make them useful for science, how spallation source is designed to produce neutron beams and the experimental instruments that will use those beams. Finally, it will be described how past neutron research has affected our everyday lives and what we might expect from the most exciting future applications.

RF H-minus ion source development in China spallation neutron source

NASA Astrophysics Data System (ADS)

Chen, W.; Ouyang, H.; Xiao, Y.; Liu, S.; Lü, Y.; Cao, X.; Huang, T.; Xue, K.

2017-08-01

China Spallation Neutron Source (CSNS) phase-I project currently uses a Penning surface plasma H- ion source, which has a life time of several weeks with occasional sparks between high voltage electrodes. To extend the life time of the ion source and prepare for the CSNS phase-II, we are trying to develop a RF negative hydrogen ion source with external antenna. The configuration of the source is similar to the DESY external antenna ion source and SNS ion source. However several changes are made to improve the stability and the life time. Firstly, Si3N4 ceramic with high thermal shock resistance, and high thermal conductivity is used for plasma chamber, which can endure an average power of 2000W. Secondly, the water-cooled antenna is brazed on the chamber to improve the energy efficiency. Thirdly, cesium is injected directly to the plasma chamber if necessary, to simplify the design of the converter and the extraction. Area of stainless steel exposed to plasma is minimized to reduce the sputtering and degassing. Instead Mo, Ta, and Pt coated materials are used to face the plasma, which makes the self-cleaning of the source possible.

Characterization of the high-energy neutron beam of the PRISMA beamline using a diamond detector

NASA Astrophysics Data System (ADS)

Cazzaniga, C.; Frost, C. D.; Minniti, T.; Schooneveld, E.; Perelli Cippo, E.; Tardocchi, M.; Rebai, M.; Gorini, G.

2016-07-01

The high-energy neutron component (En > 10 MeV) of the neutron spectrum of PRISMA, a beam-line at the ISIS spallation source, has been characterized for the first time. Neutron measurements using a Single-crystal Diamond Detector at a short-pulse source are obtained by a combination of pulse height and time of flight analysis. An XY scan provides a 2D map of the high-energy neutron beam which has a diameter of about 40 mm. The high neutron flux, that has been found to be (3.8 ± 0.7) · 105 cm-2s-1 for En > 10 MeV in the centre, opens up for a possible application of the beam-line as a high-energy neutron irradiation position. Results are of interest for the development of the ChipIR beam-line, which will feature an atmospheric-like neutron spectrum for chip irradiation experiment. Furthermore, these results demonstrate that diamond detectors can be used at spallation sources to investigate the transport of high-energy neutrons down instruments which is of interest in general to designers as high-energy neutrons are a source of background in thermal beamlines.

The National Spallation Neutron Source Target Station.

NASA Astrophysics Data System (ADS)

Gabriel, T. A.

1997-05-01

The technologies that are being utilized to design and build a state-of-the-art high powered (>= 1 MW), short pulsed (<= 1 μsec), and reliable spallation neutron source target station are discussed. The protons which directly and indirectly produce the neutrons will be obtained from a 1 GeV proton accelerator composed of an ion gun, rfq, linac, and storage ring. Many scientific and technical disciplines are required to produce a successful target station. These disciplines include engineering, remote handling, neutronics, materials, thermal hydraulics, shock analysis, etc. In the areas of engineering and remote handling special emphasis is being given to rapid and efficient assembly and disassembly of critical parts of the target station. In the neutronics area, emphasis is being given to neutron yield and pulse optimization from the moderators, and heating and activation rates throughout the station. Development of structural materials to withstand aggressive radiation environments and that are compatible with other materials is also an important area. Thermal hydraulics and shock analysis are being closely studied since large amounts of energy are being deposited in small volumes in relatively short time periods (< 1 μsec). These areas will be expanded upon in the paper.

Thermal Cycling and High-Temperature Corrosion Tests of Rare Earth Silicate Environmental Barrier Coatings

NASA Astrophysics Data System (ADS)

Darthout, Émilien; Gitzhofer, François

2017-12-01

Lutetium and yttrium silicates, enriched with an additional secondary zirconia phase, environmental barrier coatings were synthesized by the solution precursor plasma spraying process on silicon carbide substrates. A custom-made oven was designed for thermal cycling and water vapor corrosion testing. The oven can test four specimens simultaneously and allows to evaluate environmental barrier performances under similar corrosion kinetics compared to turbine engines. Coatings structural evolution has been observed by SEM on the polished cross sections, and phase composition has been analyzed by XRD. All coatings have been thermally cycled between 1300 °C and the ambient temperature, without spallation, due to their porosity and the presence of additional secondary phase which increases the thermal cycling resistance. During water vapor exposure at 1200 °C, rare earth disilicates showed a good stability, which is contradictory with the literature, due to impurities—such as Si- and Al-hydroxides—in the water vapor jets. The presence of vertical cracks allowed the water vapor to reach the substrate and then to corrode it. It has been observed that thin vertical cracks induced some spallation after 24 h of corrosion.

General-purpose readout electronics for white neutron source at China Spallation Neutron Source

NASA Astrophysics Data System (ADS)

Wang, Q.; Cao, P.; Qi, X.; Yu, T.; Ji, X.; Xie, L.; An, Q.

2018-01-01

The under-construction White Neutron Source (WNS) at China Spallation Neutron Source is a facility for accurate measurements of neutron-induced cross section. Seven spectrometers are planned at WNS. As the physical objectives of each spectrometer are different, the requirements for readout electronics are not the same. In order to simplify the development of the readout electronics, this paper presents a general method for detector signal readout. This method has advantages of expansibility and flexibility, which makes it adaptable to most detectors at WNS. In the WNS general-purpose readout electronics, signals from any kinds of detectors are conditioned by a dedicated signal conditioning module corresponding to this detector, and then digitized by a common waveform digitizer with high speed and high precision (1 GSPS at 12-bit) to obtain the full waveform data. The waveform digitizer uses a field programmable gate array chip to process the data stream and trigger information in real time. PXI Express platform is used to support the functionalities of data readout, clock distribution, and trigger information exchange between digitizers and trigger modules. Test results show that the performance of the WNS general-purpose readout electronics can meet the requirements of the WNS spectrometers.

In-situ structural integrity evaluation for high-power pulsed spallation neutron source - Effects of cavitation damage on structural vibration

NASA Astrophysics Data System (ADS)

Wan, Tao; Naoe, Takashi; Futakawa, Masatoshi

2016-01-01

A double-wall structure mercury target will be installed at the high-power pulsed spallation neutron source in the Japan Proton Accelerator Research Complex (J-PARC). Cavitation damage on the inner wall is an important factor governing the lifetime of the target-vessel. To monitor the structural integrity of the target vessel, displacement velocity at a point on the outer surface of the target vessel is measured using a laser Doppler vibrometer (LDV). The measured signals can be used for evaluating the damage inside the target vessel because of cyclic loading and cavitation bubble collapse caused by pulsed-beam induced pressure waves. The wavelet differential analysis (WDA) was applied to reveal the effects of the damage on vibrational cycling. To reduce the effects of noise superimposed on the vibration signals on the WDA results, analysis of variance (ANOVA) and analysis of covariance (ANCOVA), statistical methods were applied. Results from laboratory experiments, numerical simulation results with random noise added, and target vessel field data were analyzed by the WDA and the statistical methods. The analyses demonstrated that the established in-situ diagnostic technique can be used to effectively evaluate the structural response of the target vessel.

Sulfur and Moisture Effects on Alumina Scale and TBC Spallation

NASA Technical Reports Server (NTRS)

Smialek, James L.

2007-01-01

It has been well established that a few ppmw sulfur impurity may segregate to the interface of thermally grown alumina scales and the underlying substrate, resulting in bond degradation and premature spallation. This has been shown for NiAl and NiCrAl-based alloys, bare single crystal superalloys, or coated superalloys. The role of reactive elements (especially Y) has been to getter the sulfur in the bulk and preclude interfacial segregation. Pt additions are also very beneficial, however a similar thermodynamic explanation does not apply. The purpose of the present discussion is to highlight some observations of these effects on Rene'142, Rene'N5, PWA1480, and PWA1484. For PWA1480, we have mapped cyclic oxidation and spallation in terms of potential sulfur interfacial layers and found that a cumulative amount of about one monolayer is sufficient to degrade long term adhesion. Depending on substrate thickness, optimum performance occurs if sulfur is reduced below about 0.2-0.5 ppmw. This is accomplished in the laboratory by hydrogen annealing or commercially by melt-fluxing. Excellent 1150 C cyclic oxidation is thus demonstrated for desulfurized Rene'142, Rene'N5, and PWA1484. Alternatively, a series of N5 alloys provided by GE-AE have shown that as little as 15 ppmw of Y dopant was effective in providing remarkable scale adhesion. In support of a Y-S gettering mechanism, hydrogen annealing was unable to desulfurize these alloys from their initial level of 5 ppmw S. This impurity and critical doping level corresponds closely to YS or Y2S3 stoichiometry. In many cases, Y-doped alloys or alloys with marginal sulfur levels exhibit an oxidative sensitivity to the ambient humidity called Moisture-Induced Delayed Spallation (MIDS). After substantial scale growth, coupled with damage from repeated cycling, cold samples may spall after a period of time, breathing on them, or immersing them in water. While stress corrosion arguments may apply, we propose that the underlying cause is related to a hydrogen embrittlement reaction: Al alloy + 3 H2O = Al(OH)3 + 3H(+) + 3e(-). This mechanism is derived from an analogous moisture-induced hydrogen embrittlement mechanism originally shown for Ni3Al and FeAl intermetallics. Consequently, a cathodic hydrogen charging technique was used to demonstrate that electrolytic de-scaling occurs for these otherwise adherent alumina scales formed on Y-doped Rene'N5, in support of hydrogen effects. Finally, some TBC observations are discussed in light of all of the above. Plasma sprayed 8YSZ coatings, produced on PWA1484 without a bond coat, were found to survive more than 1000 1-hr cycles at 1100 C when desulfurized to below 0.1 ppmw. At higher sulfur (1.2 ppmw) levels, moisture sensitivity and delayed TBC failure, referred to as Desk Top Spallation, occurred at just 200 hr. Despite a large degree of scatter, a factor of 5 in life improvement is indicated for desulfurized samples in cyclic furnace tests, confirming the beneficial effect of low sulfur alloys on model TBC systems. (DTS and moisture effects are also observed on commercially applied PVD 7YSZ coatings on Rene'N5+Y with Pt-aluminide bond coats). These types of catastrophic failure were subverted on the model system by segmenting the substrate into a network of 0.010 high ribs, spaced in. apart, prior to plasma spraying. No failures occurred after 1000 cycles at 1150 C or after 2000 cycles at 1100 C, even after water immersion. The benefit is described in terms of elasticity models and a critical buckling stress.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Carpenter, J.M.

This paper reviews the early history of pulsed spallation neutron source development at Argonne and provides an overview of existing sources world wide. A number of proposals for machines more powerful than currently exist are under development, which are briefly described. The author reviews the status of the Intense Pulsed Neutron Source, its instrumentation, and its user program, and provides a few examples of applications in fundamental condensed matter physics, materials science and technology.

Data processing workflow for time of flight polarized neutrons inelastic measurements

DOE PAGES

Savici, Andrei T.; Zaliznyak, Igor A.; Ovidiu Garlea, V.; ...

2017-06-01

We discuss the data processing workflow for polarized neutron scattering measurements performed at HYSPEC spectrometer at the Spallation Neutron Source, Oak Ridge National Laboratory. The effects of the focusing Heusler crystal polarizer and the wide-angle supermirror transmission polarization analyzer are added to the data processing flow of the non-polarized case. The implementation is done using the Mantid software package.

Single-crystal diffraction instrument TriCS at SINQ

NASA Astrophysics Data System (ADS)

Schefer, J.; Könnecke, M.; Murasik, A.; Czopnik, A.; Strässle, Th; Keller, P.; Schlumpf, N.

2000-03-01

The single-crystal diffractometer TriCS at the Swiss Continuous Spallation Source (SINQ) is presently in the commissioning phase. A two-dimensional wire detector produced by EMBL was delivered in March 1999. The instrument is presently tested with a single detector. First measurements on magnetic structures have been performed. The instrument is remotely controlled using JAVA-based software and a UNIX DEC-α host computer.

Source Physics Experiment: Research in Support of Verification and Nonproliferation

DTIC Science & Technology

2011-09-01

designed to provide a carefully controlled seismic and strong motion data set from buried explosions at the Nevada National Security Site (NNSS). The...deposition partitioned into internal (heat and plastic strain) and kinetic (e.g., radiated seismic ) energy, giving more confidence in predicted free...ample information to study dry and water-saturated fractures, local lithology and topography on the radiated seismic wavefield. Spallation on

Polarized neutron scattering on HYSPEC: the HYbrid SPECtrometer at SNS

DOE PAGES

Zaliznyak, Igor A.; Savici, Andrei T.; Ovidiu Garlea, V.; ...

2017-06-20

Here, we describe some of the first polarized neutron scattering measurements performed at HYSPEC [1-4] spectrometer at the Spallation Neutron Source, Oak Ridge National Laboratory. Furthermore, we discuss details of the instrument setup and the experimental procedures in the mode with full polarization analysis. Examples of polarized neutron diffraction and polarized inelastic neutron data obtained on single crystal samples are presented.

Galactic cosmic ray composition

NASA Technical Reports Server (NTRS)

Meyer, J. P.

1986-01-01

An assessment is given of the galactic cosmic ray source (GCRS) elemental composition and its correlation with first ionization potential. The isotopic composition of heavy nuclei; spallation cross sections; energy spectra of primary nuclei; electrons; positrons; local galactic reference abundances; comparison of solar energetic particles and solar coronal compositions; the hydrogen; lead; nitrogen; helium; and germanium deficiency problems; and the excess of elements are among the topics covered.

Numerical simulations of stripping effects in high-intensity hydrogen ion linacs

DOE Office of Scientific and Technical Information (OSTI.GOV)

Carneiro, J.-P.; /Fermilab; Mustapha, B.

2008-12-01

Numerical simulations of H{sup -} stripping losses from blackbody radiation, electromagnetic fields, and residual gas have been implemented into the beam dynamics code TRACK. Estimates of the stripping losses along two high-intensity H{sup -} linacs are presented: the Spallation Neutron Source linac currently being operated at Oak Ridge National Laboratory and an 8 GeV superconducting linac currently being designed at Fermi National Accelerator Laboratory.

Major uncertainties influencing entry probe heat shield design

NASA Technical Reports Server (NTRS)

Congdon, W.

1974-01-01

Factors influencing the design of an outer planet probe heat shield are discussed. Major factors included are: uncertainties in composition and scale height of the planet atmospheres; the augmentation/attenuation of entry heating by ablation products requires more computer study and testing; carbon heat shields, especially carbon phenolic, possessing improved resistance to spallation need developing; and white silica reflecting heat shields with improved resistance to bulk vitrification need further developing.

New precision measurements of free neutron beta decay with cold neutrons

DOE PAGES

Baeßler, Stefan; Bowman, James David; Penttilä, Seppo I.; ...

2014-10-14

Precision measurements in free neutron beta decay serve to determine the coupling constants of beta decay, and offer several stringent tests of the standard model. This study describes the free neutron beta decay program planned for the Fundamental Physics Beamline at the Spallation Neutron Source at Oak Ridge National Laboratory, and finally puts it into the context of other recent and planned measurements of neutron beta decay observables.

Isotopic studies in returned lunar samples

NASA Technical Reports Server (NTRS)

Alexander, E. C., Jr.

1971-01-01

Analysis of lunar soil samples returned by Apollo 11 and 12 flights are discussed. Isotopic studies of the rare gases from Apollo 11 flight lunar samples are presented. The lunar soil analyses indicated the following: (1) high concentrations of solar wind rare gases, (2) isotopic match between solar wind gases and gas components in gas-rich meteorites, and (3) rare gases attributable to spallation reactions induced in heavier nuclides by cosmic ray particles.

Superconducting Prototype Cavities for the Spallation Neutron Source (SNS) Project

DOE Office of Scientific and Technical Information (OSTI.GOV)

Peter Kneisel; John Brawley; Richard Bundy

2001-06-01

The Spallation Neutron Source project includes a superconducting linac section in the energy range from 192 MeV to 1000 MeV. For this energy range two types of cavities are needed with geometrical beta - values of beta = 0.61 and beta = 0.81. An aggressive cavity prototyping program is being pursued at Jlab, which calls for fabricating and testing of four beta = 0.61 cavities and two beta = 0.81 cavities. Both types consist of six cells made from high purity niobium and feature one HOM coupler of the TESLA type on each beam pipe and a port for amore » high power coaxial input coupler. Three of the four beta = 0.61 cavities will be used for a cryomodule test at the end of the year 2001. At this time two cavities of each type have been fabricated and the first tests on the beta = 0.61 cavity exceeded the design values for gradient and Q - value: Eacc = 10.3 MV/m and Q = 6.5 x 10{sup 9} at 2.1K. This paper will describe the cavity design with respect to electrical and mechanical features, the fabrication efforts and the results obtained with the different cavities existing at the time of the conference.« less

Thermostructural Evaluation of Joggle Region on the Shuttle Orbiter's Wing Leading Edge

NASA Technical Reports Server (NTRS)

Walker, Sandra P.; Warren, Jerry E.

2012-01-01

An investigation was initiated to determine the cause of coating spallation occurring on the Shuttle Orbiter's wing leading edge panels in the slip-side joggle region. The coating spallation events were observed, post flight, on differing panels on different missions. As part of the investigation, the high re-entry heating occurring on the joggles was considered here as a possible cause. Thus, a thermostructural evaluation was conducted to determine the detailed state-of-stress in the joggle region during re-entry and the feasibility of a laboratory test on a local joggle specimen to replicate this state-of-stress. A detailed three-dimensional finite element model of a panel slip-side joggle region was developed. Parametric and sensitivity studies revealed significant stresses occur in the joggle during peak heating. A critical interlaminar normal stress concentration was predicted in the substrate at the coating interface and was confined to the curved joggle region. Specifically, the high interlaminar normal stress is identified to be the cause for the occurrence of failure in the form of local subsurface material separation occurring in the slip-side joggle. The predicted critical stresses are coincident with material separations that had been observed with microscopy in joggle specimens obtained from flight panels.

Water content contribution in calculus phantom ablation during Q-switched Tm:YAG laser lithotripsy.

PubMed

Zhang, Jian J; Rajabhandharaks, Danop; Xuan, Jason Rongwei; Wang, Hui; Chia, Ray W J; Hasenberg, Tom; Kang, Hyun Wook

2015-01-01

Q-switched (QS) Tm:YAG laser ablation mechanisms on urinary calculi are still unclear to researchers. Here, dependence of water content in calculus phantom on calculus ablation performance was investigated. White gypsum cement was used as a calculus phantom model. The calculus phantoms were ablated by a total 3-J laser pulse exposure (20 mJ, 100 Hz, 1.5 s) and contact mode with N=15 sample size. Ablation volume was obtained on average 0.079, 0.122, and 0.391  mm3 in dry calculus in air, wet calculus in air, and wet calculus in-water groups, respectively. There were three proposed ablation mechanisms that could explain the effect of water content in calculus phantom on calculus ablation performance, including shock wave due to laser pulse injection and bubble collapse, spallation, and microexplosion. Increased absorption coefficient of wet calculus can cause stronger spallation process compared with that caused by dry calculus; as a result, higher calculus ablation was observed in both wet calculus in air and wet calculus in water. The test result also indicates that the shock waves generated by short laser pulse under the in-water condition have great impact on the ablation volume by Tm:YAG QS laser.

Acoustic attenuation, phase and group velocities in liquid-filled pipes II: simulation for Spallation Neutron Sources and planetary exploration.

PubMed

Jiang, Jian; Baik, Kyungmin; Leighton, Timothy G

2011-08-01

This paper uses a finite element method (FEM) to compare predictions of the attenuation and sound speeds of acoustic modes in a fluid-filled pipe with those of the analytical model presented in the first paper in this series. It explains why, when the predictions of the earlier paper were compared with experimental data from a water-filled PMMA pipe, the uncertainties and agreement for attenuation data were worse than those for sound speed data. Having validated the FEM approach in this way, the versatility of FEM is thereafter demonstrated by modeling two practical applications which are beyond the analysis of the earlier paper. These applications model propagation in the mercury-filled steel pipework of the Spallation Neutron Source at the Oak Ridge National Laboratory (Tennessee), and in a long-standing design for acoustic sensors for use on planetary probes. The results show that strong coupling between the fluid and the solid walls means that erroneous interpretations are made of the data if they assume that the sound speed and attenuation in the fluid in the pipe are the same as those that would be measured in an infinite volume of identical fluid, assumptions which are common when such data have previously been interpreted.

Validation of Monte Carlo simulation of neutron production in a spallation experiment

DOE PAGES

Zavorka, L.; Adam, J.; Artiushenko, M.; ...

2015-02-25

A renewed interest in experimental research on Accelerator-Driven Systems (ADS) has been initiated by the global attempt to produce energy from thorium as a safe(r), clean(er) and (more) proliferation-resistant alternative to the uranium-fuelled thermal nuclear reactors. The ADS research has been actively pursued at the Joint Institute for Nuclear Research (JINR), Dubna, since decades. Most recently, the emission of fast neutrons was experimentally investigated at the massive (m = 512 kg) natural uranium spallation target QUINTA. The target has been irradiated with the relativistic deuteron beams of energy from 0.5 AGeV up to 4 AGeV at the JINR Nuclotron acceleratormore » in numerous experiments since 2011. Neutron production inside the target was studied through the gamma-ray spectrometry measurement of natural uranium activation detectors. Experimental reaction rates for (n,γ), (n,f) and (n,2n) reactions in uranium have provided valuable information about the neutron distribution over a wide range of energies up to some GeV. The experimental data were compared to the predictions of Monte Carlo simulations using the MCNPX 2.7.0 code. In conclusion, the results are presented and potential sources of partial disagreement are discussed later in this work.« less

Interstellar Lithium and Rubidium in the Diffuse Gas Near IC 443

NASA Astrophysics Data System (ADS)

Ritchey, Adam M.; Taylor, C. J.; Federman, S. R.; Lambert, D. L.

2011-01-01

We present an analysis of interstellar lithium and rubidium from observations made with the Hobby-Eberly Telescope at McDonald Observatory of the Li I λ6707 and Rb I λ7800 absorption lines along four lines of sight through the supernova remnant IC 443. The observations probe interstellar material polluted by the ejecta of a core-collapse (Type II) supernova and can thus be used to constrain the contribution from massive stars to the synthesis of lithium and rubidium. Production of 7Li is expected to occur through neutrino spallation in the helium and carbon shells of the progenitor star during the terminal supernova explosion, while both 6Li and 7Li are synthesized via spallation and fusion reactions involving cosmic rays accelerated by the remnant. Gamma-ray emission from IC 443 provides strong evidence for the interaction of accelerated cosmic rays with the ambient atomic and molecular gas. Rubidium is also produced by massive stars through the weak s-process in the He- and C-burning shells and the r-process during core collapse. We examine interstellar 7Li/6Li isotope ratios as well as Li/K and Rb/K ratios along each line of sight, and discuss the implications of our results in the context of nucleosynthesis associated with Type II supernovae.

Monte carlo simulations of the n_TOF lead spallation target with the Geant4 toolkit: A benchmark study

NASA Astrophysics Data System (ADS)

Lerendegui-Marco, J.; Cortés-Giraldo, M. A.; Guerrero, C.; Quesada, J. M.; Meo, S. Lo; Massimi, C.; Barbagallo, M.; Colonna, N.; Mancussi, D.; Mingrone, F.; Sabaté-Gilarte, M.; Vannini, G.; Vlachoudis, V.; Aberle, O.; Andrzejewski, J.; Audouin, L.; Bacak, M.; Balibrea, J.; Bečvář, F.; Berthoumieux, E.; Billowes, J.; Bosnar, D.; Brown, A.; Caamaño, M.; Calviño, F.; Calviani, M.; Cano-Ott, D.; Cardella, R.; Casanovas, A.; Cerutti, F.; Chen, Y. H.; Chiaveri, E.; Cortés, G.; Cosentino, L.; Damone, L. A.; Diakaki, M.; Domingo-Pardo, C.; Dressler, R.; Dupont, E.; Durán, I.; Fernández-Domínguez, B.; Ferrari, A.; Ferreira, P.; Finocchiaro, P.; Göbel, K.; Gómez-Hornillos, M. B.; García, A. R.; Gawlik, A.; Gilardoni, S.; Glodariu, T.; Gonçalves, I. F.; González, E.; Griesmayer, E.; Gunsing, F.; Harada, H.; Heinitz, S.; Heyse, J.; Jenkins, D. G.; Jericha, E.; Käppeler, F.; Kadi, Y.; Kalamara, A.; Kavrigin, P.; Kimura, A.; Kivel, N.; Kokkoris, M.; Krtička, M.; Kurtulgil, D.; Leal-Cidoncha, E.; Lederer, C.; Leeb, H.; Lonsdale, S. J.; Macina, D.; Marganiec, J.; Martínez, T.; Masi, A.; Mastinu, P.; Mastromarco, M.; Maugeri, E. A.; Mazzone, A.; Mendoza, E.; Mengoni, A.; Milazzo, P. M.; Musumarra, A.; Negret, A.; Nolte, R.; Oprea, A.; Patronis, N.; Pavlik, A.; Perkowski, J.; Porras, I.; Praena, J.; Radeck, D.; Rauscher, T.; Reifarth, R.; Rout, P. C.; Rubbia, C.; Ryan, J. A.; Saxena, A.; Schillebeeckx, P.; Schumann, D.; Smith, A. G.; Sosnin, N. V.; Stamatopoulos, A.; Tagliente, G.; Tain, J. L.; Tarifeño-Saldivia, A.; Tassan-Got, L.; Valenta, S.; Variale, V.; Vaz, P.; Ventura, A.; Vlastou, R.; Wallner, A.; Warren, S.; Woods, P. J.; Wright, T.; Žugec, P.

2017-09-01

Monte Carlo (MC) simulations are an essential tool to determine fundamental features of a neutron beam, such as the neutron flux or the γ-ray background, that sometimes can not be measured or at least not in every position or energy range. Until recently, the most widely used MC codes in this field had been MCNPX and FLUKA. However, the Geant4 toolkit has also become a competitive code for the transport of neutrons after the development of the native Geant4 format for neutron data libraries, G4NDL. In this context, we present the Geant4 simulations of the neutron spallation target of the n_TOF facility at CERN, done with version 10.1.1 of the toolkit. The first goal was the validation of the intra-nuclear cascade models implemented in the code using, as benchmark, the characteristics of the neutron beam measured at the first experimental area (EAR1), especially the neutron flux and energy distribution, and the time distribution of neutrons of equal kinetic energy, the so-called Resolution Function. The second goal was the development of a Monte Carlo tool aimed to provide useful calculations for both the analysis and planning of the upcoming measurements at the new experimental area (EAR2) of the facility.

Applications of a micro-pixel chamber (μPIC) based, time-resolved neutron imaging detector at pulsed neutron beams

NASA Astrophysics Data System (ADS)

Parker, J. D.; Harada, M.; Hattori, K.; Iwaki, S.; Kabuki, S.; Kishimoto, Y.; Kubo, H.; Kurosawa, S.; Matsuoka, Y.; Miuchi, K.; Mizumoto, T.; Nishimura, H.; Oku, T.; Sawano, T.; Shinohara, T.; Suzuki, J.-I.; Takada, A.; Tanimori, T.; Ueno, K.; Ikeno, M.; Tanaka, M.; Uchida, T.

2014-04-01

The realization of high-intensity, pulsed spallation neutron sources such as J-PARC in Japan and SNS in the US has brought time-of-flight (TOF) based neutron techniques to the fore and spurred the development of new detector technologies. When combined with high-resolution imaging, TOF-based methods become powerful tools for direct imaging of material properties, including crystal structure/internal strain, isotopic/temperature distributions, and internal and external magnetic fields. To carry out such measurements in the high-intensities and high gamma backgrounds found at spallation sources, we have developed a new time-resolved neutron imaging detector employing a micro-pattern gaseous detector known as the micro-pixel chamber (μPIC) coupled with a field-programmable-gate-array-based data acquisition system. The detector combines 100μm-level (σ) spatial and sub-μs time resolutions with low gamma sensitivity of less than 10-12 and a rate capability on the order of Mcps (mega-counts-per-second). Here, we demonstrate the application of our detector to TOF-based techniques with examples of Bragg-edge transmission and neutron resonance transmission imaging (with computed tomography) carried out at J-PARC. We also consider the direct imaging of magnetic fields with our detector using polarized neutrons.

Search for Cm-248 in the early solar system

NASA Technical Reports Server (NTRS)

Lavielle, B.; Marti, K.; Pellas, P.; Perron, C.

1992-01-01

Possible evidence for the presence of Cm-248 in the early solar system was reported from fission gas studies (Rao and Gopalan, 1973) and recently from studies of very high nuclear track densities (not less than 5 x 10 exp 8/sq cm) in the merrillite of the H4 chondrite Forest Vale (F.V.) (Pellas et al., 1987). We report here an analysis of the isotopic abundances of xenon in F.V. phosphates and results of track studies in phosphate/pyroxene contacts. The fission xenon isotopic signature clearly identifies Pu-244 as the extinct progenitor. We calculate an upper limit Cm-248/Pu-244 to be less than 0.0015 at the beginning of Xe retention in F.V. phosphates. This corresponds to an upper limit of the ratio Cm-248/U-235 of not greater than 5 x 10 exp -5 further constraining the evidence for any late addition of freshly synthesized actinide elements just prior to solar system formation. The fission track density observed after annealing the phosphates at 290C (1 hr, which essentially erases spallation recoil tracks) is also in agreement with the Pu-244 abundance inferred from fission Xe. The spallation recoil tracks produced during the 76 Ma cosmic-ray exposure account for the very high track density in merrillites.

Commissioning of cryogenic system for China Spallation Neutron Source

NASA Astrophysics Data System (ADS)

Ye, Bin; He, Chongchao; Li, Na; Ding, Meiying; Wang, Yaqiong; Yu, Zhang; He, Kun

2017-12-01

China Spallation Neutron Source(CSNS) cryogenic system provides supercritical cryogenic hydrogen to neutron moderators, including a helium refrigerator, hydrogen loop and hydrogen safety equipment. The helium refrigerator is provided by Linde with cooling capacity of 2200 W at 20 K. Hydrogen loop system mainly includes cryogenic hydrogen pipes, hydrogen circulator cold-box and accumulator cold-box. Cryogenic hydrogen pump, ortho-para convertor, helium-hydrogen heat-exchanger, hydrogen heater and accumulator are integrated in hydrogen circulation cold-box, and accumulator cold-box. Hydrogen safety equipment includes safety valves, rupture disk, hydrogen sensor, flame detector and other equipment to ensure that cryogenic system in dangerous situations will go down, vents, or takes other measures. The cryogenic system commissioning work includes four steps. First, in order to test the refrigerating capacity of refrigerator, when acceptance testing, refrigerator internal heater was used as thermal load. Second, using simulation load as heat load of moderator, hydrogen loop use helium instead of hydrogen, and cooled down to 20 K, then re-warming and test the leak detection of hydrogen loop system. Third, base on the step 2, using hydrogen as working medium, and optimized the control logic. Forth, cryogenic system with the moderators joint commissioning. Now, cryogenic system is connected with the moderators, and the forth step will be carried out in the near future.

Design progress of cryogenic hydrogen system for China Spallation Neutron Source

DOE Office of Scientific and Technical Information (OSTI.GOV)

Wang, G. P.; Zhang, Y.; Xiao, J.

2014-01-29

China Spallation Neutron Source (CSNS) is a large proton accelerator research facility with 100 kW beam power. Construction started in October 2011 and is expected to last 6.5 years. The cryogenic hydrogen circulation is cooled by a helium refrigerator with cooling capacity of 2200 W at 20 K and provides supercritical hydrogen to neutron moderating system. Important progresses of CSNS cryogenic system were concluded as follows. Firstly, process design of cryogenic system has been completed including helium refrigerator, hydrogen loop, gas distribution, and safety interlock. Secondly, an accumulator prototype was designed to mitigate pressure fluctuation caused by dynamic heat loadmore » from neutron moderation. Performance test of the accumulator has been carried out at room and liquid nitrogen temperature. Results show the accumulator with welding bellows regulates hydrogen pressure well. Parameters of key equipment have been identified. The contract for the helium refrigerator has been signed. Mechanical design of the hydrogen cold box has been completed, and the hydrogen pump, ortho-para hydrogen convertor, helium-hydrogen heat exchanger, hydrogen heater, and cryogenic valves are in procurement. Finally, Hydrogen safety interlock has been finished as well, including the logic of gas distribution, vacuum, hydrogen leakage and ventilation. Generally, design and construction of CSNS cryogenic system is conducted as expected.« less

Structure/property (constitutive and dynamic strength/damage) characterization of additively manufactured 316L SS

NASA Astrophysics Data System (ADS)

Gray, G. T., III; Livescu, V.; Rigg, P. A.; Trujillo, C. P.; Cady, C. M.; Chen, S. R.; Carpenter, J. S.; Lienert, T. J.; Fensin, S.

2015-09-01

For additive manufacturing (AM), the certification and qualification paradigm needs to evolve as there exists no "ASTM-type" additive manufacturing certified process or AM-material produced specifications. Accordingly, utilization of AM materials to meet engineering applications requires quantification of the constitutive properties of these evolving materials in comparison to conventionally-manufactured metals and alloys. Cylinders of 316L SS were produced using a LENS MR-7 laser additive manufacturing system from Optomec (Albuquerque, NM) equipped with a 1kW Yb-fiber laser. The microstructure of the AM-316L SS is detailed in both the as-built condition and following heat-treatments designed to obtain full recrystallization. The constitutive behavior as a function of strain rate and temperature is presented and compared to that of nominal annealed wrought 316L SS plate. The dynamic damage evolution and failure response of all three materials was probed using flyer-plate impact driven spallation experiments at a peak stress of 4.5 GPa to examine incipient spallation response. The spall strength of AM-produced 316L SS was found to be very similar for the peak shock stress studied to that of annealed wrought or AM-316L SS following recrystallization. The damage evolution as a function of microstructure was characterized using optical metallography.

