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Sample records for spent fuel measurements

  1. Calibration of spent fuel measurement assembly

    NASA Astrophysics Data System (ADS)

    Koleska, Michal; Viererbl, Ladislav; Marek, Milan

    2014-11-01

    The LVR-15 research reactor (Czech Republic) had been converted from the highly enriched IRT-2M to the low enriched IRT-4M fuel. For the possibility of the independent pre-transport evaluation of IRT-2M burnup, a spectrometric system was developed. This spectrometric system consists of the fuel holder, the collimator and the portable Canberra Big MAC HPGe (High Purity Germanium) detector. In order to have well reproducible and reliable experimental data for modeling of the measurement system, calibration with the 110mAg isotope with known activity was performed. This isotope was chosen for having energies similar to isotopes measured in fuel assemblies. The 110mAg isotope was prepared by irradiating of the silver foil in LVR-15 research reactor; its activity was evaluated in the LVR-15's spectrometric laboratory. From the measured data, an efficiency curve of the spectrometric system has been determined. The experimental data were compared to the calculation results with the MCNPX model of the spectrometric system.

  2. PWR and BWR spent fuel assembly gamma spectra measurements

    DOE PAGES

    Vaccaro, S.; Tobin, Stephen J.; Favalli, Andrea; ...

    2016-07-17

    A project to research the application of nondestructive assay (NDA) to spent fuel assemblies is underway. The research team comprises the European Atomic Energy Community (EURATOM), embodied by the European Commission, DG Energy, Directorate EURATOM Safeguards; the Swedish Nuclear Fuel and Waste Management Company (SKB); two universities; and several United States national laboratories. The Next Generation of Safeguards Initiative–Spent Fuel project team is working to achieve the following technical goals more easily and efficiently than in the past using nondestructive assay measurements of spent fuel assemblies: (1) verify the initial enrichment, burnup, and cooling time of facility declaration; (2) detectmore » the diversion or replacement of pins, (3) estimate the plutonium mass, (4) estimate the decay heat, and (5) determine the reactivity of spent fuel assemblies. This study focuses on spectrally resolved gamma-ray measurements performed on a diverse set of 50 assemblies [25 pressurized water reactor (PWR) assemblies and 25 boiling water reactor (BWR) assemblies]; these same 50 assemblies will be measured with neutron-based NDA instruments and a full-length calorimeter. Given that encapsulation/repository and dry storage safeguards are the primarily intended applications, the analysis focused on the dominant gamma-ray lines of 137Cs, 154Eu, and 134Cs because these isotopes will be the primary gamma-ray emitters during the time frames of interest to these applications. This study addresses the impact on the measured passive gamma-ray signals due to the following factors: burnup, initial enrichment, cooling time, assembly type (eight different PWR and six different BWR fuel designs), presence of gadolinium rods, and anomalies in operating history. As a result, to compare the measured results with theory, a limited number of ORIGEN-ARP simulations were performed.« less

  3. PWR and BWR spent fuel assembly gamma spectra measurements

    SciTech Connect

    Vaccaro, S.; Tobin, Stephen J.; Favalli, Andrea; Grogan, Brandon R.; Jansson, Peter; Liljenfeldt, Henrik; Mozin, Vladimir; Hu, Jianwei; Schwalbach, P.; Sjoland, A.; Trellue, Holly; Vo, D.

    2016-07-17

    A project to research the application of nondestructive assay (NDA) to spent fuel assemblies is underway. The research team comprises the European Atomic Energy Community (EURATOM), embodied by the European Commission, DG Energy, Directorate EURATOM Safeguards; the Swedish Nuclear Fuel and Waste Management Company (SKB); two universities; and several United States national laboratories. The Next Generation of Safeguards Initiative–Spent Fuel project team is working to achieve the following technical goals more easily and efficiently than in the past using nondestructive assay measurements of spent fuel assemblies: (1) verify the initial enrichment, burnup, and cooling time of facility declaration; (2) detect the diversion or replacement of pins, (3) estimate the plutonium mass, (4) estimate the decay heat, and (5) determine the reactivity of spent fuel assemblies. This study focuses on spectrally resolved gamma-ray measurements performed on a diverse set of 50 assemblies [25 pressurized water reactor (PWR) assemblies and 25 boiling water reactor (BWR) assemblies]; these same 50 assemblies will be measured with neutron-based NDA instruments and a full-length calorimeter. Given that encapsulation/repository and dry storage safeguards are the primarily intended applications, the analysis focused on the dominant gamma-ray lines of 137Cs, 154Eu, and 134Cs because these isotopes will be the primary gamma-ray emitters during the time frames of interest to these applications. This study addresses the impact on the measured passive gamma-ray signals due to the following factors: burnup, initial enrichment, cooling time, assembly type (eight different PWR and six different BWR fuel designs), presence of gadolinium rods, and anomalies in operating history. As a result, to compare the measured results with theory, a limited number of ORIGEN-ARP simulations were performed.

  4. PWR and BWR spent fuel assembly gamma spectra measurements

    SciTech Connect

    Vaccaro, S.; Tobin, Stephen J.; Favalli, Andrea; Grogan, Brandon R.; Jansson, Peter; Liljenfeldt, Henrik; Mozin, Vladimir; Hu, Jianwei; Schwalbach, P.; Sjoland, A.; Trellue, Holly; Vo, D.

    2016-07-17

    A project to research the application of nondestructive assay (NDA) to spent fuel assemblies is underway. The research team comprises the European Atomic Energy Community (EURATOM), embodied by the European Commission, DG Energy, Directorate EURATOM Safeguards; the Swedish Nuclear Fuel and Waste Management Company (SKB); two universities; and several United States national laboratories. The Next Generation of Safeguards Initiative–Spent Fuel project team is working to achieve the following technical goals more easily and efficiently than in the past using nondestructive assay measurements of spent fuel assemblies: (1) verify the initial enrichment, burnup, and cooling time of facility declaration; (2) detect the diversion or replacement of pins, (3) estimate the plutonium mass, (4) estimate the decay heat, and (5) determine the reactivity of spent fuel assemblies. This study focuses on spectrally resolved gamma-ray measurements performed on a diverse set of 50 assemblies [25 pressurized water reactor (PWR) assemblies and 25 boiling water reactor (BWR) assemblies]; these same 50 assemblies will be measured with neutron-based NDA instruments and a full-length calorimeter. Given that encapsulation/repository and dry storage safeguards are the primarily intended applications, the analysis focused on the dominant gamma-ray lines of 137Cs, 154Eu, and 134Cs because these isotopes will be the primary gamma-ray emitters during the time frames of interest to these applications. This study addresses the impact on the measured passive gamma-ray signals due to the following factors: burnup, initial enrichment, cooling time, assembly type (eight different PWR and six different BWR fuel designs), presence of gadolinium rods, and anomalies in operating history. As a result, to compare the measured results with theory, a limited number of ORIGEN-ARP simulations were performed.

  5. PWR and BWR spent fuel assembly gamma spectra measurements

    NASA Astrophysics Data System (ADS)

    Vaccaro, S.; Tobin, S. J.; Favalli, A.; Grogan, B.; Jansson, P.; Liljenfeldt, H.; Mozin, V.; Hu, J.; Schwalbach, P.; Sjöland, A.; Trellue, H.; Vo, D.

    2016-10-01

    A project to research the application of nondestructive assay (NDA) to spent fuel assemblies is underway. The research team comprises the European Atomic Energy Community (EURATOM), embodied by the European Commission, DG Energy, Directorate EURATOM Safeguards; the Swedish Nuclear Fuel and Waste Management Company (SKB); two universities; and several United States national laboratories. The Next Generation of Safeguards Initiative-Spent Fuel project team is working to achieve the following technical goals more easily and efficiently than in the past using nondestructive assay measurements of spent fuel assemblies: (1) verify the initial enrichment, burnup, and cooling time of facility declaration; (2) detect the diversion or replacement of pins, (3) estimate the plutonium mass, (4) estimate the decay heat, and (5) determine the reactivity of spent fuel assemblies. This study focuses on spectrally resolved gamma-ray measurements performed on a diverse set of 50 assemblies [25 pressurized water reactor (PWR) assemblies and 25 boiling water reactor (BWR) assemblies]; these same 50 assemblies will be measured with neutron-based NDA instruments and a full-length calorimeter. Given that encapsulation/repository and dry storage safeguards are the primarily intended applications, the analysis focused on the dominant gamma-ray lines of 137Cs, 154Eu, and 134Cs because these isotopes will be the primary gamma-ray emitters during the time frames of interest to these applications. This study addresses the impact on the measured passive gamma-ray signals due to the following factors: burnup, initial enrichment, cooling time, assembly type (eight different PWR and six different BWR fuel designs), presence of gadolinium rods, and anomalies in operating history. To compare the measured results with theory, a limited number of ORIGEN-ARP simulations were performed.

  6. Comparison of model predictions with measurements using the improved spent fuel attribute tester

    SciTech Connect

    Dupree, S.A.; Laub, T.W.; Arlt, R.

    1994-08-01

    Design improvements for the International Atomic Energy Agency`s Spent Fuel Attribute Tester, recommended on the basis of an optimization study, were incorporated into a new instrument fabricated under the Finnish Support Programme. The new instrument was tested at a spent fuel storage pool on September 8 and 9, 1993. The result of two of the measurements have been compared with calculations. In both cases the calculated and measured pulse height spectra in good agreement and the {sup 137}Cs gamma peak signature from the target spent fuel element is present.

  7. Spent-fuel verification measurements using passive and active radiation techniques

    SciTech Connect

    Ewing, R.I.; Seager, K.D.

    1996-08-01

    This paper describes an evolutionary development process that will lead to spent fuel measurements that directly measure fissile reactivity. First, the Fork measurement system has been used to verify the burnup of pressurized water reactor (PWR) spent-fuel assemblies at U.S. nuclear utilities. Fork measurements have demonstrated the utility of the passive Fork system to verify reactor records with a single 100-second measurement on each assembly. Second, an Advanced Fork system incorporating collimated gamma-ray spectroscopy has been designed to permit advanced calibration techniques that are independent of reactor burnup records and to allow rapid axial scanning of spent fuel assemblies. Third, an Active Fork system incorporating a neutron source to interrogate spent fuel is proposed to provide the capability to measure fissile reactivity, when compared to measurements on fresh fuel assemblies of the same design. The Advanced and Active Fork systems have wide applicability to spent fuel verification for PWR, boiling water reactor (BWR), and U.S. Department of Energy (DOE) spent fuel.

  8. Analysis of new measurements of Calvert Cliffs spent fuel samples using SCALE 6.2

    DOE PAGES

    Hu, Jianwei; Giaquinto, J. M.; Gauld, I. C.; ...

    2017-04-28

    High quality experimental data for isotopic compositions in irradiated fuel are important to spent fuel applications, including nuclear safeguards, spent fuel storage, transportation, and final disposal. The importance of these data has been increasingly recognized in recent years, particularly as countries like Finland and Sweden plan to open the world’s first two spent fuel geological repositories in 2020s, while other countries, including the United States, are considering extended dry fuel storage options. Destructive and nondestructive measurements of a spent fuel rod segment from a Combustion Engineering 14 × 14 fuel assembly of the Calvert Cliffs Unit 1 nuclear reactor havemore » been recently performed at Oak Ridge National Laboratory (ORNL). These ORNL measurements included two samples selected from adjacent axial locations of a fuel rod with initial enrichment of 3.038 wt% 235U, which achieved burnups close to 43.5 GWd/MTU. More than 50 different isotopes of 16 elements were measured using high precision measurement methods. Various investigations have assessed the quality of the new ORNL measurement data, including comparison to previous measurements and to calculation results. Previous measurement data for samples from the same fuel rod measured at ORNL are available from experiments performed at Pacific Northwest National Laboratory in the United States and the Khoplin Radium Institute in Russia. Detailed assembly models were developed using the newly released SCALE 6.2 code package to simulate depletion and decay of the measured fuel samples. Furthermore, results from this work show that the new ORNL measurements provide a good quality radiochemical assay data set for spent fuel with relatively high burnup and long cooling time, and they can serve as good benchmark data for nuclear burnup code validation and spent fuel studies.« less

  9. Web interface for control of spent fuel measurements at FCF.

    SciTech Connect

    Soltys, I. E.; Yacout, A. M.; McKnight, R. D.

    1999-10-11

    The material control and accountancy system for the Fuel Conditioning Facility (FCF) initially uses calculated values for the mass flows of irradiated EBR-11 driver fuel to be processed in the electrorefiner. These calculated values are continually verified by measurements performed by the Analytical Laboratory (AL) on samples from the fuel element chopper retained for each chopper batch. Measured values include U and Pu masses, U and Pu isotopic fractions, and burnup (via La and Tc). When the measured data become available, it is necessary to determine if the measured and calculated data are consistent. This verification involves accessing two databases and performing standard statistical analyses to produce control charts for these measurements. These procedures can now be invoked via a Web interface providing: a timely and efficient control of these measurements, a user-friendly interface, off-site remote access to the data, and a convenient means of studying correlations among the data. This paper will present the architecture of the interface and a description of the control procedures, as well as examples of the control charts and correlations.

  10. Recent advances in hardware and software are to improve spent fuel measurements

    SciTech Connect

    Staples, P.; Beddingfield, D. H.; Lestone, J. P.; Pelowitz, D. G.; Bytchkov, M.; Starovich, Z.; Harizanov, I.; Luna-Vellejo, J.; Lavender, C.

    2001-01-01

    Vast quantities of spent fuel are available for safeguard measurements, primarily in Commonwealth of Independent States (CIS) of the former Soviet Union. This spent fuel, much of which consists of long-cooling-time material, is going to become less unique in the world safeguards arena as reprocessing projects or permanent repositories continue to be delayed or postponed. The long cooling time of many of the spent fuel assemblies being prepared for intermediate term storage in the CIS countries promotes the possibility of increased accuracy in spent fuel assays. This improvement is made possible through the process of decay of the Curium isotopes and of fission products. An important point to consider for the future that could advance safeguards measurements for reverification and inspection would be to determine what safeguards requirements should be imposed upon this 'new' class of spent fuel, Improvements in measurement capability will obviously affect the safeguards requirements. What most significantly enables this progress in spent fuel measurements is the improvement in computer processing power and software enhancements leading to user-friendly Graphical User Interfaces (GUT's). The software used for these projects significantly reduces the IAEA inspector's time expenditure for both learning and operating computer and data acquisition systems, At the same time, by standardizing the spent fuel measurements, it is possible to increase reproducibility and reliability of the measurement data. Hardware systems will be described which take advantage of the increased computer control available to enable more complex measurement scenarios. A specific example of this is the active regulation of a spent fuel neutron coincident counter's {sup 3}He tubes high voltage, and subsequent scaling of measurement results to maintain a calibration for direct assay of the plutonium content of Fast Breeder Reactor spent fuel. The plutonium content has been successfully determined

  11. The spent fuel safety experiment

    SciTech Connect

    Harms, G.A.; Davis, F.J.; Ford, J.T.

    1995-08-01

    The Department of Energy is conducting an ongoing investigation of the consequences of taking fuel burnup into account in the design of spent fuel transportation packages. A series of experiments, collectively called the Spent Fuel Safety Experiment (SFSX), has been devised to provide integral benchmarks for testing computer-generated predictions of spent fuel behavior. A set of experiments is planned in which sections of unirradiated fuel rods are interchanged with similar sections of spent PWR fuel rods in a critical assembly. By determining the critical size of the arrays, one can obtain benchmark data for comparison with criticality safety calculations. The SFSX provides a direct measurement of the reactivity effects of spent PWR fuel using a well-characterized, spent fuel sample. The SFSX also provides an experimental measurement of the end-effect, i.e., the reactivity effect of the variation of the burnup profile at the ends of PWR fuel rods. The design of the SFSX is optimized to yield accurate benchmark measurements of the effects of interest, well above experimental uncertainties.

  12. Spent fuel and residue measurement instrumentation at the Sellafield nuclear fuel reprocessing facility

    SciTech Connect

    Chesterman, A.S.; Clark, P.A.

    1995-12-31

    The Sellafield reprocessing plant receives and reprocesses several thousand tonnes of spent light water reactor (LWR), advanced gas cooled reactor (AGR) and natural uranium magnesium alloy clad (Magnox) fuels each year. The safety and cost effectiveness of these operations has been supported by the development and installation, at key points in the process, of a range of special purpose radiometric instrumentation. Systems in routine operational use verify the cooling time, burn-tip and initial and final U-235 equivalent enrichment of fuel assemblies in the storage and handling ponds. Other systems determine the radionuclide inventories of fuel residues in intermediate level waste arising from plant operations. The measurement techniques employed include high resolution gamma spectrometry, passive neutron counting and neutron interrogation by the use of a Cf-252 source and deuterium-tritium (D-T) pulsed neutron generators. Details of the instruments including mechanical installation arrangements and measurement data are presented in the paper along with a discussion of possible future uses of similar instruments for burn-up credit associated with fuel and residue storage, transportation and disposal.

  13. Spent-fuel composition: a comparison of predicted and measured data

    SciTech Connect

    Thomas, C.C. Jr.; Cobb, D.D.; Ostenak, C.A.

    1981-03-01

    The uncertainty in predictions of the nuclear materials content of spent light-water reactor fuel was investigated to obtain guidelines for nondestructive spent-fuel verification and assay. Values predicted by the reactor operator were compared with measured values from fuel reprocessors for six reactors (three PWR and three BWR). The study indicates that total uranium, total plutonium, fissile uranium, fissile plutonium, and total fissile content can be predicted with biases ranging from 1 to 6% and variabilities (1-sigma) ranging from 2 to 7%. The higher values generally are associated with BWRs. Based on the results of this study, nondestructive assay measurements that are accurate and precise to 5 to 10% (1sigma) or better should be useful for quantitative analyses of typical spent fuel.

  14. Measuring the Multiplication of Spent Fuel Assemblies – It’s easier than you think!

    SciTech Connect

    Tobin, Stephen Joseph

    2016-11-09

    This is a set of eight slides which advertise how easy it can be to measure the multiplication of a spent fuel assembly. A robust (fission chambers), rapid (under 15 minutes), direct (multiplication is measured, not photons from fission fragments) measurement of multiplication is possible.

  15. Spent fuel pyroprocessing demonstration

    SciTech Connect

    McFarlane, L.F.; Lineberry, M.J.

    1995-05-01

    A major element of the shutdown of the US liquid metal reactor development program is managing the sodium-bonded spent metallic fuel from the Experimental Breeder Reactor-II to meet US environmental laws. Argonne National Laboratory has refurbished and equipped an existing hot cell facility for treating the spent fuel by a high-temperature electrochemical process commonly called pyroprocessing. Four products will be produced for storage and disposal. Two high-level waste forms will be produced and qualified for disposal of the fission and activation products. Uranium and transuranium alloys will be produced for storage pending a decision by the US Department of Energy on the fate of its plutonium and enriched uranium. Together these activities will demonstrate a unique electrochemical treatment technology for spent nuclear fuel. This technology potentially has significant economic and technical advantages over either conventional reprocessing or direct disposal as a high-level waste option.

  16. Measurement of plutonium in spent nuclear fuel by self-induced x-ray fluorescence

    SciTech Connect

    Hoover, Andrew S; Rudy, Cliff R; Tobin, Steve J; Charlton, William S; Stafford, A; Strohmeyer, D; Saavadra, S

    2009-01-01

    Direct measurement of the plutonium content in spent nuclear fuel is a challenging problem in non-destructive assay. The very high gamma-ray flux from fission product isotopes overwhelms the weaker gamma-ray emissions from plutonium and uranium, making passive gamma-ray measurements impossible. However, the intense fission product radiation is effective at exciting plutonium and uranium atoms, resulting in subsequent fluorescence X-ray emission. K-shell X-rays in the 100 keV energy range can escape the fuel and cladding, providing a direct signal from uranium and plutonium that can be measured with a standard germanium detector. The measured plutonium to uranium elemental ratio can be used to compute the plutonium content of the fuel. The technique can potentially provide a passive, non-destructive assay tool for determining plutonium content in spent fuel. In this paper, we discuss recent non-destructive measurements of plutonium X-ray fluorescence (XRF) signatures from pressurized water reactor spent fuel rods. We also discuss how emerging new technologies, like very high energy resolution microcalorimeter detectors, might be applied to XRF measurements.

  17. Measurement techniques in dry-powdered processing of spent nuclear fuels.

    SciTech Connect

    Bowers, D. L.; Hong, J.-S.; Kim, H.-D.; Persiani, P. J.; Wolf, S. F.

    1999-07-21

    High-performance liquid chromatography (HPLC) with inductively coupled plasma mass spectrometry (ICPMS) detection, {alpha}-spectrometry ({alpha}-S), and {gamma}-spectrometry ({gamma}-S) were used for the determination of nuclide content in five samples excised from a high-burnup fuel rod taken from a pressurized water reactor (PWR). The samples were prepared for analysis by dissolution of dry-powdered samples. The measurement techniques required no separation of the plutonium, uranium, and fission products. The sample preparation and analysis techniques showed promise for in-line analysis of highly-irradiated spent fuels in a dry-powdered process. The analytical results allowed the determination of fuel burnup based on {sup 148}Nd, Pu, and U content. A goal of this effort is to develop the HPLC-ICPMS method for direct fissile material accountancy in the dry-powdered processing of spent nuclear fuel.

  18. Spent fuel assembly hardware: Characterization and 10 CFR 61 classification for waste disposal: Volume 1, Activation measurements and comparison with calculations for spent fuel assembly hardware

    SciTech Connect

    Luksic, A.

    1989-06-01

    Consolidation of spent fuel is under active consideration as the US Department of Energy plans to dispose of spent fuel. During consolidation, the fuel pins are removed from an intact fuel assembly and repackaged into a more compact configuration. After repackaging, approximately 30 kg of residual spent fuel assembly hardware per assembly remains that is also radioactive and requires disposal. Understanding the nature of this secondary waste stream is critical to designing a system that will properly handle, package, store, and dispose of the waste. This report presents a methodology for estimating the radionuclide inventory in irradiated spent fuel hardware. Ratios are developed that allow the use of ORIGEN2 computer code calculations to be applied to regions that are outside the fueled region. The ratios are based on the analysis of samples of irradiated hardware from spent fuel assemblies. The results of this research are presented in three volumes. In Volume 1, the development of scaling factors that can be used with ORIGEN2 calculations to estimate activation of spent fuel assembly hardware is documented. The results from laboratory analysis of irradiated spent-fuel hardware samples are also presented in Volume 1. In Volumes 2 and 3, the calculated flux profiles of spent nuclear fuel assemblies are presented for pressurized water reactors and boiling water reactors, respectively. The results presented in Volumes 2 and 3 were used to develop the scaling factors documented in Volume 1. 5 refs., 4 figs., 21 tabs.

  19. Spent Fuel Test - Climax: technical measurements. Interim report, fiscal year 1982

    SciTech Connect

    Patrick, W.C.; Ballou, L.B.; Butkovich, T.R.; Carlson, R.C.; Durham, W.B.; Hage, G.L.; Majer, E.L.; Montan, D.N.; Nyholm, R.A.; Rector, N.L.

    1983-02-01

    The Spent Fuel Test - Climax (SFT-C) is located 420 m below surface in the Climax stock granite on the Nevada Test Site. The test is being conducted for the US Department of Energy (DOE) under the technical direction of the Lawrence Livermore National Laboratory (LLNL). Eleven canisters of spent nuclear reactor fuel were emplaced, and six electrical simulators were energized April to May 1980, thus initiating a test with a planned 3- to 5-year fuel storage phase. The SFT-C operational objective of demonstrating the feasibility of packaging, transporting, storing, and retrieving highly radioactive fuel assemblies in a safe and reliable manner has been met. Three exchanges of spent fuel between the SFT-C and a surface storage facility furthered this demonstration. Technical objectives of the test led to development of a technical measurements program, which is the subject of this and two previous interim reports. Geotechnical, seismological, and test status data have been recorded on a continuing basis for the first 2-1/2 years of the test on more than 900 channels. Data continue to be acquired from the test. Some data are now available for analysis and are presented here. Highlights of activities this year include analysis of fracture data obtained during site characterization, laboratory studies of radiation effects and drilling damage in Climax granite, improved calculations of near-field heat transfer and thermomechanical response, a ventilation effects study, and further development of the data acquisition and management systems.

  20. Spent fuel storage. Facts booklet

    SciTech Connect

    1980-04-01

    In October 1977, the Department of Energy (DOE) announced a spent nuclear fuel policy where the Government would, under certain conditions, take title to and store spent nuclear fuel from commercial power reactors. The policy is intended to provide spent fuel storage until final disposition is available. DOE has programs for providing safe, long-term disposal of nuclear waste. The spent fuel storage program is one element of waste management and compliments the disposal program. The costs for spent fuel services are to be fully recovered by the Government from the utilities. This will allow the utilities to confidently consider the costs for disposition of spent fuel in their rate structure. The United States would also store limited amounts of foreign spent fuel to meet nonproliferation objectives. This booklet summarizes information on many aspects of spent fuel storage.

  1. A FAST BREEDER REACTOR SPENT FUEL MEASUREMENTS PROGRAM FOR BN-350 REACTOR

    SciTech Connect

    P. STAPLES; J. HALBIG; ET AL

    1999-04-01

    A project to verify the fissile content of fast breeder reactor spent nuclear fuel is underway in the Republic of Kasakhstan. There are a variety of assembly types with different irradiation histories and profiles in the reactor that require a variety of measurement and analysis procedures. These procedures will be discussed and compared as will the general process that has been designed to resolve any potential measurement discrepancies. The underwater counter is part of a system that is designed to assist the International Atomic Energy Agency (IAEA) in maintaining continuity of knowledge from the time of measurement until the measured item is placed in a welded container with a unique identification. In addition to satisfying IAEA requirements for the spent nuclear fuel, this measurement program is able to satisfy some of the measurement requirements for the Kasakhstan Atomic Energy Agency concerning the repackaging of the spent nuclear fuel into a standard canister. The project is currently operational in a mode requiring the IAEA's continuous presence.

  2. Criticality of spent reactor fuel

    SciTech Connect

    Harris, D.R.

    1987-01-01

    The storage capacity of spent reactor fuel pools can be greatly increased by consolidation. In this process, the fuel rods are removed from reactor fuel assemblies and are stored in close-packed arrays in a canister or skeleton. An earlier study examined criticality consideration for consolidation of Westinghouse fuel, assumed to be fresh, in canisters at the Millstone-2 spent-fuel pool and in the General Electric IF-300 shipping cask. The conclusions were that the fuel rods in the canister are so deficient in water that they are adequately subcritical, both in normal and in off-normal conditions. One potential accident, the water spill event, remained unresolved in the earlier study. A methodology is developed here for spent-fuel criticality and is applied to the water spill event. The methodology utilizes LEOPARD to compute few-group cross sections for the diffusion code PDQ7, which then is used to compute reactivity. These codes give results for fresh fuel that are in good agreement with KENO IV-NITAWL Monte Carlo results, which themselves are in good agreement with continuous energy Monte Carlo calculations. These methodologies are in reasonable agreement with critical measurements for undepleted fuel.

  3. Material accountancy measurement techniques in dry-powdered processing of nuclear spent fuels.

    SciTech Connect

    Wolf, S. F.

    1999-03-24

    The paper addresses the development of inductively coupled plasma-mass spectrometry (ICPMS), thermal ionization-mass spectrometry (TIMS), alpha-spectrometry, and gamma spectrometry techniques for in-line analysis of highly irradiated (18 to 64 GWD/T) PWR spent fuels in a dry-powdered processing cycle. The dry-powdered technique for direct elemental and isotopic accountancy assay measurements was implemented without the need for separation of the plutonium, uranium and fission product elements in the bulk powdered process. The analyses allow the determination of fuel burn-up based on the isotopic composition of neodymium and/or cesium. An objective of the program is to develop the ICPMS method for direct fissile nuclear materials accountancy in the dry-powdered processing of spent fuel. The ICPMS measurement system may be applied to the KAERI DUPIC (direct use of spent PWR fuel in CANDU reactors) experiment, and in a near-real-time mode for international safeguards verification and non-proliferation policy concerns.

  4. Direct measurement of 235U in spent fuel rods with Gamma-ray mirrors

    NASA Astrophysics Data System (ADS)

    Ruz, J.; Brejnholt, N. F.; Alameda, J. B.; Decker, T. A.; Descalle, M. A.; Fernandez-Perea, M.; Hill, R. M.; Kisner, R. A.; Melin, A. M.; Patton, B. W.; Soufli, R.; Ziock, K.; Pivovaroff, M. J.

    2015-03-01

    Direct measurement of plutonium and uranium X-rays and gamma-rays is a highly desirable non-destructive analysis method for the use in reprocessing fuel environments. The high background and intense radiation from spent fuel make direct measurements difficult to implement since the relatively low activity of uranium and plutonium is masked by the high activity from fission products. To overcome this problem, we make use of a grazing incidence optic to selectively reflect Kα and Kβ fluorescence of Special Nuclear Materials (SNM) into a high-purity position-sensitive germanium detector and obtain their relative ratios.

  5. PNNL/Euratom glass fiber optic, spent fuel neutron profile measurement system

    SciTech Connect

    SM Bowyer; JE Smart

    2000-03-03

    The glass fiber optic spent fuel neutron profile measurement system is designed to measure the neutron profile of a Castor with high reproducibility and to distinguish spent fuel Castor contents from vitrified waste Castor contents. The basic principle of the detector is that the glass fibers detect thermal neutrons. The glass is loaded with lithium enriched in Li-6, which has a high thermal neutron cross-section. A neutron is captured by the Li-6 and a He-4 and H-3 are created. Because the glass also contains Cerium in a 3{sup +} ionization state, the excitation caused by the movement of the He-4 and H-3 results in the emission of light from the cerium atoms. This light then travels to the ends of the fiber where it is detected by photon sensitive devices (e.g., photo-multiplier tubes).

  6. Spent fuel test - Climax: technical measurements. Interim report, Fiscal Year 1983

    SciTech Connect

    Patrick, W.C.; Butkovich, T.R.; Carlson, R.C.; Durham, W.B.; Ganow, H.C.; Hage, G.L.; Majer, E.L.; Montan, D.N.; Nyholm, R.A.; Rector, N.L.

    1984-02-01

    The Spent Fuel Test - Climax (SFT-C) is located 420 m below surface in the Climax stock granite on the Nevada Test Site. The test is being conducted as part of the Nevada Nuclear Waste Storage Investigations. Eleven canisters of spent nuclear reactor fuel were emplaced, and six electrical simulators were energized April-May 1980. The spent-fuel canisters were retrieved and the thermal sources were de-energized in March-April 1983 when test data indicated that test objectives were met during the 3-year storage phase. The SFT-C operational objective of demonstrating the feasibility of packaging, transporting, storing, and retrieving highly radioactive fuel assemblies in a safe and reliable manner has been met. In addition to emplacement and retrieval operations, three exchanges of spent-fuel between the SFT-C and a surface storage facility, conducted during the storage phase, furthered this demonstration. Technical objectives of the test led to development of a technical measurements program, which is the subject of this and three previous interim reports. Geotechnical, seismological, and test status data have been recorded on a continuing basis for the 3-1/2 year duration of the test on more than 900 channels. Data acquisition from the test is now limited to instrumentation calibration and evaluation activities. Data now available for analysis are presented here. Highlights of activities this year include a campaign of in situ stress measurements, mineralogical and petrological studies of pretest core samples, microfracture analyses of laboratory irradiated cores, improved calculations of near-field heat transfer and thermomechanical response during the final months of heating as well as during a six-month cool-down period, metallurgical analyses of selected test components, and further development of the data acquisition and data management systems. 27 references, 68 figures, 10 tables.

  7. The spent fuel standard - does the can-in-canister concept for plutonium immobilization measure up?

    SciTech Connect

    Gray, L W; McKibben, J M

    1999-05-27

    Critics continue to question whether or not the can-in-canister concept for immobilization and disposal of surplus plutonium meets the ''Spent Fuel Standard.'' Following this standard would make this plutonium roughly as ''inaccessible for weapons use as the much larger and growing quantity of plutonium that exists in spent fuel from commercial reactors.'' These critics take a narrower view of the ''Spent Fuel Standard'' than was intended in the National Academy reports, rather than considering the total effective barrier. This paper directly compares retrieval and recovery of plutonium from a can-in-canister to a spent fuel assembly. The conclusion from this study, as from earlier studies, is that the plutonium in the can-in-canister form is less accessible and less attractive to a potential proliferate than the plutonium that exists in spent fuel from commercial reactors.

  8. Initial measurements of BN-350 spent fuel in dry storage casks using the dual slab verification detonator

    SciTech Connect

    Santi, Peter Angelo; Browne, Michael C; Freeman, Corey R; Parker, Robert F; Williams, Richard B

    2010-01-01

    The Dual Slab Verification Detector (DSVD) has been developed, built, and characterized by Los Alamos National Laboratory in cooperation with the International Atomic Energy Agency (IAEA) as part of the dry storage safeguards system for the spent fuel from the BN-350 fast reactor. The detector consists of two rows of 3He tubes embedded in a slab of polyethylene which has been designed to be placed on the outer surface of the dry storage cask. By performing DSVD measurements at several different locations around the outer surface of the DUC, a signature 'fingerprint' can be established for each DUC based on the neutron flux emanating from inside the dry storage cask. The neutron fingerprint for each individual DUC will be dependent upon the spatial distribution of nuclear material within the cask, thus making it sensitive to the removal of a certain amount of material from the cask. An initial set of DSVD measurements have been performed on the first set of dry storage casks that have been loaded with canisters of spent fuel and moved onto the dry storage pad to both establish an initial fingerprint for these casks as well as to quantify systematic uncertainties associated with these measurements. The results from these measurements will be presented and compared with the expected results that were determined based on MCNPX simulations of the dry storage facility. The ability to safeguard spent nuclear fuel is strongly dependent on the technical capabilities of establishing and maintaining continuity of knowledge (COK) of the spent fuel as it is released from the reactor core and either reprocessed or packaged and stored at a storage facility. While the maintenance of COK is often done using continuous containment and surveillance (C/S) on the spent fuel, it is important that the measurement capabilities exist to re-establish the COK in the event of a significant gap in the continuous CIS by performing measurements that independently confirm the presence and content

  9. Spent fuel measurements. passive neutron albedo reactivity (PNAR) and photon signatures

    SciTech Connect

    Eigenbrodt, Julia; Menlove, Howard Olsen

    2016-03-29

    The International Atomic Energy Agency’s (IAEA) safeguards technical objective is the timely detection of a diversion of a significant quantity of nuclear material from peaceful activities to the manufacture of nuclear weapons or of other nuclear explosive devices or for purposes unknown, and deterrence of such diversion by the risk of early detection. An important IAEA task towards meeting this objective is the ability to accurately and reliably measure spent nuclear fuel (SNF) to verify reactor operating parameters and verify that the fuel has not been removed from reactors or SNF storage facilities. This dissertation analyzes a method to improve the state-of-the-art of nuclear material safeguards measurements using two combined measurement techniques: passive neutron albedo reactivity (PNAR) and passive spectral photon measurements.

  10. Spent fuel test - Climax: technical measurements. Interim report, fiscal year 1981

    SciTech Connect

    Patrick, W.C.; Ballou, L.B.; Butkovich, T.R.

    1982-04-30

    The Spent Fuel Test-Climax (SFT-C) is located 420 m below surface in the Climax granite stock on the Nevada Test Site. Eleven canisters of spent nuclear reactor fuel were emplaced, and six electrical simulators were energized from April to May 1980, initiating the 3- to 5-year-duration test. The SFT-C operational objective of demonstrating the feasibility of packaging, transporting, storing, and retrieving highly radioactive fuel assemblies in a safe and reliable manner has been met. Technical objectives of the test led to development of a technical measurements program, which is the subject of this report. Geotechnical, seismological, and test status data have been recorded on a continuing basis for the first 1-1/2 years of the test on more than 900 channels. Much of the acquired data are now available for analysis and are presented here. Highlights of activities this year include completion of site characterization field work, major modifications to the data acquisition and the management systems, and the addition of instrument evaluation as an explicit objective of the test.

  11. Near-field heat transfer at the spent fuel test-climax: a comparison of measurements and calculations

    SciTech Connect

    Patrick, W.C.; Montan, D.N.; Ballou, L.B.

    1981-08-21

    The Spent Fuel Test in the Climax granitic stock at the DOE Nevada Test Site is a test of the feasibility of storage and retrieval of spent nuclear reactor fuel in a deep geologic environment. Eleven spent fuel elements, together with six thermally identical electrical resistance heaters and 20 peripheral guard heaters, are emplaced 420 m below surface in a three-drift test array. This array was designed to simulate the near-field effects of thousands of canisters of nuclear waste and to evaluate the effects of heat alone, and heat plus ionizing radiation on the rock. Thermal calculations and measurements are conducted to determine thermal transport from the spent fuel and electrical resistance heaters. Calculations associated with the as-built Spent Fuel Test geometry and thermal source histories are presented and compared with thermocouple measurements made throughout the test array. Comparisons in space begin at the spent fuel canister and include the first few metres outside the test array. Comparisons in time begin at emplacement and progress through the first year of thermal loading in this multi-year test.

  12. PNNL/Euratom glass fiber-optic, spent-fuel profile measurement system

    SciTech Connect

    Bowyer, S.M.; Smart, J.E.; Hansen, R.R.

    1999-07-01

    Discussions between Euratom and Pacific Northwest National Laboratory (PNNL) revealed a need for a neutron detection system that could measure the neutron profile down the entire length of a CASTOR in one measurement. The CASTORS (dry storage casks for spent fuel and vitrified wastes) are {approximately}6 m high and 2 x 2 m square in cross section. Neutron profiles of the CASTORS are desirable for both content identification and verification. Profile measurements have traditionally been done with {sup 3}He-based detectors {approximately}1 m high that scan the length of a CASTOR as they are lifted by a crane. Geometric reproducibility errors plague this type of measurement; hence, the ability to simultaneously measure the neutron profile over the entire length of the CASTOR became highly desirable. Use of the PNNL-developed neutron-sensitive glass fibers in the construction of a 6-m-high detector was proposed, and design and construction of the detector began.

  13. Spent-fuel cooling curve for safeguard applications of gross-gamma measurements

    SciTech Connect

    Rinard, P.

    1983-04-01

    Gross-gamma detectors can be used to gather data from spent-fuel assemblies in a simple and rapid manner. Using these data, inspectors can generate a power-law curve to check the consistency of the declared values with the measured values; points outside the curve indicate erroneously declared values or removal of material. Simple types of erroneously declared values can be detected immediately, whereas subtle types may require a second measurement and more subtle types may escape detection. If measurements of passive emissions of neutrons from the assemblies are made in addition to the gamma measurements, the values of the exposures and cooling times can be estimated independent of the operator-declared values. Although not yet demonstrated, it may be possible to obtain crude estimates of the exposures and cooling times from the gamma measurments alone.

  14. Neutron spectra and dose-rate measurements around a transport cask for spent reactor fuel

    NASA Astrophysics Data System (ADS)

    Rimpler, Arndt

    1997-02-01

    A storage facility with a capacity of 420 containers is available for the interim storage of spent fuel from power reactors at the village of Gorleben in Germany. During transportation and storage of spent fuel casks radiation exposure of the personnel is dominated by neutrons. The routine control of the dose rate limits according to the transport regulations and the licence of the storage facility is performed with conventional neutron survey meters. These monitors, calibrated for fast neutrons at radionuclide neutron sources, usually overestimate the real dose rate in unknown neutron fields. In this paper, a series of measurements with several monitoring instruments near a transport cask of the CASTOR type is presented. The results are compared with reference data for the does equivalents calculated from the measured fluence spectra using a Bonner multisphere spectrometer. Besides reliable information about neutron spectra and dose rates at the container, it was found that some of the rem counters overestimate the true dose rate by a factor of 2 or more.

  15. Development of a water boil-off spent-fuel calorimeter system. [To measure decay heat generation rate

    SciTech Connect

    Creer, J.M.; Shupe, J.W. Jr.

    1981-05-01

    A calorimeter system was developed to measure decay heat generation rates of unmodified spent fuel assemblies from commercial nuclear reactors. The system was designed, fabricated, and successfully tested using the following specifications: capacity of one BWR or PWR spent fuel assembly; decay heat generation range 0.1 to 2.5 kW; measurement time of < 12 h; and an accuracy of +-10% or better. The system was acceptance tested using a dc reference heater to simulate spent fuel assembly heat generation rates. Results of these tests indicated that the system could be used to measure heat generation rates between 0.5 and 2.5 kW within +- 5%. Measurements of heat generation rates of approx. 0.1 kW were obtained within +- 15%. The calorimeter system has the potential to permit measurements of heat generation rates of spent fuel assemblies and other devices in the 12- to 14-kW range. Results of calorimetry of a Turkey Point spent fuel assembly indicated that the assembly was generating approx. 1.55 kW.

  16. Spent-fuel-storage alternatives

    SciTech Connect

    Not Available

    1980-01-01

    The Spent Fuel Storage Alternatives meeting was a technical forum in which 37 experts from 12 states discussed storage alternatives that are available or are under development. The subject matter was divided into the following five areas: techniques for increasing fuel storage density; dry storage of spent fuel; fuel characterization and conditioning; fuel storage operating experience; and storage and transport economics. Nineteen of the 21 papers which were presented at this meeting are included in this Proceedings. These have been abstracted and indexed. (ATT)

  17. Assessment of spent fuel cooling

    SciTech Connect

    Ibarra, J.G.; Jones, W.R.; Lanik, G.F.

    1997-02-01

    The paper presents the methodology, the findings, and the conclusions of a study that was done by the Nuclear Regulatory Commission`s Office for Analysis and Evaluation of Operational Data (AEOD) on loss of spent fuel pool cooling. The study involved an examination of spent fuel pool designs, operating experience, operating practices, and procedures. AEOD`s work was augmented in the area of statistics and probabilistic risk assessment by experts from the Idaho Nuclear Engineering Laboratory. Operating experience was integrated into a probabilistic risk assessment to gain insight on the risks from spent fuel pools.

  18. Intermodal transportation of spent fuel

    SciTech Connect

    Elder, H.K.

    1983-09-01

    Concepts for transportation of spent fuel in rail casks from nuclear power plant sites with no rail service are under consideration by the US Department of Energy in the Commercial Spent Fuel Management program at the Pacific Northwest Laboratory. This report identifies and evaluates three alternative systems for intermodal transfer of spent fuel: heavy-haul truck to rail, barge to rail, and barge to heavy-haul truck. This report concludes that, with some modifications and provisions for new equipment, existing rail and marine systems can provide a transportation base for the intermodal transfer of spent fuel to federal interim storage facilities. Some needed land transportation support and loading and unloading equipment does not currently exist. There are insufficient shipping casks available at this time, but the industrial capability to meet projected needs appears adequate.

  19. Active Interrogation for Spent Fuel

    SciTech Connect

    Swinhoe, Martyn Thomas; Dougan, Arden

    2015-11-05

    The DDA instrument for nuclear safeguards is a fast, non-destructive assay, active neutron interrogation technique using an external 14 MeV DT neutron generator for characterization and verification of spent nuclear fuel assemblies.

  20. Safeguards for spent fuels: Verification problems

    SciTech Connect

    Pillay, K.K.S.; Picard, R.R.

    1991-01-01

    The accumulation of large quantities of spent nuclear fuels world-wide is a serious problem for international safeguards. A number of International Atomic Energy Agency (IAEA) member states, including the US, consider spent fuel to be a material form for which safeguards cannot be terminated, even after permanent disposal in a geologic repository. Because safeguards requirements for spent fuels are different from those of conventional bulk-handling and item-accounting facilities, there is room for innovation to design a unique safeguards regime for spent fuels that satisfies the goals of the nuclear nonproliferation treaty at a reasonable cost to both the facility and the IAEA. Various strategies being pursued for long-term management of spent fuels are examined with a realistic example to illustrate the problems of verifying safeguards under the present regime. Verification of a safeguards regime for spent fuels requires a mix of standard safeguards approaches, such as quantitative verification and use of seals, with other measures that are unique to spent fuels. 17 refs.

  1. Transportation of spent MTR fuels

    SciTech Connect

    Raisonnier, D.

    1997-08-01

    This paper gives an overview of the various aspects of MTR spent fuel transportation and provides in particular information about the on-going shipment of 4 spent fuel casks to the United States. Transnucleaire is a transport and Engineering Company created in 1963 at the request of the French Atomic Energy Commission. The company followed the growth of the world nuclear industry and has now six subsidiaries and affiliated companies established in countries with major nuclear programs.

  2. Spent graphite fuel element processing

    SciTech Connect

    Holder, N.D.; Olsen, C.W.

    1981-07-01

    The Department of Energy currently sponsors two programs to demonstrate the processing of spent graphite fuel elements. General Atomic in San Diego operates a cold pilot plant to demonstrate the processing of both US and German high-temperature reactor fuel. Exxon Nuclear Idaho Company is demonstrating the processing of spent graphite fuel elements from Rover reactors operated for the Nuclear Rocket Propulsion Program. This work is done at Idaho National Engineering Laboratory, where a hot facility is being constructed to complete processing of the Rover fuel. This paper focuses on the graphite combustion process common to both programs.

  3. HFIR spent fuel management alternatives

    SciTech Connect

    Begovich, J.M.; Green, V.M.; Shappert, L.B.; Lotts, A.L.

    1992-10-15

    The High Flux Isotope Reactor (HFIR) at Martin Marietta Energy Systems' Oak Ridge National Laboratory (ORNL) has been unable to ship its spent fuel to Savannah River Site (SRS) for reprocessing since 1985. The HFIR storage pools are expected to fill up in the February 1994 to February 1995 time frame. If a management altemative to existing HFIR pool storage is not identified and implemented before the HFIR pools are full, the HFIR will be forced to shut down. This study investigated several alternatives for managing the HFIR spent fuel, attempting to identify options that could be implemented before the HFIR pools are full. The options investigated were: installing a dedicated dry cask storage facility at ORNL, increasing HFIR pool storage capacity by clearing the HFIR pools of debris and either close-packing or stacking the spent fuel elements, storing the spent fuel at another ORNL pool, storing the spent fuel in one or more hot cells at ORNL, and shipping the spent fuel offsite for reprocessing or storage elsewhere.

  4. Measurement and analysis of gamma-rays emitted from spent nuclear fuel above 3 MeV

    SciTech Connect

    Rodriguez, Douglas C.; Anderson, Elaina R.; Anderson, Kevin K.; Campbell, Luke W.; Fast, James E.; Jarman, Kenneth D.; Kulisek, Jonathan A.; Orton, Christopher R.; Runkle, Robert C.; Stave, Sean

    2013-08-28

    The Next Generation Safeguard Initiative (NGSI) includes an effort to determine the mass content of fissile isotopes contained within spent fuel through the spectroscopy of high-energy delayed gamma rays. Studies being performed indicate the primary difficulty is the ability to detect the desired signal in the presence of the intense background associated with spent fuel fission products. An enabling technology for this application is high-resolution high-purity germanium (HPGe) detectors capable of operating efficiently in at extremely high count rates. This presentation will describe the prospects of high-rate germanium detectors and delayed-gamma techniques, primarily discussing the efforts to merge these into a unique and viable system for measuring spent fuel.

  5. Ultra-High Rate Measurements of Spent Fuel Gamma-Ray Emissions

    NASA Astrophysics Data System (ADS)

    Rodriguez, Douglas; Vandevender, Brent; Wood, Lynn; Glasgow, Brian; Taubman, Matthew; Wright, Michael; Dion, Michael; Pitts, Karl; Runkle, Robert; Campbell, Luke; Fast, James

    2014-03-01

    Presently there are over 200,000 irradiated spent nuclear fuel (SNF) assemblies in the world, each containing a concerning amount of weapons-usable material. Both facility operators and safeguards inspectors want to improve composition determination. Current measurements are expensive and difficult so new methods are developed through models. Passive measurements are limited since a few specific decay products and the associated down-scatter overwhelm the gamma rays of interest. Active interrogation methods produce gamma rays beyond 3 MeV, minimizing the impact of the passive emissions that drop off sharply above this energy. New devices like the Ultra-High Rate Germanium (UHRGe) detector are being developed to advance these novel measurement methods. Designed for reasonable resolution at 106 s-1 output rates (compared to ~ 1 - 10 e 3 s-1 standards), SNF samples were directly measured using UHRGe and compared to models. Model verification further enables using Los Alamos National Laboratory SNF assembly models, developed under the Next Generation Safeguards Initiative, to determine emission and signal expectations. Measurement results and future application requirements for UHRGe will be discussed.

  6. Measurement and Analysis of Gamma-Rays Emitted From Spent Nuclear Fuel Above 3 MeV

    SciTech Connect

    Rodriguez, Douglas C.; Anderson, Elaina R.; Anderson, Kevin K.; Campbell, Luke W.; Fast, James E.; Jarman, Kenneth D.; Kulisek, Jonathan A.; Orton, Christopher R.; Runkle, Robert C.; Stave, Sean C.

    2013-12-01

    The gamma-ray spectrum of spent nuclear fuel in the 3- to 6-MeV energy range is important for active interrogation since emitted gamma rays emitted from nuclear decay are not expected to interfere with measurements in this energy region. There is, unfortunately, a dearth of empirical measurements from spent nuclear fuel in this region. This work is an initial attempt to partially ll this gap by presenting an analysis of gamma-ray spectra collected from a set of spent nuclear fuel sources using a high-purity germanium detector array. This multi-crystal array possesses a large collection volume, providing high energy resolution up to 16 MeV. The results of these measurements establish the continuum count-rate in the energy region between 3- and 6-MeV. Also assessed is the potential for peaks from passive emissions to interfere with peak measurements resulting from active interrogation delayed emissions. As one of the first documented empirical measurements of passive emissions from spent fuel for energies above 3 MeV, this work provides a foundation for active interrogation model validation and detector development.

  7. Simultaneous measurements of plutonium and uranium in spent-fuel dissolver solutions

    SciTech Connect

    Li, T.K.; Kuno, T.; Kitagawa, O.; Sato, S.; Kurosawa, A.; Kuno, Y.

    1997-11-01

    The authors have studied the isotope dilution gamma-ray spectrometry (IDGS) technique for simultaneous measurements of elemental concentrations and isotopic compositions for both plutonium and uranium in input spent-fuel dissolver solutions at a reprocessing plant. The technique under development includes both sample preparation and analysis methods. For simultaneous measurements of both plutonium and uranium, a critical issue is to develop a new method to keep both plutonium and uranium in the sample after they are separated from fission products. Furthermore, it is equally important to improve the analysis method so that the precision and accuracy of the plutonium analysis remain unaffected while uranium is retained in the sample. To keep both plutonium and uranium in the sample for simultaneous measurements, extraction chromatography is being studied and shows promise to achieve the goal of cosegregation of the plutonium and uranium. The technique uses U/TEVA{center_dot}Spec resin to separate fission products and recover both uranium and plutonium in the resin from dissolver solutions for subsequent measuring using high-resolution gamma-ray spectrometry. Owing to the fact that the U/Pu ratio is altered during the fission product separation phase, it is necessary to develop a method which could accurately correct for this effect. Such a method was developed using the unique decay properties of {sup 241}Pu to {sup 237}U and shows considerable promise in allowing for accurate determination of the {sup 235}U concentrations before the chemical extraction.

  8. The incentives and feasibility for direct measurement of spent nuclear fuel characteristics in the Federal Waste Management System

    SciTech Connect

    Not Available

    1989-08-01

    The purpose of this work is to assess the nature and extent of the need for direct measurements of spent fuel characteristics within the utility and federal portions of the waste management system, and to evaluate the capability and limitations of various measurement devices for meeting those needs. The need for direct measurement is evaluated relative to the alternative sources of the spent fuel characteristics data required for the safe and effective operation of the system. The results of this work are intended to support Federal Waste Management System (FWMS) planners by identifying the probable and potential requirements for direct measurements and for making related programmatic decisions based on the adequacy or development requirements for appropriate measurement technologies to support the needs of facility and equipment designers and operators. The designers and operators of the FWMS need to know the characteristics of the spent nuclear fuel (SNF) and related wastes that will be handled, processed, stored, transported and ultimately emplaced underground for final disposal. There are typically two basic sources of this needed information: (1) historical records of measurements made when the fuel was being fabricated or was producing energy; and (2) direct measurements made during handling prior to disposal. Historical records would include the design and fabrication records of the nuclear fuel assemblies and the subsequent utility records of reactor and core operations. 21 refs., 3 figs., 5 tabs.

  9. Spent Nuclear Fuel project, project management plan

    SciTech Connect

    Fuquay, B.J.

    1995-10-25

    The Hanford Spent Nuclear Fuel Project has been established to safely store spent nuclear fuel at the Hanford Site. This Project Management Plan sets forth the management basis for the Spent Nuclear Fuel Project. The plan applies to all fabrication and construction projects, operation of the Spent Nuclear Fuel Project facilities, and necessary engineering and management functions within the scope of the project

  10. Direct Measurement of U235 and Pu239 in Spent Fuel Rods with Gamma-Ray Mirrors

    SciTech Connect

    Ziock, Klaus-Peter; Alameda, J. B.; Brejnholt, N. F.; Decker, T. A.; Descalle, M. A.; Fernandez-Perea, M.; Hill, R. M.; Kisner, R. A.; Melin, A. M.; Patton, B. W.; Ruz, J.; Soufli, R.

    2013-09-30

    The amounts of fissile Pu and U in spent nuclear fuel are of primary concern to the safeguards community. In particular, there are issues when safeguards transitions from an item accountancy basis (such as fuel bundles) to a fissile material mass basis as occurs when spent fuel enters a reprocessing plant. Discrepancies occur because item accountancy requires estimating the content of fissile material using indirect techniques such as the fuel burn-up and item-level measurements of radiation emissions from fission by-products. Direct measurement of the fissile content by monitoring line emissions from fissile species themselves is impossible because the lines are much weaker than those emitted by shorter-lived isotopes in the fuel. The goal of this project is to develop a technique to directly measure these weaker lines despite the presence of overwhelming radiation from other isotopes. This is achieved by using gamma-ray mirrors as a narrow band-pass filter. The mirrors reflect only energies of interest toward a HPGe detector that is shielded from direct view of the spent fuel and its fierce emissions. This can significantly improve the reliability with which the mass of fissile material is tracked.

  11. Spent fuel characteristics & disposal considerations

    SciTech Connect

    Oversby, V.M.

    1996-06-01

    The fuel used in commercial nuclear power reactors is uranium, generally in the form of an oxide. The gas-cooled reactors developed in England use metallic uranium enclosed in a thin layer of Magnox. Since this fuel must be processed into a more stable form before disposal, we will not consider the characteristics of the Magnox spent fuel. The vast majority of the remaining power reactors in the world use uranium dioxide pellets in Zircaloy cladding as the fuel material. Reactors that are fueled with uranium dioxide generally use water as the moderator. If ordinary water is used, the reactors are called Light Water Reactors (LWR), while if water enriched in the deuterium isotope of hydrogen is used, the reactors are called Heavy Water reactors. The LWRs can be either pressurized reactors (PWR) or boiling water reactors (BWR). Both of these reactor types use uranium that has been enriched in the 235 isotope to about 3.5 to 4% total abundance. There may be minor differences in the details of the spent fuel characteristics for PWRs and BWRs, but for simplicity we will not consider these second-order effects. The Canadian designed reactor (CANDU) that is moderated by heavy water uses natural uranium without enrichment of the 235 isotope as the fuel. These reactors run at higher linear power density than LWRs and produce spent fuel with lower total burn-up than LWRs. Where these difference are important with respect to spent fuel management, we will discuss them. Otherwise, we will concentrate on spent fuel from LWRs.

  12. Expected total counts for the Self-Interrogation Neutron Resonance Densitometry measurements of spent nuclear fuel

    SciTech Connect

    Rossa, Riccardo; Borella, Alessandro; Van der Meer, Klaas; Labeau, Pierre-Etienne; Pauly, Nicolas

    2015-07-01

    The Self-Interrogation Neutron Resonance Densitometry (SINRD) is a passive neutron technique that aims at a direct quantification of {sup 239}Pu in spent fuel assemblies by measuring the attenuation of the neutron flux in the energy region close to the 0.3 eV resonance of {sup 239}Pu. The {sup 239}Pu mass is estimated by calculating the SINRD signature, that is the ratio between the neutron counts in the fast energy region and around the 0.3 eV resonance region. The SINRD measurement approach in this study consisted in introducing a small neutron detector in the central guide tube of a PWR 17x17 fuel assembly. In order to measure the neutron flux in the energy regions defined in the SINRD signature, different detector types were used. The response of a bare {sup 238}U fission chamber is considered for the determination of the fast neutron flux, while other thermal-epithermal detectors wrapped in neutron absorbers are envisaged to measure the neutron flux around the resonance region. This paper provides an estimation of the total neutron counts that can be achieved with the detector types proposed for the SINRD measurement. In the first section a set of detectors are evaluated in terms of total neutron counts and sensitivity to the {sup 239}Pu content, in order to identify the optimal measurement configuration for each detector type. Then a study is performed to increase the total neutron counts by increasing the detector size. The study shows that the highest total neutron counts are achieved by using either {sup 3}He or {sup 10}B proportional counters because of the high neutron efficiency of these detectors. However, the calculations indicate that the biggest contribution to the measurement uncertainty is due to the measurement of the fast neutron flux. Finally, similar sensitivity to the {sup 239}Pu content is obtained by using the different detector types for the measurement of the neutron flux close to the resonance region. Therefore, the total neutron counts

  13. Spent Nuclear Fuel Disposition

    SciTech Connect

    Wagner, John C.

    2016-05-22

    One interdisciplinary field devoted to achieving the end-state of used nuclear fuel (UNF) through reuse and/or permanent disposal. The reuse option aims to make use of the remaining energy content in UNF and reduce the amount of long-lived radioactive materials that require permanent disposal. The planned approach in the U.S., as well as in many other countries worldwide, is direct permanent disposal in a deep geologic repository. Used nuclear fuel is fuel that has been irradiated in a nuclear reactor to the point where it is no longer capable of sustaining operational objectives. The vast majority (by mass) of UNF is from electricity generation in commercial nuclear power reactors. Furthermore, the other main source of UNF in the U.S. is the Department of Energy’s (DOE) and other federal agencies’ operation of reactors in support of federal government missions, such as materials production, nuclear propulsion, research, testing, and training. Upon discharge from a reactor, UNF emits considerable heat from radioactive decay. Some period of active on-site cooling (e.g., 2 or more years) is typically required to facilitate efficient packaging and transportation to a disposition facility. Hence, the field of UNF disposition broadly includes storage, transportation and ultimate disposition. See also: Nuclear Fission (content/nuclear-fission/458400), Nuclear Fuels (/content/nuclear-fuels/458600), Nuclear Fuel Cycle (/content/nuclear-fuel-cycle/458500), Nuclear Fuels Reprocessing (/content/nuclear-fuels-reprocessing/458700), Nuclear Power (/content/nuclear-power/459600), Nuclear Reactor (/content/nuclear-reactor/460100), Radiation (/content/radiation/566300), and Radioactive Waste Management (/content/radioactive-waste-management/568900).