In situ polarized 3He system for the Magnetism Reflectometer at the Spallation Neutron Source.

PubMed

Tong, X; Jiang, C Y; Lauter, V; Ambaye, H; Brown, D; Crow, L; Gentile, T R; Goyette, R; Lee, W T; Parizzi, A; Robertson, J L

2012-07-01

We report on the in situ polarized (3)He neutron polarization analyzer developed for the time-of-flight Magnetism Reflectometer at the Spallation Neutron Source at Oak Ridge National Laboratory. Using the spin exchange optical pumping method, we achieved a (3)He polarization of 76% ± 1% and maintained it for the entire three-day duration of the test experiment. Based on transmission measurements with unpolarized neutrons, we show that the average analyzing efficiency of the (3)He system is 98% for the neutron wavelength band of 2-5 Å. Using a highly polarized incident neutron beam produced by a supermirror bender polarizer, we obtained a flipping ratio of >100 with a transmission of 25% for polarized neutrons, averaged over the wavelength band of 2-5 Å. After the cell was depolarized for transmission measurements, it was reproducibly polarized and this performance was maintained for three weeks. A high quality polarization analysis experiment was performed on a reference sample of Fe/Cr multilayer with strong spin-flip off-specular scattering. Using a combination of the position sensitive detector, time-of-flight method, and the excellent parameters of the (3)He cell, the polarization analysis of the two-dimensional maps of reflected, refracted, and off-specular scattered intensity above and below the horizon were obtained, simultaneously.

Sulfur Impurities and the Microstructure of Alumina Scales

NASA Technical Reports Server (NTRS)

Smialek, James L.

1997-01-01

The relationship between the microstructure of alumina scales, adhesion, and sulfur content was examined through a series of nickel alloys oxidized in 1100 to 1200 deg. C cyclic or isothermal exposures in air. In cyclic tests of undoped NiCrAl, adhesion was produced when the sulfur content was reduced, without any change in scale microstructure. Although interfacial voids were not observed in cyclic tests of NiCrAl, they were promoted by long-term isothermal exposures, by sulfur doping, and in most exposures of NiAl. Two single crystal superalloys, PWA 1480 and Rene' N5, were also tested, either in the as-received condition or after the sulfur content had been reduced to less than 1 ppmw by hydrogen annealing. The unannealed alloys always exhibited spalling to bare metal, but interfacial voids were not observed consistently. Desulfurized PWA 1480 and Rene' N5 exhibited remarkable adhesion and no voidage for either isothermal or cyclic exposures. The most consistent microstructural feature was that, for the cases where voids did form, the scale undersides exhibited corresponding areas with ridged oxide grain boundaries. Voids were not required for spallation nor were other microstructural features essential for adhesion. These observations are consistent with the model whereby scale spallation is controlled primarily by interfacial sulfur segregation and the consequent degradation of oxide-metal bonding.

Electron-cloud updated simulation results for the PSR, and recent results for the SNS

NASA Astrophysics Data System (ADS)

Pivi, M.; Furman, M. A.

2002-05-01

Recent simulation results for the main features of the electron cloud in the storage ring of the Spallation Neutron Source (SNS) at Oak Ridge, and updated results for the Proton Storage Ring (PSR) at Los Alamos are presented in this paper. A refined model for the secondary emission process including the so called true secondary, rediffused and backscattered electrons has recently been included in the electron-cloud code.

Study of the Erosion Corrosion of Alloys and Coatings.

DTIC Science & Technology

1987-12-01

AD-A±94 327 ST Y OF THE ROSION COROSION OF ALLO COTINGS 4 (U) PITTSBURGH UNIV PA DEPT OF MTERIRLS SCIENCE AND ENGINEERING N BIRKS ET AL. DEC 87 ARO...AVAILABILITY OF REPORT 2b. DECLASSIFICATION IOOWNGRADING SCHEDULE Approved for public release; distribution unlimited. 4 . PERFORMING ORGANIZATION REPORT...a further regime, based on scale spallation, at certain values of scale thicknesse . The inclusion of sulfur in the atmosphere results in much more

Optimizing the Hot-Corrosion Resistance-of-Novel gamma-Ni+gamma-prime-Ni3A1-Based Alloys and Coatings

DTIC Science & Technology

2006-07-01

TBC benefit Substrale limit 1 1 0 0 ---------- .- -.. . . . . . . --- I single crystal S1000 conventlonally cest allos . .- alloy. E directionally...usually heat treated or processed) forms. Developments in casting technologies made it possible to produce directionally-solidified and single - crystal ...advanced single - crystal superalloys with improved strength meant reductions in chromium and silicon contents. The scale growth and spallation rates can be

Fracture of Rolled Homogeneous Steel Armor (Nucleation Threshold Stress).

DTIC Science & Technology

1980-01-01

AD-AO81 618 ARMY ARMAMENT RESEARCH AND DEVELOPMENT COMMAND ABERD--ETC F/B 19/4 FRACTURE OF ROLLED HOMOGENEOUS STEEL ARMOR (NUCLEATION THRESHOL--ETC(U...ARBRL-MR-02984A QQ FRACTURE OF ROLLED HOMOGENEOUS STEEL ARMOR (NUCLEATION THRESHOLD STRESS) Gerald L Moss Lynn SeamanLy~ S, ,.DTIC S ELECTED January...nucleation stress, Crack threshold stress, Fracture, Fracture stress, Spallation, Armor, Rolled homogeneous steel armor M~ AS$TRACr (Vita ssf -- ebb

Elastic plate spallation

NASA Technical Reports Server (NTRS)

Oline, L.; Medaglia, J.

1972-01-01

The dynamic finite element method was used to investigate elastic stress waves in a plate. Strain displacement and stress strain relations are discussed along with the stiffness and mass matrix. The results of studying point load, and distributed load over small, intermediate, and large radii are reported. The derivation of finite element matrices, and the derivation of lumped and consistent matrices for one dimensional problems with Laplace transfer solutions are included. The computer program JMMSPALL is also included.

Integrating labview into a distributed computing environment.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kasemir, K. U.; Pieck, M.; Dalesio, L. R.

2001-01-01

Being easy to learn and well suited for a selfcontained desktop laboratory setup, many casual programmers prefer to use the National Instruments Lab-VIEW environment to develop their logic. An ActiveX interface is presented that allows integration into a plant-wide distributed environment based on the Experimental Physics and Industrial Control System (EPICS). This paper discusses the design decisions and provides performance information, especially considering requirements for the Spallation Neutron Source (SNS) diagnostics system.

Fracture Mechanics Analyses of the Slip-Side Joggle Regions of Wing-Leading-Edge Panels

NASA Technical Reports Server (NTRS)

Raju, Ivatury S.; Knight, Norman F., Jr.; Song, Kyongchan; Phillips, Dawn R.

2011-01-01

The Space Shuttle wing-leading edge consists of panels that are made of reinforced carbon-carbon. Coating spallation was observed near the slip-side region of the panels that experience extreme heating. To understand this phenomenon, a root-cause investigation was conducted. As part of that investigation, fracture mechanics analyses of the slip-side joggle regions of the hot panels were conducted. This paper presents an overview of the fracture mechanics analyses.

Space charge tune shift, fast resonance traversal, and current limits in circular accelerators

DOE Office of Scientific and Technical Information (OSTI.GOV)

Rees, G.H.

1996-06-01

Space charge tune shifts, fast resonance traversals, and current limits are important design issues for low energy, high power circular accelerators. Areas of interest are accumulator rings and fast cycling synchrotrons, and typical applications are for pulsed spallation neutron sources, heavy ion fusion storage ring drivers, and booster injectors for high energy proton and ion facilities. Aspects of the three topics are discussed in the paper. {copyright} {ital 1996 American Institute of Physics.}

First measurement of the VESUVIO neutron spectrum in the 30-80 MeV energy range using a Proton Recoil Telescope technique

NASA Astrophysics Data System (ADS)

Cazzaniga, C.; Tardocchi, M.; Croci, G.; Frost, C.; Giacomelli, L.; Grosso, G.; Hjalmarsson, A.; Rebai, M.; Rhodes, N. J.; Schooneveld, E. M.; Gorini, G.

2013-11-01

Measurements of the fast neutron energy spectrum at the ISIS spallation source are reported. The measurements were performed with a Proton Recoil Telescope consisting of a thin plastic foil placed in the neutron beam and two scintillator detectors. Results in the neutron energy range 30 MeV < En < 80 MeV are in good agreement with Monte Carlo simulations of the neutron spectrum.

Pretest predictions of surface strain and fluid pressures in mercury targets undergoing thermal shock

DOE Office of Scientific and Technical Information (OSTI.GOV)

Taleyarkhan, R.P.; Kim, S.H.; Haines, J.

The authors provide a perspective overview of pretest modeling and analysis work related to thermal shock effects in spallation neutron source targets that were designed for conducting thermal shock experiments at the Los Alamos Neutron Science Center (LANSCE). Data to be derived are to be used for benchmarking computational tools as well as to assess the efficacy of optical gauges for monitoring dynamic fluid pressures and phenomena such as the onset of cavitation.

Source Amplitudes of NTS Explosions Inferred from Rayleigh Waves at Albuquerque and Tucson

DTIC Science & Technology

1978-06-01

explosions almost always cause spallation near the free surface (e.g., Eisler and Chilton, 1964). When the spalled material falls back to the surface...spall closure), some impulse is delivered and a large signal associated with spall closure can often be observed on near- field recordings (e.g., Eisler ...made for the extent of the spall region ( Eisler and Chilton, 1964; Viecelli, 1973; Sobel, 1978). Viecelli (1973) studied the data for six explosions

Simulations of Terrestrial in-situ Cosmogenic-Nuclide Production

NASA Technical Reports Server (NTRS)

Reedy, R. C.; Nishiizumi, K.; Lal, D.; Arnold, J. R.; Englert, P. A. J.; Klein, J.; Middleton, R.; Jull, A. J. T.; Donahue, D. J.

1994-01-01

Targets of silicon and silicon dioxide were irradiated with spallation neutrons to simulate the production of long-lived radionuclides in the surface of the Earth. Gamma-ray spectroscopy was used to measure Be-7 and Na-22, and accelerator mass spectrometry was used to measure Be-10, C-14, and Al-26. The measured ratios of these nuclides are compared with calculated ratios and with ratios from other simulations and agree well with ratios inferred from terrestrial samples.

Dynamic fracture of tantalum under extreme tensile stress.

PubMed

Albertazzi, Bruno; Ozaki, Norimasa; Zhakhovsky, Vasily; Faenov, Anatoly; Habara, Hideaki; Harmand, Marion; Hartley, Nicholas; Ilnitsky, Denis; Inogamov, Nail; Inubushi, Yuichi; Ishikawa, Tetsuya; Katayama, Tetsuo; Koyama, Takahisa; Koenig, Michel; Krygier, Andrew; Matsuoka, Takeshi; Matsuyama, Satoshi; McBride, Emma; Migdal, Kirill Petrovich; Morard, Guillaume; Ohashi, Haruhiko; Okuchi, Takuo; Pikuz, Tatiana; Purevjav, Narangoo; Sakata, Osami; Sano, Yasuhisa; Sato, Tomoko; Sekine, Toshimori; Seto, Yusuke; Takahashi, Kenjiro; Tanaka, Kazuo; Tange, Yoshinori; Togashi, Tadashi; Tono, Kensuke; Umeda, Yuhei; Vinci, Tommaso; Yabashi, Makina; Yabuuchi, Toshinori; Yamauchi, Kazuto; Yumoto, Hirokatsu; Kodama, Ryosuke

2017-06-01

The understanding of fracture phenomena of a material at extremely high strain rates is a key issue for a wide variety of scientific research ranging from applied science and technological developments to fundamental science such as laser-matter interaction and geology. Despite its interest, its study relies on a fine multiscale description, in between the atomic scale and macroscopic processes, so far only achievable by large-scale atomic simulations. Direct ultrafast real-time monitoring of dynamic fracture (spallation) at the atomic lattice scale with picosecond time resolution was beyond the reach of experimental techniques. We show that the coupling between a high-power optical laser pump pulse and a femtosecond x-ray probe pulse generated by an x-ray free electron laser allows detection of the lattice dynamics in a tantalum foil at an ultrahigh strain rate of [Formula: see text] ~2 × 10 8 to 3.5 × 10 8 s -1 . A maximal density drop of 8 to 10%, associated with the onset of spallation at a spall strength of ~17 GPa, was directly measured using x-ray diffraction. The experimental results of density evolution agree well with large-scale atomistic simulations of shock wave propagation and fracture of the sample. Our experimental technique opens a new pathway to the investigation of ultrahigh strain-rate phenomena in materials at the atomic scale, including high-speed crack dynamics and stress-induced solid-solid phase transitions.

Ceramic Coatings for Corrosion Resistant Nuclear Waste Container Evaluated in Simulated Ground Water at 90?C

DOE Office of Scientific and Technical Information (OSTI.GOV)

Haslam, J J; Farmer, J C

2004-03-31

Ceramic materials have been considered as corrosion resistant coatings for nuclear waste containers. Their suitability can be derived from the fully oxidized state for selected metal oxides. Several types of ceramic coatings applied to plain carbon steel substrates by thermal spray techniques have been exposed to 90 C simulated ground water for nearly 6 years. In some cases no apparent macroscopic damage such as coating spallation was observed in coatings. Thermal spray processes examined in this work included plasma spray, High Velocity Oxy Fuel (HVOF), and Detonation Gun. Some thermal spray coatings have demonstrated superior corrosion protection for the plainmore » carbon steel substrate. In particular the HVOF and Detonation Gun thermal spray processes produced coatings with low connected porosity, which limited the growth rate of corrosion products. It was also demonstrated that these coatings resisted spallation of the coating even when an intentional flaw (which allowed for corrosion of the carbon steel substrate underneath the ceramic coating) was placed in the coating. A model for prediction of the corrosion protection provided by ceramic coatings is presented. The model includes the effect of the morphology and amount of the porosity within the thermal spray coating and provides a prediction of the exposure time needed to produce a crack in the ceramic coating.« less

Dynamic fracture of tantalum under extreme tensile stress

PubMed Central

Albertazzi, Bruno; Ozaki, Norimasa; Zhakhovsky, Vasily; Faenov, Anatoly; Habara, Hideaki; Harmand, Marion; Hartley, Nicholas; Ilnitsky, Denis; Inogamov, Nail; Inubushi, Yuichi; Ishikawa, Tetsuya; Katayama, Tetsuo; Koyama, Takahisa; Koenig, Michel; Krygier, Andrew; Matsuoka, Takeshi; Matsuyama, Satoshi; McBride, Emma; Migdal, Kirill Petrovich; Morard, Guillaume; Ohashi, Haruhiko; Okuchi, Takuo; Pikuz, Tatiana; Purevjav, Narangoo; Sakata, Osami; Sano, Yasuhisa; Sato, Tomoko; Sekine, Toshimori; Seto, Yusuke; Takahashi, Kenjiro; Tanaka, Kazuo; Tange, Yoshinori; Togashi, Tadashi; Tono, Kensuke; Umeda, Yuhei; Vinci, Tommaso; Yabashi, Makina; Yabuuchi, Toshinori; Yamauchi, Kazuto; Yumoto, Hirokatsu; Kodama, Ryosuke

2017-01-01

The understanding of fracture phenomena of a material at extremely high strain rates is a key issue for a wide variety of scientific research ranging from applied science and technological developments to fundamental science such as laser-matter interaction and geology. Despite its interest, its study relies on a fine multiscale description, in between the atomic scale and macroscopic processes, so far only achievable by large-scale atomic simulations. Direct ultrafast real-time monitoring of dynamic fracture (spallation) at the atomic lattice scale with picosecond time resolution was beyond the reach of experimental techniques. We show that the coupling between a high-power optical laser pump pulse and a femtosecond x-ray probe pulse generated by an x-ray free electron laser allows detection of the lattice dynamics in a tantalum foil at an ultrahigh strain rate of ε. ~2 × 108 to 3.5 × 108 s−1. A maximal density drop of 8 to 10%, associated with the onset of spallation at a spall strength of ~17 GPa, was directly measured using x-ray diffraction. The experimental results of density evolution agree well with large-scale atomistic simulations of shock wave propagation and fracture of the sample. Our experimental technique opens a new pathway to the investigation of ultrahigh strain-rate phenomena in materials at the atomic scale, including high-speed crack dynamics and stress-induced solid-solid phase transitions. PMID:28630909

Cross sections for production of the 15.10 MeV and other astrophysically significant gamma-ray lines through excitation and spallation of sup 12 C and sup 16 O with protons

NASA Technical Reports Server (NTRS)

Lang, F. L.; Werntz, C. W.; Crannell, C. J.; Trombka, J. I.; Chang, C. C.

1986-01-01

The ratio of the flux of 15.10-MeV gamma rays to the flux of 4.438-MeV gamma rays resulting from excitation of the corresponding states in C-12 as a sensitive measure of the spectrum of the exciting particles produced in solar flares and other cosmic sources. These gamma rays are produced predominantly by interactions with C-12 and O-16, both of which are relatively abundant in the solar photosphere. Gamma ray production cross sections for proton interactions have been reported previously for all important channels except for the production of 15.10-MeV gamma rays from O-16. The first reported measurement of the 15.10-MeV gamma ray production cross section from p + O-16 is presented here. The University of Maryland cyclotron was employed to produce 40-, 65-, and 86-MeV protons which interacted with CH2 and BeO targets. The resultant gamma ray spectra were measured with a high-purity germanium semiconductor detector at 70, 90, 110, 125, and 140 degrees relative to the direction of the incident beam for each proton energy. Other gamma ray lines resulting from direct excitation and spallation reactions with C-12 and 0-16 were observed as well, and their gamma ray production cross sections described.

Effects of Grain Size on Ultrasonic Attenuation in Type 316L Stainless Steel

PubMed Central

Wan, Tao; Wakui, Takashi; Futakawa, Masatoshi; Obayashi, Hironari

2017-01-01

A lead bismuth eutectic (LBE) spallation target will be installed in the Target Test Facility (TEF-T) in the Japan Proton Accelerator Research Complex (J-PARC). The spallation target vessel filled with LBE is made of type 316L stainless steel. However, various damages, such as erosion/corrosion damage and liquid metal embrittlement caused by contact with flowing LBE at high temperature, and irradiation hardening caused by protons and neutrons, may be inflicted on the target vessel, which will deteriorate the steel and might break the vessel. To monitor the target vessel for prevention of an accident, an ultrasonic technique has been proposed to establish off-line evaluation for estimating vessel material status during the target maintenance period. Basic R&D must be carried out to clarify the dependency of ultrasonic wave propagation behavior on material microstructures and obtain fundamental knowledge. As a first step, ultrasonic waves scattered by the grains of type 316L stainless steel are investigated using new experimental and numerical approaches in the present study. The results show that the grain size can be evaluated exactly and quantitatively by calculating the attenuation coefficient of the ultrasonic waves scattered by the grains. The results also show that the scattering regimes of ultrasonic waves depend heavily on the ratio of wavelength to average grain size, and are dominated by grains of extraordinarily large size along the wave propagation path. PMID:28773115

Antideuterons in cosmic rays: sources and discovery potential

DOE Office of Scientific and Technical Information (OSTI.GOV)

Herms, Johannes; Ibarra, Alejandro; Vittino, Andrea

Antibaryons are produced in our Galaxy in collisions of high energy cosmic rays with the interstellar medium and in old supernova remnants, and possibly, in exotic sources such as primordial black hole evaporation or dark matter annihilations and decays. The search for signals from exotic sources in antiproton data is hampered by large backgrounds from spallation which, within theoretical errors, can solely account for the current data. Due to the higher energy threshold for antideuteron production, which translates into a suppression of the low energy flux from spallations, antideuteron searches have been proposed as a probe for exotic sources. Wemore » perform in this paper a comprehensive analysis of the antideuteron fluxes at the Earth expected from known and hypothetical sources in our Galaxy, and we calculate their maximal values consistent with current antiproton data from AMS-02. We find that supernova remnants generate a negligible flux, whereas primordial black hole evaporation and dark matter annihilations or decays may dominate the total flux at low energies. On the other hand, we find that the (detection of cosmic antideuterons) would require, for the scenarios studied in this paper and assuming optimistic values of the coalescence momentum and solar modulation, an increase of the experimental sensitivity compared to ongoing and planned instruments by at least a factor of 2. Finally, we briefly comment on the prospects for antihelium-3 detection.« less

Ship Effect Neutron Measurements And Impacts On Low-Background Experiments

DOE Office of Scientific and Technical Information (OSTI.GOV)

Aguayo Navarrete, Estanislao; Kouzes, Richard T.; Siciliano, Edward R.

2013-10-01

The primary particles entering the upper atmosphere as cosmic rays create showers in the atmosphere that include a broad spectrum of secondary neutrons, muons and protons. These cosmic-ray secondaries interact with materials at the surface of the Earth, yielding prompt backgrounds in radiation detection systems, as well as inducing long-lived activities through spallation events, dominated by the higher-energy neutron secondaries. For historical reasons, the multiple neutrons produced in spallation cascade events are referred to as “ship effect” neutrons. Quantifying the background from cosmic ray induced activities is important to low-background experiments, such as neutrino-less double beta decay. Since direct measurementsmore » of the effects of shielding on the cosmic-ray neutron spectrum are not available, Monte Carlo modeling is used to compute such effects. However, there are large uncertainties (orders of magnitude) in the possible cross-section libraries and the cosmic-ray neutron spectrum for the energy range needed in such calculations. The measurements reported here were initiated to validate results from Monte Carlo models through experimental measurements in order to provide some confidence in the model results. The results indicate that the models provide the correct trends of neutron production with increasing density, but there is substantial disagreement between the model and experimental results for the lower-density materials of Al, Fe and Cu.« less

Neutronics performance and activation calculation of dense tungsten granular target for China-ADS

NASA Astrophysics Data System (ADS)

Zhang, Yaling; Li, Jianyang; Zhang, Xunchao; Cai, Hanjie; Yan, Xuesong; Yu, Lin; Fu, Fen; Lin, Ping; Gao, Xiaofei; Zhang, Zhilei; Zhang, Yanshi; Yang, Lei

2017-11-01

Spallation target, which constitutes the physical and functional interface between the high power accelerator and the subcritical core, is one of the most important components in Accelerator Driven Subcritical System (ADS). In this paper, we investigated the neutronics performance, the radiation damage and the activation of dense tungsten granular flow spallation target by using the Monte Carlo programs GMT and FLUKA at the proton energy of 250 MeV with a beam current of 10 mA . First, the leaking neutron yield, leaking neutron energy spectrum and laterally leaking neutron distribution at several time nodes and with different target parameters are explored. After that, the displacement per atom (DPA) and the helium/hydrogen production for tungsten grains and structural materials with stainless steel 316L are estimated. Finally, the radioactivity, residual dose rate and afterheat of granular target are presented. Results indicate that granule diameter below 1 cm and the beam profile diameter have negligible impact on neutronics performance, while the target diameter and volume fraction of grain have notable influence. The maximum DPA for target vessel (beam tube) is about 1.0 (1.6) DPA/year in bare target, and increased to 2.6 (2.8) DPA/year in fission environment. Average DPA for tungsten grains is relatively low. The decline rate of radioactivity and afterheat with cooling time grows with the decrease of the irradiation time.

Irradiation of amorphous Ta42Si13N45 film with a femtosecond laser pulse

NASA Astrophysics Data System (ADS)

Romano, V.; Meier, M.; Theodore, N. D.; Marble, D. K.; Nicolet, M.-A.

2011-07-01

Films of 260 nm thickness, with atomic composition Ta42Si13N45, on 4″ silicon wafers, have been irradiated in air with single laser pulses of 200 femtoseconds duration and 800 nm wave length. As sputter-deposited, the films are structurally amorphous. A laterally truncated Gaussian beam with a near-uniform fluence of ˜0.6 J/cm2 incident normally on such a film ablates 23 nm of the film. Cross-sectional transmission electron micrographs show that the surface of the remaining film is smooth and flat on a long-range scale, but contains densely distributed sharp nanoprotrusions that sometimes surpass the height of the original surface. Dark field micrographs of the remaining material show no nanograins. Neither does glancing angle X-ray diffraction with a beam illuminating many diffraction spots. By all evidence, the remaining film remains amorphous after the pulsed femtosecond irradiation. The same single pulse, but with an enhanced and slightly peaked fluence profile, creates a spot with flat peripheral terraces whose lateral extents shrink with depth, as scanning electron and atomic force micrographs revealed. Comparison of the various figures suggests that the sharp nanoprotrusions result from an ejection of material by brittle fraction and spallation, not from ablation by direct beam-solid interaction. Conditions under which spallation should dominate over ablation are discussed.

Spallative production of Li, Be and B in superbubbles

NASA Astrophysics Data System (ADS)

Parizot, Etienne

We investigate the spallative production of the light elements (Li, Be and B) associated with the evolution of a superbubble (SB) blown by repeated supernova explosions in an OB association. It is shown that if about ten percent of the SN energy can power the acceleration of particles from the material inside the SB, the observed abundances of LiBeB in halo stars, as a function of O, can be explained in a fully consistent way over several decades of metallicity. We investigate two different energy spectra for the EPs: the standard cosmic ray source spectrum and a specific `SB spectrum' as results from Bykov's SB acceleration mechanism. We find that the latter spectrum is more efficient in producing LiBeB, and that the SNR spectrum can be reconciled with the observational data if an imperfect mixing of the SN ejecta with the rest of the SB material and/or a selective acceleration is invoked (enhancing the C and O abundance amongst the EPs by a factor of ˜ 6). One consequence of the model is that the observed linear growth of Be and B abundances as a function of the metallicity expresses a dilution line rather than a continuous, monotonic increase throughout the Galaxy. We also find that the recent 6 Li observations in halo stars fit equally well in the framework of the SB model (see Parizot & Drury, 1999c, for more details).

Simulation of cosmic irradiation conditions in thick target arrangements

NASA Technical Reports Server (NTRS)

Theis, S.; Englert, P.; Reedy, R. C.; Arnold, J. R.

1986-01-01

One approach to simulate 2-pi irradiation conditions of planetary surfaces which has been widely applied in the past are bombardments of so called thick targets. A very large thick target was exposed recently to 2.1 GeV protons at the Bevatron-Bevalac in Berkeley. In a 100x100x180 cm steel-surrounded granodiorite target radioactive medium and high energy spallation products of the incident primary and of secondary particles were analyzed along the beam axis down to depths of 140 g/cm(2) in targets such as Cu, Ni, Co, Fe, T, Si, SiO2 and Al. Activities of these nuclides were exclusively determined via instrumental gamma-ray spectroscopy. Relative yields of neutron capture and spallation products induced in Co and Cu targets during the thick target bombardment are shown as a function of depth. The majority of the medium energy products such as Co-58 from Co targets exhibit a maximum at shallow depths of 40-60 g/cm(2) and then decrease exponentially. In a comparable 600 MeV proton bombarded thick target such a slight maximum for medium energy products was not observed. Rather, Co-58 activities in Co decreased steadily with the highest activity at the surface. The activities of the n-capture product Co-60 increase steadily starting at the surface. This indicates the rapidly growing flux of low energy neutrons within the target.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Albertazzi, Bruno; Ozaki, Norimasa; Zhakhovsky, Vasily

The understanding of fracture phenomena of a material at extremely high strain rates is a key issue for a wide variety of scientific research ranging from applied science and technological developments to fundamental science such as laser-matter interaction and geology. Despite its interest, its study relies on a fine multiscale description, in between the atomic scale and macroscopic processes, so far only achievable by large-scale atomic simulations. Direct ultrafast real-time monitoring of dynamic fracture (spallation) at the atomic lattice scale with picosecond time resolution was beyond the reach of experimental techniques. We show that the coupling between a high-power opticalmore » laser pump pulse and a femtosecond x-ray probe pulse generated by an x-ray free electron laser allows detection of the lattice dynamics in a tantalum foil at an ultrahigh strain rate of Embedded Image ~2 × 10 8 to 3.5 × 10 8 s -1. A maximal density drop of 8 to 10%, associated with the onset of spallation at a spall strength of ~17 GPa, was directly measured using x-ray diffraction. The experimental results of density evolution agree well with large-scale atomistic simulations of shock wave propagation and fracture of the sample. Our experimental technique opens a new pathway to the investigation of ultrahigh strain-rate phenomena in materials at the atomic scale, including high-speed crack dynamics and stress-induced solid-solid phase transitions.« less

Cyclic oxidation behavior of some plasma-sprayed coatings in Na2SO4-60%V2O5 environment

NASA Astrophysics Data System (ADS)

Singh, Harpreet; Prakash, Satya; Puri, Devendra; Phase, D. M.

2006-12-01

Cyclic oxidation behavior of plasma-sprayed NiCrAlY, Ni-20Cr, Ni3Al, and Stellite-6 coatings was investigated in an aggressive environment of Na2SO4-60%V2O5 by thermogravimetric techniques for 50 cycles. These coatings were deposited on a Ni-base superalloy, namely Superni 600; 10Fe-15.5Cr-0.5Mn-0.2C-Bal Ni (wt.%). X-ray diffraction, scanning electron microscopy/energy dispersive x-ray (SEM/EDX), and electron probe microanalyzer (EPMA) techniques were used to analyze the oxidation products. The uncoated superalloy suffered accelerated oxidation in the form of intense spallation of its oxide scale. After deposition of the NiCrAlY coating, the superalloy showed a minimum mass gain, whereas after application of the Stellite-6 coating, a maximum mass gain was observed among the coatings studied. All of the coatings were found to be useful in reducing the spallation of the substrate superalloy. Moreover, the coatings were successful in maintaining continuous surface contact with the base superalloy during the cyclic oxidation. The phases revealed for the oxidized coatings were mainly the oxides of chromium and/or aluminum and the spinels containing nickel-chromium/cobalt-chromium/nickel-aluminum mixed oxides, which are reported to be protective against high-temperature oxidation/hot corrosion.

Degradation of nonmodified and rhodium modified aluminide coating deposited on CMSX 4 superalloy.

PubMed

Zagula-Yavorska, Maryana; Wierzbińska, Małgorzata; Gancarczyk, Kamil; Sieniawski, Jan

2016-07-01

The Ni-base superalloy CMSX 4 used in the turbine blades of aircraft engines was coated with rhodium layer (0.5-μm thick). Next coated CMSX 4 superalloy was aluminized by the CVD method. The rhodium modified aluminide coating and nonmodified aluminide coating were oxidized at 1100°C at the air atmosphere. The rhodium modified aluminide coating showed about twice better oxidation resistance than the nonmodified one. The spallation equal 62% of the total area was observed on the surface of the nonmodified coating whereas only 36% spallation area was observed on the surface of the rhodium modified aluminide coating after the oxidation test. The oxide layer formed on the surface of the nonmodified coating was composed of nonprotective (Ni,Cr)Al2 O4 and (Ni,Cr)O phases. Aluminium in the coating reacts with oxygen, forming a protective α-Al2 O3 oxide on the surface of the rhodium modified aluminide coating. When the oxide cracks and spalls due to oxidation, additional aluminium from the coating diffuses to the surface to form the oxide. The presence of protective Al2 O3 oxide on the surface of the rhodium modified aluminide coating slows coating degradation. Therefore, rhodium modified aluminide coating has better oxidation resistance than the nonmodified one. © 2016 The Authors Journal of Microscopy © 2016 Royal Microscopical Society.

Thermohydraulic behavior of the liquid metal target of a spallation neutron source

DOE Office of Scientific and Technical Information (OSTI.GOV)

Takeda, Y.

1996-06-01

The author presents work done on three main problems. (1) Natural circulation in double coaxial cylindircal container: The thermohydraulic behaviour of the liquid metal target of the spallation neutron source at PSI has been investigated. The configuration is a natural-circulation loop in a concentric double-tube-type container. The results show that the natural-circulation loop concept is valid for the design phase of the target construction, and the current specified design criteria will be fulfilled with the proposed parameter values. (2) Flow around the window: Water experiments were performed for geometry optimisation of the window shape of the SINQ container for avoidingmore » generating recirculation zones at peripheral area and the optimal cooling of the central part of the beam entrance window. Flow visualisation technique was mainly used for various window shapes, gap distance between the window and the guide tube edge. (3) Flow in window cooling channels: Flows in narrow gaps of cooling channels of two different types of windows were studied by flow visualisation techniques. One type is a slightly curved round cooling channel and the other is hemispherical shape, both of which have only 2 mm gap distance and the water inlet is located on one side and flows out from the opposite side. In both cases, the central part of the flow area has lower velocity than peripheral area.« less

Mercury target R&D for the Oak Ridge spallation neutron source

DOE Office of Scientific and Technical Information (OSTI.GOV)

Haines, J.R.; DiStefano, J.; Farrell, K.