  14. Spent Nuclear Fuel Disposition

    DOE PAGES

    Wagner, John C.

    2016-05-22

    One interdisciplinary field devoted to achieving the end-state of used nuclear fuel (UNF) through reuse and/or permanent disposal. The reuse option aims to make use of the remaining energy content in UNF and reduce the amount of long-lived radioactive materials that require permanent disposal. The planned approach in the U.S., as well as in many other countries worldwide, is direct permanent disposal in a deep geologic repository. Used nuclear fuel is fuel that has been irradiated in a nuclear reactor to the point where it is no longer capable of sustaining operational objectives. The vast majority (by mass) of UNFmore » is from electricity generation in commercial nuclear power reactors. Furthermore, the other main source of UNF in the U.S. is the Department of Energy’s (DOE) and other federal agencies’ operation of reactors in support of federal government missions, such as materials production, nuclear propulsion, research, testing, and training. Upon discharge from a reactor, UNF emits considerable heat from radioactive decay. Some period of active on-site cooling (e.g., 2 or more years) is typically required to facilitate efficient packaging and transportation to a disposition facility. Hence, the field of UNF disposition broadly includes storage, transportation and ultimate disposition. See also: Nuclear Fission (content/nuclear-fission/458400), Nuclear Fuels (/content/nuclear-fuels/458600), Nuclear Fuel Cycle (/content/nuclear-fuel-cycle/458500), Nuclear Fuels Reprocessing (/content/nuclear-fuels-reprocessing/458700), Nuclear Power (/content/nuclear-power/459600), Nuclear Reactor (/content/nuclear-reactor/460100), Radiation (/content/radiation/566300), and Radioactive Waste Management (/content/radioactive-waste-management/568900).« less

  15. SEU43 fuel bundle shielding analysis during spent fuel transport

    SciTech Connect

    Margeanu, C. A.; Ilie, P.; Olteanu, G.

    2006-07-01

    The basic task accomplished by the shielding calculations in a nuclear safety analysis consist in radiation doses calculation, in order to prevent any risks both for personnel protection and impact on the environment during the spent fuel manipulation, transport and storage. The paper investigates the effects induced by fuel bundle geometry modifications on the CANDU SEU spent fuel shielding analysis during transport. For this study, different CANDU-SEU43 fuel bundle projects, developed in INR Pitesti, have been considered. The spent fuel characteristics will be obtained by means of ORIGEN-S code. In order to estimate the corresponding radiation doses for different measuring points the Monte Carlo MORSE-SGC code will be used. Both codes are included in ORNL's SCALE 5 programs package. A comparison between the considered SEU43 fuel bundle projects will be also provided, with CANDU standard fuel bundle taken as reference. (authors)

  16. Spent fuel data for waste storage programs

    SciTech Connect

    Greene, E M

    1980-09-01

    Data on LWR spent fuel were compiled for dissemination to participants in DOE-sponsored waste storage programs. Included are mechanical descriptions of the existing major types of LWR fuel assemblies, spent LWR fuel fission product inventories and decay heat data, and inventories of LWR spent fuel currently in storage, with projections of future quantities.

  17. Spent Fuel Test-Climax: technical measurements data management system description and data presentation

    SciTech Connect

    Carlson, R.C.

    1985-08-01

    The Spent Fuel Test-Climax (SFT-C) was located 420 m below surface in the Climax Stock granite on the Nevada Test Site. The test was conducted under the technical direction of the Lawrence Livermore National Laboratory (LLNL) as part of the Nevada Nuclear Waste Storage Investigations (NNWSI) for the US Department of Energy. Eleven canisters of spent nuclear reactor fuel were emplaced, along with six electrical simulators, in April-May 1980. The spent fuel canisters were retrieved and the electrical simulators de-energized in March-April 1983. During the test, just over 1000 MW-hr of thermal energy was deposited in the site, causing temperature changes 100{sup 0}C near the canisters, and about 5{sup 0} in the tunnels. More than 900 channels of geotechnical, seismological, and test status data were recorded on nearly continuous basis for about 3-1/2 years, ending in September 1983. Most geotechnical instrumentation was known to be temperature sensitive, and thus would require temperature compensation before interpretation. Accordingly, a 10-in. reel of digital tape was off-loaded and shipped to Livermore every 4 to 8 weeks, where the data were verified, organized into 45 one-million-word files, and temperature corrected. The purpose of this report is to document the receipt and processing of the data by LLNL Livermore personnel, present facts about the history of the instruments which may be important to the interpretation of the data, present the data themselves in graphical form for each instrument over its operating lifetime, document the forms and locations in which the data will be archived, and offer the data to the geotechnical community for future use in understanding and predicting the effects of the storage of heat-generating waste in hard rocks such as granite.

  18. Characteristics of spent nuclear fuel

    SciTech Connect

    Notz, K.J.

    1988-04-01

    The Office of Civilian Radioactive Waste Management (OCRWM) is responsible for the spent fuels and other wastes that will, or may, eventually be disposed of in a geological repository. The two major sources of these materials are commercial light-water reactor (LWR) spent fuel and immobilized high-level waste (HLW). Other wastes that may require long-term isolation include non-LWR spent fuels and miscellaneous sources such as activated metals. This report deals with spent fuels, but for completeness, the other sources are described briefly. Detailed characterizations are required for all of these potential repository wastes. These characteristics include physical, chemical, and radiological properties. The latter must take into account decay as a function of time. In addition, the present inventories and projected quantities of the various wastes are needed. This information has been assembled in a Characteristics Data Base which provides data in four formats: hard copy standard reports, menu-driven personal computer (PC) data bases, program-level PC data bases, and mainframe computer files. 5 refs., 3 figs., 4 tabs.

  19. Nondestructive verification and assay systems for spent fuels

    SciTech Connect

    Cobb, D.D.; Phillips, J.R.; Bosler, G.E.; Eccleston, G.W.; Halbig, J.K.; Hatcher, C.R.; Hsue, S.T.

    1982-04-01

    This is an interim report of a study concerning the potential application of nondestructive measurements on irradiated light-water-reactor (LWR) fuels at spent-fuel storage facilities. It describes nondestructive measurement techniques and instruments that can provide useful data for more effective in-plant nuclear materials management, better safeguards and criticality safety, and more efficient storage of spent LWR fuel. In particular, several nondestructive measurement devices are already available so that utilities can implement new fuel-management and storage technologies for better use of existing spent-fuel storage capacity. The design of an engineered prototype in-plant spent-fuel measurement system is approx. 80% complete. This system would support improved spent-fuel storage and also efficient fissile recovery if spent-fuel reprocessing becomes a reality.

  20. Analysis of experimental measurements of PWR fresh and spent fuel assemblies using Self-Interrogation Neutron Resonance Densitometry

    NASA Astrophysics Data System (ADS)

    LaFleur, Adrienne M.; Menlove, Howard O.

    2015-05-01

    Self-Interrogation Neutron Resonance Densitometry (SINRD) is a new NDA technique that was developed at Los Alamos National Laboratory (LANL) to improve existing nuclear safeguards measurements for LWR fuel assemblies. The SINRD detector consists of four fission chambers (FCs) wrapped with different absorber filters to isolate different parts of the neutron energy spectrum and one ion chamber (IC) to measure the gross gamma rate. As a result, two different techniques can be utilized using the same SINRD detector unit and hardware. These techniques are the Passive Neutron Multiplication Counter (PNMC) method and the SINRD method. The focus of the work described in this paper is the analysis of experimental measurements of fresh and spent PWR fuel assemblies that were performed at LANL and the Korea Atomic Energy Research Institute (KAERI), respectively, using the SINRD detector. The purpose of these experiments was to assess the following capabilities of the SINRD detector: 1) reproducibility of measurements to quantify systematic errors, 2) sensitivity to water gap between detector and fuel assembly, 3) sensitivity and penetrability to the removal of fuel rods from the assembly, and 4) use of PNMC/SINRD ratios to quantify neutron multiplication and/or fissile content. The results from these simulations and measurements provide valuable experimental data that directly supports safeguards research and development (R&D) efforts on the viability of passive neutron NDA techniques and detector designs for partial defect verification of spent fuel assemblies.

  1. Direct measurement of 235U in spent fuel rods with Gamma-ray mirrors

    SciTech Connect

    Ruz, J.; Brejnholt, N. F.; Alameda, J. B.; Decker, T. A.; Descalle, M. A.; Fernandez-Perea, M.; Hill, R. M.; Kisner, R. A.; Melin, A. M.; Patton, B. W.; Soufli, R.; Ziock, K.; Pivovaroff, M. J.

    2015-12-22

    We report here that direct measurement of plutonium and uranium X-rays and gamma-rays is a highly desirable nondestructive analysis method for the use in reprocessing fuel environments. The high background and intense radiation from spent fuel make direct measurements difficult to implement since the relatively low activity of uranium and plutonium is masked by the high activity from fission products. To overcome this problem, we make use of a grazing incidence optic to selectively reflect Kα and Kβ fluorescence of Special Nuclear Materials (SNM) into a high-purity position-sensitive germanium detector and obtain their relative ratios.

  2. Spent-fuel storage requirements

    NASA Astrophysics Data System (ADS)

    1982-06-01

    Spent fuel storage requirements, as projected through the year 2000 for U.S. LWRs, were calculated using information supplied by the utilities reflecting plant status as of December 31, 1981. Projections through the year 2000 combined fuel discharge projections of the utilities with the assumed discharges of typical reactors required to meet the nuclear capacity of 165 GWe projected by the Energy Information Administration for the year 2000. Three cases were developed and are summarized. A reference case, or maximum at-reactor capacity case, assumes that all reactor storage pools are increased to their maximum capacities as estimated by the utilities for spent fuel storage utilizing currently licensed technologies. The reference case assumes no transshipments between pools except as current licensed by the Nuclear Regulatory Commission. This case identifies an initial requirement for 13 MTU of additional storage in 1984, and a cumulative requirement for 14,490 MTU additional storage in the year 2000.

  3. Geomechanics of the Spent Fuel Test: Climax

    SciTech Connect

    Wilder, D.G.; Yow, J.L. Jr.

    1987-07-01

    Three years of geomechanical measurements were made at the Spent Fuel Test-Climax (SFT-C) 1400 feet underground in fractured granitic rock. Heating of the rock mass resulted from emplacement of spent fuel as well as the heating by electrical heaters. Cooldown of the rock occurred after the spent fuel was removed and the heaters were turned off. The measurements program examines both gross and localized responses of the rock mass to thermal loading, to evaluate the thermomechanical response of sheared and fractured rock with that of relatively unfractured rock, to compare the magnitudes of displacements during mining with those induced by extensive heating of the rock mass, and to check assumptions regarding symmetry and damaged zones made in numerical modeling of the SFT-C. 28 refs., 113 figs., 10 tabs.

  4. Nuclear Resonance Fluorescence to Measure Plutonium Mass in Spent Nuclear Fuel

    SciTech Connect

    Ludewigt, Bernhard A; Quiter, Brian J.; Ambers, Scott D.

    2011-01-14

    The Next Generation Safeguard Initiative (NGSI) of the U.S Department of Energy is supporting a multi-lab/university collaboration to quantify the plutonium (Pu) mass in spent nuclear fuel (SNF) assemblies and to detect the diversion of pins with non-destructive assay (NDA) methods. The following 14 NDA techniques are being studied: Delayed Neutrons, Differential Die-Away, Differential Die-Away Self-Interrogation, Lead Slowing Down Spectrometer, Neutron Multiplicity, Passive Neutron Albedo Reactivity, Total Neutron (Gross Neutron), X-Ray Fluorescence, {sup 252}Cf Interrogation with Prompt Neutron Detection, Delayed Gamma, Nuclear Resonance Fluorescence, Passive Prompt Gamma, Self-integration Neutron Resonance Densitometry, and Neutron Resonance Transmission Analysis. Understanding and maturity of the techniques vary greatly, ranging from decades old, well-understood methods to new approaches. Nuclear Resonance Fluorescence (NRF) is a technique that had not previously been studied for SNF assay or similar applications. Since NRF generates isotope-specific signals, the promise and appeal of the technique lies in its potential to directly measure the amount of a specific isotope in an SNF assay target. The objectives of this study were to design and model suitable NRF measurement methods, to quantify capabilities and corresponding instrumentation requirements, and to evaluate prospects and the potential of NRF for SNF assay. The main challenge of the technique is to achieve the sensitivity and precision, i.e., to accumulate sufficient counting statistics, required for quantifying the mass of Pu isotopes in SNF assemblies. Systematic errors, considered a lesser problem for a direct measurement and only briefly discussed in this report, need to be evaluated for specific instrument designs in the future. Also, since the technical capability of using NRF to measure Pu in SNF has not been established, this report does not directly address issues such as cost, size

  5. SFCOMPO 2.0 - A relational database of spent fuel isotopic measurements, reactor operational histories, and design data

    NASA Astrophysics Data System (ADS)

    Michel-Sendis, Franco; Martinez-González, Jesus; Gauld, Ian

    2017-09-01

    SFCOMPO-2.0 is a database of experimental isotopic concentrations measured in destructive radiochemical analysis of spent nuclear fuel (SNF) samples. The database includes corresponding design description of the fuel rods and assemblies, relevant operating conditions and characteristics of the host reactors necessary for modelling and simulation. Aimed at establishing a thorough, reliable, and publicly available resource for code and data validation of safety-related applications, SFCOMPO-2.0 is developed and maintained by the OECD Nuclear Energy Agency (NEA). The SFCOMPO-2.0 database is a Java application which is downloadable from the NEA website.

  6. Measurements and Characterization of Neutron and Gamma Dose Quantities in the Vicinity of an Independent Spent Fuel Storage Installation

    SciTech Connect

    Darois, E.L.; Keefer, D.G.; Plazeski, P.E.; Connell, J.

    2006-07-01

    As part of the decommissioning of the Maine Yankee Atomic Power Company (MYAPCo) nuclear power plant, the spent nuclear fuel is being temporarily stored in a dry cask storage facility on a portion of the original licensed property. Each of the spent nuclear fuel (SNF) storage casks hold approximately 25 spent fuel assemblies. Additional storage casks for the greater-than-Class C waste (GTCC) are also used. This waste is contained in 64 casks (60 SNF, 4 GTCC), each of which contain a substantial amount of concrete for shielding and structural purposes. The vertical concrete casks (VCCs) are typically separated by a distance of 4 and 6 feet. The storage casks are effective personnel radiation shields for most of the gamma and neutron radiation emitted from the fuel. However measurable gamma and neutron radiation levels are present in the vicinity of the casks. In order to establish a controlled area boundary around the facility such that a member of the public annual dose level of 0.25-mSv could be demonstrated, measurements of gamma and neutron dose equivalents were conducted. External gamma exposure rates were measured with a Pressurized Ion Chamber (PIC). Neutron absorbed dose and dose equivalent rates were measured with a Rossi-type tissue equivalent proportional counter (TEPC). Both gamma and neutron measurements were made at increasing distances from the facility as well as at a background location. The results of the measurements show that the distance to the 0.25-mSv per year boundary for 100% occupancy conditions varies from 321 feet to 441 feet from the geometric center of the storage pads, depending on the direction from the pad. For the TEPC neutron measurements, the average quality factor from the facilities was approximately 7.4. This quality factor compares well with the average quality factor of 7.6 that was measured during a calibration performed with a bare Cf-252 source. (authors)

  7. Spent fuel receipt scenarios study

    SciTech Connect

    Ballou, L.B.; Montan, D.N.; Revelli, M.A.

    1990-09-01

    This study reports on the results of an assignment from the DOE Office of Civilian Radioactive Waste Management to evaluate of the effects of different scenarios for receipt of spent fuel on the potential performance of the waste packages in the proposed Yucca Mountain high-level waste repository. The initial evaluations were performed and an interim letter report was prepared during the fall of 1988. Subsequently, the scope of work was expanded and additional analyses were conducted in 1989. This report combines the results of the two phases of the activity. This study is a part of a broader effort to investigate the options available to the DOE and the nuclear utilities for selection of spent fuel for acceptance into the Federal Waste Management System for disposal. Each major element of the system has evaluated the effects of various options on its own operations, with the objective of providing the basis for performing system-wide trade-offs and determining an optimum acceptance scenario. Therefore, this study considers different scenarios for receipt of spent fuel by the repository only from the narrow perspective of their effect on the very-near-field temperatures in the repository following permanent closure. This report is organized into three main sections. The balance of this section is devoted to a statement of the study objective, a summary of the assumptions. The second section of the report contains a discussion of the major elements of the study. The third section summarizes the results of the study and draws some conclusions from them. The appendices include copies of the waste acceptance schedule and the existing and projected spent fuel inventory that were used in the study. 10 refs., 27 figs.

  8. Status of the nuclear measurement stations for the process control of spent fuel reprocessing at AREVA NC/La Hague

    SciTech Connect

    Eleon, Cyrille; Passard, Christian; Hupont, Nicolas; Estre, Nicolas; Battel, Benjamin; Doumerc, Philippe; Dupuy, Thierry; Batifol, Marc; Grassi, Gabriele

    2015-07-01

    Nuclear measurements are used at AREVA NC/La Hague for the monitoring of spent fuel reprocessing. The process control is based on gamma-ray spectroscopy, passive neutron counting and active neutron interrogation, and gamma transmission measurements. The main objectives are criticality and safety, online process monitoring, and the determination of the residual fissile mass and activities in the metallic waste remained after fuel shearing and dissolution (empty hulls, grids, end pieces), which are put in radioactive waste drums before compaction. The whole monitoring system is composed of eight measurement stations which will be described in this paper. The main measurement stations no. 1, 3 and 7 are needed for criticality control. Before fuel element shearing for dissolution, station no. 1 allows determining the burn-up of the irradiated fuel by gamma-ray spectroscopy with HP Ge (high purity germanium) detectors. The burn-up is correlated to the {sup 137}Cs and {sup 134}Cs gamma emission rates. The fuel maximal mass which can be loaded in one bucket of the dissolver is estimated from the lowest burn-up fraction of the fuel element. Station no. 3 is dedicated to the control of the correct fuel dissolution, which is performed with a {sup 137}Cs gamma ray measurement with a HP Ge detector. Station no. 7 allows estimating the residual fissile mass in the drums filled with the metallic residues, especially in the hulls, from passive neutron counting (spontaneous fission and alpha-n reactions) and active interrogation (fission prompt neutrons induced by a pulsed neutron generator) with proportional {sup 3}He detectors. The measurement stations have been validated for the reprocessing of Uranium Oxide (UOX) fuels with a burn-up rate up to 60 GWd/t. This paper presents a brief overview of the current status of the nuclear measurement stations. (authors)

  9. U and Pu Gamma-Ray Measurements of Spent Fuel Using a Gamma-Ray Mirror Band-Pass Filter

    SciTech Connect

    Ziock, Klaus-Peter; Alameda, J.B.; Brejnholt, N.F.; Decker, T.A.; Descalle, M.A.; Fernandez-Perea, M.; Hill, R.M.; Kisner, R.A.; Melin, A.M.; Patton, B.W.; Ruz, J.; Soufli, R.; Pivovaroff, M.J.

    2014-01-01

    Abstract. We report on the use of grazing incidence gamma-ray mirrors to serve as a narrow band-pass filter for advanced non-destructive analysis (NDA) of spent nuclear fuel. The purpose of the mirrors is to limit the radiation reaching a HPGe detector to narrow spectral bands around characteristic emission lines from fissile isotopes in the fuel. This overcomes the normal rate issues when performing gamma-ray NDA measurements. In a proof-of-concept experiment, a set of simple flat gamma-ray mirrors were used to directly observe the atomic florescence lines from U and Pu from spent fuel pins with the detector located in a shirt-sleeve environment. The mirrors, consisting of highly polished silicon substrates deposited with WC/SiC multilayer coatings, successfully deflected the lines of interest while the intense primary radiation beam from the fuel was blocked by a lead beam stop. The gamma-ray multilayer coatings that make the mirrors work at the gamma-ray energies used here (~ 100 keV) have been experimentally tested at energies as high as 645 keV, indicating that direct observation of nuclear emission lines from 239Pu should be possible with an appropriately designed optic and shielding configuration.

  10. Measurements on spent-fuel assemblies at Arkansas Nuclear One using the Fork system. Final report, January 1995

    SciTech Connect

    Ewing, R.I.; Bronowski, D.R.; Bosler, G.E.; Siebelist, R.; Priore, J.; Hansford, C.H.; Sullivan, S.

    1997-03-01

    The Fork measurement system has been used to examine spent-fuel assemblies at the two reactors of Arkansas Nuclear One, operated by Entergy Operations, Inc. The Unit 1 reactor is a Babcock and Wilcox (B and W) design, and the Unit 2 reactor is a Combustion Engineering (CE) design. The neutron and gamma-ray emissions from individual spent-fuel assemblies were measured in the storage pools by raising each assembly pathway out of the storage rack and performing a measurement near the center of the assembly. The overall accuracy of the measurements after corrections is about 2%. Thirty-four assemblies were examined at Unit 1, and forty-one assemblies at Unit 2. The average deviation of the burnup measurements from the calibration was 3.0% at Unit 1 and 3.5% at Unit 2, indicating 2 to 3% random variation among the reactor records. There was no indication of clearly anomalous assemblies. Axial Scans of the variation in neutron and gamma ray emission were obtained by collecting data at several locations along the length of three assemblies at Unit 2. Two of these assemblies were nonstandard in that each contained a small neutron source. The sources were detected by the axial scans. The test program was a cooperative effort involving Sandia National Laboratories, Los Alamos National Laboratory, Entergy Operations, Inc., the Electric Power Research Institute, and the Office of Civilian Radioactive Waste Management of the US Department of Energy.

  11. Measurement and Analysis Plan for Investigation of Spent-Fuel Assay Using Lead Slowing-Down Spectroscopy

    SciTech Connect

    Smith, Leon E.; Haas, Derek A.; Gavron, Victor A.; Imel, G. R.; Ressler, Jennifer J.; Bowyer, Sonya M.; Danon, Y.; Beller, D.

    2009-09-25

    Under funding from the Department of Energy Office of Nuclear Energy’s Materials, Protection, Accounting, and Control for Transmutation (MPACT) program (formerly the Advanced Fuel Cycle Initiative Safeguards Campaign), Pacific Northwest National Laboratory (PNNL) and Los Alamos National Laboratory (LANL) are collaborating to study the viability of lead slowing-down spectroscopy (LSDS) for spent-fuel assay. Based on the results of previous simulation studies conducted by PNNL and LANL to estimate potential LSDS performance, a more comprehensive study of LSDS viability has been defined. That study includes benchmarking measurements, development and testing of key enabling instrumentation, and continued study of time-spectra analysis methods. This report satisfies the requirements for a PNNL/LANL deliverable that describes the objectives, plans and contributing organizations for a comprehensive three-year study of LSDS for spent-fuel assay. This deliverable was generated largely during the LSDS workshop held on August 25-26, 2009 at Rensselaer Polytechnic Institute (RPI). The workshop itself was a prominent milestone in the FY09 MPACT project and is also described within this report.

  12. Transportation accident scenarios for commercial spent fuel

    SciTech Connect

    Wilmot, E L

    1981-02-01

    A spectrum of high severity, low probability, transportation accident scenarios involving commercial spent fuel is presented together with mechanisms, pathways and quantities of material that might be released from spent fuel to the environment. These scenarios are based on conclusions from a workshop, conducted in May 1980 to discuss transportation accident scenarios, in which a group of experts reviewed and critiqued available literature relating to spent fuel behavior and cask response in accidents.

  13. Spent nuclear fuel reprocessing modeling

    SciTech Connect

    Tretyakova, S.; Shmidt, O.; Podymova, T.; Shadrin, A.; Tkachenko, V.; Makeyeva, I.; Tkachenko, V.; Verbitskaya, O.; Schultz, O.; Peshkichev, I.

    2013-07-01

    The long-term wide development of nuclear power requires new approaches towards the realization of nuclear fuel cycle, namely, closed nuclear fuel cycle (CNFC) with respect to fission materials. Plant nuclear fuel cycle (PNFC), which is in fact the reprocessing of spent nuclear fuel unloaded from the reactor and the production of new nuclear fuel (NF) at the same place together with reactor plant, can be one variant of CNFC. Developing and projecting of PNFC is a complicated high-technology innovative process that requires modern information support. One of the components of this information support is developed by the authors. This component is the programme conducting calculations for various variants of process flow sheets for reprocessing SNF and production of NF. Central in this programme is the blocks library, where the blocks contain mathematical description of separate processes and operations. The calculating programme itself has such a structure that one can configure the complex of blocks and correlations between blocks, appropriate for any given flow sheet. For the ready sequence of operations balance calculations are made of all flows, i.e. expenses, element and substance makeup, heat emission and radiation rate are determined. The programme is open and the block library can be updated. This means that more complicated and detailed models of technological processes will be added to the library basing on the results of testing processes using real equipment, in test operating mode. The development of the model for the realization of technical-economic analysis of various variants of technologic PNFC schemes and the organization of 'operator's advisor' is expected. (authors)

  14. Radioactivity of spent TRIGA fuel

    SciTech Connect

    Usang, M. D. Nabil, A. R. A.; Alfred, S. L.; Hamzah, N. S.; Abi, M. J. B.; Rawi, M. Z. M.; Abu, M. P.

    2015-04-29

    Some of the oldest TRIGA fuel in the Malaysian Reaktor TRIGA PUSPATI (RTP) is approaching the limit of its end of life with burn-up of around 20%. Hence it is prudent for us to start planning on the replacement of the fuel in the reactor and other derivative activities associated with it. In this regard, we need to understand all of the risk associated with such operation and one of them is to predict the radioactivity of the fuel, so as to estimate the safety of our working conditions. The radioactivity of several fuels are measured and compared with simulation results to confirm the burnup levels of the selected fuels. The radioactivity measurement are conducted inside the water tank to reduce the risk of exposure and in this case the detector wrapped in plastics are lowered under water. In nuclear power plant, the general practice was to continuously burn the fuel. In research reactor, most operations are based on the immediate needs of the reactor and our RTP for example operate periodically. By integrating the burnup contribution for each core configuration, we simplify the simulation of burn up for each core configuration. Our results for two (2) fuel however indicates that the dose from simulation underestimate the actual dose from our measurements. Several postulates are investigated but the underlying reason remain inconclusive.

  15. Radioactivity of spent TRIGA fuel

    NASA Astrophysics Data System (ADS)

    Usang, M. D.; Nabil, A. R. A.; Alfred, S. L.; Hamzah, N. S.; Abi, M. J. B.; Rawi, M. Z. M.; Abu, M. P.

    2015-04-01

    Some of the oldest TRIGA fuel in the Malaysian Reaktor TRIGA PUSPATI (RTP) is approaching the limit of its end of life with burn-up of around 20%. Hence it is prudent for us to start planning on the replacement of the fuel in the reactor and other derivative activities associated with it. In this regard, we need to understand all of the risk associated with such operation and one of them is to predict the radioactivity of the fuel, so as to estimate the safety of our working conditions. The radioactivity of several fuels are measured and compared with simulation results to confirm the burnup levels of the selected fuels. The radioactivity measurement are conducted inside the water tank to reduce the risk of exposure and in this case the detector wrapped in plastics are lowered under water. In nuclear power plant, the general practice was to continuously burn the fuel. In research reactor, most operations are based on the immediate needs of the reactor and our RTP for example operate periodically. By integrating the burnup contribution for each core configuration, we simplify the simulation of burn up for each core configuration. Our results for two (2) fuel however indicates that the dose from simulation underestimate the actual dose from our measurements. Several postulates are investigated but the underlying reason remain inconclusive.

  16. Nondestructive verification and assay systems for spent fuels. Technical appendixes

    SciTech Connect

    Cobb, D.D.; Phillips, J.R.; Baker, M.P.

    1982-04-01

    Six technical appendixes are presented that provide important supporting technical information for the study of the application of nondestructive measurements to spent-fuel storage. Each appendix addresses a particular technical subject in a reasonably self-contained fashion. Appendix A is a comparison of spent-fuel data predicted by reactor operators with measured data from reprocessors. This comparison indicates a rather high level of uncertainty in previous burnup calculations. Appendix B describes a series of nondestructive measurements at the GE-Morris Operation Spent-Fuel Storage Facility. This series of experiments successfully demonstrated a technique for reproducible positioning of fuel assemblies for nondestructive measurement. The experimental results indicate the importance of measuring the axial and angular burnup profiles of irradiated fuel assemblies for quantitative determination of spent-fuel parameters. Appendix C is a reasonably comprehensive bibliography of reports and symposia papers on spent-fuel nondestructive measurements to April 1981. Appendix D is a compendium of spent-fuel calculations that includes isotope production and depletion calculations using the EPRI-CINDER code, calculations of neutron and gamma-ray source terms, and correlations of these sources with burnup and plutonium content. Appendix E describes the pulsed-neutron technique and its potential application to spent-fuel measurements. Although not yet developed, the technique holds the promise of providing separate measurements of the uranium and plutonium fissile isotopes. Appendix F describes the experimental program and facilities at Los Alamos for the development of spent-fuel nondestructive measurement systems. Measurements are reported showing that the active neutron method is sensitive to the replacement of a single fuel rod with a dummy rod in an unirradiated uranium fuel assembly.

  17. Thermal analysis of thermo-gravimetric measurements of spent nuclear fuel oxidation rates

    SciTech Connect

    Cramer, E.R.

    1997-10-09

    A detailed thermal analysis was completed of the sample temperatures in the Thermo-Gravimetric Analysis (TGA) system used to measure irradiated N Reactor fuel oxidation rates. Sample temperatures during the oxidation process did not show the increase which was postulated as a result of the exothermic reactions. The analysis shows the axial conduction of heat in the sample holder effectively removes the added heat and only a very small, i.e., <10 C, increase in temperature is calculated. A room temperature evaporation test with water showed the sample thermocouple sensitivity to be more than adequate to account for a temperature change of approximately 5 C. Therefore, measured temperatures in the TGA are within approximately 10 C of the actual sample temperatures and no adjustments to reported data to account for the heat input from the oxidation process are necessary.

  18. Expected count rate for the Self- Interrogation Neutron Resonance Densitometry measurements of spent nuclear fuel

    SciTech Connect

    Rossa, Riccardo; Labeau, Pierre-Etienne; Pauly, Nicolas

    2015-07-01

    The Self-Interrogation Neutron Resonance Densitometry (SINRD) is a passive neutron technique that aims at a direct quantification of {sup 239}Pu in the fuel assemblies by measuring the attenuation of the neutron flux in the energy region close to the 0.3 eV resonance of {sup 239}Pu. The {sup 239}Pu mass is estimated by calculating the SINRD signature, that is the ratio between the neutron flux integrated over the fast energy region and around the 0.3 eV resonance region. The SINRD measurement approach considered in this study consists in introducing a small neutron detector in the central guide tube of a PWR 17x17 fuel assembly. In order to measure the neutron flux in the energy regions defined in the SINRD signature, different detector types are used. The response of a bare {sup 238}U fission chamber is considered for the determination of the fast neutron flux, while other thermal-epithermal detectors wrapped in neutron absorbers are envisaged to measure the neutron flux around the resonance region. This paper provides an estimation of the count rate that can be achieved with the detector types proposed for the SINRD measurement. In the first section a set of detectors are evaluated in terms of count rate and sensitivity to the {sup 239}Pu content, in order to identify the optimal measurement configuration for each detector type. Then a study is performed to increase the count rate by increasing the detector size. The study shows that the highest count rate is achieved by using either {sup 3}He or {sup 10}B proportional counters because of the high neutron efficiency of these detectors. However, the calculations indicate that the biggest contribution to the measurement uncertainty is due to the measurement of the fast neutron flux. Finally, similar sensitivity to the {sup 239}Pu content is obtained by using the different detector types for the measurement of the neutron flux close to the resonance region. Therefore, the count rate associated to each detector type

  19. Spent Nuclear Fuel (SNF) Project Execution Plan

    SciTech Connect

    LEROY, P.G.

    2000-11-03

    The Spent Nuclear Fuel (SNF) Project supports the Hanford Site Mission to cleanup the Site by providing safe, economic, environmentally sound management of Site spent nuclear fuel in a manner that reduces hazards by staging it to interim onsite storage and deactivates the 100 K Area facilities.

  20. Spent Nuclear Fuel Vibration Integrity Study

    SciTech Connect

    Wang, Jy-An John; Wang, Hong; Jiang, Hao; Yan, Yong; Bevard, Bruce Balkcom

    2016-01-01

    The objective of this research is to collect dynamic experimental data on spent nuclear fuel (SNF) under simulated transportation environments using the Cyclic Integrated Reversible-Bending Fatigue Tester (CIRFT), the hot-cell testing technology developed at Oak Ridge National Laboratory (ORNL). The collected CIRFT data will be utilized to support ongoing spent fuel modeling activities, and support SNF transportation related licensing issues. Recent testing to understand the effects of hydride reorientation on SNF vibration integrity is also being evaluated. CIRFT results have provided insight into the fuel/clad system response to transportation related loads. The major findings of CIRFT on the HBU SNF are as follows: SNF system interface bonding plays an important role in SNF vibration performance, Fuel structure contributes to the SNF system stiffness, There are significant variations in stress and curvature of SNF systems during vibration cycles resulting from segment pellets and clad interaction, and SNF failure initiates at the pellet-pellet interface region and appears to be spontaneous. Because of the non-homogeneous composite structure of the SNF system, finite element analyses (FEA) are needed to translate the global moment-curvature measurement into local stress-strain profiles. The detailed mechanisms of the pellet-pellet and pellet-clad interactions and the stress concentration effects at the pellet-pellet interface cannot be readily obtained directly from a CIRFT system measurement. Therefore, detailed FEA is used to understand the global test response, and that data will also be presented.

  1. ATR Spent Fuel Options Study

    SciTech Connect

    Connolly, Michael James; Bean, Thomas E.; Brower, Jeffrey O.; Luke, Dale E.; Patterson, M. W.; Robb, Alan K.; Sindelar, Robert; Smith, Rebecca E.; Tonc, Vincent F.; Tripp, Julia L.; Winston, Philip L.

    2017-01-01

    The Advanced Test Reactor (ATR) is a materials and fuels test nuclear reactor that performs irradiation services for the U.S. Department of Energy (DOE) Office of Nuclear Energy (NE), Naval Reactors, the National Nuclear Security Administration (NNSA), and other research programs. ATR achieved initial criticality in 1967 and is expected to operate in support of needed missions until the year 2050 or beyond. It is anticipated that ATR will generate approximately 105 spent nuclear fuel (SNF) elements per year through the year 2050. Idaho National Laboratory (INL) currently stores 2,008 ATR SNF elements in dry storage, 976 in wet storage, and expects to have 1,000 elements in wet storage before January 2017. A capability gap exists at INL for long-term (greater than the year 2050) management, in compliance with the Idaho Settlement Agreement (ISA), of ATR SNF until a monitored retrievable geological repository is open. INL has significant wet and dry storage capabilities that are owned by the DOE Office of Environmental Management (EM) and operated and managed by Fluor Idaho, which include the Idaho Nuclear Technology and Engineering Center’s (INTEC’s) CPP-666, CPP-749, and CPP-603. In addition, INL has other capabilities owned by DOE-NE and operated and managed by Battelle Energy Alliance, LLC (BEA), which are located at the Materials and Fuel Complex (MFC). Additional storage capabilities are located on the INL Site at the Naval Reactors Facility (NRF). Current INL SNF management planning, as defined in the Fluor Idaho contract, shows INTEC dry fuel storage, which is currently used for ATR SNF, will be nearly full after transfer of an additional 1,000 ATR SNF from wet storage. DOE-NE tasked BEA with identifying and analyzing options that have the potential to fulfill this capability gap. BEA assembled a team comprised of SNF management experts from Fluor Idaho, Savannah River Site (SRS), INL/BEA, and the MITRE Corp with an objective of developing and analyzing

  2. Rack for storing spent nuclear fuel elements

    DOEpatents

    Rubinstein, Herbert J.; Clark, Philip M.; Gilcrest, James D.

    1978-06-20

    A rack for storing spent nuclear fuel elements in which a plurality of aligned rows of upright enclosures of generally square cross-sectional areas contain vertically disposed fuel elements. The enclosures are fixed at the lower ends thereof to a base. Pockets are formed between confronting walls of adjacent enclosures for receiving high absorption neutron absorbers, such as Boral, cadmium, borated stainless steel and the like for the closer spacing of spent fuel elements.

  3. Thermal Cooling Limits of Sbotaged Spent Fuel Pools

    SciTech Connect

    Dr. Thomas G. Hughes; Dr. Thomas F. Lin

    2010-09-10

    To develop the understanding and predictive measures of the post “loss of water inventory” hazardous conditions as a result of the natural and/or terrorist acts to the spent fuel pool of a nuclear plant. This includes the thermal cooling limits to the spent fuel assembly (before the onset of the zircaloy ignition and combustion), and the ignition, combustion, and the subsequent propagation of zircaloy fire from one fuel assembly to others

  4. Development of self-interrogation neutron resonance densitometry (SINRD) to measure U-235 and Pu-239 content in a PWR spent fuel assembly

    SciTech Connect

    Lafleur, Adrienne M; Charlton, William S; Menlove, Howard O; Swinhoe, Martyn T

    2009-01-01

    The use of Self-Interrogation Neutron Resonance Densitometry (SINRD) to measure the {sup 235}U and {sup 239}Pu content in a PWR spent fuel assembly was investigated via Monte Carlo N-Particle eXtended transport code (MCNPX) simulations. The sensitivity of SINRD is based on using the same fissile materials in the fission chambers as are present in the fuel because the effect of resonance absorption lines in the transmitted flux is amplified by the corresponding (n, f) reaction peaks in fission chamber. These simulations utilize the {sup 244}Cm spontaneous fission neutrons to self-interrogate the fuel pins. The amount of resonance absorption of these neutrons in the fuel can be measured using {sup 235}U and {sup 239}Pu fission chambers placed adjacent to the assembly. We used ratios of different fission chambers to reduce the sensitivity of the measurements to extraneous material present in fuel. The development of SINRD to measure the fissile content in spent fuel is of great importance to the improvement of nuclear safeguards and material accountability. Future work includes the use of this technique to measure the fissile content in FBR spent fuel and heavy metal product from reprocessing methods.

  5. Safeguards aspects of spent-fuel management

    SciTech Connect

    Richter, B.; Stein, G.; Remagen, H.H.; Weh, R.

    1989-11-01

    In the Federal Republic of Germany, the concept of spent-fuel management is based on a closed fuel cycle that has the following principal features: (1) intermediate dry storage of spent fuel; (2) reprocessing; (3) thermal recycling of unconsumed nuclear material; and (4) conditioning and final disposal of radioactive waste. Complementary to this concept, methods and techniques for the direct final disposal of spent fuel are under development, including investigations of licensing issues. Furthermore, a licensing procedure is under way for the construction of a pilot conditioning plant close to the Gorleben dry storage facility. Apart from operational safety and environmental protection, the issue of international safeguards is of paramount interest. This paper discusses safeguards aspects of spent-fuel management related to direct final disposal.

  6. Apparatus for shearing spent nuclear fuel assemblies

    DOEpatents

    Weil, Bradley S.; Metz, III, Curtis F.

    1980-01-01

    A method and apparatus are described for shearing spent nuclear fuel assemblies of the type comprising an array of fuel pins disposed within an outer metal shell or shroud. A spent fuel assembly is first compacted in a known manner and then incrementally sheared using fixed and movable shear blades having matched laterally projecting teeth which slidably intermesh to provide the desired shearing action. Incremental advancement of the fuel assembly after each shear cycle is limited to a distance corresponding to the lateral projection of the teeth to ensure fuel assembly breakup into small uniform segments which are amenable to remote chemical processing.

  7. Spent Fuel Background Report Volume I

    SciTech Connect

    Abbott, D.

    1994-03-01

    This report is an overview of current spent nuclear fuel management in the DOE complex. Sources of information include published literature, internal DOE documents, interviews with site personnel, and information provided by individual sites. Much of the specific information on facilities and fuels was provided by the DOE sites in response to the questionnaire for data for spent fuels and facilities data bases. This information is as accurate as is currently available, but is subject to revision pending results of further data calls. Spent fuel is broadly classified into three categories: (a) production fuels, (b) special fuels, and (c) naval fuels. Production fuels, comprising about 80% of the total inventory, are those used at Hanford and Savannah River to produce nuclear materials for defense. Special fuels are those used in a wide variety of research, development, and testing activities. Special fuels include fuel from DOE and commercial reactors used in research activities at DOE sites. Naval fuels are those developed and used for nuclear-powered naval vessels and for related research and development. Given the recent DOE decision to curtail reprocessing, the topic of main concern in the management of spent fuel is its storage. Of the DOE sites that have spent nuclear fuel, the vast majority is located at three sites-Hanford, INEL, and Savannah River. Other sites with spent fuel include Oak Ridge, West Valley, Brookhaven, Argonne, Los Alamos, and Sandia. B&W NESI Lynchburg Technology Center and General Atomics are commercial facilities with DOE fuel. DOE may also receive fuel from foreign research reactors, university reactors, and other commercial and government research reactors. Most DOE spent fuel is stored in water-filled pools at the reactor facilities. Currently an engineering study is being performed to determine the feasibility of using dry storage for DOE-owned spent fuel currently stored at various facilities. Delays in opening the deep geologic

  8. Advances in HTGR spent fuel treatment technology

    SciTech Connect

    Holder, N.D.; Lessig, W.S.

    1984-08-01

    GA Technologies, Inc. has been investigating the burning of spent reactor graphite under Department of Energy sponsorship since 1969. Several deep fluidized bed burners have been used at the GA pilot plant to develop graphite burning techniques for both spent fuel recovery and volume reduction for waste disposal. Since 1982 this technology has been extended to include more efficient circulating bed burners. This paper includes updates on high-temperature gas-cooled reactor fuel cycle options and current results of spent fuel treatment testing for fluidized and advanced circulating bed burners.

  9. Spent Nuclear Fuel Project dose management plan

    SciTech Connect

    Bergsman, K.H.

    1996-03-01

    This dose management plan facilitates meeting the dose management and ALARA requirements applicable to the design activities of the Spent Nuclear Fuel Project, and establishes consistency of information used by multiple subprojects in ALARA evaluations. The method for meeting the ALARA requirements applicable to facility designs involves two components. The first is each Spent Nuclear Fuel Project subproject incorporating ALARA principles, ALARA design optimizations, and ALARA design reviews throughout the design of facilities and equipment. The second component is the Spent Nuclear Fuel Project management providing overall dose management guidance to the subprojects and oversight of the subproject dose management efforts.

  10. Safeguards issues in spent fuel consolidation facilities

    SciTech Connect

    Belew, W.L.; Moran, B.W.

    1991-01-01

    In the nuclear power industry, the fuel assembly is the basic unit for nuclear material accountancy. The safeguards procedures for the spent fuel assemblies, therefore, are based on an item accountancy approach. When fuel consolidation occurs in at-reactor'' or away-from-reactor'' facilities, the fuel assemblies are disassembled and cease to be the basic unit containing nuclear material. Safeguards can no longer be based on item accountancy of fuel assemblies. The spent fuel pins containing plutonium are accessible, and the possibilities for diversion of spent fuel for clandestine reprocessing to recover the plutonium are increased. Thus, identifying the potential safeguards concerns created by operation of these facilities is necessary. Potential safeguards techniques to address these concerns also must be identified so facility designs may include the equipment and systems required to provide an acceptable level of assurance that the international safeguards objectives can be met when these facilities come on-line. The objectives of this report are (1) to identify the safeguards issues associated with operation of spent fuel consolidation facilities, (2) to provide a preliminary assessment of the assessment of the safeguards vulnerabilities introduced, and (3) to identify potential safeguards approaches that could meet international safeguards requirements. The safeguards aspects of spent fuel consolidation are addressed in several recent reports and papers. 11 refs., 3 figs., 3 tabs.

  11. Spent fuel storage requirements 1993--2040

    SciTech Connect

    Not Available

    1994-09-01

    Historical inventories of spent fuel are combined with U.S. Department of Energy (DOE) projections of future discharges from commercial nuclear reactors in the United States to provide estimates of spent fuel storage requirements through the year 2040. The needs are estimated for storage capacity beyond that presently available in the reactor storage pools. These estimates incorporate the maximum capacities within current and planned in-pool storage facilities and any planned transshipments of spent fuel to other reactors or facilities. Existing and future dry storage facilities are also discussed. The nuclear utilities provide historical data through December 1992 on the end of reactor life are based on the DOE/Energy Information Administration (EIA) estimates of future nuclear capacity, generation, and spent fuel discharges.

  12. Measurement of Spent Fuel Assemblies - Overview of the Status of the Technology for Initiating Discussion at NATIONAL RESEARCH CENTRE KURCHATOV INSTITUTE June 2013

    SciTech Connect

    SISKIND B.; N /A

    2013-06-03

    This presentation provides an overview of the status of the technology for the measurement of the fissile material content of spent nuclear reactor fuel. The emphasis is on how the needs of the U.S. Nuclear Regulatory Commission and the International Atomic Energy Agency are met by the available technology and what more needs to be done in this area.

  13. Method for shearing spent nuclear fuel assemblies

    DOEpatents

    Weil, Bradley S.; Watson, Clyde D.

    1977-01-01

    A method is disclosed for shearing spent nuclear fuel assemblies of the type wherein a plurality of long metal tubes packed with ceramic fuel are supported in a spaced apart relationship within an outer metal shell or shroud which provides structural support to the assembly. Spent nuclear fuel assemblies are first compacted in a stepwise manner between specially designed gag-compactors and then sheared into short segments amenable to chemical processing by shear blades contoured to mate with the compacted surface of the fuel assembly.

  14. Pyrochemical processing of DOE spent nuclear fuel

    SciTech Connect

    Laidler, J.J.

    1995-02-01

    A compact, efficient method for conditioning spent nuclear fuel is under development. This method, known as pyrochemical processing, or {open_quotes}pyroprocessing,{close_quotes} provides a separation of fission products from the actinide elements present in spent fuel and further separates pure uranium from the transuranic elements. The process can facilitate the timely and environmentally-sound treatment of the highly diverse collection of spent fuel currently in the inventory of the United States Department of Energy (DOE). The pyroprocess utilizes elevated-temperature processes to prepare spent fuel for fission product separation; that separation is accomplished by a molten salt electrorefining step that provides efficient (>99.9%) separation of transuranics. The resultant waste forms from the pyroprocess, are stable under envisioned repository environment conditions and highly leach-resistant. Treatment of any spent fuel type produces a set of common high-level waste forms, one a mineral and the other a metal alloy, that can be readily qualified for repository disposal and avoid the substantial costs that would be associated with the qualification of the numerous spent fuel types included in the DOE inventory.

  15. Integrated process for reprocessing spent nuclear fuel

    SciTech Connect

    Forsberg, C.W.

    1991-03-06

    This invention is comprised of a process for recovering nuclear fuel from spent fuel assemblies that employs a single canister process container. The cladding and fuel are oxidized in the container, the fuel is dissolved and removed from the container for separation from the aqueous phase, the aqueous phase containing radioactive waste is returned to the container. This container is also the disposal vessel. Add solidification agents and compress container for long term storage.

  16. Spent Nuclear Fuel Project Technical Databook

    SciTech Connect

    Reilly, M.A.

    1998-10-23

    The Spent Nuclear Fuel (SNF) Project Technical Databook is developed for use as a common authoritative source of fuel behavior and material parameters in support of the Hanford SNF Project. The Technical Databook will be revised as necessary to add parameters as their Databook submittals become available.

  17. Spent fuel pin temperature PC code

    SciTech Connect

    Fischer, L.E.

    1985-03-01

    During an annual outage, a Pressurized Water Reactor (PWR) may discharge 60 or more spent fuel bundles into its storage pool. Most early PWRs were built to store 3 to 5 years of spent fuel in their pools and are beginning to exceed their capacities. One method currently being developed and licensed for expanding spent fuel storage capabilities is the dry storage of spent fuel in large casks. To reduce the probability of gross failures of fuel cladding during dry storage in casks, the fuel pin temperatures must be shown to remain within acceptable limits. LLNL has developed, for the Nuclear Regulatory Commission, a personal computer (PC) code for calculating fuel pin temperatures on the IBM PC. The code uses the Wooton-Epstein Correlation to calculate the pin temperatures and has been benchmarked against test data. An iterative type of solution is used to calculate the fuel pin temperatures for specified heat fluxes and pin configurations. The PC code is useful in performing confirmatory analyses and comparing the results with those submitted by applicants applying for storage licenses. 5 references, 2 tables.

  18. Is Spent Fuel or Waste from Reprocessed Spent Fuel Simpler to Dispose of?

    DTIC Science & Technology

    1981-06-12

    the space in a repository for processed high-level waste has not included the disposal of transuranic waste from the co.mercial fuel cycle which will...AD-AI06 573 GENERAL ACCOUNTING OFFICE WASHINGTON OC ENERGY AND M-ETC F/G 18/7 i S PENT FUEL OR WASTE FROM REPROCESSED SPENT FUEL SIMPLER TO D--TC(U...the Congress entitled "Is Spent Fuel or Waste from Reprocessed Spent Fuel Simpler to Dispose of?" (EID-81-78, June 12, 1981)z Insert the following

  19. Spent Nuclear Fuel Transport Reliability Study

    SciTech Connect

    Wang, Jy-An John; Wang, Hong; Jiang, Hao

    2016-01-01

    This conference paper was orignated and shorten from the following publisehd PTS documents: 1. Jy-An Wang, Hao Jiang, and Hong Wang, Dynamic Deformation Simulation of Spent Nuclear Fuel Assembly and CIRFT Deformation Sensor Stability Investigation, ORNL/SPR-2015/662, November 2015. 2. Jy-An Wang, Hong Wang, Mechanical Fatigue Testing of High-Burnup Fuel for Transportation Applications, NUREG/CR-7198, ORNL/TM-2014/214, May 2015. 3. Jy-An Wang, Hong Wang, Hao Jiang, Yong Yan, Bruce Bevard, Spent Nuclear Fuel Vibration Integrity Study 16332, WM2016 Conference, March 6 10, 2016, Phoenix, Arizona.

  20. Detecting pin diversion from pressurized water reactors spent fuel assemblies

    DOEpatents

    Ham, Young S.; Sitaraman, Shivakumar

    2017-01-10

    Detecting diversion of spent fuel from Pressurized Water Reactors (PWR) by determining possible diversion including the steps of providing a detector cluster containing gamma ray and neutron detectors, inserting the detector cluster containing the gamma ray and neutron detectors into the spent fuel assembly through the guide tube holes in the spent fuel assembly, measuring gamma ray and neutron radiation responses of the gamma ray and neutron detectors in the guide tube holes, processing the gamma ray and neutron radiation responses at the guide tube locations by normalizing them to the maximum value among each set of responses and taking the ratio of the gamma ray and neutron responses at the guide tube locations and normalizing the ratios to the maximum value among them and producing three signatures, gamma, neutron, and gamma-neutron ratio, based on these normalized values, and producing an output that consists of these signatures that can indicate possible diversion of the pins from the spent fuel assembly.

  1. Measuring the Noble Metal and Iodine Composition of Extracted Noble Metal Phase from Spent Nuclear Fuel Using Instrumental Neutron Activation Analysis

    SciTech Connect

    Palomares, R. I.; Dayman, Kenneth J.; Landsberger, Sheldon; Biegalski, Steven R.; Soderquist, Chuck Z.; Casella, Amanda J.; Brady Raap, Michaele C.; Schwantes, Jon M.

    2015-04-01

    Mass quantities of noble metal and iodine nuclides in the metallic noble metal phase extracted from spent fuel are measured using instrumental neutron activation analysis (NAA). Nuclide presence is predicted using fission yield analysis, and mass quantification is derived from standard gamma spectroscopy and radionuclide decay analysis. The nuclide compositions of noble metal phase derived from two dissolution methods, UO2 fuel dissolved in nitric acid and UO2 fuel dissolved in ammonium-carbonate and hydrogen-peroxide solution, are compared. Lastly, the implications of the rapid analytic speed of instrumental NAA are discussed in relation to potential nuclear forensics applications.

  2. Hanford spent fuel inventory baseline

    SciTech Connect

    Bergsman, K.H.

    1994-07-15

    This document compiles technical data on irradiated fuel stored at the Hanford Site in support of the Hanford SNF Management Environmental Impact Statement. Fuel included is from the Defense Production Reactors (N Reactor and the single-pass reactors; B, C, D, DR, F, H, KE and KW), the Hanford Fast Flux Test Facility Reactor, the Shipping port Pressurized Water Reactor, and small amounts of miscellaneous fuel from several commercial, research, and experimental reactors.

  3. Corrosion of spent Advanced Test Reactor fuel

    SciTech Connect

    Lundberg, L.B.; Croson, M.L.

    1994-11-01

    The results of a study of the condition of spent nuclear fuel elements from the Advanced Test Reactor (ATR) currently being stored underwater at the Idaho National Engineering Laboratory (INEL) are presented. This study was motivated by a need to estimate the corrosion behavior of dried, spent ATR fuel elements during dry storage for periods up to 50 years. The study indicated that the condition of spent ATR fuel elements currently stored underwater at the INEL is not very well known. Based on the limited data and observed corrosion behavior in the reactor and in underwater storage, it was concluded that many of the fuel elements currently stored under water in the facility called ICPP-603 FSF are in a degraded condition, and it is probable that many have breached cladding. The anticipated dehydration behavior of corroded spent ATR fuel elements was also studied, and a list of issues to be addressed by fuel element characterization before and after forced drying of the fuel elements and during dry storage is presented.

  4. Considerations for Possible Light Impact of Spent Nuclear Fuel for Safeguards Measurements

    SciTech Connect

    Brian K. Castle; Kelly D. Ellis

    2012-09-01

    This effort is designed to be a preliminary study to determine the appropriateness of lightly contacting SNF with zirconium-based cladding, in wet storage, for the purpose of taking safeguards measurements. Contact will likely consist of an initial impact followed by a light tensile load on the exterior surface of the SNF cladding. In the past, concerns have been raised that contacting SNF cladding could result in a loss of long-term mechanical integrity due to crack initiation, uncontrolled crack propagation, and a mechanical exfoliation of the protective oxide layer. The mechanical integrity concerns are addressed with an analytic model that evaluates the threshold impact limits for degraded, but undamaged SNF cladding. Aqueous corrosion concerns, associated with exfoliation of the protective oxide layer, are addressed with a qualitative argument, focusing on the possible corrosion mechanisms of zirconium-based cladding.

  5. Determining initial enrichment, burnup, and cooling time of pressurized-water-reactor spent fuel assemblies by analyzing passive gamma spectra measured at the Clab interim-fuel storage facility in Sweden

    NASA Astrophysics Data System (ADS)

    Favalli, A.; Vo, D.; Grogan, B.; Jansson, P.; Liljenfeldt, H.; Mozin, V.; Schwalbach, P.; Sjöland, A.; Tobin, S. J.; Trellue, H.; Vaccaro, S.

    2016-06-01

    The purpose of the Next Generation Safeguards Initiative (NGSI)-Spent Fuel (SF) project is to strengthen the technical toolkit of safeguards inspectors and/or other interested parties. The NGSI-SF team is working to achieve the following technical goals more easily and efficiently than in the past using nondestructive assay measurements of spent fuel assemblies: (1) verify the initial enrichment, burnup, and cooling time of facility declaration; (2) detect the diversion or replacement of pins; (3) estimate the plutonium mass [which is also a function of the variables in (1)]; (4) estimate the decay heat; and (5) determine the reactivity of spent fuel assemblies. Since August 2013, a set of measurement campaigns has been conducted at the Central Interim Storage Facility for Spent Nuclear Fuel (Clab), in collaboration with Swedish Nuclear Fuel and Waste Management Company (SKB). One purpose of the measurement campaigns was to acquire passive gamma spectra with high-purity germanium and lanthanum bromide scintillation detectors from Pressurized Water Reactor and Boiling Water Reactor spent fuel assemblies. The absolute 137Cs count rate and the 154Eu/137Cs, 134Cs/137Cs, 106Ru/137Cs, and 144Ce/137Cs isotopic ratios were extracted; these values were used to construct corresponding model functions (which describe each measured quantity's behavior over various combinations of burnup, cooling time, and initial enrichment) and then were used to determine those same quantities in each measured spent fuel assembly. The results obtained in comparison with the operator declared values, as well as the methodology developed, are discussed in detail in the paper.

  6. Determining initial enrichment, burnup, and cooling time of pressurized-water reactor spent fuel assemblies by analyzing passive gamma spectra measured at the Clab interim-fuel storage facility in Sweden

    SciTech Connect

    Favalli, Andrea; Vo, D.; Grogan, Brandon R.; Jansson, Peter; Liljenfeldt, Henrik; Mozin, Vladimir; Schwalbach, P.; Sjoland, A.; Tobin, Stephen J.; Trellue, Holly; Vaccaro, S.

    2016-02-26

    The purpose of the Next Generation Safeguards Initiative (NGSI)–Spent Fuel (SF) project is to strengthen the technical toolkit of safeguards inspectors and/or other interested parties. The NGSI–SF team is working to achieve the following technical goals more easily and efficiently than in the past using nondestructive assay measurements of spent fuel assemblies: (1) verify the initial enrichment, burnup, and cooling time of facility declaration; (2) detect the diversion or replacement of pins; (3) estimate the plutonium mass [which is also a function of the variables in (1)]; (4) estimate the decay heat; and (5) determine the reactivity of spent fuel assemblies. Since August 2013, a set of measurement campaigns has been conducted at the Central Interim Storage Facility for Spent Nuclear Fuel (Clab), in collaboration with Swedish Nuclear Fuel and Waste Management Company (SKB). One purpose of the measurement campaigns was to acquire passive gamma spectra with high-purity germanium and lanthanum bromide scintillation detectors from Pressurized Water Reactor and Boiling Water Reactor spent fuel assemblies. The absolute 137Cs count rate and the 154Eu/137Cs, 134Cs/137Cs, 106Ru/137Cs, and 144Ce/137Cs isotopic ratios were extracted; these values were used to construct corresponding model functions (which describe each measured quantity’s behavior over various combinations of burnup, cooling time, and initial enrichment) and then were used to determine those same quantities in each measured spent fuel assembly. Furthermore, the results obtained in comparison with the operator declared values, as well as the methodology developed, are discussed in detail in the paper.

  7. Spent fuel container alignment device and method

    DOEpatents

    Jones, Stewart D.; Chapek, George V.

    1996-01-01

    An alignment device is used with a spent fuel shipping container including a plurality of fuel pockets for spent fuel arranged in an annular array and having a rotatable cover including an access opening therein. The alignment device includes a lightweight plate which is installed over the access opening of the cover. A laser device is mounted on the plate so as to emit a laser beam through a laser admittance window in the cover into the container in the direction of a pre-established target associated with a particular fuel pocket. An indexing arrangement on the container provides an indication of the angular position of the rotatable cover when the laser beam produced by the laser is brought into alignment with the target of the associated fuel pocket.

  8. Spent Nuclear Fuel Alternative Technology Decision Analysis

    SciTech Connect

    Shedrow, C.B.

    1999-11-29

    The Westinghouse Savannah River Company (WSRC) made a FY98 commitment to the Department of Energy (DOE) to recommend a technology for the disposal of aluminum-based spent nuclear fuel (SNF) at the Savannah River Site (SRS). The two technologies being considered, direct co-disposal and melt and dilute, had been previously selected from a group of eleven potential SNF management technologies by the Research Reactor Spent Nuclear Fuel Task Team chartered by the DOE''s Office of Spent Fuel Management. To meet this commitment, WSRC organized the SNF Alternative Technology Program to further develop the direct co-disposal and melt and dilute technologies and ultimately provide a WSRC recommendation to DOE on a preferred SNF alternative management technology.

  9. Laser surveillance system for spent fuel

    SciTech Connect

    Fiarman, S; Zucker, M S; Bieber, Jr, A M

    1980-01-01

    A laser surveillance system installed at spent fuel storage pools will provide the safeguard inspector with specific knowledge of spent fuel movement that cannot be obtained with current surveillance systems. The laser system will allow for the division of the pool's spent fuel inventory into two populations - those assemblies which have been moved and those which haven't - which is essential for maximizing the efficiency and effectiveness of the inspection effort. We have designed, constructed, and tested a laser system and have used it with a simulated BWR assembly. The reflected signal from the zircaloy rods depends on the position of the assembly, but in all cases is easily discernable from the reference scan of background with no assembly.

  10. Laser Surveillance System for Spent Fuel

    SciTech Connect

    Fiarman, S.; Zucker, M. S.; Bieber, Jr., A. M.

    1980-01-01

    A laser surveillance system installed at spent fuel storage pools (SFSP's) will provide the safeguard inspector with specific knowledge of spent fuel movement that cannot be obtained with current surveillance systems. The laser system will allow for the division of the pool's spent fuel inventory into two populations - those assemblies which have been moved and those which haven't - which is essential for maximizing the efficiency and effectiveness of the inspection effort. We have designed, constructed, and tested a full size laser system operating in air and have used an array of 6 zircaloy BWR tubes to simulate an assembly. The reflective signal from the zircaloy rods is a strong function of position of the assembly, but in all cases is easily discernable from the reference scan of the background with no assembly. A design for a SFSP laser surveillance system incorporating laser ranging is discussed. 10 figures.

  11. Pyrochemical Treatment of Spent Nuclear Fuel

    SciTech Connect

    K. M. Goff; K. L. Howden; G. M. Teske; T. A. Johnson

    2005-10-01

    Over the last 10 years, pyrochemical treatment of spent nuclear fuel has progressed from demonstration activities to engineering-scale production operations. As part of the Advanced Fuel Cycle Initiative within the U.S. Department of Energy’s Office of Nuclear Energy, Science and Technology, pyrochemical treatment operations are being performed as part of the treatment of fuel from the Experimental Breeder Reactor II at the Idaho National Laboratory. Integral to these treatment operations are research and development activities that are focused on scaling further the technology, developing and implementing process improvements, qualifying the resulting high-level waste forms, and demonstrating the overall pyrochemical fuel cycle.

  12. Spent fuel treatment at ANL-West

    SciTech Connect

    Goff, K.M.; Benedict, R.W.; Levinskas, D.

    1994-12-31

    At Argonne National Laboratory-West (ANL-West) there are several thousand kilograms of metallic spent nuclear fuel containing bond sodium. This fuel will be treated in the Fuel Cycle Facility at ANL-West to produce stable waste forms for storage and disposal. The treatment operations will employ a pyrochemical process that also has applications for treating most of the fuel types within the Department of Energy complex. The treatment equipment is in its last stage of readiness, and operations will begin in the Fall of 1994.

  13. Determining initial enrichment, burnup, and cooling time of pressurized-water reactor spent fuel assemblies by analyzing passive gamma spectra measured at the Clab interim-fuel storage facility in Sweden

    DOE PAGES

    Favalli, Andrea; Vo, D.; Grogan, Brandon R.; ...

    2016-02-26

    The purpose of the Next Generation Safeguards Initiative (NGSI)–Spent Fuel (SF) project is to strengthen the technical toolkit of safeguards inspectors and/or other interested parties. The NGSI–SF team is working to achieve the following technical goals more easily and efficiently than in the past using nondestructive assay measurements of spent fuel assemblies: (1) verify the initial enrichment, burnup, and cooling time of facility declaration; (2) detect the diversion or replacement of pins; (3) estimate the plutonium mass [which is also a function of the variables in (1)]; (4) estimate the decay heat; and (5) determine the reactivity of spent fuelmore » assemblies. Since August 2013, a set of measurement campaigns has been conducted at the Central Interim Storage Facility for Spent Nuclear Fuel (Clab), in collaboration with Swedish Nuclear Fuel and Waste Management Company (SKB). One purpose of the measurement campaigns was to acquire passive gamma spectra with high-purity germanium and lanthanum bromide scintillation detectors from Pressurized Water Reactor and Boiling Water Reactor spent fuel assemblies. The absolute 137Cs count rate and the 154Eu/137Cs, 134Cs/137Cs, 106Ru/137Cs, and 144Ce/137Cs isotopic ratios were extracted; these values were used to construct corresponding model functions (which describe each measured quantity’s behavior over various combinations of burnup, cooling time, and initial enrichment) and then were used to determine those same quantities in each measured spent fuel assembly. Furthermore, the results obtained in comparison with the operator declared values, as well as the methodology developed, are discussed in detail in the paper.« less

  14. Inspection and Gamma-Ray Dose Rate Measurements of the Annulus of the VSC-17 Concrete Spent Nuclear Fuel Storage Cask

    SciTech Connect

    P. L. Winston

    2007-09-01

    The air cooling annulus of the Ventilated Storage Cask (VSC)-17 spent fuel storage cask was inspected using a Toshiba 7 mm (1/4”) CCD video camera. The dose rates observed in the annular space were measured to provide a reference for the activity to which the camera(s) being tested were being exposed. No gross degradation, pitting, or general corrosion was observed.

  15. Spent fuel behavior in dry storage

    NASA Astrophysics Data System (ADS)

    Johnson, A. B., Jr.; Pankaskie, P. J.; Gilbert, E. R.

    1982-02-01

    Dry storage is emerging as an attractive and timely alternative to complement wet storage, and assist utilities to meet interim storage needs. Spent fuel is handled and stored under dry conditions. Dry storage of irradiated Zircaloy clad fuel in metal casks, drywells, silos and vaults is demonstrated. Hot cell and laboratory studies also are underway to investigate specific phenomena related to cladding behavior in dry storage. A substantial fraction of the LWR spent fuel inventory has aged for relatively long times and has relatively low decay heats. This suggests that much of the fuel inventory can be stored at relatively low temperatures. Alternatively, rod consolidation of the older can be considered without exceeding maximum cladding temperatures.

  16. BR-100 spent fuel shipping cask development

    SciTech Connect

    McGuinn, E.J.; Childress, P.C.

    1990-01-01

    Continued public acceptance of commercial nuclear power is contingent to a large degree on the US Department of Energy (DOE) establishing an integrated waste management system for spent nuclear fuel. As part of the from-reactor transportation segment of this system, the B W Fuel Company (BWFC) is under contract to the DOE to develop a spent-fuel cask that is compatible with both rail and barge modes of transportation. Innovative design approaches were the keys to achieving a cask design that maximizes payload capacity and cask performance. The result is the BR-100, a 100-ton rail/barge cask with a capacity of 21 PWR or 52 BWR ten-year cooled, intact fuel assemblies. 3 figs.

  17. Spent nuclear fuel project product specification

    SciTech Connect

    Pajunen, A.L.

    1998-01-30

    Product specifications are limits and controls established for each significant parameter that potentially affects safety and/or quality of the Spent Nuclear Fuel (SNF) packaged for transport to dry storage. The product specifications in this document cover the spent fuel packaged in MultiCanister Overpacks (MCOs) to be transported throughout the SNF Project. The SNF includes N Reactor fuel and single-pass reactor fuel. The FRS removes the SNF from the storage canisters, cleans it, and places it into baskets. The MCO loading system places the baskets into MCO/Cask assembly packages. These packages are then transferred to the Cold Vacuum Drying (CVD) Facility. After drying at the CVD Facility, the MCO cask packages are transferred to the Canister Storage Building (CSB), where the MCOs are removed from the casks, staged, inspected, sealed (by welding), and stored until a suitable permanent disposal option is implemented. The key criteria necessary to achieve these goals are documented in this specification.

  18. Spent nuclear fuel project integrated schedule plan

    SciTech Connect

    Squires, K.G.

    1995-03-06

    The Spent Nuclear Fuel Integrated Schedule Plan establishes the organizational responsibilities, rules for developing, maintain and status of the SNF integrated schedule, and an implementation plan for the integrated schedule. The mission of the SNFP on the Hanford site is to provide safe, economic, environmentally sound management of Hanford SNF in a manner which stages it to final disposition. This particularly involves K Basin fuel.

  19. Cosmic-ray imaging of spent fuel casks

    NASA Astrophysics Data System (ADS)

    Guardincerri, Elena; Durham, J. Matthew; Morris, Christopher; Poulson, Daniel; Plaud-Ramos, Kenie; Fabritius, Joseph; Bacon, Jeffrey; Winston, Philip; Chichester, David

    2015-10-01

    Muon radiography was used to image the inside of a partially loaded Westinghouse MC-10 dry cask containing spent nuclear fuel at Idaho National Laboratory. We present here the results of a 100 hours long measurement taken in May 2015 with two muon trackers placed outside the cask. The data clearly show the location of the missing fuel bundles and demonstrate the feasibility of using cosmic rays to monitor fuel casks against illicit diversion of their content.

  20. Remote inspection of the IFSF spent fuel storage rack

    SciTech Connect

    Uldrich, E.D.

    1996-05-01

    The Irradiated Fuel Storage Facility (IFSF) is a dry storage facility for spent nuclear fuels located at the Idaho Chemical Processing Plant; it was constructed in the 1970`s specifically for the Fort Saint Vrain spent reactor fuels. Currently, it is being used for various spent fuels. It was not known if IFSF would met current DOE seismic criteria, so re-analysis was started, with the rack being analyzed first. The rack was inspected to determine the as-built condition. LazrLyne and VideoRuler were used in lieu of using a tape measure with the camera. It was concluded that when a visual inspection shows widely varying weld sizes, the engineer has to use all resources available to determine the most probable specified weld sizes.

  1. Total quality in spent fuel pool reracking

    SciTech Connect

    Cranston, J.S.; Taglianetti, J.N.; Schaeffer, D.G.; Bradbury, R.B.; Cacciapouti, R.J.

    1993-12-31

    The nuclear utility environment is one of strict cost control under prescriptive regulations and increasing public scrutiny. This paper presents the results of A Total Quality approach, by a dedicated team, that addresses the need for increased on-site spent fuel storage in this environment. Innovations to spent fuel pool reracking, driven by utilities` specific technical needs and shrinking budgets, have resulted in both product improvements and lower prices. A Total Quality approach to the entire turnkey project is taken, thereby creating synergism and process efficiency in each of the major phases of the project: design and analysis, licensing, fabrication, installation and disposal. Specific technical advances and the proven quality of the team members minimizes risk to the utility and its shareholders and provides a complete, cost effective service. Proper evaluation of spent fuel storage methods and vendors requires a full understanding of currently available customer driven initiatives that reduce cost while improving quality. In all phases of a spent fuel reracking project, from new rack design and analysis through old rack disposal, the integration of diverse experts, at all levels and throughout all phases of a reracking project, better serves utility needs. This Total Quality environment in conjunction with many technical improvements results in a higher quality product at a lower cost.

  2. Spent Nuclear Fuel (SNF) Project Product Specification

    SciTech Connect

    PAJUNEN, A.L.

    2000-01-20

    This document establishes the limits and controls for the significant parameters that could potentially affect the safety and/or quality of the Spent Nuclear Fuel (SNF) packaged for processing, transport, and storage. The product specifications in this document cover the SNF packaged in Multi-Canister Overpacks to be transported throughout the SNF Project.

  3. Spent nuclear fuel project product specification

    SciTech Connect

    PAJUNEN, A.L.

    1999-02-25

    This document establishes the limits and controls for the significant parameters that could potentially affect the safety and/or quality of the Spent Nuclear Fuel (SNF) packaged for processing, transport, and storage. The product specifications in this document cover the SNF packaged in Multi-Canister Overpacks to be transported throughout the SNF Project.

  4. The effect of fuel type in unsaturated spent fuel tests

    SciTech Connect

    Finn, P.A.; Gong, M.; Bates, J.K.; Emery, J.W.; Hoh, J.C.

    1994-04-01

    Two well-characterized types of spent nuclear fuel (ATM-103 and ATM-106) were tested under simulated unsaturated conditions with simulated groundwater at 90{degree}C. The actinides present in the leachate were measured after periods of approximately 60, 120, and 275 days. The vessels were acid stripped after 120 and 275 days. Both colloidal and soluble actinide species were detected in the leachates which had pHs ranging from 4 to 7. Alpha spectroscopy studies of filtered and unfiltered leachates showed that large amounts of actinides may be bound in colloids. The uranium phases identified in the colloids were schoepite and soddyite. The actinide release behavior of the two fuels appears to be different. The ATM-106 fuel began to release actinides later than the ATM-103 fuel, but after 275 days, it had released more. The amount of americium released from the two fuels was a higher percentage of the maximum amount of americium present than was the percentage of the simultaneous amount of uranium released.

  5. Numerical Estimation of the Spent Fuel Ratio

    SciTech Connect

    Lindgren, Eric R.; Durbin, Samuel; Wilke, Jason; Margraf, J.; Dunn, T. A.

    2016-01-01

    Sabotage of spent nuclear fuel casks remains a concern nearly forty years after attacks against shipment casks were first analyzed and has a renewed relevance in the post-9/11 environment. A limited number of full-scale tests and supporting efforts using surrogate materials, typically depleted uranium dioxide (DUO 2 ), have been conducted in the interim to more definitively determine the source term from these postulated events. However, the validity of these large- scale results remain in question due to the lack of a defensible spent fuel ratio (SFR), defined as the amount of respirable aerosol generated by an attack on a mass of spent fuel compared to that of an otherwise identical surrogate. Previous attempts to define the SFR in the 1980's have resulted in estimates ranging from 0.42 to 12 and include suboptimal experimental techniques and data comparisons. Because of the large uncertainty surrounding the SFR, estimates of releases from security-related events may be unnecessarily conservative. Credible arguments exist that the SFR does not exceed a value of unity. A defensible determination of the SFR in this lower range would greatly reduce the calculated risk associated with the transport and storage of spent nuclear fuel in dry cask systems. In the present work, the shock physics codes CTH and ALE3D were used to simulate spent nuclear fuel (SNF) and DUO 2 targets impacted by a high-velocity jet at an ambient temperature condition. These preliminary results are used to illustrate an approach to estimate the respirable release fraction for each type of material and ultimately, an estimate of the SFR. This page intentionally blank

  6. Spent fuel dry storage technology development: thermal evaluation of sealed storage cask containing spent fuel

    SciTech Connect

    Schmitten, P.F.; Wright, J.B.

    1980-08-01

    A PWR spent fuel assembly was encapsulated inside the E-MAD Hot Bay and placed in a instrumented above surface storage cell during December 1978 for thermal testing. Instrumentation provided to measure canister, liner and concrete temperatures consisted of thermocouples which were inserted into tubes on the outside of the canister and liner and in three radial positions in the concrete. Temperatures from the SSC test assembly have been recorded throughout the past 16 months. Canister and liner temperatures have reached their peak values of 200{sup 0}F and 140{sup 0}F, respectively. Computer predictions of the transient and steady-state temperatures show good agreement with the test data.

  7. Plasma method for processing spent nuclear fuel

    SciTech Connect

    Timofeev, A. V.

    2007-11-15

    Plasma methods for processing spent nuclear fuel are analyzed. It is shown that, by ICR heating in a nonuniform magnetic field, the energy of the heated ash ions can be increased substantially, while nuclear fuel ions can be kept cold. Two methods for extracting heated ash ions from a cold plasma flow are considered, specifically, that by increasing the ion gyroradius and that due to ion drift in a curved magnetic field. It is found that the required degree of separation of ash and fuel ions can be achieved in systems with quite moderate parameters.

  8. Historical overview of domestic spent fuel shipments

    SciTech Connect

    Pope, R.B.; Wankerl, M.W. ); Armstrong, S.; Hamberger, C., Schmid, S. )

    1991-01-01

    The purpose of this paper is to provide available historical data on most commercial and research reactor spent fuel shipments that have been completed in the United States between 1964 and 1989. This information includes data on the sources of spent fuel that has been shipped, the types of shipping casks used, the number of fuel assemblies that have been shipped, and the number of shipments that have been made. The data are updated periodically to keep abreast of changes. Information on shipments is provided for planning purposes; to support program decisions of the US Department of Energy's (DOE's) Office of Civilian Radioactive Waste Management (OCRWM); and to inform interested members of the public, federal, state, and local government, Indian tribes, and the transportation community. 5 refs., 7 figs., 2 tabs.

  9. Report on interim storage of spent nuclear fuel

    SciTech Connect

    Not Available

    1993-04-01

    The report on interim storage of spent nuclear fuel discusses the technical, regulatory, and economic aspects of spent-fuel storage at nuclear reactors. The report is intended to provide legislators state officials and citizens in the Midwest with information on spent-fuel inventories, current and projected additional storage requirements, licensing, storage technologies, and actions taken by various utilities in the Midwest to augment their capacity to store spent nuclear fuel on site.

  10. 77 FR 76952 - Rescinding Spent Fuel Pool Exclusion Regulations

    Federal Register 2010, 2011, 2012, 2013, 2014

    2012-12-31

    ...; ] NUCLEAR REGULATORY COMMISSION 10 CFR Part 51 Rescinding Spent Fuel Pool Exclusion Regulations AGENCY... fuel pool storage impacts from license renewal environmental reviews. This action is necessary...

  11. Determination of plutonium content in TRR spent fuel by nondestructive neutron counting

    NASA Astrophysics Data System (ADS)

    Chen, Yen-Fu; Sheu, Rong-Jiun; Chiao, Ling-Huan; Yuan, Ming-Chen; Jiang, Shiang-Huei

    2010-07-01

    For the nuclear safeguard purpose, this work aims to nondestructively determine the plutonium content in the Taiwan Research Reactor (TRR) spent fuel rods in the storage pool before the stabilization process, which transforms the metal spent fuel rods into oxide powder. A SPent-fuel-Neutron-Counter (SPNC) system was designed and constructed to carry out underwater scan measurements of neutrons emitting from the spent fuel rod, from which the 240Pu mass in the fuel rod will be determined. The SAS2 H control module of the SCALE 5.1 code package was applied to calculate the 240Pu-to-Pu mass ratio in the TRR spent fuel rod according to the given power history. This paper presents the methodology and design of our detector system as well as the measurements of four TRR spent fuel rods in the storage pool and the comparison of the measured results with the facility declared values.

  12. International safeguards for spent fuel storage

    NASA Astrophysics Data System (ADS)

    Kratzer, M.; Wonder, E.; Immerman, W.; Crane, F.

    1981-08-01

    The nonproliferation effectiveness and political and economic acceptability of prospective improvements in international safeguard techniques for LWR spent fuel storage were analyzed. Although the applicability of item accounting considerably eases the safeguarding of stored spent fuel, the problem of verification is potentially serious. A number of simple gamma and neutron nondestructive assay techniques were found to offer considerable improvements, of a qualitative rather than quantiative nature, in verification-related data and information, and possess the major advantage of intruding very littel on facility operations. A number of improved seals and monitors appear feasible as well, but improvements in the timeliness of detection will not occur unless the frequency of inspection is increased or a remote monitoring capability is established. Limitations on IAEA Safeguards resources and on the integration of results from material accounting and containment and surveillance remain problems.

  13. International safeguards for spent fuel storage

    SciTech Connect

    Kratzer, M.; Wonder, E.; Immerman, W.; Crane, F.

    1981-08-01

    This report analyzes the nonproliferation effectiveness and political and economic acceptability of prospective improvements in international safeguard techniques for LWR spent fuel storage. Although the applicability of item accounting considerably eases the safeguarding of stored spent fuel, the problem of verification is potentially serious. A number of simple gamma and neutron nondestructive assay techniques were found to offer considerable improvements, of a qualitative rather than quantitative nature, in verification-related data and information, and possess the major advantage of intruding very little on facility operations. A number of improved seals and monitors appear feasible as well, but improvements in the timeliness of detection will not occur unless the frequency of inspection is increased or a remote monitoring capability is established. Limitations on IAEA Safeguards resources and on the integration of results from material accounting and containment and surveillance remain problems.

  14. Storage assembly for spent nuclear fuel

    SciTech Connect

    Lapides, M.E.

    1982-04-27

    A technique for storing spent fuel rods from a nuclear reactor is disclosed herein. This technique utilizes a housing including a closed inner chamber for containing the fuel rods and a thermally conductive member located partially within the housing chamber and partially outside the housing for transferring heat generated by the fuel rods from the chamber to the ambient surroundings. Particulate material is located within the chamber and surrounds the fuel rods contained therein. This material is selected to serve as a heat transfer media between the contained cells and the heat transferring member and, at the same time, stand ready to fuse into a solid mass around the contained cells if the heat transferring member malfunctions or otherwise fails to transfer the generated heat out of the housing chamber in a predetermined way.

  15. Spent Fuel Working Group Report. Volume 1

    SciTech Connect

    O`Toole, T.

    1993-11-01

    The Department of Energy is storing large amounts of spent nuclear fuel and other reactor irradiated nuclear materials (herein referred to as RINM). In the past, the Department reprocessed RINM to recover plutonium, tritium, and other isotopes. However, the Department has ceased or is phasing out reprocessing operations. As a consequence, Department facilities designed, constructed, and operated to store RINM for relatively short periods of time now store RINM, pending decisions on the disposition of these materials. The extended use of the facilities, combined with their known degradation and that of their stored materials, has led to uncertainties about safety. To ensure that extended storage is safe (i.e., that protection exists for workers, the public, and the environment), the conditions of these storage facilities had to be assessed. The compelling need for such an assessment led to the Secretary`s initiative on spent fuel, which is the subject of this report. This report comprises three volumes: Volume I; Summary Results of the Spent Fuel Working Group Evaluation; Volume II, Working Group Assessment Team Reports and Protocol; Volume III; Operating Contractor Site Team Reports. This volume presents the overall results of the Working Group`s Evaluation. The group assessed 66 facilities spread across 11 sites. It identified: (1) facilities that should be considered for priority attention. (2) programmatic issues to be considered in decision making about interim storage plans and (3) specific vulnerabilities for some of these facilities.

  16. Spent Nuclear Fuel Alternative Technology Risk Assessment

    SciTech Connect

    Perella, V.F.

    1999-11-29

    A Research Reactor Spent Nuclear Fuel Task Team (RRTT) was chartered by the Department of Energy (DOE) Office of Spent Fuel Management with the responsibility to recommend a course of action leading to a final technology selection for the interim management and ultimate disposition of the foreign and domestic aluminum-based research reactor spent nuclear fuel (SNF) under DOE''s jurisdiction. The RRTT evaluated eleven potential SNF management technologies and recommended that two technologies, direct co-disposal and an isotopic dilution alternative, either press and dilute or melt and dilute, be developed in parallel. Based upon that recommendation, the Westinghouse Savannah River Company (WSRC) organized the SNF Alternative Technology Program to further develop the direct co-disposal and melt and dilute technologies and provide a WSRC recommendation to DOE for a preferred SNF alternative management technology. A technology risk assessment was conducted as a first step in this recommendation process to determine if either, or both, of the technologies posed significant risks that would make them unsuitable for further development. This report provides the results of that technology risk assessment.

  17. Spent fuel behavior under abnormal thermal transients during dry storage

    SciTech Connect

    Stahl, D.; Landow, M.P.; Burian, R.J.; Pasupathi, V.

    1986-01-01

    This study was performed to determine the effects of abnormally high temperatures on spent fuel behavior. Prior to testing, calculations using the CIRFI3 code were used to determine the steady-state fuel and cask component temperatures. The TRUMP code was used to determine transient heating rates under postulated abnormal events during which convection cooling of the cask surfaces was obstructed by a debris bed covering the cask. The peak rate of temperature rise during the first 6 h was calculated to be about 15/sup 0/C/h, followed by a rate of about 1/sup 0/C/h. A Turkey Point spent fuel rod segment was heated to approx. 800/sup 0/C. The segment deformed uniformly with an average strain of 17% at failure and a local strain of 60%. Pretest characterization of the spent fuel consisted of visual examination, profilometry, eddy-current examination, gamma scanning, fission gas collection, void volume measurement, fission gas analysis, hydrogen analysis of the cladding, burnup analysis, cladding metallography, and fuel ceramography. Post-test characterization showed that the failure was a pinhole cladding breach. The results of the tests showed that spent fuel temperatures in excess of 700/sup 0/C are required to produce a cladding breach in fuel rods pressurized to 500 psing (3.45 MPa) under postulated abnormal thermal transient cask conditions. The pinhole cladding breach that developed would be too small to compromise the confinement of spent fuel particles during an abnormal event or after normal cooling conditions are restored. This behavior is similar to that found in other slow ramp tests with irradiated and nonirradiated rod sections and nonirradiated whole rods under conditions that bracketed postulated abnormal heating rates. This similarity is attributed to annealing of the irradiation-strengthened Zircaloy cladding during heating. In both cases, the failure was a benign, ductile pinhole rupture.

  18. Cosmic ray muons for spent nuclear fuel monitoring

    NASA Astrophysics Data System (ADS)

    Chatzidakis, Stylianos

    There is a steady increase in the volume of spent nuclear fuel stored on-site (at reactor) as currently there is no permanent disposal option. No alternative disposal path is available and storage of spent nuclear fuel in dry storage containers is anticipated for the near future. In this dissertation, a capability to monitor spent nuclear fuel stored within dry casks using cosmic ray muons is developed. The motivation stems from the need to investigate whether the stored content agrees with facility declarations to allow proliferation detection and international treaty verification. Cosmic ray muons are charged particles generated naturally in the atmosphere from high energy cosmic rays. Using muons for proliferation detection and international treaty verification of spent nuclear fuel is a novel approach to nuclear security that presents significant advantages. Among others, muons have the ability to penetrate high density materials, are freely available, no radiological sources are required and consequently there is a total absence of any artificial radiological dose. A methodology is developed to demonstrate the applicability of muons for nuclear nonproliferation monitoring of spent nuclear fuel dry casks. Purpose is to use muons to differentiate between spent nuclear fuel dry casks with different amount of loading, not feasible with any other technique. Muon scattering and transmission are used to perform monitoring and imaging of the stored contents of dry casks loaded with spent nuclear fuel. It is shown that one missing fuel assembly can be distinguished from a fully loaded cask with a small overlapping between the scattering distributions with 300,000 muons or more. A Bayesian monitoring algorithm was derived to allow differentiation of a fully loaded dry cask from one with a fuel assembly missing in the order of minutes and negligible error rate. Muon scattering and transmission simulations are used to reconstruct the stored contents of sealed dry casks

  19. Safety Aspects of Dry Spent Fuel Storage and Spent Fuel Management - 13559

    SciTech Connect

    Botsch, W.; Smalian, S.; Hinterding, P.

    2013-07-01

    Dry storage systems are characterized by passive and inherent safety systems ensuring safety even in case of severe incidents or accidents. After the events of Fukushima, the advantages of such passively and inherently safe dry storage systems have become more and more obvious. As with the storage of all radioactive materials, the storage of spent nuclear fuel (SF) and high-level radioactive waste (HLW) must conform to safety requirements. Following safety aspects must be achieved throughout the storage period: - safe enclosure of radioactive materials, - safe removal of decay heat, - securing nuclear criticality safety, - avoidance of unnecessary radiation exposure. The implementation of these safety requirements can be achieved by dry storage of SF and HLW in casks as well as in other systems such as dry vault storage systems or spent fuel pools, where the latter is neither a dry nor a passive system. Furthermore, transport capability must be guaranteed during and after storage as well as limitation and control of radiation exposure. The safe enclosure of radioactive materials in dry storage casks can be achieved by a double-lid sealing system with surveillance of the sealing system. The safe removal of decay heat must be ensured by the design of the storage containers and the storage facility. The safe confinement of radioactive inventory has to be ensured by mechanical integrity of fuel assembly structures. This is guaranteed, e.g. by maintaining the mechanical integrity of the fuel rods or by additional safety measures for defective fuel rods. In order to ensure nuclear critically safety, possible effects of accidents have also to be taken into consideration. In case of dry storage it might be necessary to exclude the re-positioning of fissile material inside the container and/or neutron moderator exclusion might be taken into account. Unnecessary radiation exposure can be avoided by the cask or canister vault system itself. In Germany dry storage of SF in

  20. Application of curium measurements for safeguarding at reprocessing plants. Study 1: High-level liquid waste and Study 2: Spent fuel assemblies and leached hulls

    SciTech Connect

    Rinard, P.M.; Menlove, H.O.

    1996-03-01

    In large-scale reprocessing plants for spent fuel assemblies, the quantity of plutonium in the waste streams each year is large enough to be important for nuclear safeguards. The wastes are drums of leached hulls and cylinders of vitrified high-level liquid waste. The plutonium amounts in these wastes cannot be measured directly by a nondestructive assay (NDA) technique because the gamma rays emitted by plutonium are obscured by gamma rays from fission products, and the neutrons from spontaneous fissions are obscured by those from curium. The most practical NDA signal from the waste is the neutron emission from curium. A diversion of waste for its plutonium would also take a detectable amount of curium, so if the amount of curium in a waste stream is reduced, it can be inferred that there is also a reduced amount of plutonium. This report studies the feasibility of tracking the curium through a reprocessing plant with neutron measurements at key locations: spent fuel assemblies prior to shearing, the accountability tank after dissolution, drums of leached hulls after dissolution, and canisters of vitrified high-level waste after separation. Existing pertinent measurement techniques are reviewed, improvements are suggested, and new measurements are proposed. The authors integrate these curium measurements into a safeguards system.

  1. Advanced waste forms from spent nuclear fuel

    SciTech Connect

    Ackerman, J.P.; McPheeters, C.C.

    1995-12-31

    More than one hundred spent nuclear fuel types, having an aggregate mass of more than 5000 metric tons (2700 metric tons of heavy metal), are stored by the United States Department of Energy. This paper proposes a method for converting this wide variety of fuel types into two waste forms for geologic disposal. The method is based on a molten salt electrorefining technique that was developed for conditioning the sodium-bonded, metallic fuel from the Experimental Breeder Reactor-II (EBR-II) for geologic disposal. The electrorefining method produces two stable, optionally actinide-free, high-level waste forms: an alloy formed from stainless steel, zirconium, and noble metal fission products, and a ceramic waste form containing the reactive metal fission products. Electrorefining and its accompanying head-end process are briefly described, and methods for isolating fission products and fabricating waste forms are discussed.

  2. Direct Measurement of Initial Enrichment, Burn-up and Cooling Time of Spent Fuel Assembly with a Differential Die-Away Technique Based Instrument

    SciTech Connect

    Henzl, Vladimir; Swinhoe, Martyn T.; Tobin, Stephen J.

    2012-07-13

    An outline of this presentation of what a Differential Die-Away (DDA) instrument can do are: (1) Principle of operation of DDA instrument; (2) Determination of initial enrichment (IE) ({sigma} < 5%); (3) Determination of burn up (BU) ({sigma} {approx} 6%); (4) Determination of cooling time (CT) ({sigma} {approx} 20-50%); and (5) DDA instrument as a standalone device. DDA response (fresh fuel vs. spent fuel) is: (1) Fresh fuel => DDA response increases (die-away time is longer) with increasing fissile content; and (2) Spent fuel => DDA response decreases (die-away time is shorter) with higher burn-up (i.e. more neutron absorbers present).

  3. Technical Development on Burn-up Credit for Spent LWR Fuel

    SciTech Connect

    Gauld, I.C.

    2001-12-26

    Technical development on burn-up credit for spent LWR fuels had been performed at JAERI since 1990 under the contract with Science and Technology Agency of Japan entitled ''Technical Development on Criticality Safety Management for Spent LWR Fuels.'' Main purposes of this work are to obtain the experimental data on criticality properties and isotopic compositions of spent LWR fuels and to verify burnup and criticality calculation codes. In this work three major experiments of exponential experiments for spent fuel assemblies to obtain criticality data, non-destructive gamma-ray measurement of spent fuel rods for evaluating axial burn-up profiles, and destructive analyses of spent fuel samples for determining precise burn-up and isotopic compositions were carried out. The measured data obtained were used for validating calculation codes as well as an examination of criticality safety analyses. Details of the work are described in this report.

  4. Hanford spent nuclear fuel project update

    SciTech Connect

    Williams, N.H.

    1997-08-19

    Twenty one hundred metric tons of spent nuclear fuel (SNF) are currently stored in the Hanford Site K Basins near the Columbia River. The deteriorating conditions of the fuel and the basins provide engineering and management challenges to assure safe current and future storage. DE and S Hanford, Inc., part of the Fluor Daniel Hanford, Inc. lead team on the Project Hanford Management Contract, is constructing facilities and systems to move the fuel from current pool storage to a dry interim storage facility away from the Columbia River, and to treat and dispose of K Basins sludge, debris and water. The process starts in K Basins where fuel elements will be removed from existing canisters, washed, and separated from sludge and scrap fuel pieces. Fuel elements will be placed in baskets and loaded into Multi-Canister Overpacks (MCOs) and into transportation casks. The MCO and cask will be transported to the Cold Vacuum Drying Facility, where free water within the MCO will be removed under vacuum at slightly elevated temperatures. The MCOs will be sealed and transported via the transport cask to the Canister Storage Building.

  5. Direct Measurement of Initial Enrichment and Burn-up of Spent Fuel Assembly with a Differential Die-Away Technique Based Instrument

    SciTech Connect

    Henzl, Vladimir; Swinhoe, Martyn T.; Tobin, Stephen J.

    2012-07-16

    A key objective of the Next Generation Safeguards Initiative (NGSI) is to utilize non-destructive assay (NDA) techniques to determine the elemental plutonium (Pu) content in a commercial-grade nuclear spent fuel assembly (SFA). In the third year of the NGSI Spent Fuel NDA project, the research focus is on the integration of a few NDA techniques. One of the reoccurring challenges to the accurate determination of Pu content has been the explicit dependence of the measured signal on the presence of neutron absorbers which build up in the assembly in accordance with its operating and irradiation history. The history of any SFA is often summarized by the parameters of burn-up (BU), initial enrichment (IE) and cooling time (CT). While such parameters can typically be provided by the operator, the ability to directly measure and verify them would significantly enhance the autonomy of the IAEA inspectorate. Within this paper, we demonstrate that an instrument based on a Differential Die-Away technique is in principle capable of direct measurement of IE and, should the CT be known, also the BU.

  6. Systems impacts of spent fuel disassembly alternatives

    SciTech Connect

    Not Available

    1984-07-01

    Three studies were completed to evaluate four alternatives to the disposal of intact spent fuel assemblies in a geologic repository. A preferred spent fuel waste form for disposal was recommended on consideration of (1) package design and fuel/package interaction, (2) long-term, in-repository performance of the waste form, and (3) overall process performance and costs for packaging, handling, and emplacement. The four basic alternative waste forms considered were (1) end fitting removal, (2) fission gas venting, (3) disassembly and close packing, and (4) shearing/immobilization. None of the findings ruled out any alternative on the basis of waste package considerations or long-term performance of the waste form. The third alternative offers flexibility in loading that may prove attractive in the various geologic media under consideration, greatly reduces the number of packages, and has the lowest unit cost. These studies were completed in October, 1981. Since then Westinghouse Electric Corporation and the Office of Nuclear Waste Isolation have completed studies in related fields. This report is now being published to provide publicly the background material that is contained within. 47 references, 28 figures, 31 tables.

  7. Pyroprocess for processing spent nuclear fuel

    DOEpatents

    Miller, William E.; Tomczuk, Zygmunt

    2002-01-01

    This is a pyroprocess for processing spent nuclear fuel. The spent nuclear fuel is chopped into pieces and placed in a basket which is lowered in to a liquid salt solution. The salt is rich in ZrF.sub.4 and containing alkali or alkaline earth fluorides, and in particular, the salt chosen was LiF-50 mol % ZrF.sub.4 with a eutectic melting point of 500.degree. C. Prior to lowering the basket, the salt is heated to a temperature of between 550.degree. C. and 700.degree. C. in order to obtain a molten solution. After dissolution the oxides of U, Th, rare earth and other like oxides, the salt bath solution is subject to hydro-fluorination to remove the oxygen and then to a fluorination step to remove U as gaseous UF.sub.6. In addition, after dissolution, the basket contains PuO.sub.2 and undissolved parts of the fuel rods, and the basket and its contents are processed to remove the Pu.

  8. Spent fuel management status perspectives in Korea

    SciTech Connect

    Park, H.S.; Lee, J.S.; Kim, B.T. )

    1992-01-01

    Concomitant with steadily increasing nuclear power program in Korea, a national radioactive waste management program has been in initial implementation stage for several years. In late 1990, however, a serious confrontation was witnessed at Anmyon area where residents expressed strong opposition against any possibility to consider that site as a potential candidate for waste disposal by the Authority. As far as spent fuel management is concerned, an interim storage policy was adopted by Korean Atomic Energy Commission. A decision to build a centralized wet storage facility was made followed by a conceptual design. Due to the incident at Anmyon site, the public has became more concerned about radioactive wastes management. Parallel efforts are being made to ameliorate public acceptance in regard to radioactive waste management and in particular to spent fuel management. There are substantial uncertainties, however, whether any site could be found given that precarious mood has been prevailing against radioactive wastes throughout the world. In the meantime waiting for successful siting, various research and development for future perspectives are in order. Of particular importance in such endeavor is to provide technological impetus for future perspectives as well as public acceptance through safety demonstrations of certain viable technology alternatives. The dry storage option, for instance, is acclaimed for intrinsic safety and lower cost as prospective alternative. Combined with rod consolidation, dry storage technologies which have not extensively applied in the past, could be considered as a technological basis for longer term management of spent fuel. Conscious of such global trend, some appropriate programs in preparation for such perspectives have been launched by KAERI.

  9. Some factors to consider in handling and storing spent fuel

    SciTech Connect

    Bailey, W.J.

    1985-11-01

    This report includes information from various studies performed under the Wet Storage Task of the Behavior of Spent Fuel in Storage Project of the Commercial Spent Fuel Management (CSFM) Program at Pacific Northwest Laboratory. Wet storage experience has been summarized earlier in several other reports. This report summarizes pertinent items noted during FY 1985 concerning recent developments in the handling and storage of spent fuel and associated considerations. The subjects discussed include recent publications, findings, and developments associated with: (1) storage of water reactor spent fuel in water pools, (2) extended-burnup fuel, (3) fuel assembly reconstitution and reinsertion, (4) rod consolidation, (5) variations in the US Nuclear Regulatory Commission's definition of failed fuel, (6) detection of failed fuel rods, and (7) extended integrity of spent fuel. A list of pertinent publications is included.

  10. DOE SPENT NUCLEAR FUEL DISPOSAL CONTAINER

    SciTech Connect

    F. Habashi

    1998-06-26

    The DOE Spent Nuclear Fuel Disposal Container (SNF DC) supports the confinement and isolation of waste within the Engineered Barrier System of the Mined Geologic Disposal System (MGDS). Disposal containers are loaded and sealed in the surface waste handling facilities, transferred to the underground through the access mains, and emplaced in emplacement drifts. The DOE Spent Nuclear Fuel Disposal Container provides long term confinement of DOE SNF waste, and withstands the loading, transfer, emplacement, and retrieval loads and environments. The DOE SNF Disposal Containers provide containment of waste for a designated period of time, and limit radionuclide release thereafter. The disposal containers maintain the waste in a designated configuration, withstand maximum handling and rockfall loads, limit the individual waste canister temperatures after emplacement. The disposal containers also limit the introduction of moderator into the disposal container during the criticality control period, resist corrosion in the expected repository environment, and provide complete or limited containment of waste in the event of an accident. Multiple disposal container designs may be needed to accommodate the expected range of DOE Spent Nuclear Fuel. The disposal container will include outer and inner barrier walls and outer and inner barrier lids. Exterior labels will identify the disposal container and contents. Differing metal barriers will support the design philosophy of defense in depth. The use of materials with different failure mechanisms prevents a single mode failure from breaching the waste package. The corrosion-resistant inner barrier and inner barrier lid will be constructed of a high-nickel alloy and the corrosion-allowance outer barrier and outer barrier lid will be made of carbon steel. The DOE Spent Nuclear Fuel Disposal Containers interface with the emplacement drift environment by transferring heat from the waste to the external environment and by protecting

  11. Surrogate Spent Nuclear Fuel Vibration Integrity Investigation

    SciTech Connect

    Wang, Jy-An John; Wang, Hong; Bevard, Bruce Balkcom; Howard, Rob L; Flanagan, Michelle; Bjorkman, Gordon

    2014-01-01

    Transportation packages for spent nuclear fuel (SNF) must meet safety requirements under normal and accident conditions as specified by federal regulations. During transportation, SNF experiences unique conditions and challenges to cladding integrity due to the vibrational and impact loading encountered during road or rail shipment. ORNL has been developing testing capabilities that can be used to improve our understanding of the impacts of vibration loading on SNF integrity, especially for high burn-up SNF in normal transportation operation conditions. This information can be used to meet nuclear industry and U.S. Nuclear Regulatory Commission needs in the area of safety of SNF storage and transportation operations.

  12. Thermomechanical modeling of the Spent Fuel Test-Climax

    SciTech Connect

    Butkovich, T.R.; Patrick, W.C.

    1986-02-01

    The Spent Fuel Test-Climax (SFT-C) was conducted to evaluate the feasibility of retrievable deep geologic storage of commercially generated spent nuclear-reactor fuel assemblies. One of the primary aspects of the test was to measure the thermomechanical response of the rock mass to the extensive heating of a large volume of rock. Instrumentation was emplaced to measure stress changes, relative motion of the rock mass, and tunnel closures during three years of heating from thermally decaying heat sources, followed by a six-month cooldown period. The calculations reported here were performed using the best available input parameters, thermal and mechanical properties, and power levels which were directly measured or inferred from measurements made during the test. This report documents the results of these calculations and compares the results with selected measurements made during heating and cooling of the SFT-C.

  13. Transportation capabilities study of DOE-owned spent nuclear fuel

    SciTech Connect

    Clark, G.L.; Johnson, R.A.; Smith, R.W.; Abbott, D.G.; Tyacke, M.J.

    1994-10-01

    This study evaluates current capabilities for transporting spent nuclear fuel owned by the US Department of Energy. Currently licensed irradiated fuel shipping packages that have the potential for shipping the spent nuclear fuel are identified and then matched against the various spent nuclear fuel types. Also included are the results of a limited investigation into other certified packages and new packages currently under development. This study is intended to support top-level planning for the disposition of the Department of Energy`s spent nuclear fuel inventory.

  14. Spent Fuel Reprocessing: More Value for Money Spent in a Geological Repository?

    SciTech Connect

    Kaplan, P.; Vinoche, R.; Devezeaux, J-G.; Bailly, F.

    2003-02-25

    Today, each utility or country operating nuclear power plants can select between two long-term spent fuel management policies: either, spent fuel is considered as waste to dispose of through direct disposal or, spent fuel is considered a resource of valuable material through reprocessing-recycling. Reading and listening to what is said in the nuclear community, we understand that most people consider that the choice of policy is, actually, a choice among two technical paths to handle spent fuel: direct disposal versus reprocessing. This very simple situation has been recently challenged by analysis coming from countries where both policies are on survey. For example, ONDRAF of Belgium published an interesting study showing that, economically speaking for final disposal, it is worth treating spent fuel rather than dispose of it as a whole, even if there is no possibility to recycle the valuable part of it. So, the question is raised: is there such a one-to-one link between long term spent fuel management political option and industrial option? The purpose of the presentation is to discuss the potential advantages and drawbacks of spent fuel treatment as an implementation of the policy that considers spent fuel as waste to dispose of. Based on technical considerations and industrial experience, we will study qualitatively, and quantitatively when possible, the different answers proposed by treatment to the main concerns of spent-fuel-as-a-whole geological disposal.

  15. A Monte Carlo based spent fuel analysis safeguards strategy assessment

    SciTech Connect

    Fensin, Michael L; Tobin, Stephen J; Swinhoe, Martyn T; Menlove, Howard O; Sandoval, Nathan P

    2009-01-01

    Safeguarding nuclear material involves the detection of diversions of significant quantities of nuclear materials, and the deterrence of such diversions by the risk of early detection. There are a variety of motivations for quantifying plutonium in spent fuel assemblies by means of nondestructive assay (NDA) including the following: strengthening the capabilities of the International Atomic Energy Agencies ability to safeguards nuclear facilities, shipper/receiver difference, input accountability at reprocessing facilities and burnup credit at repositories. Many NDA techniques exist for measuring signatures from spent fuel; however, no single NDA technique can, in isolation, quantify elemental plutonium and other actinides of interest in spent fuel. A study has been undertaken to determine the best integrated combination of cost effective techniques for quantifying plutonium mass in spent fuel for nuclear safeguards. A standardized assessment process was developed to compare the effective merits and faults of 12 different detection techniques in order to integrate a few techniques and to down-select among the techniques in preparation for experiments. The process involves generating a basis burnup/enrichment/cooling time dependent spent fuel assembly library, creating diversion scenarios, developing detector models and quantifying the capability of each NDA technique. Because hundreds of input and output files must be managed in the couplings of data transitions for the different facets of the assessment process, a graphical user interface (GUI) was development that automates the process. This GUI allows users to visually create diversion scenarios with varied replacement materials, and generate a MCNPX fixed source detector assessment input file. The end result of the assembly library assessment is to select a set of common source terms and diversion scenarios for quantifying the capability of each of the 12 NDA techniques. We present here the generalized

  16. HTGR Spent Fuel Treatment Program. HTGR Spent Fuel Treatment Development Program Plan

    SciTech Connect

    Not Available

    1984-12-01

    The spent fuel treatment (SFT) program plan addresses spent fuel volume reduction, packaging, storage, transportation, fuel recovery, and disposal to meet the needs of the HTGR Lead Plant and follow-on plants. In the near term, fuel refabrication will be addressed by following developments in fresh fuel fabrication and will be developed in the long term as decisions on the alternatives dictate. The formulation of this revised program plan considered the implications of the Nuclear Waste Policy Act of 1982 (NWPA) which, for the first time, established a definitive national policy for management and disposal of nuclear wastes. Although the primary intent of the program is to address technical issues, the divergence between commercial and government interests, which arises as a result of certain provisions of the NWPA, must be addressed in the economic assessment of technically feasible alternative paths in the management of spent HTGR fuel and waste. This new SFT program plan also incorporates a significant cooperative research and development program between the United States and the Federal Republic of Germany. The major objective of this international program is to reduce costs by avoiding duplicate efforts.

  17. Dosimetry at an interim storage for spent nuclear fuel.

    PubMed

    Králík, M; Kulich, V; Studeny, J; Pokorny, P

    2007-01-01

    The Czech nuclear power plant Dukovany started its operation in 1985. All fuel spent from 1985 up to the end of 2005 is stored at a dry interim storage, which was designed for 60 CASTOR-440/84 casks. Each of these casks can accommodate 84 fuel assemblies from VVER 440 reactors. Neutron-photon mixed fields around the casks were characterized in terms of ambient dose equivalent measured by standard area dosemeters. Except this, neutron spectra were measured by means of a Bonner sphere spectrometer, and the measured spectra were used to derive the corresponding ambient dose equivalent due to neutrons.

  18. Buckling analysis of spent fuel basket

    SciTech Connect

    Lee, A.S.; Bumpas, S.E.

    1995-05-01

    The basket for a spent fuel shipping cask is subjected to compressive stresses that may cause global instability of the basket assemblies or local buckling of the individual members. Adopting the common buckling design practice in which the stability capacity of the entire structure is based on the performance of the individual members of the assemblies, the typical spent fuel basket, which is composed of plates and tubular structural members, can be idealized as an assemblage of columns, beam-columns and plates. This report presents the flexural buckling formulas for five load cases that are common in the basket buckling analysis: column under axial loads, column under axial and bending loads, plate under uniaxial loads, plate under biaxial loadings, and plate under biaxial loads and lateral pressure. The acceptance criteria from the ASME Boiler and Pressure Vessel Code are used to determine the adequacy of the basket components. Special acceptance criteria are proposed to address the unique material characteristics of austenitic stainless steel, a material which is frequently used in the basket assemblies.

  19. K Basin spent nuclear fuel characterization

    SciTech Connect

    LAWRENCE, L.A.

    1999-02-10

    The results of the characterization efforts completed for the N Reactor fuel stored in the Hanford K Basins were Collected and summarized in this single referencable document. This summary provides a ''road map'' for what was done and the results obtained for the fuel characterization program initiated in 1994 and scheduled for completion in 1999 with the fuel oxidation rate measurement under moist inert atmospheres.

  20. Spent fuel management fee methodology and computer code user's manual.

    SciTech Connect

    Engel, R.L.; White, M.K.

    1982-01-01

    The methodology and computer model described here were developed to analyze the cash flows for the federal government taking title to and managing spent nuclear fuel. The methodology has been used by the US Department of Energy (DOE) to estimate the spent fuel disposal fee that will provide full cost recovery. Although the methodology was designed to analyze interim storage followed by spent fuel disposal, it could be used to calculate a fee for reprocessing spent fuel and disposing of the waste. The methodology consists of two phases. The first phase estimates government expenditures for spent fuel management. The second phase determines the fees that will result in revenues such that the government attains full cost recovery assuming various revenue collection philosophies. These two phases are discussed in detail in subsequent sections of this report. Each of the two phases constitute a computer module, called SPADE (SPent fuel Analysis and Disposal Economics) and FEAN (FEe ANalysis), respectively.

  1. Investigation of the condition of spent-fuel pool components

    SciTech Connect

    Kustas, F.M.; Bates, S.O.; Opitz, B.E.; Johnson, A.B. Jr.; Perez, J.M. Jr.; Farnsworth, R.K.

    1981-09-01

    It is currently projected that spent nuclear fuel, which is discharged from the reactor and then stored in water pools, may remain in those pools for several decades. Other studies have addressed the expected integrity of the spent fuel during extended water storage; this study assesses the integrity of metallic spent fuel pool components. Results from metallurgical examinations of specimens taken from stainless steel and aluminum components exposed in spent fuel pools are presented. Licensee Event Reports (LERs) relating to problems with spent fuel components were assessed and are summarized to define the types of operational problems that have occurred. The major conclusions of this study are: aluminum and stainless steel spent fuel pool components have a good history of performance in both deionized and borated water pools. Although some operational problems involving pool components have occurred, these problems have had minimal impacts.

  2. US Spent (Used) Fuel Status, Management and Likely Directions- 12522

    SciTech Connect

    Jardine, Leslie J.

    2012-07-01

    As of 2010, the US has accumulated 65,200 MTU (42,300 MTU of PWR's; 23,000 MTU of BWR's) of spent (irradiated or used) fuel from 104 operating commercial nuclear power plants situated at 65 sites in 31 States and from previously shutdown commercial nuclear power plants. Further, the Department of Energy (DOE) has responsibility for an additional 2458 MTU of DOE-owned defense and non defense spent fuel from naval nuclear power reactors, various non-commercial test reactors and reactor demonstrations. The US has no centralized large spent fuel storage facility for either commercial spent fuel or DOE-owned spent fuel. The 65,200 MTU of US spent fuel is being safely stored by US utilities at numerous reactor sites in (wet) pools or (dry) metal or concrete casks. As of November 2010, the US had 63 'independent spent fuel storage installations' (or ISFSI's) licensed by the US Nuclear Regulatory Commission located at 57 sites in 33 states. Over 1400 casks loaded with spent fuel for dry storage are at these licensed ISFSI's; 47 sites are located at commercial reactor sites and 10 are located 'away' from a reactor (AFR's) site. DOE's small fraction of a 2458 MTU spent fuel inventory, which is not commercial spent fuel, is with the exception of 2 MTU, being stored at 4 sites in 4 States. The decades old US policy of a 'once through' fuel cycle with no recycle of spent fuel was set into a state of 'mass confusion or disruption' when the new US President Obama's administration started in early 2010 stopping the only US geologic disposal repository at the Yucca Mountain site in the State of Nevada from being developed and licensed. The practical result is that US nuclear power plant operators will have to continue to be responsible for managing and storing their own spent fuel for an indefinite period of time at many different sites in order to continue to generate electricity because there is no current US government plan, schedule or policy for taking possession of

  3. BWR Spent Nuclear Fuel Integrity Research and Development Survey for UKABWR Spent Fuel Interim Storage

    SciTech Connect

    Bevard, Bruce Balkcom; Mertyurek, Ugur; Belles, Randy; Scaglione, John M.

    2015-10-01

    The objective of this report is to identify issues and support documentation and identify and detail existing research on spent fuel dry storage; provide information to support potential R&D for the UKABWR (United Kingdom Advanced Boiling Water Reactor) Spent Fuel Interim Storage (SFIS) Pre-Construction Safety Report; and support development of answers to questions developed by the regulator. Where there are gaps or insufficient data, Oak Ridge National Laboratory (ORNL) has summarized the research planned to provide the necessary data along with the schedule for the research, if known. Spent nuclear fuel (SNF) from nuclear power plants has historically been stored on site (wet) in spent fuel pools pending ultimate disposition. Nuclear power users (countries, utilities, vendors) are developing a suite of options and set of supporting analyses that will enable future informed choices about how best to manage these materials. As part of that effort, they are beginning to lay the groundwork for implementing longer-term interim storage of the SNF and the Greater Than Class C (CTCC) waste (dry). Deploying dry storage will require a number of technical issues to be addressed. For the past 4-5 years, ORNL has been supporting the U.S. Department of Energy (DOE) in identifying these key technical issues, managing the collection of data to be used in issue resolution, and identifying gaps in the needed data. During this effort, ORNL subject matter experts (SMEs) have become expert in understanding what information is publicly available and what gaps in data remain. To ensure the safety of the spent fuel under normal and frequent conditions of wet and subsequent dry storage, intact fuel must be shown to: 1.Maintain fuel cladding integrity; 2.Maintain its geometry for cooling, shielding, and subcriticality; 3.Maintain retrievability, and damaged fuel with pinhole or hairline cracks must be shown not to degrade further. Where PWR (pressurized water reactor) information is

  4. Arrival condition of spent fuel after storage, handling, and transportation

    SciTech Connect

    Bailey, W.J.; Pankaskie, P.J.; Langstaff, D.C.; Gilbert, E.R.; Rising, K.H.; Schreiber, R.E.

    1982-11-01

    This report presents the results of a study conducted to determine the probable arrival condition of spent light-water reactor (LWR) fuel after handling and interim storage in spent fuel storage pools and subsequent handling and accident-free transport operations under normal or slightly abnormal conditions. The objective of this study was to provide information on the expected condition of spent LWR fuel upon arrival at interim storage or fuel reprocessing facilities or at disposal facilities if the fuel is declared a waste. Results of a literature survey and data evaluation effort are discussed. Preliminary threshold limits for storing, handling, and transporting unconsolidated spent LWR fuel are presented. The difficulty in trying to anticipate the amount of corrosion products (crud) that may be on spent fuel in future shipments is also discussed, and potential areas for future work are listed. 95 references, 3 figures, 17 tables.

  5. Simulated Performance of the Integrated Passive Neutron Albedo Reactivity and Self-Interrogation Neutron Resonance Densitometry Detector Designed for Spent Fuel Measurement at the Fugen Reactor in Japan

    SciTech Connect

    Ulrich, Timothy J. II; Lafleur, Adrienne M.; Menlove, Howard O.; Swinhoe, Martyn T.; Tobin, Stephen J.; Seya, Michio; Bolind, Alan M.

    2012-07-16

    An integrated nondestructive assay instrument, which combined the Passive Neutron Albedo Reactivity (PNAR) and the Self-Interrogation Neutron Resonance Densitometry (SINRD) techniques, is the research focus for a collaborative effort between Los Alamos National Laboratory (LANL) and the Japanese Atomic Energy Agency as part of the Next Generation Safeguard Initiative. We will quantify the anticipated performance of this experimental system in two physical environments: (1) At LANL we will measure fresh Low Enriched Uranium (LEU) assemblies for which the average enrichment can be varied from 0.2% to 3.2% and for which Gd laced rods will be included. (2) At Fugen we will measure spent Mixed Oxide (MOX-B) and LEU spent fuel assemblies from the heavy water moderated Fugen reactor. The MOX-B assemblies will vary in burnup from {approx}3 GWd/tHM to {approx}20 GWd/tHM while the LEU assemblies ({approx}1.9% initial enrichment) will vary from {approx}2 GWd/tHM to {approx}7 GWd/tHM. The estimated count rates will be calculated using MCNPX. These preliminary results will help the finalization of the hardware design and also serve a guide for the experiment. The hardware of the detector is expected to be fabricated in 2012 with measurements expected to take place in 2012 and 2013. This work is supported by the Next Generation Safeguards Initiative, Office of Nuclear Safeguards and Security, National Nuclear Security Administration.

  6. Concentration of uranium and plutonium in unsaturated spent fuel tests.

    SciTech Connect

    Finn, P. A.

    1998-04-15

    Commercial spent fuel is being tested under oxidizing conditions at 90 C in drip tests with simulated groundwater to evaluate its long-term performance in a potential repository at Yucca Mountain [1-4]. The tests allow us to monitor the dissolution behavior of the spent fuel matrix and the release rates of individual radionuclides. This paper reports the U and Pu concentrations in the leachates of drip tests during 3.7 years of reaction. Changes in these concentrations are correlated with changes in the measured pH and the appearance of alteration products on the fuel surface. Although there is little thermodynamic information at 90 C for either uranyl or plutonium compounds, some data are available at 25 C [5-8]. The literature data for the U and Pu solubilities of U and Pu compounds were compared to the U and Pu concentrations in the leachates. We also compare Wilson's [9] U and Pu concentrations in semi-static tests at 85 C on spent fuel with our results.