1996-06-01

The conceptual design for the Oak Ridge Spallation Neutron Source (ORSNS) incorporates liquid mercury as its reference target material. A flowing liquid target was selected mainly because of the increased power handling capability possible with the convective transport process. The major reasons for choosing mercury as the liquid target material are because it: (1) is a liquid at room temperature, (2) has good heat transport properties, and (3) has a high atomic number and mass density resulting in high neutron yield and source brightness. Since liquid targets are not widely utilized in presently operating accelerator targets and because of themore » challenges posed by the intense, pulsed thermal energy deposition ({approximately}20-100 kJ deposited during each 1-10 {mu}s pulse), considerable R&D is planned for the mercury target concept. The key feasibility issue that will be addressed in early R&D efforts are the effects of the thermal shock environment, which will include development and testing of approaches to mitigate these effects. Materials compatiblity and ES&H issues associated with the use of liquid mercury are also of major importance in early R&D efforts. A brief description of the mercury target design concept, results of initial evaluations of its performance characteristics, identification of its critical issues, and an outline of the R&D program aimed at addressing these issues will be presented.« less

Moisture-Induced Delayed Alumina Scale Spallation on a Ni(Pt)Al Coating (Preprint)

DTIC Science & Technology

2009-04-01

with increase in p(H2O) [21,35 Janakiraman 1999, Maris- Sida 2003]. However the same effect was not especially evident for the more oxidation resistant...Tolpygo 2007, Maris- sida 2003). Crystallographically aligned surface striations and pits are also evident, presumably an artifact of the CVD...A similar but less severe effect was reported for the same coating on Rene´N5 (35 Maris- Sida , 2003), exhibiting a loss of 1 mg/cm2 in wet air

SNS Proton Beam Window Disposal

NASA Astrophysics Data System (ADS)

Popova, Irina; Gallmeier, Franz X.; Trotter, Steven

2017-09-01

In order to support the disposal of the proton beam window assembly of the Spallation Neutron Source beamline to the target station, waste classification analyses are performed. The window has a limited life-time due to radiation-induced material damage. Analyses include calculation of the radionuclide inventory and shielding analyses for the transport package/container to ensure that the container is compliant with the transportation and waste management regulations. In order to automate this procedure and minimize manual work a script in Perl language was written.

Mercury Thermal Hydraulic Loop (MTHL) Summary Report

DOE Office of Scientific and Technical Information (OSTI.GOV)

Felde, David K.; Crye, Jason Michael; Wendel, Mark W.

2017-03-01

The Spallation Neutron Source (SNS) is a high-power linear accelerator built at Oak Ridge National Laboratory (ORNL) which incorporates the use of a flowing liquid mercury target. The Mercury Thermal Hydraulic Loop (MTHL) was constructed to investigate and verify the heat transfer characteristics of liquid mercury in a rectangular channel. This report provides a compilation of previously reported results from the water-cooled and electrically heated straight and curved test sections that simulate the geometry of the window cooling channel in the target nose region.

Moisture-Induced Delamination Video of an Oxidized Thermal Barrier Coating

NASA Technical Reports Server (NTRS)

Smialek, James L.; Zhu, Dongming; Cuy, Michael D.

2008-01-01

PVD TBC coatings were thermally cycled to near-failure at 1150 C. Normal failure occurred after 200-300 1-hr cycles with only moderate weight gains (0.5 mg/cm2). Delamination and buckling was often delayed until well after cooldown (desktop spallation), but could be instantly induced by the application of water drops, as shown in an accompanying video-recording. Moisture therefore plays a primary role in delayed desktop TBC failure. Hydrogen embrittlement is proposed as the underlying mechanism.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Lindroos M.; Calaga R.; Bousson S.

In 2003 the joint European effort to design a European Spallation Source (ESS) resulted in a set of reports, and in May 2009 Lund was agreed to be the ESS site. The ESS Scandinavia office has since then worked on setting all the necessary legal and organizational matters in place so that the Design Update and construction can be started in January 2011, in collaboration with European partners. The Design Update phase is expected to end in 2012, to be followed by a construction phase, with first neutrons expected in 2018-2019.

A Compendium of Scale Surface Microstructures: Ni(pt)al Coatings Oxidized at 1150 C for 2000 1-h Cycles

NASA Technical Reports Server (NTRS)

Smialek, James L.; Garg, Anita

2010-01-01

The surface structure of scales formed on Ni(Pt)Al coatings was characterized by SEM/EDS/BSE in plan view. Two nominally identical {100} samples of aluminide coated CMSX4 single crystal were oxidized at 1150 C for 2000 1-h cycles and were found to produce somewhat disparate behavior. One sample, with less propensity for coating grain boundary ridge deformation, presented primarily alpha-Al2O3 scale structures, with minimal weight loss and spallation. The original scale structure, still retained over most of the sample, consisted of the classic theta-alpha transformation-induced ridge network structure, with approx. 25 nm crystallographic steps and terraces indicative of surface rearrangement to low energy alumina planes. The scale grain boundary ridges were often decorated with a fine, uniform distribution of (Hf,Ti)O2 particles. Another sample, producing steady state weight losses, exhibited much interfacial spallation and a complex assortment of different structures. Broad areas of interfacial spalling, crystallographically-faceted (Ni,Co)(Al,Cr)2O4 spinel, with an alpha-Al2O3 base scale, were the dominant features. Other regions exhibited nodular spinel grains, with fine or (Ta,Ti)-rich (rutile) particles decorating or interspersed with the spinel. While these features were consistent with a coating that presented more deformation at extruded grain boundaries, the root cause of the different behavior between the duplicate samples could not be conclusively identified.

Dynamic fracture of tantalum under extreme tensile stress

DOE PAGES

Albertazzi, Bruno; Ozaki, Norimasa; Zhakhovsky, Vasily; ...

2017-06-02

The understanding of fracture phenomena of a material at extremely high strain rates is a key issue for a wide variety of scientific research ranging from applied science and technological developments to fundamental science such as laser-matter interaction and geology. Despite its interest, its study relies on a fine multiscale description, in between the atomic scale and macroscopic processes, so far only achievable by large-scale atomic simulations. Direct ultrafast real-time monitoring of dynamic fracture (spallation) at the atomic lattice scale with picosecond time resolution was beyond the reach of experimental techniques. We show that the coupling between a high-power opticalmore » laser pump pulse and a femtosecond x-ray probe pulse generated by an x-ray free electron laser allows detection of the lattice dynamics in a tantalum foil at an ultrahigh strain rate of Embedded Image ~2 × 10 8 to 3.5 × 10 8 s -1. A maximal density drop of 8 to 10%, associated with the onset of spallation at a spall strength of ~17 GPa, was directly measured using x-ray diffraction. The experimental results of density evolution agree well with large-scale atomistic simulations of shock wave propagation and fracture of the sample. Our experimental technique opens a new pathway to the investigation of ultrahigh strain-rate phenomena in materials at the atomic scale, including high-speed crack dynamics and stress-induced solid-solid phase transitions.« less

Investigation of Spheromak Plasma Cooling through Metallic Liner Spallation during Compression

NASA Astrophysics Data System (ADS)

Ross, Keeton; Mossman, Alex; Young, William; Ivanov, Russ; O'Shea, Peter; Howard, Stephen

2016-10-01

Various magnetic-target fusion (MTF) reactor concepts involve a preliminary magnetic confinement stage, followed by a metallic liner implosion that compresses the plasma to fusion conditions. The process is repeated to produce a pulsed, net-gain energy system. General Fusion, Inc. is pursuing one scheme that involves the compression of spheromak plasmas inside a liner formed by a collapsing vortex of liquid Pb-Li. The compression is driven by focused acoustic waves launched by gas-driven piston impacts. Here we describe a project to exploring the effects of possible liner spallation during compression on the spheromaks temperature, lifetime, and stability. We employ a 1 J, 10 ns pulsed YAG laser at 532nm focused onto a thin film of Li or Al to inject a known quantity of metallic impurities into a spheromak plasma and then measure the response. Diagnostics including visible and ultraviolet spectrometers, ion Doppler, B-probes, and Thomson scattering are used for plasma characterization. We then plan to apply the trends measured under these controlled conditions to evaluate the role of wall impurities during `field shots', where spheromaks are compressed through a chemically driven implosion of an aluminum flux conserver. The hope is that with further study we could more accurately include the effect of wall impurities on the fusion yield of a reactor-scale MTF system. Experimental procedures and results are presented, along with their relation to other liner-driven, MTF schemes. -/a

Cavitation Damage Experiments for Mercury Spallation Targets At the LANSCE WNR in 2008

DOE Office of Scientific and Technical Information (OSTI.GOV)

Riemer, Bernie; Wendel, Mark W; Felde, David K

2010-01-01

Proton beam experiments investigating cavitation damage in short pulse mercury spallation targets were performed at LANSCE WNR in July of 2008. They included two main areas for investigation: damage dependence on mercury velocity using geometry more prototypic to the SNS target than previously employed and damage dependence on incident proton beam flux intensity. The flow dependence experiment employed six test targets with mercury velocity in the channel ranging from 0 to more than 4 m/s. Each was hit with 100 WNR beam pulses with peak proton flux equivalent to that of SNS operating at 2.7 MW. Damage dependence on incidentmore » proton beam flux intensity was also investigated with three intensity levels used on simple rectangular shaped targets without mercury flow. Intensity variation was imposed by focusing the beam differently while maintaining protons per pulse. This kept total energy deposited in each target constant. A fourth test target was hit with various beams: constant protons and varied spot size; constant spot size and varied protons. No damage will be assessed in this case. Instead, acoustic emissions associated with cavitation collapse were measured by laser Doppler vibrometer (LDV) from readings of exterior vessel motions as well as by mercury wetted acoustic transducers. This paper will provide a description of the experiment and present available results. Damage assessment will require several months before surface analysis can be completed and was not available in time for IWSMT-9.« less

Cyclic Oxidation Testing and Modelling: A NASA Lewis Perspective

NASA Technical Reports Server (NTRS)

Smialek, J. L.; Nesbitt, J. A.; Barrett, C. A.; Lowell, C. E.

2000-01-01

The Materials Division of the NASA Lewis Research Center has been heavily involved in the cyclic oxidation of high temperature materials for 30 years. Cyclic furnace and burner rig apparati have been developed, refined, and replicated to provide a large scale facility capable of evaluating many materials by a standard technique. Material behavior is characterized by weight change data obtained throughout the test, which has been modelled in a step-wise process of scale growth and spallation. This model and a coupled diffusion model have successfully described cyclic behavior for a number of systems and have provided insights regarding life prediction and variations in the spalling process. Performance ranking and mechanistic studies are discussed primarily for superalloys and coating alloys. Similar cyclic oxidation studies have been performed on steels, intermetallic compounds, thermal barrier coatings, ceramics, and ceramic composites. The most common oxidation test was performed in air at temperatures ranging from 800 deg. to 1600 C, for times up to 10000 h, and for cycle durations of 0.1 to 1000 h. Less controlled, but important, test parameters are the cooling temperature and humidity level. Heating and cooling rates are not likely to affect scale spallation. Broad experience has usually allowed for considerable focus and simplification of these test parameters, while still revealing the principal aspects of material behavior and performance. Extensive testing has been performed to statistically model the compositional effects of experimental alloys and to construct a comprehensive database of complex commercial alloys.

Ranking and validation of spallation models for isotopic production cross sections of heavy residua

NASA Astrophysics Data System (ADS)

Sharma, Sushil K.; Kamys, Bogusław; Goldenbaum, Frank; Filges, Detlef

2017-07-01

The production cross sections of isotopically identified residual nuclei of spallation reactions induced by 136Xe projectiles at 500AMeV on hydrogen target were analyzed in a two-step model. The first stage of the reaction was described by the INCL4.6 model of an intranuclear cascade of nucleon-nucleon and pion-nucleon collisions whereas the second stage was analyzed by means of four different models; ABLA07, GEM2, GEMINI++ and SMM. The quality of the data description was judged quantitatively using two statistical deviation factors; the H-factor and the M-factor. It was found that the present analysis leads to a different ranking of models as compared to that obtained from the qualitative inspection of the data reproduction. The disagreement was caused by sensitivity of the deviation factors to large statistical errors present in some of the data. A new deviation factor, the A factor, was proposed, that is not sensitive to the statistical errors of the cross sections. The quantitative ranking of models performed using the A-factor agreed well with the qualitative analysis of the data. It was concluded that using the deviation factors weighted by statistical errors may lead to erroneous conclusions in the case when the data cover a large range of values. The quality of data reproduction by the theoretical models is discussed. Some systematic deviations of the theoretical predictions from the experimental results are observed.

Theoretical investigation of the thermal hydraulic behaviour of a slab-type liquid metal target

DOE Office of Scientific and Technical Information (OSTI.GOV)

Dury, T.V.; Smith, B.L.

1996-06-01

The thermal hydraulics codes CFDS-FLOW3D and ASTEC have been used to simulate a slabtype design of ESS spallation target. This design is single-skinned, and of tapering form (in the beam direction), with rounded sides in a cross-section through a plane normal to the beam. The coolant fluid used is mercury, under forced circulation, with an inlet temperature of 180{degrees}C. The goal of these computer studies was to understand the behaviour of the coolant flow, and hence to arrive at a design which optimises the heat extraction for a given beam power - in the sense of: (1) minimising the peakmore » local fluid temperature within the target, (2) maintaining an acceptable temperature level and distribution over and through the target outer wall, (3) keeping the overall fluid pressure loss through the complete target to a minimum, (4) staying within the physical limits of overall size required, particularly in the region of primary spallation. Two- and three-dimensional models have been used, with different arrangements and design of internal baffles, and different coolant flow distributions at the target inlet. Nominal total inlet mass flow was 245 kg/s, and a heat deposition profile used which was based on the proton beam energy distribution. This gave a nominal total heat load of 3.23 MW - of which 8.2kW were deposited in the window steel.« less

Overview of the Neutron experimental facilities at LANSCE

DOE Office of Scientific and Technical Information (OSTI.GOV)

Mocko, Michal

2016-06-30

This presentation gives an overview of the neutron experimental facilities at LANSCE. The layout is mentioned in detail, with a map of the south-side experimental facilities, information on Target-4 and the Lujan Center. Then it goes into detail about neutron sources, specifically continuous versus pulsed. Target 4 is then discussed. In conclusion, we have introduced the south-side experimental facilities in operation at LANSCE. 1L target and Target 4 provide complementary neutron energy spectra. Two spallation neutron sources taken together cover more than 11 orders of magnitude in neutron energy.

Source amplitudes of NTS explosions inferred from Rayleigh waves at Albuquerque and Tucson. Topical report

DOE Office of Scientific and Technical Information (OSTI.GOV)

Bache, T.C.; Rodi, W.L.; Mason, B.F.

1978-06-01

Comparing observed and synthetic seismograms, source amplitudes of NTS explosions are inferred from Rayleigh wave recordings from the WWSSN stations at Albuquerque, New Mexico (ALQ) and Tucson, Arizona (TUC). The potential influence of source complexities, particularly surface spallation and related phenomena, is studied in detail. As described in earlier work by Bache, Rodi and Harkrider, the earth model for the synthetic were converted from observations at ALQ and TUC. The agreement of observed and synthetic seismograms is quite good and is sensitive to important features of the source.

A high-rate 10B-loaded liquid scintillation detector for parity-violation studies in neutron resonances

NASA Astrophysics Data System (ADS)

Yen, Yi-Fen; Bowman, J. D.; Bolton, R. D.; Crawford, B. E.; Delheij, P. P. J.; Hart, G. W.; Haseyama, T.; Frankle, C. M.; Iinuma, M.; Knudson, J. N.; Masaike, A.; Masuda, Y.; Matsuda, Y.; Mitchell, G. E.; Penttilä, S. I.; Roberson, N. R.; Seestrom, S. J.; Sharapov, E.; Shimizu, H. M.; Smith, D. A.; Stephenson, S. L.; Szymanski, J. J.; Yoo, S. H.; Yuan, V. W.

2000-06-01

We have developed a large-area 10B-loaded liquid scintillation detector for parity-violation studies in neutron resonances with high instantaneous neutron fluxes from the LANSCE short-pulse spallation source. The detector has an efficiency of 95%, 85% and 71% at neutron energies of 10, 100 and 1000 eV, respectively. The neutron mean capture time in the detector is (416±5) ns. We describe the detector and the current-mode signal processing system, that can handle neutron rates up to 500 MHz.

Shielding and Activation Analyses for BTF Facility at SNS

NASA Astrophysics Data System (ADS)

Popova, Irina; Gallmeier, Franz X.

2017-09-01

The beam test facility (BTF), which simulates front end of the Spallation Neutron Source (SNS), has been built at the SNS, and is preparing for commissioning. The BTF has been assembled and will operate in one of service buildings at the site. The 2.5 MeV proton beam, produced in the facility, will be stopped in the beam dump. In order to support BTF project from radiation protection site, neutronics simulations and activation analyses were performed to evaluate the necessary shielding around the facility and radionuclide inventory of the beam stop.

The very low angle detector for high-energy inelastic neutron scattering on the VESUVIO spectrometer

NASA Astrophysics Data System (ADS)

Perelli Cippo, E.; Gorini, G.; Tardocchi, M.; Pietropaolo, A.; Andreani, C.; Senesi, R.; Rhodes, N. J.; Schooneveld, E. M.

2008-05-01

The Very Low Angle Detector (VLAD) bank has been installed on the VESUVIO spectrometer at the ISIS spallation neutron source. The new device allows for high-energy inelastic neutron scattering measurements, at energies above 1 eV, maintaining the wave vector transfer lower than 10Å-1. This opens a still unexplored region of the kinematical (q, ω) space, enabling new and challenging experimental investigations in condensed matter. This paper describes the main instrumental features of the VLAD device, including instrument design, detector response, and calibration procedure.

Note: Versatile sample stick for neutron scattering experiments in high electric fields

DOE Office of Scientific and Technical Information (OSTI.GOV)

Bartkowiak, M., E-mail: marek.bartkowiak@psi.ch; White, J. S.; Laboratory for Quantum Magnetism, Ecole Polytechnique Fédérale de Lausanne

2014-02-15

We present a versatile high voltage sample stick that fits into all cryomagnets and standard cryostats at the Swiss Spallation Neutron Source, Paul Scherrer Institut, and which provides a low effort route to neutron scattering experiments that combine electric field with low temperature and magnetic field. The stick allows for voltages up to 5 kV and can be easily adapted for different scattering geometries. We discuss the design consideration and thermal behavior of the stick, and give one example to showcase the abilities of the device.

Two-dimensional beam profiles and one-dimensional projections

NASA Astrophysics Data System (ADS)

Findlay, D. J. S.; Jones, B.; Adams, D. J.

2018-05-01

One-dimensional projections of improved two-dimensional representations of transverse profiles of particle beams are proposed for fitting to data from harp-type monitors measuring beam profiles on particle accelerators. Composite distributions, with tails smoothly matched on to a central (inverted) parabola, are shown to give noticeably better fits than single gaussian and single parabolic distributions to data from harp-type beam profile monitors all along the proton beam transport lines to the two target stations on the ISIS Spallation Neutron Source. Some implications for inferring beam current densities on the beam axis are noted.

Ceramic thermal barrier coatings for commercial gas turbine engines

NASA Technical Reports Server (NTRS)

Meier, Susan Manning; Gupta, Dinesh K.; Sheffler, Keith D.

1991-01-01

The paper provides an overview of the short history, current status, and future prospects of ceramic thermal barrier coatings for gas turbine engines. Particular attention is given to plasma-sprayed and electron beam-physical vapor deposited yttria-stabilized (7 wt pct Y2O3) zirconia systems. Recent advances include improvements in the spallation life of thermal barrier coatings, improved bond coat composition and spraying techniques, and improved component design. The discussion also covers field experience, life prediction modeling, and future directions in ceramic coatings in relation to gas turbine engine design.

Lithium synthesis in microquasar accretion.

PubMed

Iocco, Fabio; Pato, Miguel

2012-07-13

We study the synthesis of lithium isotopes in the hot tori formed around stellar mass black holes by accretion of the companion star. We find that sizable amounts of both stable isotopes 6Li and 7Li can be produced, the exact figures varying with the characteristics of the torus and reaching as much as 10(-2) M⊙ for each isotope. This mass output is enough to contaminate the entire Galaxy at a level comparable with the original, pregalactic amount of lithium and to overcome other sources such as cosmic-ray spallation or stellar nucleosynthesis.

Steps Towards Large Scale Production of High-Spin Hafnium Isomers by Spallation Reactions

DTIC Science & Technology

2008-02-25

and 22Na radionuclides are schematically shown in Fig. 6. The 511 keV γ–ray line correspond to the positron annihilation peak. A large Compton...The annihilation of the positron emitted following the β+–decay of 22Na leads to the 511 keV peak in the γ–ray spectra. Gamma–ray activity spectra...figure. Gamma–rays are labeled with the radionuclide to which they belong. The 511 keV γ–ray line is the positron annihilation peak and correspond to

Determination of the axial-vector weak coupling constant with ultracold neutrons.

PubMed

Liu, J; Mendenhall, M P; Holley, A T; Back, H O; Bowles, T J; Broussard, L J; Carr, R; Clayton, S; Currie, S; Filippone, B W; García, A; Geltenbort, P; Hickerson, K P; Hoagland, J; Hogan, G E; Hona, B; Ito, T M; Liu, C-Y; Makela, M; Mammei, R R; Martin, J W; Melconian, D; Morris, C L; Pattie, R W; Pérez Galván, A; Pitt, M L; Plaster, B; Ramsey, J C; Rios, R; Russell, R; Saunders, A; Seestrom, S J; Sondheim, W E; Tatar, E; Vogelaar, R B; VornDick, B; Wrede, C; Yan, H; Young, A R

2010-10-29

A precise measurement of the neutron decay β asymmetry A₀ has been carried out using polarized ultracold neutrons from the pulsed spallation ultracold neutron source at the Los Alamos Neutron Science Center. Combining data obtained in 2008 and 2009, we report A₀ = -0.119 66±0.000 89{-0.001 40}{+0.001 23}, from which we determine the ratio of the axial-vector to vector weak coupling of the nucleon g{A}/g{V}=-1.275 90{-0.004 45}{+0.004 09}.

Moisture-Induced Delamination Video of an Oxidized Thermal Barrier Coating

NASA Technical Reports Server (NTRS)

Smialek, James L.; Zhu, Dongming; Cuy, Michael D.

2008-01-01

PVD TBC coatings were thermally cycled to near-failure at 1150 C. Normal failure occurred after 200 to 300 1-hr cycles with only moderate weight gains (0.5 mg/sq cm). Delamination and buckling was often delayed until well after cooldown (desktop spallation), but could be instantly induced by the application of water drops, as shown in a video clip which can be viewed by clicking on figure 2 of this report. Moisture therefore plays a primary role in delayed desktop TBC failure. Hydrogen embrittlement is proposed as the underlying mechanism.

WORKER INHALATION DOSE COEFFICIENTS FOR RADIONUCLIDES NOT PREVIOUSLY IDENTIFIED IN ICRP PUBLICATION 68

DOE Office of Scientific and Technical Information (OSTI.GOV)

McLaughlin, David A; Schwahn, Scott O

2011-01-01

While inhalation dose coefficients are provided for about 800 radionuclides in International Commission on Radiological Protection (ICRP) Publication 68, many radionuclides of practical dosimetric interest for facilities such as high-energy proton accelerators are not specifically addressed, nor are organ-specific dose coefficients tabulated. The ICRP Publication 68 methodology is used, along with updated radiological decay data and metabolic data, to identify committed equivalent dose coefficients [hT(50)] and committed effective dose coefficients [e(50)] for radionuclides produced at the Oak Ridge National Laboratory s Spallation Neutron Source.

Accelerator driven neutron source design via beryllium target and 208Pb moderator for boron neutron capture therapy in alternative treatment strategy by Monte Carlo method.

PubMed

Khorshidi, Abdollah

2017-01-01

The reactor has increased its area of application into medicine especially boron neutron capture therapy (BNCT); however, accelerator-driven neutron sources can be used for therapy purposes. The present study aimed to discuss an alternative method in BNCT functions by a small cyclotron with low current protons based on Karaj cyclotron in Iran. An epithermal neutron spectrum generator was simulated with 30 MeV proton energy for BNCT purposes. A low current of 300 μA of the proton beam in spallation target concept via 9Be target was accomplished to model neutron spectrum using 208Pb moderator around the target. The graphite reflector and dual layer collimator were planned to prevent and collimate the neutrons produced from proton interactions. Neutron yield per proton, energy distribution, flux, and dose components in the simulated head phantom were estimated by MCNPX code. The neutron beam quality was investigated by diverse filters thicknesses. The maximum epithermal flux transpired using Fluental, Fe, Li, and Bi filters with thicknesses of 7.4, 3, 0.5, and 4 cm, respectively; as well as the epithermal to thermal neutron flux ratio was 161. Results demonstrated that the induced neutrons from a low energy and low current proton may be effective in tumor therapy using 208Pb moderator with average lethargy and also graphite reflector with low absorption cross section to keep the generated neutrons. Combination of spallation-based BNCT and proton therapy can be especially effective, if a high beam intensity cyclotron becomes available.

Measurement of interface strength by a laser spallation technique

NASA Astrophysics Data System (ADS)

Gupta, V.; Argon, A. S.; Parks, D. M.; Cornie, J. A.

A LASER spallation experiment has been developed to measure the strength of planar interfaces between a substrate and a thin coating (in the thickness range of 0.3-3 μm). In this technique a laser pulse of a high enough energy and a pre-determined duration is converted into a pressure pulse of a critical amplitude and width that is sent through the substrate toward the free surface with the coating. The reflected tensile wave from the free surface of the coating pries-off the coating. The critical stress amplitude that accomplishes the removal of the coating is determined from a computer simulation of the process. The simulation itself is verified by means of a piezo-electric crystal probe that is capable of mapping out the profile of the stress pulse generated by the laser pulse. Interface strength values ranging from 3.7 to 10.5 GPa were determined for the Si/SiC system. For the interfaces between pyrolytic graphite and SiC coatings an average strength of 7.2 GPA was measured, while the corresponding interface strength between a Pitch-55 type ribbon with a fiber-like morphology and SiC coatings was found to be 0.23 GPa. Intrinsic strengths of SiC coatings and Si crystal were also determined using this technique. These were, on the average, 8.6 GPa for Si crystals and 11.9 GPa for a SiC coating. Furthermore, the potential of the laser technique to determine the interface toughness was also demonstrated, provided well-characterizable flaws can be planted on the interface.

Operational performance characteristics of the WISH detector array on the ISIS spallation neutron source

NASA Astrophysics Data System (ADS)

Duxbury, D.; Khalyavin, D.; Manuel, P.; Raspino, D.; Rhodes, N.; Schooneveld, E.; Spill, E.

2014-12-01

The performance of the position sensitive neutron detector array of the WISH diffractometer is discussed. WISH (Wide angle In a Single Histogram) is one of the seven instruments currently available for users on the second target station (TS2) of the ISIS spallation neutron source, and is used mainly for magnetic studies of materials. WISH is instrumented with an array of 10 detector panels, covering an angular range of 320o, orientated in two semi-cylindrical annuli around a central sample position at a radius of 2.2m. In total the 10 detector panels are composed of 1520 3He based position sensitive detector tubes. Each tube has an active length of one metre, a diameter of 8mm and is filled with 3He at 15 bar. The specification for the WISH detectors included a neutron detection efficiency of 50% at a neutron wavelength of 1Å with good gamma rejection. A position resolution better than 8 mm FWHM along the length of the tubes was also required which has been met experimentally. Results obtained from the detector arrays showing pulse height and positional information both prior to and post installation are shown. The first 5 of the 10 detector panels have been operational since 2009, and comparable diffraction data from powder and single crystal samples taken from the remaining 5 panels (installation completed in 2013) shows that we have a detector array with a highly stable performance which is easily assembled and maintained. Finally some real user data is shown, highlighting the excellent quality of data attainable with this instrument.

On scaling cosmogenic nuclide production rates for altitude and latitude using cosmic-ray measurements

NASA Astrophysics Data System (ADS)

Desilets, Darin; Zreda, Marek

2001-11-01

The wide use of cosmogenic nuclides for dating terrestrial landforms has prompted a renewed interest in characterizing the spatial distribution of terrestrial cosmic rays. Cosmic-ray measurements from neutron monitors, nuclear emulsions and cloud chambers have played an important role in developing new models for scaling cosmic-ray neutron intensities and, indirectly, cosmogenic production rates. Unfortunately, current scaling models overlook or misinterpret many of these data. In this paper, we describe factors that must be considered when using neutron measurements to determine scaling formulations for production rates of cosmogenic nuclides. Over the past 50 years, the overwhelming majority of nucleon flux measurements have been taken with neutron monitors. However, in order to use these data for scaling spallation reactions, the following factors must be considered: (1) sensitivity of instruments to muons and to background, (2) instrumental biases in energy sensitivity, (3) solar activity, and (4) the way of ordering cosmic-ray data in the geomagnetic field. Failure to account for these factors can result in discrepancies of as much as 7% in neutron attenuation lengths measured at the same location. This magnitude of deviation can result in an error on the order of 20% in cosmogenic production rates scaled from 4300 m to sea level. The shapes of latitude curves of nucleon flux also depend on these factors to a measurable extent, thereby causing additional uncertainties in cosmogenic production rates. The corrections proposed herein significantly improve our ability to transfer scaling formulations based on neutron measurements to scaling formulations applicable to spallation reactions, and, therefore, constitute an important advance in cosmogenic dating methodology.

Conceptual design of the time-of-flight backscattering spectrometer MIRACLES, at the European Spallation Source

NASA Astrophysics Data System (ADS)

Tsapatsaris, N.; Lechner, R. E.; Markó, M.; Bordallo, H. N.

2016-08-01

In this work, we present the conceptual design of the backscattering time-of-flight spectrometer MIRACLES approved for construction at the long-pulse European Spallation Source (ESS). MIRACLES's unparalleled combination of variable resolution, high flux, extended energy, and momentum transfer (0.2-6 Å-1) ranges will open new avenues for neutron backscattering spectroscopy. Its remarkable flexibility can be attributed to 3 key elements: the long-pulse time structure and low repetition rate of the ESS neutron source, the chopper cascade that tailors the moderator pulse in the primary part of the spectrometer, and the bent Si(111) analyzer crystals arranged in a near-backscattering geometry in the secondary part of the spectrometer. Analytical calculations combined with instrument Monte-Carlo simulations show that the instrument will provide a variable elastic energy resolution, δ(ħ ω), between 2 and 32 μeV, when using a wavelength of λ ≈ 6.267 Å (Si(111)-reflection), with an energy transfer range, ħ ω, centered at the elastic line from -600 to +600 μeV. In addition, when selecting λ ≈ 2.08 Å (i.e., the Si(333)-reflection), δ(ħ ω) can be relaxed to 300 μeV and ħ ω from about 10 meV in energy gain to ca -40 meV in energy loss. Finally, the dynamic wavelength range of MIRACLES, approximately 1.8 Å, can be shifted within the interval of 2-20 Å to allow the measurement of low-energy inelastic excitations.

Conceptual design of the time-of-flight backscattering spectrometer, MIRACLES, at the European Spallation Source.

PubMed

Tsapatsaris, N; Lechner, R E; Markó, M; Bordallo, H N

2016-08-01

In this work, we present the conceptual design of the backscattering time-of-flight spectrometer MIRACLES approved for construction at the long-pulse European Spallation Source (ESS). MIRACLES's unparalleled combination of variable resolution, high flux, extended energy, and momentum transfer (0.2-6 Å(-1)) ranges will open new avenues for neutron backscattering spectroscopy. Its remarkable flexibility can be attributed to 3 key elements: the long-pulse time structure and low repetition rate of the ESS neutron source, the chopper cascade that tailors the moderator pulse in the primary part of the spectrometer, and the bent Si(111) analyzer crystals arranged in a near-backscattering geometry in the secondary part of the spectrometer. Analytical calculations combined with instrument Monte-Carlo simulations show that the instrument will provide a variable elastic energy resolution, δ(ħ ω), between 2 and 32 μeV, when using a wavelength of λ ≈ 6.267 Å (Si(111)-reflection), with an energy transfer range, ħ ω, centered at the elastic line from -600 to +600 μeV. In addition, when selecting λ ≈ 2.08 Å (i.e., the Si(333)-reflection), δ(ħ ω) can be relaxed to 300 μeV and ħ ω from about 10 meV in energy gain to ca -40 meV in energy loss. Finally, the dynamic wavelength range of MIRACLES, approximately 1.8 Å, can be shifted within the interval of 2-20 Å to allow the measurement of low-energy inelastic excitations.

Cross-sections of residual nuclei from deuteron irradiation of thin thorium target at energy 7 GeV

NASA Astrophysics Data System (ADS)

Vespalec, Radek; Adam, Jindrich; Baldin, Anton Alexandrovich; Khushvaktov, Jurabek; Solnyshkin, Alexander Alexandrovich; Tsoupko-Sitnikov, Vsevolod Mikhailovich; Tyutyunikov, Sergey Ivanovich; Vrzalova, Jitka; Zavorka, Lukas; Zeman, Miroslav

2017-09-01

The residual nuclei yields are of great importance for the estimation of basic radiation-technology characteristics (like a total target activity, production of long-lived nuclides etc.) of accelerator driven systems planned for transmutation of spent nuclear fuel and for a design of radioisotopes production facilities. Experimental data are also essential for validation of nuclear codes describing various stages of a spallation reaction. Therefore, the main aim of this work is to add new experimental data in energy region of relativistic deuterons, as similar data are missing in nuclear databases. The sample made of thin natural thorium foil was irradiated at JINR Nuclotron accelerator with a deuteron beam of the total kinetic energy 7 GeV. Integral number of deuterons was determined with the use of aluminum activation detectors. Products of deuteron induced spallation reaction were qualified and quantified by means of gamma-ray spectroscopy method. Several important spectroscopic corrections were applied to obtain results of high accuracy. Experimental cumulative and independent cross-sections were determined for more than 80 isotopes including meta-stable isomers. The total uncertainty of results rarely exceeded 9%. Experimental results were compared with MCNP6.1 Monte-Carlo code predictions. Generally, experimental and calculated cross-sections are in a reasonably good agreement, with the exception of a few light isotopes in a fragmentation region, where the calculations are highly under-estimated. Measured data will be useful for future development of high-energy nuclear codes. After completion, final data will be added into the EXFOR database.

The negligible chondritic contribution in the lunar soils water.