  7. Characterization plan for Hanford spent nuclear fuel

    SciTech Connect

    Abrefah, J.; Thornton, T.A.; Thomas, L.E.; Berting, F.M.; Marschman, S.C.

    1994-12-01

    Reprocessing of spent nuclear fuel (SNF) at the Hanford Site Plutonium-Uranium Extraction Plant (PUREX) was terminated in 1972. Since that time a significant quantity of N Reactor and Single-Pass Reactor SNF has been stored in the 100 Area K-East (KE) and K-West (KW) reactor basins. Approximately 80% of all US Department of Energy (DOE)-owned SNF resides at Hanford, the largest portion of which is in the water-filled KE and KW reactor basins. The basins were not designed for long-term storage of the SNF and it has become a priority to move the SNF to a more suitable location. As part of the project plan, SNF inventories will be chemically and physically characterized to provide information that will be used to resolve safety and technical issues for development of an environmentally benign and efficient extended interim storage and final disposition strategy for this defense production-reactor SNF.

  8. Spent nuclear fuel project technical databook

    SciTech Connect

    Reilly, M.A.

    1998-07-22

    The Spent Nuclear Fuel (SNF) project technical databook provides project-approved summary tables of selected parameters and derived physical quantities, with nominal design and safety basis values. It contains the parameters necessary for a complete documentation basis of the SNF Project technical and safety baseline. The databook is presented in two volumes. Volume 1 presents K Basins SNF related information. Volume 2 (not yet available) will present selected sludge and water information, as it relates to the sludge and water removal projects. The values, within this databook, shall be used as the foundation for analyses, modeling, assumptions, or other input to SNF project safety analyses or design. All analysis and modeling using a parameter available in this databook are required to use and cite the appropriate associated value, and document any changes to those values (i.e., analysis assumptions, equipment conditions, etc). Characterization and analysis efforts are ongoing to validate, or update these values.

  9. Nevada commercial spent nuclear fuel transportation experience

    SciTech Connect

    1991-09-01

    The purpose of this report is to present an historic overview of commercial reactor spent nuclear fuel (SNF) shipments that have occurred in the state of Nevada, and to review the accident and incident experience for this type of shipments. Results show that between 1964 and 1990, 309 truck shipments covering approximately 40,000 miles moved through Nevada; this level of activity places Nevada tenth among the states in the number of truck shipments of SNF. For the same period, 15 rail shipments moving through the State covered approximately 6,500 miles, making Nevada 20th among the states in terms of number of rail shipments. None of these shipments had an accident or an incident associated with them. Because the data for Nevada are so limited, national data on SNF transportation and the safety of truck and rail transportation in general were also assessed.

  10. Spent nuclear fuel storage -- Performance tests and demonstrations

    SciTech Connect

    McKinnon, M.A.; DeLoach, V.A.

    1993-04-01

    This report summarizes the results of heat transfer and shielding performance tests and demonstrations conducted from 1983 through 1992 by or in cooperation with the US Department of Energy (DOE), Office of Commercial Radioactive Waste Management (OCRWM). The performance tests consisted of 6 to 14 runs involving one or two loadings, usually three backfill environments (helium, nitrogen, and vacuum backfills), and one or two storage system orientations. A description of the test plan, spent fuel load patterns, results from temperature and dose rate measurements, and fuel integrity evaluations are contained within the report.

  11. Determination of total Pu content in a Spent Fuel Assembly by Measuring Passive Neutron Count rate and Multiplication with the Differential Die-Away Instrument

    SciTech Connect

    Henzl, Vladimir; Croft, Stephen; Swinhoe, Martyn T.; Tobin, Stephen J.

    2012-07-18

    A key objective of the Next Generation Safeguards Initiative (NGSI) is to evaluate and develop non-destructive assay (NDA) techniques to determine the elemental plutonium content in a commercial-grade nuclear spent fuel assembly (SFA) [1]. Within this framework, we investigate by simulation a novel analytical approach based on combined information from passive measurement of the total neutron count rate of a SFA and its multiplication determined by the active interrogation using an instrument based on a Differential Die-Away technique (DDA). We use detailed MCNPX simulations across an extensive set of SFA characteristics to establish the approach and demonstrate its robustness. It is predicted that Pu content can be determined by the proposed method to a few %.

  12. Spent Fuel Storage Operational Experience With Increased Crud Activities

    SciTech Connect

    Barnabas, I.; Eigner, T.; Gresits, I.; Ordagh, M.

    2008-07-01

    A significant part of the electricity production in Hungary is provided by 4 units of VVER 440 nuclear reactors at the Paks Nuclear Power Plant. Interim dry storage of the spent fuel assemblies that are generated during the operation of the reactors is provided in a Modular Vault Dry Storage (MVDS) facility that is located in the immediate vicinity of the Paks Nuclear Power Plant. The storage capacity of the MVDS is being continuously extended in accordance with spent the fuel production rate from the four reactors. An accident occurred at unit 2 of the Paks Nuclear Power Plant in 2003, when thirty irradiated fuel assemblies were damaged during a cleaning process. The fuel assemblies were not inside the reactor at the time of the accident, but in a separate tank within the adjacent fuel decay pool. As a result of this accident, contamination from the badly damaged fuel assemblies spread to the decay pool water and also became deposited onto the surface of (hermetic) spent fuel assemblies within the decay pool. Therefore, it was necessary to review the design basis of the MVDS and assess the effects of taking the surface contaminated spent fuel assemblies into dry storage. The contaminated hermetic assemblies were transferred from the unit 2 pool to the interim storage facility in the period between 2005 and 2007. Continuous inspection and measurement was carried out during the transfer of these fuel assemblies. On the basis of the design assessments and measurement of the results during the fuel transfer, it was shown that radiological activity values increased due to the consequences of the accident but that these levels did not compromise the release and radiation dose limits for the storage facility. The aim of this paper is to show the effect on the operation of the MVDS interim storage facility as a result of the increased activity values due to the accident that occurred in 2003, as well as to describe the measurements that were taken, and their results and

  13. Operational and technical results from the Spent Fuel Test - Climax

    SciTech Connect

    Patrick, W.C.

    1985-01-01

    The technical feasibility of short-term storage and retrieval of spent nuclear fuel assemblies has recently been demonstrated in a test of deep geologic storage at the US Department of Energy Nevada Test Site (NTS). Handling systems and procedures developed and deployed on this test functioned safely and reliably to emplace eleven intact spent-fuel assemblies and retrieve them three years later. Three exchanges of spent fuel were conducted at regular intervals during the storage period to maintain the proficiency of personnel and the readiness of the handling system. Technical data was collected using nearly 1000 instruments. These data show that the mechanical and thermal properties of granites are compatible with nuclear waste isolation objectives. Measured and calculated temperatures are in excellent agreement, confirming the adequacy of available heat transfer codes. Radiation transport calculations were of high quality, exceeding the accuracy of available long-term dosimetry techniques which were used on the test. We also found good agreement between measured and calculated displacements within the rock mass. 28 references, 4 figures.

  14. An approach to meeting the spent fuel standard

    SciTech Connect

    Makhijani, A.

    1996-05-01

    The idea of the spent fuel standard is that there should be a high surface gamma radiation to prevent theft. For purposes of preventing theft, containers should be massive, and the plutonium should be difficult to extract. This report discusses issues associated with the spent fuel standard.

  15. Breeder Spent Fuel Handling Program multipurpose cask design basis document

    SciTech Connect

    Duckett, A.J.; Sorenson, K.B.

    1985-09-01

    The Breeder Spent Fuel Handling (BSFH) Program multipurpose cask Design Basis Document defines the performance requirements essential to the development of a legal weight truck cask to transport FFTF spent fuel from reactor to a reprocessing facility and the resultant High Level Waste (HLW) to a repository. 1 ref.

  16. Storage of LWR spent fuel in air: Volume 1: Design and operation of a spent fuel oxidation test facility

    SciTech Connect

    Thornhill, C.K.; Campbell, T.K.; Thornhill, R.E.

    1988-12-01

    This report describes the design and operation and technical accomplishments of a spent-fuel oxidation test facility at the Pacific Northwest Laboratory. The objective of the experiments conducted in this facility was to develop a data base for determining spent-fuel dry storage temperature limits by characterizing the oxidation behavior of light-water reactor (LWR) spent fuels in air. These data are needed to support licensing of dry storage in air as an alternative to spent-fuel storage in water pools. They are to be used to develop and validate predictive models of spent-fuel behavior during dry air storage in an Independent Spent Fuel Storage Installation (ISFSI). The present licensed alternative to pool storage of spent fuel is dry storage in an inert gas environment, which is called inerted dry storage (IDS). Licensed air storage, however, would not require monitoring for maintenance of an inert-gas environment (which IDS requires) but does require the development of allowable temperature limits below which UO/sub 2/ oxidation in breached fuel rods would not become a problem. Scoping tests at PNL with nonirradiated UO/sub 2/ pellets and spent-fuel fragment specimens identified the need for a statistically designed test matrix with test temperatures bounding anticipated maximum acceptable air-storage temperatures. This facility was designed and operated to satisfy that need. 7 refs.

  17. Determination of Plutonium Content in Spent Fuel with Nondestructive Assay

    SciTech Connect

    Tobin, S. J.; Sandoval, N. P.; Fensin, M. L.; Lee, S. Y.; Ludewigt, Bernhard A.; Menlovea, H. O.; Quiter, B. J.; Rajasingume, A.; Schearf, M. A.; Smith, L. E.; Swinhoe, M. T.; Thompson, S. J.

    2009-06-30

    There are a variety of reasons for quantifying plutonium (Pu) in spent fuel such as independently verifying the Pu content declared by a regulated facility, making shipper/receiver mass declarations, and quantifying the input mass at a reprocessing facility. As part of the Next Generation Safeguards Initiative, NA-241 has recently funded a multilab/university collaboration to determine the elemental Pu mass in spent fuel assemblies. This research effort is anticipated to be a five year effort: the first part of which is a two years Monte Carlo modeling effort to integrate and down-select among 13 nondestructive assay (NDA) technologies, followed by one year for fabricating instruments and then two years for measuring spent fuel. This paper gives a brief overview of the approach being taken for the Monte Carlo research effort. In addition, preliminary results for the first NDA instrument studied in detail, delayed neutron detection, will be presented. In order to cost effectively and robustly model the performance of several NDA techniques, an"assembly library" was created that contains a diverse range of pressurized water reactor spent fuel assemblies (burnup, enrichment, cooling time) similar to that which exists in spent pools today and in the future, diversion scenarios that capture a range of possible rod removal options, spatial and isotopic detail needed to accurately quantify the capability of all the NDA techniques so as to enable integration. Integration is being designed into this study from the beginning since it is expected that the best performance will be obtained by combining a few NDA techniques. The performance of each instrument will be quantified for the full assembly library in three different media: air, water and borated water. In this paper the preliminary capability of delayed neutron detection will be quantified for the spent fuel library for all three media. The 13 NDA techniques being researched are the following: Delayed Gamma, Delayed

  18. Shippingport Spent Fuel Canister System Description

    SciTech Connect

    JOHNSON, D.M.

    2001-06-26

    In 1978 and 1979, a total of 72 blanket fuel assemblies (BFAs), irradiated during the operating cycles of the Shippingport Atomic Power Station's Pressurized Water Reactor (PWR) Core 2 from April 1965 to February 1974, were transferred to the Hanford Site and stored in underwater storage racks in Cell 2R at the 221-T Canyon (T-Plant). The initial objective was to recover the produced plutonium in the BFAs, but this never occurred and the fuel assemblies have remained within the water storage pool to the present time. The Shippingport Spent Fuel Canister (SSFC) is a confinement system that provides safe transport functions (in conjunction with the TN-WHC cask) and storage for the BFAs at the Canister Storage Building (CSB). The current plan is for these BFAs to be retrieved from wet storage and loaded into SSFCs for dry storage. The sealed SSFCs containing BFAs will be vacuum dried, internally backfilled with helium, and leak tested to provide suitable confinement for the BFAs during transport and storage. Following completion of the drying and inerting process, the SSFCs are to be delivered to the CSB for closure welding and long-term interim storage. The CSH will provide safe handling and dry storage for the SSFCs containing the BFAs. The purpose of this document is to describe the SSFC system and interface equipment, including the technical basis for the system, design descriptions, and operations requirements. It is intended that this document will be periodically updated as more equipment design and performance specification information becomes available.

  19. Shippingport Spent Fuel Canister System Description

    SciTech Connect

    JOHNSON, D.M.

    2000-03-27

    In 1978 and 1979, a total of 72 blanket fuel assemblies (BFAs), irradiated during the operating cycles of the Shippingport Atomic Power Station's Pressurized Water Reactor (PWR) Core 2 from April 1965 to February 1974, were transferred to the Hanford Site and stored in underwater storage racks in Cell 2R at the 221-T Canyon (T-Plant). The initial objective was to recover the produced plutonium in the BFAs, but this never occurred and the fuel assemblies have remained within the water storage pool to the present time. The Shippingport Spent Fuel Canister (SSFC) is a confinement system that provides safe transport functions (in conjunction with the TN-WHC cask) and storage for the BFAs at the Canister Storage Building (CSB). The current plan is for these BFAs to be retrieved from wet storage and loaded into SSFCs for dry storage. The sealed SSFCs containing BFAs will be vacuum dried, internally backfilled with helium, and leak tested to provide suitable confinement for the BFAs during transport and storage. Following completion of the drying and inerting process, the SSFCs are to be delivered to the CSB for closure welding and long-term interim storage. The CSB will provide safe handling and dry storage for the SSFCs containing the BFAs. The purpose of this document is to describe the SSFC system and interface equipment, including the technical basis for the system, design descriptions, and operations requirements. It is intended that this document will be periodically updated as more equipment design and performance specification information becomes available.

  20. Case histories of West Valley spent fuel shipments: Final report

    SciTech Connect

    Not Available

    1987-01-01

    In 1983, NRC/FC initiated a study on institutional issues related to spent fuel shipments originating at the former spent fuel processing facility in West Valley, New York. FC staff viewed the shipment campaigns as a one-time opportunity to document the institutional issues that may arise with a substantial increase in spent fuel shipping activity. NRC subsequently contracted with the Aerospace Corporation for the West Valley Study. This report contains a detailed description of the events which took place prior to and during the spent fuel shipments. The report also contains a discussion of the shipment issues that arose, and presents general findings. Most of the institutional issues discussed in the report do not fall under NRC's transportation authority. The case histories provide a reference to agencies and other institutions that may be involved in future spent fuel shipping campaigns. 130 refs., 7 figs., 19 tabs.

  1. DEVELOPMENT OF ELECTROCHEMICAL REDUCTION TECHNOLOGY FOR SPENT OXIDE FUELS

    SciTech Connect

    Hur, Jin-Mok; Seo, Chung-Seok; Kim, Ik-Soo; Hong, Sun-Seok; Kang, Dae-Seung; Park, Seong-Won

    2003-02-27

    The Advanced Spent Fuel Conditioning Process (ACP) has been under development at Korea Atomic Energy Research Institute (KAERI) since 1997. The concept is to convert spent oxide fuel into metallic form and to remove high heat-load fission products such as Cs and Sr from the spent fuel. The heat power, volume, and radioactivity of spent fuel can decrease by a factor of a quarter via this process. For the realization of ACP, a concept of electrochemical reduction of spent oxide fuel in Li2O-LiCl molten salt was proposed and several cold tests using fresh uranium oxides have been carried out. In this new electrochemical reduction process, electrolysis of Li2O and reduction of uranium oxide are taking place simultaneously at the cathode part of electrolysis cell. The conversion of uranium oxide to uranium metal can reach more than 99% ensuring the feasibility of this process.

  2. An extension of the validation of SCALE (SAS2H) isotopic predictions for PWR spent fuel

    SciTech Connect

    DeHart, M.D.; Hermann, O.W.

    1996-09-01

    Isotopic characterization of spent fuel via depletion and decay calculations is necessary for determination of source terms. Unlike fresh fuel assumptions typically used in criticality safety analysis of spent fuel configurations, burnup credit applications also rely on depletion and decay calculations to predict spent fuel composition; these isotopics are used in subsequent criticality calculations to assess the reduced worth of spent fuel. To validate the depletion codes and data, experiment is compared with predictions; such comparisons have been done in earlier ORNL work. This report describes additional independent measurements and corresponding calculations as a supplement. The current work includes measured isotopic data from 19 spent fuel samples from the Italian Trino Vercelles PWR and the US Turkey Point-3 PWR. In addition, an approach to determine biases and uncertainties between calculated and measured isotopic concentrations is discussed, together with a method to statistically combine these terms to obtain a conservative estimate of spent fuel isotopic concentrations. Results on combination of measured-to-calculated ratios are presented. The results described herein represent an extension to a new reactor design and spent fuel samples with enrichment as high as 3.9 wt% {sup 235}U. Consistency with the earlier work for each of two different cross-section libraries suggests that the estimated biases for each of the isotopes in the earlier work are reasonably good estimates.

  3. Regeneration of ammonia borane spent fuel

    SciTech Connect

    Sutton, Andrew David; Davis, Benjamin L; Gordon, John C

    2009-01-01

    A necessary target in realizing a hydrogen (H{sub 2}) economy, especially for the transportation sector, is its storage for controlled delivery, presumably to an energy producing fuel cell. In this vein, the U.S. Department of Energy's Centers of Excellence (CoE) in Hydrogen Storage have pursued different methodologies, including metal hydrides, chemical hydrides, and sorbents, for the expressed purpose of supplanting gasoline's current > 300 mile driving range. Chemical H{sub 2} storage has been dominated by one appealing material, ammonia borane (H{sub 3}N-BH{sub 3}, AB), due to its high gravimetric capacity of H{sub 2} (19.6 wt %) and low molecular weight (30.7 g mol{sup -1}). In addition, AB has both hydridic and protic moieties, yielding a material from which H{sub 2} can be readily released in contrast to the loss of H{sub 2} from C{sub 2}H{sub 6} which is substantially endothermic. As such, a number of publications have described H{sub 2} release from amine boranes, yielding various rates depending on the method applied. The viability of any chemical H{sub 2} storage system is critically dependent on efficient recyclability, but reports on the latter subject are sparse, invoke the use of high energy reducing agents, and suffer from low yields. Our group is currently engaged in trying to find and fully demonstrate an energy efficient regeneration process for the spent fuel from H{sub 2} depleted AB with a minimum number of steps. Although spent fuel composition depends on the dehydrogenation method, we have focused our efforts on the spent fuel resulting from metal-based catalysis, which has thus far shown the most promise. Metal-based catalysts have produced the fastest rates for a single equivalent of H{sub 2} released from AB and up to 2.5 equiv. of H{sub 2} can be produced within 2 hours. While ongoing work is being carried out to tailor the composition of spent AB fuel, a method has been developed for regenerating the predominant product, polyborazylene

  4. Spent-fuel characterization with small CZT detectors

    NASA Astrophysics Data System (ADS)

    Berndt, R.; Mortreau, P.

    2006-08-01

    CdTe detectors may be utilised as miniature instruments for the measurement of gamma spectra in safeguards applications [R. Arlt, V. Gryshchuk, P. Sumah, Nucl. Instr. and Meth. A 428 (1999) 127]. This is applicable for measurements both to fresh fuel and irradiated nuclear fuel. The spectrum analysis, however, is more complicated than with Ge detectors. Some reasons are: the peaks are asymmetric, the peak/Compton ratio is low, peak parameters depend on the count rate and on the properties of individual detector crystals. We developed a spectrum-unfolding code for spectra obtained with CdTe detectors. The code makes use of a series of pattern spectra of the individual instrument. It is applied to fission-product spectra and allows the coarse characterisation of the spent fuel in safeguards inspections.

  5. Spent-fuel dry-storage testing at E-MAD (March 1978-March 1982)

    SciTech Connect

    Unterzuber, R.; Milnes, R.D.; Marinkovich, B.A.; Kubancsek, G.M.

    1982-09-01

    From March 1978 through March 1982, spent fuel dry storage tests were conducted at the Engine Maintenance, Assembly and Disassembly (E-MAD) facility on the Nevada Test Site to confirm that commercial reactor spent fuel could be encapsulated and passively stored in one or more interim dry storage cell concepts. These tests were: electrically heated drywell, isolated and adjacent drywell, concrete silo, fuel assembly internal temperature measurement, and air-cooled vault. This document presents the test data and results as well as results from supporting test operations (spent fuel calorimetry and canister gas sampling).

  6. Concrete Shield Performance of the VSC-17 Spent Nuclear Fuel Cask

    SciTech Connect

    Koji Shirai

    2006-04-01

    The VSC-17 Spent Nuclear Fuel Storage Cask was surveyed for degradation of the concrete shield by radiation measurement, temperature measurement, and ultrasonic testing. No general loss of shielding function was identified.

  7. The synchronous active neutron detection system for spent fuel assay

    SciTech Connect

    Pickrell, M.M.; Kendall, P.K.

    1994-10-01

    The authors have begun to develop a novel technique for active neutron assay of fissile material in spent nuclear fuel. This approach will exploit the unique operating features of a 14-MeV neutron generator developed by Schlumberger. This generator and a novel detection system will be applied to the direct measurement of the fissile material content in spent fuel in place of the indirect measures used at present. The technique they are investigating is termed synchronous active neutron detection (SAND). It closely follows a method that has been used routinely in other branches of physics to detect very small signals in the presence of large backgrounds. Synchronous detection instruments are widely available commercially and are termed {open_quotes}lock-in{close_quotes} amplifiers. The authors have implemented a digital lock-in amplifier in conjunction with the Schlumberger neutron generator to explore the possibility of synchronous detection with active neutrons. This approach is possible because the Schlumberger system can operate at up to a 50% duty factor, in effect, a square wave of neutron yield. The results to date are preliminary but quite promising. The system is capable of resolving the fissile material contained in a small fraction of the fuel rods in a cold fuel assembly. It also appears to be quite resilient to background neutron interference. The interrogating neutrons appear to be nonthermal and penetrating. Although a significant amount of work remains to fully explore the relevant physics and optimize the instrument design, the underlying concept appears sound.

  8. Equipment designs for the spent LWR fuel dry storage demonstration

    SciTech Connect

    Steffen, R.J.; Kurasch, D.H.; Hardin, R.T.; Schmitten, P.F.

    1980-01-01

    In conjunction with the Spent Fuel Handling and Packaging Program (SFHPP) equipment has been designed, fabricated and successfully utilized to demonstrate the packaging and interim dry storage of spent LWR fuel. Surface and near surface storage configurations containing PWR fuel assemblies are currently on test and generating baseline data. Specific areas of hardware design focused upon include storage cell components and the support related equipment associated with encapsulation, leak testing, lag storage, and emplacement operations.

  9. Spent nuclear fuel discharges from U.S. reactors 1994

    SciTech Connect

    1996-02-01

    Spent Nuclear Fuel Discharges from US Reactors 1994 provides current statistical data on fuel assemblies irradiated at commercial nuclear reactors operating in the US. This year`s report provides data on the current inventories and storage capacities at these reactors. Detailed statistics on the data are presented in four chapters that highlight 1994 spent fuel discharges, storage capacities and inventories, canister and nonfuel component data, and assembly characteristics. Five appendices, a glossary, and bibliography are also included. 10 figs., 34 tabs.

  10. Cell for a spent nuclear fuel rack

    SciTech Connect

    Flynn, W.M.

    1987-09-22

    This patent describes a cell for a spent fuel rack, comprising: a sheet metal element having an inside surface and an outside surface, and including a first flat wall portion, a second flat wall portion disposed perpendicularly to the first wall portion, a third flat wall portion disposed perpendicularly to the second wall portion and parallel to the first wall portion, a fourth flat wall portion disposed perpendicularly to the first and third wall portions and parallel to the second wall portion, an elongated bent region joining the first and second wall portions, an additional elongated bent region joining the second and third wall portions, a further elongated bent region joining the third and fourth wall portions, another elongated flat platform portion that is disposed parallel to the fourth wall portion but that is not coplanar with the fourth wall portion, and another elongated flat platform portion that is disposed parallel to the first wall portion but that is not coplanar with the first wall portion; means for joining the another platform portions; four sheets of neutron poison; and four sheet metal wrappers, each securing a respective neutron poison sheet to a respective wall portion.

  11. Disposition of ORNL's Spent Nuclear Fuel

    SciTech Connect

    Turner, D. W.; DeMonia, B. C.; Horton, L. L.

    2002-02-26

    This paper describes the process of retrieving, repackaging, and preparing Oak Ridge spent nuclear fuel (SNF) for off-site disposition. The objective of the Oak Ridge SNF Project is to safely, reliably, and efficiently manage SNF that is stored on the Oak Ridge Reservation until it can be shipped off-site. The project required development of several unique processes and the design and fabrication of special equipment to enable the successful retrieval, transfer, and repackaging of Oak Ridge SNF. SNF was retrieved and transferred to a hot cell for repackaging. After retrieval of SNF packages, the storage positions were decontaminated and stainless steel liners were installed to resolve the vulnerability of water infiltration. Each repackaged SNF canister has been transferred from the hot cell back to dry storage until off-site shipments can be made. Three shipments of aluminum-clad SNF were made to the Savannah River Site (SRS), and five shipments of non-aluminum-clad SNF are planned to the Idaho National Engineering and Environmental Laboratory (INEEL). Through the integrated cooperation of several organizations including the U.S. Department of Energy (DOE), Bechtel Jacobs Company LLC (BJC), Oak Ridge National Laboratory (ORNL), and various subcontractors, preparations for the disposition of SNF in Oak Ridge have been performed in a safe and successful manner.

  12. EBR-II spent fuel treatment demonstration project status

    SciTech Connect

    Benedict, R.W.; Henslee, S.P.

    1998-07-01

    The application of electrometallurgical technology to spent nuclear fuel treatment is being demonstrated by treating 410 kg uranium spent driver fuel and 1,200 kg uranium spent blanket fuel from the Experimental Breeder Reactor-II (EBR-II) spent driver and blanket fuel. This fuel is a metallic uranium alloy and contains elemental sodium, which is a reactive material. Since reactive material is considered hazardous by US Environmental Protection Agency regulations, this fuel requires treatment before disposal in a geologic repository. The EBR-II spent fuel treatment demonstration conditions this fuel in an integrated process where the fuel is converted into three different products: low enriched uranium (LEU), ceramic waste and metallic waste. This demonstration was initiated in June 1996 and has treated approximately 50% of the driver fuel. The higher throughput equipment that will be used for blanket treatment processes has been installed in the hot cell facility and is being tested with depleted uranium. Metal waste forms have been produced from the irradiated metals from the driver fuel. Ceramic waste process equipment has been built and is being tested before installation in the hot cell facilities. This paper discusses the processes and the current results from the first 20 months of operation.

  13. Spent Fuel Transportation Package Performance Study - Experimental Design Challenges

    SciTech Connect

    Snyder, A. M.; Murphy, A. J.; Sprung, J. L.; Ammerman, D. J.; Lopez, C.

    2003-02-25

    Numerous studies of spent nuclear fuel transportation accident risks have been performed since the late seventies that considered shipping container design and performance. Based in part on these studies, NRC has concluded that the level of protection provided by spent nuclear fuel transportation package designs under accident conditions is adequate. [1] Furthermore, actual spent nuclear fuel transport experience showcase a safety record that is exceptional and unparalleled when compared to other hazardous materials transportation shipments. There has never been a known or suspected release of the radioactive contents from an NRC-certified spent nuclear fuel cask as a result of a transportation accident. In 1999 the United States Nuclear Regulatory Commission (NRC) initiated a study, the Package Performance Study, to demonstrate the performance of spent fuel and spent fuel packages during severe transportation accidents. NRC is not studying or testing its current regulations, a s the rigorous regulatory accident conditions specified in 10 CFR Part 71 are adequate to ensure safe packaging and use. As part of this study, NRC currently plans on using detailed modeling followed by experimental testing to increase public confidence in the safety of spent nuclear fuel shipments. One of the aspects of this confirmatory research study is the commitment to solicit and consider public comment during the scoping phase and experimental design planning phase of this research.

  14. Loss of spent fuel pool cooling PRA: Model and results

    SciTech Connect

    Siu, N.; Khericha, S.; Conroy, S.; Beck, S.; Blackman, H.

    1996-09-01

    This letter report documents models for quantifying the likelihood of loss of spent fuel pool cooling; models for identifying post-boiling scenarios that lead to core damage; qualitative and quantitative results generated for a selected plant that account for plant design and operational practices; a comparison of these results and those generated from earlier studies; and a review of available data on spent fuel pool accidents. The results of this study show that for a representative two-unit boiling water reactor, the annual probability of spent fuel pool boiling is 5 {times} 10{sup {minus}5} and the annual probability of flooding associated with loss of spent fuel pool cooling scenarios is 1 {times} 10{sup {minus}3}. Qualitative arguments are provided to show that the likelihood of core damage due to spent fuel pool boiling accidents is low for most US commercial nuclear power plants. It is also shown that, depending on the design characteristics of a given plant, the likelihood of either: (a) core damage due to spent fuel pool-associated flooding, or (b) spent fuel damage due to pool dryout, may not be negligible.

  15. Spent Nuclear Fuel (SNF) Project Product Specification

    SciTech Connect

    PAJUNEN, A.L.

    2000-12-07

    The process for removal of Spent Nuclear Fuel (SNF) from the K Basins has been divided into major sub-systems. The Fuel Retrieval System (FRS) removes fuel from the existing storage canisters, cleans it, and places it into baskets. The multi-canister overpack (MCO) loading system places the baskets into an MCO that has been pre-loaded in a cask. The cask, containing a loaded MCO, is then transferred to the Cold Vacuum Drying (CVD) Facility. After drying at the CVD Facility, the cask, and MCO, are transferred to the Canister Storage Building (CSB), where the MCO is removed from the cask, staged, inspected, sealed (by welding), and stored until a suitable permanent disposal option is implemented. The purpose of this document is to specify the process related characteristics of an MCO at the interface between major process systems. The characteristics are derived from the primary technical documents that form the basis for safety analysis and design calculations. This document translates the calculation assumptions into implementation requirements and describes the method of verifying that the requirement is achieved. These requirements are used to define validation test requirements and describe requirements that influence multiple sub-project safety analysis reports. This product specification establishes limits and controls for each significant process parameter at interfaces between major sub-systems that potentially affect the overall safety and/or quality of the SNF packaged for processing, transport, and interim dry storage. The product specifications in this document cover the SNF packaged in MCOs to be transported throughout the SNF Project. The description of the product specifications are organized in the document as follows: Section 2.0--Summary listing of product specifications at each major sub-system interface. Section 3.0--Summary description providing guidance as to how specifications are complied with by equipment design or processing within a major

  16. Determining plutonium in spent fuel with nondestructive assay techniques

    SciTech Connect

    Tobin, Stephen J; Charlton, William S; Fensin, Michael L; Menlove, Howard O; Hoover, A S; Quiter, B J; Rajasingam, A; Swinhoe, M T; Thompson, S J; Charlton, W S; Ehinger, M H; Sandoval, N P; Saavedra, S F; Strohmeyer, D

    2009-01-01

    There are a variety of motivations for quantifying plutonium in used (spent) fuel assemblies by means of nondestructive assay including the following: shipper/receiver difference, input accountability at reprocessing facilities and burnup credit at repositories or fuel storage facilities. Twelve NDA techniques were identified that provide information about the composition of an assembly. Unfortunately, none of these techniques is capable of determining the Pu mass in an assembly on its own. However, it is expected that the Pu mass can be quantified by combining a few of the techniques. Determining which techniques to combine and estimating the expected performance of such a system is the purpose of the research effort recently begun. The research presented here is a complimentarily experimental effort. This paper will focus on experimental results of one of the twelve non-destructive assay techniques - passive neutron albedo reactivity. The passive neutron albedo reactivity techniques work by changing the multiplication the pin experiences between two separate measurements. Since a single spent fuel pin has very little multiplication, this is a challenging measurement situation for the technique. Singles and Doubles neutron count rate were measured at Oak Ridge National Laboratory for three different burnup pins to test the capability of the passive neutron albedo reactivity technique.

  17. Application of ALARA principles to shipment of spent nuclear fuel

    SciTech Connect

    Greenborg, J.; Brackenbush, L.W.; Murphy, D.W. Burnett, R.A.; Lewis, J.R.

    1980-05-01

    The public exposure from spent fuel shipment is very low. In view of this low exposure and the perfect safety record for spent fuel shipment, existing systems can be considered satisfactory. On the other hand, occupational exposure reduction merits consideration and technology improvement to decrease dose should concentrate on this exposure. Practices that affect the age of spent fuel in shipment and the number of times the fuel must be shipped prior to disposal have the largest impact. A policy to encourage a 5-year spent fuel cooling period prior to shipment coupled with appropriate cask redesign to accommodate larger loads would be consistent with ALARA and economic principles. And finally, bypassing high population density areas will not in general reduce shipment dose.

  18. Recycling of nuclear spent fuel with AIROX processing

    SciTech Connect

    Majumdar, D.; Jahshan, S.N.; Allison, C.M.; Kuan, P.; Thomas, T.R.

    1992-12-01

    This report examines the concept of recycling light water reactor (LWR) fuel through use of a dry-processing technique known as the AIROX (Atomics International Reduction Oxidation) process. In this concept, the volatiles and the cladding from spent LWR fuel are separated from the fuel by the AIROX process. The fuel is then reenriched and made into new fuel pins with new cladding. The feasibility of the concept is studied from a technical and high level waste minimization perspective.

  19. West Valley facility spent fuel handling, storage, and shipping experience

    SciTech Connect

    Bailey, W.J.

    1990-11-01

    The result of a study on handling and shipping experience with spent fuel are described in this report. The study was performed by Pacific Northwest Laboratory (PNL) and was jointly sponsored by the US Department of Energy (DOE) and the Electric Power Research Institute (EPRI). The purpose of the study was to document the experience with handling and shipping of relatively old light-water reactor (LWR) fuel that has been in pool storage at the West Valley facility, which is at the Western New York Nuclear Service Center at West Valley, New York and operated by DOE. A subject of particular interest in the study was the behavior of corrosion product deposits (i.e., crud) deposits on spent LWR fuel after long-term pool storage; some evidence of crud loosening has been observed with fuel that was stored for extended periods at the West Valley facility and at other sites. Conclusions associated with the experience to date with old spent fuel that has been stored at the West Valley facility are presented. The conclusions are drawn from these subject areas: a general overview of the West Valley experience, handling of spent fuel, storing of spent fuel, rod consolidation, shipping of spent fuel, crud loosening, and visual inspection. A list of recommendations is provided. 61 refs., 4 figs., 5 tabs.

  20. The EBR-II spent fuel treatment program

    SciTech Connect

    Lineberry, M.J.; McFarlane, H.F.

    1995-12-01

    Argonne National Laboratory has refurbished and equipped an existing hot cell facility for demonstrating a high-temperature electrometallurgical process for treating spent nuclear fuel from the Experimental Breeder Reactor-11. Two waste forms will be produced and qualified for geologic disposal of the fission and activation products. Relatively pure uranium will be separated for storage. Following additional development, transuranium elements will be blended into one of the high-level waste streams. The spent fuel treatment program will help assess the viability of electrometallurgical technology as a spent fuel management option.

  1. Neutron Generators for Spent Fuel Assay

    SciTech Connect

    Ludewigt, Bernhard A

    2010-12-30

    The Next Generation Safeguards Initiative (NGSI) of the U.S. DOE has initiated a multi-lab/university collaboration to quantify the plutonium (Pu) mass in, and detect the diversion of pins from, spent nuclear fuel (SNF) assemblies with non-destructive assay (NDA). The 14 NDA techniques being studied include several that require an external neutron source: Delayed Neutrons (DN), Differential Die-Away (DDA), Delayed Gammas (DG), and Lead Slowing-Down Spectroscopy (LSDS). This report provides a survey of currently available neutron sources and their underlying technology that may be suitable for NDA of SNF assemblies. The neutron sources considered here fall into two broad categories. The term 'neutron generator' is commonly used for sealed devices that operate at relatively low acceleration voltages of less than 150 kV. Systems that employ an acceleration structure to produce ion beam energies from hundreds of keV to several MeV, and that are pumped down to vacuum during operation, rather than being sealed units, are usually referred to as 'accelerator-driven neutron sources.' Currently available neutron sources and future options are evaluated within the parameter space of the neutron generator/source requirements as currently understood and summarized in section 2. Applicable neutron source technologies are described in section 3. Commercially available neutron generators and other source options that could be made available in the near future with some further development and customization are discussed in sections 4 and 5, respectively. The pros and cons of the various options and possible ways forward are discussed in section 6. Selection of the best approach must take a number of parameters into account including cost, size, lifetime, and power consumption, as well as neutron flux, neutron energy spectrum, and pulse structure that satisfy the requirements of the NDA instrument to be built.

  2. Robotic Spent Fuel Monitoring – It is time to improve old approaches and old techniques!

    SciTech Connect

    Tobin, Stephen Joseph; Dasari, Venkateswara Rao; Trellue, Holly Renee

    2016-12-13

    This report describes various approaches and techniques associated with robotic spent fuel monitoring. The purpose of this description is to improve the quality of measured signatures, reduce the inspection burden on the IAEA, and to provide frequent verification.

  3. Nondestructive assay of spent boiling water reactor fuel by active neutron interrogation

    SciTech Connect

    Blakeman, E.D.; Ricker, C.W.; Ragan, G.L.; Difilippo, F.C.; Slaughter, G.G.

    1981-01-01

    Spent boiling water reactor (BWR) fuel from Dresden I was assayed for total fissile mass, using the active neutron interrogation method. The nondestructive assay (NDA) system used has four Sb-Be sources for interrogation of the fuels; the induced fission neutrons from the fuel are counted by four lead-shielded methane-filled proportional counters biased above the energy of the source neutrons. Spent fuel rods containing 9 kg of heavy metal were chopped into 5-cm segments and loaded into three 1-liter cans. The three cans were assayed in seven combinations of one, two, or three cans, enabling an evaluation of the precision and accuracy of the NDA system for different amounts of fissile material. The fissile mass in each combination was determined by comparing the induced-fission-neutron counts with the counts obtained from a known standard comprising chopped segments of unirradiated Dresden fuel. These masses were compared to the masses determined by chemical analyses of the spent fuel. The results from the nondestructive assays agreed with results from the chemical analyses to within 2 to 3%. Similar agreement was obtained when two combinations of canned spent fuel were used as standards for the nondesctuctive assays. The assay of BWR spent fuel served as a test of the NDA system which was developed at the Oak Ridge National Laboratory for the assay of spent liquid metal fast breeder reactor (LMFBR) fuel subassemblies at the heat-end of a reprocessing plant. Results of previous experiments and calculations reported earlier using simulated LMFBR fuel subassemblies indicated that the NDA system can measure the fissile masses of spent fuel subassemblies to within an accuracy of 3%. Results of the assays of spent BWR fuel reported herein support this conclusion.

  4. An Extension of the Validation of SCALE (SAS2H) Isotopic Predictions for PWR Spent Fuel

    SciTech Connect

    DeHart, M.D.

    1993-01-01

    Isotopic characterization of spent fuel via depletion and decay calculations is necessary for determination of source terms for subsequent system analyses involving heat transfer, radiation shielding, isotopic migration, etc. Unlike fresh fuel assumptions typically employed in the criticality safety analysis of spent fuel configurations, burnup credit applications also rely on depletion and decay calculations to predict the isotopic composition of spent fuel. These isotopics are used in subsequent criticality calculations to assess the reduced worth of spent fuel. To validate the codes and data used in depletion approaches, experimental measurements are compared with numerical predictions for relevant spent fuel samples. Such comparisons have been performed in earlier work at the Oak Ridge National Laboratory (ORNL). This report describes additional independent measurements and corresponding calculations, which supplement the results of the earlier work. The current work includes measured isotopic data from 19 spent fuel samples obtained from the Italian Trino Vercelles pressurized-water reactor (PWR) and the U.S. Turkey Point Unit 3 PWR. In addition, an approach to determine biases and uncertainties between calculated and measured isotopic concentrations is discussed, together with a method to statistically combine these terms to obtain a conservative estimate of spent fuel isotopic concentrations. Results are presented based on the combination of measured-to-calculated ratios for earlier work and the current analyses. The results described herein represent an extension to a new reactor design not included in the earlier work, and spent fuel samples with enrichment as high as 3.9 wt % {sup 235}U. Results for the current work are found to be, for the most part, consistent with the findings of the earlier work. This consistency was observed for results obtained from each of two different cross-section libraries and suggests that the estimated biases determined for

  5. Development of the ACP safeguards neutron counter for PWR spent fuel rods

    NASA Astrophysics Data System (ADS)

    Lee, Tae-Hoon; Menlove, Howard O.; Lee, Sang-Yoon; Kim, Ho-Dong

    2008-04-01

    An advanced neutron multiplicity counter has been developed for measuring spent fuel in the Advanced spent fuel Conditioning Process (ACP) at the Korea Atomic Energy Research Institute (KAERI). The counter uses passive neutron multiplicity counting to measure the 244Cm content in spent fuel. The input to the ACP process is spent fuel from pressurized water reactors (PWRs), and the high intensity of the gamma-ray exposure from spent fuel requires a careful design of the counter to measure the neutrons without gamma-ray interference. The nuclear safeguards for the ACP facility requires the measurement of the spent fuel input to the process and the Cm/Pu ratio for the plutonium mass accounting. This paper describes the first neutron counter that has been used to measure the neutron multiplicity distribution from spent fuel rods. Using multiple samples of PWR spent fuel rod-cuts, the singles (S), doubles (D), and triples (T) rates of the neutron distribution for the 244Cm nuclide were measured and calibration curves were produced. MCNPX code simulations were also performed to obtain the three counting rates and to compare them with the measurement results. The neutron source term was evaluated by using the ORIGEN-ARP code. The results showed systematic difference of 21-24% in the calibration graphs between the measured and simulation results. A possible source of the difference is that the burnup codes have a 244Cm uncertainty greater than ±15% and it would be systematic for all of the calibration samples. The S/D and D/T ratios are almost constant with an increment of the 244Cm mass, and this indicates that the bias is in the 244Cm neutron source calculation using the ORIGEN-ARP source code. The graphs of S/D and D/T ratios show excellent agreement between measurement and MCNPX simulation results.

  6. Proliferation resistance assessment of various methods of spent nuclear fuel storage and disposal

    NASA Astrophysics Data System (ADS)

    Kollar, Lenka

    the spent fuel pool, 0.42 for dry cask storage, 0.36 for the operating geological repository, and 0.28 for the closed geological repository. Therefore, the spent fuel pool is currently the most proliferation resistant method for storing spent fuel. The extrinsic attributes, mainly involving safeguards measures, affect the total PR value the most. As a result, several recommendations are made to improve the proliferation resistance of spent fuel. These recommendations include employing more advanced safeguards measures, such as verification techniques and remote monitoring, for dry cask storage and the geological repository. Dry cask storage facilities should also be located at the plant and in a secure building to minimize the proliferation risk. Finally, the cost-benefit analysis of increased safeguards needs to be considered. Taking these recommendations into account, the PR values of dry cask storage and the closed geological would be significantly increased, to 0.57 and 0.51, respectively. As a result, with increased safeguards to the safeguards level of the spent fuel pool, dry cask storage would be the most proliferation resistant method to store spent fuel. Therefore, the IAEA should continue to develop remote monitoring and cask storage verification techniques in order to improve the proliferation resistance of spent fuel.

  7. Method for storing spent nuclear fuel in repositories

    DOEpatents

    Schweitzer, D.G.; Sastre, C.; Winsche, W.

    A method for storing radioactive spent fuel in repositories containing sulfur as the storage medium is disclosed. Sulfur is non-corrosive and not subject to radiation damage. Thus, storage periods of up to 100 years are possible.

  8. Method for storing spent nuclear fuel in repositories

    DOEpatents

    Schweitzer, Donald G.; Sastre, Cesar; Winsche, Warren

    1981-01-01

    A method for storing radioactive spent fuel in repositories containing sulfur as the storage medium is disclosed. Sulfur is non-corrosive and not subject to radiation damage. Thus, storage periods of up to 100 years are possible.

  9. Safeguards for spent fuel in an irretrievable storage facility

    SciTech Connect

    Richter, B.; Stein, G. )

    1992-01-01

    Ultimately, high-level waste from the reprocessing of German spent fuel, spent light water reactor (LWR) fuel assemblies that will not be reprocessed, and spent THTR-300 fuel will be disposed of in a geologic repository in the Gorleben salt dome, provided it will be licensed; the exploration of the salt dome is under way. Because of its fissile material content, particularly plutonium, the International Atomic Energy Agency will not release spent fuel from safeguards, although the irradiated material will be packaged in huge containers and irretrievably buried in the salt. International safeguards in an irretrievable storage facility will have to be designed accordingly. This paper discusses various safeguards aspects, investigations, and results. Technical aspects were presented in a previous paper.

  10. Scientists warn of 'trillion-dollar' spent-fuel risk

    NASA Astrophysics Data System (ADS)

    Gwynne, Peter

    2016-07-01

    A study by two Princeton University physicists suggests that a major fire in the spent nuclear fuel stored on the sites of US nuclear reactors could “dwarf the horrific consequences of the Fukushima accident”.

  11. Spent nuclear fuel Canister Storage Building CDR Review Committee report

    SciTech Connect

    Dana, W.P.

    1995-12-01

    The Canister Storage Building (CSB) is a subproject under the Spent Nuclear Fuels Major System Acquisition. This subproject is necessary to design and construct a facility capable of providing dry storage of repackaged spent fuels received from K Basins. The CSB project completed a Conceptual Design Report (CDR) implementing current project requirements. A Design Review Committee was established to review the CDR. This document is the final report summarizing that review

  12. Spent-fuel dry-storage-concept evaluation

    SciTech Connect

    Singh, K.N.; LaRiviere, J.R.

    1981-01-01

    This report gives an assessment of several dry modes for interim storage of commercial light water reactor (LWR) spent fuel and recommends the dry well concept. The Dry Storage Facility (DSF) will receive, encapsulate, and store the canisterized spent fuel in vertical dry wells located near the ground surface. The canisters are designed to be retrievable. The study is based on locating the DSF at Hanford. However, only minor changes would be required if another site with similar climatic conditions were chosen.

  13. In-Field Performance Testing of the Fork Detector for Quantitative Spent Fuel Verification

    SciTech Connect

    Gauld, Ian C.; Hu, Jianwei; De Baere, P.; Vaccaro, S.; Schwalbach, P.; Liljenfeldt, Henrik; Tobin, Stephen

    2015-01-01

    Expanding spent fuel dry storage activities worldwide are increasing demands on safeguards authorities that perform inspections. The European Atomic Energy Community (EURATOM) and the International Atomic Energy Agency (IAEA) require measurements to verify declarations when spent fuel is transferred to difficult-to-access locations, such as dry storage casks and the repositories planned in Finland and Sweden. EURATOM makes routine use of the Fork detector to obtain gross gamma and total neutron measurements during spent fuel inspections. Data analysis is performed by modules in the integrated Review and Analysis Program (iRAP) software, developed jointly by EURATOM and the IAEA. Under the framework of the US Department of Energy–EURATOM cooperation agreement, a module for automated Fork detector data analysis has been developed by Oak Ridge National Laboratory (ORNL) using the ORIGEN code from the SCALE code system and implemented in iRAP. EURATOM and ORNL recently performed measurements on 30 spent fuel assemblies at the Swedish Central Interim Storage Facility for Spent Nuclear Fuel (Clab), operated by the Swedish Nuclear Fuel and Waste Management Company (SKB). The measured assemblies represent a broad range of fuel characteristics. Neutron count rates for 15 measured pressurized water reactor assemblies are predicted with an average relative standard deviation of 4.6%, and gamma signals are predicted on average within 2.6% of the measurement. The 15 measured boiling water reactor assemblies exhibit slightly larger deviations of 5.2% for the gamma signals and 5.7% for the neutron count rates, compared to measurements. These findings suggest that with improved analysis of the measurement data, existing instruments can provide increased verification of operator declarations of the spent fuel and thereby also provide greater ability to confirm integrity of an assembly. These results support the application of the Fork detector as a fully quantitative spent fuel

  14. Development, Testing and Validation of a Waste Assay System for the Measurement and Characterisation of Active Spent Fuel Element Debris From UK Magnox Reactors - 12533

    SciTech Connect

    Mason, John A.; Burke, Kevin J.; Looman, Marc R.; Towner, Antony C.N.; Phillips, Martin E.

    2012-07-01

    This paper describes the development, testing and validation of a waste measurement instrument for characterising active remote handled radioactive waste arising from the operation of Magnox reactors in the United Kingdom. Following operation in UK Magnox gas cooled reactors and a subsequent period of cooling, parts of the magnesium-aluminium alloy cladding were removed from spent fuel and the uranium fuel rods with the remaining cladding were removed to Sellafield for treatment. The resultant Magnox based spent fuel element debris (FED), which constitutes active intermediate level waste (ILW) has been stored in concrete vaults at the reactor sites. As part of the decommissioning of the FED vaults the FED must be removed, measured and characterised and placed in intermediate storage containers. The present system was developed for use at the Trawsfynydd nuclear power station (NPS), which is in the decommissioning phase, but the approach is potentially applicable to FED characterisation at all of the Magnox reactors. The measurement system consists of a heavily shielded and collimated high purity Germanium (HPGe) detector with electromechanical cooling and a high count-rate preamplifier and digital multichannel pulse height analyser. The HPGe based detector system is controlled by a software code, which stores the measurement result and allows a comprehensive analysis of the measured FED data. Fuel element debris is removed from the vault and placed on a tray to a uniform depth of typically 10 cm for measurement. The tray is positioned approximately 1.2 meters above the detector which views the FED through a tungsten collimator with an inverted pyramid shape. At other Magnox sites the positions may be reversed with the shielded and collimated HPGe detector located above the tray on which the FED is measured. A comprehensive Monte Carlo modelling and analysis of the measurement process has been performed in order to optimise the measurement geometry and eliminate

  15. Reactor-specific spent fuel discharge projections: 1986 to 2020

    SciTech Connect

    Heeb, C.M.; Walling, R.C.; Purcell, W.L.

    1987-03-01

    The creation of five reactor-specific spent fuel data bases that contain information on the projected amounts of spent fuel to be discharged from US commercial nuclear reactors through the year 2020 is described. The data bases contain detailed spent-fuel information from existing, planned, and projected pressurized water reactors (PWR) and boiling water reactors (BWR). The projections are based on individual reactor information supplied by the US reactor owners. The basic information is adjusted to conform to Energy Information Agency (EIA) forecasts for nuclear installed capacity, generation, and spent fuel discharged. The EIA cases considered are: (1) No new orders with extended burnup, (2) No new orders with constant burnup, (3) Upper reference (which assumes extended burnup), (4) Upper reference with constant burnup, and (5) Lower reference (which assumes extended burnup). Detailed, by-reactor tables are provided for annual discharged amounts of spent fuel, for storage requirements assuming maximum-at-reactor storage, and for storage requirements assuming maximum-at-reactor plus intra-utility transshipment of spent fuel. 6 refs., 8 figs., 8 tabs.

  16. Reactor-specific spent fuel discharge projections, 1987-2020

    SciTech Connect

    Walling, R.C.; Heeb, C.M.; Purcell, W.L.

    1988-03-01

    The creation of five reactor-specific spent fuel data bases that contain information on the projected amounts of spent fuel to be discharged from U.S. commercial nuclear reactors through the year 2020 is described. The data bases contain detailed spent fuel information from existing, planned, and projected pressurized water reactors (PWR) and boiling water eactors (BWR), and one existing high temperature gas reactor (HTGR). The projections are based on individual reactor information supplied by the U.S. reactor owners. The basic information is adjusted to conform to Energy Information Administration (EIA) forecasts for nuclear installed capacity, generation, and spent fuel discharged. The EIA cases considered are: No New Orders (assumes increasing burnup), No New Orders with No Increased Burnup, Upper Reference (assumes increasing burnup), Upper Reference with No Increased Burnup, and Lower Reference (assumes increasing burnup). Detailed, by-reactor tables are provided for annual discharged amounts of spent fuel, for storage requirements assuming maximum at-reactor storage, and for storage requirements assuming maximum at-reactor storage plus intra-utility transshipment of spent fuel. 8 refs., 8 figs., 10 tabs.

  17. Reactor-specific spent fuel discharge projections: 1985 to 2020

    SciTech Connect

    Heeb, C.M.; Libby, R.A.; Walling, R.C.; Purcell, W.L.

    1986-09-01

    The creation of four spent-fuel data bases that contain information on the projected amounts of spent fuel to be discharged from US commercial nuclear reactors through the year 2020 is described. The data bases contain detailed spent-fuel information from existing, planned, and projected pressurized water reactors (PWR) and boiling water reactors (BWR). The projections are based on individual reactor information supplied by the US reactor owners. The basic information is adjusted to conform to Energy Information Agency (EIA) forecasts for nuclear installed capacity, generation, and spent fuel discharged. The EIA cases considered are: (1) No New Orders with Extended Burnup, (2) No New Orders with Constant Burnup, (3) Middle Case with Extended Burnup, and (4) Middle Case with Constant Burnup. Detailed, by-reactor tables are provided for annual discharged amounts of spent fuel, for storage requirements assuming maximum-at-reactor storage, and for storage requirements assuming maximum-at-reactor plus intra-utility transshipment of spent fuel.

  18. Conditioning of spent nuclear fuel for permanent disposal

    SciTech Connect

    Laidler, J.J.

    1994-10-01

    A compact, efficient method for conditioning spent nuclear fuel is under development This method, known as pyrochemical processing, or {open_quotes}pyroprocessing,{close_quotes} provides a separation of fission products from the actinide elements present in spent fuel and further separates pure uranium from the transuranic elements. The process can facilitate the timely and environmentally-sound treatment of the highly diverse collection of spent fuel currently in the inventory of the United States Department of Energy (DOE). The pyroprocess utilizes elevated-temperature processes to prepare spent fuel for fission product separation; that separation is accomplished by a molten salt electrorefining step that provides efficient (99.9%) separation of transuranics. The resultant waste forms from the pyroprocess are stable under envisioned repository environment conditions and highly leach-resistant. Treatment of any spent fuel type produces a set of common high-level waste forms, one a mineral and the other a metal alloy, that can be readily qualified for repository disposal and preclude the substantial costs that would be associated with the qualification of the numerous spent fuel types included in the DOE inventory.

  19. Conditioning of spent nuclear fuel for permanent disposal

    SciTech Connect

    Laidler, J.J.

    1994-12-31

    A compact, efficient method for conditioning spent nuclear fuel is under development. This method, known as pyrochemical processing, or pyroprocessing, provides a separation of fission products from the actinide elements present in spent fuel and further separates pure uranium from the transuranic elements. The process can facilitate the timely and environmentally-sound treatment of the highly diverse collection of spent fuel currently in the inventory of the US Department of Energy (DOE). The pyroprocess utilizes elevated-temperature processes to prepare spent fuel for fission product separation; that separation is accomplished by a molten salt electrorefining step that provides efficient (> 99.9%) separation of transuranics. The resultant waste forms from the pyroprocess are stable under envisioned repository environment conditions and highly leach-resistant. Treatment of any spent fuel type produces a set of common high-level waste forms, one a mineral and the other a metal alloy, that can be readily qualified for repository disposal and that avoid the substantial costs that would be associated with the qualification of the numerous spent fuel types included in the DOE inventory.

  20. Compton suppressed LaBr3 detection system for use in nondestructive spent fuel assay

    NASA Astrophysics Data System (ADS)

    Bender, S.; Heidrich, B.; Ünlü, K.

    2015-06-01

    Current methods for safeguarding and accounting for spent nuclear fuel in reprocessing facilities are extremely resource and time intensive. The incorporation of autonomous passive gamma-ray detectors into the procedure could make the process significantly less burdensome. In measured gamma-ray spectra from spent nuclear fuel, the Compton continuum from dominant fission product photopeaks obscure the lower energy lines from other isotopes. The application of Compton suppression to gamma-ray measurements of spent fuel may reduce this effect and allow other less intense, lower energy peaks to be detected, potentially improving the accuracy of multivariate analysis algorithms. Compton suppressed spectroscopic measurements of spent nuclear fuel using HPGe, LaBr3, and NaI(Tl) primary detectors were performed. Irradiated fuel was measured in two configurations: as intact fuel elements viewed through a collimator and as feed solutions in a laboratory to simulate the measurement of a dissolved process stream. These two configurations allowed the direct assessment and quantification of the differences in measured gamma-ray spectra from the application of Compton suppression. In the first configuration, several irradiated fuel elements of varying cooling times from the Penn State Breazeale Reactor spent fuel inventory were measured using the three collimated Compton suppression systems. In the second geometry, Compton suppressed measurements of two samples of Approved Test Material commercial fuel elements were recorded inside the guard detector annulus to simulate the siphoning of small quantities from the main process stream for long dwell measurement periods. Compton suppression was found to improve measured gamma-ray spectra of spent fuel for multivariate analysis by notably lowering the Compton continuum from dominant photopeaks such as 137Cs and 140La, due to scattered interactions in the detector, which allowed more spectral features to be resolved. There was a

  1. DECONTAMINATION OF ZIRCALOY CLADDING HULLS FROM SPENT NUCLEAR FUEL

    SciTech Connect

    Rudisill, T.

    2010-09-29

    adsorb neutrons generating higher actinides in the bulk material. During fuel irradiation, {sup 92}Zr is also converted to radioactive {sup 93}Zr by neutron adsorption. Methods for decontaminating and conditioning irradiated Zircaloy cladding hulls have been investigated in Europe, Japan, and the US during the last 35 years; however, a method to decontaminate the hulls to an activity level which meets US acceptance criteria for disposal as a LLW was not deployed on a commercial scale. The feasibility of decontaminating spent fuel cladding hulls was investigated as part of the GNEP Separations Campaign. Small-scale experiments were used to demonstrate the removal of the ZrO{sub 2} layer from Zircaloy coupons using dilute solutions ({le}1.0 M) of HF. The most effective conditions resulted in dissolution rates which were less than approximately 2 mg/cm{sup 2}-min. With dissolution rates in this range, uniform removal of the oxide layer was obtained and a minimal amount of Zircaloy metal was dissolved. To test the HF decontamination process, experiments were subsequently performed using actual spent fuel cladding hulls. Decontamination experiments were performed to measure the fission product and actinide concentrations as a function of the depth of the surface removed from the cladding hull. The experimental methods used to perform these experiments and a discussion of the results and observations are presented in the following sections.

  2. Spent nuclear fuel discharges from US reactors 1993

    SciTech Connect

    Not Available

    1995-02-01

    The Energy Information Administration (EIA) of the U.S. Department of Energy (DOE) administers the Nuclear Fuel Data Survey, Form RW-859. This form is used to collect data on fuel assemblies irradiated at commercial nuclear reactors operating in the United States, and the current inventories and storage capacities of those reactors. These data are important to the design and operation of the equipment and facilities that DOE will use for the future acceptance, transportation, and disposal of spent fuels. The data collected and presented identifies trends in burnup, enrichment, and spent nuclear fuel discharged form commercial light-water reactor as of December 31, 1993. The document covers not only spent nuclear fuel discharges; but also site capacities and inventories; canisters and nonfuel components; and assembly type characteristics.

  3. Historical overview of domestic spent fuel shipments: Update

    SciTech Connect

    Not Available

    1991-07-01

    This report presents available historic data on most commercial and research reactor spent fuel shipments in the United States from 1964 through 1989. Data include sources of the spent fuel shipped, types of shipping casks used, number of fuel assemblies shipped, and number of shipments made. This report also addresses the shipment of spent research reactor fuel. These shipments have not been documented as well as commercial power reactor spent fuel shipment activity. Available data indicate that the greatest number of research reactor fuel shipments occurred in 1986. The largest campaigns in 1986 were from the Brookhaven National Laboratory, Brooklyn, New York, to the Idaho Chemical Processing Plant (ICPP) and from the Oak Ridge National Laboratory's High Flux Isotope Reactor (HFIR) in Tennessee and the Rockwell International Reactor in California to the Savannah River Plant near Aiken, South Carolina. For all years addressed in this report, DOE facilities in Idaho Falls and Savannah River were the major recipients of research reactor spent fuel. In 1989, 10 shipments were received at the Idaho facilities. These originated from universities in California, Michigan, and Missouri. 9 refs., 12 figs., 7 tabs.

  4. Reactive Behavior of K-Basin Spent Nuclear Fuel

    SciTech Connect

    Abrefah, John; Siciliano, Edward R.; Damschen, Dennis W.; Schlahta, Stephan N.

    2002-12-31

    The Hanford Spent Nuclear Fuel Project focuses its efforts on determining how to safely move the degraded N-Reactor spent fuel from water-stored basins to a dry storage facility. As part of this effort, the project initiated experimental studies to address issues relating to the chemical reactivity of the degraded/corroded metallic uranium material. The studies generated a limited set of data on chemical reaction rates of the N-Reactor spent fuel in dry air, moist air, and moist-inert atmospheres for comparison with published data on unirradiated/ irradiated metallic uranium. Based on the laboratory data, the project chose to use a conservative enhancement factor in analyzing the oxidation behavior of the spent metallic fuel. However, there is a need for the project to increase the fuel throughput for the drying treatment process by implementing certain design optimization steps. The study discussed in this paper re-evaluated the previous laboratory data in conjunction with the Cold Vacuum Drying (CVD) process experience and determined whether the built-in level of conservatism could accommodate the potential changes in the process without compromising public and worker safety. Evaluations based on laboratory data on samples taken from the N-Reactor spent fuel showed no reactivity enhancement in moist atmosphere. The established reaction rate constant was used to accurately determine the reactive surface areas of corroded N-Reactor fuel elements. The method was then used to provide a good estimate of the exposed uranium surface area in the loaded MCOs.

  5. Classification of spent reactor fuel for nuclear forensics.

    PubMed

    Jones, Andrew E; Turner, Phillip; Zimmerman, Colin; Goulermas, John Y

    2014-06-03

    In this paper we demonstrate the use of pattern recognition and machine learning techniques to determine the reactor type from which spent reactor fuel has originated. This has been done using the isotopic and elemental measurements of the sample and proves to be very useful in the field of nuclear forensics. Nuclear materials contain many variables (impurities and isotopes) that are very difficult to consider individually. A method that considers all material parameters simultaneously is advantageous. Currently the field of nuclear forensics focuses on the analysis of key material properties to determine details about the materials processing history, for example, utilizing known half-lives of isotopes can determine when the material was last processed (Stanley, F. E. J. Anal. At. Spectrom. 2012, 27, 1821; Varga, Z.; Wallenius, M.; Mayer, K.; Keegan, E.; Millet, S. Anal. Chem. 2009, 81, 8327-8334). However, it has been demonstrated that multivariate statistical analysis of isotopic concentrations can complement these method and are able to make use of a greater level of information through dimensionality reduction techniques (Robel, M.; Kristo, M. J. J. Environ. Radioact. 2008, 99, 1789-1797; Robel, M.; Kristo, M. J.; Heller, M. A. Nuclear Forensic Inferences Using Iterative Multidimensional Statistics. In Proceedings of the Institute of Nuclear Materials Management 50th Annual Meeting, Tucson, AZ, July 2009; 12 pages; Nicolaou, G. J. Environ. Radioact. 2006, 86, 313-318; Pajo, L.; Mayer, K.; Koch, L. Fresenius' J. Anal. Chem. 2001, 371, 348-352). There has been some success in using such multidimensional statistical methods to determine details about the history of spent reactor fuel (Robel, M.; Kristo, M. J. J. Environ. Radioact. 2008, 99, 1789-1797). Here, we aim to expand on these findings by pursuing more robust dimensionality reduction techniques based on manifold embedding which are able to better capture the intrinsic data set information. Furthermore, we

  6. Assessment of Nuclear Resonance Fluorescence for Spent Nuclear Fuel Assay

    SciTech Connect

    Quiter, Brian; Ludewigt, Bernhard; Ambers, Scott

    2011-06-30

    In nuclear resonance fluorescence (NRF) measurements, resonances are excited by an external photon beam leading to the emission of gamma rays with specific energies that are characteristic of the emitting isotope. NRF promises the unique capability of directly quantifying a specific isotope without the need for unfolding the combined responses of several fissile isotopes as is required in other measurement techniques. We have analyzed the potential of NRF as a non-destructive analysis technique for quantitative measurements of Pu isotopes in spent nuclear fuel (SNF). Given the low concentrations of 239Pu in SNF and its small integrated NRF cross sections, the main challenge in achieving precise and accurate measurements lies in accruing sufficient counting statistics in a reasonable measurement time. Using analytical modeling, and simulations with the radiation transport code MCNPX that has been experimentally tested recently, the backscatter and transmission methods were quantitatively studied for differing photon sources and radiation detector types. Resonant photon count rates and measurement times were estimated for a range of photon source and detection parameters, which were used to determine photon source and gamma-ray detector requirements. The results indicate that systems based on a bremsstrahlung source and present detector technology are not practical for high-precision measurements of 239Pu in SNF. Measurements that achieve the desired uncertainties within hour-long measurements will either require stronger resonances, which may be expressed by other Pu isotopes, or require quasi-monoenergetic photon sources with intensities that are approximately two orders of magnitude higher than those currently being designed or proposed.This work is part of a larger effort sponsored by the Next Generation Safeguards Initiative to develop an integrated instrument, comprised of individual NDA techniques with complementary features, that is fully capable of

  7. A metallic fuel cycle concept from spent oxide fuel to metallic fuel

    SciTech Connect

    Fujita, Reiko; Kawashima, Masatoshi; Yamaoka, Mitsuaki; Arie, Kazuo; Koyama, Tadafumi

    2007-07-01

    A Metallic fuel cycle concept for Self-Consistent Nuclear Energy System (SCNES) has been proposed in a companion papers. The ultimate goal of the SCNES is to realize sustainable energy supply without endangering the environment and humans. For future transition period from LWR era to SCNES era, a new metallic fuel recycle concept from LWR spent fuel has been proposed in this paper. Combining the technology for electro-reduction of oxide fuels and zirconium recovery by electrorefining in molten salts in the nuclear recycling schemes, the amount of radioactive waste reduced in a proposed metallic fuel cycle concept. If the recovery ratio of zirconium metal from the spent zirconium waste is 95%, the cost estimation in zirconium recycle to the metallic fuel materials has been estimated to be less than 1/25. (authors)

  8. Overview of the spent nuclear fuel project at Hanford

    SciTech Connect

    Daily, J.L.; Fulton, J.C.; Gerber, E.W.; Culley, G.E.

    1995-02-01

    The Spent Nuclear Fuel Project`s mission at Hanford is to {open_quotes}Provide safe, economic and environmentally sound management of Hanford spent nuclear fuel in a manner which stages it to final disposition.{close_quotes} The inventory of spent nuclear fuel (SNF) at the Hanford Site covers a wide variety of fuel types (production reactor to space reactor) in many facilities (reactor fuel basins to hot cells) at locations all over the Site. The 2,129 metric tons of Hanford SNF represents about 80% of the total US Department of Energy (DOE) inventory. About 98.5% of the Hanford SNF is 2,100 metric tons of metallic uranium production reactor fuel currently stored in the 1950s vintage K Basins in the 100 Area. This fuel has been slowly corroding, generating sludge and contaminating the basin water. This condition, coupled with aging facilities with seismic vulnerabilities, has been identified by several groups, including stakeholders, as being one of the most urgent safety and environmental concerns at the Hanford Site. As a direct result of these concerns, the Spent Nuclear Fuel Project was recently formed to address spent fuel issues at Hanford. The Project has developed the K Basins Path Forward to remove fuel from the basins and place it in dry interim storage. Alternatives that addressed the requirements were developed and analyzed. The result is a two-phased approach allowing the early removal of fuel from the K Basins followed by its stabilization and interim storage consistent with the national program.

  9. Separator assembly for use in spent nuclear fuel shipping cask

    DOEpatents

    Bucholz, James A.

    1983-01-01

    A separator assembly for use in a spent nuclear fuel shipping cask has a honeycomb-type wall structure defining parallel cavities for holding nuclear fuel assemblies. Tubes formed of an effective neutron-absorbing material are embedded in the wall structure around each of the cavities and provide neutron flux traps when filled with water.

  10. Shippingport Spent Fuel Canister (SSFC) Design Report Project W-518

    SciTech Connect

    JOHNSON, D.M.

    2000-01-27

    The SSFC Design Report Describes A spent fuel canister for Shippingport Core 2 blanket fuel assemblies. The design of the SSFC is a minor modification of the MCO. The modification is limited to the Shield Plug which remains unchanged with regard to interfaces with the canister shell. The performance characteristics remain those for the MCO, which bounds the payload of the SSFC.

  11. Foreign experience in extended dry storage of spent nuclear fuel

    SciTech Connect

    Schneider, K.J.; Mitchell, S.J.

    1992-06-01

    Most countries with nuclear power are planning for spent nuclear fuel (or high-level waste from reprocessing of spent fuel) to be disposed of in national deep geological repositories starting in the time period of about 2010 to 2050. While spent fuel has been stored in water basins for the early years after discharge from the reactors, interim dry storage for extended periods (i.e., several tens of years) is being implemented or considered in an increasing number of countries. Dry storage technology is generally considered to be developed on a world-wide basis, and is being initiated and/ or expanded in a number of countries. This paper presents a summary of status and experience in dry storage of spent fuel in other countries, with emphasis on zirconium-clad fuels. Past activities, current status, future plans, research and development, and experience in dry storage are summarized for Argentina, Canada, France, former West Germany, former East Germany, India, Italy, Japan, South Korea, Spain, Switzerland, United Kingdom, and the former Soviet Union. Conclusions from their experience are presented. Their experience to date supports the expectations that proper dry storage should provide for safe extended dry storage of spent fuel.

  12. Natural convection heat transfer within horizontal spent nuclear fuel assemblies

    SciTech Connect

    Canaan, R.E.

    1995-12-01

    Natural convection heat transfer is experimentally investigated in an enclosed horizontal rod bundle, which characterizes a spent nuclear fuel assembly during dry storage and/or transport conditions. The basic test section consists of a square array of sixty-four stainless steel tubular heaters enclosed within a water-cooled rectangular copper heat exchanger. The heaters are supplied with a uniform power generation per unit length while the surrounding enclosure is maintained at a uniform temperature. The test section resides within a vacuum/pressure chamber in order to subject the assembly to a range of pressure statepoints and various backfill gases. The objective of this experimental study is to obtain convection correlations which can be used in order to easily incorporate convective effects into analytical models of horizontal spent fuel systems, and also to investigate the physical nature of natural convection in enclosed horizontal rod bundles in general. The resulting data consist of: (1) measured temperatures within the assembly as a function of power, pressure, and backfill gas; (2) the relative radiative contribution for the range of observed temperatures; (3) correlations of convective Nusselt number and Rayleigh number for the rod bundle as a whole; and (4) correlations of convective Nusselt number as a function of Rayleigh number for individual rods within the array.

  13. Spent Fuel Ratio Estimates from Numerical Models in ALE3D

    SciTech Connect

    Margraf, J. D.; Dunn, T. A.

    2016-08-02

    Potential threat of intentional sabotage of spent nuclear fuel storage facilities is of significant importance to national security. Paramount is the study of focused energy attacks on these materials and the potential release of aerosolized hazardous particulates into the environment. Depleted uranium oxide (DUO2) is often chosen as a surrogate material for testing due to the unreasonable cost and safety demands for conducting full-scale tests with real spent nuclear fuel. To account for differences in mechanical response resulting in changes to particle distribution it is necessary to scale the DUO2 results to get a proper measure for spent fuel. This is accomplished with the spent fuel ratio (SFR), the ratio of respirable aerosol mass released due to identical damage conditions between a spent fuel and a surrogate material like depleted uranium oxide (DUO2). A very limited number of full-scale experiments have been carried out to capture this data, and the oft-questioned validity of the results typically leads to overly-conservative risk estimates. In the present work, the ALE3D hydrocode is used to simulate DUO2 and spent nuclear fuel pellets impacted by metal jets. The results demonstrate an alternative approach to estimate the respirable release fraction of fragmented nuclear fuel.

  14. Characterization of spent fuel approved testing material: ATM-103

    SciTech Connect

    Guenther, R.J.; Blahnik, D.E.; Campbell, T.K.; Jenquin, U.P.; Mendel, J.E.; Thomas, L.E.; Thornhill, C.K.

    1988-04-01

    The characterization data obtained to date are described for Approved Testing Material (ATM)-103, which is spent fuel from Assembly D101 of pressurized-water reactor Calvert Cliffs, No. 1. This report is one in a series being written by the Materials Characterization Center (MCC) at Pacific Northwest Laboratory (PNL) on spent fuel ATMs. The ATMs are receiving extensive examinations to provide a source of well-characterized spent fuel for testing in the US nuclear waste repository program. ATM-103 consists of 176 full-length irradiated fuel rods with rod-average burnups of about 2600 GJ/kgM (30 MWd/kgM) and less than 1% fission gas release. Characterization data include 1) as-fabricated fuel design, irradiation history, and subsequent storage and handling; 2) isotopic gamma scans; 3) fission gas analyses; 4) ceramography of the fuel and metallography of the cladding; 5) special fuels studies involving analytical transmission electron microscopy (AEM); 6) calculated nuclide inventories and radioactivities in the fuel and cladding; and 7) radiochemical analyses of the fuel and cladding. Additional analyses of the fuel are being conducted and will be included in planned revisions of this report. 10 refs., 103 figs., 63 tabs.

  15. Characterization of spent fuel approved testing material---ATM-105

    SciTech Connect

    Guenther, R.J.; Blahnik, D.E.; Campbell, T.K.; Jenquin, U.P.; Mendel, J.E.; Thomas, L.E.; Thornhill, C.K.

    1991-12-01

    The characterization data obtained to data are described for Approved Testing Material 105 (ATM-105), which is spent fuel from Bundles CZ346 and CZ348 of the Cooper Nuclear Power Plant, a boiling-water reactor. This report is one in a series being prepared by the Materials Characterization Center at Pacific Northwest Laboratory (PNL) on spent fuel ATMs. The ATMs are receiving extensive examinations to provide a source of well-characterized spent fuel for testing in the US Department of Energy Office of Civilian Radioactive Waste Management (OCRWM) Program. ATM-105 consists of 88 full-length irradiated fuel rods with rod-average burnups of about 2400 GJ/kgM (28 MWd/kgM) and expected fission gas release of about 1%. Characterization data include (1) descriptions of as-fabricated fuel design, irradiation history, and subsequent storage and handling; (2) isotopic gamma scans; (3) fission gas analyses; (4) ceramography of the fuel and metallography of the cladding; (5) special fuel studies involving analytical transmission electron microscopy (AEM); (6) calculated nuclide inventories and radioactivities in the fuel and cladding; and (7) radiochemical analyses of the fuel and cladding. Additional analyses of the fuel are being conducted and will be included in planned revisions of this report.

  16. Analysis of subcritical experiments using fresh and spent research reactor fuel assemblies

    NASA Astrophysics Data System (ADS)

    Zino, John Frederick

    1999-11-01

    This research investigated the concepts associated with crediting the burnup of spent nuclear fuel assemblies for the purposes of criticality safety. To accomplish this, a collaborative experimental research program was undertaken between Westinghouse, the University of Missouri Research Reactor (MURR) facility and Oak Ridge National Laboratory (ORNL). The purpose of the program was to characterize the subcritical behavior of a small array of fresh and spent MURR fuel assemblies using the 252Cf Source-driven noise technique. An aluminum test rig was built which was capable of holding up to four, highly enriched (93.15 wt.% 235U) MURR fuel assemblies in a 2 x 2 array. The rig was outfitted with one source and four detector drywells which allowed researchers to perform active neutron noise measurements on the array of fuel assemblies. The 1 atmosphere gas 3He neutron detectors used to perform the measurements were quenched with CF4 gas to allow improved discrimination of the neutron signals in the very high gamma-ray fields associated with spent fuel (˜8000 R/hr). In addition, the detector drywells were outfitted with 1″ lead collars to provide additional gamma-ray shielding from the spent fuel. Reactivity changes were induced in the subcritical lattice by replacing individual fresh assemblies (in a 4-assembly array) with spent assemblies of known, maximum burnup (143 Mw-D). The absolute and relative measured reactivity changes were then compared to those predicted by three-dimensional Monte Carlo calculations. The purpose of these comparisons was to investigate the accuracy of modern transport theory depletion calculations to accurately simulate the reactivity effects of burnup in spent nuclear fuel. A total of seven subcritical measurements were performed at the MURR reactor facility on July 20th and 27th, 1998. These measurements generated several estimates of prompt neutron decay constants (alpha) and ratios of spectral densities through frequency correlations

  17. Development of Techniques for Spent Fuel Assay – Differential Dieaway Final Report

    SciTech Connect

    Swinhoe, Martyn Thomas; Goodsell, Alison; Ianakiev, Kiril Dimitrov; Iliev, Metodi; Desimone, David J.; Rael, Carlos D.; Henzl, Vladimir; Polk, Paul John

    2016-07-28

    This report summarizes the work done under a DNDO R&D funded project on the development of the differential dieaway method to measure plutonium in spent fuel. There are large amounts of plutonium that are contained in spent fuel assemblies, and currently there is no way to make quantitative non-destructive assay. This has led NA24 under the Next Generation Safeguards Initiative (NGSI) to establish a multi-year program to investigate, develop and implement measurement techniques for spent fuel. The techniques which are being experimentally tested by the existing NGSI project do not include any pulsed neutron active techniques. The present work covers the active neutron differential dieaway technique and has advanced the state of knowledge of this technique as well as produced a design for a practical active neutron interrogation instrument for spent fuel. Monte Carlo results from the NGSI effort show that much higher accuracy (1-2%) for the Pu content in spent fuel assemblies can be obtained with active neutron interrogation techniques than passive techniques, and this would allow their use for nuclear material accountancy independently of any information from the operator. The main purpose of this work was to develop an active neutron interrogation technique for spent nuclear fuel.

  18. Subcritical transmutation of spent nuclear fuel

    NASA Astrophysics Data System (ADS)

    Sommer, Christopher M.

    2011-07-01

    A series of fuel cycle simulations were performed using CEA's reactor physics code ERANOS 2.0 to analyze the transmutation performance of the Subcritical Advanced Burner Reactor (SABR). SABR is a fusion-fission hybrid reactor that combines the leading sodium cooled fast reactor technology with the leading tokamak plasma technology based on ITER physics. Two general fuel cycles were considered for the SABR system. The first fuel cycle is one in which all of the transuranics from light water reactors are burned in SABR. The second fuel cycle is a minor actinide burning fuel cycle in which all of the minor actinides and some of the plutonium produced in light water reactors are burned in SABR, with the excess plutonium being set aside for starting up fast reactors in the future. The minor actinide burning fuel cycle is being considered in European Scenario Studies. The fuel cycles were evaluated on the basis of TRU/MA transmutation rate, power profile, accumulated radiation damage, and decay heat to the repository. Each of the fuel cycles are compared against each other, and the minor actinide burning fuel cycles are compared against the EFIT transmutation system, and a low conversion ratio fast reactor.

  19. Hanford`s spent nuclear fuel retrieval: an agressive agenda

    SciTech Connect

    Shen, E.J., Westinghouse Hanford

    1996-12-06

    Starting December 1997, spent nuclear fuel that has been stored in the K Reactor Fuel Storage Basins will be retrieved over a two year period and repackaged for long term dry storage. The aging and sometimes corroding fuel elements will be recovered and processed using log handled tools and teleoperated manipulator technology. The U.S. Department of Energy (DOE) is committed to this urgent schedule because of the environmental threats to the groundwater and nearby the Columbia River.

  20. Hot startup experience with electrometallurgical treatment of spent nuclear fuel

    SciTech Connect

    Benedict, R.W.; Lineberry, M.J.; McFarlane, H.F.; Rigg, R.H.

    1997-10-01

    The treatment of spent metal fuel from the EBR-II fast reactor commenced in June of 1996 at the Fuel Conditioning Facility on the Argonne-West site in Idaho, USA. During the first year of hot operations, 20 fuel assemblies entered processing and 6 low enrichment uranium product ingots were produced. Results are presented for the various process steps with decontamination factors achieved and equipment operational history reported.

  1. Methodology for determining criteria for storing spent fuel in air

    SciTech Connect

    Reid, C.R.; Gilbert, E.R.

    1986-11-01

    Dry storage in an air atmosphere is a method being considered for spent light water reactor (LWR) fuel as an alternative to storage in an inert gas environment. However, methods to predict fuel integrity based on oxidation behavior of the fuel first must be evaluated. The linear cumulative damage method has been proposed as a technique for defining storage criteria. Analysis of limited nonconstant temperature data on nonirradiated fuel samples indicates that this approach yields conservative results for a strictly decreasing-temperature history. On the other hand, the description of damage accumulation in terms of remaining life concepts provides a more general framework for making predictions of failure. Accordingly, a methodology for adapting remaining life concepts to UO/sub 2/ oxidation has been developed at Pacific Northwest Laboratory. Both the linear cumulative damage and the remaining life methods were used to predict oxidation results for spent fuel in which the temperature was decreased with time to simulate the temperature history in a dry storage cask. The numerical input to the methods was based on oxidation data generated with nonirradiated UO/sub 2/ pellets. The calculated maximum allowable storage temperatures are strongly dependent on the temperature-time profile and emphasize the conservatism inherent in the linear cumulative damage model. Additional nonconstant temperature data for spent fuel are needed to both validate the proposed methods and to predict temperatures applicable to actual spent fuel storage.

  2. Status of spent-fuel shipping cask development

    SciTech Connect

    Hall, I.K.; Hinschberger, T.S.

    1989-01-01

    The purpose of the Cask Systems Development Program is to develop a variety of cask systems that can safely and economically transport commercial spent fuel and high-level waste from the generating sites to a federal geologic repository or monitored retrievable storage (MRS) facility. This paper is limited to a discussion of the status of from-reactor spent-fuel cask development; future cask development plans include MRS-to-repository casks, specialty casks for nonstandard spent fuel and nonfuel materials, and defense high-level waste casks. Spent-fuel casks must be available in the late 1990s to support the U.S. Department of Energy (DOE) Office of Civilian Radioactive Waste Management (OCRWM) shipments from utilities. DOE-Idaho, with the support of EG G Idaho, Inc., Sandia National Laboratories, and selected cask developing contractors, has been assigned the responsibility for developing a new generation of cask systems. Four categories of spent fuel casks were initially proposed: (1) legal weight truck (LWT) casks (2) overweight truck (OWT) casks (3) rail/barge (R/B) casks (4) dual purpose (DP) storage/transport casks. Casks are being designed for reduced occupational radiation exposure at the receiving facility by facilitating the use of remote handling equipment. Automation of remote handling systems may be used to reduce cask turnaround time. Reducing turnaround time promotes reduced radiation exposure to occupational workers and improves cask utilization efficiency.

  3. Integrated approach to trailer design for spent fuel casks

    SciTech Connect

    Osborne, D.M.; Burgoyne, R.M.; Grenier, R.M.; Meyer, R.J.

    1989-02-01

    General Atomics (GA) is developing the GA-4 and GA-9 spent fuel transportation systems. The scope of our contract includes spent fuel casks, legal weight trailers, and ancillary equipment. Recent structural failures of spent fuel trailers have focused attention on trailer design. As a major element of spent fuel transportation systems, the concerns address the adequacy of trailer performance requirements, structural design and analysis, and in-service inspection and maintenance procedures. In response to these concerns, GA has applied an integrated approach to the design of the GA-4 and GA-9 transportation systems. The objectives are to design reliable, high-integrity trailers and to demonstrate their performance by test. Once the design is complete, a prototype trailer will be fabricated and a performance test program conducted in accordance with a comprehensive test program. GA`s trailer test program will include both design and operations elements, and will be used to optimize the operations and maintenance plan. The results of this program will provide positive public and regulatory perception of trailer durability and will support the development of industry standards for both legal weight and overweight trailers for spent fuel applications. 2 figs.

  4. Integrated approach to trailer design for spent fuel casks

    SciTech Connect

    Osborne, D.M.; Burgoyne, R.M.; Grenier, R.M.; Meyer, R.J.

    1989-02-01

    General Atomics (GA) is developing the GA-4 and GA-9 spent fuel transportation systems. The scope of our contract includes spent fuel casks, legal weight trailers, and ancillary equipment. Recent structural failures of spent fuel trailers have focused attention on trailer design. As a major element of spent fuel transportation systems, the concerns address the adequacy of trailer performance requirements, structural design and analysis, and in-service inspection and maintenance procedures. In response to these concerns, GA has applied an integrated approach to the design of the GA-4 and GA-9 transportation systems. The objectives are to design reliable, high-integrity trailers and to demonstrate their performance by test. Once the design is complete, a prototype trailer will be fabricated and a performance test program conducted in accordance with a comprehensive test program. GA's trailer test program will include both design and operations elements, and will be used to optimize the operations and maintenance plan. The results of this program will provide positive public and regulatory perception of trailer durability and will support the development of industry standards for both legal weight and overweight trailers for spent fuel applications. 2 figs.

  5. Remote monitoring design concepts for spent fuel storage facilities

    SciTech Connect

    Hale, W.R.; Johnson, C.S.

    1996-08-01

    For the past two years Sandia National Laboratories (SNL) has been involved in developing and installing Remote Monitoring Systems (RMS) at a number of sites around the world. Through the cooperation of the various countries and facilities, it has been possible to collect data on the requirements and performance of these systems that are for monitoring the movement of spent nuclear fuel. The data collected shows that the front end detection method can be a very useful concept to reduce the amount of data that has to be collected and, more importantly, reviewed by inspectors. Spent fuel storage monitoring is a major part of the non-proliferation monitoring that must be done since spent fuel is the by-product of all the power and research reactors worldwide. The movement of spent fuel is easier in many respects to monitor since it always requires protective shielding. This paper will describe a number of the Remote Monitoring Systems that have been installed to monitor spent fuel movement and the resulting decrease in data from the use of a sensor-driven front detection system. The reduction of the data collected and stored is also important to remote monitoring since it decreases the time required to transmit the data to a review site.

  6. CASMO-2 spent-fuel-rack criticality analysis

    SciTech Connect

    Napolitano, D.G.; Heinrichs, D.P.; Gorski, J.P.

    1986-01-01

    In recent years, utilities have needed to increase their spent-fuel storage capacity. Both Maine Yankee pressurized water reactor (PWR) and Vermont Yankee boiling water reactor (BWR) have increased their spent-fuel rack capacity by decreasing the canister center-to-center spacing while adding fixed poison. Licensing criticality analysis of such changes in spent-fuel rack design have been performed at Yankee Atomic Electric Co. (YAEC) using NITAWL-KENO-IV and the 123-group XSDRN library. However, KENO/Monte Carlo analysis has inherent drawbacks when applied to spent-fuel rack design and modification. These include statistical uncertainty and long computer time. In contrast, the transport theory code, CASMO-2, provides deterministic and fast criticality analysis. Also, since collapsed and transport-corrected cross sections are generated, PDQ can be used to analyze large array problems which are prohibitively expensive using KENO. In this work, the authors apply the CASMO-PDQ methodology to the Maine Yankee and Vermont Yankee high-density spent-fuel rack designs, and compare the final results against KENO.

  7. Separation of actinides from spent nuclear fuel: A review.

    PubMed

    Veliscek-Carolan, Jessica

    2016-11-15

    This review summarises the methods currently available to extract radioactive actinide elements from solutions of spent nuclear fuel. This separation of actinides reduces the hazards associated with spent nuclear fuel, such as its radiotoxicity, volume and the amount of time required for its' radioactivity to return to naturally occurring levels. Separation of actinides from environmental water systems is also briefly discussed. The actinide elements typically found in spent nuclear fuel include uranium, plutonium and the minor actinides (americium, neptunium and curium). Separation methods for uranium and plutonium are reasonably well established. On the other hand separation of the minor actinides from lanthanide fission products also present in spent nuclear fuel is an ongoing challenge and an area of active research. Several separation methods for selective removal of these actinides from spent nuclear fuel will be described. These separation methods include solvent extraction, which is the most commonly used method for radiochemical separations, as well as the less developed but promising use of adsorption and ion-exchange materials. Crown Copyright © 2016. Published by Elsevier B.V. All rights reserved.

  8. Microbial Biofilm Growth on Irradiated, Spent Nuclear Fuel Cladding

    SciTech Connect

    S.M. Frank

    2009-02-01

    A fundamental criticism regarding the potential for microbial influenced corrosion in spent nuclear fuel cladding or storage containers concerns whether the required microorganisms can, in fact, survive radiation fields inherent in these materials. This study was performed to unequivocally answer this critique by addressing the potential for biofilm formation, the precursor to microbial-influenced corrosion, in radiation fields representative of spent nuclear fuel storage environments. This study involved the formation of a microbial biofilm on irradiated spent nuclear fuel cladding within a hot cell environment. This was accomplished by introducing 22 species of bacteria, in nutrient-rich media, to test vessels containing irradiated cladding sections and that was then surrounded by radioactive source material. The overall dose rate exceeded 2 Gy/h gamma/beta radiation with the total dose received by some of the bacteria reaching 5 × 103 Gy. This study provides evidence for the formation of biofilms on spent-fuel materials, and the implication of microbial influenced corrosion in the storage and permanent deposition of spent nuclear fuel in repository environments.

  9. Characterization of spent fuel approved testing material: ATM-106

    SciTech Connect

    Guenther, R.J.; Blahnik, D.E.; Campbell, T.K.; Jenquin, U.P.; Mendel, J.E.; Thornhill, C.K.

    1988-10-01

    The characterization data obtained to date are described for Approved Testing Material (ATM)-106 spent fuel from Assembly BT03 of pressurized-water reactor Calvert Cliffs No. 1. This report is one in a series being prepared by the Materials Characterization Center at Pacific Northwest Laboratory on spent fuel ATMs. The ATMs are receiving extensive examinations to provide a source of well- characterized spent fuel for testing in the US Department of Energy Office of Civilian Radioactive Waste Management (OCWRM) program. ATM-106 consists of 20 full-length irradiated fuel rods with rod-average burnups of about 3700 GJ/kgM (43 MWd/kgM) and expected fission gas release of /approximately/10%. Characterization data include (1) as-fabricated fuel design, irradiation history, and subsequent storage and handling; (2) isotopic gamma scans; (3) fission gas analyses; (4) ceramography of the fuel and metallography of the cladding; (5) calculated nuclide inventories and radioactivities in the fuel and cladding; and (6) radiochemical analyses of the fuel and cladding. Additional analyses of the fuel rod are being conducted and will be included in planned revisions of this report. 12 refs., 110 figs., 81 tabs.

  10. Characterization of spent fuel approved testing material--ATM-104

    SciTech Connect

    Guenther, R.J.; Blahnik, D.E.; Jenquin, U.P.; Mendel, J.E.; Thomas, L.E.; Thornhill, C.K.

    1991-12-01

    The characterization data obtained to date are described for Approved Testing Material 104 (ATM-104), which is spent fuel from Assembly DO47 of the Calvert Cliffs Nuclear Power Plant (Unit 1), a pressurized-water reactor. This report is one in a series being prepared by the Materials Characterization Center at Pacific Northwest Laboratory (PNL) on spent fuel ATMs. The ATMs are receiving extensive examinations to provide a source of well-characterized spent fuel for testing in the US Department of Energy Office of Civilian Radioactive Waste Management (OCRWM) Program. ATM-104 consists of 128 full-length irradiated fuel rods with rod-average burnups of about 42 MWd/kgM and expected fission gas release of about 1%. A variety of analyses were performed to investigate cladding characteristics, radionuclide inventory, and redistribution of fission products. Characterization data include (1) fabricated fuel design, irradiation history, and subsequent storage and handling history; (2) isotopic gamma scans; (3) fission gas analyses; (4) ceramography of the fuel and metallography of the cladding; (5) special fuel studies involving analytical transmission electron microscopy (AEM) and electron probe microanalyses (EPMA); (6) calculated nuclide inventories and radioactivities in the fuel and cladding; and (7) radiochemical analyses of the fuel and cladding.

  11. Accelerated Closure of the Spent Nuclear Fuel (SNF) project

    SciTech Connect

    RUTHERFORD, W.W.

    2001-02-01

    The K East and K West Basins, built in the early 1950s, have been used to store irradiated nuclear fuel from the Hanford N Reactor. This fuel, which is referred to as spent nuclear fuel (SNF), has been stored underwater since 1975 in KE Basin and since 1981 in KW Basin. There are 54,000 N Reactor fuel assemblies in 3,800 canisters in the K West Basin, and 51,000 fuel assemblies in 3,700 canisters in the K East Basin that total 2,100 metric tons of SNF.

  12. The burnup dependence of light water reactor spent fuel oxidation

    SciTech Connect

    Hanson, B.D.

    1998-07-01

    Over the temperature range of interest for dry storage or for placement of spent fuel in a permanent repository under the conditions now being considered, UO{sub 2} is thermodynamically unstable with respect to oxidation to higher oxides. The multiple valence states of uranium allow for the accommodation of interstitial oxygen atoms in the fuel matrix. A variety of stoichiometric and nonstoichiometric phases is therefore possible as the fuel oxidizers from UO{sub 2} to higher oxides. The oxidation of UO{sub 2} has been studied extensively for over 40 years. It has been shown that spent fuel and unirradiated UO{sub 2} oxidize via different mechanisms and at different rates. The oxidation of LWR spent fuel from UO{sub 2} to UO{sub 2.4} was studied previously and is reasonably well understood. The study presented here was initiated to determine the mechanism and rate of oxidation from UO{sub 2.4} to higher oxides. During the early stages of this work, a large variability in the oxidation behavior of samples oxidized under nearly identical conditions was found. Based on previous work on the effect of dopants on UO{sub 2} oxidation and this initial variability, it was hypothesized that the substitution of fission product and actinide impurities for uranium atoms in the spent fuel matrix was the cause of the variable oxidation behavior. Since the impurity concentration is roughly proportional to the burnup of a specimen, the oxidation behavior of spent fuel was expected to be a function of both temperature and burnup. This report (1) summarizes the previous oxidation work for both unirradiated UO{sub 2} and spent fuel (Section 2.2) and presents the theoretical basis for the burnup (i.e., impurity concentration) dependence of the rate of oxidation (Sections 2.3, 2.4, and 2.5), (2) describes the experimental approach (Section 3) and results (Section 4) for the current oxidation tests on spent fuel, and (3) establishes a simple model to determine the activation energies

  13. Validation of SCALE (SAS2H) isotopic predictions for BWR spent fuel

    SciTech Connect

    Hermann, O.W.; DeHart, M.D.

    1998-09-01

    Thirty spent fuel samples obtained from boiling-water-reactor (BWR) fuel pins have been modeled at Oak Ridge National Laboratory using the SAS2H sequence of the SCALE code system. The SAS2H sequence uses transport methods combined with the depletion and decay capabilities of the ORIGEN-S code to estimate the isotopic composition of fuel as a function of its burnup history. Results of these calculations are compared with chemical assay measurements of spent fuel inventories for each sample. Results show reasonable agreement between measured and predicted isotopic concentrations for important actinides; however, little data are available for most fission products considered to be important for spent fuel concerns (e.g., burnup credit, shielding, source-term calculations, etc.). This work is a follow-up to earlier works that studied the ability to predict spent fuel compositions in pressurized-water-reactor (PWR) fuel pins. Biases and uncertainties associated with BWR isotopic predictions are found to be larger than those of PWR calculations. Such behavior is expected, as the operation of a BWR is significantly more complex than that of a PWR plant, and in general the design of a BWR has a more heterogeneous configuration than that of a PWR. Nevertheless, this work shows that the simple models employed using SAS2H to represent such complexities result in agreement to within 5% (and often less than 1%) or less for most nuclides important for spent fuel applications. On the other hand, however, the set of fuel samples analyzed represent a small subset of the BWR fuel population, and results reported herein may not be representative of the full population of BWR spent fuel.

  14. Validation of SCALE (SAS2H) Isotopic Predictions for BWR Spent Fuel

    SciTech Connect

    Hermann, O.W.

    1998-01-01

    Thirty spent fuel samples obtained from boiling-water-reactor (BWR) fuel pins have been modeled at Oak Ridge National Laboratory using the SAS2H sequence of the SCALE code system. The SAS2H sequence uses transport methods combined with the depletion and decay capabilities of the ORIGEN-S code to estimate the isotopic composition of fuel as a function of its burnup history. Results of these calculations are compared with chemical assay measurements of spent fuel inventories for each sample. Results show reasonable agreement between measured and predicted isotopic concentrations for important actinides; however, little data are available for most fission products considered to be important for spent fuel concerns (e.g., burnup credit, shielding, source-term calculations, etc.). This work is a follow-up to earlier works that studied the ability to predict spent fuel compositions in pressurized-water-reactor (PWR) fuel pins. Biases and uncertainties associated with BWR isotopic predictions are found to be larger than those of PWR calculations. Such behavior is expected, as the operation of a BWR is significantly more complex than that of a PWR plant, and in general the design of a BWR has a more heterogeneous configuration than that of a PWR. Nevertheless, this work shows that the simple models employed using SAS2H to represent such complexities result in agreement to within 5% (and often less than 1%) or less for most nuclides important for spent fuel applications. On the other hand, however, the set of fuel samples analyzed represent a small subset of the BWR fuel population, and results reported herein may not be representative of the full population of BWR spent fuel.

  15. Spent-Fuel Test - Climax: An evaluation of the technical feasibility of geologic storage of spent nuclear fuel in granite: Executive summary of final results

    SciTech Connect

    Patrick, W.C.

    1986-09-02

    This summary volume outlines results that are covered in more detail in the final report of the Spent-Fuel Test - Climate project. The project was conducted between 1978 and 1983 in the granitic Climax stock at the Nevada Test Site. Results indicate that spent fuel can be safely stored for periods of years in this host medium and that nuclear waste so emplaced can be safely retrieved. We also evaluated the effects of heat and radiation (alone and in combination) on emplacement canisters and the surrounding rock mass. Storage of the spent-fuel affected the surrounding rock mass in measurable ways, but did not threaten the stability or safety of the facility at any time.

  16. Determining reactor flux from xenon-136 and cesium-135 in spent fuel

    NASA Astrophysics Data System (ADS)

    Hayes, A. C.; Jungman, Gerard

    2012-10-01

    The ability to infer reactor flux from spent fuel or seized fissile material would enhance the tools of nuclear forensics and nuclear nonproliferation significantly. We show that reactor flux can be inferred from the ratios of xenon-136 to xenon-134 and cesium-135 to cesium-137. If the average flux of a reactor is known, the flux inferred from measurements of spent fuel could help determine whether that spent fuel was loaded as a blanket or close to the mid-plane of the reactor. The cesium ratio also provides information on reactor shutdowns during the irradiation of fuel, which could prove valuable for identifying the reactor in question through comparisons with satellite reactor heat monitoring data. We derive analytic expressions for these correlations and compare them to experimental data and to detailed reactor burn simulations. The enrichment of the original uranium fuel affects the correlations by up to 3%, but only at high flux.

  17. Cosmic ray muon computed tomography of spent nuclear fuel in dry storage casks

    SciTech Connect

    Poulson, Daniel Cris; Durham, J. Matthew; Guardincerri, Elena; Morris, Christopher; Bacon, Jeffrey Darnell; Plaud-Ramos, Kenie Omar; Morley, Deborah Jean; Hecht, Adam A.

    2016-10-22

    Radiography with cosmic ray muon scattering has proven to be a successful method of imaging nuclear material through heavy shielding. Of particular interest is monitoring dry storage casks for diversion of plutonium contained in spent reactor fuel. Using muon tracking detectors that surround a cylindrical cask, cosmic ray muon scattering can be simultaneously measured from all azimuthal angles, giving complete tomographic coverage of the cask interior. This article describes the first application of filtered back projection algorithms, typically used in medical imaging, to cosmic ray muon scattering imaging. The specific application to monitoring spent nuclear fuel in dry storage casks is investigated via GEANT4 simulations. With a cylindrical muon tracking detector surrounding a typical spent fuel cask, simulations indicate that missing fuel bundles can be detected with a statistical significance of ~18σ in less than two days exposure and a sensitivity at 1σ to a 5% missing portion of a fuel bundle. Finally, we discuss potential detector technologies and geometries.

  18. Dissolution of Spent Nuclear Fuel in Carbonate-Peroxide Solution

    SciTech Connect

    Soderquist, Chuck Z.; Hanson, Brady D.

    2010-01-31

    This study shows that spent UO2 fuel can be completely dissolved in a carbonate-peroxide solution apparently without attacking the metallic Mo-Tc-Ru-Rh-Pd fission product phase. Samples of spent nuclear fuel were pulverized and sieved to a uniform size, then duplicate aliquots were weighed into beakers for analysis. One set was dissolved in near-boiling 10M nitric acid, and the other set was dissolved in a solution of ammonium carbonate and hydrogen peroxide at room temperature. All the resulting fuel solutions were then analyzed for Sr-90, Tc-99, Cs-137, plutonium, and Am-241. For all the samples, the concentrations of Cs-137, Sr-90, plutonium, and Am-241 were the same for both the nitric acid dissolution and the ammonium carbonate-hydrogen peroxide dissolution, but the technetium concentration of the ammonium carbonate-hydrogen peroxide fuel solution was only about 25% of the same fuels dissolved in hot nitric acid.

  19. Mission Need Statement: Idaho Spent Fuel Facility Project

    SciTech Connect

    Barbara Beller

    2007-09-01

    Approval is requested based on the information in this Mission Need Statement for The Department of Energy, Idaho Operations Office (DOE-ID) to develop a project in support of the mission established by the Office of Environmental Management to "complete the safe cleanup of the environmental legacy brought about from five decades of nuclear weapons development and government-sponsored nuclear energy research". DOE-ID requests approval to develop the Idaho Spent Fuel Facility Project that is required to implement the Department of Energy's decision for final disposition of spent nuclear fuel in the Geologic Repository at Yucca Mountain. The capability that is required to prepare Spent Nuclear Fuel for transportation and disposal outside the State of Idaho includes characterization, conditioning, packaging, onsite interim storage, and shipping cask loading to complete shipments by January 1,2035. These capabilities do not currently exist in Idaho.

  20. Application of spent fuel treatment technology to plutonium immobilization

    SciTech Connect

    McPheeters, C.C; Ackerman, J.P.; Gay, E.C., Johnson, G.K.

    1996-05-01

    The purpose of the electrometallurgical treatment technology being developed at Argonne National Laboratory (ANL) is to convert certain spent nuclear fuels into waste forms that are suitable for disposal in a geological repository for nuclear waste. The spent fuels of interest are those that cannot be safely stored for a long time in their current condition, and those that cannot be qualified for repository disposal. This paper explores the possibility of applying this electrometallurgical treatment technology to immobilization of surplus fissile materials, primarily plutonium. Immobilization of surplus fissile materials by electrometallurgical treatment could be done in the same facilities, at the same time. and in the same equipment as the proposed treatment of the present inventory of spent nuclear fuel. The cost and schedule savings of this simultaneous treatment scheme would be significant.

  1. Information handbook on independent spent fuel storage installations

    SciTech Connect

    Raddatz, M.G.; Waters, M.D.

    1996-12-01

    In this information handbook, the staff of the U.S. Nuclear Regulatory Commission describes (1) background information regarding the licensing and history of independent spent fuel storage installations (ISFSIs), (2) a discussion of the licensing process, (3) a description of all currently approved or certified models of dry cask storage systems (DCSSs), and (4) a description of sites currently storing spent fuel in an ISFSI. Storage of spent fuel at ISFSIs must be in accordance with the provisions of 10 CFR Part 72. The staff has provided this handbook for information purposes only. The accuracy of any information herein is not guaranteed. For verification or for more details, the reader should refer to the respective docket files for each DCSS and ISFSI site. The information in this handbook is current as of September 1, 1996.

  2. Status of Proposed Repository for Latin-American Spent Fuel

    SciTech Connect

    Ferrada, J.J.

    2004-10-04

    This report compiles preliminary information that supports the premise that a repository is needed in Latin America and analyzes the nuclear situation (mainly in Argentina and Brazil) in terms of nuclear capabilities, inventories, and regional spent-fuel repositories. The report is based on several sources and summarizes (1) the nuclear capabilities in Latin America and establishes the framework for the need of a permanent repository, (2) the International Atomic Energy Agency (IAEA) approach for a regional spent-fuel repository and describes the support that international institutions are lending to this issue, (3) the current situation in Argentina in order to analyze the Argentinean willingness to find a location for a deep geological repository, and (4) the issues involved in selecting a location for the repository and identifies a potential location. This report then draws conclusions based on an analysis of this information. The focus of this report is mainly on spent fuel and does not elaborate on other radiological waste sources.

  3. Applying fast calorimetry on a spent nuclear fuel calorimeter

    SciTech Connect

    Liljenfeldt, Henrik

    2015-04-15

    Recently at Los Alamos National Laboratory, sophisticated prediction algorithms have been considered for the use of calorimetry for treaty verification. These algorithms aim to predict the equilibrium temperature based on early data and therefore be able to shorten the measurement time while maintaining good accuracy. The algorithms have been implemented in MATLAB and applied on existing equilibrium measurements from a spent nuclear fuel calorimeter located at the Swedish nuclear fuel interim storage facility. The results show significant improvements in measurement time in the order of 15 to 50 compared to equilibrium measurements, but cannot predict the heat accurately in less time than the currently used temperature increase method can. This Is both due to uncertainties in the calibration of the method as well as identified design features of the calorimeter that limits the usefulness of equilibrium type measurements. The conclusions of these findings are discussed, and suggestions of both improvements of the current calorimeter as well as what to keep in mind in a new design are given.

  4. Initiation of depleted uranium oxide and spent fuel testing for the spent fuel sabotage aerosol ratio program.

    SciTech Connect

    Gregson, Michael Warren; Mo, Tin; Sorenson, Ken Bryce; Loiseau, Olivier; Nolte, Oliver; Hibbs, Russell S.; Molecke, Martin Alan; Slater-Thompson, Nancy; Autrusson, Bruno A.; Koch, Wolfgang; Pretzsch, Gunter Guido; Tsai, Han-Chung; Billone, Michael C.; Lange, Florentin; Young, Francis I.

    2004-08-01

    The authors provide a detailed overview of an on-going, multinational test program that is developing aerosol data for some spent fuel sabotage scenarios on spent fuel transport and storage casks. Experiments are being performed to quantify the aerosolized materials plus volatilized fission products generated from actual spent fuel and surrogate material test rods, due to impact by a high-energy-density device. The program participants in the United States plus Germany, France and the United Kingdom, part of the international Working Group for Sabotage Concerns of Transport and Storage Casks (WGSTSC) have strongly supported and coordinated this research program. Sandia National Laboratories has the lead role for conducting this research program; test program support is provided by both the US Department of Energy and the US Nuclear Regulatory Commission. The authors provide a summary of the overall, multiphase test design and a description of all explosive containment and aerosol collection test components used. They focus on the recently initiated tests on 'surrogate' spent fuel, unirradiated depleted uranium oxide and forthcoming actual spent fuel tests, and briefly summarize similar results from completed surrogate tests that used non-radioactive, sintered cerium oxide ceramic pellets in test rods.

  5. SPENT FUEL MANAGEMENT AT THE SAVANNAH RIVER SITE

    SciTech Connect

    Vormelker, P; Robert Sindelar, R; Richard Deible, R

    2007-11-03

    Spent nuclear fuels are received from reactor sites around the world and are being stored in the L-Basin at the Savannah River Site (SRS) in Aiken, South Carolina. The predominant fuel types are research reactor fuel with aluminum-alloy cladding and aluminum-based fuel. Other fuel materials include stainless steel and Zircaloy cladding with uranium oxide fuel. Chemistry control and corrosion surveillance programs have been established and upgraded since the early 1990's to minimize corrosion degradation of the aluminum cladding materials, so as to maintain fuel integrity and minimize personnel exposure from radioactivity in the basin water. Recent activities have been initiated to support additional decades of wet storage which include fuel inspection and corrosion testing to evaluate the effects of specific water impurity species on corrosion attack.

  6. German program for vitrified HLW and spent fuel management

    SciTech Connect

    Lutze, W.; Closs, K.D.; Tittel, G.; Brennecke, P.; Kunz, W.

    1993-12-31

    The paper covers four topics: management of vitrified waste, management of spent fuel, final disposal, and the repository safety assessment. At present, German spent fuel is reprocessed abroad and vitrified high-level radioactive waste will be returned for disposal. Interim storage of this waste in Germany will be necessary until the planned repository at Gorleben becomes available. Two interim storage facilities have been built. Additionally, about 60 m{sup 3} of HAWC (highly active waste concentrate) produced at the reprocessing plant in Karlsruhe prior to shutdown will be vitrified at the PAMELA plant in Mol, Belgium, following plant adaptations and the installation of a new melter. Direct disposal of spent fuel is being developed to technical maturity. A pilot conditioning and encapsulation plant is under construction at Gorleben, and repository-related demonstration tests are being performed. Layout and optimization studies for a common repository for reprocessing waste and spent fuel are underway, and a safeguards plan for spent fuel disposal has been developed. Results from these activities will be available early enough to be incorporated into the repository licensing procedure. The Gorleben salt dome has been selected for the construction and operation of a repository for all types of radioactive waste, especially heat generating, such as vitrified waste and spent fuel elements. Experimental research is being carried out to characterize and understand the long-term physico-chemical and geochemical behavior of the waste forms in the near field of the repository and the aquatic chemistry of radionuclides in the near and far fields.

  7. Systems for the Intermodal Routing of Spent Nuclear Fuel

    SciTech Connect

    Peterson, Steven K; Liu, Cheng

    2015-01-01

    The safe and secure movement of spent nuclear fuel from shutdown and active reactor facilities to intermediate or long term storage sites may, in some instances, require the use of several modes of transportation to accomplish the move. To that end, a fully operable multi-modal routing system is being developed within Oak Ridge National Laboratory s (ORNL) WebTRAGIS (Transportation Routing Analysis Geographic Information System). This study aims to provide an overview of multi-modal routing, the existing state of the TRAGIS networks, the source data needs, and the requirements for developing structural relationships between various modes to create a suitable system for modeling the transport of spent nuclear fuel via a multimodal network. Modern transportation systems are comprised of interconnected, yet separate, modal networks. Efficient transportation networks rely upon the smooth transfer of cargoes at junction points that serve as connectors between modes. A key logistical impediment to the shipment of spent nuclear fuel is the absence of identified or designated transfer locations between transport modes. Understanding the potential network impacts on intermodal transportation of spent nuclear fuel is vital for planning transportation routes from origin to destination. By identifying key locations where modes intersect, routing decisions can be made to prioritize cost savings, optimize transport times and minimize potential risks to the population and environment. In order to facilitate such a process, ORNL began the development of a base intermodal network and associated routing code. The network was developed using previous intermodal networks and information from publicly available data sources to construct a database of potential intermodal transfer locations with likely capability to handle spent nuclear fuel casks. The coding development focused on modifying the existing WebTRAGIS routing code to accommodate intermodal transfers and the selection of

  8. OECD NEA Benchmark Database of Spent Nuclear Fuel Isotopic Compositions for World Reactor Designs

    SciTech Connect

    Gauld, Ian C; Sly, Nicholas C; Michel-Sendis, Franco

    2014-01-01

    Experimental data on the isotopic concentrations in irradiated nuclear fuel represent one of the primary methods for validating computational methods and nuclear data used for reactor and spent fuel depletion simulations that support nuclear fuel cycle safety and safeguards programs. Measurement data have previously not been available to users in a centralized or searchable format, and the majority of accessible information has been, for the most part, limited to light-water-reactor designs. This paper describes a recent initiative to compile spent fuel benchmark data for additional reactor designs used throughout the world that can be used to validate computer model simulations that support nuclear energy and nuclear safeguards missions. Experimental benchmark data have been expanded to include VVER-440, VVER-1000, RBMK, graphite moderated MAGNOX, gas cooled AGR, and several heavy-water moderated CANDU reactor designs. Additional experimental data for pressurized light water and boiling water reactor fuels has also been compiled for modern assembly designs and more extensive isotopic measurements. These data are being compiled and uploaded to a recently revised structured and searchable database, SFCOMPO, to provide the nuclear analysis community with a centrally-accessible resource of spent fuel compositions that can be used to benchmark computer codes, models, and nuclear data. The current version of SFCOMPO contains data for eight reactor designs, 20 fuel assembly designs, more than 550 spent fuel samples, and measured isotopic data for about 80 nuclides.

  9. Spent fuel dissolution studies FY 1991 to 1994

    SciTech Connect

    Gray, W.J.; Wilson, C.N.

    1995-12-01

    Dissolution and transport as a result of groundwater flow are generally accepted as the primary mechanisms by which radionuclides from spent fuel placed in a geologic repository could be released to the biosphere. To help provide a source term for performance assessment calculations, dissolution studies on spent fuel and unirradiated uranium oxides have been conducted over the past few years at Pacific Northwest National Laboratory (PNNL) in support of the Yucca Mountain Site Characterization Project. This report describes work for fiscal years 1991 through 1994. The objectives of these studies and the associated conclusions, which were based on the limited number of tests conducted so far, are described in the following subsections.

  10. NUHOMS modular spent-fuel storage system: Performance testing

    SciTech Connect

    Strope, L.A.; McKinnon, M.A. ); Dyksterhouse, D.J.; McLean, J.C. )

    1990-09-01

    This report documents the results of a heat transfer and shielding performance evaluation of the NUTECH HOrizontal MOdular Storage (NUHOMS{reg sign}) System utilized by the Carolina Power and Light Co. (CP L) in an Independent Spent Fuel Storage Installation (ISFSI) licensed by the US Nuclear Regulatory Commission (NRC). The ISFSI is located at CP L's H. B. Robinson Nuclear Plant (HBR) near Hartsville, South Carolina. The demonstration included testing of three modules, first with electric heaters and then with spent fuel. The results indicated that the system was conservatively designed, with all heat transfer and shielding design criteria easily met. 5 refs., 45 figs., 9 tabs.

  11. Fast facility spent-fuel and waste assay instrument. [Fluorinel Dissolution and Fuel Storage (FAST) Facility

    SciTech Connect

    Eccleston, G.W.; Johnson, S.S.; Menlove, H.O.; Van Lyssel, T.; Black, D.; Carlson, B.; Decker, L.; Echo, M.W.

    1983-01-01

    A delayed-neutron assay instrument was installed in the Fluorinel Dissolution and Fuel Storage Facility at Idaho National Engineering Laboratory. The dual-assay instrument is designed to measure both spent fuel and waste solids that are produced from fuel processing. A set of waste standards, fabricated by Los Alamos using uranium supplied by Exxon Nuclear Idaho Company, was used to calibrate the small-sample assay region of the instrument. Performance testing was completed before installation of the instrument to determine the effects of uranium enrichment, hydrogenous materials, and neutron poisons on assays. The unit was designed to measure high-enriched uranium samples in the presence of large neutron backgrounds. Measurements indicate that the system can assay low-enriched uranium samples with moderate backgrounds if calibrated with proper standards.

  12. Reactor-specific spent fuel discharge projections, 1984 to 2020

    SciTech Connect

    Heeb, C.M.; Libby, R.A.; Holter, G.M.

    1985-04-01

    The original spent fuel utility data base (SFDB) has been adjusted to produce agreement with the EIA nuclear energy generation forecast. The procedure developed allows the detail of the utility data base to remain intact, while the overall nuclear generation is changed to match any uniform nuclear generation forecast. This procedure adjusts the weight of the reactor discharges as reported on the SFDB and makes a minimal (less than 10%) change in the original discharge exposures in order to preserve discharges of an integral number of fuel assemblies. The procedure used in developing the reactor-specific spent fuel discharge projections, as well as the resulting data bases themselves, are described in detail in this report. Discussions of the procedure cover the following topics: a description of the data base; data base adjustment procedures; addition of generic power reactors; and accuracy of the data base adjustments. Reactor-specific discharge and storage requirements are presented. Annual and cumulative discharge projections are provided. Annual and cumulative requirements for additional storage are shown for the maximum at-reactor (AR) storage assumption, and for the maximum AR with transshipment assumption. These compare directly to the storage requirements from the utility-supplied data, as reported in the Spent Fuel Storage Requirements Report. The results presented in this report include: the disaggregated spent fuel discharge projections; and disaggregated projections of requirements for additional spent fuel storage capacity prior to 1998. Descriptions of the methodology and the results are included in this report. Details supporting the discussions in the main body of the report, including descriptions of the capacity and fuel discharge projections, are included. 3 refs., 6 figs., 12 tabs.