PubMed

Stephant, Alice; Robert, François

2014-10-21

Recent data from Apollo samples demonstrate the presence of water in the lunar interior and at the surface, challenging previous assumption that the Moon was free of water. However, the source(s) of this water remains enigmatic. The external flux of particles and solid materials that reach the surface of the airless Moon constitute a hydrogen (H) surface reservoir that can be converted to water (or OH) during proton implantation in rocks or remobilization during magmatic events. Our original goal was thus to quantify the relative contributions to this H surface reservoir. To this end, we report NanoSIMS measurements of D/H and (7)Li/(6)Li ratios on agglutinates, volcanic glasses, and plagioclase grains from the Apollo sample collection. Clear correlations emerge between cosmogenic D and (6)Li revealing that almost all D is produced by spallation reactions both on the surface and in the interior of the grains. In grain interiors, no evidence of chondritic water has been found. This observation allows us to constrain the H isotopic ratio of hypothetical juvenile lunar water to δD ≤ -550‰. On the grain surface, the hydroxyl concentrations are significant and the D/H ratios indicate that they originate from solar wind implantation. The scattering distribution of the data around the theoretical D vs. (6)Li spallation correlation is compatible with a chondritic contribution <15%. In conclusion, (i) solar wind implantation is the major mechanism responsible for hydroxyls on the lunar surface, and (ii) the postulated chondritic lunar water is not retained in the regolith.

Localized atomic segregation in the spalled area of a Zr50Cu40Al10 bulk metallic glasses induced by laser-shock experiment

NASA Astrophysics Data System (ADS)

Jodar, B.; Loison, D.; Yokoyama, Y.; Lescoute, E.; Nivard, M.; Berthe, L.; Sangleboeuf, J.-C.

2018-02-01

Laser-shock experiments were performed on a ternary {Zr50{Cu}40{Al}10} bulk metallic glass. A spalling process was studied through post-mortem analyses conducted on a recovered sample and spall. Scanning electron microscopy magnification of fracture surfaces revealed the presence of a peculiar feature known as cup-cone. Cups are found on sample fracture surface while cones are observed on spall. Two distinct regions can be observed on cups and cones: a smooth viscous-like region in the center and a flat one with large vein-pattern in the periphery. Energy dispersive spectroscopy measurements conducted on these features emphasized atomic distribution discrepancies both on the sample and spall. We propose a mechanism for the initiation and the growth of these features but also a process for atomic segregation during spallation. Cup and cones would originate from cracks arising from shear bands formation (softened paths). These shear bands result from a quadrupolar-shaped atomic disorder engendered around an initiation site by shock wave propagation. This disorder turns into a shear band when tensile front reaches spallation plane. During the separation process, temperature gain induced by shock waves and shear bands generation decreases material viscosity leading to higher atomic mobility. Once in a liquid-like form, atomic clusters migrate and segregate due to inertial effects originating from particle velocity variation (interaction of release waves). As a result, a high rate of copper is found in sample cups and high zirconium concentration is found on spall cones.

Preliminary Evaluation of Cavitation-Erosion Resistance of Ti-Alloys in Mercury for the Spallation Neutron Source

DOE Office of Scientific and Technical Information (OSTI.GOV)

Pawel, Steven J; Mansur, Louis K

2010-01-01

A number of Ti-based alloys in both the mill-annealed and 20% cold-worked conditions were subjected to sonication conditions in Hg using a vibratory horn to assess relative cavitation-erosion resistance. Weight loss as a function of exposure time was roughly proportional to hardness for all alloys/conditions examined, with Ti-6Al-4V (Ti-Grade 5) and Ti-6Al-2Sn-4Zr-2Mo yielding the best resistance to cavitation-erosion as evidenced by low weight losses and little or no tendency to form pits on the exposed surface. Unalloyed Ti (Ti-Grade 4) and Ti-0.12Pd (Ti-Grade 7) exhibited greater weight losses by a factor or about two and about five, respectively, with Ti-0.12Pdmore » particularly prone to pitting development. The mean erosion rates of the best two Ti-alloys examined here were about a factor of three higher than identically tested 316LN stainless steel following a low temperature carburizing treatment, but this difference is considered minor given that the rate for both materials is very low/manageable and represents a through-thickness property for the Ti-alloys. A nitriding surface treatment was also evaluated as a potential method to further increase the cavitation-erosion resistance of these alloys in Hg, but the selected treatment proved largely ineffective. Recommendations for further work to evaluate the efficacy of Ti-based alloys for use in high-powered targets for the Spallation Neutron Source are given.« less

Multipacting on the trailing edge of proton beam bunches in the PSR and SNS

NASA Astrophysics Data System (ADS)

Danilov, V.; Aleksandrov, A.; Galambos, J.; Jeon, D.; Holmes, J.; Olsen, D.

1999-12-01

The Proton Storage Ring (PSR) in Los Alamos has a fast intensity-limiting instability, which may result from an electron cloud interaction with the circulating proton beam leading to a transverse mode coupling instability. The most probable mechanism of the electron creation is multipacting. Though the effect depends on many parameters, a model is presented which predicts a large electron creation in the vacuum chamber. A comparison of this effect between the PSR in Los Alamos and the Spallation Neutron Source (SNS) in Oak Ridge is given. In addition, several possibilities to reduce multipactor are discussed.

GEANT4 benchmark with MCNPX and PHITS for activation of concrete

NASA Astrophysics Data System (ADS)

Tesse, Robin; Stichelbaut, Frédéric; Pauly, Nicolas; Dubus, Alain; Derrien, Jonathan

2018-02-01

The activation of concrete is a real problem from the point of view of waste management. Because of the complexity of the issue, Monte Carlo (MC) codes have become an essential tool to its study. But various codes or even nuclear models exist in MC. MCNPX and PHITS have already been validated for shielding studies but GEANT4 is also a suitable solution. In these codes, different models can be considered for a concrete activation study. The Bertini model is not the best model for spallation while BIC and INCL model agrees well with previous results in literature.

The magnitude of impact damage on LDEF materials

NASA Technical Reports Server (NTRS)

Allbrooks, Martha; Atkinson, Dale

1992-01-01

The purpose of this report is to document the magnitude and types of impact damage to materials and systems on the LDEF. This report will provide insights which permit NASA and industry space-systems designers to more rapidly identify potential problems and hazards in placing a spacecraft in low-Earth orbit (LEO). This report is structured to provide (1) a background on LDEF, (2) an introduction to the LEO meteoroid and debris environments, and (3) descriptions of the types of damage caused by impacts into structural materials, and contamination caused by spallation and ejecta from impact events.

Numerical modeling of the destruction of steel plates with a gradient substrate

NASA Astrophysics Data System (ADS)

Orlov, M. Yu.; Glazyrin, V. P.; Orlov, Yu. N.

2017-10-01

The paper presents the results of numerical simulation of the shock loading process of steel barriers with a gradient substrate. In an elastic plastic axisymmetric statement, a shock is simulated along the normal in the range of initial velocities up to 300 m / s. A range of initial velocities was revealed, in which the presence of a substrate "saved" the obstacle from spallation. New tasks were announced to deepen scientific knowledge about the behavior of unidirectional gradient barriers at impact. The results of calculations are obtained in the form of graphs, calculated configurations of the "impact - barrier" and tables.

Evaluation of Side Stream Filtration Technology at Oak Ridge National Laboratory

DOE Office of Scientific and Technical Information (OSTI.GOV)

Boyd, Brian K.

2014-08-01

This technology evaluation was performed by Pacific Northwest National Laboratory and Oak Ridge National Laboratory on behalf of the Federal Energy Management Program. The objective was to quantify the benefits side stream filtration provides to a cooling tower system. The evaluation assessed the performance of an existing side stream filtration system at a cooling tower system at Oak Ridge National Laboratory’s Spallation Neutron Source research facility. This location was selected because it offered the opportunity for a side-by-side comparison of a system featuring side stream filtration and an unfiltered system.

Deep inelastic neutron scattering on 207Pb and NaHF 2 as a test of a detectors array on the VESUVIO spectrometer

NASA Astrophysics Data System (ADS)

Pietropaolo, A.; Senesi, R.

2008-01-01

A prototype array of resonance detectors for deep inelastic neutron scattering experiments has been installed on the VESUVIO spectrometer, at the ISIS spallation neutron source. Deep inelastic neutron scattering measurements on a reference lead sample and on NaHF 2 molecular system are presented. Despite on an explorative level, the results obtained for the values of mean kinetic energy are found in good agreement with the theoretical predictions, thus assessing the potential capability of the device for a routine use on the instrument.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Clarke, S. D.; Wieger, B. M.; Enqvist, A.

For the first time, the complete neutron multiplicity distribution has been measured in this study from the photofission of 235U induced by high-energy spallation γ rays arriving ahead of the neutron beam at the Los Alamos Neutron Science Center. The resulting average neutron multiplicity 3.80 ± 0.08 (stat.) neutrons per photofission is in general agreement with previous measurements. In addition, unique measurements of the prompt fission energy spectrum of the neutrons from photofission and the angular correlation of two-neutron energies emitted in photofission also were made. Finally, the results are compared to calculations with the complete event fission model FREYA.

Laser and optical system for laser assisted hydrogen ion beam stripping at SNS

DOE PAGES

Liu, Y.; Rakhman, A.; Menshov, A.; ...

2016-12-01

A high-efficiency laser assisted hydrogen ion (H-) beam stripping was recently successfully carried out in the Spallation Neutron Source (SNS) accelerator. The experiment was not only an important step toward foil-less H- stripping for charge exchange injection, it also set up a first example of using megawatt ultraviolet (UV) laser source in an operational high power proton accelerator facility. This study reports in detail the design, installation, and commissioning result of a macro-pulsed multi-megawatt UV laser system and laser beam transport line for the laser stripping experiment.

Production Potential of 47Sc Using Spallation Neutron Flux at the Los Alamos Isotope Production Facility

DTIC Science & Technology

2014-03-27

Kowash, PhD (Chairman) Date //signed// 14 March 2014 LTC Stephen McHale, PhD (Member) Date //signed// 10 March 2014 Dr. Jonathan Engle, PhD (Member) Date ...signed// 14 March 2014 Dr. Justin Clinton, PhD (Member) Date AFIT-ENP-14-M-02 Abstract Scandium-47 (T1/2 = 3.41d) forms stable complexes with...0.2 µCi g−1 µAh−1 in the 47Ti and 50Ti-oxide samples, respectively. Radioisotopic purities of 47Sc in excess of 90% are achieved by activation of 47Ti

Application of activation methods on the Dubna experimental transmutation set-ups.

PubMed

Stoulos, S; Fragopoulou, M; Adloff, J C; Debeauvais, M; Brandt, R; Westmeier, W; Krivopustov, M; Sosnin, A; Papastefanou, C; Zamani, M; Manolopoulou, M

2003-02-01

High spallation neutron fluxes were produced by irradiating massive heavy targets with proton beams in the GeV range. The experiments were performed at the Dubna High Energy Laboratory using the nuclotron accelerator. Two different experimental set-ups were used to produce neutron spectra convenient for transmutation of radioactive waste by (n,x) reactions. By a theoretical analysis neutron spectra can be reproduced from activation measurements. Thermal-epithermal and fast-super-fast neutron fluxes were estimated using the 197Au, 238U (n,gamma) and (n,2n) reactions, respectively. Depleted uranium transmutation rates were also studied in both experiments.

Status of the NPDGamma experiment

NASA Astrophysics Data System (ADS)

Fry, J.; Alarcon, R.; Allen, R.; Askanazi, E.; Balascuta, S.; Barron-Palos, L.; Baeßler, S.; Barzilov, A.; Blessinger, C.; Blyth, D.; Bowman, J. D.; Calarco, J. R.; Chupp, T. E.; Coppola, C. E.; Crawford, C.; Craycraft, K.; Dabaghyan, M.; Evans, D.; Favela, J.; Fieseler, C.; Fomin, N.; Fox, W.; Freedman, S.; Frlež, E.; Fu, C.; Garcia, C.; Garishvili, I.; Gericke, M. T.; Gillis, R. C.; Grammer, K.; Greene, G. L.; Hamblen, J.; Hayes, C.; Hersman, F. W.; Ino, T.; Iverson, E. B.; Jones, G. L.; Kabir, L.; Kucucker, S.; Lauss, B.; Li, Y.; Mahurin, R.; Maldonado-Velazquez, M.; McCrea, M.; Masuda, Y.; Mei, J.; Milburn, R.; Mitchell, G. S.; Mueller, P.; Muto, S.; Musgrave, M.; Nann, H.; Novikov, I.; Page, S.; Parsons, D.; Počanić, D.; Penttilä, S. I.; Ramsay, W. D.; Salas-Bacci, A.; Santra, S.; Seo, P.-N.; Sharapov, E.; Sharma, M.; Simmons, F.; Smith, T.; Snow, W. M.; Stuart, J.; Tang, E.; Tang, Z.; Thomison, J.; Tong, T.; Vanderwerp, J.; Waldecker, S.; Wilburn, W. S.; Xu, W.; Yuan, V.; Zhang, Y.

2017-11-01

The NPDGamma experiment measures the parity-violating (PV) gamma asymmetry from polarized cold neutrons captured on protons at the Spallation Neutron Source (SNS) at Oak Ridge National Laboratory (ORNL). The (PV) neutron spin asymmetry A γ of photons from polarized cold neutron capture on protons is proportional to the Δ I=1 long range weak meson coupling h_{π }1 between nucleons in the hadronic weak interaction (HWI). Liquid para-hydrogen production data taking concluded in April 2014 and once the background aluminum asymmetry measurements are complete, the PV asymmetry A γ can be extracted. Preliminary results of the analysis of A γ are presented.

Laser and optical system for laser assisted hydrogen ion beam stripping at SNS

DOE Office of Scientific and Technical Information (OSTI.GOV)

Liu, Y.; Rakhman, A.; Menshov, A.

A high-efficiency laser assisted hydrogen ion (H-) beam stripping was recently successfully carried out in the Spallation Neutron Source (SNS) accelerator. The experiment was not only an important step toward foil-less H- stripping for charge exchange injection, it also set up a first example of using megawatt ultraviolet (UV) laser source in an operational high power proton accelerator facility. This study reports in detail the design, installation, and commissioning result of a macro-pulsed multi-megawatt UV laser system and laser beam transport line for the laser stripping experiment.

Chamber for mechanical testing in H2 with observation by neutron scattering

NASA Astrophysics Data System (ADS)

Connolly, Matthew; Bradley, Peter; Slifka, Andrew; Drexler, Elizabeth

2017-06-01

A gas-pressure chamber has been designed, constructed, and tested at a moderate pressure (3.4 MPa, 500 psi) and has the capability of mechanical loading of steel specimens for neutron scattering measurements. The chamber will allow a variety of in situ neutron scattering measurements: in particular, diffraction, quasielastic scattering, inelastic scattering, and imaging. The chamber is compatible with load frames available at the user facilities at the NIST Center for Neutron Research and Oak Ridge National Laboratory Spallation Neutron Source. A demonstration of neutron Bragg edge imaging using the chamber is presented.

Study of wave form compensation at CSNS/RCS magnets

NASA Astrophysics Data System (ADS)

Xu, S. Y.; Fu, S. N.; Wang, S.; Kang, W.; Qi, X.; Li, L.; Deng, C. D.; Zhou, J. X.

2018-07-01

A method of wave form compensation for magnets of the Rapid Cycling Synchrotron (RCS), which is based on transfer function between magnetic field and exciting current, was investigated on the magnets of RCS of Chinese Spallation Neutron Source (CSNS). By performing wave form compensation, the magnetic field ramping function for RCS magnets can be accurately controlled to the given wave form, which is not limited to sine function. The method of wave form compensation introduced in this paper can be used to reduce the magnetic field tracking errors, and can also be used to accurately control the betatron tune for RCS.

Micrometeoroid Impacts on the Hubble Space Telescope Wide Field and Planetary Camera 2: Larger Particles

NASA Technical Reports Server (NTRS)

Kearsley, A. T.; Grime, G. W.; Webb, R. P.; Jeynes, C.; Palitsin, V.; Colaux, J. L.; Ross, D. K.; Anz-Meador, P.; Liou, J. C.; Opiela, J.;

INCREASED UNDERSTANDING OF BEAM LOSSES FROM THE SNS LINAC PROTON EXPERIMENT

DOE Office of Scientific and Technical Information (OSTI.GOV)

Aleksandrov, Alexander V; Shishlo, Andrei P; Plum, Michael A

Beam loss is a major concern for high power hadron accelerators such as the Spallation Neutron Source (SNS). An unexpected beam loss in the SNS superconducting linac (SCL) was observed during the power ramp up and early operation. Intra-beam-stripping (IBS) loss, in which interactions between H- particles within the accelerated bunch strip the outermost electron, was recently identified as a possible cause of the beam loss. A set of experiments using proton beam acceleration in the SNS linac was conducted, which supports IBS as the primary beam loss mechanism in the SNS SCL.

ICANS-XIV. The fourteenth meeting of the international collaboration on advanced neutron sources.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Carpenter, J. M., ed.; Tobin, C. A., ed.

1999-02-10

The meeting began with a reception on Sunday evening. Monday's plenary sessions included status reports on the four operating spallation neutron sources, IPNS, ISIS, KENS, and the Lujan Center; on the INR source under construction at Troitsk; on the IBR-2 pulsed reactor at Dubna; and on proposals for five new installations. We also heard reports on spin-off activities: the ASTE tests (liquid mercury target tests at the AGS accelerator at Brookhaven), the ACoM activities (developments aimed to provide cold moderators suitable for high-power pulsed sources), and the International Workshop on Cold Moderators for Pulsed Neutron Sources, held in September 1997more » at Argonne. Jose Alonso and Bob Macek delivered enlightening invited talks overviewing linear accelerators and rings for spallation neutron sources. The rest of the meeting was devoted to targets and moderators and to instrumentation in a normal rotation of ICANS topics. There were altogether 84 oral reports and 23 poster presentations. On Tuesday and on Wednesday morning, we divided into separate series of sessions on Instrumentation and on Targets and Moderators. In the first, we had reports and discussions on instrumentation and techniques, on computer software, on instrument suites, and on new instruments and equipment. In the second series were sessions on liquid target systems, on solid target systems, on neutron production and target physics, on moderator physics and performance, and on target and moderator neutronics. The Tuesday evening meetings went on until 10:00, making for a 14-hour working day. That everyone willingly endured the long hours is a credit to the dedication of the attendees. On Wednesday afternoon, we boarded buses for the 1-hour trip to Argonne, where attendees toured IPNS and the Advanced Photon Source. Returning to Starved Rock, we enjoyed boat rides on the Illinois River and then a barbecue banquet dinner at the Lodge. All day Thursday and Friday morning, the attendees, in small working groups, discussed next-generation powder diffractometers, critical heat flux limitations on solid targets, monte carlo instrument simulation, prospects for high- and low-energy spectroscopy, small angle scattering and reflectometry, and the roles of solid and liquid targets in high-power pulsed spallation sources. Representatives of the laboratories participating in ICANS met Thursday evening to discuss the outcome of ICANS XIV and to decide whether, where, and when the next meeting would take place. They agreed to meet again in about 2 years in Japan. After the lunch break on Friday, the working group chairs presented the findings of their groups to the participants in a final plenary session, and the meeting adjourned with good feelings of accomplishment.« less

Final Report on MEGAPIE Target Irradiation and Post-Irradiation Examination

DOE Office of Scientific and Technical Information (OSTI.GOV)

Yong, Dai

2015-06-30

Megawatt pilot experiment (MEGAPIE) was successfully performed in 2006. One of the important goals of MEGAPIE is to understand the behaviour of structural materials of the target components exposed to high fluxes of high-energy protons and spallation neutrons in flowing LBE (liquid lead-bismuth eutectic) environment by conducting post-irradiation examination (PIE). The PIE includes four major parts: non-destructive test, radiochemical analysis of production and distribution of radionuclides produced by spallation reaction in LBE, analysis of LBE corrosion effects on structural materials, T91 and SS 316L steels, and mechanical testing of the T91 and SS 316L steels irradiated in the lower partmore » of the target. The non-destructive test (NDT) including visual inspection and ultrasonic measurement was performed in the proton beam window area of the T91 calotte of the LBE container, the most intensively irradiated part of the MEGAPIE target. The visual inspection showed no visible failure and the ultrasonic measurement demonstrated no detectable change in thickness in the beam window area. Gamma mapping was also performed in the proton beam window area of the AlMg 3 safety-container. The gamma mapping results were used to evaluate the accumulated proton fluence distribution profile, the input data for determining irradiation parameters. Radiochemical analysis of radionuclides produced by spallation reaction in LBE is to improve the understanding of the production and distribution of radionuclides in the target. The results demonstrate that the radionuclides of noble metals, 207Bi, 194Hg/Au are rather homogeneously distributed within the target, while radionuclides of electropositive elements are found to be deposited on the steel-LBE interface. The corrosion effect of LBE on the structural components under intensive irradiation was investigated by metallography. The results show that no evident corrosion damages. However, unexpected deep cracks were found in the EBW (electron beam weld) of the LBE container in the intensive irradiation zone of the target, which should be formed during irradiation. In the SS 316L steel of the flow guide tube, inclusions or precipitates enriched with O, Si, S, Ca, Ti and Mn were observed. Many of them are very long, up to a few mm, and located on grain boundaries along the extrusion direction of the tube. The degradation of the mechanical properties of the T91 and SS 316L steels has been investigated by conducting tensile tests on the specimens extracted from the T91 and SS 316L components in the intensive irradiation region. The results obtained from the proton beam window of the T91 calotte exhibit a good ductility of T91 steel after irradiation at 6-7 dpa (displacement per atom) in contact with flowing LBE.« less

Electrostatic levitation facility optimized for neutron diffraction studies of high temperature liquids at a spallation neutron source

DOE PAGES

Mauro, N. A.; Vogt, A. J.; Derendorf, K. S.; ...

2016-01-01

Neutron diffraction studies of metallic liquids provide valuable information about inherent topological and chemical ordering on multiple length scales as well as insight into dynamical processes at the level of a few atoms. But, there exist very few facilities in the world that allow such studies to be made of reactive metallic liquids in a containerless environment, and these are designed for use at reactor-based neutron sources. We present an electrostatic levitation facility, NESL (for Neutron ElectroStatic Levitator), which takes advantage of the enhanced capabilities and increased neutron flux available at spallation neutron sources (SNSs). NESL enables high quality elasticmore » and inelastic neutron scattering experiments to be made of reactive metallic and other liquids in the equilibrium and supercooled temperature regime. The apparatus is comprised of a high vacuum chamber, external and internal neutron collimation optics, and a sample exchange mechanism that allows up to 30 samples to be processed between chamber openings. Two heating lasers allow excellent sample temperature homogeneity, even for samples approaching 500 mg, and an automated temperature control system allows isothermal measurements to be conducted for times approaching 2 h in the liquid state, with variations in the average sample temperature of less than 0.5%. Furthermore, to demonstrate the capabilities of the facility for elastic scattering studies of liquids, a high quality total structure factor for Zr 64Ni 36 measured slightly above the liquidus temperature is presented from experiments conducted on the nanoscale-ordered materials diffractometer (NOMAD) beam line at the SNS after only 30 min of acquisition time for a small sample ( 100 mg).« less

Overview of the Neutron Radiography and Computed Tomography at the Oak Ridge National Laboratory and Applications

DOE Office of Scientific and Technical Information (OSTI.GOV)

Bilheux, Hassina Z; Bilheux, Jean-Christophe; Tremsin, Anton S

2015-01-01

The Oak Ridge National Laboratory (ORNL) Neutron Sciences Directorate (NScD) has installed a neutron imaging (NI) beam line at the High Flux Isotope Reactor (HFIR) cold guide hall. The CG-1D beam line produces cold neutrons for a broad range of user research spanning from engineering to material research, additive manufacturing, vehicle technologies, archaeology, biology, and plant physiology. Recent efforts have focused on increasing flux and spatial resolution. A series of selected engineering applications is presented here. Historically and for more than four decades, neutron imaging (NI) facilities have been installed exclusively at continuous (i.e. reactor-based) neutron sources rather than atmore » pulsed sources. This is mainly due to (1) the limited number of accelerator-based facilities and therefore the fierce competition for beam lines with neutron scattering instruments, (2) the limited flux available at accelerator-based neutron sources and finally, (3) the lack of high efficiency imaging detector technology capable of time-stamping pulsed neutrons with sufficient time resolution. Recently completed high flux pulsed proton-driven neutron sources such as the ORNL Spallation Neutron Source (SNS) at ORNL and the Japanese Spallation Neutron Source (JSNS) of the Japan Proton Accelerator Research Complex (J-PARC) in Japan produce high neutron fluxes that offer new and unique opportunities for NI techniques. Pulsed-based neutron imaging facilities RADEN and IMAT are currently being built at J-PARC and the Rutherford National Laboratory in the U.K., respectively. ORNL is building a pulsed neutron imaging beam line called VENUS to respond to the U.S. based scientific community. A team composed of engineers, scientists and designers has developed a conceptual design of the future VENUS imaging instrument at the SNS.« less

Conceptual moderator studies for the Spallation Neutron Source short-pulse second target station

DOE PAGES

Gallmeier, F. X.; Lu, W.; Riemer, B. W.; ...

2016-06-14

We identified candidate moderator configurations for a short-pulse second target station (STS) at the Oak Ridge National Laboratory Spallation Neutron Source (SNS) using a global optimizer framework built around the MCNPX particle transport code. Neutron brightness metrics were selected as the figure-of-merit. We assumed that STS would use one out of six proton pulses produced by an SNS accelerator upgraded to operate at 1.3 GeV proton energy, 2.8 MW power and 60 Hz repetition rate. The simulations indicate that the peak brightness can be increased by a factor of 5 and 2.5 on a per proton pulse basis compared tomore » the SNS first target station for both coupled and decoupled para-hydrogen moderators, respectively. Additional increases by factors of 3 and 2 were demonstrated for coupled and decoupled moderators, respectively, by reducing the area of neutron emission from 100 × 100 mm 2 to 20 × 20 mm 2. Furthermore, this increase in brightness has the potential to translate to an increase of beam intensity at the instruments’ sample positions even though the total neutron emission of the smaller moderator is less than that of the larger. This is especially true for instruments with small samples (beam dimensions). The increased fluxes in the STS moderators come at accelerated poison and de-coupler burnout and higher radiation-induced material damage rates per unit power, which overall translate into lower moderator lifetimes. Our first effort decoupled group moderators into a cluster collectively positioning them at the peak neutron production zone in the target and having a three-port neutron emission scheme that complements that of a cylindrical coupled moderator.« less

Conceptual moderator studies for the Spallation Neutron Source short-pulse second target station

NASA Astrophysics Data System (ADS)

Gallmeier, F. X.; Lu, W.; Riemer, B. W.; Zhao, J. K.; Herwig, K. W.; Robertson, J. L.

2016-06-01

Candidate moderator configurations for a short-pulse second target station (STS) at the Oak Ridge National Laboratory Spallation Neutron Source (SNS) have been identified using a global optimizer framework built around the MCNPX particle transport code. Neutron brightness metrics were selected as the figure-of-merit. We assumed that STS would use one out of six proton pulses produced by an SNS accelerator upgraded to operate at 1.3 GeV proton energy, 2.8 MW power and 60 Hz repetition rate. The simulations indicate that the peak brightness can be increased by a factor of 5 and 2.5 on a per proton pulse basis compared to the SNS first target station for both coupled and decoupled para-hydrogen moderators, respectively. Additional increases by factors of 3 and 2 were demonstrated for coupled and decoupled moderators, respectively, by reducing the area of neutron emission from 100 × 100 mm2 to 20 × 20 mm2. This increase in brightness has the potential to translate to an increase of beam intensity at the instruments' sample positions even though the total neutron emission of the smaller moderator is less than that of the larger. This is especially true for instruments with small samples (beam dimensions). The increased fluxes in the STS moderators come at accelerated poison and de-coupler burnout and higher radiation-induced material damage rates per unit power, which overall translate into lower moderator lifetimes. A first effort was undertaken to group decoupled moderators into a cluster collectively positioning them at the peak neutron production zone in the target and having a three-port neutron emission scheme that complements that of a cylindrical coupled moderator.

Conceptual moderator studies for the Spallation Neutron Source short-pulse second target station

DOE Office of Scientific and Technical Information (OSTI.GOV)

Gallmeier, F. X.; Lu, W.; Riemer, B. W.

We identified candidate moderator configurations for a short-pulse second target station (STS) at the Oak Ridge National Laboratory Spallation Neutron Source (SNS) using a global optimizer framework built around the MCNPX particle transport code. Neutron brightness metrics were selected as the figure-of-merit. We assumed that STS would use one out of six proton pulses produced by an SNS accelerator upgraded to operate at 1.3 GeV proton energy, 2.8 MW power and 60 Hz repetition rate. The simulations indicate that the peak brightness can be increased by a factor of 5 and 2.5 on a per proton pulse basis compared tomore » the SNS first target station for both coupled and decoupled para-hydrogen moderators, respectively. Additional increases by factors of 3 and 2 were demonstrated for coupled and decoupled moderators, respectively, by reducing the area of neutron emission from 100 × 100 mm 2 to 20 × 20 mm 2. Furthermore, this increase in brightness has the potential to translate to an increase of beam intensity at the instruments’ sample positions even though the total neutron emission of the smaller moderator is less than that of the larger. This is especially true for instruments with small samples (beam dimensions). The increased fluxes in the STS moderators come at accelerated poison and de-coupler burnout and higher radiation-induced material damage rates per unit power, which overall translate into lower moderator lifetimes. Our first effort decoupled group moderators into a cluster collectively positioning them at the peak neutron production zone in the target and having a three-port neutron emission scheme that complements that of a cylindrical coupled moderator.« less

Conceptual moderator studies for the Spallation Neutron Source short-pulse second target station

DOE Office of Scientific and Technical Information (OSTI.GOV)

Gallmeier, F. X., E-mail: gallmeierfz@ornl.gov; Lu, W.; Riemer, B. W.

Candidate moderator configurations for a short-pulse second target station (STS) at the Oak Ridge National Laboratory Spallation Neutron Source (SNS) have been identified using a global optimizer framework built around the MCNPX particle transport code. Neutron brightness metrics were selected as the figure-of-merit. We assumed that STS would use one out of six proton pulses produced by an SNS accelerator upgraded to operate at 1.3 GeV proton energy, 2.8 MW power and 60 Hz repetition rate. The simulations indicate that the peak brightness can be increased by a factor of 5 and 2.5 on a per proton pulse basis comparedmore » to the SNS first target station for both coupled and decoupled para-hydrogen moderators, respectively. Additional increases by factors of 3 and 2 were demonstrated for coupled and decoupled moderators, respectively, by reducing the area of neutron emission from 100 × 100 mm{sup 2} to 20 × 20 mm{sup 2}. This increase in brightness has the potential to translate to an increase of beam intensity at the instruments’ sample positions even though the total neutron emission of the smaller moderator is less than that of the larger. This is especially true for instruments with small samples (beam dimensions). The increased fluxes in the STS moderators come at accelerated poison and de-coupler burnout and higher radiation-induced material damage rates per unit power, which overall translate into lower moderator lifetimes. A first effort was undertaken to group decoupled moderators into a cluster collectively positioning them at the peak neutron production zone in the target and having a three-port neutron emission scheme that complements that of a cylindrical coupled moderator.« less

H- radio frequency source development at the Spallation Neutron Source.

PubMed

Welton, R F; Dudnikov, V G; Gawne, K R; Han, B X; Murray, S N; Pennisi, T R; Roseberry, R T; Santana, M; Stockli, M P; Turvey, M W

2012-02-01

The Spallation Neutron Source (SNS) now routinely operates nearly 1 MW of beam power on target with a highly persistent ∼38 mA peak current in the linac and an availability of ∼90%. H(-) beam pulses (∼1 ms, 60 Hz) are produced by a Cs-enhanced, multicusp ion source closely coupled with an electrostatic low energy beam transport (LEBT), which focuses the 65 kV beam into a radio frequency quadrupole accelerator. The source plasma is generated by RF excitation (2 MHz, ∼60 kW) of a copper antenna that has been encased with a thickness of ∼0.7 mm of porcelain enamel and immersed into the plasma chamber. The ion source and LEBT normally have a combined availability of ∼99%. Recent increases in duty-factor and RF power have made antenna failures a leading cause of downtime. This report first identifies the physical mechanism of antenna failure from a statistical inspection of ∼75 antennas which ran at the SNS, scanning electron microscopy studies of antenna surface, and cross sectional cuts and analysis of calorimetric heating measurements. Failure mitigation efforts are then described which include modifying the antenna geometry and our acceptance∕installation criteria. Progress and status of the development of the SNS external antenna source, a long-term solution to the internal antenna problem, are then discussed. Currently, this source is capable of delivering comparable beam currents to the baseline source to the SNS and, an earlier version, has briefly demonstrated unanalyzed currents up to ∼100 mA (1 ms, 60 Hz) on the test stand. In particular, this paper discusses plasma ignition (dc and RF plasma guns), antenna reliability, magnet overheating, and insufficient beam persistence.

Effects of environment and frequency on the fatigue behavior of the spallation neutron source (SNS) target container material - 316 LN stainless steel

NASA Astrophysics Data System (ADS)

Tian, Hongbo

As the candidate target container material of the new Spallation Neutron Source (SNS) being designed and constructed at the Oak Ridge National Laboratory (ORNL), Type 316 low-carbon nitrogen-added (LN) stainless steel (SS) will operate in an aggressive environment, subjected to intense fluxes of high-energy protons and neutrons while exposed to liquid mercury. The current project is oriented toward materials studies regarding the effects of test environment and frequency on the fatigue behavior of 316 LN SS. In order to study the structural applications of this material and improve the fundamental understanding of the fatigue damage mechanisms, fatigue tests were performed in air and mercury environments at various frequencies and R ratios (R = sigma min/sigmamax, sigmamin and sigmamax are the applied minimum and maximum stresses, respectively). Fatigue data were developed for the structural design and engineering applications of this material. Specifically, high-cycle fatigue tests, fatigue crack-propagation tests, and ultrahigh cycle fatigue tests up to 10 9 cycles were conducted in air and mercury with test frequencies from 10 Hz to 700 Hz. Microstructure characterizations were performed using optical microscopy (OM), scanning-electron microscopy (SEM), and transmission-electron microscopy (TEM). It was found that mercury doesn't seem to have a large impact on the crack-initiation behavior of 316 LN SS. However, the crack-propagation mechanisms in air and mercury are different in some test conditions. Transgranular cracks seem to be the main mechanism in air, and intergranular in mercury. A significant specimen self-heating effect was found during high-cycle faituge. Theoretical calculation was performed to predict temperature responses of the material subjected to cyclic deformation. The predicted cyclic temperature evolution seems to be in good agreement with the experimental results.