  13. Spent fuel dry storage technology development: thermal evaluation of isolated drywells containing spent fuel (1 kW PWR spent fuel assembly)

    SciTech Connect

    Unterzuber, R; Wright, J B

    1980-09-01

    A spent fuel Isolated Drywell Test was conducted at the Engine-Maintenance, Assembly and Disassembly (E-MAD) facility on the Nevada Test Site. Two PWR spent fuel assemblies having a decay heat level of approximately 1.1 kW were encapsulated inside the E-MAD Hot Bay and placed in instrumented near-surface drywell storage cells. Temperatures from the two isolated drywells and the adjacent soil have been recorded throughout the 19 month Isolated Drywell Test. Canister and drywell liner temperatures reached their peak values (254{sup 0}F and 203{sup 0}F, respectively) during August 1979. Thereafter, all temperatures decreased and showed a cycling pattern which responded to seasonal atmospheric temperature changes. A computer model was utilized to predict the thermal response of the drywell. Computer predictions of the drywell temperatures and the temperatures of the surrounding soil are presented and show good agreement with the test data.

  14. Anticipating Potential Waste Acceptance Criteria for Defense Spent Nuclear Fuel

    SciTech Connect

    Rechard, R.P.; Lord, M.E.; Stockman, C.T.; McCurley, R.D.

    1997-12-31

    The Office of Environmental Management of the U.S. Department of Energy is responsible for the safe management and disposal of DOE owned defense spent nuclear fuel and high level waste (DSNF/DHLW). A desirable option, direct disposal of the waste in the potential repository at Yucca Mountain, depends on the final waste acceptance criteria, which will be set by DOE`s Office of Civilian Radioactive Waste Management (OCRWM). However, evolving regulations make it difficult to determine what the final acceptance criteria will be. A method of anticipating waste acceptance criteria is to gain an understanding of the DOE owned waste types and their behavior in a disposal system through a performance assessment and contrast such behavior with characteristics of commercial spent fuel. Preliminary results from such an analysis indicate that releases of 99Tc and 237Np from commercial spent fuel exceed those of the DSNF/DHLW; thus, if commercial spent fuel can meet the waste acceptance criteria, then DSNF can also meet the criteria. In large part, these results are caused by the small percentage of total activity of the DSNF in the repository (1.5%) and regulatory mass (4%), and also because commercial fuel cladding was assumed to provide no protection.

  15. Treatment of oxide spent fuel using the lithium reduction process

    SciTech Connect

    Karell, E.J.; Pierce, R.D.; Mulcahey, T.P.

    1996-05-01

    The wide variety in the composition of DOE spent nuclear fuel complicates its long-term disposition because of the potential requirement to individually qualify each type of fuel for repository disposal. Argonne National Laboratory (ANL) has developed the electrometallurgical treatment technique to convert all of these spent fuel types into a single set of disposal forms, simplifying the qualification process. While metallic fuels can be directly processed using the electrometallurgical treatment technique, oxide fuels must first be reduced to the metallic form. The lithium reduction process accomplishes this pretreatment. In the lithium process the oxide components of the fuel are reduced using lithium at 650 C in the presence of molten LiCl, yielding the corresponding metals and Li{sub 2}O. The reduced metal components are then separated from the LiCl salt phase and become the feed material for electrometallurgical treatment. A demonstration test of the lithium reduction process was successfully conducted using a 10-kg batch of simulated oxide spent fuel and engineering-scale equipment specifically constructed for that purpose. This paper describes the lithium process, the equipment used in the demonstration test, and the results of the demonstration test.

  16. MANAGING SPENT NUCLEAR FUEL WASTES AT THE IDAHO NATIONAL LABORATORY

    SciTech Connect

    Hill, Thomas J

    2005-09-01

    The Idaho National Engineering Laboratory (INL) has a large inventory of diverse types of spent nuclear fuel (SNF). This legacy is in part due to the history of the INL as the National Reactor Testing Station, in part to its mission to recover highly enriched uranium from SNF and in part to it’s mission to test and examine SNF after irradiation. The INL also has a large diversity of SNF storage facility, some dating back 50 years in the site history. The success of the INL SNF program is measured by its ability to: 1) achieve safe existing storage, 2) continue to receive SNF from other locations, both foreign and domestic, 3) repackage SNF from wet storage to interim dry storage, and 4) prepare the SNF for dispositioning in a federal repository. Because of the diversity in the SNF and the facilities at the INL, the INL is addressing almost very condition that may exist in the SNF world. Many of solutions developed by the INL are applicable to other SNF storage sites as they develop their management strategy. The SNF being managed by the INL are in a variety of conditions, from intact assemblies to individual rods or plates to powders, rubble, and metallurgical mounts. Some of the fuel has been in wet storage for over forty years. The fuel is stored bare, or in metal cans and either wet under water or dry in vaults, caissons or casks. Inspections have shown varying degrees of corrosion and degradation of the fuel and the storage cans. Some of the fuel has been recanned under water, and the conditions of the fuel inside the second or third can are unknown. The fuel has been stored in one of 10 different facilities: five wet pools and one casks storage pad, one vault, two generations of caisson facilities, and one modular Independent Spent Fuel Storage Installation (ISFSI). The wet pools range from forty years old to the most modern pool in the US Department of Energy (DOE) complex. The near-term objective is moving the fuel in the older wet storage facilities to

  17. Impact of Nuclear Data Uncertainties on Calculated Spent Fuel Nuclide Inventories and Advanced NDA Instrument Response

    DOE PAGES

    Hu, Jianwei; Gauld, Ian C.

    2014-12-01

    The U.S. Department of Energy’s Next Generation Safeguards Initiative Spent Fuel (NGSI-SF) project is nearing the final phase of developing several advanced nondestructive assay (NDA) instruments designed to measure spent nuclear fuel assemblies for the purpose of improving nuclear safeguards. Current efforts are focusing on calibrating several of these instruments with spent fuel assemblies at two international spent fuel facilities. Modelling and simulation is expected to play an important role in predicting nuclide compositions, neutron and gamma source terms, and instrument responses in order to inform the instrument calibration procedures. As part of NGSI-SF project, this work was carried outmore » to assess the impacts of uncertainties in the nuclear data used in the calculations of spent fuel content, radiation emissions and instrument responses. Nuclear data is an essential part of nuclear fuel burnup and decay codes and nuclear transport codes. Such codes are routinely used for analysis of spent fuel and NDA safeguards instruments. Hence, the uncertainties existing in the nuclear data used in these codes affect the accuracies of such analysis. In addition, nuclear data uncertainties represent the limiting (smallest) uncertainties that can be expected from nuclear code predictions, and therefore define the highest attainable accuracy of the NDA instrument. This work studies the impacts of nuclear data uncertainties on calculated spent fuel nuclide inventories and the associated NDA instrument response. Recently developed methods within the SCALE code system are applied in this study. The Californium Interrogation with Prompt Neutron instrument was selected to illustrate the impact of these uncertainties on NDA instrument response.« less

  18. Impact of Nuclear Data Uncertainties on Calculated Spent Fuel Nuclide Inventories and Advanced NDA Instrument Response

    SciTech Connect

    Hu, Jianwei; Gauld, Ian C.

    2014-12-01

    The U.S. Department of Energy’s Next Generation Safeguards Initiative Spent Fuel (NGSI-SF) project is nearing the final phase of developing several advanced nondestructive assay (NDA) instruments designed to measure spent nuclear fuel assemblies for the purpose of improving nuclear safeguards. Current efforts are focusing on calibrating several of these instruments with spent fuel assemblies at two international spent fuel facilities. Modelling and simulation is expected to play an important role in predicting nuclide compositions, neutron and gamma source terms, and instrument responses in order to inform the instrument calibration procedures. As part of NGSI-SF project, this work was carried out to assess the impacts of uncertainties in the nuclear data used in the calculations of spent fuel content, radiation emissions and instrument responses. Nuclear data is an essential part of nuclear fuel burnup and decay codes and nuclear transport codes. Such codes are routinely used for analysis of spent fuel and NDA safeguards instruments. Hence, the uncertainties existing in the nuclear data used in these codes affect the accuracies of such analysis. In addition, nuclear data uncertainties represent the limiting (smallest) uncertainties that can be expected from nuclear code predictions, and therefore define the highest attainable accuracy of the NDA instrument. This work studies the impacts of nuclear data uncertainties on calculated spent fuel nuclide inventories and the associated NDA instrument response. Recently developed methods within the SCALE code system are applied in this study. The Californium Interrogation with Prompt Neutron instrument was selected to illustrate the impact of these uncertainties on NDA instrument response.

  19. Test plan for thermogravimetric analyses of BWR spent fuel oxidation

    SciTech Connect

    Einziger, R.E.

    1988-12-01

    Preliminary studies indicated the need for additional low-temperature spent fuel oxidation data to determine the behavior of spent fuel as a waste form for a tuffy repository. Short-term thermogravimetric analysis tests were recommended in a comprehensive technical approach as the method for providing scoping data that could be used to (1) evaluate the effects of variables such as moisture and burnup on the oxidation rate, (2) determine operative mechanisms, and (3) guide long-term, low-temperature oxidation testing. The initial test series studied the temperature and moisture effects on pressurized water reactor fuel as a function of particle and grain size. This document presents the test matrix for studying the oxidation behavior of boiling water reactor fuel in the temperature range of 140 to 225{degree}C. 17 refs., 7 figs., 3 tabs.

  20. Spent fuel utilization in a compact traveling wave reactor

    NASA Astrophysics Data System (ADS)

    Hartanto, Donny; Kim, Yonghee

    2012-06-01

    In recent years, several innovative designs of nuclear reactors are proposed. One of them is Traveling Wave Reactor (TWR). The unique characteristic of a TWR is the capability of breeding its own fuel in the reactor. The reactor is fueled by mostly depleted, natural uranium or spent nuclear fuel and a small amount of enriched uranium to initiate the fission process. Later on in the core, the reactor gradually converts the non-fissile material into the fissile in a process like a traveling wave. In this work, a TWR with spent nuclear fuel blanket was studied. Several parameters such as reactivity coefficients, delayed neutron fraction, prompt neutron generation lifetime, and fission power, were analyzed. The discharge burnup composition was also analyzed. The calculation is performed by a continuous energy Monte Carlo code McCARD.

  1. Annual report, FY 1979 Spent fuel and fuel pool component integrity.

    SciTech Connect

    Johnson, A.B. Jr.; Bailey, W.J.; Schreiber, R.E.; Kustas, F.M.

    1980-05-01

    International meetings under the BEFAST program and under INFCE Working Group No. 6 during 1978 and 1979 continue to indicate that no cases of fuel cladding degradation have developed on pool-stored fuel from water reactors. A section from a spent fuel rack stand, exposed for 1.5 y in the Yankee Rowe (PWR) pool had 0.001- to 0.003-in.-deep (25- to 75-..mu..m) intergranular corrosion in weld heat-affected zones but no evidence of stress corrosion cracking. A section of a 304 stainless steel spent fuel storage rack exposed 6.67 y in the Point Beach reactor (PWR) spent fuel pool showed no significant corrosion. A section of 304 stainless steel 8-in.-dia pipe from the Three Mile Island No. 1 (PWR) spent fuel pool heat exchanger plumbing developed a through-wall crack. The crack was intergranular, initiating from the inside surface in a weld heat-affected zone. The zone where the crack occurred was severely sensitized during field welding. The Kraftwerk Union (Erlangen, GFR) disassembled a stainless-steel fuel-handling machine that operated for 12 y in a PWR (boric acid) spent fuel pool. There was no evidence of deterioration, and the fuel-handling machine was reassembled for further use. A spent fuel pool at a Swedish PWR was decontaminated. The procedure is outlined in this report.

  2. NAC-1 cask dose rate calculations for LWR spent fuel

    SciTech Connect

    CARLSON, A.B.

    1999-02-24

    A Nuclear Assurance Corporation nuclear fuel transport cask, NAC-1, is being considered as a transport and storage option for spent nuclear fuel located in the B-Cell of the 324 Building. The loaded casks will be shipped to the 200 East Area Interim Storage Area for dry interim storage. Several calculations were performed to assess the photon and neutron dose rates. This report describes the analytical methods, models, and results of this investigation.

  3. Air Shipment of Spent Nuclear Fuel from Romania to Russia

    SciTech Connect

    Igor Bolshinsky; Ken Allen; Lucian Biro; Alexander Buchelnikov

    2010-10-01

    Romania successfully completed the world’s first air shipment of spent nuclear fuel transported in Type B(U) casks under existing international laws and without shipment license special exceptions when the last Romanian highly enriched uranium (HEU) spent nuclear fuel was transported to the Russian Federation in June 2009. This air shipment required the design, fabrication, and licensing of special 20 foot freight containers and cask tiedown supports to transport the eighteen TUK 19 shipping casks on a Russian commercial cargo aircraft. The new equipment was certified for transport by road, rail, water, and air to provide multi modal transport capabilities for shipping research reactor spent fuel. The equipment design, safety analyses, and fabrication were performed in the Russian Federation and transport licenses were issued by both the Russian and Romanian regulatory authorities. The spent fuel was transported by truck from the VVR S research reactor to the Bucharest airport, flown by commercial cargo aircraft to the airport at Yekaterinburg, Russia, and then transported by truck to the final destination in a secure nuclear facility at Chelyabinsk, Russia. This shipment of 23.7 kg of HEU was coordinated by the Russian Research Reactor Fuel Return Program (RRRFR), as part of the U.S. Department of Energy Global Threat Reduction Initiative (GTRI), in close cooperation with the Rosatom State Atomic Energy Corporation and the International Atomic Energy Agency, and was managed in Romania by the National Commission for Nuclear Activities Control (CNCAN). This paper describes the planning, shipment preparations, equipment design, and license approvals that resulted in the safe and secure air shipment of this spent nuclear fuel.

  4. Spent fuel sabotage aerosol ratio program : FY 2004 test and data summary.

    SciTech Connect

    Brucher, Wenzel; Koch, Wolfgang; Pretzsch, Gunter Guido; Loiseau, Olivier; Mo, Tin; Billone, Michael C.; Autrusson, Bruno A.; Young, F. I.; Coats, Richard Lee; Burtseva, Tatiana; Luna, Robert Earl; Dickey, Roy R.; Sorenson, Ken Bryce; Nolte, Oliver; Thompson, Nancy Slater; Hibbs, Russell S.; Gregson, Michael Warren; Lange, Florentin; Molecke, Martin Alan; Tsai, Han-Chung

    2005-07-01

    This multinational, multi-phase spent fuel sabotage test program is quantifying the aerosol particles produced when the products of a high energy density device (HEDD) interact with and explosively particulate test rodlets that contain pellets of either surrogate materials or actual spent fuel. This program has been underway for several years. This program provides data that are relevant to some sabotage scenarios in relation to spent fuel transport and storage casks, and associated risk assessments. The program also provides significant technical and political benefits in international cooperation. We are quantifying the Spent Fuel Ratio (SFR), the ratio of the aerosol particles released from HEDD-impacted actual spent fuel to the aerosol particles produced from surrogate materials, measured under closely matched test conditions, in a contained test chamber. In addition, we are measuring the amounts, nuclide content, size distribution of the released aerosol materials, and enhanced sorption of volatile fission product nuclides onto specific aerosol particle size fractions. These data are the input for follow-on modeling studies to quantify respirable hazards, associated radiological risk assessments, vulnerability assessments, and potential cask physical protection design modifications. This document includes an updated description of the test program and test components for all work and plans made, or revised, during FY 2004. It also serves as a program status report as of the end of FY 2004. All available test results, observations, and aerosol analyses plus interpretations--primarily for surrogate material Phase 2 tests, series 2/5A through 2/9B, using cerium oxide sintered ceramic pellets are included. Advanced plans and progress are described for upcoming tests with unirradiated, depleted uranium oxide and actual spent fuel test rodlets. This spent fuel sabotage--aerosol test program is coordinated with the international Working Group for Sabotage Concerns of

  5. Effects of Water in Canisters Containing DOE Spent Nuclear Fuel

    SciTech Connect

    P. A. Lessing

    1998-10-01

    This document is a starting analysis in an attempt to quantify the potential of problems resulting from the presence of condensed water and water vapor in sealed storage canisters containing spent nuclear fuel (SNF). Of the 55 spent fuel types, it was determined that only three types required study to evaluate the effects of water, these types were represented by: (1) zirconium clad N-Reactor fuel, (2) aluminum clad Advanced Test Reactor (ATR) or Materials Test Reactor (MTR) fuel, (3) damaged and/or melted zirconium clad Three Mile Island (TMI) fuel. The spent fuel types were briefly described and potential problems were generalized into four catagories: (1) effects of water and the source(s) of that water, (2) effects of hydrogen generated from water, (3) pyrophoricity of uranium hydride, (4) swelling or cavitation. An extensive literature search was conducted, chemical reactions considered, and simple pressurization sensitivity calculations performed. Using the available information, conclusions were drawn and issues identified that need further consideration or analysis.

  6. High Burn-Up Spent Nuclear Fuel Vibration Integrity Study

    SciTech Connect

    Wang, Jy-An John; Wang, Hong; Jiang, Hao; Bevard, Bruce Balkcom; Howard, Rob L; Scaglione, John M

    2015-01-01

    The Oak Ridge National Laboratory (ORNL) has developed the cyclic integrated reversible-bending fatigue tester (CIRFT) approach to successfully demonstrate the controllable fatigue fracture on high burnup (HBU) spent nuclear fuel (SNF) in a normal vibration mode. CIRFT enables examination of the underlying mechanisms of SNF system dynamic performance. Due to the inhomogeneous composite structure of the SNF system, the detailed mechanisms of the pellet-pellet and pellet-clad interactions and the stress concentration effects at the pellet-pellet interface cannot be readily obtained from a CIRFT system measurement. Therefore, finite element analyses (FEAs) are used to translate the global moment-curvature measurement into local stress-strain profiles for further investigation. The major findings of CIRFT on the HBU SNF are as follows: SNF system interface bonding plays an important role in SNF vibration performance. Fuel structure contributes to SNF system stiffness. There are significant variations in stress and curvature of SNF systems during vibration cycles resulting from segment pellets and clad interactions. SNF failure initiates at the pellet-pellet interface region and appears to be spontaneous.

  7. Criticality safety considerations in the geologic disposal of spent nuclear fuel assemblies

    NASA Astrophysics Data System (ADS)

    Gore, B. F.; McNair, G. W.; Heaberlin, S. W.

    1980-05-01

    Features of geologic disposal which hamper the demonstration that criticality cannot occur therein include possible changes of shape and form, intrusion of water as a neutron moderator, and selective leaching of spent fuel constituents. If the criticality safety of spent fuels disposal depends on burnup, independent measurements verifying the burnup should be performed prior to disposal. The status of nondestructive analysis method which might provide such verification is discussed. Calculations were performed to assess the potential for increasing the allowed size of a spent fuel disposal canister if potential water intrusion were limited by close packing the enclosed rods. Several factors were identified which severely limited the potential of this application. The theoretical limit of hexagonal close packing cannot be achieved due to fuel rod bowing. It is concluded the disposal canisters should be sized on the basis of assumed optimum moderation.

  8. Maintaining Continuity of Knowledge of Spent Fuel Pools: Tool Survey

    SciTech Connect

    Benz, Jacob M.; Smartt, Heidi A.; Tanner, Jennifer E.; MacDougall, Matthew R.

    2016-08-30

    This report examines supplemental tools that can be used in addition to optical surveillance cameras to maintain CoK in low-to-no light conditions, and increase the efficiency and effectiveness of spent fuel CoK, including item counting and ID verification, in challenging conditions.

  9. Pinhole Breaches in Spent Fuel Containers: Some Modeling Considerations

    SciTech Connect

    Casella, Andrew M.; Loyalka, Sudarsham K.; Hanson, Brady D.

    2006-06-04

    This paper replaces PNNL-SA-48024 and incorporates the ANS reviewer's comments, including the change in the title. Numerical methods to solve the equations for gas diffusion through very small breaches in spent fuel containers are presented and compared with previous literature results.

  10. Spent nuclear fuel project design basis capacity study

    SciTech Connect

    Cleveland, K.J.

    1996-09-09

    A parametric study of the Spent Nuclear Fuel Project system capacity is presented. The study was completed using a commercially available software package to develop a summary level model of the major project systems. Alternative configurations, sub-system cycle times, and operating scenarios were tested to identify their impact on total project duration and equipment requirements.

  11. Spent fuel test. Climax data acquisition system integration report

    SciTech Connect

    Nyholm, R.A.; Brough, W.G.; Rector, N.L.

    1982-06-01

    The Spent Fuel Test - Climax (SFT-C) is a test of the retrievable, deep geologic storage of commercially generated, spent nuclear reactor fuel in granitic rock. Eleven spent fuel assemblies, together with 6 electrical simulators and 20 guard heaters, are emplaced 420 m below the surface in the Climax granite at the Nevada Test Site. On June 2, 1978, Lawrence Livermore National Laboratory (LLNL) secured funding for the SFT-C, and completed spent fuel emplacement May 28, 1980. This multi-year duration test is located in a remote area and is unattended much of the time. An extensive array of radiological safety and geotechnical instrumentation is deployed to monitor the test performance. A dual minicomputer-based data acquisition system collects and processes data from more than 900 analog instruments. This report documents the design and functions of the hardware and software elements of the Data Acquisition System and describes the supporting facilities which include environmental enclosures, heating/air-conditioning/humidity systems, power distribution systems, fire suppression systems, remote terminal stations, telephone/modem communications, and workshop areas. 9 figures.

  12. Status of spent-fuel transportation system development

    SciTech Connect

    Chapman, R.L.; Hall, I.K.

    1988-01-01

    The purpose of the Cask Systems Development Program (CSDP) is to develop a variety of cask systems that can safely and economically be used to move commercial spent fuel and high-level waste from the generator to the federal repository or monitored retrievable storage facility. There are four initiatives to the CSDP, but only the first, from reactor casks, has been activated. This paper is limited to a discussion of the status of that initiative. Schedule objectives for the CSDP include development of spent-fuel cask systems by 1995 to support the Office of Civilian Radioactive Waste Management shipments of spent fuel from utilities beginning in the late 1990s. The US Department of Energy (DOE)-Idaho, with the support of EG G Idaho, Inc., Sandia National Laboratories, and selected cask development contractors, has been assigned the responsibility for developing a family of cask systems that are suitable for the task. Initially, four categories of spent-fuel casks were to be developed. They are legal-weight truck (LWT) casks, overweight truck (OWT) casks, rail/barge (R/B) casks, and dual purpose (DP) (storage/transport) casks. For a variety of reasons, OWT and DP cask development activities have been deferred. Program goals include developing a family of casks that will permit minimizing total system life cycle costs, ensure safety to the general public and to occupational workers, and attain public confidence in the transportation system.

  13. Review of Drying Methods for Spent Nuclear Fuel

    SciTech Connect

    Large, W.S.

    1999-10-21

    SRTC is developing technology for direct disposal of aluminum spent nuclear fuel (SNF). The development program includes analyses and tests to support design and safe operation of a facility for ''road ready'' dry storage of SNF-filled canisters. The current technology development plan includes review of available SNF drying methods and recommendation of a drying method for aluminum SNF.

  14. Monitoring of spent nuclear fuel with antineutrino detectors

    NASA Astrophysics Data System (ADS)

    Brdar, Vedran

    2017-09-01

    We put forward the possibility of employing antineutrino detectors in order to control the amounts of spent nuclear fuel in repositories or, alternatively, to precisely localize the underground sources of nuclear material. For instance, we discuss the applicability in determining a possible leakage of stored nuclear material which would aid in preventing environmental problems. The long-term storage facilities are also addressed.

  15. Severe accidents in spent fuel pools in support of generic safety, Issue 82

    SciTech Connect

    Sailor, V.L.; Perkins, K.R.; Weeks, J.R.; Connell, H.R.

    1987-07-01

    This investigation provides an assessment of the likelihood and consequences of a severe accident in a spent fuel storage pool - the complete draining of the pool. Potential mechanisms and conditions for failure of the spent fuel, and the subsequent release of the fission products, are identified. Two older PWR and BWR spent fuel storage pool designs are considered based on a preliminary screening study which tried to identify vulnerabilities. Internal and external events and accidents are assessed. Conditions which could lead to failure of the spent fuel Zircaloy cladding as a result of cladding rupture or as a result of a self-sustaining oxidation reaction are presented. Propagation of a cladding fire to older stored fuel assemblies is evaluated. Spent fuel pool fission product inventory is estimated and the releases and consequences for the various cladding scenarios are provided. Possible preventive or mitigative measures are qualitatively evaluated. The uncertainties in the risk estimate are large, and areas where additional evaluations are needed to reduce uncertainty are identified.

  16. Validation of Inverse Methods Applied to Forensic Analysis of Spent Fuel

    SciTech Connect

    Broadhead, Bryan L; Weber, Charles F

    2010-01-01

    Inverse depletion/decay methods are useful tools for application to nuclear forensics. Previously, inverse methods were applied to the generic case of predicting the burnup, initial enrichment, and cooling time for selected spent nuclear fuels based on measured actinide and fission product concentrations. These existing measurements were not developed or optimized for use by these inverse techniques, and hence previous work demonstrated the prediction of only the fuel burnup, initial enrichment, and cooling time. Previously, nine spent fuel samples from an online data compilation were randomly selected for study. This work set out to demonstrate the full prediction capabilities using measured isotopic data, but with a more deliberate selection of fuel samples. The current approach is to evaluate nuclides within the same element to see if complementary information can be obtained in addition to the reactor burnup, enrichment, and cooling. Specifically, the reactor power and the fuel irradiation time values are desired to achieve the maximum prediction capabilities of these techniques.

  17. Department of Energy Programmatic Spent Nuclear Fuel Management and Idaho National Engineering Laboratory Environmental Restoration and Waste Management Programs Draft Environmental Impact Statement. Volume 1, Appendix C, Savannah River Site Spent Nuclear Fuel Mangement Program

    SciTech Connect

    Not Available

    1994-06-01

    The US Department of Energy (DOE) is engaged in two related decision making processes concerning: (1) the transportation, receipt, processing, and storage of spent nuclear fuel (SNF) at the DOE Idaho National Engineering Laboratory (INEL) which will focus on the next 10 years; and (2) programmatic decisions on future spent nuclear fuel management which will emphasize the next 40 years. DOE is analyzing the environmental consequences of these spent nuclear fuel management actions in this two-volume Environmental Impact Statement (EIS). Volume 1 supports broad programmatic decisions that will have applicability across the DOE complex and describes in detail the purpose and need for this DOE action. Volume 2 is specific to actions at the INEL. This document, which limits its discussion to the Savannah River Site (SRS) spent nuclear fuel management program, supports Volume 1 of the EIS. Following the introduction, Chapter 2 contains background information related to the SRS and the framework of environmental regulations pertinent to spent nuclear fuel management. Chapter 3 identifies spent nuclear fuel management alternatives that DOE could implement at the SRS, and summarizes their potential environmental consequences. Chapter 4 describes the existing environmental resources of the SRS that spent nuclear fuel activities could affect. Chapter 5 analyzes in detail the environmental consequences of each spent nuclear fuel management alternative and describes cumulative impacts. The chapter also contains information on unavoidable adverse impacts, commitment of resources, short-term use of the environment and mitigation measures.

  18. Modelling of the spent fuel oxidation: Toward the operational model

    NASA Astrophysics Data System (ADS)

    Rouyer, J.; Poulesquen, A.; Desgranges, L.; Ferry, C.

    2009-12-01

    As part of a long-lasting dry storage, the oxidation of the spent fuel linked to an accidental supply of oxygen into the spent fuel rod, may have consequences that must be assessed. Indeed, the oxidation of the UO 2 fuel up to U 3O 8 phase brings about a volume swelling of about 31% together with a bulking which may increase the initial defect of the cladding and thus lead to the release of fission products which remains embedded in nanometric gains or fine particles. From the oxidation model first developed (grain model), a new model has been proposed to describe the oxidation of spent fuel. The latter is based on a transposition of the graded grain model for unirradiated powders to irradiated grains. The modification of the grain model concerns the structural evolutions and the stoichiometric ranges during the oxidation. The convolution between the irradiated grain model and the propagation of the oxidation front along the grain boundaries allow to describe the oxidation kinetics of a spent fuel fragment. A criterion of grain breaking, based on experimental observations, has been proposed. The model has been parametrized from the experimental data of the literature and obtained as part of the French PRECCI's program. The harmony between the model and the experimental data either in terms of mass gain curves or of the oxygen diffusion coefficients in the UO 2 matrix is satisfactory. From this mechanistic model, an operational model for dry storage is proposed. On one hand, a simplified model (qualitative one) allowing to link the operational parameters (irradiation history) such as the burn up, the linear power or else the released gas fraction to a time for cracks to appear in the grains has been proposed. This model allows to display the time for the fractures in the fuel to appear (or a time before fracturing) according to the review of the treated fuels. On the other hand, a predictive operational model taking only the temperature into account is proposed.

  19. Management of super-grade plutonium in spent nuclear fuel

    SciTech Connect

    McFarlane, H. F.; Benedict, R. W.

    2000-03-20

    This paper examines the security and safeguards implications of potential management options for DOE's sodium-bonded blanket fuel from the EBR-II and the Fermi-1 fast reactors. The EBR-II fuel appears to be unsuitable for the packaging alternative because of DOE's current safeguards requirements for plutonium. Emerging DOE requirements, National Academy of Sciences recommendations, draft waste acceptance requirements for Yucca Mountain and IAEA requirements for similar fuel also emphasize the importance of safeguards in spent fuel management. Electrometallurgical treatment would be acceptable for both fuel types. Meeting the known requirements for safeguards and security could potentially add more than $200M in cost to the packaging option for the EBR-II fuel.

  20. Near-term commercial spent fuel shipping cask requirements

    SciTech Connect

    Daling, P.M.

    1984-11-01

    This report describes an analysis of the near-term commercial light water reactor (LWR) spent fuel transportation system. The objective was to determine if the existing commercial spent fuel shipping cask fleet is adequate to provide the needed transportation services for the period of time the US government would be authorized to accept spent fuel for Federal Interim Storage (FIS). A spent fuel shipping cask supply-demand analysis was performed to evaluate the existing fleet size. The results of the shipping cask handling capability study indicated that by weight, 75% of the spent fuel shipments will be by truck (overweight plus legal-weight truck). From the results of the shipping cask supply-demand analysis it was concluded that, if utilities begin large-scale applications for FIS, the five legal-weight truck (LWT) casks currently in service would be inadequate to perform all of the needed shipments as early as 1987. This further assumes that a western site would be selected for the FIS facility. If the FIS site were to be located in the East, the need for additional LWT casks would be delayed by about two years. The overweight truck (OWT) cask fleet (two PWR and two BWR versions) will be adequate through 1992 if some shipments to FIS can be made several years before a reactor is projected to lose full core reserve. This is because OWT cask requirements increase gradually over the next several years. The feasibility of shipping before losing full core reserve has not been evaluated. Cask utilization requirements in later years will be reduced if some shipments can be made prior to the time they are actually needed. The existing three rail casks are adequate to perform near-term shipments. 18 references, 4 figures, 18 tables.

  1. Regulation of spent nuclear fuel shipment: A state perspective

    SciTech Connect

    Halstead, R.J.; Sinderbrand, C.; Woodbury, D.

    1987-01-01

    In 1985, the Wisconsin Department of Natural Resources (WDNR) sought to regulate rail shipments of spent nuclear fuel through the state, because federal regulations did not adequately protect the environmentally sensitive corridor along the route of the shipments. A state interagency working group identified five serious deficiencies in overall federal regulatory scheme: 1) failure to consider the safety or environmental risks associated with selected routes; 2) abscence of route-specific emergency response planning; 3) failure of the NRC to regulate the carrier of spent nuclear fuel or consider its safety record; 4) abscence of requirements for determination of need for, or the propriety of, specific shipments of spent nuclear fuel; and 5) the lack of any opportunity for meaningful public participation with respect to the decision to transport spent nuclear fuel. Pursuant to Wisconsin's hazardous substance statutes, the WDNR issues an order requiring the utility to file a spill prevention and mitigation plan or cease shipping through Wisconsin. A state trial court judge upheld the utility's challenge to Wisconsin's spill plan requirements, based on federal preemption of state authority. The state is now proposing federal legislation which would require: 1) NRC determination of need prior to approval of offsite shipment of spent fuel by the licensees; 2) NRC assessment of the potential environmental impacts of shipments along the proposed route, and comparative evaluation of alternative modes and routes; and 3) NRC approval of a route-specific emergency response and mitigation plan, including local training and periodic exercises. Additionally, the proposed legislation would authorize States and Indian Tribes to establish regulatory programs providing for permits, inspection, contingency plans for monitoring, containments, cleanup and decontamination, surveillance, enforcement and reasonable fees. 15 refs.

  2. Surrogate/spent fuel sabotage : aerosol ratio test program and Phase 2 test results.

    SciTech Connect

    Borek, Theodore Thaddeus III; Thompson, N. Slater; Sorenson, Ken Bryce; Hibbs, R.S.; Nolte, Oliver; Molecke, Martin Alan; Autrusson, Bruno; Young, F. I.; Koch, Wolfgang; Brochard, Didier; Pretzsch, Gunter Guido; Lange, Florentin

    2004-05-01

    A multinational test program is in progress to quantify the aerosol particulates produced when a high energy density device, HEDD, impacts surrogate material and actual spent fuel test rodlets. This program provides needed data that are relevant to some sabotage scenarios in relation to spent fuel transport and storage casks, and associated risk assessments; the program also provides significant political benefits in international cooperation. We are quantifying the spent fuel ratio, SFR, the ratio of the aerosol particles released from HEDD-impacted actual spent fuel to the aerosol particles produced from surrogate materials, measured under closely matched test conditions. In addition, we are measuring the amounts, nuclide content, size distribution of the released aerosol materials, and enhanced sorption of volatile fission product nuclides onto specific aerosol particle size fractions. These data are crucial for predicting radiological impacts. This document includes a thorough description of the test program, including the current, detailed test plan, concept and design, plus a description of all test components, and requirements for future components and related nuclear facility needs. It also serves as a program status report as of the end of FY 2003. All available test results, observations, and analyses - primarily for surrogate material Phase 2 tests using cerium oxide sintered ceramic pellets are included. This spent fuel sabotage - aerosol test program is coordinated with the international Working Group for Sabotage Concerns of Transport and Storage Casks, WGSTSC, and supported by both the U.S. Department of Energy and Nuclear Regulatory Commission.

  3. Burnup determination and age dating of spent nuclear fuel using noble gas isotopic analysis

    SciTech Connect

    Charlton, W.S.; Perry, R.T.; Parish, T.A.; Hemberger, P.H.

    1999-07-01

    During the chopping and dissolving phases of reprocessing, gases (such as tritium, krypton, xenon, iodine, carbon dioxide, nitrogen oxide, and steam) are released. These gases are traditionally transferred to a gas-treatment system for treatment, release, and/or recycle. Because of their chemically inert nature, the xenon and krypton noble gases are generally released directly into the loser atmosphere through the facility's stack. These gases (being fission products) contain information about the fuel being reprocessed and may prove a valuable monitor of reprocessing activities. Two properties of the fuel that may prove valuable from a safeguards standpoint are the fuel burnup and the fuel age (or time since discharge from the reactor). Both can be used to aid in confirming declared activities, and the burnup is generally indicative of the usability of the fuel for fabricating nuclear explosives. A study has been ongoing at Los Alamos National Laboratory to develop a methodology to determine spent-fuel parameters from measured xenon and/or krypton isotopic ratios on-stack at reprocessing facilities. This study has resulted in the generation of the NOVA data analysis code, which links to a comprehensive database of reactor physics parameters (calculated using the Monteburns 3.01 code system). NOVA has been satisfactorily tested for burnup determination of weapons-grade fuel from a US production reactor. Less effort has been spent quantifying NOVA's ability to predict burnup and fuel age for power reactor fuel. The authors describe the results predicted by NOVA for xenon and krypton isotopic ratios measured after the dissolution of spent-fuel samples from the Borssele reactor. The Borssele reactor is a 450-MW(electric) pressurized water reactor (PWR) consisting of 15 x 15 KWU assemblies. The spent-fuel samples analyzed were single fuel rods removed from one assembly and dissolved at the La Hague reprocessing facility. The assembly average burnup was estimated at 32

  4. Comparative analysis of LWR and FBR spent fuels for nuclear forensics evaluation

    SciTech Connect

    Permana, Sidik; Suzuki, Mitsutoshi; Su'ud, Zaki

    2012-06-06

    Some interesting issues are attributed to nuclide compositions of spent fuels from thermal reactors as well as fast reactors such as a potential to reuse as recycled fuel, and a possible capability to be manage as a fuel for destructive devices. In addition, analysis on nuclear forensics which is related to spent fuel compositions becomes one of the interesting topics to evaluate the origin and the composition of spent fuels from the spent fuel foot-prints. Spent fuel compositions of different fuel types give some typical spent fuel foot prints and can be estimated the origin of source of those spent fuel compositions. Some technics or methods have been developing based on some science and technological capability including experimental and modeling or theoretical aspects of analyses. Some foot-print of nuclear forensics will identify the typical information of spent fuel compositions such as enrichment information, burnup or irradiation time, reactor types as well as the cooling time which is related to the age of spent fuels. This paper intends to evaluate the typical spent fuel compositions of light water (LWR) and fast breeder reactors (FBR) from the view point of some foot prints of nuclear forensics. An established depletion code of ORIGEN is adopted to analyze LWR spent fuel (SF) for several burnup constants and decay times. For analyzing some spent fuel compositions of FBR, some coupling codes such as SLAROM code, JOINT and CITATION codes including JFS-3-J-3.2R as nuclear data library have been adopted. Enriched U-235 fuel composition of oxide type is used for fresh fuel of LWR and a mixed oxide fuel (MOX) for FBR fresh fuel. Those MOX fuels of FBR come from the spent fuels of LWR. Some typical spent fuels from both LWR and FBR will be compared to distinguish some typical foot-prints of SF based on nuclear forensic analysis.

  5. Comparative analysis of LWR and FBR spent fuels for nuclear forensics evaluation

    NASA Astrophysics Data System (ADS)

    Permana, Sidik; Suzuki, Mitsutoshi; Su'ud, Zaki

    2012-06-01

    Some interesting issues are attributed to nuclide compositions of spent fuels from thermal reactors as well as fast reactors such as a potential to reuse as recycled fuel, and a possible capability to be manage as a fuel for destructive devices. In addition, analysis on nuclear forensics which is related to spent fuel compositions becomes one of the interesting topics to evaluate the origin and the composition of spent fuels from the spent fuel foot-prints. Spent fuel compositions of different fuel types give some typical spent fuel foot prints and can be estimated the origin of source of those spent fuel compositions. Some technics or methods have been developing based on some science and technological capability including experimental and modeling or theoretical aspects of analyses. Some foot-print of nuclear forensics will identify the typical information of spent fuel compositions such as enrichment information, burnup or irradiation time, reactor types as well as the cooling time which is related to the age of spent fuels. This paper intends to evaluate the typical spent fuel compositions of light water (LWR) and fast breeder reactors (FBR) from the view point of some foot prints of nuclear forensics. An established depletion code of ORIGEN is adopted to analyze LWR spent fuel (SF) for several burnup constants and decay times. For analyzing some spent fuel compositions of FBR, some coupling codes such as SLAROM code, JOINT and CITATION codes including JFS-3-J-3.2R as nuclear data library have been adopted. Enriched U-235 fuel composition of oxide type is used for fresh fuel of LWR and a mixed oxide fuel (MOX) for FBR fresh fuel. Those MOX fuels of FBR come from the spent fuels of LWR. Some typical spent fuels from both LWR and FBR will be compared to distinguish some typical foot-prints of SF based on nuclear forensic analysis.

  6. Dose reduction improvements in storage basins of spent nuclear fuel

    SciTech Connect

    Huang, Fan-Hsiung F.

    1997-08-13

    Spent nuclear fuel in storage basins at the Hanford Site has corroded and contaminated basin water, which has leaked into the soil; the fuel also had deposited a layer of radioactive sludge on basin floors. The SNF is to be removed from the basins to protect the nearby Columbia River. Because the radiation level is high, measures have been taken to reduce the background dose rate to as low as reasonably achievable (ALARA) to prevent radiation doses from becoming the limiting factor for removal of the SW in the basins to long-term dry storage. All activities of the SNF Project require application of ALARA principles for the workers. On the basis of these principles dose reduction improvements have been made by first identifying radiological sources. Principal radiological sources in the basin are basin walls, basin water, recirculation piping and equipment. Dose reduction activities focus on cleaning and coating basin walls to permit raising the water level, hydrolasing piping, and placing lead plates. In addition, the transfer bay floor will be refinished to make decontamination easier and reduce worker exposures in the radiation field. The background dose rates in the basin will be estimated before each task commences and after it is completed; these dose reduction data will provide the basis for cost benefit analysis.

  7. Adsorption of spent fuel storage pool contaminants into metal surfaces

    SciTech Connect

    Reaves, K.; Kunze, J.; Lu, Kang ); Bennett, P.C. )

    1990-01-01

    Shipping casks, after being submerged in spent fuel pools for the purpose of loading or unloading fuel, resist complete removal of the adsorbed contamination. To systematically study the mechanisms involved, 122 metal surface samples were immersed in the spent fuel storage pool of the Callaway Power Plant for periods of 7 to 30 days. After being removed from the pool, all samples were washed and wiped (with cloth) using demineralized water. They were then gamma counted for absolute activity, by using Eu-152 as an energy efficiency calibrator, applied uniformly to unexposed sample surfaces. Swipes were taken after each of 3 days of such environmental conditioning. Following this conditioning, selected samples were again counted to determine absolute contamination remaining on the samples. 2 refs., 1 tab.

  8. Heat Transfer Modeling of Dry Spent Nuclear Fuel Storage Facilities

    SciTech Connect

    Lee, S.Y.

    1999-01-13

    The present work was undertaken to provide heat transfer model that accurately predicts the thermal performance of dry spent nuclear fuel storage facilities. One of the storage configurations being considered for DOE Aluminum-clad Spent Nuclear Fuel (Al-SNF), such as the Material and Testing Reactor (MTR) fuel, is in a dry storage facility. To support design studies of storage options a computational and experimental program has been conducted at the Savannah River Site (SRS). The main objective is to develop heat transfer models including natural convection effects internal to an interim dry storage canister and to geological codisposal Waste Package (WP). Calculated temperatures will be used to demonstrate engineering viability of a dry storage option in enclosed interim storage and geological repository WP and to assess the chemical and physical behaviors of the Al-SNF in the dry storage facilities. The current paper describes the modeling approaches and presents the computational results along with the experimental data.

  9. Technical strategy for the management of INEEL spent nuclear fuel

    SciTech Connect

    1997-03-01

    This report presents evaluations, findings, and recommendations of the Idaho National Engineering and Environmental Laboratory (INEEL) Spent Nuclear Fuel Task Team. The technical strategy developed by the Task Team includes stabilization, near term storage, packaging, transport, and ultimate disposal. Key issues identified and discussed include waste characterization, criticality, packaging, waste form performance, and special fuels. Current plans focus on onsite needs, and include three central elements: (1) resolution of near-term vulnerabilities, (2) consolidation of storage locations, and (3) achieving dry storage in transportable packages. In addition to the Task Team report, appendices contain information on the INEEL spent fuel inventory; regulatory decisions and agreements; and analyses of criticality, packaging, storage, transportation, and system performance of a geological repository. 16 refs., 6 figs., 4 tabs.

  10. Storage of LWR spent fuel in air. Volume 3, Results from exposure of spent fuel to fluorine-contaminated air

    SciTech Connect

    Cunningham, M.E.; Thomas, L.E.

    1995-06-01

    The Behavior of Spent Fuel in Storage (BSFS) Project has conducted research to develop data on spent nuclear fuel (irradiated U0{sub 2}) that could be used to support design, licensing, and operation of dry storage installations. Test Series B conducted by the BSFS Project was designed as a long-term study of the oxidation of spent fuel exposed to air. It was discovered after the exposures were completed in September 1990 that the test specimens had been exposed to an atmosphere of bottled air contaminated with an unknown quantity of fluorine. This exposure resulted in the test specimens reacting with both the oxygen and the fluorine in the oven atmospheres. The apparent source of the fluorine was gamma radiation-induced chemical decomposition of the fluoro-elastomer gaskets used to seal the oven doors. This chemical decomposition apparently released hydrofluoric acid (HF) vapor into the oven atmospheres. Because the Test Series B specimens were exposed to a fluorine-contaminated oven atmosphere and reacted with the fluorine, it is recommended that the Test Series B data not be used to develop time-temperature limits for exposure of spent nuclear fuel to air. This report has been prepared to document Test Series B and present the collected data and observations.

  11. 78 FR 3853 - Retrievability, Cladding Integrity and Safe Handling of Spent Fuel at an Independent Spent Fuel...

    Federal Register 2010, 2011, 2012, 2013, 2014

    2013-01-17

    .... ACTION: Request for comments for potential rulemaking. SUMMARY: The regulations for packaging and... potential policy issues and requirements related to retrievability, cladding integrity, and safe handling of spent fuel as the lead issue for evaluating compatibility of storage and transportation regulations....

  12. Freshly induced short-lived gamma-ray activity as a measure of fission rates in lightly re-irradiated spent fuel

    NASA Astrophysics Data System (ADS)

    Kröhnert, H.; Perret, G.; Murphy, M. F.; Chawla, R.

    2010-12-01

    A new measurement technique has been developed to determine fission rates in burnt fuel, following re-irradiation in a zero-power research reactor. The development has been made in the frame of the LIFE@PROTEUS program at the Paul Scherrer Institute, which aims at characterizing the interfaces between fresh and highly burnt fuel assemblies in modern LWRs. To discriminate against the high intrinsic gamma-ray activity of the burnt fuel, the proposed measurement technique uses high-energy gamma-rays, above 2000 keV, emitted by short-lived fission products freshly produced in the fuel. To demonstrate the feasibility of this technique, a fresh UO 2 sample and a 36 GWd/t burnt UO 2 sample were irradiated in the PROTEUS reactor and their gamma-ray activities were recorded directly after irradiation. For both fresh and the burnt fuel samples, relative fission rates were derived for different core positions, based on the short-lived 142La (2542 keV), 89Rb (2570 keV), 138Cs (2640 keV) and 95Y (3576 keV) gamma-ray lines. Uncertainties on the inter-position fission rate ratios were mainly due to the uncertainties on the net-area of the gamma-ray peaks and were about 1-3% for the fresh sample, and 3-6% for the burnt one. Thus, for the first time, it has been shown that the short-lived gamma-ray activity, induced in burnt fuel by irradiation in a zero-power reactor, can be used as a quantitative measure of the fission rate. For both fresh and burnt fuel, the measured results agreed, within the uncertainties, with Monte Carlo (MCNPX) predictions.

  13. Spent fuel dissolution rates as a function of burnup and water chemistry

    SciTech Connect

    Gray, W.J.

    1998-06-01

    To help provide a source term for performance-assessment calculations, dissolution studies on light-water-reactor (LWR) spent fuel have been conducted over the past few years at Pacific Northwest National Laboratory in support of the Yucca Mountain Site Characterization Project. This report describes that work for fiscal years 1996 through mid-1998 and includes summaries of some results from previous years for completeness. The following conclusions were based on the results of various flowthrough dissolution rate tests and on tests designed to measure the inventories of {sup 129}I located within the fuel/cladding gap region of different spent fuels: (1) Spent fuels with burnups in the range 30 to 50 MWd/kgM all dissolved at about the same rate over the conditions tested. To help determine whether the lack of burnup dependence extends to higher and lower values, tests are in progress or planned for spent fuels with burnups of 13 and {approximately} 65 MWd/kgM. (2) Oxidation of spent fuel up to the U{sub 4}O{sub 9+x} stage does not have a large effect on intrinsic dissolution rates. However, this degree of oxidation could increase the dissolution rates of relatively intact fuel by opening the grain boundaries, thereby increasing the effective surface area that is available for contact by water. From a disposal viewpoint, this is a potentially more important consideration than the effect on intrinsic rates. (3) The gap inventories of {sup 129}I were found to be smaller than the fission gas release (FGR) for the same fuel rod with the exception of the rod with the highest FGR. Several additional fuels would have to be tested to determine whether a generalized relationship exists between FGR and {sup 129}I gap inventory for US LWR fuels.

  14. Radiochemical analyses of several spent fuel Approved Testing Materials

    SciTech Connect

    Guenther, R.J.; Blahnik, D.E.; Wildung, N.J.

    1994-09-01

    Radiochemical characterization data are described for UO{sub 2} and UO{sub 2} plus 3 wt% Gd{sub 2}O{sub 3} commercial spent nuclear fuel taken from a series of Approved Testing Materials (ATMs). These full-length nuclear fuel rods include MLA091 of ATM-103, MKP070 of ATM-104, NBD095 and NBD131 of ATM-106, and ADN0206 of ATM-108. ATMs 103, 104, and 106 were all irradiated in the Calvert Cliffs Nuclear Power Plant (Reactor No.1), a pressurized-water reactor that used fuel fabricated by Combustion Engineering. ATM-108 was part of the same fuel bundle designed as ATM-105 and came from boiling-water reactor fuel fabricated by General Electric and irradiated in the Cooper Nuclear Power Plant. Rod average burnups and expected fission gas releases ranged from 2,400 to 3,700 GJ/kgM. (25 to 40 Mwd/kgM) and from less than 1% to greater than 10%, respectively, depending on the specific ATM. The radiochemical analyses included uranium and plutonium isotopes in the fuel, selected fission products in the fuel, fuel burnup, cesium and iodine on the inner surfaces of the cladding, {sup 14}C in the fuel and cladding, and analyses of the gases released to the rod plenum. Supporting examinations such as fuel rod design and material descriptions, power histories, and gamma scans used for sectioning diagrams are also included. These ATMs were examined as part of the Materials Characterization Center Program conducted at Pacific Northwest Laboratory provide a source of well-characterized spent fuel for testing in support of the US Department of Energy Office of Civilian Radioactive Waste Management Program.

  15. Extending dry storage of spent LWR fuel for 100 years.

    SciTech Connect

    Einziger, R. E.

    1998-12-16

    Because of delays in closing the back end of the fuel cycle in the U.S., there is a need to extend dry inert storage of spent fuel beyond its originally anticipated 20-year duration. Many of the methodologies developed to support initial licensing for 20-year storage should be able to support the longer storage periods envisioned. This paper evaluates the applicability of existing information and methodologies to support dry storage up to 100 years. The thrust of the analysis is the potential behavior of the spent fuel. In the USA, the criteria for dry storage of LWR spent fuel are delineated in 10 CFR 72 [1]. The criteria fall into four general categories: maintain subcriticality, prevent the release of radioactive material above acceptable limits, ensure that radiation rates and doses do not exceed acceptable levels, and maintain retrievability of the stored radioactive material. These criteria need to be considered for normal, off-normal, and postulated accident conditions. The initial safety analysis report submitted for licensing evaluated the fuel's ability to meet the requirements for 20 years. It is not the intent to repeat these calculations, but to look at expected behavior over the additional 80 years, during which the temperatures and radiation fields are lower. During the first 20 years, the properties of the components may change because of elevated temperatures, presence of moisture, effects of radiation, etc. During normal storage in an inert atmosphere, there is potential for the cladding mechanical properties to change due to annealing or interaction with cask materials. The emissivity of the cladding could also change due to storage conditions. If there is air leakage into the cask, additional degradation could occur through oxidation in breached rods, which could lead to additional fission gas release and enlargement of cladding breaches. Air in-leakage could also affect cover gas conductivity, cladding oxidation, emissivity changes, and

  16. 10 CFR 72.214 - List of approved spent fuel storage casks.

    Code of Federal Regulations, 2010 CFR

    2010-01-01

    ... STORAGE OF SPENT NUCLEAR FUEL, HIGH-LEVEL RADIOACTIVE WASTE, AND REACTOR-RELATED GREATER THAN CLASS C WASTE General License for Storage of Spent Fuel at Power Reactor Sites § 72.214 List of approved...

  17. Spent reactor fuel benchmark composition data for code validation

    SciTech Connect

    Bierman, S.R.

    1991-09-01

    To establish criticality safety margins utilizing burnup credit in the storage and transport of spent reactor fuels requires a knowledge of the uncertainty in the calculated fuel composition used in making the reactivity assessment. To provide data for validating such calculated burnup fuel compositions, radiochemical assays are being obtained as part of the United States Department of Energy From-Reactor Cask Development Program. Destructive assay data are being obtained from representative reactor fuels having experienced irradiation exposures up to about 55 GWD/MTM. Assay results and associated operating histories on the initial three samples analyzed in this effort are presented. The three samples were taken from different axial regions of the same fuel rod and represent radiation exposures of about 27, 37, and 44 GWD/MTM. The data are presented in a benchmark type format to facilitate identification/referencing and computer code input.

  18. Safeguards techniques in a pilot conditioning plant for spent fuel

    SciTech Connect

    Leitner, E.; Rudolf, K.; Weh, R. )

    1991-01-01

    The pilot conditioning plant at Gorleben, Germany, is designed as a multi-purpose plant. Its primary task is the conditioning of spent fuel assemblies into a form suitable for final disposal. As a pilot plant, it allows furthermore for the development and testing of various conditioning techniques. In terms of international safeguards, the pilot conditioning plant is basically considered an item facility. Entire fuel assemblies enter the plant in transport casks, whereas bins filled with fuel rods or canisters containing cut fuel rods leave the facility in final disposal packages (e.g. POLLUX). Each POLLUX final disposal package content is uniquely correlated to a definite number of fuel assemblies which have entered the conditioning process. For this type of facility, containment/surveillance (C/S) should take over the major role in nuclear material safeguards. This paper discusses the safeguards at the Gorleben plant.

  19. Quantifying the passive gamma signal from spent nuclear fuel in support of determining the plutonium content in spent nuclear fuel with nondestructive assay

    SciTech Connect

    Fensin, Michael L; Tobin, Steven J; Menlove, Howard O; Swinhoe, Martyn T

    2009-01-01

    The objective of safeguarding nuclear material is to deter diversions of significant quantities of nuclear materials by timely monitoring and detection. There are a variety of motivations for quantifying plutonium in spent fuel (SF), by means of nondestructive assay (NDA), in order to meet this goal. These motivations include the following: strengthening the capabilities of the International Atomic Energy Agencies ability to safeguard nuclear facilities, shipper/receiver difference, input accountability at reprocessing facilities and burnup credit at repositories. Many NDA techniques exist for measuring signatures from SF; however, no single NDA technique can, in isolation, quantify elemental plutonium in SF. A study has been undertaken to determine the best integrated combination of 13 NDA techniques for characterizing Pu mass in spent fuel. This paper focuses on the development of a passive gamma measurement system in support the spent fuel assay system. Gamma ray detection for fresh nuclear fuel focuses on gamma ray emissions that directly coincide with the actinides of interest to the assay. For example, the 186-keV gamma ray is generally used for {sup 235}U assay and the 384-keV complex is generally used for assaying plutonium. In spent nuclear fuel, these signatures cannot be detected as the Compton continuum created from the fission products dominates the signal in this energy range. For SF, the measured gamma signatures from key fission products ({sup 134}Cs, {sup 137}Cs, {sup 154}Eu) are used to ascertain burnup, cooling time, and fissile content information. In this paper the Monte Carlo modeling set-up for a passive gamma spent fuel assay system will be described. The set-up of the system includes a germanium detector and an ion chamber and will be used to gain passive gamma information that will be integrated into a system for determining Pu in SF. The passive gamma signal will be determined from a library of {approx} 100 assemblies that have been

  20. Interim Storage of Hanford Spent Fuel & Associated Sludge

    SciTech Connect

    MAKENAS, B.J.

    2002-07-01

    The Hanford site is currently dealing with a number of types of Spent Nuclear Fuel. The route to interim dry storage for the various fuel types branches along two different paths. Fuel types such as metallic N reactor fuel and Shippingport Core 2 Blanket assemblies are being placed in approximately 4 m long canisters which are then stored in tubes below grade in a new canister storage building. Other fuels such as TRIGA{trademark} and Light Water Reactor fuel will be relocated and stored in stand-alone casks on a concrete pad. Varying degrees of sophistication are being applied with respect to the drying and/or evacuation of the fuel interim storage canisters depending on the reactivity of the fuel, the degree of damaged fuel and the previous storage environment. The characterization of sludge from the Hanford K Basins is nearly complete and canisters are being designed to store the sludge (including uranium particles from fuel element cleaning) on an interim basis.

  1. U. S. spent-fuel disposal strategies and International safeguards

    SciTech Connect

    Pillay, K.K.; Picard, R.R.; Hafer, J.F. )

    1993-08-01

    Domestic safeguards for fissile nuclear materials are universal, and a variety of international safeguards regimes are applicable, in most member states of the International Atomic Energy Agency (IAEA), to declared nuclear facilities dedicated to peaceful missions. The U.S. strategy to dispose of all spent nuclear fuels (SNFs) and high-level wastes (HLWs) in engineered geologic repositories has a sometimes-overlooked consequence, namely, the need to maintain domestic and international safeguards in perpetuity. The Office of Civilian Radioactive Waste Management of the U.S. Department of Energy (DOE), which has the responsibility to accept and store the spent fuels in the long term either in surface facilities or in engineered geologic repositories, has yet to include safeguards issues in their mission plan.'' There are several stages in the nuclear fuel cycle where materials usable in weapons are available for diversion. This discussion, however, is limited to the potential diversion of spent fuels for clandestine plutonium recovery. The concepts proposed here highlight safeguards elements necessary for a pragmatic safeguards system for SNF from nuclear power generation. The efforts required to initiate and maintain a verifiable international safeguards regime are examined in the context of a typical storage facility in the United States.

  2. Electrometallurgical treatment of oxide spent fuel - engineering-scale development.

    SciTech Connect

    Karell, E. J.

    1998-04-22

    Argonne National Laboratory (ANL) has developed the electrometallurgical treatment process for conditioning various Department of Energy (DOE) spent fuel types for long-term storage or disposal. This process uses electrorefining to separate the constituents of spent fuel into three product streams: metallic uranium, a metal waste form containing the cladding and noble metal fission products, and a ceramic waste form containing the transuranics, and rare earth, alkali, and alkaline earth fission products. While metallic fuels can be directly introduced into the electrorefiner, the actinide components of oxide fuels must first be reduced to the metallic form. The Chemical Technology Division of AFT has developed a process to reduce the actinide oxides that uses lithium at 650 C in the presence of molten LiCl, yielding the actinide metals and Li{sub 2}O. A significant amount of work has already been accomplished to investigate the basic chemistry of the lithium reduction process and to demonstrate its applicability to the treatment of light-water reactor- (LWR-) type spent fuel. The success of this work has led to conceptual plans to construct a pilot-scale oxide reduction facility at ANL's Idaho site. In support of the design effort, a series of laboratory- and engineering-scale experiments is being conducted using simulated fuel. These experiments have focused on the engineering issues associated with scaling-up the process and proving compatibility between the reduction and electrorefining steps. Specific areas of investigation included reduction reaction kinetics, evaluation of various fuel basket designs, and issues related to electrorefining the reduced product. This paper summarizes the results of these experiments and outlines plans for future work.

  3. Report on interim storage of spent nuclear fuel. Midwestern high-level radioactive waste transportation project

    SciTech Connect

    Not Available

    1993-04-01

    The report on interim storage of spent nuclear fuel discusses the technical, regulatory, and economic aspects of spent-fuel storage at nuclear reactors. The report is intended to provide legislators state officials and citizens in the Midwest with information on spent-fuel inventories, current and projected additional storage requirements, licensing, storage technologies, and actions taken by various utilities in the Midwest to augment their capacity to store spent nuclear fuel on site.

  4. Simulation of differential die-away instrument’s response to asymmetrically burned spent nuclear fuel

    SciTech Connect

    Martinik, Tomas; Henzl, Vladimir; Grape, Sophie; Svard, Staffan Jacobsson; Jansson, Peter; Swinhoe, Martyn T.; Tobin, Stephen J.

    2015-03-04

    Here, previous simulation studies of Differential Die–Away (DDA) instrument’s response to active interrogation of spent nuclear fuel from a pressurized water reactor (PWR) yielded promising results in terms of its capability to accurately measure or estimate basic spent fuel assembly (SFA) characteristics, such as multiplication, initial enrichment (IE) and burn-up (BU) as well as the total plutonium content. These studies were however performed only for a subset of idealized SFAs with a symmetric BU with respect to its longitudinal axis. Therefore, to complement the previous results, additional simulations have been performed of the DDA instrument’s response to interrogation of asymmetrically burned spent nuclear fuel in order to determine whether detailed assay of SFAs from all 4 sides will be necessary in real life applications or whether a cost and time saving single sided assay could be used to achieve results of similar quality as previously reported in case of symmetrically burned SFAs.

  5. 78 FR 32077 - List of Approved Spent Fuel Storage Casks: MAGNASTOR® System

    Federal Register 2010, 2011, 2012, 2013, 2014

    2013-05-29

    ... COMMISSION 10 CFR Part 72 RIN 3150-AJ22 List of Approved Spent Fuel Storage Casks: MAGNASTOR System AGENCY... Commission (NRC) is withdrawing a direct final rule that would have revised its spent fuel storage... ``List of Approved Spent Fuel Storage Casks.'' The NRC is taking this action because it has received...

  6. 78 FR 59073 - Pacific Gas and Electric Company; Humboldt Bay Independent Spent Fuel Storage Installation...

    Federal Register 2010, 2011, 2012, 2013, 2014

    2013-09-25

    ... PG&E to receive, possess, store, and transfer spent nuclear fuel and associated radioactive materials..., and transfer spent nuclear fuel and associated radioactive materials resulting from the operation of... storage of spent fuel and associated radioactive materials at the HB ISFSI. Pursuant to 10 CFR 72.46(d...

  7. 10 CFR 72.214 - List of approved spent fuel storage casks.

    Code of Federal Regulations, 2011 CFR

    2011-01-01

    ... STORAGE OF SPENT NUCLEAR FUEL, HIGH-LEVEL RADIOACTIVE WASTE, AND REACTOR-RELATED GREATER THAN CLASS C WASTE General License for Storage of Spent Fuel at Power Reactor Sites § 72.214 List of approved spent... Standardized NUHOMS® Horizontal Modular Storage System for Irradiated Nuclear Fuel. Docket Number: 72-1004...

  8. 77 FR 24585 - List of Approved Spent Fuel Storage Casks: HI-STORM 100, Revision 8

    Federal Register 2010, 2011, 2012, 2013, 2014

    2012-04-25

    ... 3150-AJ05 List of Approved Spent Fuel Storage Casks: HI-STORM 100, Revision 8 AGENCY: Nuclear... amends the NRC's spent fuel storage regulations by revising the Holtec International HI-STORM 100 System... International HI-STORM 100 System listing within the ``List of Approved Spent Fuel Storage Casks'' to include...

  9. 77 FR 7211 - Pacific Gas and Electric Company, Diablo Canyon Independent Spent Fuel Storage Installation...

    Federal Register 2010, 2011, 2012, 2013, 2014

    2012-02-10

    ... COMMISSION Pacific Gas and Electric Company, Diablo Canyon Independent Spent Fuel Storage Installation... Pacific Gas and Electric Company (PG&E) for the Diablo Canyon (DC) Independent Spent Fuel Storage... for the MPC Helium backfill pressure range. 5. TS 3.1.2, ``Spent Fuel Storage Cask (SFSC) Heat Removal...

  10. 77 FR 60482 - Yankee Atomic Electric Company; Yankee Rowe Independent Spent Fuel Storage Installation, Staff...

    Federal Register 2010, 2011, 2012, 2013, 2014

    2012-10-03

    ... COMMISSION Yankee Atomic Electric Company; Yankee Rowe Independent Spent Fuel Storage Installation, Staff Evaluation; Exemption 1.0 Background Yankee Atomic Electric Company (YAEC, the licensee) is the holder of... for the storage of spent fuel in an Independent Spent Fuel Storage Installation (ISFSI) to...

  11. Response of spent LWR fuel to extreme environments

    SciTech Connect

    Sandoval, R.P.; Burian, R.J.; Kok, K.D.; DiSalvo, R.; Balmert, M.E.; Freeman-Kelly, R.; Fentiman, A.W.

    1986-01-01

    The research reported in this paper addresses the radiological source term which could arise when irradiated fuel in transport from a commercial light water reactor is exposed to the extreme environments postulated for some transportation accidents, specifically those involving a fire. The release of spent fuel radionuclides to the environment requires a breach of both the cask and the fuel rod cladding. Past research has given significant emphasis to evaluating the response of the shipping cask to mechanical and/or thermal loads from hypothetical accidents. Less consideration has been given to evaluating the response of the fuel rods to these environments. In this paper, the response of the fuel rods to an extreme thermal event was experimentally evaluated and the quantity of solid fuel material that could be released from the fuel rods to the cask cavity was estimated. Briefly, the objectives of this study were as follows: (1) Identify those conditions within a transportation cask which might produce fuel-rod cladding failure, emphasizing conditions associated with fires, and (2) Determine by experiment and analysis the nature of the source term so produced. The release of radionuclides from coolant or deposits on the outer surfaces of the fuel assembly was not addressed in this study. 6 figs., 2 figs.

  12. Re-examining the Dissolution of Spent Fuel: A Comparison of Different Methods for Calculating Rates

    SciTech Connect

    Hanson, B D; Stout, R B

    2004-04-09

    Dissolution rates for spent fuel have typically been reported in terms of a rate normalized to the surface area of the specimen. Recent evidence has shown that neither the geometric surface area nor that measured with BET accurately predicts the effective surface area of spent fuel. Dissolution rates calculated from results obtained by flowthrough tests were reexamined comparing the cumulative releases and surface area normalized rates. While initial surface area is important for comparison of different rates, it appears that normalizing to the surface area introduces unnecessary uncertainty compared to using cumulative or fractional release rates. Discrepancies in past data analyses are mitigated using this alternative method.

  13. Spent fuel sabotage aerosol test program :FY 2005-06 testing and aerosol data summary.

    SciTech Connect

    Gregson, Michael Warren; Brockmann, John E.; Nolte, O. (Fraunhofer institut fur toxikologie und experimentelle Medizin, Germany); Loiseau, O. (Institut de radioprotection et de Surete Nucleaire, France); Koch, W. (Fraunhofer institut fur toxikologie und experimentelle Medizin, Germany); Molecke, Martin Alan; Autrusson, Bruno (Institut de radioprotection et de Surete Nucleaire, France); Pretzsch, Gunter Guido (Gesellschaft fur anlagen- und Reaktorsicherheit, Germany); Billone, M. C. (Argonne National Laboratory, USA); Lucero, Daniel A.; Burtseva, T.; Brucher, W (Gesellschaft fur anlagen- und Reaktorsicherheit, Germany); Steyskal, Michele D.

    2006-10-01

    This multinational, multi-phase spent fuel sabotage test program is quantifying the aerosol particles produced when the products of a high energy density device (HEDD) interact with and explosively particulate test rodlets that contain pellets of either surrogate materials or actual spent fuel. This program has been underway for several years. This program provides source-term data that are relevant to some sabotage scenarios in relation to spent fuel transport and storage casks, and associated risk assessments. This document focuses on an updated description of the test program and test components for all work and plans made, or revised, primarily during FY 2005 and about the first two-thirds of FY 2006. It also serves as a program status report as of the end of May 2006. We provide details on the significant findings on aerosol results and observations from the recently completed Phase 2 surrogate material tests using cerium oxide ceramic pellets in test rodlets plus non-radioactive fission product dopants. Results include: respirable fractions produced; amounts, nuclide content, and produced particle size distributions and morphology; status on determination of the spent fuel ratio, SFR (the ratio of respirable particles from real spent fuel/respirables from surrogate spent fuel, measured under closely matched test conditions, in a contained test chamber); and, measurements of enhanced volatile fission product species sorption onto respirable particles. We discuss progress and results for the first three, recently performed Phase 3 tests using depleted uranium oxide, DUO{sub 2}, test rodlets. We will also review the status of preparations and the final Phase 4 tests in this program, using short rodlets containing actual spent fuel from U.S. PWR reactors, with both high- and lower-burnup fuel. These data plus testing results and design are tailored to support and guide, follow-on computer modeling of aerosol dispersal hazards and radiological consequence

  14. EURATOM safeguards efforts in the development of spent fuel verification methods by non-destructive assay

    SciTech Connect

    Matloch, L.; Vaccaro, S.; Couland, M.; De Baere, P.; Schwalbach, P.

    2015-07-01

    The back end of the nuclear fuel cycle continues to develop. The European Commission, particularly the Nuclear Safeguards Directorate of the Directorate General for Energy, implements Euratom safeguards and needs to adapt to this situation. The verification methods for spent nuclear fuel, which EURATOM inspectors can use, require continuous improvement. Whereas the Euratom on-site laboratories provide accurate verification results for fuel undergoing reprocessing, the situation is different for spent fuel which is destined for final storage. In particular, new needs arise from the increasing number of cask loadings for interim dry storage and the advanced plans for the construction of encapsulation plants and geological repositories. Various scenarios present verification challenges. In this context, EURATOM Safeguards, often in cooperation with other stakeholders, is committed to further improvement of NDA methods for spent fuel verification. In this effort EURATOM plays various roles, ranging from definition of inspection needs to direct participation in development of measurement systems, including support of research in the framework of international agreements and via the EC Support Program to the IAEA. This paper presents recent progress in selected NDA methods. These methods have been conceived to satisfy different spent fuel verification needs, ranging from attribute testing to pin-level partial defect verification. (authors)

  15. Molten tin reprocessing of spent nuclear fuel elements

    DOEpatents

    Heckman, Richard A.

    1983-01-01

    A method and apparatus for reprocessing spent nuclear fuel is described. Within a containment vessel, a solid plug of tin and nitride precipitates supports a circulating bath of liquid tin therein. Spent nuclear fuel is immersed in the liquid tin under an atmosphere of nitrogen, resulting in the formation of nitride precipitates. The layer of liquid tin and nitride precipitates which interfaces the plug is solidified and integrated with the plug. Part of the plug is melted, removing nitride precipitates from the containment vessel, while a portion of the plug remains solidified to support the liquid tin and nitride precipitates remaining in the containment vessel. The process is practiced numerous times until substantially all of the precipitated nitrides are removed from the containment vessel.

  16. Prototype spent-fuel canister design, analysis, and test

    SciTech Connect

    Leisher, W.B.; Eakes, R.G.; Duffey, T.A.

    1982-03-01

    Sandia National Laboratories was asked by the US Energy Research and Development Administration (now US Department of Energy) to design the spent fuel shipping cask system for the Clinch River Breeder Reactor Plant (CRBRP). As a part of this task, a canister which holds liquid sodium and the spent fuel assembly was designed, analyzed, and tested. The canister body survived the regulatory Type-B 9.1-m (30-ft) drop test with no apparent leakage. However, the commercially available metal seal used in this design leaked after the tests. This report describes the design approach, analysis, and prototype canister testing. Recommended work for completing the design, when funding is available, is included.

  17. ALARA assessment of spent fuel and nuclear waste transportation systems

    SciTech Connect

    Sutherland, S. H.

    1980-01-01

    The effects of ALARA (as low as reasonably achievable) on transportation system costs were evaluated for LWR spent fuel, high-level commercial and defense wastes, and remotely handled TRU waste. Three dose rate specifications were used: 10 mrem/h at 2m, 5 mrem/h, and 2 mrem/h. The evaluation was done for wastes and LWR spent fuel 1, 3, 5, and 10 years old. Gamma shield materials were depleted uranium, lead, and steel; the neutron shield material was water. Results for a 7-element PWR cask show that uranium shielding is the lightest, and that the increased weight of the low dose rate casks results in 1 to 2 million dollars increase in lifetime transportation costs. 6 figures, 3 tables. (DLC)

  18. The Idaho Spent Fuel Project Update-January, 2003

    SciTech Connect

    Roberts, R.; Tulberg, D.; Carter, C.

    2003-02-25

    The Department of Energy awarded a privatized contract to Foster Wheeler Environmental Corporation in May 2000 for the design, licensing, construction and operation of a spent nuclear fuel repackaging and storage facility. The Foster Wheeler Environmental Team consists of Foster Wheeler Environmental Corp. (the primary contractor), Alstec, RWE-Nukem, RIO Technical Services, Winston and Strawn, and Utility Engineering. The Idaho Spent Fuel (ISF) facility is an integral part of the DOE-EM approach to accelerating SNF disposition at the Idaho National Engineering and Environmental Laboratory (INEEL). Construction of this facility is also important in helping DOE to meet the provisions of the Idaho Settlement Agreement. The ISF Facility is a substantial facility with heavy shielding walls in the repackaging and storage bays and state-of-the-art features required to meet the provisions of 10 CFR 72 requirements. The facility is designed for a 40-year life.

  19. Review of spent-fuel photon and neutron source spectra

    SciTech Connect

    Hermann, O.W.; Alexander, C.W.

    1986-01-01

    The calculations of spent-fuel photon and neutron spectra have been significantly improved over the past several years. Methods for performing these computations at ORNL have been implemented in the ORIGEN2 and ORIGEN-S codes and the SAS2 control module of the SCALE system. The codes use photon data for delayed gamma rays, x-rays, spontaneous fission gamma rays, (..cap alpha..,n) reaction gamma rays, bremsstrahlung and decay constants, taken mainly from the Evaluated Nuclear Data Structure File. The data for neutron source strengths and spectral distributions of spontaneous fission and (..cap alpha..,n) reactions were compiled from several different research projects. Brief discussions of the codes, the spectral data and the range of applicability are presented. Also, several examples of spent-fuel photon and neutron spectra are included. 29 refs.

  20. Spent fuel assembly hardware: Characterization and 10 CFR 61 classification for waste disposal: Volume 3, Calculated activity profiles of spent nuclear fuel assembly hardware for boiling water reactors

    SciTech Connect

    Short, S.M.; Luksic, A.T.; Schutz, M.E.

    1989-06-01

    Consolidation of spent fuel is under active consideration as the US Department of Energy plans to dispose of spent fuel as required by the Nuclear Waste Policy Act of 1982. During consolidation, the fuel pins are removed from an intact fuel assembly and repackaged into a more compact configuration. After repackaging, approximately 30 kg of residual spent fuel assembly hardware per assembly that is also radioactive and required disposal. Understanding the nature of this secondary waste stream is critical to designing a system that will properly handle, package, store, and dispose of the waste. This report presents a methodology for estimating the radionuclide inventory in irradiated spent fuel hardware. Ratios are developed that allow the use of ORIGEN2 computer code calculations to be applied to regions that are outside the fueled region. The ratios are based on the analysis of samples of irradiated hardware from spent fuel assemblies. The results of this research are presented in three volumes. In Volume 1, the development of scaling factors that can be used with ORIGEN2 calculations to estimate activation of spent fuel assembly hardware is documented. The results from laboratory analysis of irradiated spent-fuel hardware samples are also presented in Volume 1. In Volume 2 and 3, the calculated flux profiles of spent nuclear fuel assemblies are presented for pressurized water reactors and boiling water reactors, respectively. The results presented in Volumes 2 and 3 were used to develop the scaling factors documented in Volume 1.

  1. Spent fuel assembly hardware: Characterization and 10 CFR 61 classification for waste disposal: Volume 2, Calculated activity profiles of spent nuclear fuel assembly hardware for pressurized water reactors

    SciTech Connect

    Short, S.M.; Luksic, A.T.; Lotz, T.L.; Schutz, M.E.

    1989-06-01

    Consolidation of spent fuel is under active consideration as the US Department of Energy plans to dispose of spent fuel as required by the Nuclear Waste Policy Act of 1982. During consolidation, the fuel pins are removed from an intact fuel assembly and repackaged into a more compact configuration. After repackaging, approximately 30 kg of residual spent fuel assembly hardware per assembly remains that is also radioactive and requires disposal. Understanding the nature of this secondary waste stream is critical to designing a system that will properly handle, package, store, and dispose of the waste. This report present a methodology for estimating the radionuclide inventory in irradiated spent fuel hardware. Ratios are developed that allow the use of ORIGEN2 computer code calculations to be applied to regions that are outside the fueled region. The ratios are based on the analysis of samples of irradiated hardware from spent fuel assemblies. The results of this research are presented in three volumes. In Volume 1, the development of scaling factors that can be used with ORIGEN2 calculations to estimate activation of spent fuel assembly hardware is documented. The results from Laboratory analysis of irradiated spent-fuel hardware samples are also presented in Volume 1. In Volumes 2 and 3, the calculated flux profiles of spent nuclear fuel assemblies are presented for pressurized water reactors and boiling water reactors, respectively. The results presented in Volumes 2 and 3 were used to develop the scaling factors documented in Volume 1.

  2. Method For Processing Spent (Trn,Zr)N Fuel

    DOEpatents

    Miller, William E.; Richmann, Michael K.

    2004-07-27

    A new process for recycling spent nuclear fuels, in particular, mixed nitrides of transuranic elements and zirconium. The process consists of two electrorefiner cells in series configuration. A transuranic element such as plutonium is reduced at the cathode in the first cell, zirconium at the cathode in the second cell, and nitrogen-15 is released and captured for reuse to make transuranic and zirconium nitrides.

  3. Naval Spent Nuclear Fuel disposal Container System Description Document

    SciTech Connect

    N. E. Pettit

    2001-07-13

    The Naval Spent Nuclear Fuel Disposal Container System supports the confinement and isolation of waste within the Engineered Barrier System of the Monitored Geologic Repository (MGR). Disposal containers/waste packages are loaded and sealed in the surface waste handling facilities, transferred underground through the access drifts using a rail mounted transporter, and emplaced in emplacement drifts. The Naval Spent Nuclear Fuel Disposal Container System provides long term confinement of the naval spent nuclear fuel (SNF) placed within the disposal containers, and withstands the loading, transfer, emplacement, and retrieval operations. The Naval Spent Nuclear Fuel Disposal Container System provides containment of waste for a designated period of time and limits radionuclide release thereafter. The waste package maintains the waste in a designated configuration, withstands maximum credible handling and rockfall loads, limits the waste form temperature after emplacement, resists corrosion in the expected handling and repository environments, and provides containment of waste in the event of an accident. Each naval SNF disposal container will hold a single naval SNF canister. There will be approximately 300 naval SNF canisters, composed of long and short canisters. The disposal container will include outer and inner cylinder walls and lids. An exterior label will provide a means by which to identify a disposal container and its contents. Different materials will be selected for the waste package inner and outer cylinders. The two metal cylinders, in combination with the Emplacement Drift System, drip shield, and the natural barrier will support the design philosophy of defense-in-depth. The use of materials with different properties prevents a single mode failure from breaching the waste package. The inner cylinder and inner cylinder lids will be constructed of stainless steel while the outer cylinder and outer cylinder lids will be made of high-nickel alloy.

  4. Spent Nuclear Fuel Project Canister Storage Building Functions and Requirements

    SciTech Connect

    KLEM, M.J.

    2000-10-18

    In 1998, a major change in the technical strategy for managing Multi Canister Overpacks (MCO) while stored within the Canister Storage Building (CSB) occurred. The technical strategy is documented in Baseline Change Request (BCR) No. SNF-98-006, Simplified SNF Project Baseline (MCO Sealing) (FDH 1998). This BCR deleted the hot conditioning process initially adopted for the Spent Nuclear Fuel Project (SNF Project) as documented in WHC-SD-SNF-SP-005, Integrated Process Strategy for K Basins Spent Nuclear Fuel (WHC 199.5). In summary, MCOs containing Spent Nuclear Fuel (SNF) from K Basins would be placed in interim storage following processing through the Cold Vacuum Drying (CVD) facility. With this change, the needs for the Hot Conditioning System (HCS) and inerting/pressure retaining capabilities of the CSB storage tubes and the MCO Handling Machine (MHM) were eliminated. Mechanical seals will be used on the MCOs prior to transport to the CSB. Covers will be welded on the MCOs for the final seal at the CSB. Approval of BCR No. SNF-98-006, imposed the need to review and update the CSB functions and requirements baseline documented herein including changing the document title to ''Spent Nuclear Fuel Project Canister Storage Building Functions and Requirements.'' This revision aligns the functions and requirements baseline with the CSB Simplified SNF Project Baseline (MCO Sealing). This document represents the Canister Storage Building (CSB) Subproject technical baseline. It establishes the functions and requirements baseline for the implementation of the CSB Subproject. The document is organized in eight sections. Sections 1.0 Introduction and 2.0 Overview provide brief introductions to the document and the CSB Subproject. Sections 3.0 Functions, 4.0 Requirements, 5.0 Architecture, and 6.0 Interfaces provide the data described by their titles. Section 7.0 Glossary lists the acronyms and defines the terms used in this document. Section 8.0 References lists the

  5. Spent nuclear fuel canister storage building conceptual design report

    SciTech Connect

    Swenson, C.E.

    1996-01-01

    This Conceptual Design Report provides the technical basis for the Spent Nuclear Fuels Project, Canister Storage Building, and as amended by letter (correspondence number 9555700, M.E. Witherspoon to E.B. Sellers, ``Technical Baseline and Updated Cost Estimate for the Canister Storage Building``, dated October 24, 1995), includes the project cost baseline and Criteria to be used as the basis for starting detailed design in fiscal year 1995.

  6. Machine Vision Tests for Spent Fuel Scrap Characteristics

    SciTech Connect

    BERGER, W.W.

    2000-04-27

    The purpose of this work is to perform a feasibility test of a Machine Vision system for potential use at the Hanford K basins during spent nuclear fuel (SNF) operations. This report documents the testing performed to establish functionality of the system including quantitative assessment of results. Fauske and Associates, Inc., which has been intimately involved in development of the SNF safety basis, has teamed with Agris-Schoen Vision Systems, experts in robotics, tele-robotics, and Machine Vision, for this work.

  7. SPENT FUEL CASK IMPACT LIMITER ATTACHMENT DESIGN DEFICIENCIES

    SciTech Connect

    Leduc, D; Jeffery England, J

    2007-10-16

    A recent structural analysis of the T-3 Spent Fuel Containment Cask found problems with the design of the attachment system. Assumptions in the original SARP concerning the loading in the attachment bolts were found to be inaccurate in certain drop orientations. Similar weaknesses in the attachment system designs of other casks were also noted. This paper documents the lessons learned and their applicability to impact limiter attachment system designs.

  8. Method for reprocessing and separating spent nuclear fuels

    DOEpatents

    Krikorian, Oscar H.; Grens, John Z.; Parrish, Sr., William H.

    1983-01-01

    Spent nuclear fuels, including actinide fuels, volatile and non-volatile fission products, are reprocessed and separated in a molten metal solvent housed in a separation vessel made of a carbon-containing material. A first catalyst, which promotes the solubility and permeability of carbon in the metal solvent, is included. By increasing the solubility and permeability of the carbon in the solvent, the rate at which actinide oxides are reduced (carbothermic reduction) is greatly increased. A second catalyst, included to increase the affinity for nitrogen in the metal solvent, is added to increase the rate at which actinide nitrides form after carbothermic reduction is complete.

  9. Regeneration of ammonia borane from spent fuel materials.

    PubMed

    Summerscales, Owen T; Gordon, John C

    2013-07-28

    A shift to the hydrogen economy requires the development of an effective hydrogen fuel carrier with high volumetric and gravimetric storage capacity. Ammonia borane (AB) has emerged as a leading candidate due to its light weight and multiple protic (N-H) and hydridic (B-H) hydrogens. As a consequence, much work has been directed towards fine tuning the release of H2 from AB, in addition to its regeneration from the dehydrogenated "spent fuel" materials. This review summarizes the development of these regeneration methodologies.

  10. Method for reprocessing and separating spent nuclear fuels. [Patent application

    DOEpatents

    Krikorian, O.H.; Grens, J.Z.; Parrish, W.H. Sr.

    1982-01-19

    Spent nuclear fuels, including actinide fuels, volatile and nonvolatile fission products, are reprocessed and separated in a molten metal solvent housed in a separation vessel made of a carbon-containing material. A first catalyst, which promotes the solubility and permeability of carbon in the metal solvent, is included. By increasing the solubility and permeability of the carbon in the solvent, the rate at which actinide oxides are reduced (carbothermic reduction) is greatly increased. A second catalyst, included to increase the affinity for nitrogen in the metal solvent, is added to increase the rate at which actinide nitrides form after carbothermic reduction is complete.

  11. Thermal analysis of cold vacuum drying of spent nuclear fuel

    SciTech Connect

    Piepho, M.G.

    1998-07-20

    The thermal analysis examined transient thermal and chemical behavior of the Multi canister Overpack (MCO) container for a broad range of cases that represent the Cold Vacuum Drying (CVD) processes. The cases were defined to consider both normal and off-normal operations at the CVD Facility for an MCO with Mark IV N, Reactor spent fuel in four fuel baskets and one scrap basket. This analysis provides the basis for the MCO thermal behavior at the CVD Facility for its Phase 2 Safety Analysis Report (revision 4).

  12. Preliminary Design Report Shippingport Spent Fuel Drying and Inerting System

    SciTech Connect

    JEPPSON, D.W.

    2000-05-18

    A process description and system flow sheets have been prepared to support the design/build package for the Shippingport Spent Fuel Canister drying and inerting process skid. A process flow diagram was prepared to show the general steps to dry and inert the Shippingport fuel loaded into SSFCs for transport and dry storage. Flow sheets have been prepared to show the flows and conditions for the various steps of the drying and inerting process. Calculations and data supporting the development of the flow sheets are included.

  13. Proposed high throughput electrorefining treatment for spent N- Reactor fuel

    SciTech Connect

    Gay, E.C.; Miller, W.E.; Laidler, J.J.

    1996-05-01

    A high-throughput electrorefining process is being adapted to treat spent N-Reactor fuel for ultimate disposal in a geologic repository. Anodic dissolution tests were made with unirradiated N-Reactor fuel to determine the type of fragmentation necessary to provide fuel segments suitable for this process. Based on these tests, a conceptual design was produced of a plant-scale electrorefiner. In this design, the diameter of an electrode assembly is about 1.07 m (42 in.). Three of these assemblies in an electrorefiner would accommodate a 3-metric-ton batch of N-Reactor fuel that would be processed at a rate of 42 kg of uranium per hour.

  14. DOE-owned spent nuclear fuel program plan

    SciTech Connect

    1995-11-01

    The Department of Energy (DOE) has produced spent nuclear fuel (SNF) for many years as part of its various missions and programs. The historical process for managing this SNF was to reprocess it whereby valuable material such as uranium or plutonium was chemically separated from the wastes. These fuels were not intended for long-term storage. As the need for uranium and plutonium decreased, it became necessary to store the SNF for extended lengths of time. This necessity resulted from a 1992 DOE decision to discontinue reprocessing SNF to recover strategic materials (although limited processing of SNF to meet repository acceptance criteria remains under consideration, no plutonium or uranium extraction for other uses is planned). Both the facilities used for storage, and the fuel itself, began experiencing aging from this extended storage. New efforts are now necessary to assure suitable fuel and facility management until long-term decisions for spent fuel disposition are made and implemented. The Program Plan consists of 14 sections as follows: Sections 2--6 describe objectives, management, the work plan, the work breakdown structure, and the responsibility assignment matrix. Sections 7--9 describe the program summary schedules, site logic diagram, SNF Program resource and support requirements. Sections 10--14 present various supplemental management requirements and quality assurance guidelines.

  15. Spent fuel and HLW transportation the French experience

    SciTech Connect

    Giraud, J.P.; Charles, J.L.

    1995-12-31

    With 53 nuclear power plants in operation at EDF and a fuel cycle with recycling policy of the valuable materials, COGEMA is faced with the transport of a wide range of radioactive materials. In this framework, the transport activity is a key link in closing the fuel cycle. COGEMA has developed a comprehensive Transport Organization System dealing with all the sectors of the fuel cycle. The paper will describe the status of transportation of spent fuel and HLW in France and the experience gathered. The Transport Organization System clearly defines the role of all actors where COGEMA, acting as the general coordinator, specifies the tasks to be performed and brings technical and commercial support to its various subcontractors: TRANSNUCLEAIRE, specialized in casks engineering and transport operations, supplies packaging and performs transport operations, LEMARECHAL and CELESTIN operate transport by truck in the Vicinity of the nuclear sites while French Railways are in charge of spent fuel transport by train. HLW issued from the French nuclear program is stored for 30 years in an intermediate storage installation located at the La Hague reprocessing plant. Ultimately, these canisters will be transported to the disposal site. COGEMA has set up a comprehensive transport organization covering all operational aspects including adapted procedures, maintenance programs and personnel qualification.

  16. Recovery of actinides from LWR spent fuel by pyrochemistry

    SciTech Connect

    McPheeters, C.C.; Pierce, R.D.; Johnson, G.K.; Poa, D.S.

    1993-12-31

    Recovery of transuranium elements from light-water reactor spent fuel for burnup in the integral fast reactor is an attractive alternative to the current once-through, low burn-up fuel cycle. Argonne National Laboratory is developing pyrochemical methods for recovery of these actinide elements. The processes involve reducing the oxide fuel to metals, separation of the transuranium elements from the bulk uranium, and consolidating the trans uranium product as a metal ingot suitable for introduction into the integral fast reactor fuel cycle. The process streams are recycled where possible to minimize wastes. The process steps have been proven in small-scale experiments, and the process is being scaleup up for {open_quotes}engineering-scale{close_quotes} demonstration (20-kg batch size). This engineering-scale system is in the construction stage, and it is expected to be in operation by late 1993. Future plans include additional demonstration of the processes with actual light-water reactor spent fuel, development of qualified waste forms, and development of a preliminary design for a full-scale processing plant.

  17. Partial Defect Verification of Spent Fuel Assemblies by PDET: Principle and Field Testing in Interim Spent Fuel Storage Facility (CLAB) in Sweden

    SciTech Connect

    Ham, Y.S.; Kerr, P.; Sitaraman, S.; Swan, R.; Rossa, R.; Liljenfeldt, H.

    2015-07-01

    The need for the development of a credible method and instrument for partial defect verification of spent fuel has been emphasized over a few decades in the safeguards communities as the diverted spent fuel pins can be the source of nuclear terrorism or devices. The need is increasingly more important and even urgent as many countries have started to transfer spent fuel to so called 'difficult-to-access' areas such as dry storage casks, reprocessing or geological repositories. Partial defect verification is required by IAEA before spent fuel is placed into 'difficult-to-access' areas. Earlier, Lawrence Livermore National Laboratory (LLNL) has reported the successful development of a new, credible partial defect verification method for pressurized water reactor (PWR) spent fuel assemblies without use of operator data, and further reported the validation experiments using commercial spent fuel assemblies with some missing fuel pins. The method was found to be robust as the method is relatively invariant to the characteristic variations of spent fuel assemblies such as initial fuel enrichment, cooling time, and burn-up. Since then, the PDET system has been designed and prototyped for 17x17 PWR spent fuel assemblies, complete with data acquisition software and acquisition electronics. In this paper, a summary description of the PDET development followed by results of the first successful field testing using the integrated PDET system and actual spent fuel assemblies performed in a commercial spent fuel storage site, known as Central Interim Spent fuel Storage Facility (CLAB) in Sweden will be presented. In addition to partial defect detection initial studies have determined that the tool can be used to verify the operator declared average burnup of the assembly as well as intra-assembly burnup levels. (authors)

  18. Direct disposal of spent fuel: developing solutions tailored to Japan

    SciTech Connect

    Kawamura, Hideki; McKinley, Ian G

    2013-07-01

    With the past Government policy of 100% reprocessing in Japan now open to discussion, options for direct disposal of spent fuel (SF) are now being considered in Japan. The need to move rapidly ahead in developing spent fuel management concepts is closely related to the ongoing debate on the future of nuclear power in Japan and the desire to understand the true costs of the entire life cycle of different options. Different scenarios for future nuclear power - and associated decisions on extent of reprocessing - will give rise to quite different inventories of SF with different disposal challenges. Although much work has been carried out spent fuel disposal within other national programmes, the potential for mining the international knowledge base is limited by the boundary conditions for disposal in Japan. Indeed, with a volunteer approach to siting, no major salt deposits and few undisturbed sediments, high tectonic activity, relatively corrosive groundwater and no deserts, it is evident that a tailored solution is needed. Nevertheless, valuable lessons can be learned from projects carried out worldwide, if focus is placed on basic principles rather than implementation details. (authors)

  19. Thermoelectric powered wireless sensors for spent fuel monitoring

    SciTech Connect

    Carstens, T.; Corradini, M.; Blanchard, J.; Ma, Z.

    2011-07-01

    This paper describes using thermoelectric generators to power wireless sensors to monitor spent nuclear fuel during dry-cask storage. OrigenArp was used to determine the decay heat of the spent fuel at different times during the service life of the dry-cask. The Engineering Equation Solver computer program modeled the temperatures inside the spent fuel storage facility during its service life. The temperature distribution in a thermoelectric generator and heat sink was calculated using the computer program Finite Element Heat Transfer. From these temperature distributions the power produced by the thermoelectric generator was determined as a function of the service life of the dry-cask. In addition, an estimation of the path loss experienced by the wireless signal can be made based on materials and thickness of the structure. Once the path loss is known, the transmission power and thermoelectric generator power requirements can be determined. This analysis estimates that a thermoelectric generator can produce enough power for a sensor to function and transmit data from inside the dry-cask throughout its service life. (authors)

  20. Analysis of Experimental Data for High Burnup PWR Spent Fuel Isotopic Validation - Vandellos II Reactor

    SciTech Connect

    Ilas, Germina; Gauld, Ian C

    2011-01-01

    This report is one of the several recent NUREG/CR reports documenting benchmark-quality radiochemical assay data and the use of the data to validate computer code predictions of isotopic composition for spent nuclear fuel, to establish the uncertainty and bias associated with code predictions. The experimental data analyzed in the current report were acquired from a high-burnup fuel program coordinated by Spanish organizations. The measurements included extensive actinide and fission product data of importance to spent fuel safety applications, including burnup credit, decay heat, and radiation source terms. Six unique spent fuel samples from three uranium oxide fuel rods were analyzed. The fuel rods had a 4.5 wt % {sup 235}U initial enrichment and were irradiated in the Vandellos II pressurized water reactor operated in Spain. The burnups of the fuel samples range from 42 to 78 GWd/MTU. The measurements were used to validate the two-dimensional depletion sequence TRITON in the SCALE computer code system.

  1. Commercial Spent Nuclear Fuel Waste Package Misload Analysis

    SciTech Connect

    J.K. Knudson

    2003-10-02

    The purpose of this calculation is to estimate the probability of misloading a commercial spent nuclear fuel waste package with a fuel assembly(s) that has a reactivity (i.e., enrichment and/or burnup) outside the waste package design. The waste package designs are based on the expected commercial spent nuclear fuel assemblies and previous analyses (Macheret, P. 2001, Section 4.1 and Table 1). For this calculation, a misloaded waste package is defined as a waste package that has a fuel assembly(s) loaded into it with an enrichment and/or burnup outside the waste package design. An example of this type of misload is a fuel assembly designated for the 21-PWR Control Rod waste package being incorrectly loaded into a 21-PWR Absorber Plate waste package. This constitutes a misloaded 21-PWR Absorber Plate waste package, because the reactivity (i.e., enrichment and/or burnup) of a 21-PWR Control Rod waste package fuel assembly is outside the design of a 21-PWR Absorber Plate waste package. These types of misloads (i.e., fuel assembly with enrichment and/or burnup outside waste package design) are the only types that are evaluated in this calculation. This calculation utilizes information from ''Frequency of SNF Misload for Uncanistered Fuel Waste Package'' (CRWMS M&O 1998) as the starting point. The scope of this calculation is limited to the information available. The information is based on the whole population of fuel assemblies and the whole population of waste packages, because there is no information about the arrival of the waste stream at this time. The scope of this calculation deviates from that specified in ''Technical Work Plan for: Risk and Criticality Department'' (BSC 2002a, Section 2.1.30) in that only waste package misload is evaluated. The remaining issues identified (i.e., flooding and geometry reconfiguration) will be addressed elsewhere. The intended use of the calculation is to provide information and inputs to the Preclosure Safety Analysis

  2. Commercial Spent Nuclear Fuel Waste Package Misload Analysis

    SciTech Connect

    A. Alsaed

    2005-07-28

    The purpose of this calculation is to estimate the probability of misloading a commercial spent nuclear fuel waste package with a fuel assembly(s) that has a reactivity (i.e., enrichment and/or burnup) outside the waste package design. The waste package designs are based on the expected commercial spent nuclear fuel assemblies and previous analyses (Macheret, P. 2001, Section 4.1 and Table 1). For this calculation, a misloaded waste package is defined as a waste package that has a fuel assembly(s) loaded into it with an enrichment and/or burnup outside the waste package design. An example of this type of misload is a fuel assembly designated for the 21-PWR Control Rod waste package being incorrectly loaded into a 21-PWR Absorber Plate waste package. This constitutes a misloaded 21-PWR Absorber Plate waste package, because the reactivity (i.e., enrichment and/or burnup) of a 21-PWR Control Rod waste package fuel assembly is outside the design of a 21-PWR Absorber Plate waste package. These types of misloads (i.e., fuel assembly with enrichment and/or burnup outside waste package design) are the only types that are evaluated in this calculation. This calculation utilizes information from ''Frequency of SNF Misload for Uncanistered Fuel Waste Package'' (CRWMS M&O 1998) as the starting point. The scope of this calculation is limited to the information available. The information is based on the whole population of fuel assemblies and the whole population of waste packages, because there is no information about the arrival of the waste stream at this time. The scope of this calculation deviates from that specified in ''Technical Work Plan for: Risk and Criticality Department'' (BSC 2002a, Section 2.1.30) in that only waste package misload is evaluated. The remaining issues identified (i.e., flooding and geometry reconfiguration) will be addressed elsewhere. The intended use of the calculation is to provide information and inputs to the Preclosure Safety Analysis

  3. Studies and research concerning BNFP: spent fuel dry storage studies at the Barnwell Nuclear Fuel Plant

    SciTech Connect

    Anderson, Kenneth J.

    1980-09-01

    Conceptual designs are presented utilizing the Barnwell Nuclear Fuel Plant for the dry interim storage of spent light water reactor fuel. Studies were conducted to determine feasible approaches to storing spent fuel by methods other than wet pool storage. Fuel that has had an opportunity to cool for several years, or more, after discharge from a reactor is especially adaptable to dry storage since its thermal load is greatly reduced compared to the thermal load immediately following discharge. A thermal analysis was performed to help in determining the feasibility of various spent fuel dry storage concepts. Methods to reject the heat from dry storage are briefly discussed, which include both active and passive cooling systems. The storage modes reviewed include above and below ground caisson-type storage facilities and numerous variations of vault, or hot cell-type, storage facilities.

  4. A Second Look at Neutron Resonance Transmission Analysis as a Spent Fuel NDA Technique

    SciTech Connect

    James W .Sterbentz; David L. Chichester

    2011-07-01

    Many different nondestructive analysis techniques are currently being investigated as a part of the United States Department of Energy's Next Generation Safeguards Initiative (NGSI) seeking methods to quantify plutonium in spent fuel. Neutron Resonance Transmission Analysis (NRTA) is one of these techniques. Having first been explored in the mid-1970s for the analysis of individual spent-fuel pins a second look, using advanced simulation and modeling methods, is now underway to investigate the suitability of the NRTA technique for assaying complete spent nuclear fuel assemblies. The technique is similar to neutron time-of-flight methods used for cross-section determinations but operates over only the narrow 0.1-20 eV range where strong, distinguishable resonances exist for both the plutonium (239, 240, 241,242Pu) and uranium (235,236,238U) isotopes of interest in spent fuel. Additionally, in this energy range resonances exists for six important fission products (99Tc, 103Rh, 131Xe, 133Cs, 145Nd, and 152Sm) which provide additional information to support spent fuel plutonium assay determinations. Initial modeling shows excellent agreement with previously published experimental data for measurements of individual spent-fuel pins where plutonium assays were demonstrated to have a precision of 2-4%. Within the simulation and modeling analyses of this project scoping studies have explored fourteen different aspects of the technique including the neutron source, drift tube configurations, and gross neutron transmission as well as the impacts of fuel burn up, cooling time, and fission-product interferences. These results show that NRTA may be a very capable experimental technique for spent-fuel assay measurements. The results suggest sufficient transmission strength and signal differentiability is possible for assays through up to 8 pins. For an 8-pin assay (looking at an assembly diagonally), 64% of the pins in a typical 17 ? 17 array of a pressurized water reactor fuel

  5. Behavior of iodine in the dissolution of spent nuclear fuels

    SciTech Connect

    Sakurai, Tsutomu; Komatsu, Kazunori; Takahashi, A.

    1997-08-01

    The results of laboratory-scale experiments concerning the behavior of iodine in the dissolution of spent nuclear fuels, which were carried out at the Japan Atomic Energy Research Institute, are summarized. Based on previous and new experimental results, the difference in quantity of residual iodine in the fuel solution between laboratory-scale experiments and reprocessing plants is discussed, Iodine in spent fuels is converted to the following four states: (1) oxidation into I{sub 2} by nitric acid, (2) oxidation into I{sub 2} by nitrous acid generated in the dissolution, (3) formation of a colloid of insoluble iodides such as AgI and PdI{sub 2}, and (4) deposition on insoluble residue. Nitrous acid controls the amount of colloid formed. As a result, up to 10% of iodine in spent fuels is retained in the fuel solution, up to 3% is deposited on insoluble residue, and the balance volatilizes to the off-gas, Contrary to earlier belief, when the dissolution is carried out in 3 to 4 M HNO{sub 3} at 100{degrees}C, the main iodine species in a fuel solution is a colloid, not iodate, Immediately after its formation, the colloid is unstable and decomposes partially in the hot nitric acid solution through the following reaction: AgI(s) + 2HNO{sub 3}(aq) = {1/2}I{sub 2}(aq) + AgNO{sub 3}(aq) + NO{sub 2}(g) + H{sub 2}O(1). For high concentrations of gaseous iodine, I{sub 2}(g), and NO{sub 2}, this reaction is reversed towards formation of the colloid (AgI). Since these concentrations are high near the liquid surface of a plant-scale dissolver, there is a possibility that the colloid is formed there through this reversal, Simulations performed in laboratory-scale experiments demonstrated this reversal, This phenomenon can be one reason the quantity of residual iodine in spent fuels is higher in reprocessing plants than in laboratory-scale experiments. 17 refs., 5 figs., 3 tabs.

  6. Corrosion of Spent Nuclear Fuel: The Long-Term Assessment

    SciTech Connect

    Ewing, Rodney C.

    2003-09-14

    The successful disposal of spent nuclear fuel (SNF) is one of the most serious challenges to the successful completion of the nuclear fuel cycle and the future of nuclear power generation. In the United States, 21 percent of the electricity is generated by 107 commercial nuclear power plants (NPP), each of which generates 20 metric tons of spent nuclear fuel annually. In 1996, the total accumulation of spent nuclear fuel was 33,700 metric tons of heavy metal (MTHM) stored at 70 sites around the country. The end-of-life projection for current nuclear power plants (NPP) is approximately 86,000 MTHM. In the proposed nuclear waste repository at Yucca Mountain over 95% of the radioactivity originates from spent nuclear fuel. World-wide in 1998, approximately 130,000 MTHM of SNF have accumulated, most of it located at 236 NPP in 36 countries. Annual production of SNF is approximately 10,000 MTHM, containing about 100 tons of ''reactor grade'' plutonium. Any reasonable increase in the proportion of energy production by NPP, i.e., as a substitute for hydrocarbon-based sources of energy, will significantly increase spent nuclear fuel production. Spent nuclear fuel is essentially UO{sub 2} with approximately 4-5 atomic percent actinides and fission product elements. A number of these elements have long half-lives hence, the long-term behavior of the UO{sub 2} is an essential concern in the evaluation of the safety and risk of a repository for spent nuclear fuel. One of the unique and scientifically most difficult aspects of the successful disposal of spent nuclear fuel is the extrapolation of short-term laboratory data (hours to years) to the long time periods (10{sup 3} to 10{sup 5} years) as required by the performance objectives set in regulations, i.e. 10 CFR 60. The direct verification of these extrapolations or interpolations is not possible, but methods must be developed to demonstrate compliance with government regulations and to satisfy the public that there is a

  7. Climax spent fuel dosimetry. Short term exposure, 8 March 1983

    SciTech Connect

    Quam, W.; DeVore, T.

    1984-06-01

    The second short-term exposure (performed 8 March 1983) in Hole CFH3 at the Climax Spent Fuel Test site is described. These short-term (1 hour long) exposures are intended to provide an independent measurement of the exposure rate at the wall and the 0.51-m and 0.66-m locations. Only CaF{sub 2} TLD`s were used in the second short-term exposure. Harshaw chips were cut to 0.32 x 0.18 x 0.09 cm size and aged by several exposure/readout/bakeout cycles until all odd chips were weeded out and the remaining chips exhibited stable sensitivities. Exposure at Climax was done by removing the existing long-term dosimetry strings and inserting identical strings using the CaF{sub 2} TLD`s in the stainless steel holders. The first short-term exposure produced absorbed doses as high as {similar_to}000 rads-LiF. The linearity corrections determined for the CaF{sub 2} TLD`s at these exposure levels were {similar_to}2%. The present post-exposure calibration method used calibration doses very close to those encountered in the field.

  8. Extending Spent Fuel Storage until Transport for Reprocessing or Disposal

    SciTech Connect

    Carlsen, Brett; Chiguer, Mustapha; Grahn, Per; Sampson, Michele; Wolff, Dietmar; Bevilaqua, Arturo; Wasinger, Karl; Saegusa, Toshiari; Seelev, Igor

    2016-09-01

    Spent fuel (SF) must be stored until an end point such as reprocessing or geologic disposal is imple-mented. Selection and implementation of an end point for SF depends upon future funding, legisla-tion, licensing and other factors that cannot be predicted with certainty. Past presumptions related to the availability of an end point have often been wrong and resulted in missed opportunities for properly informing spent fuel management policies and strategies. For example, dry cask storage systems were originally conceived to free up needed space in reactor spent fuel pools and also to provide SFS of up to 20 years until reprocessing and/or deep geological disposal became available. Hundreds of dry cask storage systems are now employed throughout the world and will be relied upon well beyond the originally envisioned design life. Given present and projected rates for the use of nuclear power coupled with projections for SF repro-cessing and disposal capacities, one concludes that SF storage will be prolonged, potentially for several decades. The US Nuclear Regulatory Commission has recently considered 300 years of storage to be appropriate for the characterization and prediction of ageing effects and ageing management issues associated with extending SF storage and subsequent transport. This paper encourages addressing the uncertainty associated with the duration of SF storage by de-sign – rather than by default. It suggests ways that this uncertainty may be considered in design, li-censing, policy, and strategy decisions and proposes a framework for safely extending spent fuel storage until SF can be transported for reprocessing or disposal – regardless of how long that may be. The paper however is not intended to either encourage or facilitate needlessly extending spent fuel storage durations. Its intent is to ensure a design and safety basis with sufficient margin to accommodate the full range of potential future scenarios. Although the focus is primarily on

  9. An approach to determine a defensible spent fuel ratio.

    SciTech Connect

    Durbin, Samuel G.; Lindgren, Eric Richard

    2014-03-01

    Sabotage of spent nuclear fuel casks remains a concern nearly forty years after attacks against shipment casks were first analyzed and has a renewed relevance in the post-9/11 environment. A limited number of full-scale tests and supporting efforts using surrogate materials, typically depleted uranium dioxide (DUO2), have been conducted in the interim to more definitively determine the source term from these postulated events. In all the previous studies, the postulated attack of greatest interest was by a conical shape charge (CSC) that focuses the explosive energy much more efficiently than bulk explosives. However, the validity of these large-scale results remain in question due to the lack of a defensible Spent Fuel Ratio (SFR), defined as the amount of respirable aerosol generated by an attack on a mass of spent fuel compared to that of an otherwise identical DUO2 surrogate. Previous attempts to define the SFR have resulted in estimates ranging from 0.42 to 12 and include suboptimal experimental techniques and data comparisons. Different researchers have suggested using SFR values of 3 to 5.6. Sound technical arguments exist that the SFR does not exceed a value of unity. A defensible determination of the SFR in this lower range would greatly reduce the calculated risk associated with the transport and dry storage of spent nuclear fuel. Currently, Oak Ridge National Laboratory (ORNL) is in possession of several samples of spent nuclear fuel (SNF) that were used in the original SFR studies in the 1980s and were intended for use in a modern effort at Sandia National Laboratories (SNL) in the 2000s. A portion of these samples are being used for a variety of research efforts. However, the entirety of SNF samples at ORNL is scheduled for disposition at the Waste Isolation Pilot Plant (WIPP) by approximately the end of 2015. If a defensible SFR is to be determined for use in storage and transportation security analyses, the need to begin this effort

  10. Spent Fuel Test-Climax: An evaluation of the technical feasibility of geologic storage of spent nuclear fuel in granite: Final report

    SciTech Connect

    Patrick, W.C.

    1986-03-30

    In the Climax stock granite on the Nevada Test Site, eleven canisters of spent nuclear reactor fuel were emplaced, and six electrical simulators were energized. When test data indicated that the test objectives were met during the 3-year storage phase, the spent-fuel canisters were retrieved and the thermal sources were de-energized. The project demonstrated the feasibility of packaging, transporting, storing, and retrieving highly radioactive fuel assemblies in a safe and reliable manner. In addition to emplacement and retrieval operations, three exchanges of spent-fuel assemblies between the SFT-C and a surface storage facility, conducted during the storage phase, furthered this demonstration. The test led to development of a technical measurements program. To meet these objectives, nearly 1000 instruments and a computer-based data acquisition system were deployed. Geotechnical, seismological, and test status data were recorded on a continuing basis for the three-year storage phase and six-month monitored cool-down of the test. This report summarizes the engineering and scientific endeavors which led to successful design and execution of the test. The design, fabrication, and construction of all facilities and handling systems are discussed, in the context of test objectives and a safety assessment. The discussion progresses from site characterization and experiment design through data acquisition and analysis of test data in the context of design calculations. 117 refs., 52 figs., 81 tabs.

  11. Testing and analyses of the TN-24P PWR spent-fuel dry storage cask loaded with consolidated fuel

    SciTech Connect

    McKinnon, M A; Michener, T E; Jensen, M F; Rodman, G R

    1989-02-01

    A performance test of a Transnuclear, Inc. TN-24P storage cask configured for pressurized water reactor (PWR) spent fuel was performed. The work was performed by the Pacific Northwest Laboratory (PNL) and Idaho National Engineering Laboratory (INEL) for the US Department of Energy Office of Civilian Radioactive Waste Management (OCRWM) and the Electric Power Research Institute. The performance test consisted of loading the TN-24P cask with 24 canisters of consolidated PWR spent fuel from Virginia Power's Surry and Florida Power and Light's Turkey Point reactors. Cask surface and fuel canister guide tube temperatures were measured, as were cask surface gamma and neutron dose rates. Testing was performed with vacuum, nitrogen, and helium backfill environments in both vertical and horizontal cask orientations. Transnuclear, Inc., arranged to have a partially insulated run added to the end of the test to simulate impact limiters. Limited spent fuel integrity data were also obtained. From both heat transfer and shielding perspectives, the TN-24P cask with minor refinements can be effectively implemented at reactor sites and central storage facilities for safe storage of unconsolidated and consolidated spent fuel. 35 refs., 93 figs., 17 tabs.

  12. Dry Storage of Research Reactor Spent Nuclear Fuel - 13321

    SciTech Connect

    Adams, T.M.; Dunsmuir, M.D.; Leduc, D.R.; Severynse, T.F.; Sindelar, R.L.; Moore, E.N.

    2013-07-01

    Spent fuel from domestic and foreign research reactors is received and stored at the Savannah River Site's L Area Material Storage (L Basin) Facility. This DOE-owned fuel consists primarily of highly enriched uranium in metal, oxide or silicide form with aluminum cladding. Upon receipt, the fuel is unloaded and transferred to basin storage awaiting final disposition. Disposition alternatives include processing via the site's H Canyon facility for uranium recovery, or packaging and shipment of the spent fuel to a waste repository. A program has been developed to provide a phased approach for dry storage of the L Basin fuel. The initial phase of the dry storage program will demonstrate loading, drying, and storage of fuel in twelve instrumented canisters to assess fuel performance. After closure, the loaded canisters are transferred to pad-mounted concrete overpacks, similar to those used for dry storage of commercial fuel. Unlike commercial spent fuel, however, the DOE fuel has high enrichment, very low to high burnup, and low decay heat. The aluminum cladding presents unique challenges due to the presence of an oxide layer that forms on the cladding surface, and corrosion degradation resulting from prolonged wet storage. The removal of free and bound water is essential to the prevention of fuel corrosion and radiolytic generation of hydrogen. The demonstration will validate models predicting pressure, temperature, gas generation, and corrosion performance, provide an engineering scale demonstration of fuel handling, drying, leak testing, and canister backfill operations, and establish 'road-ready' storage of fuel that is suitable for offsite repository shipment or retrievable for onsite processing. Implementation of the Phase I demonstration can be completed within three years. Phases II and III, leading to the de-inventory of L Basin, would require an additional 750 canisters and 6-12 years to complete. Transfer of the fuel from basin storage to dry storage

  13. Determination of plutonium in spent nuclear fuel using high resolution X-ray

    SciTech Connect

    McIntosh, Kathryn G.; Reilly, Sean D.; Havrilla, George J.

    2015-05-30

    Characterization of Pu is an essential aspect of safeguards operations at nuclear fuel reprocessing facilities. A novel analysis technique called hiRX (high resolution X-ray) has been developed for the direct measurement of Pu in spent nuclear fuel dissolver solutions. hiRX is based on monochromatic wavelength dispersive X-ray fluorescence (MWDXRF), which provides enhanced sensitivity and specificity compared with conventional XRF techniques. A breadboard setup of the hiRX instrument was calibrated using spiked surrogate spent fuel (SSF) standards prepared as dried residues. Samples of actual spent fuel were utilized to evaluate the performance of the hiRX. The direct detection of just 39 ng of Pu is demonstrated. Initial quantitative results, with error of 4–27% and precision of 2% relative standard deviation (RSD), were obtained for spent fuel samples. The limit of detection for Pu (100 s) within an excitation spot of 200 μm diameter was 375 pg. This study demonstrates the potential for the hiRX technique to be utilized for the rapid, accurate, and precise determination of Pu. Moreover, the results highlight the analytical capability of hiRX for other applications requiring sensitive and selective nondestructive analyses.

  14. Determination of plutonium in spent nuclear fuel using high resolution X-ray

    DOE PAGES

    McIntosh, Kathryn G.; Reilly, Sean D.; Havrilla, George J.

    2015-05-30

    Characterization of Pu is an essential aspect of safeguards operations at nuclear fuel reprocessing facilities. A novel analysis technique called hiRX (high resolution X-ray) has been developed for the direct measurement of Pu in spent nuclear fuel dissolver solutions. hiRX is based on monochromatic wavelength dispersive X-ray fluorescence (MWDXRF), which provides enhanced sensitivity and specificity compared with conventional XRF techniques. A breadboard setup of the hiRX instrument was calibrated using spiked surrogate spent fuel (SSF) standards prepared as dried residues. Samples of actual spent fuel were utilized to evaluate the performance of the hiRX. The direct detection of just 39more » ng of Pu is demonstrated. Initial quantitative results, with error of 4–27% and precision of 2% relative standard deviation (RSD), were obtained for spent fuel samples. The limit of detection for Pu (100 s) within an excitation spot of 200 μm diameter was 375 pg. This study demonstrates the potential for the hiRX technique to be utilized for the rapid, accurate, and precise determination of Pu. Moreover, the results highlight the analytical capability of hiRX for other applications requiring sensitive and selective nondestructive analyses.« less

  15. Accelerator-driven transmutation of spent fuel elements

    DOEpatents

    Venneri, Francesco; Williamson, Mark A.; Li, Ning

    2002-01-01

    An apparatus and method is described for transmuting higher actinides, plutonium and selected fission products in a liquid-fuel subcritical assembly. Uranium may also be enriched, thereby providing new fuel for use in conventional nuclear power plants. An accelerator provides the additional neutrons required to perform the processes. The size of the accelerator needed to complete fuel cycle closure depends on the neutron efficiency of the supported reactors and on the neutron spectrum of the actinide transmutation apparatus. Treatment of spent fuel from light water reactors (LWRs) using uranium-based fuel will require the largest accelerator power, whereas neutron-efficient high temperature gas reactors (HTGRs) or CANDU reactors will require the smallest accelerator power, especially if thorium is introduced into the newly generated fuel according to the teachings of the present invention. Fast spectrum actinide transmutation apparatus (based on liquid-metal fuel) will take full advantage of the accelerator-produced source neutrons and provide maximum utilization of the actinide-generated fission neutrons. However, near-thermal transmutation apparatus will require lower standing

  16. Spent fuel drying system test results (second dry-run)

    SciTech Connect

    Klinger, G.S.; Oliver, B.M.; Abrefah, J.; Marschman, S.C.; MacFarlan, P.J.; Ritter, G.A.

    1998-07-01

    The water-filled K-Basins in the Hanford 100 Area have been used to store N-Reactor spent nuclear fuel (SNF) since the 1970s. Because some leaks have been detected in the basins and some of the fuel is breached due to handling damage and corrosion, efforts are underway to remove the fuel elements from wet storage. An Integrated Process Strategy (IPS) has been developed to package, dry, transport, and store these metallic uranium fuel elements in an interim storage facility on the Hanford Site (WHC 1995). Information required to support the development of the drying processes, and the required safety analyses, is being obtained from characterization tests conducted on fuel elements removed from the K-Basins. A series of whole element drying tests (reported in separate documents, see Section 7.0) have been conducted by Pacific Northwest National Laboratory (PNNL) on several intact and damaged fuel elements recovered from both the K-East and K-West Basins. This report documents the results of the second dry-run test, which was conducted without a fuel element. With the concurrence of project management, the test protocol for this run, and subsequent drying test runs, was modified. These modifications were made to allow for improved data correlation with drying procedures proposed under the IPS. Details of these modifications are discussed in Section 3.0.