Acoustic emission and fatigue damage induced in plasma-sprayed hydroxyapatite coating layers.

PubMed

Laonapakul, Teerawat; Otsuka, Yuichi; Nimkerdphol, Achariya Rakngarm; Mutoh, Yoshiharu

2012-04-01

In order to improve the adhesive strength of hydroxyapatite (HAp) coatings, grit blasting with Al(2)O(3) powder and then wet blasting with HAp/Ti mixed powders was carried out on a commercially pure Ti (cp-Ti) substrate. Subsequently, an HAp/Ti bond coat layer and HAp top coat layer were deposited by plasma spraying. Fatigue tests of the HAp-coated specimens were carried out under four-point bending. Acoustic emission (AE) signals during the entire fatigue test were monitored to investigate the fatigue cracking behavior of the HAp-coated specimens. The HAp-coated specimens could survive up to 10(7) cycles without spallation of the HAp coating layers at the stress amplitude of 120 MPa. The HAp-coated specimens without HAp/Ti bond coat layer showed shorter fatigue life and easy crack nucleation compared to the HAp-coated specimens with HAp/Ti bond coat layer. The delamination and spallation of the HAp top coat with HAp/Ti bond coat on cp-Ti was not observed until the crack propagated into the cp-Ti during the final fracture stage of the fatigue cycle. Therefore, the HAp/Ti bond coat layer was found to greatly improve the fatigue damage resistance of the HAp coating layer. Three stages of the fatigue failure behavior of the HAp top coat with HAp/Ti bond coat on a cp-Ti substrate can be clearly estimated by the AE monitoring technique. These stages are cracks nucleating and propagating in the coating layer, cracks propagating in the substrate, and cracks propagating unstably to final fracture. Copyright © 2011 Elsevier Ltd. All rights reserved.

A Venus/Saturn Mission Study: 45deg Sphere-Cone Rigid Aeroshells and Ballistic Entries

NASA Technical Reports Server (NTRS)

Prabhu, Dinesh K.; Allen, Gary A.; Cappuccio, Gelsomina

2012-01-01

The present study considers ballistic entries into the atmospheres of Saturn and Venus using a 45deg sphere-cone rigid aeroshell (a legacy shape that has been successfully used in the Pioneer Venus and Galileo missions). For a number of entry mass and diameter combinations (i.e., various entries ballistic coefficients), entry velocities, and heading angles, the trajectory space in terms of entry flight path angles between skip out and -30deg is explored with a 3DOF trajectory code, TRAJ. Assuming that the thermal protection material of choice is carbon phenolic of flight heritage, the entry flight path angle space is constrained a posteriori by the mechanical and thermal performance parameters of the material. For mechanical performance, a 200 g limit is place on the peak deceleration load and 10 bar is assumed as the spallation pressure threshold for the legacy material. It is shown that both constraints cannot be active simultaneously. For thermal performance, a minimum margined heat flux threshold of 2.5 kW/sq cm is assumed for the heritage material. Using these constraints, viable entry flight path angle corridors are determined. Analysis of the results also hints at the existence of a "critical" ballistic coefficient beyond which the steepest possible entries are determined by the spallation pressure threshold. The results are verified against known performance of the various probes used in the Galileo and Pioneer Venus missions. It is hoped that the results presented here will serve as a baseline in the development of a new class of ablative materials for Venus and Saturn missions being considered in a future New Frontiers class of NASA missions.

Laser lift-off scribing of the CZTSe thin-film solar cells at different pulse durations

DOE PAGES

Markauskas, Edgaras; Gečys, Paulius; Repins, Ingrid; ...

2017-04-27

Here, the transition to fully sized solar modules requires additional three-step laser structuring processes to preserve small-scale cell efficiencies over the large areas. The adjacent cell isolation (the P3 scribe) was found to be the most sensitive process in the case of laser induced damage. The laser induced layer lift-off mechanism seems to be a very attractive process for the P3 patterning, since almost all the laser affected material is removed by mechanical spallation. However, a laser induced layer spallation behavior together with scribe electrical validation under the different laser pulse durations was not investigated extensively in the past. Therefore,more » we report our novel results on the P2 and P3 laser lift-off processing of the Cu 2ZnSn(S, Se 4) (CZTSe) thin-film solar cells covering the pulse duration range from 300 fs to 60 ps. Shorter sub-ps pulses enabled us to process smaller P2 and P3 craters, although the lift-off threshold fluences were higher compared to the longer ps pulses. In the case of the layer lift-off, the laser radiation had to penetrate through the layer stack down to the CZTSe/Mo interface. At shorter sub-ps pulses, the nonlinear effects triggered absorption of the laser radiation in the bulk of the material, resulting in increased damage of the CZTSe layer. The Raman measurements confirmed the CZTSe surface stoichiometry changes for shorter pulses. Furthermore, shorter pulses induced higher electrical conductivity of a scribe, resulting in lower photo-electrical efficiency during the mini-module simulation. In the case of the P3 lift-off scribing, the 10 ps pulses were more favorable than shorter femtosecond pulses.« less

Electrostatic levitation facility optimized for neutron diffraction studies of high temperature liquids at a spallation neutron source

DOE Office of Scientific and Technical Information (OSTI.GOV)

Mauro, N. A., E-mail: namauro@noctrl.edu; Vogt, A. J.; Derendorf, K. S.

2016-01-15

Neutron diffraction studies of metallic liquids provide valuable information about inherent topological and chemical ordering on multiple length scales as well as insight into dynamical processes at the level of a few atoms. However, there exist very few facilities in the world that allow such studies to be made of reactive metallic liquids in a containerless environment, and these are designed for use at reactor-based neutron sources. We present an electrostatic levitation facility, NESL (for Neutron ElectroStatic Levitator), which takes advantage of the enhanced capabilities and increased neutron flux available at spallation neutron sources (SNSs). NESL enables high quality elasticmore » and inelastic neutron scattering experiments to be made of reactive metallic and other liquids in the equilibrium and supercooled temperature regime. The apparatus is comprised of a high vacuum chamber, external and internal neutron collimation optics, and a sample exchange mechanism that allows up to 30 samples to be processed between chamber openings. Two heating lasers allow excellent sample temperature homogeneity, even for samples approaching 500 mg, and an automated temperature control system allows isothermal measurements to be conducted for times approaching 2 h in the liquid state, with variations in the average sample temperature of less than 0.5%. To demonstrate the capabilities of the facility for elastic scattering studies of liquids, a high quality total structure factor for Zr{sub 64}Ni{sub 36} measured slightly above the liquidus temperature is presented from experiments conducted on the nanoscale-ordered materials diffractometer (NOMAD) beam line at the SNS after only 30 min of acquisition time for a small sample (∼100 mg)« less

IPNS upgrade: A feasibility study

DOE Office of Scientific and Technical Information (OSTI.GOV)

NONE

1995-04-01

Many of Argonne National Laboratory`s (ANL`s) scientific staff members were very active in R&D work related to accelerator-based spoliation sources in the 1970s and early 1980s. In 1984, the Seitz/Eastman Panel of the National Academy of Sciences reviewed U.S. materials science research facilities. One of the recommendations of this panel was that the United States build a reactor-based steady-state source, the Advanced Neutron Source (ANS), at Oak Ridge National Laboratory. Subsequently, R&D activities related to the design of an accelerator-based source assumed a lower priority. The resumption of pulsed-source studies in this country started simultaneously with design activities in Europemore » aimed at the European Spallation Source (ESS). The European Community funded a workshop in September 1991 to define the parameters of the ESS. Participants in this workshop included both accelerator builders and neutron source users. A consortium of European countries has proposed to build a 5-MW pulsed source, and a feasibility study is currently under way. Soon after the birth of the ESS, a small group at ANL set about bringing themselves up to date on pulsed-source information since 1984 and studied the feasibility of upgrading ANL`s Intense Pulsed Neutron Source (IPNS) to 1 MW by means of a rapidly cycling synchrotron that could be housed, along with its support facilities, in existing buildings. In early 1993, the Kohn panel recommended that (1) design and construction of the ANS should be completed according to the proposed project schedule and (2) development of competitive proposals for cost-effective design and construction of a 1-MW pulsed spallation source should be authorized immediately.« less

Formation of high heat resistant coatings by using gas tunnel type plasma spraying.

PubMed

Kobayashi, A; Ando, Y; Kurokawa, K

2012-06-01

Zirconia sprayed coatings are widely used as thermal barrier coatings (TBC) for high temperature protection of metallic structures. However, their use in diesel engine combustion chamber components has the long run durability problems, such as the spallation at the interface between the coating and substrate due to the interface oxidation. Although zirconia coatings have been used in many applications, the interface spallation problem is still waiting to be solved under the critical conditions such as high temperature and high corrosion environment. The gas tunnel type plasma spraying developed by the author can make high quality ceramic coatings such as Al2O3 and ZrO2 coating compared to other plasma spraying method. A high hardness ceramic coating such as Al2O3 coating by the gas tunnel type plasma spraying, were investigated in the previous study. The Vickers hardness of the zirconia (ZrO2) coating increased with decreasing spraying distance, and a higher Vickers hardness of about Hv = 1200 could be obtained at a shorter spraying distance of L = 30 mm. ZrO2 coating formed has a high hardness layer at the surface side, which shows the graded functionality of hardness. In this study, ZrO2 composite coatings (TBCs) with Al2O3 were deposited on SS304 substrates by gas tunnel type plasma spraying. The performance such as the mechanical properties, thermal behavior and high temperature oxidation resistance of the functionally graded TBCs was investigated and discussed. The resultant coating samples with different spraying powders and thickness are compared in their corrosion resistance with coating thickness as variables. Corrosion potential was measured and analyzed corresponding to the microstructure of the coatings. High Heat Resistant Coatings, Gas Tunnel Type Plasma Spraying, Hardness,

Laser lift-off scribing of the CZTSe thin-film solar cells at different pulse durations

DOE Office of Scientific and Technical Information (OSTI.GOV)

Markauskas, Edgaras; Gečys, Paulius; Repins, Ingrid

Here, the transition to fully sized solar modules requires additional three-step laser structuring processes to preserve small-scale cell efficiencies over the large areas. The adjacent cell isolation (the P3 scribe) was found to be the most sensitive process in the case of laser induced damage. The laser induced layer lift-off mechanism seems to be a very attractive process for the P3 patterning, since almost all the laser affected material is removed by mechanical spallation. However, a laser induced layer spallation behavior together with scribe electrical validation under the different laser pulse durations was not investigated extensively in the past. Therefore,more » we report our novel results on the P2 and P3 laser lift-off processing of the Cu 2ZnSn(S, Se 4) (CZTSe) thin-film solar cells covering the pulse duration range from 300 fs to 60 ps. Shorter sub-ps pulses enabled us to process smaller P2 and P3 craters, although the lift-off threshold fluences were higher compared to the longer ps pulses. In the case of the layer lift-off, the laser radiation had to penetrate through the layer stack down to the CZTSe/Mo interface. At shorter sub-ps pulses, the nonlinear effects triggered absorption of the laser radiation in the bulk of the material, resulting in increased damage of the CZTSe layer. The Raman measurements confirmed the CZTSe surface stoichiometry changes for shorter pulses. Furthermore, shorter pulses induced higher electrical conductivity of a scribe, resulting in lower photo-electrical efficiency during the mini-module simulation. In the case of the P3 lift-off scribing, the 10 ps pulses were more favorable than shorter femtosecond pulses.« less

Analysis of structure and deformation behavior of AISI 316L tensile specimens from the second operational target module at the Spallation Neutron Source

DOE PAGES

Gussev, Maxim N.; McClintock, David A.; Garner, Frank

2015-08-05

In an earlier publication, tensile testing was performed on specimens removed from the first two operational targets of the Spallation Neutron Source (SNS). There were several anomalous features in the results. First, some specimens had very large elongations (up to 57%) while others had significantly smaller values. Second, there was a larger than the usual amount of data scatter in the elongation results. Third, the stress-strain diagrams of nominally similar specimens spanned a wide range of behavior ranging from expected irradiation-induced hardening to varying levels of force drop after yield point and indirect signs of "traveling deformation wave" behavior associatedmore » with strain-induced martensite formation. To investigate the cause(s) of such variable tensile behavior, several specimens from Target 2, spanning the range of observed tensile behavior, were chosen for detailed microstructural examination using electron backscattering analysis (EBSD). It was also shown that the steel employed in the construction of the target contained an unexpected bimodal grain size distribution, containing very large out-of-specification grains surrounded by necklaces of grains of within-specification sizes. The large grains were frequently comparable to the width of the gauge section of the tensile specimen. Moreover, the propensity to form martensite during deformation was shown to be accelerated by radiation but also to be very sensitive to the relative orientation of the grains with respect to the tensile axis. Specimens having large grains in the gauge that were most favorably oriented for production of martensite strongly exhibited the traveling deformation wave phenomenon, while those specimens with less favorably oriented grains had lesser or no degree of the wave effect, thereby accounting for the larger than expected data scatter.« less

Long-term oxidation of candidate cast iron and stainless steel exhaust system alloys from 650 to 800 °C in air with water vapor

DOE PAGES

Brady, Michael P.; Muralidharan, Govindarajan; Leonard, Donovan .; ...

2014-08-29

Here, the oxidation behavior of SiMo cast iron, Ni-resist D 5S cast iron, cast chromia-forming austenitic stainless steels of varying Cr/Ni content based on CF8C plus, HK, and HP, and a developmental cast alumina-forming austenitic (AFA) stainless steel of interest for diesel exhaust system components were studied for up to 5000 h at 650-800 °C in air with 10% H 2O. At 650 °C, the Ni-resist D5S exhibited moderately better oxidation resistance than did the SiMo cast iron. However, the D5S suffered from oxide scale spallation issues at 700 °C and higher, whereas the oxide scales formed on SiMo castmore » iron remained adherent from 700-800 °C despite oxide scales hundreds of microns thick. The oxidation of the SiMo cast iron exhibited unusual temperature dependence, with periods of slower oxidation kinetics at 750-800 °C compared to 650-700 °C due to continuous silica-rich scale formation at the higher temperatures. The oxidation of the cast chromia-forming austenitics trended with the level of Cr and Ni additions, with small mass losses consistent with Cr oxy-hydroxide volatilization processes for the higher 25Cr/25-35Ni HK and HP type alloys, and transition to rapid Fe-base oxide formation and scale spallation in the lower 19Cr/12Ni CF8C plus type alloy. In contrast, small positive mass changes consistent with protective alumina scale formation were observed for the cast AFA alloy under all conditions studied. Implications of these findings for diesel exhaust system components are discussed.« less

SINGLE EVENT EFFECTS TEST FACILITY AT OAK RIDGE NATIONAL LABORATORY

DOE Office of Scientific and Technical Information (OSTI.GOV)

Riemer, Bernie; Gallmeier, Franz X; Dominik, Laura J

2015-01-01

Increasing use of microelectronics of ever diminishing feature size in avionics systems has led to a growing Single Event Effects (SEE) susceptibility arising from the highly ionizing interactions of cosmic rays and solar particles. Single event effects caused by atmospheric radiation have been recognized in recent years as a design issue for avionics equipment and systems. To ensure a system meets all its safety and reliability requirements, SEE induced upsets and potential system failures need to be considered, including testing of the components and systems in a neutron beam. Testing of ICs and systems for use in radiation environments requiresmore » the utilization of highly advanced laboratory facilities that can run evaluations on microcircuits for the effects of radiation. This paper provides a background of the atmospheric radiation phenomenon and the resulting single event effects, including single event upset (SEU) and latch up conditions. A study investigating requirements for future single event effect irradiation test facilities and developing options at the Spallation Neutron Source (SNS) is summarized. The relatively new SNS with its 1.0 GeV proton beam, typical operation of 5000 h per year, expertise in spallation neutron sources, user program infrastructure, and decades of useful life ahead is well suited for hosting a world-class SEE test facility in North America. Emphasis was put on testing of large avionics systems while still providing tunable high flux irradiation conditions for component tests. Makers of ground-based systems would also be served well by these facilities. Three options are described; the most capable, flexible, and highest-test-capacity option is a new stand-alone target station using about one kW of proton beam power on a gas-cooled tungsten target, with dual test enclosures. Less expensive options are also described.« less

Single Event Effects Test Facility Options at the Oak Ridge National Laboratory

DOE Office of Scientific and Technical Information (OSTI.GOV)

Riemer, Bernie; Gallmeier, Franz X; Dominik, Laura J

2015-01-01

Increasing use of microelectronics of ever diminishing feature size in avionics systems has led to a growing Single Event Effects (SEE) susceptibility arising from the highly ionizing interactions of cosmic rays and solar particles. Single event effects caused by atmospheric radiation have been recognized in recent years as a design issue for avionics equipment and systems. To ensure a system meets all its safety and reliability requirements, SEE induced upsets and potential system failures need to be considered, including testing of the components and systems in a neutron beam. Testing of integrated circuits (ICs) and systems for use in radiationmore » environments requires the utilization of highly advanced laboratory facilities that can run evaluations on microcircuits for the effects of radiation. This paper provides a background of the atmospheric radiation phenomenon and the resulting single event effects, including single event upset (SEU) and latch up conditions. A study investigating requirements for future single event effect irradiation test facilities and developing options at the Spallation Neutron Source (SNS) is summarized. The relatively new SNS with its 1.0 GeV proton beam, typical operation of 5000 h per year, expertise in spallation neutron sources, user program infrastructure, and decades of useful life ahead is well suited for hosting a world-class SEE test facility in North America. Emphasis was put on testing of large avionics systems while still providing tunable high flux irradiation conditions for component tests. Makers of ground-based systems would also be served well by these facilities. Three options are described; the most capable, flexible, and highest-test-capacity option is a new stand-alone target station using about one kW of proton beam power on a gas-cooled tungsten target, with dual test enclosures. Less expensive options are also described.« less

Study on the Fire Damage Characteristics of the New Qidaoliang Highway Tunnel: Field Investigation with Computational Fluid Dynamics (CFD) Back Analysis

PubMed Central

Lai, Hongpeng; Wang, Shuyong; Xie, Yongli

2016-01-01

In the New Qidaoliang Tunnel (China), a rear-end collision of two tanker trunks caused a fire. To understand the damage characteristics of the tunnel lining structure, in situ investigation was performed. The results show that the fire in the tunnel induced spallation of tunnel lining concrete covering 856 m3; the length of road surface damage reached 650 m; the sectional area had a maximum 4% increase, and the mechanical and electrical facilities were severely damaged. The maximum area loss happened at the fire spot with maximum observed concrete spallation up to a thickness of 35.4 cm. The strength of vault and side wall concrete near the fire source was significantly reduced. The loss of concrete strength of the side wall near the inner surface of tunnel was larger than that near the surrounding rock. In order to perform back analysis of the effect of thermal load on lining structure, simplified numerical simulation using computational fluid dynamics (CFD) was also performed, repeating the fire scenario. The simulated results showed that from the fire breaking out to the point of becoming steady, the tunnel experienced processes of small-scale warming, swirl around fire, backflow, and longitudinal turbulent flow. The influence range of the tunnel internal temperature on the longitudinal downstream was far greater than on the upstream, while the high temperature upstream and downstream of the transverse fire source mainly centered on the vault or the higher vault waist. The temperature of each part of the tunnel near the fire source had no obvious stratification phenomenon. The temperature of the vault lining upstream and downstream near the fire source was the highest. The numerical simulation is found to be in good agreement with the field observations. PMID:27754455

Study on the Fire Damage Characteristics of the New Qidaoliang Highway Tunnel: Field Investigation with Computational Fluid Dynamics (CFD) Back Analysis.

PubMed

Lai, Hongpeng; Wang, Shuyong; Xie, Yongli

2016-10-15

In the New Qidaoliang Tunnel (China), a rear-end collision of two tanker trunks caused a fire. To understand the damage characteristics of the tunnel lining structure, in situ investigation was performed. The results show that the fire in the tunnel induced spallation of tunnel lining concrete covering 856 m³; the length of road surface damage reached 650 m; the sectional area had a maximum 4% increase, and the mechanical and electrical facilities were severely damaged. The maximum area loss happened at the fire spot with maximum observed concrete spallation up to a thickness of 35.4 cm. The strength of vault and side wall concrete near the fire source was significantly reduced. The loss of concrete strength of the side wall near the inner surface of tunnel was larger than that near the surrounding rock. In order to perform back analysis of the effect of thermal load on lining structure, simplified numerical simulation using computational fluid dynamics (CFD) was also performed, repeating the fire scenario. The simulated results showed that from the fire breaking out to the point of becoming steady, the tunnel experienced processes of small-scale warming, swirl around fire, backflow, and longitudinal turbulent flow. The influence range of the tunnel internal temperature on the longitudinal downstream was far greater than on the upstream, while the high temperature upstream and downstream of the transverse fire source mainly centered on the vault or the higher vault waist. The temperature of each part of the tunnel near the fire source had no obvious stratification phenomenon. The temperature of the vault lining upstream and downstream near the fire source was the highest. The numerical simulation is found to be in good agreement with the field observations.

Helium Bubble Injection Solution To The Cavitation Damage At The Spallation Neutron Source

DOE Office of Scientific and Technical Information (OSTI.GOV)

Francis, M. W.; Ruggles, A. E.

2009-03-10

The Spallation Neutron Source (SNS) is one of the largest science projects in the United States, with total cost near 1.4 Billion Dollars. The limiting factor of the facility had always been assumed to be the lifetime of the target window due to radiation damage. After further investigation, the lifetime of the target was determined not to be limited by radiation damage but by cavitation damage. The cavitation damage derives from pressure waves caused by the beam energy deposition. Vapor bubbles form when low to negative pressures occur in the mercury near the stainless steel target window due to wavemore » interaction with the structure. Collapse of these bubbles can focus wave energy in small liquid jets that erode the window surface. Compressibility of the mercury can be enhanced to reduce the amplitude of the pressure wave caused by the beam energy deposition. To enhance compressibility, small (10 to 30 micron diameter) gas bubbles could be injected into the bulk of the mercury. Solubility and diffusivity parameters of inert gas in mercury are required for a complete mechanical simulation and engineering of these strategies. Using current theoretical models, one obtains a theoretical Henry coefficient of helium in mercury on the order of 3.9E15 Pa-molHg/molHe at 300 K. This low solubility was confirmed by a direct, offline experimental method. Mercury was charged with helium and any pressure change was recorded. Any pressure change was attributed to gas going into solution. Therefore, with the sensitivity of the experiment, a lower limit of 9E12 Pa-molHg/molHe was placed on the mercury-helium system. These values guarantee a stable bubble lifetime needed within the SNS mercury target to mitigate cavitation issues.« less

SIMULATION AND MOCKUP OF SNS JET-FLOW TARGET WITH WALL JET FOR CAVITATION DAMAGE MITIGATION

DOE Office of Scientific and Technical Information (OSTI.GOV)

Wendel, Mark W; Geoghegan, Patrick J; Felde, David K

2014-01-01

Pressure waves created in liquid mercury pulsed spallation targets at the Spallation Neutron Source (SNS) at Oak Ridge National Laboratory induce cavitation damage on the stainless steel target container. The cavitation damage is thought to limit the lifetime of the target for power levels at and above 1 MW. Severe through-wall cavitation damage on an internal wall near the beam entrance window has been observed in spent-targets. Surprisingly though, there is very little damage on the walls that bound an annular mercury channel that wraps around the front and outside of the target. The mercury flow through this channel ismore » characterized by smooth, attached streamlines. One theory to explain this lack of damage is that the uni-directional flow biases the direction of the collapsing cavitation bubble, reducing the impact pressure and subsequent damage. The theory has been reinforced by in-beam separate effects data. For this reason, a second-generation SNS mercury target has been designed with an internal wall jet configuration intended to protect the concave wall where damage has been observed. The wall jet mimics the annular flow channel streamlines, but since the jet is bounded on only one side, the momentum is gradually diffused by the bulk flow interactions as it progresses around the cicular path of the target nose. Numerical simulations of the flow through this jet-flow target have been completed, and a water loop has been assembled with a transparent test target in order to visualize and measure the flow field. This paper presents the wall jet simulation results, as well as early experimental data from the test loop.« less

Correlation between simulations and cavitation-induced erosion damage in Spallation Neutron Source target modules after operation

DOE Office of Scientific and Technical Information (OSTI.GOV)

Riemer, Bernie; McClintock, David A; Kaminskas, Saulius

2014-01-01

An explicit finite element (FE) technique developed for estimating dynamic strain in the Spallation Neutron Source (SNS) mercury target module vessel is now providing insight into cavitation damage patterns observed in used targets. The technique uses an empirically developed material model for the mercury that describes liquid-like volumetric stiffness combined with a tensile pressure cut-off limit that approximates cavitation. The longest period each point in the mercury is at the tensile cut-off threshold is denoted its saturation time. Now, the pattern of saturation time can be obtained from these simulations and is being positively correlated with observed damage patterns andmore » is interpreted as a qualitative measure of damage potential. Saturation time has been advocated by collaborators at J-Parc as a factor in predicting bubble nuclei growth and collapse intensity. The larger the ratio of maximum bubble size to nucleus, the greater the bubble collapse intensity to be expected; longer saturation times result in greater ratios. With the recent development of a user subroutine for the FE solver saturation time is now provided over the entire mercury domain. Its pattern agrees with spots of damage seen above and below the beam axis on the SNS inner vessel beam window and elsewhere. The other simulation result being compared to observed damage patterns is mercury velocity at the wall. Related R&D has provided evidence for the damage mitigation that higher wall velocity provides. In comparison to observations in SNS targets, inverse correlation of high velocity to damage is seen. In effect, it is the combination of the patterns of saturation time and low velocity that seems to match actual damage patterns.« less

Unusual Oxidative Limitations for Al-MAX Phases

NASA Technical Reports Server (NTRS)

Smialek, James L.

2017-01-01

Alumina-forming MAX phases are well-known for their excellent oxidation resistance, rivaling many metallic NiAl, NiCrAl, and FeCrAl counterparts and with upper temperature capability possible to approximately1400C. However a number of limitations have been emerging that need to be acknowledged to permit robust performance in demanding applications. Ti2AlC and Ti3AlC2 possess excellent scale adhesion, cyclic oxidation/moisture/volatility resistance, and TBC compatibility. However they are very sensitive to Al content and flux in order to maintain an exclusive Al2O3 scale without runaway oxidation of ubiquitous TiO2 transient scales. Accelerated oxidation has been shown to occur for Al-depleted, damaged, or roughened surfaces at temperatures less than 1200C. Conversely, Cr2AlC is less sensitive to transients, but exhibits volatile losses at 1200C or above if common Cr7C3 impurity phases are present. Poor scale adhesion is exhibited after oxidation at 1150C or above, where spallation occurs at the Cr7C3 (depletion zone) interface. Delayed spallation is significant and suggests a moisture-induced phenomenon similar to non-adherent metallic systems. Re-oxidation of this surface does not reproduce the initial pure Al2O3 behavior, but initiates a less-protective scale. Cr2AlC has also been shown to have good long term bonding with superalloys at 800C, but exhibits significant Beta-NiAl + Cr7C3 diffusion zones at 1100C and above. This may set limits on Cr2AlC as a high temperature TBC bond coat on Ni-based superalloys, while improving corrosion resistance in lower temperature applications.

HERSCHEL FINDS EVIDENCE FOR STELLAR WIND PARTICLES IN A PROTOSTELLAR ENVELOPE: IS THIS WHAT HAPPENED TO THE YOUNG SUN?

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ceccarelli, C.; López-Sepulcre, A.; Dominik, C.

2014-07-20

There is evidence that the young Sun emitted a high flux of energetic (≥10 MeV) particles. The collisions of these particles with the material at the inner edge of the Protosolar Nebula disk induced spallation reactions that formed short-lived radionuclei, like {sup 10}Be, whose trace is now visible in some meteorites. However, it is poorly known exactly when this happened, and whether and how it affected the solar system. Here, we present indirect evidence for an ejection of energetic particles in the young protostar, OMC-2 FIR 4, similar to that experienced by the young solar system. In this case, the energeticmore » particles collide with the material in the protostellar envelope, enhancing the abundance of two molecular ions, HCO{sup +} and N{sub 2}H{sup +}, whose presence is detected via Herschel observations. The flux of energetic particles at a distance of 1 AU from the emitting source, estimated from the measured abundance ratio of HCO{sup +} and N{sub 2}H{sup +}, can easily account for the irradiation required by meteoritic observations. These new observations demonstrate that the ejection of ≥10 MeV particles is a phenomenon occurring very early in the life of a protostar, before the disappearance of the envelope from which the future star accretes. The whole envelope is affected by the event, which sets constraints on the magnetic field geometry in the source and opens up the possibility that the spallation reactions are not limited to the inner edge of the Protosolar Nebula disk.« less

SPEAR — ToF neutron reflectometer at the Los Alamos Neutron Science Center

NASA Astrophysics Data System (ADS)

Dubey, M.; Jablin, M. S.; Wang, P.; Mocko, M.; Majewski, J.

2011-11-01

This article discusses the Surface ProfilE Analysis Reflectometer (SPEAR), a vertical scattering geometry time-of-flight reflectometer, at the Los Alamos National Laboratory Lujan Neutron Scattering Center. SPEAR occupies flight path 9 and receives spallation neutrons from a polychromatic, pulsed (20Hz) source that pass through a liquid-hydrogen moderator at 20K coupled with a Be filter to shift their energy spectrum. The spallation neutrons are generated by bombarding a tungsten target with 800MeV protons obtained from an accelerator. The process produces an integrated neutron flux of ˜ 3.4×106 cm-2 s-1 at a proton current of 100 μA. SPEAR employs choppers and frame overlap mirrors to obtain a neutron wavelength range of 4.5-16 Å. SPEAR uses a single 200mm long 3He linear position-sensitive detector with ˜ 2 mm FWHM resolution for simultaneous studies of both specular and off-specular scattering. SPEAR's moderated neutrons are collimated into a beam which impinges from above upon a level sample with an average angle of 0.9° to the horizontal, to facilitate air-liquid interface studies. In the vertical direction, the beam converges at the sample position. The neutrons can be further collimated to the desired divergence by finely slitting the beam using a set of two 10B4C slit packages. The instrument is ideally suited to study organic and inorganic thin films with total thicknesses between 5 and 3000 Å in a variety of environments. Specifically designed sample chambers available at the instrument provide the opportunity to study biological systems at the solid-liquid interface. SPEAR's unique experimental capabilities are demonstrated by specific examples in this article. Finally, an outlook for SPEAR and perspectives on future instrumentation are discussed.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Fedrigo, Anna, E-mail: anna.fedrigo@nbi.ku.dk; Istituto dei Sistemi Complessi, Consiglio Nazionale delle Ricerche, 50019 Sesto Fiorentino; European Spallation Source ESS AB, SE-221 00 Lund

VESPA, Vibrational Excitation Spectrometer with Pyrolytic-graphite Analysers, aims to probe molecular excitations via inelastic neutron scattering. It is a thermal high resolution inverted geometry time-of-flight instrument designed to maximise the use of the long pulse of the European Spallation Source. The wavelength frame multiplication technique was applied to provide simultaneously a broad dynamic range (about 0-500 meV) while a system of optical blind choppers allows to trade flux for energy resolution. Thanks to its high flux, VESPA will allow the investigation of dynamical and in situ experiments in physical chemistry. Here we describe the design parameters and the corresponding McStasmore » simulations.« less

Event-Based Processing of Neutron Scattering Data

DOE PAGES

Peterson, Peter F.; Campbell, Stuart I.; Reuter, Michael A.; ...

2015-09-16

Many of the world's time-of-flight spallation neutrons sources are migrating to the recording of individual neutron events. This provides for new opportunities in data processing, the least of which is to filter the events based on correlating them with logs of sample environment and other ancillary equipment. This paper will describe techniques for processing neutron scattering data acquired in event mode that preserve event information all the way to a final spectrum, including any necessary corrections or normalizations. This results in smaller final errors, while significantly reducing processing time and memory requirements in typical experiments. Results with traditional histogramming techniquesmore » will be shown for comparison.« less

Future prospects for measurements of mass hierarchy and CP violation

NASA Astrophysics Data System (ADS)

Lang, Karol

2015-03-01

We present a brief overview of current plans to pursue two challenging goals, resolution of the neutrino mass hierarchy and determination of the CP phase of the PMNS neutrino mixing matrix. Future prospects include large atmospheric experiments, PINGU, ORCA, and INO-ICAL, medium baseline reactor experiments, JUNO and RENO- 50, and long baseline accelerator experiments, LBNE, LBNO, and Hyper-Kamiokande. There are also new initiatives emerging, ESSνSB at the European Spallation Source, and CHIPS in the NuMI neutrino beam. This is a multifaceted, vigorous, and technically difficult world-wide program. It will likely take more than a decade to start reaping its benefits.

Indications for a High-Rigidity Break in the Cosmic-Ray Diffusion Coefficient

NASA Astrophysics Data System (ADS)

Génolini, Yoann; Serpico, Pasquale D.; Boudaud, Mathieu; Caroff, Sami; Poulin, Vivian; Derome, Laurent; Lavalle, Julien; Maurin, David; Poireau, Vincent; Rosier, Sylvie; Salati, Pierre; Vecchi, Manuela

2017-12-01

Using cosmic-ray boron to carbon ratio (B/C) data recently released by the Ams-02 experiment, we find indications (decisive evidence, in Bayesian terms) in favor of a diffusive propagation origin for the broken power-law spectra found in protons (p ) and helium nuclei (He). The result is robust with respect to currently estimated uncertainties in the cross sections, and in the presence of a small component of primary boron, expected because of spallation at the acceleration site. Reduced errors at high energy as well as further cosmic ray nuclei data (as absolute spectra of C, N, O, Li, Be) may definitively confirm this scenario.

Microcraters formed in glass by low density projectiles

NASA Technical Reports Server (NTRS)

Mandeville, J.-C.; Vedder, J. F.

1971-01-01

Microcraters were produced in soda-lime glass by the impact of low density projectiles of polystyrene with masses between 0.7 and 62 picograms and velocities between 2 and 14 kilometers per second. The morphology of the craters depends on the velocity and angle of incidence of the projectiles. The transitions in morphology of the craters formed by polystyrene spheres occur at higher velocities than they do for more dense projectiles. For oblique impact, the craters are elongated and shallow with the spallation threshold occuring at higher velocity. For normal incidence, the total displaced mass of the target material per unit of projectile kinetic energy increases slowly with the energy.

Improving the work function of the niobium surface of SRF cavities by plasma processing

DOE Office of Scientific and Technical Information (OSTI.GOV)

Tyagi, P. V.; Doleans, M.; Hannah, B.

2016-01-01

An in situ plasma processing technique using chemically reactive oxygen plasma to remove hydrocarbons from superconducting radio frequency cavity surfaces at room temperature was developed at the spallation neutron source, at Oak Ridge National Laboratory. To understand better the interaction between the plasma and niobium surface, surface studies on small samples were performed. In this article, we report the results from those surface studies. The results show that plasma processing removes hydrocarbons from top surface and improves the surface work function by 0.5₋1.0 eV. Improving the work function of RF surface of cavities can help to improve their operational performance.

Covariances for the 56Fe radiation damage cross sections

NASA Astrophysics Data System (ADS)

Simakov, Stanislav P.; Koning, Arjan; Konobeyev, Alexander Yu.

2017-09-01

The energy-energy and reaction-reaction covariance matrices were calculated for the n + 56Fe damage cross-sections by Total Monte Carlo method using the TENDL-2013 random files. They were represented in the ENDF-6 format and added to the unperturbed evaluation file. The uncertainties for the spectrum averaged radiation quantities in the representative fission, fusion and spallation facilities were first time assessed as 5-25%. Additional 5 to 20% have to be added to the atom displacement rate uncertainties to account for accuracy of the primary defects simulation in materials. The reaction-reaction correlation were shown to be 1% or less.

CSNS computing environment Based on OpenStack

NASA Astrophysics Data System (ADS)

Li, Yakang; Qi, Fazhi; Chen, Gang; Wang, Yanming; Hong, Jianshu

2017-10-01

Cloud computing can allow for more flexible configuration of IT resources and optimized hardware utilization, it also can provide computing service according to the real need. We are applying this computing mode to the China Spallation Neutron Source(CSNS) computing environment. So, firstly, CSNS experiment and its computing scenarios and requirements are introduced in this paper. Secondly, the design and practice of cloud computing platform based on OpenStack are mainly demonstrated from the aspects of cloud computing system framework, network, storage and so on. Thirdly, some improvments to openstack we made are discussed further. Finally, current status of CSNS cloud computing environment are summarized in the ending of this paper.

Foil cycling technique for the VESUVIO spectrometer operating in the resonance detector configuration

NASA Astrophysics Data System (ADS)

Schooneveld, E. M.; Mayers, J.; Rhodes, N. J.; Pietropaolo, A.; Andreani, C.; Senesi, R.; Gorini, G.; Perelli-Cippo, E.; Tardocchi, M.

2006-09-01

This article reports a novel experimental technique, namely, the foil cycling technique, developed on the VESUVIO spectrometer (ISIS spallation source) operating in the resonance detector configuration. It is shown that with a proper use of two foils of the same neutron absorbing material it is possible, in a double energy analysis process, to narrow the width of the instrumental resolution of a spectrometer operating in the resonance detector configuration and to achieve an effective subtraction of the neutron and gamma backgrounds. Preliminary experimental results, obtained from deep inelastic neutron scattering measurements on lead, zirconium hydride, and deuterium chloride samples, are presented.

Dual initiation strip charge apparatus and methods for making and implementing the same

DOEpatents

Jakaboski, Juan-Carlos [Albuquerque, NM; Todd,; Steven, N [Rio Rancho, NM; Polisar, Stephen [Albuquerque, NM; Hughs, Chance [Tijeras, NM

2011-03-22

A Dual Initiation Strip Charge (DISC) apparatus is initiated by a single initiation source and detonates a strip of explosive charge at two separate contacts. The reflection of explosively induced stresses meet and create a fracture and breach a target along a generally single fracture contour and produce generally fragment-free scattering and no spallation. Methods for making and implementing a DISC apparatus provide numerous advantages over previous methods of creating explosive charges by utilizing steps for rapid prototyping; by implementing efficient steps and designs for metering consistent, repeatable, and controlled amount of high explosive; and by utilizing readily available materials.

Converter target chemistry - A new challenge to radioanalytical chemistry.

PubMed

Choudhury, Dibyasree; Lahiri, Susanta

2018-07-01

The 1-2 GeV proton induced spallation reaction on the high Z materials like Hg, or lead bismuth eutectic (LBE), popularly known as converter targets, will produce strong flux of fast neutrons which would further react with fissile materials to produce intense radioactive ion beam (RIB). LBE offers suitability for use as converters over Hg but it suffers from the demerit of radiotoxic polonium production. These targets may be viewed as a store house of clinically important and other exotic radionuclides. For application of those radionuclides, radiochemical separation from bulk target material is of utmost importance. Copyright © 2018 Elsevier Ltd. All rights reserved.

Solar flare and galactic cosmic ray studies of Apollo 14 and 15 samples.

NASA Technical Reports Server (NTRS)

Crozaz, G.; Drozd, R.; Hohenberg, C. M.; Hoyt, H. P., Jr.; Ragan, D.; Walker, R. M.; Yuhas, D.

1972-01-01

Thermoluminescence (TL) measurements in rock 14310 show a strong depth dependence consistent with that expected from solar flares. This effect should prove useful in studying solar flare fluctuations in the time interval of 100 to 100,000 years. Rare gas spallation ages for rock 14301, 14306, and 14311 are respectively 102 plus or minus 30, 25 plus or minus 2, and 661 plus or minus 72 m.y. The 14306 value supports the idea that Cone Crater was formed 25 million years ago. Groupings of exposure ages suggest the dates of other major cratering events. Galactic track data in 14310 show little depth dependence.

Development of time projection chamber for precise neutron lifetime measurement using pulsed cold neutron beams

NASA Astrophysics Data System (ADS)

Arimoto, Y.; Higashi, N.; Igarashi, Y.; Iwashita, Y.; Ino, T.; Katayama, R.; Kitaguchi, M.; Kitahara, R.; Matsumura, H.; Mishima, K.; Nagakura, N.; Oide, H.; Otono, H.; Sakakibara, R.; Shima, T.; Shimizu, H. M.; Sugino, T.; Sumi, N.; Sumino, H.; Taketani, K.; Tanaka, G.; Tanaka, M.; Tauchi, K.; Toyoda, A.; Tomita, T.; Yamada, T.; Yamashita, S.; Yokoyama, H.; Yoshioka, T.

2015-11-01

A new time projection chamber (TPC) was developed for neutron lifetime measurement using a pulsed cold neutron spallation source at the Japan Proton Accelerator Research Complex (J-PARC). Managing considerable background events from natural sources and the beam radioactivity is a challenging aspect of this measurement. To overcome this problem, the developed TPC has unprecedented features such as the use of polyether-ether-ketone plates in the support structure and internal surfaces covered with 6Li-enriched tiles to absorb outlier neutrons. In this paper, the design and performance of the new TPC are reported in detail.

DANCE : a 4[pi] barium fluoride detector for measuring neutron capture on unstable nuclei /.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ullmann, J. L.; Haight, Robert C.; Hunt, L. F.

2002-01-01

Measurements of neutron capture on unstable nuclei are important for studies of s-process nucleosynthesis, nuclear waste transmutation, and stewardship science. A 160-element, 4{pi} barium fluoride detector array, and associated neutron flight path, is being constructed to make capture measurements at the moderated neutron spallation source at LANSCE. Measurements can be made on as little as 1 mg of sample material over energies from near thermal to near 100 keV. The design of the DANCE array is described and neutron flux measurements from flight path commissioning are shown. The array is expected to be complete by the end of 2002.

Neutron diffraction measurements on a reference metallic sample with a high-efficiency GEM side-on 10B-based thermal neutron detector

NASA Astrophysics Data System (ADS)

Pietropaolo, A.; Claps, G.; Fedrigo, A.; Grazzi, F.; Höglund, C.; Murtas, F.; Scherillo, A.; Schmidt, S.; Schooneveld, E. M.

2018-03-01

The upgraded version of the GEM side-on thermal neutron detector was successfully tested in a neutron diffraction experiment on a reference sample using the INES diffractometer at the ISIS spallation neutron source, UK. The performance of the new 10B4C-based detector is compared to that of a standard 3He tube, operating at the instrument as a part of the detectors assembly. The results show that the upgraded detector has a better resolution and an efficiency of the same order of magnitude of a 3He-based detector.

Characterization of the Multi-Blade 10B-based detector at the CRISP reflectometer at ISIS for neutron reflectometry at ESS

NASA Astrophysics Data System (ADS)

Piscitelli, F.; Mauri, G.; Messi, F.; Anastasopoulos, M.; Arnold, T.; Glavic, A.; Höglund, C.; Ilves, T.; Lopez Higuera, I.; Pazmandi, P.; Raspino, D.; Robinson, L.; Schmidt, S.; Svensson, P.; Varga, D.; Hall-Wilton, R.

2018-05-01

The Multi-Blade is a Boron-10-based gaseous thermal neutron detector developed to face the challenge arising in neutron reflectometry at neutron sources. Neutron reflectometers are challenging instruments in terms of instantaneous counting rate and spatial resolution. This detector has been designed according to the requirements given by the reflectometers at the European Spallation Source (ESS) in Sweden. The Multi-Blade has been installed and tested on the CRISP reflectometer at the ISIS neutron and muon source in U.K.. The results on the detailed detector characterization are discussed in this manuscript.

Search for Time Reversal Violating Effects: R-Correlation Measurement in Neutron Decay.

PubMed

Bodek, K; Ban, G; Beck, M; Bialek, A; Bryś, T; Czarnecki, A; Fetscher, W; Gorel, P; Kirch, K; Kistryn, St; Kozela, A; Kuźniak, M; Lindroth, A; Naviliat-Cuncic, O; Pulut, J; Serebrov, A; Severijns, N; Stephan, E; Zejma, J

2005-01-01

An experiment aiming at the simultaneous determination of both transversal polarization components of electrons emitted in the decay of free neutrons begins data taking using the polarized cold neutron beam (FUNSPIN) from the Swiss Neutron Spallation Source (SINQ) at the Paul-Scherrer Institute, Villigen. A non-zero value of R due to the e(-) polarization component, which is perpendicular to the plane spanned by the spin of the decaying neutron and the electron momentum, would signal a violation of time reversal symmetry and thus physics beyond the Standard Model. Present status of the project and the results from analysis of the first data sample will be discussed.

Comparison of isothermal and cyclic oxidation behavior of twenty-five commercial sheet alloys at 1150 C

NASA Technical Reports Server (NTRS)

Barrett, C. A.; Lowell, C. E.

1974-01-01

The cyclic and isothermal oxidation resistance of 25 high-temperature Ni-, Co-, and Fe-base sheet alloys after 100 hours in air at 1150 C was compared. The alloys were evaluated in terms of their oxidation, scaling, and vaporization rates and their tendency for scale spallation. These values were used to develop an oxidation rating parameter based on effective thickness change, as calculated from a mass balance. The calculated thicknesses generally agreed with the measured values, including grain boundary oxidation, to within a factor of 3. Oxidation behavior was related to composition, particularly Cr and Al content.

Photonuclear Contributions to SNS Pulse Shapes

DOE Office of Scientific and Technical Information (OSTI.GOV)

McClanahan, Tucker C.; Iverson, Erik B.; Gallmeier, Franz X.

Short-pulsed sources like the Spallation Neutron Source (SNS) and ISIS produce bursts of neutron pulses at rates of 10-60 Hz, with sub-microsecond proton pulses impacting on high-Z target materials. Moderators are grouped around the target to receive the fast neutrons generated from spallation reactions to moderate them effciently to thermal and sub-thermal energies and to feed narrow neutron pulses to neutron scattering instruments. The scattering instruments use the neutrons as a probe for material investigations, and make use of time-of-flight (TOF) methods for resolving the neutron energy. The energy resolution of scattering instruments depends on the narrow time-structure of themore » neutron pulses, while neutrons in the long tail of the emission time distributions can degrade the instrument performance and add undesired background to measurements. The SNS neutronics team is investigating a possible source term impacting the background at short-pulsed spallation sources. The ISIS TS2 project claims to have significantly reduced neutron scattering instrument background levels by the elimination or reduction of iron shielding in the target-moderator-reflector assembly. An alternative hypothesis, also proposed by ISIS, suggests that this apparent reduction arises from moving beamline shielding away from the neutron guide channels, reducing albedo down the beamlines. In both hypotheses, the background neutrons in question are believed to be generated by photonuclear reactions. If the background neutrons are indeed generated via photonuclear channels, then they are generated in a time-dependent fashion, since most of the high-energy photons capable of inducing photonuclear production are gone within a few microseconds following the proton pulse. To evaluate this e ect, we have enabled photonuclear reactions in a series of studies for the SNS first target station (FTS) taking advantage of its Monte Carlo model. Using a mixture of ENDF/B VII.0 and TENDL-2014 photonuclear cross sections available and the CEM03 physics model within MCNPX 2.6.0 in the simulation, we are able to estimate the impact of photoneutron production on both overall neutron production and delayed neutron production. We find that a significant number of photon-induced neutrons are produced a few milliseconds after the proton pulse, following prompt gamma emission through the capture of neutrons in the slowing-down and thermalization processes. We name these "slowing-down delayed neutrons" to distinguish them from either "activation-delayed neutrons" or "beta-delayed neutrons." The beta-delayed and activation-delayed neutrons were not part of this study, and will be addressed elsewhere. While these other delayed neutron channels result in the time-independent (constant) production of fast neutrons outside of the prompt pulse, the slowing-down delayed neutrons also a ect the shape of the pulses. Although numerically insignificant in most cases, we describe a set of scenarios related to T0-chopper operation in which the slowing-down delayed neutrons may be important.« less

Condensed-matter research at the Los Alamos pulsed neutron source (WNR)

DOE Office of Scientific and Technical Information (OSTI.GOV)

Eckert, J.

1982-01-01

The experimental program at the WNR in condensed matter research at present is aimed principally at utilizing the high epithermal neutron flux available at a spallation neutron source. Interesting new results have been obtained in several areas including hydrogen vibrations in metals, chemical vibrational spectroscopy and the structure of liquids. For example, extensive vibrational spectra were obtained of hydrogen in Nb which could be described in terms of a three-dimensional localized anharmonic oscillator, deuterium substitution methods were used to determine the variation with 0-0 distance of the hydrogen bending mode frequency in extremely short intramolecular hydrogen bonds, and model-independent partialmore » structure factors were determined for liquid water.« less

Plastic fiber scintillator response to fast neutrons

NASA Astrophysics Data System (ADS)

Danly, C. R.; Sjue, S.; Wilde, C. H.; Merrill, F. E.; Haight, R. C.

2014-11-01

The Neutron Imaging System at NIF uses an array of plastic scintillator fibers in conjunction with a time-gated imaging system to form an image of the neutron emission from the imploded capsule. By gating on neutrons that have scattered from the 14.1 MeV DT energy to lower energy ranges, an image of the dense, cold fuel around the hotspot is also obtained. An unmoderated spallation neutron beamline at the Weapons Neutron Research facility at Los Alamos was used in conjunction with a time-gated imaging system to measure the yield of a scintillating fiber array over several energy bands ranging from 1 to 15 MeV. The results and comparison to simulation are presented.

Plastic fiber scintillator response to fast neutrons.

PubMed

Danly, C R; Sjue, S; Wilde, C H; Merrill, F E; Haight, R C

2014-11-01

The Neutron Imaging System at NIF uses an array of plastic scintillator fibers in conjunction with a time-gated imaging system to form an image of the neutron emission from the imploded capsule. By gating on neutrons that have scattered from the 14.1 MeV DT energy to lower energy ranges, an image of the dense, cold fuel around the hotspot is also obtained. An unmoderated spallation neutron beamline at the Weapons Neutron Research facility at Los Alamos was used in conjunction with a time-gated imaging system to measure the yield of a scintillating fiber array over several energy bands ranging from 1 to 15 MeV. The results and comparison to simulation are presented.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kasemir, Kay; Pearson, Matthew R

For several years, the Control System Studio (CS-Studio) Scan System has successfully automated the operation of beam lines at the Oak Ridge National Laboratory (ORNL) High Flux Isotope Reactor (HFIR) and Spallation Neutron Source (SNS). As it is applied to additional beam lines, we need to support simultaneous adjustments of temperatures or motor positions. While this can be implemented via virtual motors or similar logic inside the Experimental Physics and Industrial Control System (EPICS) Input/Output Controllers (IOCs), doing so requires a priori knowledge of experimenters requirements. By adding support for the parallel control of multiple process variables (PVs) to themore » Scan System, we can better support ad hoc automation of experiments that benefit from such simultaneous PV adjustments.« less

High-pressure studies on Ba-doped cobalt perovskites by neutron diffraction

NASA Astrophysics Data System (ADS)

Cao, Huibo; Garlea, Vasile; Wang, Fangwei; Dos Santos, Antonio; Cheng, Zhaohua

2012-02-01

Cobalt perovskite possess rich structural, magnetic and electrical properties depending on the subtle balance of the interactions among the spin, charge, and orbital degrees of freedom. Divalent hole-doped cobalt perovskites LaA^2+CoO3 exhibit structural phase transitions, metal-insulator transitions, and multi-magnetic phase transitions. High-pressure measurement is believed to mimic the size effects of the doped ions. We performed neutron diffraction experiments on selected Ba-doped LaCoO3 under pressures up to 6.3 GPa at SNAP at Spallation Neutron Source of ORNL. This work focuses on the high-pressure effects of the selected Ba-doped samples and the change of the phase diagram with pressure.

S=2 quasi-one-dimensional spin waves in CrCl2

NASA Astrophysics Data System (ADS)

Stone, Matthew; Ehlers, Georg; Granroth, Garrett

2014-03-01

We examine the magnetic excitation spectrum in the S = 2 Heisenberg antiferromagnet CrCl2. Inelastic neutron scattering measurements on powder samples are able to determine the significant exchange interactions in this system. A large anisotropy gap is observed in the spectrum below the Néel temperature and the ratio of the two largest exchange constants is Jc /Jb = 9 . 1 +/- 2 . 2 . However, no sign of a gapped quantum spin liquid excitation was found in the paramagnetic phase. The research was performed at Oak Ridge National Laboratory's Spallation Neutron Source and was sponsored by the Scientific User Facilities Division, Office of Basic Energy Sciences, US Department of Energy.

Experimental Report: ORNL Proposal ID IPTS 8937

DOE Office of Scientific and Technical Information (OSTI.GOV)

Mirmelstein, A.

2014-02-03

Neutron scattering experiment was performed using fine-resolution Fermi chopper spectrometer “SEQUOIA” installed at the Spallation Neutron Source, ORNL. Although this spectrometer is designed to measure inelastic neutron scattering spectra, during experiments a signal of elastic scattering is also recorded. The coherent nuclear component of this elastic scattering provides Bragg diffraction pattern of a sample, i.e., CeNi single crystal in our case. Therefore, it is possible to follow the CeNi structural variations as a function of pressure and to register structural phase transition. Measurements were performed at the temperature of 15 K under pressure of zero (ambient pressure at 15 K),more » 400, 800, and 2200 bars.« less

Vacuum System Upgrade for Extended Q-Range Small-Angle Neutron Scattering Diffractometer (EQ-SANS) at SNS

DOE PAGES

Stone, Christopher M.; Williams, Derrick C.; Price, Jeremy P.

2016-09-23

The Extended Q-Range Small-Angle Neutron Scattering Diffractometer (EQ-SANS) instrument at the Spallation Neutron Source (SNS), Oak Ridge, Tennessee, incorporates a 69m3 detector vessel with a vacuum system which required an upgrade with respect to performance, ease of operation, and maintenance. The upgrade focused on improving pumping performance as well as optimizing system design to minimize opportunity for operational error. This upgrade provided the following practical contributions: Reduced time required to evacuate from atmospheric pressure to 2mTorr from 500-1,000 minutes to 60-70 minutes Provided turn-key automated control with a multi-faceted interlock for personnel and machine safety.

The ^58,60Ni(n,α) Reactions from Threshold to 50 MeV

NASA Astrophysics Data System (ADS)

Haight, R. C.; Bateman, F. B.; Sterbenz, S. M.; Chadwick, M. B.; Young, P. G.; Grimes, S. M.; Wasson, O. A.; Vonach, H.; Maier-Komor, P.

1996-10-01

Information on nuclear level densities over a wide range of excitation energies can be obtained from data on (n,α) reactions.(M. B. Chadwick et al., this meeting) We have measured α-particle emission cross sections, angular distributions and emission spectra for neutrons up to 50 MeV on targets of ^58Ni and ^60Ni using the pulsed spallation source of fast neutrons at the Los Alamos Neutron Science Center. The results will be compared with our previous measurements on ^59Co.(S. M. Grimes et al., Nuclear Science and Engineering in press) The possibilities of extending this method to much heavier nuclides will be discussed.

Installation Status of the Electron Beam Profiler for the Fermilab Main Injector

DOE Office of Scientific and Technical Information (OSTI.GOV)

Thurman-Keup, R.; Alvarez, M.; Fitzgerald, J.

2015-11-06

The planned neutrino program at Fermilab requires large proton beam intensities in excess of 2 MW. Measuring the transverse profiles of these high intensity beams is challenging and often depends on non-invasive techniques. One such technique involves measuring the deflection of a probe beam of electrons with a trajectory perpendicular to the proton beam. A device such as this is already in use at the Spallation Neutron Source at ORNL and the installation of a similar device is underway in the Main Injector at Fermilab. The present installation status of the electron beam profiler for the Main Injector will bemore » discussed together with some simulations and test stand results.« less

Modeling Oxidation Induced Stresses in Thermal Barrier Coatings

NASA Technical Reports Server (NTRS)

Ferguson, B. L.; Freborg, A. M.; Petrus, G. J.; Brindley, William J.

1998-01-01

The use of thermal barrier coatings (TBC's) in gas turbines has increased dramatically in recent years, due mainly to the need for component protection from ever increasing service temperatures. Oxidation of the bond coat has been identified as an important contributing factor to spallation of the ceramic top coat during service. Additional variables found to influence TBC thermal cycle life include bond coat coefficient of thermal expansion, creep behavior of both the ceramic and bond coat layers, and modulus of elasticity. The purpose of this work was to characterize the effects of oxidation on the stress states within the TBC system, as well as to examine the interaction of oxidation with other factors affecting TBC life.

Hybrid systems for transuranic waste transmutation in nuclear power reactors: state of the art and future prospects

NASA Astrophysics Data System (ADS)

Yurov, D. V.; Prikhod'ko, V. V.

2014-11-01

The features of subcritical hybrid systems (HSs) are discussed in the context of burning up transuranic wastes from the U-Pu nuclear fuel cycle. The advantages of HSs over conventional atomic reactors are considered, and fuel cycle closure alternatives using HSs and fast neutron reactors are comparatively evaluated. The advantages and disadvantages of two HS types with neutron sources (NSs) of widely different natures -- nuclear spallation in a heavy target by protons and nuclear fusion in magnetically confined plasma -- are discussed in detail. The strengths and weaknesses of HSs are examined, and demand for them for closing the U-Pu nuclear fuel cycle is assessed.

Neutron total cross-section of hydrogenous and deuterated 1- and 2-propanol and n-butanol measured using the VESUVIO spectrometer

NASA Astrophysics Data System (ADS)

Rodríguez Palomino, L. A.; Dawidowski, J.; Márquez Damián, J. I.; Cuello, G. J.; Romanelli, G.; Krzystyniak, M.

2017-10-01

This work presents the total cross sections of a set of normal and deuterated alcohols (hydrogenous 1- and 2-propanol and n-butanol, 1-propanol(OD) and fully deuterated 2-propanol and n-butanol), measured at spectrometer VESUVIO (ISIS spallation neutron source, United Kingdom). Granada's Synthetic Model was applied to describe those systems and a satisfactory agreement with the measured total cross section was achieved in the range of energies from 10-3 to 100 eV. The input parameters of the model were determined from the essential features of the vibrational spectra of the atoms that compose the systems, which were studied using Molecular Dynamics.

Aerodynamic laser-heated contactless furnace for neutron scattering experiments at elevated temperatures

NASA Astrophysics Data System (ADS)

Landron, Claude; Hennet, Louis; Coutures, Jean-Pierre; Jenkins, Tudor; Alétru, Chantal; Greaves, Neville; Soper, Alan; Derbyshire, Gareth

2000-04-01

Conventional radiative furnaces require sample containment that encourages contamination at elevated temperatures and generally need windows which restrict the entrance and exit solid angles required for diffraction and scattering measurements. We describe a contactless windowless furnace based on aerodynamic levitation and laser heating which has been designed for high temperature neutron scattering experiments. Data from initial experiments are reported for crystalline and amorphous oxides at temperatures up to 1900 °C, using the spallation neutron source ISIS together with our laser-heated aerodynamic levitator. Accurate reproduction of thermal expansion coefficients and radial distribution functions have been obtained, demonstrating the utility of aerodynamic levitation methods for neutron scattering methods.

Vacuum System Upgrade for Extended Q-Range Small-Angle Neutron Scattering Diffractometer (EQ-SANS) at SNS

DOE Office of Scientific and Technical Information (OSTI.GOV)

Stone, Christopher M.; Williams, Derrick C.; Price, Jeremy P.

The Extended Q-Range Small-Angle Neutron Scattering Diffractometer (EQ-SANS) instrument at the Spallation Neutron Source (SNS), Oak Ridge, Tennessee, incorporates a 69m3 detector vessel with a vacuum system which required an upgrade with respect to performance, ease of operation, and maintenance. The upgrade focused on improving pumping performance as well as optimizing system design to minimize opportunity for operational error. This upgrade provided the following practical contributions: Reduced time required to evacuate from atmospheric pressure to 2mTorr from 500-1,000 minutes to 60-70 minutes Provided turn-key automated control with a multi-faceted interlock for personnel and machine safety.

The diffuse gamma-ray background, light element abundances, and signatures of early massive star formation

NASA Technical Reports Server (NTRS)

Silk, Joseph; Schramm, David N.

1992-01-01

Attention is drawn to a potentially observable flux of diffuse extragalactic gamma rays produced by inelastic cosmic-ray interactions that is inevitably a by-product of spallation-synthesized Be. The epoch of cosmic ray-induced Population II light element nucleosynthesis is constrained to be at redshift greater than 0.5. A spectral feature in the diffuse extragalactic gamma-ray background with amplitude 0.1 above 10 MeV is predicted if the Be is synthesized at z less than 10. The possibility is discussed that the cosmic-ray flux responsible for Population II Be and B synthesis may be associated with a precursor hypothesized Population III.

Energy-resolved fast neutron resonance radiography at CSNS

NASA Astrophysics Data System (ADS)

Tan, Zhixin; Tang, Jingyu; Jing, Hantao; Fan, Ruirui; Li, Qiang; Ning, Changjun; Bao, Jie; Ruan, Xichao; Luan, Guangyuan; Feng, Changqin; Zhang, Xianpeng

2018-05-01

The white neutron beamline at the China Spallation Neutron Source will be used mainly for nuclear data measurements. It will be characterized by high flux and broad energy spectra. To exploit the beamline as a neutron imaging source, we propose a liquid scintillator fiber array for fast neutron resonance radiography. The fiber detector unit has a small exposed area, which will limit the event counts and separate the events in time, thus satisfying the requirements for single-event time-of-flight (SEToF) measurement. The current study addresses the physical design criteria for ToF measurement, including flux estimation and detector response. Future development and potential application of the technology are also discussed.

Performance of the New Los Alamos UCN Source and Implications for Future Experiments

NASA Astrophysics Data System (ADS)

Makela, Mark; LANL UCN Team

2017-01-01

The Los Alamos Ultracold Neutron (UCN) source was replaced during this past summer and has been commissioned during the last few months. The new source is the result of lessons learned during the 10 year operation of the first UCN source and extensive Monte Carlo analysis. The new source is a spallation driven source based on a solid deuterium UCN moderator similar the previous one. This talk will present an overview of the new source design and the results of commissioning tests. The talk will conclude with a brief overview of the implications of source performance on the neutron lifetime and LANL nEDM experiments. This work was funded by LANL LDRD.

Late-time particle emission from laser-produced graphite plasma

NASA Astrophysics Data System (ADS)

Harilal, S. S.; Hassanein, A.; Polek, M.

2011-09-01

We report a late-time "fireworks-like" particle emission from laser-produced graphite plasma during its evolution. Plasmas were produced using graphite targets excited with 1064 nm Nd: yttrium aluminum garnet (YAG) laser in vacuum. The time evolution of graphite plasma was investigated using fast gated imaging and visible emission spectroscopy. The emission dynamics of plasma is rapidly changing with time and the delayed firework-like emission from the graphite target followed a black-body curve. Our studies indicated that such firework-like emission is strongly depended on target material properties and explained due to material spallation caused by overheating the trapped gases through thermal diffusion along the layer structures of graphite.

Science-based stockpile stewardship at LANSCE

DOE Office of Scientific and Technical Information (OSTI.GOV)

Browne, J.

1995-10-01

Let me tell you a little about the Los Alamos Neutron Science Center (LANSCE) and how some of the examples you heard about from Sig Hecker and John Immele fit together in this view of a different world in the future where defense, basic and industrial research overlap. I am going to talk about science-based stockpile stewardship at LANSCE; the accelerator production of tritium (APT), which I think has a real bearing on the neutron road map; the world-class neutron science user facility, for which I will provide some examples so you can see the connection with defense science; andmore » lastly, testing concepts for a high-power spallation neutron target and waste transmutation.« less

Development of a moderator system for the High Brilliance Neutron Source project

NASA Astrophysics Data System (ADS)

Dabruck, J. P.; Cronert, T.; Rücker, U.; Bessler, Y.; Klaus, M.; Lange, C.; Butzek, M.; Hansen, W.; Nabbi, R.; Brückel, T.

2016-11-01

The project for an accelerator based high brilliance neutron source HBS driven by Forschungszentrum Jülich forsees the use of the nuclear Be(p,n) or Be(d,n) reaction with accelerated particles in the lower MeV energy range. The lower neutron production compared to spallation has to be compensated by improving the neutron extraction process and optimizing the brilliance. Design and optimiziation of the moderator system are conducted with MCNP and will be validated with measurements at the AKR-2 training reactor by means of a prototype assembly where, e.g., the effect of different liquid H2 ortho/para ratios will be investigated and controlled in realtime via online heat capacity measurements.

Measurement of the energy and multiplicity distributions of neutrons from the photofission of U 235

DOE PAGES

Clarke, S. D.; Wieger, B. M.; Enqvist, A.; ...

2017-06-20

For the first time, the complete neutron multiplicity distribution has been measured in this study from the photofission of 235U induced by high-energy spallation γ rays arriving ahead of the neutron beam at the Los Alamos Neutron Science Center. The resulting average neutron multiplicity 3.80 ± 0.08 (stat.) neutrons per photofission is in general agreement with previous measurements. In addition, unique measurements of the prompt fission energy spectrum of the neutrons from photofission and the angular correlation of two-neutron energies emitted in photofission also were made. Finally, the results are compared to calculations with the complete event fission model FREYA.

A novel small-angle neutron scattering detector geometry

PubMed Central

Kanaki, Kalliopi; Jackson, Andrew; Hall-Wilton, Richard; Piscitelli, Francesco; Kirstein, Oliver; Andersen, Ken H.

2013-01-01

A novel 2π detector geometry for small-angle neutron scattering (SANS) applications is presented and its theoretical performance evaluated. Such a novel geometry is ideally suited for a SANS instrument at the European Spallation Source (ESS). Motivated by the low availability and high price of 3He, the new concept utilizes gaseous detectors with 10B as the neutron converter. The shape of the detector is inspired by an optimization process based on the properties of the conversion material. Advantages over the detector geometry traditionally used on SANS instruments are discussed. The angular and time resolutions of the proposed detector concept are shown to satisfy the requirements of the particular SANS instrument. PMID:24046504

SNS Central Helium Liquefier spare Carbon Bed installation and commissioning

NASA Astrophysics Data System (ADS)

DeGraff, B.; Howell, M.; Kim, S.; Neustadt, T.

2017-12-01

The Spallation Neutron Source (SNS) Central Helium Liquefier (CHL) at Oak Ridge National Laboratory (ORNL) has been without major operations downtime since operations were started back in 2006. This system utilizes a vessel filled with activated carbon as the final major component to remove oil vapor from the compressed helium circuit prior to insertion into the system’s cryogenic cold box. The need for a spare carbon bed at SNS due to the variability of carbon media lifetime calculation to adsorption efficiency will be discussed. The fabrication, installation and commissioning of this spare carbon vessel will be presented. The novel plan for connecting the spare carbon vessel piping to the existing infrastructure will be presented.

Energy-dispersive neutron imaging and diffraction of magnetically driven twins in a Ni2MnGa single crystal magnetic shape memory alloy

NASA Astrophysics Data System (ADS)

Kabra, Saurabh; Kelleher, Joe; Kockelmann, Winfried; Gutmann, Matthias; Tremsin, Anton

2016-09-01

Single crystals of a partially twinned magnetic shape memory alloy, Ni2MnGa, were imaged using neutron diffraction and energy-resolved imaging techniques at the ISIS spallation neutron source. Single crystal neutron diffraction showed that the crystal produces two twin variants with a specific crystallographic relationship. Transmission images were captured using a time of flight MCP/Timepix neutron counting detector. The twinned and untwinned regions were clearly distinguishable in images corresponding to narrow-energy transmission images. Further, the spatially-resolved transmission spectra were used to elucidate the orientations of the crystallites in the different volumes of the crystal.

SNS STRIPPER FOIL FAILURE MODES AND THEIR CURES

DOE Office of Scientific and Technical Information (OSTI.GOV)

Galambos, John D; Luck, Chris; Plum, Michael A

2010-01-01

The diamond stripper foils in use at the Spallation Neutron Source worked successfully with no failures until May 3, 2009, when we started experiencing a rash of foil system failures after increasing the beam power to ~840 kW. The main contributors to the failures are thought to be 1) convoy electrons, stripped from the incoming H beam, that strike the foil bracket and may also reflect back from the electron catcher, and 2) vacuum breakdown from the charge developed on the foil by secondary electron emission. In this paper we will detail these and other failure mechanisms, and describe themore » improvements we have made to mitigate them.« less

Modeling and Characterization of the Magnetocaloric Effect in Ni2MnGa Materials

DOE Office of Scientific and Technical Information (OSTI.GOV)

Nicholson, Don M; Odbadrakh, Khorgolkhuu; Shassere, Benjamin

2014-01-01

Magnetic shape memory alloys have great promise as magneto-caloric effect refrigerant materials due to their combined magnetic and structural transitions. Computational and experimental research is reported on the Ni2MnGa material system. The magnetic states of this system are explored using the Wang-Landau statistical approach in conjunction with the Locally Self-consistent Multiple-Scattering method. The effects of alloying agents on the transition temperatures of the Ni2MnGa alloy are investigated using differential scanning calorimetry and superconducting quantum interference device. Experiments are performed at the Spallation Neutron Source at Oak Ridge National Laboratory to observe the structural and magnetic phase transformations.

Spallation yield of neutrons produced in thick lead target bombarded with 250 MeV protons

NASA Astrophysics Data System (ADS)

Chen, L.; Ma, F.; Zhanga, X. Y.; Ju, Y. Q.; Zhang, H. B.; Ge, H. L.; Wang, J. G.; Zhou, B.; Li, Y. Y.; Xu, X. W.; Luo, P.; Yang, L.; Zhang, Y. B.; Li, J. Y.; Xu, J. K.; Liang, T. J.; Wang, S. L.; Yang, Y. W.; Gu, L.

2015-01-01

The neutron yield from thick target of Pb irradiated with 250 MeV protons has been studied experimentally. The neutron production was measured with the water-bath gold method. The thermal neutron distributions in the water were determined according to the measured activities of Au foils. Corresponding results calculated with the Monte Carlo code MCNPX were compared with the experimental data. It was found out that the Au foils with cadmium cover significantly changed the spacial distribution of the thermal neutron field. The corrected neutron yield was deduced to be 2.23 ± 0.19 n/proton by considering the influence of the Cd cover on the thermal neutron flux.

Analysis of radiation environmental safety for China's Spallation Neutron Source (CSNS)

NASA Astrophysics Data System (ADS)

Wang, Qing-Bin; Wu, Qing-Biao; Ma, Zhong-Jian; Zhang, Qing-Jiang; Li, Nan; Wu, Jing-Min; Liu, Jian; Zhang, Gang

2010-07-01

The China Spallation Neutron Source (CSNS) is going to be located in Dalang Town, Dongguan City in the Guangdong Province. In this paper we report the results of the parameters related with environment safety based on experiential calculations and Monte Carlo simulations. The main project of the accelerator is an under ground construction. On top there is a 0.5 m concrete and 5.0 m soil covering for shielding, which can reduce the dose out of the tunnel's top down to 0.2 μSv/h. For the residents on the boundary of the CSNS, the dose produced by skyshine, which is caused by the penetrated radiation leaking from the top of the accelerator, is no more than 0.68 μSv/a. When CSNS is operating normally, the maximal annual effective dose due to the emission of gas from the tunnel is 2.40×10-3 mSv/a to the public adult, and 2.29×10-3 mSv/a to a child, both values are two orders of magnitude less than the limiting value for control and management. CSNS may give rise to an activation of the soil and groundwater in the nearest tunnels, where the main productions are 3H, 7Be, 22Na, 54Mn, etc. But the specific activity is less than the exempt specific activity in the national standard GB13376-92. So it is safe to say that the environmental impact caused by the activation of soil and groundwater is insignificant. To sum up, for CSNS, as a powerful neutron source device, driven by a high-energy high-current proton accelerator, a lot of potential factors affecting the environment exist. However, as long as effective shieldings for protection are adopted and strict rules are drafted, the environmental impact can be kept under control within the limits of the national standard.

Superconducting Prototype Cavities for the Spallation Neutron Source (SNS) Project

DOE Office of Scientific and Technical Information (OSTI.GOV)

G. Ciovati, P. Kneisel , J. Brawley, R. Bundy, I. Campisi, K. Davis; K. Macha; D. Machie

2001-09-01

The Spallation Neutron Source project includes a superconducting linac section in the energy range from 192 MeV to 1000 MeV, operating at a frequency of 805 MHz at 2.1 K. For this energy range two types of cavities are needed with geometrical beta - values of beta= 0.61 and beta= 0.81. An aggressive cavity prototyping program is being pursued at Jlab, which calls for fabricating and testing of four beta= 0.61 cavities and two beta= 0.81 cavities. Both types consist of six cells made from high purity niobium and feature one HOM coupler on each beam pipe and a portmore » for a high power coaxial input coupler. Three of the four beta= 0.61 cavities will be used for a cryomodule test in early 2002. At this time four medium beta cavities and one high beta cavity have been completed at JLab. The first tests on the beta=0.61 cavity and the beta= 0.81 exceeded the design values for gradient and Q - value: E{sub acc} = 1 0.3 MV/m and Q = 5 x 10{sup 9} at 2.1K for beta= 0.61 and E{sub acc} = 12.3 MV/m and Q = 5 x 10{sup 9} at 2.1K for beta= 0.81. One of the medium beta cavities has been equipped with an integrated helium vessel and measurements of the static and dynamic Lorentz force detuning will be done and compared to the ''bare'' cavities. In addition two single cell cavities have been fabricated, equipped with welded-on HOM couplers. They are being used to evaluate the HOM couplers with respect to multipacting, fundamental mode rejection and HOM damping as far as possible in a single cell. This paper will describe the cavity design with respect to electrical and mechanical features, the fabrication efforts and the results obtained with the different cavities existing at the time of this workshop.« less

Superconducting Prototype Cavities for the Spallation Neutron Source (SNS) Project

DOE Office of Scientific and Technical Information (OSTI.GOV)

G. Ciovati; P. Kneisel; K. Davis

2002-06-01

The Spallation Neutron Source project includes a superconducting linac section in the energy range from 186 MeV to 1000 MeV operating at a frequency of 805 MHz at 2.1 K. For this energy range two types of cavities are needed with geometrical Beta-values of Beta=0.61 and Beta=0.81. An aggressive cavity prototyping program is being pursued at JLab, which calls for fabricating and testing of four Beta=0.61 cavities and two Beta=0.81 cavities. Both types consist of six cells made from high purity niobium and feature one HOM coupler of the TESLA type on each beam pipe and a port for amore » high power coaxial input coupler. Three of the four Beta=0.61 cavities will be used for a cryomodule test in early 2002. At this time, four medium beta cavities and one high beta cavity have been completed and tested at JLab. In addition, the three medium beta cavities for the prototype cryomodule have been equipped with the integrated Ti-Helium vessel, successfully retested and will be assembled into a cavity string. Results from the cryo-module test should be available by the time of the conference. The tests on the Beta=0.61 cavity and the Beta=0.81 cavity exceeded the design values for gradient and Q - value: E{sub acc} =10.1 MV/m and Q = 5 x 10{sup 9} at 2.1K for Beta=0.61 and E{sub acc} = 12.3 MV/m and Q=5 x 10{sup 9} at 2.1K for Beta = 0.81. The medium beta cavities reached gradients between E{sub acc} = 15 MV/m and 21 MV/m. This paper will describe the test results obtained with the various cavities, some aspects of the HOM damping at cryogenic temperatures, results from microphonics and Lorentz force detuning tests and the cavity string assembly at the time of this workshop.« less

The ESS neutrino facility for CP violation discovery

NASA Astrophysics Data System (ADS)

Baussan, Eric; Bouquerel, Elian; Dracos, Marcos

2017-09-01

The comparatively large value of the neutrino mixing angle θ 13 measured in 2012 by neutrino reactor experiments has opened the possibility to observe for the first time CP violation in the leptonic sector. The measured value of θ 13 also privileges the 2nd oscillation maximum for the discovery of CP violation instead of the usually used 1st oscillation maximum. The sensitivity at the 2nd oscillation maximum is about three times higher than at the 1st oscillation maximum implying a significantly lower sensitivity to systematic errors. Measuring at the 2nd oscillation maximum necessitates a very intense neutrino beam with the appropriate energy. The world’s most intense pulsed spallation neutron source, the European Spallation Source, has a proton linac with 5 MW power and 2 GeV energy. This linac also has the potential to become the proton driver of the world’s most intense neutrino beam with very high potential for the discovery of neutrino CP violation. The physics performance of that neutrino Super Beam in conjunction with a megaton Water Cherenkov neutrino detector installed ca 1000 m down in a mine at a distance of about 500 km from ESS has been evaluated. In addition, the use of such a detector will make it possible to extent the physics program to proton decay, atmospheric neutrinos and astrophysics searches. The ESS proton linac upgrade, the accumulator ring needed for proton pulse compression, the target station optimization and the physics potential are described. In addition to the production of neutrinos, this facility will also be a copious source of muons which could be used to feed a low energy nuSTORM facility, a future neutrino factory or a muon collider. The ESS linac, under construction, will reach full operation at 5 MW by 2023 after which the upgrades for the neutrino facility could start.

Sns Moderator Poison Design and Experiment Validation of the Moderator Performance

NASA Astrophysics Data System (ADS)

Lu, W.; Iverson, E. B.; Ferguson, P. D.; Crabtree, J. A.; Gallmeier, F. X.; Remec, I.; Baxter, D. V.; Lavelle, C. M.

2009-08-01

The Spallation Neutron Source (SNS) at Oak Ridge National Laboratory reached 180 kW in August 2007, becoming the brightest pulsed neutron source in the world. At its full power of 1.4 MW, SNS will have thermal neutron fluxes approximately an order of magnitude greater than any existing pulsed spallation source. It thus brings a serious challenge to the lifetime of the moderator poison sheets. The SNS moderators are integrated with the inner reflector plug (IRP) at a cost of $2 million a piece. A replacement of the IRP presents a significant drawback to the facility due to the activation and the operation cost. Although there are many factors limiting the lifetime of the IRP, such as radiation damage to the structural material and helium production in beryllium, the limiting factor is the lifetime of the moderator poison sheets. The current operating target system of SNS was built with thick Gd poison sheets at a projected lifetime of 3 years. A recent design based on the MCNPX calculation proposed to replace the Gd poison sheets with even thicker Cd poison sheets, aiming to extend the poison sheet lifetime from 3 to 4 years accompanied by an approximate 5% gain of the moderator performance. An experiment was carried out to verify the calculated moderator performance at the Low Energy Neutron Source (LENS), Indiana University, where the spectra of two polyethylene moderators were measured. The moderators are Cd-decoupled and are poisoned with 0.8 mm Gd and 1.2 mm Cd, respectively. The preliminary analysis of the experiment data shows that the characteristics of the measured spectra of the Gd- and Cd-poisoned moderators agree well with what the calculation predicted. A better moderator performance is observed in the Cd-poisoned moderator. The measured ratio of Cd over Gd on the moderator performance is in a reasonable agreement with the calculation. Further investigation is underway for a better understanding of the difference between the experiment and the calculation.

Thermal hydraulic design and decay heat removal of a solid target for a spallation neutron source

NASA Astrophysics Data System (ADS)

Takenaka, N.; Nio, D.; Kiyanagi, Y.; Mishima, K.; Kawai, M.; Furusaka, M.

2005-08-01

Thermal hydraulic design and thermal stress calculations were conducted for a water-cooled solid target irradiated by a MW-class proton beam for a spallation neutron source. Plate type and rod bundle type targets were examined. The thickness of the plate and the diameter of the rod were determined based on the maximum and the wall surface temperature. The thermal stress distributions were calculated by a finite element method (FEM). The neutronics performance of the target is roughly proportional to its average density. The averaged densities of the designed targets were calculated for tungsten plates, tantalum clad tungsten plates, tungsten rods sheathed by tantalum and Zircaloy and they were compared with mercury density. It was shown that the averaged density was highest for the tungsten plates and was high for the tantalum cladding tungsten plates, the tungsten rods sheathed by tantalum and Zircaloy in order. They were higher than or equal to that of mercury for the 1 2 MW proton beams. Tungsten target without the cladding or the sheath is not practical due to corrosion by water under irradiation condition. Therefore, the tantalum cladding tungsten plate already made successfully by HIP and the sheathed tungsten rod are the candidate of high performance solid targets. The decay heat of each target was calculated. It was low enough low compared to that of ISIS for the target without tantalum but was about four times as high as that of ISIS when the thickness of the tantalum cladding was 0.5 mm. Heat removal methods of the decay heat with tantalum were examined. It was shown that a special cooling system was required for the target exchange when tantalum was used for the target. It was concluded that the tungsten rod target sheathed with stainless steel or Zircaloy was the most reliable from the safety considerations and had similar neutronics performance to that of mercury.

R&D of A MW-class solid-target for a spallation neutron source

NASA Astrophysics Data System (ADS)

Kawai, Masayoshi; Furusaka, Michihiro; Kikuchi, Kenji; Kurishita, Hiroaki; Watanabe, Ryuzo; Li, Jing-Feng; Sugimoto, Katsuhisa; Yamamura, Tsutomu; Hiraoka, Yutaka; Abe, Katsunori; Hasegawa, Akira; Yoshiie, Masatoshi; Takenaka, Hiroyuki; Mishima, Katsuichiro; Kiyanagi, Yoshiaki; Tanabe, Tetsuo; Yoshida, Naoaki; Igarashi, Tadashi

2003-05-01

R&D for a MW-class solid target composed of tungsten was undertaken to produce a pulsed intense neutron source for a future neutron scattering-facility. In order to solve the corrosion of tungsten, tungsten target blocks were clad with tantalum by means of HIP'ing, brazing and electrolytic coating in a molten salt bath. The applicability of the HIP'ing method was tested through fabricating target blocks for KENS (spallation neutron source at KEK). A further investigation to certify the optimum HIP conditions was made with the small punch test method. The results showed that the optimum temperature was 1500 °C at which the W/Ta interface gave the strongest fracture strength. In the case of the block with a hole for thermocouple, it was found that the fabrication preciseness of a straight hole and a tantalum sheath influenced the results. The development of a tungsten stainless-steel alloy was tried to produce a bare tungsten target, using techniques in powder metallurgy. Corrosion tests for various tungsten alloys were made while varying the water temperature and velocity. The mass loss of tungsten in very slow water at 180 °C was as low as 0.022 mg/y, but increased remarkably with water velocity. Simulation experiments for radiation damage to supplement the STIP-III experiments were made to investigate material hardening by hydrogen and helium, and microstructures irradiated by electrons. Both experiments showed consistent results on the order of the dislocation numbers and irradiation hardness among the different tungsten materials. Thermal-hydraulic designs were made for two types of solid target system of tungsten: slab and rod geometry as a function of the proton beam power. The neutronic performance of a solid target system was compared with that of mercury target based on Monte Carlo calculations by using the MCNP code.

High Speed Dynamics in Brittle Materials

NASA Astrophysics Data System (ADS)

Hiermaier, Stefan

2015-06-01

Brittle Materials under High Speed and Shock loading provide a continuous challenge in experimental physics, analysis and numerical modelling, and consequently for engineering design. The dependence of damage and fracture processes on material-inherent length and time scales, the influence of defects, rate-dependent material properties and inertia effects on different scales make their understanding a true multi-scale problem. In addition, it is not uncommon that materials show a transition from ductile to brittle behavior when the loading rate is increased. A particular case is spallation, a brittle tensile failure induced by the interaction of stress waves leading to a sudden change from compressive to tensile loading states that can be invoked in various materials. This contribution highlights typical phenomena occurring when brittle materials are exposed to high loading rates in applications such as blast and impact on protective structures, or meteorite impact on geological materials. A short review on experimental methods that are used for dynamic characterization of brittle materials will be given. A close interaction of experimental analysis and numerical simulation has turned out to be very helpful in analyzing experimental results. For this purpose, adequate numerical methods are required. Cohesive zone models are one possible method for the analysis of brittle failure as long as some degree of tension is present. Their recent successful application for meso-mechanical simulations of concrete in Hopkinson-type spallation tests provides new insight into the dynamic failure process. Failure under compressive loading is a particular challenge for numerical simulations as it involves crushing of material which in turn influences stress states in other parts of a structure. On a continuum scale, it can be modeled using more or less complex plasticity models combined with failure surfaces, as will be demonstrated for ceramics. Models which take microstructural cracking directly into account may provide a more physics-based approach for compressive failure in the future.

L2 Milestone 5433: Characterization of Dynamic Behavior of AM and Conventionally Processed Stainless Steel (316L and 304L)

DOE Office of Scientific and Technical Information (OSTI.GOV)

Gray, George Thompson; Livescu, Veronica; Rigg, P. A.

For additive manufacturing (AM) of metallic materials, the certification and qualification paradigm needs to evolve as there currently exists no broadly accepted “ASTM- or DIN-type” additive manufacturing certified process or AM-material produced specifications. Accordingly, design, manufacture, and thereafter implementation and insertion of AM materials to meet engineering applications requires detailed quantification of the constitutive (strength and damage) properties of these evolving materials, across the spectrum of metallic AM methods, in comparison/contrast to conventionally-manufactured metals and alloys. This report summarizes the 316L SS research results and presents initial results of the follow-on study of 304L SS. For the AM-316L SS investigation,more » cylindrical samples of 316L SS were produced using a LENS MR-7 laser additive manufacturing system from Optomec (Albuquerque, NM) equipped with a 1kW Yb-fiber laser. The microstructure of the AM-316L SS was characterized in both the “as-built” Additively Manufactured state and following a heat-treatment designed to obtain full recrystallization to facilitate comparison with annealed wrought 316L SS. The dynamic shock-loading-induced damage evolution and failure response of all three 316L SS materials was quantified using flyer-plate impact driven spallation experiments at peak stresses of 4.5 and 6.35 GPa. The results of these studies are reported in detail in the first section of the report. Publication of the 316L SS results in an archival journal is planned. Following on from the 316L SS completed work, initial results on a study of AM 304L SS are in progress and presented herein. Preliminary results on the structure/dynamic spallation property behavior of AM-304L SS fabricated using both the directed-energy LENS and an EOS powder-bed AM techniques in comparison to wrought 304L SS is detailed in this Level 2 Milestone report.« less

Small Gas Bubble Experiment for Mitigation of Cavitation Damage and Pressure Waves in Short-pulse Mercury Spallation Targets

DOE Office of Scientific and Technical Information (OSTI.GOV)

Wendel, Mark W; Felde, David K; Sangrey, Robert L

2014-01-01

Populations of small helium gas bubbles were introduced into a flowing mercury experiment test loop to evaluate mitigation of beam-pulse induced cavitation damage and pressure waves. The test loop was developed and thoroughly tested at the Spallation Neutron Source (SNS) prior to irradiations at the Los Alamos Neutron Science Center - Weapons Neutron Research Center (LANSCE-WNR) facility. Twelve candidate bubblers were evaluated over a range of mercury flow and gas injection rates by use of a novel optical measurement technique that accurately assessed the generated bubble size distributions. Final selection for irradiation testing included two variations of a swirl bubblermore » provided by Japan Proton Accelerator Research Complex (J-PARC) collaborators and one orifice bubbler developed at SNS. Bubble populations of interest consisted of sizes up to 150 m in radius with achieved gas void fractions in the 10^-5 to 10^-4 range. The nominal WNR beam pulse used for the experiment created energy deposition in the mercury comparable to SNS pulses operating at 2.5 MW. Nineteen test conditions were completed each with 100 pulses, including variations on mercury flow, gas injection and protons per pulse. The principal measure of cavitation damage mitigation was surface damage assessment on test specimens that were manually replaced for each test condition. Damage assessment was done after radiation decay and decontamination by optical and laser profiling microscopy with damaged area fraction and maximum pit depth being the more valued results. Damage was reduced by flow alone; the best mitigation from bubble injection was between half and a quarter that of flow alone. Other data collected included surface motion tracking by three laser Doppler vibrometers (LDV), loop wall dynamic strain, beam diagnostics for charge and beam profile assessment, embedded hydrophones and pressure sensors, and sound measurement by a suite of conventional and contact microphones.« less

Large ejecta fragments from asteroids. [Abstract only

NASA Technical Reports Server (NTRS)

Asphaug, E.

1994-01-01

The asteroid 4 Vesta, with its unique basaltic crust, remains a key mystery of planetary evolution. A localized olivine feature suggests excavation of subcrustal material in a crater or impact basin comparable in size to the planetary radius (R(sub vesta) is approximately = 280 km). Furthermore, a 'clan' of small asteroids associated with Vesta (by spectral and orbital similarities) may be ejecta from this impact 151 and direct parents of the basaltic achondrites. To escape, these smaller (about 4-7 km) asteroids had to be ejected at speeds greater than the escape velocity, v(sub esc) is approximately = 350 m/s. This evidence that large fragments were ejected at high speed from Vesta has not been reconciled with the present understanding of impact physics. Analytical spallation models predict that an impactor capable of ejecting these 'chips off Vesta' would be almost the size of Vesta! Such an impact would lead to the catastrophic disruption of both bodies. A simpler analysis is outlined, based on comparison with cratering on Mars, and it is shown that Vesta could survive an impact capable of ejecting kilometer-scale fragments at sufficient speed. To what extent does Vesta survive the formation of such a large crater? This is best addressed using a hydrocode such as SALE 2D with centroidal gravity to predict velocities subsequent to impact. The fragmentation outcome and velocity subsequent to the impact described to demonstrate that Vesta survives without large-scale disassembly or overturning of the crust. Vesta and its clan represent a valuable dataset for testing fragmentation hydrocodes such as SALE 2D and SPH 3D at planetary scales. Resolution required to directly model spallation 'chips' on a body 100 times as large is now marginally possible on modern workstations. These boundaries are important in near-surface ejection processes and in large-scale disruption leading to asteroid families and stripped cores.

COHERENT constraints to conventional and exotic neutrino physics

NASA Astrophysics Data System (ADS)

Papoulias, D. K.; Kosmas, T. S.

2018-02-01

The process of neutral-current coherent elastic neutrino-nucleus scattering, consistent with the Standard Model (SM) expectation, has been recently measured by the COHERENT experiment at the Spallation Neutron Source. On the basis of the observed signal and our nuclear calculations for the relevant Cs and I isotopes, the extracted constraints on both conventional and exotic neutrino physics are updated. The present study concentrates on various SM extensions involving vector and tensor nonstandard interactions as well as neutrino electromagnetic properties, with an emphasis on the neutrino magnetic moment and the neutrino charge radius. Furthermore, models addressing a light sterile neutrino state and scenarios with new propagator fields—such as vector Z' and scalar bosons—are examined, and the corresponding regions excluded by the COHERENT experiment are presented.

Note: Detector collimators for the nanoscale ordered materials diffractometer instrument at the Spallation Neutron Source

DOE Office of Scientific and Technical Information (OSTI.GOV)

Tamalonis, A.; Weber, J. K. R.; Neuefeind, J. C.

2015-09-01

Five neutron collimator designs were constructed and tested at the nanoscale ordered materials diffractometer (NOMAD) instrument. Collimators were made from High Density PolyEthylene (HDPE) or 5% borated HDPE. In all cases, collimators improved the signal to background ratio and reduced detection of secondary scattering. In the Q-range 10-20 (angstrom) -1, signal to background ratio improved by factors of approximately 1.6 and 2.0 for 50 and 100 mm deep collimators, respectively. In the Q-range 40-50 angstrom -1, the improvement factors were 1.8 and 2.7. Secondary scattering as measured at Q similar to 9.5 angstrom -1 was significantly decreased when the collimatorsmore » were installed.« less

The Particle Accelerator Simulation Code PyORBIT

DOE Office of Scientific and Technical Information (OSTI.GOV)

Gorlov, Timofey V; Holmes, Jeffrey A; Cousineau, Sarah M

2015-01-01

The particle accelerator simulation code PyORBIT is presented. The structure, implementation, history, parallel and simulation capabilities, and future development of the code are discussed. The PyORBIT code is a new implementation and extension of algorithms of the original ORBIT code that was developed for the Spallation Neutron Source accelerator at the Oak Ridge National Laboratory. The PyORBIT code has a two level structure. The upper level uses the Python programming language to control the flow of intensive calculations performed by the lower level code implemented in the C++ language. The parallel capabilities are based on MPI communications. The PyORBIT ismore » an open source code accessible to the public through the Google Open Source Projects Hosting service.« less

Single Crystal Diffuse Neutron Scattering

DOE PAGES

Welberry, Richard; Whitfield, Ross

2018-01-11

Diffuse neutron scattering has become a valuable tool for investigating local structure in materials ranging from organic molecular crystals containing only light atoms to piezo-ceramics that frequently contain heavy elements. Although neutron sources will never be able to compete with X-rays in terms of the available flux the special properties of neutrons, viz. the ability to explore inelastic scattering events, the fact that scattering lengths do not vary systematically with atomic number and their ability to scatter from magnetic moments, provides strong motivation for developing neutron diffuse scattering methods. Here, we compare three different instruments that have been used bymore » us to collect neutron diffuse scattering data. Two of these are on a spallation source and one on a reactor source.« less

Method of producing .sup.67 Cu

DOEpatents

O'Brien, Jr., Harold A.; Barnes, John W.; Taylor, Wayne A.; Thomas, Kenneth E.; Bentley, Glenn E.

1984-01-01

A method of producing carrier-free .sup.67 Cu by proton spallation combined with subsequent chemical separation and purification is disclosed. A target consisting essentially of pressed zinc oxide is irradiated with a high energy, high current proton beam to produce a variety of spallogenic nuclides, including .sup.67 Cu and other copper isotopes. The irradiated target is dissolved in a concentrated acid solution to which a palladium salt is added. In accordance with the preferred method, the spallogenic copper is twice coprecipitated with palladium, once with metallic zinc as the precipitating agent and once with hydrogen sulfide as the precipitating agent. The palladium/copper precipitate is then dissolved in an acid solution and the copper is separated from the palladium by liquid chromatography on an anion exchange resin.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Stone, Matthew B; Niedziela, Jennifer L; Abernathy, Douglas L

The Spallation Neutron Source at Oak Ridge National Laboratory now hosts four direct geometry time-of-flight chopper spectrometers. These instruments cover a range of wave vector and energy transfer space with varying degrees of neutron flux and resolution. The regions of reciprocal and energy space available to measure at these instruments is not exclusive and overlaps significantly. We present a direct comparison of the capabilities of this instrumentation, conducted by data mining the instrument usage histories, and specific scanning regimes. In addition, one of the common science missions for these instruments is the study of magnetic excitations in condensed matter systems.more » We have measured the powder averaged spin wave spectra in one particular sample using each of these instruments, and use these data in our comparisons.« less

DOE Office of Scientific and Technical Information (OSTI.GOV)

Stone, M. B.; Abernathy, D. L.; Ehlers, G.

The Spallation Neutron Source at Oak Ridge National Laboratory now hosts four direct geometry time-of-flight chopper spectrometers. These instruments cover a range of wave-vector and energy transfer space with varying degrees of neutron flux and resolution. The regions of reciprocal and energy space available to measure at these instruments are not exclusive and overlap significantly. We present a direct comparison of the capabilities of this instrumentation, conducted by data mining the instrument usage histories, and specific scanning regimes. In addition, one of the common science missions for these instruments is the study of magnetic excitations in condensed matter systems. Wemore » have measured the powder averaged spin wave spectra in one particular sample using each of these instruments, and use these data in our comparisons.« less

Hydrogen isotopes in lunar volcanic glasses and melt inclusions reveal a carbonaceous chondrite heritage.

PubMed

Saal, Alberto E; Hauri, Erik H; Van Orman, James A; Rutherford, Malcolm J

2013-06-14

Water is perhaps the most important molecule in the solar system, and determining its origin and distribution in planetary interiors has important implications for understanding the evolution of planetary bodies. Here we report in situ measurements of the isotopic composition of hydrogen dissolved in primitive volcanic glass and olivine-hosted melt inclusions recovered from the Moon by the Apollo 15 and 17 missions. After consideration of cosmic-ray spallation and degassing processes, our results demonstrate that lunar magmatic water has an isotopic composition that is indistinguishable from that of the bulk water in carbonaceous chondrites and similar to that of terrestrial water, implying a common origin for the water contained in the interiors of Earth and the Moon.

An energy-dependent numerical model for the condensation probability, γ j

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kerby, Leslie Marie

The “condensation” probability, γ j, is an important variable in the preequilibrium stage of nuclear spallation reactions. It represents the probability that p j excited nucleons (excitons) will “condense” to form complex particle type j in the excited residual nucleus. In addition, it has a significant impact on the emission width, or probability of emitting fragment type j from the residual nucleus. Previous formulations for γ j were energy-independent and valid for fragments up to 4He only. This paper explores the formulation of a new model for γ j, one which is energy-dependent and valid for up to 28Mg, andmore » which provides improved fits compared to experimental fragment spectra.« less

A compact 10 kW solid-state RF power amplifier at 352 MHz

NASA Astrophysics Data System (ADS)

Dancila, Dragos; Hoang Duc, Long; Jobs, Magnus; Holmberg, Måns; Hjort, Adam; Rydberg, Anders; Ruber, Roger

2017-07-01

A compact 10 kW RF power amplifier at 352 MHz was developed at FREIA for the European Spallation Source, ESS. The specifications of ESS for the conception of amplifiers are related to its pulsed operation: 3.5 ms pulse length and a duty cycle of 5%. The realized amplifier is composed of eight kilowatt level modules, combined using a planar Gysel 8-way combiner. The combiner has a low insertion loss of only 0.2 dB, measured at 10 kW peak power. Each module is built around a commercially available LDMOS transistor in a singleended architecture. During the final tests, a total output peak power of 10.5 kW was measured.

The compensation of quadrupole errors and space charge effects by using trim quadrupoles

NASA Astrophysics Data System (ADS)

An, YuWen; Wang, Sheng

2011-12-01

The China Spallation Neutron Source (CSNS) accelerators consist of an H-linac and a proton Rapid Cycling Synchrotron (RCS). RCS is designed to accumulate and accelerate proton beam from 80 MeV to 1.6 GeV with a repetition rate of 25 Hz. The main dipole and quadruple magnet will operate in AC mode. Due to the adoption of the resonant power supplies, saturation errors of magnetic field cannot be compensated by power supplies. These saturation errors will disturb the linear optics parameters, such as tunes, beta function and dispersion function. The strong space charge effects will cause emittance growth. The compensation of these effects by using trim quadruples is studied, and the corresponding results are presented.

Cryogenic magnetic coil and superconducting magnetic shield for neutron electric dipole moment searches

NASA Astrophysics Data System (ADS)

Slutsky, S.; Swank, C. M.; Biswas, A.; Carr, R.; Escribano, J.; Filippone, B. W.; Griffith, W. C.; Mendenhall, M.; Nouri, N.; Osthelder, C.; Pérez Galván, A.; Picker, R.; Plaster, B.

2017-08-01

A magnetic coil operated at cryogenic temperatures is used to produce spatial, relative field gradients below 6 ppm/cm, stable for several hours. The apparatus is a prototype of the magnetic components for a neutron electric dipole moment (nEDM) search, which will take place at the Spallation Neutron Source (SNS) at Oak Ridge National Laboratory using ultra-cold neutrons (UCN). That search requires a uniform magnetic field to mitigate systematic effects and obtain long polarization lifetimes for neutron spin precession measurements. This paper details upgrades to a previously described apparatus [1], particularly the introduction of super-conducting magnetic shielding and the associated cryogenic apparatus. The magnetic gradients observed are sufficiently low for the nEDM search at SNS.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Drouhard, Margaret MEG G; Steed, Chad A; Hahn, Steven E

In this paper, we propose strategies and objectives for immersive data visualization with applications in materials science using the Oculus Rift virtual reality headset. We provide background on currently available analysis tools for neutron scattering data and other large-scale materials science projects. In the context of the current challenges facing scientists, we discuss immersive virtual reality visualization as a potentially powerful solution. We introduce a prototype immersive visual- ization system, developed in conjunction with materials scientists at the Spallation Neutron Source, which we have used to explore large crystal structures and neutron scattering data. Finally, we offer our perspective onmore » the greatest challenges that must be addressed to build effective and intuitive virtual reality analysis tools that will be useful for scientists in a wide range of fields.« less

Commissioning and First Results of the Electron Beam Profiler in the Main Injector at Fermilab

DOE Office of Scientific and Technical Information (OSTI.GOV)

Thurman-Keup, R.; Alvarez, M.; Fitzgerald, J.

2017-08-01

The planned neutrino program at Fermilab requires large proton beam intensities in excess of 2 MW. Measuring the transverse profiles of these high intensity beams is challenging and often depends on non-invasive techniques. One such technique involves measuring the deflection of a probe beam of electrons with a trajectory perpendicular to the proton beam. A device such as this is already in use at the Spallation Neutron Source at ORNL and a similar device has been installed in the Main Injector at Fermilab. Commissioning of the device is in progress with the goal of having it operational by the endmore » of the year. The status of the commissioning and initial results will be presented« less

Accelerator boom hones China's engineering expertise

NASA Astrophysics Data System (ADS)

Normile, Dennis

2018-02-01

In raising the curtain on the China Spallation Neutron Source, China has joined just four other nations in having mastered the technology of accelerating and controlling beams of protons. The $277 million facility, set to open to users this spring in Dongguan, is expected to yield big dividends in materials science, chemistry, and biology. More world class machines are on the way, as China this year starts construction on four other major accelerator facilities. The building boom is prompting a scramble to find enough engineers and technicians to finish the projects. But if they all come off as planned, the facilities would position China to tackle the next global megaproject: a giant accelerator that would pick up where Europe's Large Hadron Collider leaves off.

Oxygen diffusion barrier coating

NASA Technical Reports Server (NTRS)

Unnam, Jalaiah (Inventor); Clark, Ronald K. (Inventor)

1987-01-01

A method for coating a titanium panel or foil with aluminum and amorphous silicon to provide an oxygen barrier abrogating oxidation of the substrate metal is developed. The process is accomplished with known inexpensive procedures common in materials research laboratories, i.e., electron beam deposition and sputtering. The procedures are conductive to treating foil gage titanium and result in submicron layers which virtually add no weight to the titanium. There are no costly heating steps. The coatings blend with the substrate titanium until separate mechanical properties are subsumed by those of the substrate without cracking or spallation. This method appreciably increases the ability of titanium to mechanically perform in high thermal environments such as those witnessed on structures of space vehicles during re-entry

An energy-dependent numerical model for the condensation probability, γ j

DOE PAGES

Kerby, Leslie Marie

2016-12-09

The “condensation” probability, γ j, is an important variable in the preequilibrium stage of nuclear spallation reactions. It represents the probability that p j excited nucleons (excitons) will “condense” to form complex particle type j in the excited residual nucleus. In addition, it has a significant impact on the emission width, or probability of emitting fragment type j from the residual nucleus. Previous formulations for γ j were energy-independent and valid for fragments up to 4He only. This paper explores the formulation of a new model for γ j, one which is energy-dependent and valid for up to 28Mg, andmore » which provides improved fits compared to experimental fragment spectra.« less

Nuclear data for medical applications: An overview of present status and future needs

NASA Astrophysics Data System (ADS)

Syed, M. Qaim

2017-09-01

A brief overview of nuclear data required for medical applications is given. The major emphasis is on radionuclides for internal applications, both for diagnosis and therapy. The status of the presently available data is discussed and some of the emerging needs are outlined. Most of the needs are associated with the development of non-standard positron emitters and novel therapeutic radionuclides. Some new developments in application of radionuclides, e.g. theranostic approach, multimode imaging, radionanoparticles, etc. are described and the related nuclear data needs are discussed. The possible use of newer irradiation technologies for medical radionuclide production, e.g. intermediate energy charged-particle accelerators, high-power electron accelerators for photon production, and spallation neutron sources, will place heavy demands on nuclear data.

Ignition and monitoring technique for plasma processing of multicell superconducting radio-frequency cavities

DOE Office of Scientific and Technical Information (OSTI.GOV)

Doleans, Marc

In this study, an in-situ plasma processing technique has been developed at the Spallation Neutron Source (SNS) to improve the performance of the superconducting radio-frequency (SRF) cavities in operation. The technique uses a low-density reactive neon-oxygen plasma at room-temperature to improve the surface work function, to help remove adsorbed gases on the RF surface and to reduce its secondary emission yield. SNS SRF cavities are six-cell elliptical cavities and the plasma typically ignites in the cell where the electric field is the highest. This article will detail a technique that was developed to ignite and monitor the plasma in eachmore » cell of the SNS cavities.« less

Transverse beam stability measurement and analysis for the SNS accumulator ring

DOE PAGES

Xie, Zaipeng; Deibele, Craig; Schulte, Michael J.; ...

2015-07-01

In a Field-programmable gate array (FPGA) based transverse feedback damper system we implemented in the Spallation Neutron Source (SNS) accumulator ring with the intention to stabilize the electron-proton (e-p) instability in a frequency range from 1 MHz to 300 MHz. The transverse damper could also be used as a diagnostic tool by measuring the beam transfer function (BTF). An analysis of the BTF measurement provides the stability diagram for the production beam at SNS. Our paper describes the feedback damper system and its set-up as the BTF diagnostic tool. Experimental BTF results are presented and beam stability analysis is performedmore » based on the BTF measurements for the SNS accumulator ring.« less

Status of the DOE/NASA critical gas turbine research and technology project

NASA Technical Reports Server (NTRS)

Clark, J. S.

1980-01-01

Activities performed in order to provide an R&T data base for utility gas turbine systems burning coal-derived fuels are described. Experiments were run to determine the corrosivity effects of trace metal contaminants (and potential fuel additives) on gas turbine materials and these results were correlated in a corrosion-life prediction model. Actual fuels were burned in a burner rig hot corrosion test to verify the model. A deposition prediction model was assembled and compared with results of actual coal-derived fuel deposition tests. Thermal barrier coatings were tested to determine their potential for protecting gas turbine hardware from the corrosive contaminants. Several coatings were identified with significantly improved spallation-resistance (and, hence, corrosion resistance).

A history of neutrons in biology: the development of neutron protein crystallography at BNL and LANL.

PubMed

Schoenborn, Benno P

2010-11-01

The first neutron diffraction data were collected from crystals of myoglobin almost 42 years ago using a step-scan diffractometer with a single detector. Since then, major advances have been made in neutron sources, instrumentation and data collection and analysis, and in biochemistry. Fundamental discoveries about enzyme mechanisms, biological complex structures, protein hydration and H-atom positions have been and continue to be made using neutron diffraction. The promise of neutrons has not changed since the first crystal diffraction data were collected. Today, with the developments of beamlines at spallation neutron sources and the use of the Laue method for data collection, the field of neutrons in structural biology has renewed vitality.

Energy Production and Transmutation of Nuclear Waste by Accelerator Driven Systems

NASA Astrophysics Data System (ADS)

Zhivkov, P. K.

2018-05-01

There is a significant amount of highly radiotoxic long-life nuclear waste (NW) produced by NPP (Nuclear Power Plants). Transmutation is a process which transforms NW into less radiotoxic nuclides with a shorter period of half-life by spallation neutrons or radiative capture of neutrons produced by ADS (Accelerator Driven System). In the processes of transmutation new radioactive nuclides are produced. ADS is big energy consumer equipment. It is a method for production of a high-flux and high-energy neutron field. All these processes occur in ADS simultaneously. ADS is able to transmute actinides and produce energy simultaneously. The article considers the energy production problems in ADS. Several ideas are developed regarding the solution of the global energy supply.

Modeling spallation reactions in tungsten and uranium targets with the Geant4 toolkit

NASA Astrophysics Data System (ADS)

Malyshkin, Yury; Pshenichnov, Igor; Mishustin, Igor; Greiner, Walter

2012-02-01

We study primary and secondary reactions induced by 600 MeV proton beams in monolithic cylindrical targets made of natural tungsten and uranium by using Monte Carlo simulations with the Geant4 toolkit [1-3]. Bertini intranuclear cascade model, Binary cascade model and IntraNuclear Cascade Liège (INCL) with ABLA model [4] were used as calculational options to describe nuclear reactions. Fission cross sections, neutron multiplicity and mass distributions of fragments for 238U fission induced by 25.6 and 62.9 MeV protons are calculated and compared to recent experimental data [5]. Time distributions of neutron leakage from the targets and heat depositions are calculated. This project is supported by Siemens Corporate Technology.

Note: Detector collimators for the nanoscale ordered materials diffractometer instrument at the Spallation Neutron Source

DOE PAGES

Tamalonis, A.; Weber, J. K. R.; Neuefeind, J. C.; ...

2015-09-09

We constructed and tested five neutron collimator designs using the nanoscale ordered materials diffractometer (NOMAD) instrument. Collimators were made from High Density PolyEthylene (HDPE) or 5% borated HDPE. In all cases, collimators improved the signal to background ratio and reduced detection of secondary scattering. Moreover, in the Q-range 10-20 Å -1, signal to background ratio improved by factors of approximately 1.6 and 2.0 for 50 and 100 mm deep collimators, respectively. In the Q-range 40-50 Å -1, the improvement factors were 1.8 and 2.7. Secondary scattering as measured at Q similar to 9.5 Å -1 was significantly decreased when themore » collimators were installed.« less

Fabrication of Nanosized Lanthanum Zirconate Powder and Deposition of Thermal Barrier Coating by Plasma Spray Process

NASA Astrophysics Data System (ADS)

Mishra, S. K.; Jagdeesh, N.; Pathak, L. C.

2016-07-01

The present manuscript discusses our findings on fabrication of nanosized lanthanum zirconate powder for thermal barrier coating application and its coating by plasma spray on nickel-based superalloy substrate. Single-phase La2Zr2O7 coating of thickness of the order of 45 µm on the Ni-Cr-Al bond coat coated Ni-based superalloy substrate was deposited by plasma spray process. The layers at the interface did not show spallation and inter diffusion was very less. The microstructure, interface, porosity, and mechanical properties of different layers are investigated. The lanthanum zirconate hardness and modulus were 10.5 and 277 GPa, respectively. The load depth curve for lanthanum zirconate showed good elastic recovery around 74%.

Magnetic fringe field interference between the quadrupole and corrector magnets in the CSNS/RCS

NASA Astrophysics Data System (ADS)

Yang, Mei; Kang, Wen; Deng, Changdong; Sun, Xianjing; Li, Li; Wu, Xi; Gong, Lingling; Cheng, Da; Zhu, Yingshun; Chen, Fusan

2017-03-01

The Rapid Cycling Synchrotron (RCS) of the China Spallation Neutron Source (CSNS) employs large aperture quadrupole and corrector magnets with small aspect ratios and relatively short iron to iron separations; so the fringe field interference becomes serious which results in integral field strength reduction and extra field harmonics. We have performed 3D magnetic field simulations to investigate the magnetic field interference in the magnet assemblies and made some adjustments on the magnet arrangement. The Fourier analysis is used to quantify the integral gradient reduction and field harmonic changes of the quadrupole magnets. Some magnetic field measurements are undertaken to verify the simulation results. The simulation details and the major results are presented in this paper.

Single Crystal Diffuse Neutron Scattering

DOE Office of Scientific and Technical Information (OSTI.GOV)

Welberry, Richard; Whitfield, Ross

Diffuse neutron scattering has become a valuable tool for investigating local structure in materials ranging from organic molecular crystals containing only light atoms to piezo-ceramics that frequently contain heavy elements. Although neutron sources will never be able to compete with X-rays in terms of the available flux the special properties of neutrons, viz. the ability to explore inelastic scattering events, the fact that scattering lengths do not vary systematically with atomic number and their ability to scatter from magnetic moments, provides strong motivation for developing neutron diffuse scattering methods. Here, we compare three different instruments that have been used bymore » us to collect neutron diffuse scattering data. Two of these are on a spallation source and one on a reactor source.« less

SNS proton power upgrade

NASA Astrophysics Data System (ADS)

Howell, M.; DeGraff, B.; Galambos, J.; Kim, S.-H.

2017-12-01

The Spallation Neutron Source (SNS) at Oak Ridge National Laboratory (ORNL) is preparing for the Proton Power Upgrade (PPU) project to increase the output energy of the accelerator from 1.0 GeV to 1.3 GeV. As part of this project with the combination of increasing the output energy and beam current, the beam power capability will be doubled from 1.4MW to 2.8MW. In this project, seven new high beta cryomodules housing 28 superconducting niobium cavities will be added to the LINAC tunnel. Lessons learned from over ten years of operation will be incorporated into the new cryomodule and cavity design. The design and the fabrication of these cryomodules and how these will be integrated into the existing accelerator will be detailed in this paper.

Method for producing /sup 67/Cu

DOEpatents

O'Brien, H.A. Jr.; Barnes, J.W.; Taylor, W.A.; Thomas, K.E.; Bentley, G.E.

A method of producing carrier-free /sup 67/Cu by proton spallation combined with subsequent chemical separation and purification is disclosed. A target consisting essentially of pressed zinc oxide is irradiated with a high energy, high current proton beam to produce a variety of spallogenic nuclides, including /sup 67/Cu and other copper isotopes. The irradiated target is dissolved in a concentrated acid solution to which a palladium salt is added. In accordance with the preferred method, the spallogenic copper is twice coprecipitated with palladium, once with metallic zinc as the precipitating agent and once with hydrogen sulfide as the precipitating agent. The palladium/copper precipitate is then dissolved in an acid solution and the copper is separated from the palladium by liquid chromatography on an anion exchange resin.

Cosmogenically-produced isotopes in natural and enriched high-purity germanium detectors for the MAJORANA DEMONSTRATOR

NASA Astrophysics Data System (ADS)

Gilliss, Thomas; MAJORANA DEMONSTRATOR Collaboration

2017-01-01

The MAJORANA DEMONSTRATOR advances toward measurements of the neutrinoless double-beta decay of 76Ge. Detectors employed in the DEMONSTRATOR are subject to cosmogenic spallation during production and processing, resulting in activation of certain long-lived radioisotopes. Activation of these cosmogenic isotopes is mitigated by shielded storage of detectors and through underground operation of the DEMONSTRATOR at the 4850 ft level of the Sanford Underground Research Facility. In this work, we explore the appearance and reduction of cosmogenic contributions to the DEMONSTRATOR background spectrum. This work is supported by the U.S. Department of Energy, Office of Science, Office of Nuclear Physics, the Particle Astrophysics and Nuclear Physics Programs of the National Science Foundation, and the Sanford Underground Research Facility.

SNS Central Helium Liquefier spare Carbon Bed installation and commissioning

DOE Office of Scientific and Technical Information (OSTI.GOV)

Degraff, Brian D.; Howell, Matthew P.; Kim, Sang-Ho

The Spallation Neutron Source (SNS) Central Helium Liquefier (CHL) at Oak Ridge National Laboratory (ORNL) has been without major operations downtime since operations were started back in 2006. This system utilizes a vessel filled with activated carbon as the final major component to remove oil vapor from the compressed helium circuit prior to insertion into the system's cryogenic cold box. The need for a spare carbon bed at SNS due to the variability of carbon media lifetime calculation to adsorption efficiency will be discussed. The fabrication, installation and commissioning of this spare carbon vessel will be presented. The novel planmore » for connecting the spare carbon vessel piping to the existing infrastructure will be presented.« less

Ignition and monitoring technique for plasma processing of multicell superconducting radio-frequency cavities

DOE PAGES

Doleans, Marc

2016-12-27

In this study, an in-situ plasma processing technique has been developed at the Spallation Neutron Source (SNS) to improve the performance of the superconducting radio-frequency (SRF) cavities in operation. The technique uses a low-density reactive neon-oxygen plasma at room-temperature to improve the surface work function, to help remove adsorbed gases on the RF surface and to reduce its secondary emission yield. SNS SRF cavities are six-cell elliptical cavities and the plasma typically ignites in the cell where the electric field is the highest. This article will detail a technique that was developed to ignite and monitor the plasma in eachmore » cell of the SNS cavities.« less

Neutron capture cross section measurement of 151Sm at the CERN neutron time of flight facility (n_TOF).

PubMed

Abbondanno, U; Aerts, G; Alvarez-Velarde, F; Alvarez-Pol, H; Andriamonje, S; Andrzejewski, J; Badurek, G; Baumann, P; Becvár, F; Benlliure, J; Berthoumieux, E; Calviño, F; Cano-Ott, D; Capote, R; Cennini, P; Chepel, V; Chiaveri, E; Colonna, N; Cortes, G; Cortina, D; Couture, A; Cox, J; Dababneh, S; Dahlfors, M; David, S; Dolfini, R; Domingo-Pardo, C; Duran, I; Embid-Segura, M; Ferrant, L; Ferrari, A; Ferreira-Marques, R; Frais-Koelbl, H; Furman, W; Goncalves, I; Gallino, R; Gonzalez-Romero, E; Goverdovski, A; Gramegna, F; Griesmayer, E; Gunsing, F; Haas, B; Haight, R; Heil, M; Herrera-Martinez, A; Isaev, S; Jericha, E; Käppeler, F; Kadi, Y; Karadimos, D; Kerveno, M; Ketlerov, V; Koehler, P; Konovalov, V; Krticka, M; Lamboudis, C; Leeb, H; Lindote, A; Lopes, I; Lozano, M; Lukic, S; Marganiec, J; Marrone, S; Martinez-Val, J; Mastinu, P; Mengoni, A; Milazzo, P M; Molina-Coballes, A; Moreau, C; Mosconi, M; Neves, F; Oberhummer, H; O'Brien, S; Pancin, J; Papaevangelou, T; Paradela, C; Pavlik, A; Pavlopoulos, P; Perlado, J M; Perrot, L; Pignatari, M; Plag, R; Plompen, A; Plukis, A; Poch, A; Policarpo, A; Pretel, C; Quesada, J; Raman, S; Rapp, W; Rauscher, T; Reifarth, R; Rosetti, M; Rubbia, C; Rudolf, G; Rullhusen, P; Salgado, J; Soares, J C; Stephan, C; Tagliente, G; Tain, J; Tassan-Got, L; Tavora, L; Terlizzi, R; Vannini, G; Vaz, P; Ventura, A; Villamarin, D; Vincente, M C; Vlachoudis, V; Voss, F; Wendler, H; Wiescher, M; Wisshak, K

2004-10-15

The151Sm(n,gamma)152Sm cross section has been measured at the spallation neutron facility n_TOF at CERN in the energy range from 1 eV to 1 MeV. The new facility combines excellent resolution in neutron time-of-flight, low repetition rates, and an unsurpassed instantaneous luminosity, resulting in rather favorable signal/background ratios. The 151Sm cross section is of importance for characterizing neutron capture nucleosynthesis in asymptotic giant branch stars. At a thermal energy of kT=30 keV the Maxwellian averaged cross section of this unstable isotope (t(1/2)=93 yr) was determined to be 3100+/-160 mb, significantly larger than theoretical predictions.

Nitrogen isotopic signatures in the Acapulco meteorite

NASA Technical Reports Server (NTRS)

Sturgeon, G.; Marti, K.

1991-01-01

N isotopic abundances are reported for a bulk sample of the unique meteorite Acapulco. Although the mineral chemistry indicates a high degree of recrystallization under redox conditions between those of H and E chondrites (Palme et al., 1981), the presence of two distinct N isotopic signatures shows that the carriers of these N components were not equilibrated. In stepwise pyrolysis, the larger (65 percent) N component is released mostly below 1000 C and reveals a signature of delta(N-15) = 8.9 + or - 1.2 per mil, which is within the range observed in chondrites. A second 'light' component appears above 1000 C and has a signature of delta(N-15) less than or equal to -110.5 + or - 4.0 per mil (uncorrected for spallation N-15).

Theoretical study of a dual harmonic system and its application to the CSNS/RCS

NASA Astrophysics Data System (ADS)

Yuan, Yao-Shuo; Wang, Na; Xu, Shou-Yan; Yuan, Yue; Wang, Sheng

2015-12-01

Dual harmonic systems have been widely used in high intensity proton synchrotrons to suppress the space charge effect, as well as reduce the beam loss. To investigate the longitudinal beam dynamics in a dual rf system, the potential well, the sub-buckets in the bunch and the multi-solutions of the phase equation are studied theoretically in this paper. Based on these theoretical studies, optimization of bunching factor and rf voltage waveform are made for the dual harmonic rf system in the upgrade phase of the China Spallation Neutron Source Rapid Cycling Synchrotron (CSNS/RCS). In the optimization process, the simulation with space charge effect is done using a newly developed code, C-SCSIM. Supported by National Natural Science Foundation of China (11175193)

Beam diagnostics at high-intensity storage rings

NASA Astrophysics Data System (ADS)

Plum, Mike

1994-10-01

Beam diagnostics at high-intensity facilities feature their own special set of problems and characteristics, issues peculiar to high-intensity storage rings include beam loss, beam halos, extraction efficiency, beam in the gap, clearing electrodes, and beam-profile measurement. The Los Alamos Proton Storage Ring (PSR) is a nice example of a high-intensity storage ring. I will discuss in some detail three diagnostic systems currently in use at the PSR: the beam-loss-monitor system, the electron-clearing system, and the beam-in-the-gap monitor. Much of our discussion is inspired by the problems we have encountered and the useful things we have learned while commissioning and developing the PSR. Another inspiration is our work on the next-generation neutron-spallation source, also known as the National Center for Neutron Research (NCNR).

Liquid lithium target as a high intensity, high energy neutron source

DOEpatents

Parkin, Don M.; Dudey, Norman D.

1976-01-01

This invention provides a target jet for charged particles. In one embodiment the charged particles are high energy deuterons that bombard the target jet to produce high intensity, high energy neutrons. To this end, deuterons in a vacuum container bombard an endlessly circulating, free-falling, sheet-shaped, copiously flowing, liquid lithium jet that gushes by gravity from a rectangular cross-section vent on the inside of the container means to form a moving web in contact with the inside wall of the vacuum container. The neutrons are produced via break-up of the beam in the target by stripping, spallation and compound nuclear reactions in which the projectiles (deuterons) interact with the target (Li) to produce excited nuclei, which then "boil off" or evaporate a neutron.

Observations of the Li, Be, and B Isotopes and Constraints on Cosmic-ray Propagation

NASA Technical Reports Server (NTRS)

deNolfo, G. A.; Moskalenko, I. V.; Binns, W. R.; Christian, E. R.; Cummings, A. C.; Davis, A. J.; George, J. S.; Hink, P. L.; Israel, M. H.; Leske, R. A.;

Correlation of Upper-Atmospheric 7-Be with Solar Energetic Particle Events

NASA Technical Reports Server (NTRS)

Phillips, G. W.; Share, G. H.; King, S. E.; August, R. A.; Tylka, A. J.; Adams, J. H., Jr.; Panasyuk, M. I.; Nymmik, R. A.; Kuzhevskij, B. M.; Kulikauskas, V. S.;

Correlated topographic and structural modification on Si surface during multi-shot femtosecond laser exposures: Si nanopolymorphs as potential local structural nanomarkers

NASA Astrophysics Data System (ADS)

Ionin, A. A.; Kudryashov, S. I.; Levchenko, A. O.; Nguyen, L. V.; Saraeva, I. N.; Rudenko, A. A.; Ageev, E. I.; Potorochin, D. V.; Veiko, V. P.; Borisov, E. V.; Pankin, D. V.; Kirilenko, D. A.; Brunkov, P. N.

2017-09-01

High-pressure Si-XII and Si-III nanocrystalline polymorphs, as well as amorphous Si phase, appear consequently during multi-shot femtosecond-laser exposure of crystalline Si wafer surface above its spallation threshold along with permanently developing quasi-regular surface texture (ripples, microcones), residual hydrostatic stresses and subsurface damage, which are characterized by scanning and transmission electron microscopy, as well as by Raman micro-spectroscopy. The consequent yields of these structural Si phases indicate not only their spatially different appearance, but also potentially enable to track nanoscale, transient laser-induced high-pressure, high-temperature physical processes - local variation of ablation mechanism and rate, pressurization/pressure release, melting/resolidification, amorphization, annealing - versus cumulative laser exposure and the related development of the surface topography.

Investigations of lunar materials

NASA Technical Reports Server (NTRS)

Comstock, G. M.; Fvwaraye, A. O.; Fleischer, R. L.; Hart, H. R., Jr.

1972-01-01

The investigations were directed at determining the radiation history and surface chronology of lunar materials using the etched particle track technique. The major lunar materials studied are the igneous rocks and double core from Apollo 12, the breccia and soil samples from Apollo 14, and the core samples from Luna 16. In the course of this work two new and potentially important observations were made: (1) Cosmic ray-induced spallation-recoil tracks were identified. The density of such tracks, when compared with the density of tracks induced by a known flux of accelerator protons, yields the time of exposure of a sample within the top meter or two of moon's surface. (2) Natural, fine scale plastic deformation was found to have fragmented pre-existing charged particle tracks, allowing the dating of the mechanical event causing the deformation.

Experimental demonstration of a compact epithermal neutron source based on a high power laser

NASA Astrophysics Data System (ADS)

Mirfayzi, S. R.; Alejo, A.; Ahmed, H.; Raspino, D.; Ansell, S.; Wilson, L. A.; Armstrong, C.; Butler, N. M. H.; Clarke, R. J.; Higginson, A.; Kelleher, J.; Murphy, C. D.; Notley, M.; Rusby, D. R.; Schooneveld, E.; Borghesi, M.; McKenna, P.; Rhodes, N. J.; Neely, D.; Brenner, C. M.; Kar, S.

2017-07-01

Epithermal neutrons from pulsed-spallation sources have revolutionised neutron science allowing scientists to acquire new insight into the structure and properties of matter. Here, we demonstrate that laser driven fast (˜MeV) neutrons can be efficiently moderated to epithermal energies with intrinsically short burst durations. In a proof-of-principle experiment using a 100 TW laser, a significant epithermal neutron flux of the order of 105 n/sr/pulse in the energy range of 0.5-300 eV was measured, produced by a compact moderator deployed downstream of the laser-driven fast neutron source. The moderator used in the campaign was specifically designed, by the help of MCNPX simulations, for an efficient and directional moderation of the fast neutron spectrum produced by a laser driven source.

Fiber Optic Picosecond Laser Pulse Transmission Line for Hydrogen Ion Beam Profile Measurement

DOE Office of Scientific and Technical Information (OSTI.GOV)

Liu, Yun; Huang, Chunning; Aleksandrov, Alexander V

2013-01-01

We present a fiber optic laser pulse transmission line for non-intrusive longitudinal profile measurement of the hydrogen ion (H-) beam at the front-end of the Spallation Neutron Source (SNS) accelerator. The 80.5 MHz, 2.5 ps, multi-killowatt optical pulses are delivered to the accelerator beam line through a large mode area polarization maintaining optical fiber to ensure a high measurement stability. The transmission efficiency, output laser beam quality, pulse jitter and pulse width broadening over a 100-ft fiber line are experimentally investigated. A successful measurement of the H- beam microbunch (~130 ps) profile is obtained. Our experiment is the first demonstrationmore » of particle beam profile diagnostics using fiber optic laser pulse transmission line.« less

The O H stretching band in ice Ih derived via eV neutron spectroscopy on VESUVIO using the new very low angle detector bank

NASA Astrophysics Data System (ADS)

Perelli-Cippo, E.; Gorini, G.; Tardocchi, M.; Andreani, C.; Pietropaolo, A.; Senesi, R.; Rhodes, N. J.; Schooneveld, E. M.

2006-06-01

Strong demand exists for an experimental facility enabling new experimental investigations on condensed matter systems based on epithermal neutron scattering at high energy and low momentum transfers. This need will be met by the very low angle detector (VLAD) bank, to be installed on the VESUVIO spectrometer at the ISIS spallation neutron source. The equipment will operate in the scattering angular range 1°<2θ<5°. Scattering measurements from a polycrystalline ice sample using a VLAD prototype demonstrates the effectiveness of the detection technique adopted for the construction of the full detector array. The resulting density of states in ice is 9±2 atoms/cell, in agreement with previous measurements.

H(-) ion source developments at the SNS.

PubMed

Welton, R F; Stockli, M P; Murray, S N; Pennisi, T R; Han, B; Kang, Y; Goulding, R H; Crisp, D W; Sparks, D O; Luciano, N P; Carmichael, J R; Carr, J

2008-02-01

The U.S. Spallation Neutron Source (SNS) will require substantially higher average and pulse H(-) beam currents than can be produced from conventional ion sources such as the base line SNS source. H(-) currents of 40-50 mA (SNS operations) and 70-100 mA (power upgrade project) with a rms emittance of 0.20-0.35pi mm mrad and a approximately 7% duty factor will be needed. We are therefore investigating several advanced ion source concepts based on rf plasma excitation. First, the performance characteristics of an external antenna source based on an Al(2)O(3) plasma chamber combined with an external multicusp magnetic configuration, an elemental Cs system, and plasma gun will be discussed. Second, the first plasma measurements of a helicon-driven H(-) ion source will also be presented.

A Deterministic Interfacial Cyclic Oxidation Spalling Model. Part 1; Model Development and Parametric Response

NASA Technical Reports Server (NTRS)

Smialek, James L.

2002-01-01

An equation has been developed to model the iterative scale growth and spalling process that occurs during cyclic oxidation of high temperature materials. Parabolic scale growth and spalling of a constant surface area fraction have been assumed. Interfacial spallation of the only the thickest segments was also postulated. This simplicity allowed for representation by a simple deterministic summation series. Inputs are the parabolic growth rate constant, the spall area fraction, oxide stoichiometry, and cycle duration. Outputs include the net weight change behavior, as well as the total amount of oxygen and metal consumed, the total amount of oxide spalled, and the mass fraction of oxide spalled. The outputs all follow typical well-behaved trends with the inputs and are in good agreement with previous interfacial models.

The abundance of boron in three halo stars

NASA Technical Reports Server (NTRS)

Duncan, Douglas K.; Lambert, David L.; Lemke, Michael

1992-01-01

B abundances for three halo stars: HD 140283, HD 19445, and HD 201891 are presented. Using recent determinations of the Be abundance in HD 140283, B/Be of 10 +5/-4 is found for this star, and similar ratios are inferred for HD 19445 and HD 201891. This ratio is equal to the minimum value of 10 expected from a synthesis of B and Be by high-energy cosmic-ray spallation reactions in the interstellar medium. It is shown that the accompanying synthesis of Li by alpha on alpha fusion reactions is probably a minor contributor to the observed 'primordial' Li of halo stars. The observed constant ratios of B/O and Be/O are expected if the principal channel of synthesis involves cosmic-ray CNO nuclei from the supernovae colliding with interstellar protons.

The Los ALamos Neutron Science Center Hydrogen Moderator System

NASA Astrophysics Data System (ADS)

Jarmer, J. J.; Knudson, J. N.

2006-04-01

At the Los Alamos Neutron Science Center (LANSCE), spallation neutrons are produced by an 800-MeV proton beam interacting with tungsten targets. Gun-barrel-type penetrations through the heavy concrete and steel shielding that surround the targets collimate neutrons to form neutron beams used for scattering experiments. Two liquid hydrogen moderators of one-liter volume each are positioned adjacent to the neutron-production targets. Some of the neutrons that pass through a moderator interact with or scatter from protons in the hydrogen. The neutron-proton interaction reduces the energy or moderates neutrons to lower energies. Lower energy "moderated" neutrons are the most useful for some neutron scattering experiments. We provide a description of the LANSCE hydrogen-moderator system and its cryogenic performance with proton beams of up to 125 micro-amp average current.

Thermal neutron radiative capture on cadmium as a counting technique at the INES beam line at ISIS: A preliminary investigation of detector cross-talk.

PubMed

Festa, G; Grazzi, F; Pietropaolo, A; Scherillo, A; Schooneveld, E M

2017-12-01

Experimental tests are presented that assess the cross-talk level among three scintillation detectors used as neutron counters exploiting the thermal neutron radiative capture on Cd. The measurements were done at the INES diffractometer operating at the ISIS spallation neutron source (Rutherford Appleton Laboratory, UK). These tests follow a preliminary set of measurements performed on the same instrument to study the effectiveness of this thermal neutron counting strategy in neutron diffraction measurements, typically performed on INES using squashed 3 He filled gas tubes. The experimental data were collected in two different geometrical configurations of the detectors and compared to results of Monte Carlo simulations, performed using the MCNP code. Copyright © 2017 Elsevier Ltd. All rights reserved.

Cosmogenic radionuclides in stone meteorites

NASA Technical Reports Server (NTRS)

Cressy, P. J., Jr.

1976-01-01

This document presents the techniques and compilation of results of cosmogenic Al-26 measurements at Goddard Space Flight Center on 91 samples of 76 stone meteorites. Short-lived radionuclides, including Na-22, Sc-46, Mn-54, and Co-60, were measured in 13 of these meteorites. About one-third of these data has not previously been published. The results are discussed briefly in terms of (1) depletion of Al-26 and natural potassium due to weathering, (2) possible exposure of several chondrites to an unusually high cosmic-ray flux, (3) comparison of Al-26, Na-22, Sc-46, and Mn5-54 in chondrites with the spallation Ne-22/Ne-21 ratio as a shielding indicator, and (4) comparison of (Al-26)-(Ne-22)/Ne-21 data for achondrite classes with the chondrite trend.

H- ion source developments at the SNSa)

NASA Astrophysics Data System (ADS)

Welton, R. F.; Stockli, M. P.; Murray, S. N.; Pennisi, T. R.; Han, B.; Kang, Y.; Goulding, R. H.; Crisp, D. W.; Sparks, D. O.; Luciano, N. P.; Carmichael, J. R.; Carr, J.

2008-02-01

The U.S. Spallation Neutron Source (SNS) will require substantially higher average and pulse H- beam currents than can be produced from conventional ion sources such as the base line SNS source. H- currents of 40-50mA (SNS operations) and 70-100mA (power upgrade project) with a rms emittance of 0.20-0.35πmmmrad and a ˜7% duty factor will be needed. We are therefore investigating several advanced ion source concepts based on rf plasma excitation. First, the performance characteristics of an external antenna source based on an Al2O3 plasma chamber combined with an external multicusp magnetic configuration, an elemental Cs system, and plasma gun will be discussed. Second, the first plasma measurements of a helicon-driven H- ion source will also be presented.

Kinetics analysis and quantitative calculations for the successive radioactive decay process

NASA Astrophysics Data System (ADS)

Zhou, Zhiping; Yan, Deyue; Zhao, Yuliang; Chai, Zhifang

2015-01-01

The general radioactive decay kinetics equations with branching were developed and the analytical solutions were derived by Laplace transform method. The time dependence of all the nuclide concentrations can be easily obtained by applying the equations to any known radioactive decay series. Taking the example of thorium radioactive decay series, the concentration evolution over time of various nuclide members in the family has been given by the quantitative numerical calculations with a computer. The method can be applied to the quantitative prediction and analysis for the daughter nuclides in the successive decay with branching of the complicated radioactive processes, such as the natural radioactive decay series, nuclear reactor, nuclear waste disposal, nuclear spallation, synthesis and identification of superheavy nuclides, radioactive ion beam physics and chemistry, etc.