  17. Spent fuel temperature and age determination from the analysis of uranium and plutonium isotopics

    SciTech Connect

    Scott, Mark R; Eccleston, George W; Bedell, Jeffrey J; Lockard, Chanelle M

    2009-01-01

    The capability to determine the age (time since irradiation) of spent fuel can be useful for verification and safeguards. While the age of spent fuel can be determined based on measurements of short-lived fission products, these measurements are not routinely done nor generally reported. As an alternative, age can also be determined if the uranium (U) and plutonium (Pu) isotopic values are available. Uranium isotopics are not strongly affected by fuel temperature, and bumup is determined from the {sup 235}U and {sup 236}U isotopic values. Age is calculated after estimating the {sup 241}Pu at the end of irradiation while accounting for the fuel temperature, which is determined from {sup 239}Pu or {sup 240}Pu. Burnup and age determinations are calibrated to reactor models that provide uranium and plutonium isotopics over the range of fuel irradiation. The reactor model must contain sufficient fidelity on details of the reactor type, fuel burnup, irradiation history, initial fuel enrichment and fuel temperature to obtain accurate isotopic calculations. If the latter four are unknown, they can be derived from the uranium and plutonium isotopics. Fuel temperature has a significant affect on the production of plutonium isotopics; therefore, one group cross section reactor models, such as ORIGEN, cannot be used for these calculations. Multi-group cross section set codes, such as Oak Ridge National Laboratory's TRITON code, must be used.

  18. APPLICATIONS OF CURRENT TECHNOLOGY FOR CONTINUOUS MONITORING OF SPENT FUEL

    SciTech Connect

    Drayer, R.

    2013-06-09

    Advancements in technology have opened many opportunities to improve upon the current infrastructure surrounding the nuclear fuel cycle. Embedded devices, very small sensors, and wireless technology can be applied to Security, Safety, and Nonproliferation of Spent Nuclear Fuel. Security, separate of current video monitoring systems, can be improved by integrating current wireless technology with a variety of sensors including motion detection, altimeter, accelerometer, and a tagging system. By continually monitoring these sensors, thresholds can be set to sense deviations from nominal values. Then alarms or notifications can be activated as needed. Safety can be improved in several ways. First, human exposure to ionizing radiation can be reduced by using a wireless sensor package on each spent fuel cask to monitor radiation, temperature, humidity, etc. Since the sensor data is monitored remotely operator stay-time is decreased and distance from the spent fuel increased, so the overall radiation exposure is reduced as compared to visual inspections. The second improvement is the ability to monitor continuously rather than periodically. If changes occur to the material, alarm thresholds could be set and notifications made to provide advanced notice of negative data trends. These sensor packages could also record data to be used for scientific evaluation and studies to improve transportation and storage safety. Nonproliferation can be improved for spent fuel transportation and storage by designing an integrated tag that uses current infrastructure for reporting and in an event; tracking can be accomplished using the Iridium satellite system. This technology is similar to GPS but with higher signal strength and penetration power, but lower accuracy. A sensor package can integrate all or some of the above depending on the transportation and storage requirements and regulations. A sensor package can be developed using off the shelf technology and applying it to each

  19. An integrated approach for determining plutonium mass in spent fuel assemblies with nondestructive assay

    SciTech Connect

    Swinhoe, Martyn T; Tobin, Stephen J; Fensin, Mike L; Menlove, Howard O

    2009-01-01

    There are a variety of reasons for quantifying plutonium (Pu) in spent fuel. Below, five motivations are listed: (1) To verify the Pu content of spent fuel without depending on unverified information from the facility, as requested by the IAEA ('independent verification'). New spent fuel measurement techniques have the potential to allow the IAEA to recover continuity of knowledge and to better detect diversion. (2) To assure regulators that all of the nuclear material of interest leaving a nuclear facility actually arrives at another nuclear facility ('shipper/receiver'). Given the large stockpile of nuclear fuel at reactor sites around the world, it is clear that in the coming decades, spent fuel will need to be moved to either reprocessing facilities or storage sites. Safeguarding this transportation is of significant interest. (3) To quantify the Pu in spent fuel that is not considered 'self-protecting.' Fuel is considered self-protecting by some regulatory bodies when the dose that the fuel emits is above a given level. If the fuel is not self-protecting, then the Pu content of the fuel needs to be determined and the Pu mass recorded in the facility's accounting system. This subject area is of particular interest to facilities that have research-reactor spent fuel or old light-water reactor (LWR) fuel. It is also of interest to regulators considering changing the level at which fuel is considered self-protecting. (4) To determine the input accountability value at an electrochemical processing facility. It is not expected that an electrochemical reprocessing facility will have an input accountability tank, as is typical in an aqueous reprocessing facility. As such, one possible means of determining the input accountability value is to measure the Pu content in the spent fuel that arrives at the facility. (5) To fully understand the composition of the fuel in order to efficiently and safely pack spent fuel into a long-term repository. The NDA of spent fuel can

  20. SPENT NUCLEAR FUEL WASTE PACKAGE FILLER TESTING TECHNICAL GUIDELINES DOCUMENT

    SciTech Connect

    J.A. Cogar

    1996-08-28

    The purpose of this work is to provide supporting calculations for determination of the radiation source terms specific to subsurface shielding design and analysis. These calculations are not intended to provide the absolute values of the source terms, which are under the charter of the Waste Package Operations (WPO) Group. Rather, the calculations focus on evaluation of the various combinations of fuel enrichment, burnup and cooling time for a given decay heat output, consistent with the waste package (WP) thermal design basis. The objective is to determine the worst-case combination of the fuel characteristics (enrichment, burnup and cooling time) which would give the maximum radiation fields for subsurface shielding considerations. The calculations are limited to PWR fuel only, since the WP design is currently evolving with thinner walls and a reduced heat load as compared to the viability assessment (VA) reference design. The results for PWR fuel will provide a comparable indication of the trend for BWR fuel, as their characteristics are similar. The source term development for defense high-level waste and other spent nuclear fuel (SNF) is the responsibility of the WPO Group, and therefore, is not included this work. This work includes the following items responsive to the stated purpose and objective: (1) Determine the possible fuel parameters (initial enrichment, burnup and cooling time), that give the same decay heat value as specified for the waste package thermal design; (2) Obtain the neutron and gamma source terms for the various combinations of the fuel parameters for use in radiation field calculations; and (3) Calculate radiation fields on the surfaces of the waste package and its transporter to quantify the effects of the fuel parameters with the same decay heat value for use in identifying the worst-case combination of the fuel parameters.

  1. Isotopic evidence of natural uranium and spent fuel uranium releases into the environment.

    PubMed

    Pourcelot, L; Boulet, B; Le Corre, C; Loyen, J; Fayolle, C; Tournieux, D; Van Hecke, W; Martinez, B; Petit, J

    2011-02-01

    Uranium and plutonium isotopes were measured in soils, sediments and waters in an area subject to the past and present discharges from the uranium conversion plant of Malvési (France). The isotopes (236)U and (239)Pu are well known activation products of uranium and they prove to be powerful tracers of spent fuel releases in soils and sediments. On the other hand (234)U and (238)U activities measured in waters can be used to distinguish between releases and background uranium sources. Such findings contribute to improve the monitoring of the actinides releases by nuclear fuel facilities (mining sites, conversion, enrichment and fuel plants, reprocessing plants).

  2. Spent fuel sabotage test program, characterization of aerosol dispersal : interim final report.

    SciTech Connect

    Gregson, Michael Warren; Brockmann, John E.; Loiseau, Olivier; Klennert, Lindsay A.; Nolte, Oliver; Molecke, Martin Alan; Autrusson, Bruno A.; Koch, Wolfgang; Pretzsch, Gunter Guido; Brucher, Wenzel; Steyskal, Michele D.

    2008-03-01

    This multinational, multi-phase spent fuel sabotage test program is quantifying the aerosol particles produced when the products of a high energy density device (HEDD) interact with and explosively particulate test rodlets that contain pellets of either surrogate materials or actual spent fuel. This program provides source-term data that are relevant to plausible sabotage scenarios in relation to spent fuel transport and storage casks and associated risk assessments. We present details and significant results obtained from this program from 2001 through 2007. Measured aerosol results include: respirable fractions produced; amounts, nuclide content, and produced particle size distributions and morphology; measurements of volatile fission product species enhanced sorption--enrichment factors onto respirable particles; and, status on determination of the spent fuel ratio, SFR, needed for scaling studies. Emphasis is provided on recent Phase 3 tests using depleted uranium oxide pellets plus non-radioactive fission product dopants in surrogate spent fuel test rodlets, plus the latest surrogate cerium oxide results and aerosol laboratory supporting calibration work. The DUO{sub 2}, CeO{sub 2}, plus fission product dopant aerosol particle results are compared with available historical data. We also provide a status review on continuing preparations for the final Phase 4 in this program, tests using individual short rodlets containing actual spent fuel from U.S. PWR reactors, with both high- and lower-burnup fuel. The source-term data, aerosol results, and program design have been tailored to support and guide follow-on computer modeling of aerosol dispersal hazards and radiological consequence assessments. This spent fuel sabotage, aerosol test program was performed primarily at Sandia National Laboratories, with support provided by both the U.S. Department of Energy and the Nuclear Regulatory Commission. This program has significant input from, and is cooperatively

  3. Using X-ray, K-edge densitometry in spent fuel characterization

    SciTech Connect

    Jensen, T.; Aljundi, T.; Gray, J.N.

    1998-06-01

    There are instances where records for spent nuclear fuel are incomplete, as well as cases where fuel assemblies have deteriorated during storage. To bring these materials into compliance for long term storage will require determination of parameters such as enrichment, total fissionable material, and burnup. To obtain accurate estimates of these parameters will require the combination of information from different inspection techniques. A method which can provide an accurate measure of the total uranium in the spent fuel is X-ray K-edge densitometry. To assess the potential for applying this method in spent fuel characterization, the authors have measured the amount of uranium in stacks of reactor fuel plates containing nuclear materials of different enrichments and alloys. They have obtained good agreement with expected uranium concentrations ranging from 60 mg/cm{sup 2} to 3,000 mg/cm{sup 2}, and have demonstrated that these measurements can be made in a high radiation field (> 200 mR/hr).

  4. Determination of BWR Spent Nuclear Fuel Assembly Effective Thermal Conductivity

    SciTech Connect

    Matthew D. Hinds

    2001-10-17

    The purpose of this calculation is to provide an effective thermal conductivity for use in predicting peak cladding temperatures in boiling water reactor (BWR) fuel assemblies with 7x7,8x8, and 9x9 rod arrays. The first objective of this calculation is to describe the development and application of a finite element representation that predicts peak spent nuclear fuel temperatures for BWR assemblies. The second objective is to use the discrete representation to develop a basis for determining an effective thermal conductivity (described later) for a BWR assembly with srneared/homogeneous properties and to investigate the thermal behavior of a spent fuel assembly. The scope of this calculation is limited to a steady-state two-dimensional representation of the waste package interior region. This calculation is subject to procedure AP-3.124, Calculations (Ref. 27) and guided by the applicable technical work plan (Ref. 14). While these evaluations were originally developed for the thermal analysis of conceptual waste package designs emplaced in the potential repository at Yucca Mountain, the methodology applies to storage and transportation thermal analyses as well. Note that the waste package sketch in Attachment V depicts a preliminary design, and should not be interpreted otherwise.

  5. Storage of LWR (light-water-reactor) spent fuel in air

    SciTech Connect

    Thomas, L.E.; Charlot, L.A.; Coleman, J.E. ); Knoll, R.W. )

    1989-12-01

    An experimental program is being conducted at Pacific Northwest Laboratory (PNL) to determine the oxidation response of light-water-reactor (LWR) spent fuels under conditions appropriate to fuel storage in air. The program is designed to investigate several independent variables that might affect the oxidation behavior of spent fuel. Included are temperature (135 to 230{degree}C), fuel burnup (to about 34 MWd/kgM), reactor type (pressurized and boiling water reactors), moisture level in the air, and the presence of a high gamma field. In continuing tests with declad spent fuel and nonirradiated UO{sub 2} specimens, oxidation rates were monitored by weight-gain measurements and the microstructures of subsamples taken during the weighing intervals were characterized by several analytical methods. The oxidation behavior indicated by weight gain and time to form powder will be reported in Volume III of this series. The characterization results obtained from x-ray diffractometry, transmission electron microscopy, scanning electron microscopy, and Auger electron spectrometry of oxidized fuel samples are presented in this report. 28 refs., 21 figs., 3 tabs.

  6. A Non-Proliferating Fuel Cycle: No Enrichment, Reprocessing or Accessible Spent Fuel - 12375

    SciTech Connect

    Parker, Frank L.

    2012-07-01

    Current fuel cycles offer a number of opportunities for access to plutonium, opportunities to create highly enriched uranium and access highly radioactive wastes to create nuclear weapons and 'dirty' bombs. The non-proliferating fuel cycle however eliminates or reduces such opportunities and access by eliminating the mining, milling and enrichment of uranium. The non-proliferating fuel cycle also reduces the production of plutonium per unit of energy created, eliminates reprocessing and the separation of plutonium from the spent fuel and the creation of a stream of high-level waste. It further simplifies the search for land based deep geologic repositories and interim storage sites for spent fuel in the USA by disposing of the spent fuel in deep sub-seabed sediments after storing the spent fuel at U.S. Navy Nuclear Shipyards that have the space and all of the necessary equipment and security already in place. The non-proliferating fuel cycle also reduces transportation risks by utilizing barges for the collection of spent fuel and transport to the Navy shipyards and specially designed ships to take the spent fuel to designated disposal sites at sea and to dispose of them there in deep sub-seabed sediments. Disposal in the sub-seabed sediments practically eliminates human intrusion. Potential disposal sites include Great Meteor East and Southern Nares Abyssal Plain. Such sites then could easily become international disposal sites since they occur in the open ocean. It also reduces the level of human exposure in case of failure because of the large physical and chemical dilution and the elimination of a major pathway to man-seawater is not potable. Of course, the recovery of uranium from sea water and the disposal of spent fuel in sub-seabed sediments must be proven on an industrial scale. All other technologies are already operating on an industrial scale. If externalities, such as reduced terrorist threats, environmental damage (including embedded emissions), long

  7. The shutdown reactor: Optimizing spent fuel storage cost

    SciTech Connect

    Pennington, C.W.

    1995-12-31

    Several studies have indicated that the most prudent way to store fuel at a shutdown reactor site safely and economically is through the use of a dry storage facility licensed under 10CFR72. While such storage is certainly safe, is it true that the dry ISFSI represents the safest and most economical approach for the utility? While no one is really able to answer that question definitely, as yet, Holtec has studied this issue for some time and believes that both an economic and safety case can be made for an optimization strategy that calls for the use of both wet and dry ISFSI storage of spent fuel at some plants. For the sake of brevity, this paper summarizes some of Holtec`s findings with respect to the economics of maintaining some fuel in wet storage at a shutdown reactor. The safety issue, or more importantly the perception of safety of spent fuel in wet storage, still varies too much with the eye of the beholder, and until a more rigorous presentation of safety analyses can be made in a regulatory setting, it is not practically useful to argue about how many angels can sit on the head of a safety-related pin. Holtec is prepared to present such analyses, but this does not appear to be the proper venue. Thus, this paper simply looks at certain economic elements of a wet ISFSI at a shutdown reactor to make a prima facie case that wet storage has some attractiveness at a shutdown reactor and should not be rejected out of hand. Indeed, an optimization study at certain plants may well show the economic vitality of keeping some fuel in the pool and converting the NRC licensing coverage from 10CFR50 to 10CFR72. If the economics look attractive, then the safety issue may be confronted with a compelling interest.

  8. Differential die-away technique for determination of the fissile contents in spent fuel assembly

    SciTech Connect

    Lee, Tachoon; Menlove, Howard O; Swinhoe, Nartyn T; Tobin, Stephen J

    2010-01-01

    Monte Carlo simulations were performed for the differential die-away (DDA) technique to quantify its capability to measure the fissile contents in spent fuel assemblies of 64 different cases in terms of initial enrichment, burnup, and cooling time. The DDA count rate varies according to the contents of fissile isotopes such as {sup 235}U, {sup 239}Pu, and {sup 241}Pu contained in the spent fuel assembly. The effective {sup 239}Pu concept was introduced to quantify the total fissile mass of spent fuel by weighting the relative signal contributions of {sup 235}U and {sup 241}Pu compared to that of {sup 239}Pu. The Monte Carlo simulation results show that the count rate of the DDA instrument for a spent fuel assembly of 4% initial enrichment, 45 GWD/MTU burnup, and 5 year cooling time is {approx} 9.8 x 10{sup 4} counts per second (c/s) with the 100-Hz repeated interrogation pattern of 0 to 10 {micro}s interrogation, 0.2 ms to 1 ms counting time, and 1 x 10{sup 9} n/s neutron source. The {sup 244}Cm neutron background count rate for this counting time scheme is {approx} 1 x 10{sup 4} c/s, and thus the signal to background ratio is {approx}10.

  9. Smelting Associated with the Advanced Spent Fuel Conditioning Process

    SciTech Connect

    Hur, J-M.; Jeong, M-S.; Lee, W-K.; Cho, S-H.; Seo, C-S.; Park, S-W.

    2004-10-03

    The smelting process associated with the advanced spent fuel conditioning process (ACP) of Korea Atomic Energy Research Institute was studied by using surrogate materials. Considering the vaporization behaviors of input materials, the operation procedure of smelting was set up as (1) removal of residual salts, (2) melting of metal powder, and (3) removal of dross from a metal ingot. The behaviors of porous MgO crucible during smelting were tested and the chemical stability of MgO in the salt-being atmosphere was confirmed.

  10. Corrosion of Spent Nuclear Fuel: The Long-Term Assessment

    SciTech Connect

    Rodney C. Ewing

    2004-10-07

    Spent nuclear fuel, essentially U{sub 2}, accounts for over 95% of the total radioactivity of all of the radioactive wastes in the United States that require disposal, disposition or remediation. The UO{sub 2} in SNF is not stable under oxiding conditions and may also be altered under reducing conditions. The alteration of SNF results in the formation of new uranium phases that can cause the release or retardation of actinide and fission product radionuclides. Over the long term, and depending on the extent to which the secondary uranium phases incorporate fission products and actinides, these alteration phases become the near-field source term.

  11. Closure Mechanism and Method for Spent Nuclear Fuel Canisters

    SciTech Connect

    Doman, Marvin J.

    2004-11-23

    A canister is provided for storing, transporting, and/or disposing of spent nuclear fuel. The canister includes a canister shell, a top shield plug disposed within the canister, and a leak-tight closure arrangement. The closure arrangement includes a shear ring which forms a containment boundary of the canister, and which is welded to the canister shell and top shield plug. An outer seal plate, forming an outer seal, is disposed above the shear ring and is welded to the shield plug and the canister.

  12. Contaminated sediment removal from a spent fuel storage canal

    SciTech Connect

    Geber, K R

    1993-01-01

    A leaking underground spent fuel transfer canal between a decommissioned reactor and a radiochemical separations building at the Oak Ridge National Laboratory (ORNL) was found to contain RCRA-hazardous and radioactive sediment. Closure of the Part B RCRA permitted facility required the use of an underwater robotic vacuum and a filtration-containment system to separate and stabilize the contaminated sediment. This paper discusses the radiological controls established to maintain contamination and exposures As Low As Reasonably Achievable (ALARA) during the sediment removal.

  13. Radiochemical Assays of Irradiated VVER-440 Fuel for Use in Spent Fuel Burnup Credit Activities

    SciTech Connect

    Jardine, L J

    2005-04-25

    The objective of this spent fuel burnup credit work was to study and describe a VVER-440 reactor spent fuel assembly (FA) initial state before irradiation, its operational irradiation history and the resulting radionuclide distribution in the fuel assembly after irradiation. This work includes the following stages: (1) to pick out and select a specific spent (irradiated) FA for examination; (2) to describe the FA initial state before irradiation; (3) to describe the irradiation history, including thermal calculations; (4) to examine the burnup distribution of select radionuclides along the FA height and cross-section; (5) to examine the radionuclide distributions; (6) to determine the Kr-85 release into the plenum; (7) to select and prepare FA rod specimens for destructive examinations; (8) to determine the radionuclide compositions, isotope masses and burnup in the rod specimens; and (9) to analyze, document and process the results. The specific workscope included the destructive assay (DA) of spent fuel assembly rod segments with an {approx}38.5 MWd/KgU burnup from a single VVER-440 fuel assembly from the Novovorenezh reactor in Russia. Based on irradiation history criteria, four rods from the fuel assembly were selected and removed from the assembly for examination. Next, 8 sections were cut from the four rods and sent for destructive analysis of radionuclides by radiochemical analyses. The results were documented in a series of seven reports over a period of {approx}1 1/2 years.

  14. Study on Gaseous Effluent Treatment for Dissolution Step of Spent Nuclear Fuel Reprocessing

    SciTech Connect

    Mineo, H.; Iizuka, M.; Fujisaki, S.; Hotoku, S.; Asakura, T.; Uchiyama, G.

    2002-02-27

    Behavior of radioiodine and carbon-14 during spent fuel dissolution was studied in a bench-scale reprocessing test rig where 29 and 44 GWdt-1 spent fuels were respectively dissolved. Decontamination factor of AGS (silica-gel impregnated with silver nitrate) column for iodine-129 removal was measured to be more than 36,000. The measurement of iodine-129 profile in the adsorption column showed that the nuclide was effectively trapped by the adsorbent. Measurement of iodine-129 in the dissolver solution after the iodine-stripping operation using NO2 gas at 363 K, revealed that less than 0.57% of total iodine-129 generated, which was estimated by ORIGEN II calculation, was remained in the dissolver solution. Also, measurement of iodine-129 by an iodine-stripping operation from the dissolver solution using potassium iodate showed that another 2.72% of total iodine-129 precipitated as iodide. In addition, about 70 % of total iodine generated was measured in the AGS columns. Rest of iodine-129 was supposed to adsorb to a HEPA filter and the inner surface of dissolver off-gas lines. Those results on iodine-129 distribution were found to be almost identical to the results obtained in the study using iodine-131 as tracer and the results reported by other works. It was demonstrated that the two-steps iodine-stripping method using potassium iodate could expel additional iodine from the solution, more effectively than iodine-stripping operation using NO2 gas. Iodine-131 was also detected on the AGS columns at the spent fuel dissolution. Increasing burnup showed larger amount of iodine-131 since amount of curium-244 contained in the spent fuel increased with the burnup. Release of carbon-14 as carbon dioxide during dissolution was found to occur when the release of krypton-85. From the 14CO2 measurement, initial nitrogen-14 concentration in the fuel was estimated to be about several ppm, which was within the range reported.

  15. Determining plutonium mass in spent fuel using Cf-252 interrogation with prompt neutron detection

    SciTech Connect

    Hu, Jianwei; Tobin, Stephen J; Menlove, Howard O; Croft, Stephen

    2010-01-01

    {sup 252}Cf Interrogation with Prompt Neutron (CIPN) detection is proposed as one of 14 NDA techniques to determine Pu mass in spent fuel assemblies (FAs). CIPN is a low-cost and portable instrument, and it looks like a modified fork detector combined with an active interrogation source. Fission chamber (FC) is chosen as neutron detector because of its insensitivity to {gamma} radiation. The CIPN assay is comprised of two measurements, a background count and an active count, without and with the {sup 252}Cf source next to the fuel respectively. The net signal above background is primarily due to the multiplication of Cf source neutrons caused by the fissile content. The capability of CIPN to detect diversion and to determine fissile content was quantified using MCNPX simulations. New schemes were proposed (such as burnup and cooling time correction, etc.) and the results show that the fissile content of a target spent fuel assembly can be determined using CIPN signal.

  16. Managing Spent Nuclear Fuel at the Idaho National Laboratory

    SciTech Connect

    Thomas Hill; Denzel L. Fillmore

    2005-10-01

    The Idaho National Laboratory (INL) has a large inventory of diverse types of spent nuclear fuel (SNF). This legacy derives from the history of the INL as the National Reactor Testing Station, and from its mission to recover HEU from SNF and to test and examine SNF after irradiation. The INL also has a large diversity of SNF storage facilities, some 50 years old. SNF at INL has many forms—from intact assemblies down to metallurgical mounts, and some fuel has been wet stored for over 40 years. SNF is stored bare or in metal cans under water, or dry in vaults, caissons or casks. Inspection shows varying corrosion and degradation of the SNF and its storage cans. SNF has been stored in 10 different facilities: 5 pools, one cask storage pad, one vault, two generations of caisson facilities, and one modular Independent Spent Fuel Storage Installation (ISFSI). The pools range in age from 40 years old to the most modern in the US Department of Energy (DOE) complex. The near-term objective is to move SNF from older pools to interim dry storage, allowing shutdown and decommissioning of the older facilities. This move involves drying methods that are dependent on fuel type. The long-term objective is to have INL SNF in safe dry storage and ready to be shipped to the National Repository. The unique features of the INL SNF requires special treatments and packaging to meet the proposed repository acceptance criteria and SNF will be repackaged in standardized canisters for shipment and disposal in the National Repository. Disposal will use the standardized canisters that can be co-disposed with High Level Waste glass logs to limit the total fissile material in a repository waste package. The DOE standardized canister also simplifies the repository handling of the multitude of DOE SNF sizes and shapes.

  17. Fast Reactor Spent Fuel Processing: Experience and Criticality Safety

    SciTech Connect

    Chad Pope

    2007-05-01

    This paper discusses operational and criticality safety experience associated with the Idaho National Laboratory Fuel Conditioning Facility which uses a pyrometallurgical process to treat spent fast reactor metallic fuel. The process is conducted in an inert atmosphere hot cell. The process starts with chopping metallic fuel elements into a basket. The basket is lowered into molten salt (LiCl-KCl) along with a steel mandrel. Active metal fission products, transuranic metals and sodium metal in the spent fuel undergo chemical oxidation and form chlorides. Voltage is applied between the basket, which serves as an anode, and the mandrel, which serves as a cathode, causing metallic uranium in the spent fuel to undergo electro-chemical oxidation thereby forming uranium chloride. Simultaneously at the cathode, uranium chloride undergoes electro-chemical reduction and deposits uranium metal onto the mandrel. The uranium metal and accompanying entrained salt are placed in a distillation furnace where the uranium melts forming an ingot and the entrained salt boils and subsequently condenses in a separate crucible. The uranium ingots are placed in long term storage. During the ten year operating history, over one hundred criticality safety evaluations were prepared. All criticality safety related limits and controls for the entire process are contained in a single document which required over thirty revisions to accommodate the process changes. Operational implementation of the limits and controls includes use of a near real-time computerized tracking system. The tracking system uses an Oracle database coupled with numerous software applications. The computerized tracking system includes direct fuel handler interaction with every movement of material. Improvements to this system during the ten year history include introduction of web based operator interaction, tracking of moderator materials and the development of a plethora database queries to assist in day to day

  18. Study of Compton suppression for use in spent nuclear fuel assay

    NASA Astrophysics Data System (ADS)

    Bender, Sarah

    The focus of this study has been to assess Compton suppressed gamma-ray detection systems for the multivariate analysis of spent nuclear fuel. This objective has been achieved using direct measurement of samples of irradiated fuel elements in two geometrical configurations with Compton suppression systems. In order to address the objective to quantify the number of additionally resolvable photopeaks, direct Compton suppressed spectroscopic measurements of spent nuclear fuel in two configurations were performed: as intact fuel elements and as dissolved feed solutions. These measurements directly assessed and quantified the differences in measured gamma-ray spectrum from the application of Compton suppression. Several irradiated fuel elements of varying cooling time from the Penn State Breazeale Reactor spent fuel inventory were measured using three Compton suppression systems that utilized different primary detectors: HPGe, LaBr3, and NaI(Tl). The application of Compton suppression using a LaBr3 primary detector to the measurement of the current core fuel element, which presented the highest count rate, allowed four additional spectral features to be resolved. In comparison, the HPGe-CSS was able to resolve eight additional photopeaks as compared to the standalone HPGe measurement. Measurements with the NaI(Tl) primary detector were unable to resolve any additional peaks, due to its relatively low resolution. Samples of Approved Test Material (ATM) commercial fuel elements were obtained from Pacific Northwest National Laboratory. The samples had been processed using the beginning stages of the PUREX method and represented the unseparated feed solution from a reprocessing facility. Compton suppressed measurements of the ATM fuel samples were recorded inside the guard detector annulus, to simulate the siphoning of small quantities from the main process stream for long dwell measurement periods. Photopeak losses were observed in the measurements of the dissolved ATM

  19. Spent fuel and high-level radioactive waste transportation report

    SciTech Connect

    Not Available

    1989-11-01

    This publication is intended to provide its readers with an introduction to the issues surrounding the subject of transportation of spent nuclear fuel and high-level radioactive waste, especially as those issues impact the southern region of the United States. It was originally issued by the Southern States Energy Board (SSEB) in July 1987 as the Spent Nuclear Fuel and High-Level Radioactive Waste Transportation Primer, a document patterned on work performed by the Western Interstate Energy Board and designed as a ``comprehensive overview of the issues.`` This work differs from that earlier effort in that it is designed for the educated layman with little or no background in nuclear waste issues. In addition, this document is not a comprehensive examination of nuclear waste issues but should instead serve as a general introduction to the subject. Owing to changes in the nuclear waste management system, program activities by the US Department of Energy and other federal agencies and developing technologies, much of this information is dated quickly. While this report uses the most recent data available, readers should keep in mind that some of the material is subject to rapid change. SSEB plans periodic updates in the future to account for changes in the program. Replacement pages sew be supplied to all parties in receipt of this publication provided they remain on the SSEB mailing list.

  20. Spent nuclear fuel recycling with plasma reduction and etching

    DOEpatents

    Kim, Yong Ho

    2012-06-05

    A method of extracting uranium from spent nuclear fuel (SNF) particles is disclosed. Spent nuclear fuel (SNF) (containing oxides of uranium, oxides of fission products (FP) and oxides of transuranic (TRU) elements (including plutonium)) are subjected to a hydrogen plasma and a fluorine plasma. The hydrogen plasma reduces the uranium and plutonium oxides from their oxide state. The fluorine plasma etches the SNF metals to form UF6 and PuF4. During subjection of the SNF particles to the fluorine plasma, the temperature is maintained in the range of 1200-2000 deg K to: a) allow any PuF6 (gas) that is formed to decompose back to PuF4 (solid), and b) to maintain stability of the UF6. Uranium (in the form of gaseous UF6) is easily extracted and separated from the plutonium (in the form of solid PuF4). The use of plasmas instead of high temperature reactors or flames mitigates the high temperature corrosive atmosphere and the production of PuF6 (as a final product). Use of plasmas provide faster reaction rates, greater control over the individual electron and ion temperatures, and allow the use of CF4 or NF3 as the fluorine sources instead of F2 or HF.

  1. Spent fuel and high-level radioactive waste transportation report

    SciTech Connect

    Not Available

    1990-11-01

    This publication is intended to provide its readers with an introduction to the issues surrounding the subject of transportation of spent nuclear fuel and high-level radioactive waste, especially as those issues impact the southern region of the United States. It was originally issued by the Southern States Energy Board (SSEB) in July 1987 as the Spent Nuclear Fuel and High-Level Radioactive Waste Transportation Primer, a document patterned on work performed by the Western Interstate Energy Board and designed as a ``comprehensive overview of the issues.`` This work differs from that earlier effort in that it is designed for the educated layman with little or no background in nuclear waste issues. In addition, this document is not a comprehensive examination of nuclear waste issues but should instead serve as a general introduction to the subject. Owing to changes in the nuclear waste management system, program activities by the US Department of Energy and other federal agencies and developing technologies, much of this information is dated quickly. While this report uses the most recent data available, readers should keep in mind that some of the material is subject to rapid change. SSEB plans periodic updates in the future to account for changes in the program. Replacement pages will be supplied to all parties in receipt of this publication provided they remain on the SSEB mailing list.

  2. Thermal hydraulic feasibility assessment for the Spent Nuclear Fuel Project

    SciTech Connect

    Heard, F.J.; Cramer, E.R.; Beaver, T.R.; Thurgood, M.J.

    1996-01-01

    A series of scoping analyses have been completed investigating the thermal-hydraulic performance and feasibility of the Spent Nuclear Fuel Project (SNFP) Integrated Process Strategy (IPS). The SNFP was established to develop engineered solutions for the expedited removal, stabilization, and storage of spent nuclear fuel from the K Basins at the U.S. Department of Energy`s Hanford Site in Richland, Washington. The subject efforts focused on independently investigating, quantifying, and establishing the governing heat production and removal mechanisms for each of the IPS operations and configurations, obtaining preliminary results for comparison with and verification of other analyses, and providing technology-based recommendations for consideration and incorporation into the design bases for the SNFP. The goal was to develop a series fo thermal-hydraulic models that could respond to all process and safety-related issues that may arise pertaining to the SNFP. A series of sensitivity analyses were also performed to help identify those parameters that have the greatest impact on energy transfer and hence, temperature control. It is anticipated that the subject thermal-hydraulic models will form the basis for a series of advanced and more detailed models that will more accurately reflect the thermal performance of the IPS and alleviate the necessity for some of the more conservative assumptions and oversimplifications, as well as form the basis for the final process and safety analyses.

  3. Spent Fuel and High-Level Radioactive Waste Transportation Report

    SciTech Connect

    Not Available

    1992-03-01

    This publication is intended to provide its readers with an introduction to the issues surrounding the subject of transportation of spent nuclear fuel and high-level radioactive waste, especially as those issues impact the southern region of the United States. It was originally issued by SSEB in July 1987 as the Spent Nuclear Fuel and High-Level Radioactive Waste Transportation Primer, a document patterned on work performed by the Western Interstate Energy Board and designed as a ``comprehensive overview of the issues.`` This work differs from that earlier effort in that it is designed for the educated layman with little or no background in nuclear waste Issues. In addition. this document is not a comprehensive examination of nuclear waste issues but should instead serve as a general introduction to the subject. Owing to changes in the nuclear waste management system, program activities by the US Department of Energy and other federal agencies and developing technologies, much of this information is dated quickly. While this report uses the most recent data available, readers should keep in mind that some of the material is subject to rapid change. SSEB plans periodic updates in the future to account for changes in the program. Replacement pages will be supplied to all parties in receipt of this publication provided they remain on the SSEB mailing list.

  4. Increase of inherent protection level in spent nuclear fuel

    SciTech Connect

    Krasnobaev, A.; Kryuchkov, E.; Glebov, V.

    2006-07-01

    The paper is devoted to upgrading inherent proliferation protection of fissionable nuclear materials (FNM). Some possibilities were investigated to form high radiation barrier inside spent fuel assemblies (SFA) discharged from power reactors of VVER-1000 type and research reactors of IRT type. The radiation barrier is estimated in the terms of rate of equivalent dose (RED) at 30-cm distance from SFA. The values of RED were calculated with application of the computer code package SCALE 4.3. The paper considers the criteria adopted for estimation of FNM proliferation resistance. The paper presents numerical results on a component-wise analysis of the radiation barrier in SFA from reactors of VVER-1000 and IRT type and on capability of various radionuclides to prolong action of the radiation barrier. Isotopic admixtures were selected and amounts of these admixtures were evaluated for significant prolongation of the radiation barrier action at the levels of the radiation standards used for estimation of FNM proliferation resistance. The paper considers vulnerability of the radiation barriers in respect to thermal processing of spent fuel. (authors)

  5. Utilization of TRISO Fuel with LWR Spent Fuel in Fusion-Fission Hybrid Reactor System

    NASA Astrophysics Data System (ADS)

    Acır, Adem; Altunok, Taner

    2010-10-01

    HTRs use a high performance particulate TRISO fuel with ceramic multi-layer coatings due to the high burn up capability and very neutronic performance. TRISO fuel because of capable of high burn up and very neutronic performance is conducted in a D-T fusion driven hybrid reactor. In this study, TRISO fuels particles are imbedded body-centered cubic (BCC) in a graphite matrix with a volume fraction of 68%. The neutronic effect of TRISO coated LWR spent fuel in the fuel rod used hybrid reactor on the fuel performance has been investigated for Flibe, Flinabe and Li20Sn80 coolants. The reactor operation time with the different first neutron wall loads is 24 months. Neutron transport calculations are evaluated by using XSDRNPM/SCALE 5 codes with 238 group cross section library. The effect of TRISO coated LWR spent fuel in the fuel rod used hybrid reactor on tritium breeding (TBR), energy multiplication (M), fissile fuel breeding, average burn up values are comparatively investigated. It is shown that the high burn up can be achieved with TRISO fuel in the hybrid reactor.

  6. Spent fuel sabotage test program, characterization of aerosol dispersal : technical review and analysis supplement.

    SciTech Connect

    Durbin, Samuel G.; Lindgren, Eric Richard

    2009-07-01

    This project seeks to provide vital data required to assess the consequences of a terrorist attack on a spent fuel transportation cask. One such attack scenario involves the use of conical shaped charges (CSC), which are capable of damaging a spent fuel transportation cask. In the event of such an attack, the amount of radioactivity that may be released as respirable aerosols is not known with great certainty. Research to date has focused on measuring the aerosol release from single short surrogate fuel rodlets subjected to attack by a small CSC device in various aerosol chamber designs. The last series of three experiments tested surrogate fuel rodlets made with depleted uranium oxide ceramic pellets in a specially designed double chamber aerosol containment apparatus. This robust testing apparatus was designed to prevent any radioactive release and allow high level radioactive waste disposal of the entire apparatus following testing of actual spent fuel rodlets as proposed. DOE and Sandia reviews of the project to date identified a number of issues. The purpose of this supplemental report is to address and document the DOE review comments and to resolve the issues identified in the Sandia technical review.

  7. Cosmic ray muon computed tomography of spent nuclear fuel in dry storage casks

    DOE PAGES

    Poulson, Daniel Cris; Durham, J. Matthew; Guardincerri, Elena; ...

    2017-10-22

    Radiography with cosmic ray muon scattering has proven to be a successful method of imaging nuclear material through heavy shielding. Of particular interest is monitoring dry storage casks for diversion of plutonium contained in spent reactor fuel. Using muon tracking detectors that surround a cylindrical cask, cosmic ray muon scattering can be simultaneously measured from all azimuthal angles, giving complete tomographic coverage of the cask interior. This article describes the first application of filtered back projection algorithms, typically used in medical imaging, to cosmic ray muon scattering imaging. The specific application to monitoring spent nuclear fuel in dry storage casksmore » is investigated via GEANT4 simulations. With a cylindrical muon tracking detector surrounding a typical spent fuel cask, simulations indicate that missing fuel bundles can be detected with a statistical significance of ~18σ in less than two days exposure and a sensitivity at 1σ to a 5% missing portion of a fuel bundle. Finally, we discuss potential detector technologies and geometries.« less

  8. 78 FR 40199 - Draft Spent Fuel Storage and Transportation Interim Staff Guidance

    Federal Register 2010, 2011, 2012, 2013, 2014

    2013-07-03

    ... COMMISSION Draft Spent Fuel Storage and Transportation Interim Staff Guidance AGENCY: Nuclear Regulatory... Regulatory Commission (NRC) requests public comment on Draft Spent Fuel Storage and Transportation Interim... Integrity for Continued Storage of High Burnup Fuel Beyond 20 Years.'' The draft SFST-ISG provides...

  9. Optimization of the Spent Fuel Attribute Tester using radiation transport calculations

    SciTech Connect

    Laub, T.W.; Dupree, S.A.; Arlt, R.

    1993-07-01

    The International Atomic Energy Agency uses the Spent Fuel Attribute Tester (SFAT) to measure gamma signatures from fuel assemblies stored in spent fuel pools. It consists of a shielded, collimated NaI(Tl) detector attached to an air-filled pipe. The purpose of the present study was to define design changes, within operational constraints, that would improve the target assembly {sup 137}Cs signal relative to the background signals from adjacent assemblies. This improvement is essential to reducing to an acceptable level the measurement time during an inspection. Monte Carlo calculations of the entire geometry were impractical, therefore, a hybrid method was developed that combined one-dimensional discrete ordinates models of the spent fuel pool, three-dimensional Monte Carlo calculations of the SFAT, and detector response calculations. The method compared well with measurements taken with the existing baseline SFAT. Calculations predicted significant improvements in signal-to-noise ratio. Recommended changes included shortening the pipe and increasing its wall thickness, placing low-Z filters in the crystal line of sight, reducing the thickness of shielding around the collimator aperture and adding shielding around the crystal, and reducing the diameter of the crystal. An instrument incorporating these design changes is being fabricated in Finland and will be tested this year.

  10. Sustainability Considerations in Spent Light-water Nuclear Fuel Retrievability

    SciTech Connect

    Wood, Thomas W.; Rothwell, Geoffrey

    2012-01-10

    This paper examines long-term cost differences between two competing Light Water Reactor (LWR) fuels: Uranium Oxide (UOX) and Mixed Uranium Oxide-Plutonium Oxide (MOX). Since these costs are calculated on a life-cycle basis, expected savings from lower future MOX fuel prices can be used to value the option of substituting MOX for UOX, including the value of maintaining access to the used UOX fuel that could be reprocessed to make MOX. The two most influential cost drivers are the price of natural uranium and the cost of reprocessing. Significant and sustained reductions in reprocessing costs and/or sustained increases in uranium prices are required to give positive value to the retrievability of Spent Nuclear Fuel. While this option has positive economic value, it might not be exercised for 50 to 200 years. Therefore, there are many years for a program during which reprocessing technology can be researched, developed, demonstrated, and deployed. Further research is required to determine whether the cost of such a program would yield positive net present value and/or increases the sustainability of LWR energy systems.

  11. Spent fuel drying system test results (first dry-run)

    SciTech Connect

    Klinger, G.S.; Oliver, B.M.; Abrefah, J.; Marschman, S.C.; MacFarlan, P.J.; Ritter, G.A.

    1998-07-01

    The water-filled K-Basins in the Hanford 100 Area have been used to store N-Reactor spent nuclear fuel (SNF) since the 1970s. Because some leaks in the basin have been detected and some of the fuel is breached due to handling damage and corrosion, efforts are underway to remove the fuel elements from wet storage. An Integrated Process Strategy (IPS) has been developed to package, dry, transport, and store these metallic uranium fuel elements in an interim storage facility on the Hanford Site. Information required to support the development of the drying processes, and the required safety analyses, is being obtained from characterization tests conducted on fuel elements removed from the K-Basins. A series of whole element drying tests (reported in separate documents, see Section 7.0) have been conducted by Pacific Northwest National Laboratory (PNNL) on several intact and damaged fuel elements recovered from both the K-East and K-West Basins. This report documents the results of the first dry-run test, which was conducted without a fuel element. The empty test apparatus was subjected to a combination of low- and high-temperature vacuum drying treatments that were intended to mimic, wherever possible, the fuel treatment strategies of the IPS. The data from this dry-run test can serve as a baseline for the first two fuel element tests, 1990 (Run 1) and 3128W (Run 2). The purpose of this dry-run was to establish the background levels of hydrogen in the system, and the hydrogen generation and release characteristics attributable to the test system without a fuel element present. This test also serves to establish the background levels of water in the system and the water release characteristics. The system used for the drying test series was the Whole Element Furnace Testing System, described in Section 2.0, which is located in the Postirradiation Testing Laboratory (PTL, 327 Building). The test conditions and methodology are given in section 3.0, and the experimental

  12. Hanford K Basins spent nuclear fuels project update

    SciTech Connect

    Hudson, F.G.

    1997-10-17

    Twenty one hundred metric tons of spent nuclear fuel are stored in two concrete pools on the Hanford Site, known as the K Basins, near the Columbia River. The deteriorating conditions of the fuel and the basins provide engineering and management challenges to assure safe current and future storage. DE and S Hanford, Inc., part of the Fluor Daniel Hanford, Inc. lead team on the Project Hanford Management Contract, is constructing facilities and systems to move the fuel from current wet pool storage to a dry interim storage facility away from the Columbia River, and to treat and dispose of K Basins sludge, debris and water. The process starts in the K Basins where fuel elements will be removed from existing canisters, washed, and separated from sludge and scrap fuel pieces. Fuel elements will be placed in baskets and loaded into Multi-Canister Overpacks (MCOs) and into transportation casks. The MCO and cask will be transported into the Cold Vacuum Drying Facility, where free water within the MCO will be removed under vacuum at slightly elevated temperatures. The MCOs will be sealed and transported via the transport cask to the Canister Storage Building (CSB) in the 200 Area for staging prior to hot conditioning. The conditioning step to remove chemically bound water is performed by holding the MCO at 300 C under vacuum. This step is necessary to prevent excessive pressure buildup during interim storage that could be caused by corrosion. After conditioning, MCOs will remain in the CSB for interim storage until a national repository is completed.

  13. Photon dose rates from spent fuel assemblies with relation to self-protection (Rev. 1)

    SciTech Connect

    Pond, R.B.; Matos, J.E.

    1996-02-01

    Photon dose rates as a function of fission product decay times have been calculated for spent fuel assemblies typical of MTR-type research and test reactors. Based upon these dose rates, the length of time that a spent fuel assembly will be self-protecting (dose rate greater than 100 rem/h at 1 m in air) can be estimated knowing the mass of fuel burned, the fraction of fuel burned, and the fuel assembly specific power density.

  14. Non-destructive assay of spent nuclear fuel using passive neutron Albedo reactivity

    SciTech Connect

    Evans, L G; Schear, M A; Croft, S; Tobin, S J; Swinhoe, M T; Menlove, H O

    2010-01-01

    Passive Neutron Albedo Reactivity (PNAR) is one of fourteen techniques that has been researched and evaluated to form part of a comprehensive and integrated detection system for the non-destructive assay (NDA) of spent nuclear fuel. PNAR implemented with {sup 3}He tubes for neutron detection (PNAR-{sup 3}He) is the measurement of time correlated neutrons from a spent fuel assembly with and without a Cadmium (Cd) layer surrounding the assembly. PNAR utilizes the self-interrogation of the fuel via reflection of neutrons born in the fuel assembly back in to the fuel assembly. The neutrons originate primarily from spontaneous fission events within the fuel itself (Curium-244) but are amplified by multiplication. The presence and removal of the Cd provides two measurement conditions with different neutron energy spectra and therefore different interrogating neutron characteristics. Cd has a high cross-section of absorption for slow neutrons and therefore greatly reduces the low energy (thermal) neutron fluence rate returning. The ratios of the Singles, Doubles and Triples count rates obtained in each case are known as the Cd ratios, which are related to fissile content. A potential safeguards application for which PNAR-{sup 3}He is particularly suited is 'fingerprinting'. Fingerprinting could function as an alternative to plutonium (Pu) mass determination; providing confidence that material was not diverted during transport between sites. PNAR-{sup 3}He has six primary NDA signatures: Singles, Doubles and Triples count rates measured with two energy spectra at both shipping and receiving sites. This is to uniquely identify the fuel assembly, and confirm no changes have taken place during transport. Changes may indicate all attempt to divert material for example. Here, the physics of the PNAR-{sup 3}He concept will be explained, alongside a discussion on the development of a prototypical PNAR-{sup 3}He instrument using simulation. The capabilities and performance of the

  15. Spent fuel handling system for a geologic storage test at the Nevada Test Site

    SciTech Connect

    Duncan, J.E.; House, P.A.; Wright, G.W.

    1980-05-01

    The Lawrence Livermore Laboratory is conducting a test of the geologic storage of encapsulated spent commercial reactor fuel assemblies in a granitic rock at the Nevada Test Site. The test, known as the Spent Fuel Test-Climax (SFT-C), is sponsored by the US Department of Energy, Nevada Operations Office. Eleven pressurized-water-reactor spent fuel assemblies are stored retrievably for three to five years in a linear array in the Climax stock at a depth of 420 m.

  16. Spent Fuel NDA Research Path for the Sweden Encapsulation-Repository

    SciTech Connect

    Tobin, Stephen J.; Trellue, Holly R.; Liljenfeldt, Henrik

    2015-01-22

    This set of slides provides a description of research performed to date on spent fuel NDA: Next Generation Safeguards Initiative Spent Fuel Project, and NDA analysis and research planned for CLINK. The general purpose is strengthening the technical toolkit of safeguard inspectors. Data mining is being applied to determine the optimal mathematical structure to match the complexity of spent fuel NDA signals and to enable a range of quantities to be estimated.

  17. Nuclear mass inventory, photon dose rate and thermal decay heat of spent research reactor fuel assemblies

    SciTech Connect

    Pond, R.B.; Matos, J.E.

    1996-12-31

    This document has been prepared to assist research reactor operators possessing spent fuel containing enriched uranium of United States origin to prepare part of the documentation necessary to ship this fuel to the United States. Data are included on the nuclear mass inventory, photon dose rate, and thermal decay heat of spent research reactor fuel assemblies. Isotopic masses of U, Np, Pu and Am that are present in spent research reactor fuel are estimated for MTR, TRIGA and DIDO-type fuel assembly types. The isotopic masses of each fuel assembly type are given as functions of U-235 burnup in the spent fuel, and of initial U-235 enrichment and U-235 mass in the fuel assembly. Photon dose rates of spent MTR, TRIGA and DIDO-type fuel assemblies are estimated for fuel assemblies with up to 80% U-235 burnup and specific power densities between 0.089 and 2.857 MW/kg[sup 235]U, and for fission product decay times of up to 20 years. Thermal decay heat loads are estimated for spent fuel based upon the fuel assembly irradiation history (average assembly power vs. elapsed time) and the spent fuel cooling time.

  18. A Critical Review of Practice of Equating the Reactivity of Spent Fuel to Fresh Fuel in Burnup Credit Criticality Safety Analyses for PWR Spent Fuel Pool Storage

    SciTech Connect

    Wagner, J.C.; Parks, C.V.

    2000-09-01

    This research examines the practice of equating the reactivity of spent fuel to that of fresh fuel for the purpose of performing burnup credit criticality safety analyses for PWR spent fuel pool (SFP) storage conditions. The investigation consists of comparing k{sub inf} estimates based on reactivity equivalent fresh fuel enrichment (REFFE) to k{sub inf} estimates using the actual spent fuel isotopics. Analyses of selected storage configurations common in PWR SFPs show that this practice yields nonconservative results (on the order of a few tenths of a percent) in configurations in which the spent fuel is adjacent to higher-reactivity assemblies (e.g., fresh or lower-burned assemblies) and yields conservative results in configurations in which spent fuel is adjacent to lower-reactivity assemblies (e.g., higher-burned fuel or empty cells). When the REFFE is determined based on unborated water moderation, analyses for storage conditions with soluble boron present reveal significant nonconservative results associated with the use of the REFFE. This observation is considered to be important, especially considering the recent allowance of credit for soluble boron up to 5% in reactivity. Finally, it is shown that the practice of equating the reactivity of spent fuel to fresh fuel is acceptable, provided the conditions for which the REFFE was determined remain unchanged. Determination of the REFFE for a reference configuration and subsequent use of the REFFE for different configurations violates the basis used for the determination of the REFFE and, thus, may lead to inaccurate, and possibly, nonconservative estimates of reactivity. A significant concentration ({approximately}2000 ppm) of soluble boron is typically (but not necessarily required to be) present in PWR SFPs, of which only a portion ({le} 500 ppm) may be credited in safety analyses. Thus, a large subcritical margin currently exists that more than accounts for errors or uncertainties associated with the use of

  19. HIGH ENERGY DELAYED GAMMA SPECTROSCOPY FOR PLUTONIUM ASSAY OF SPENT REACTOR FUEL

    SciTech Connect

    Campbell, Luke W.; Smith, L. E.; Misner, Alex C.

    2011-07-18

    Nuclear safeguards requires accountancy of plutonium present in spent reactor fuels. Current non-destructive methods do not directly measure plutonium content but instead rely on indirect measurements that require operator declarations of the fuel history. Delayed gamma spectroscopy is one method being investigated which can overcome these limitations. Delayed gamma rays from fission depend on the isotopic fission yield of the fissile isotope, and thus can be used to fingerprint the isotopes undergoing fission. However, difficulties arise because of the intense background due to long lived fission radionuclides already present in the fuel. We report on progress on simulated measurements of the delayed gamma spectrum in the presence of this background, using neutrons from a D-T source thermalized in an interrogation chamber slipped over a fuel assembly. By focusing on delayed gammas in the 3 to 4 MeV range, the passive spectrum becomes negligible, while allowing the preferential attenuation of the passive background to acceptable levels.

  20. Determination of actinide and fission-product isotopes in very-high-burnup spent nuclear fuel.

    SciTech Connect

    Sullivan, V. S.; Bowers, D. L.; Clark, M. A.; Graczyk, D. G.; Tsai, Y.; Streets, W. E.; Vander Pol, M. H.; Billone, M. C.

    2008-07-01

    A work plan was desired that would produce data for a wide array of actinide and fission-product isotopes with reasonably good accuracy and relatively low cost. An analysis scheme involving a fairly small number of separations, dilutions, and measurement methods was used to generate information on 74 isotopes in two spent-fuel samples of >70 GWd/MTU burnup. Some of the measured isotopes are of high interest for burnup-credit evaluations and had not been reported previously for high-burnup fuels.

  1. Radio-toxicity of spent fuel of the advanced heavy water reactor.

    PubMed

    Anand, S; Singh, K D S; Sharma, V K

    2010-01-01

    The Advanced Heavy Water Reactor (AHWR) is a new power reactor concept being developed at Bhabha Atomic Research Centre, Mumbai. The reactor retains many desirable features of the existing Pressurised Heavy Water Reactor (PHWR), while incorporating new, advanced safety features. The reactor aims to utilise the vast thorium resources available in India. The reactor core will use plutonium as the make-up fuel, while breeding (233)U in situ. On account of this unique combination of fuel materials, the operational characteristics of the fuel as determined by its radioactivity, decay heat and radio-toxicity are being viewed with great interest. Radio-toxicity of the spent fuel is a measure of potential radiological hazard to the members of the public and also important from the ecological point of view. The radio-toxicity of the AHWR fuel is extremely high to start with, being approximately 10(4) times that of the fresh natural U fuel used in a PHWR, and continues to remain relatively high during operation and subsequent cooling. A unique feature of this fuel is the peak observed in its radio-toxicity at approximately 10(5) y of decay cooling. The delayed increase in fuel toxicity has been traced primarily to a build-up of (229)Th, (230)Th and (226)Ra. This phenomenon has been observed earlier for thorium-based fuels and is confirmed for the AHWR fuel. This paper presents radio-toxicity data for AHWR spent fuel up to a period of 10(6) y and the results are compared with the radio-toxicity of PHWR.

  2. Spent-Fuel Storage Facility Project. Progress report, June 1-September 30, 1979

    SciTech Connect

    Cobb, D.D.

    1980-06-01

    The Los Alamos Scientific Laboratory (LASL) safeguards groups (Q-1, Q-2, Q-3, Q-4, and Q-5) and the nuclear data group (T-2) are participating in the US Department of Energy Away-From-Reactor Spent-Fuel Storage Program. This report presents the status of the LASL Spent-Fuel Storage Facility Project being performed under the direction of Savannah River Laboratory. Four task areas are: concept development, spent-fuel assay, spent-fuel verification, and automated data-base management.

  3. Status of work at PNL supporting dry storage of spent fuel

    SciTech Connect

    Cunningham, M.E.; McKinnon, M.A.; Michener, T.E.; Thomas, L.E.; Thornhill, C.K.

    1993-01-01

    This report discusses three projects related to dry storage of light-water reactor spent fuel which are being conducted at Pacific Northwest Laboratory. Performance testing of six dry storage systems (four metal casks and two concrete storage systems) has been completed and results compiled. Two computer codes for predicting spent fuel and storage system thermal performance, COBRA-SFS and HYDRA-II, have been developed and have been reviewed by the US Nuclear Regulatory Commission. Air oxidation testing of spent fuel was conducted from 1984 through 1990 to obtain data to support recommendations of temperature-time limits for air dry storage of spent light-water reactor fuel.

  4. BWR Spent Nuclear Fuel Interfacial Bonding Efficiency Study

    SciTech Connect

    Wang, Jy-An John; Jiang, Hao

    2015-04-30

    The objective of this project is to perform a systematic study of spent nuclear fuel (SNF, also known as “used nuclear fuel” [UNF]) integrity under simulated transportation environments using the Cyclic Integrated Reversible-Bending Fatigue Tester (CIRFT) hot-cell testing technology developed at Oak Ridge National Laboratory (ORNL) in August 2013. Under Nuclear Regulatory Commission (NRC) sponsorship, ORNL completed four benchmark tests, four static tests, and twelve dynamic or cycle tests on H. B. Robinson (HBR) high burn-up (HBU) fuel. The clad of the HBR fuels was made of Zircaloy-4. Testing was continued in fiscal year (FY) 2014 using Department of Energy (DOE) funds. Additional CIRFT testing was conducted on three HBR rods; two specimens failed, and one specimen was tested to over 2.23 × 107 cycles without failing. The data analysis on all the HBR SNF rods demonstrated that it is necessary to characterize the fatigue life of the SNF rods in terms of (1) the curvature amplitude and (2) the maximum absolute of curvature extremes. The maximum extremes are significant because they signify the maximum tensile stress for the outer fiber of the bending rod. CIRFT testing has also addressed a large variation in hydrogen content on the HBR rods. While the load amplitude is the dominant factor that controls the fatigue life of bending rods, the hydrogen content also has an important effect on the lifetime attained at each load range tested. In FY 15, eleven SNF rod segments from the Limerick BWR were tested using the ORNL CIRFT equipment; one test under static conditions and ten tests under dynamic loading conditions. Under static unidirectional loading, a moment of 85 N·m was obtained at a maximum curvature of 4.0 m-1. The specimen did not show any sign of failure during three repeated loading cycles to a similar maximum curvature. Ten cyclic tests were conducted with amplitudes varying from 15.2 to 7.1 N·m. Failure was observed in nine of

  5. Reducing uncertainties affecting the assessment of the long-term corrosion behavior of spent nuclear fuel.

    PubMed

    Fanghänel, Thomas; Rondinella, Vincenzo V; Glatz, Jean-Paul; Wiss, Thierry; Wegen, Detlef H; Gouder, Thomas; Carbol, Paul; Serrano-Purroy, Daniel; Papaioannou, Dimitrios

    2013-04-01

    Reducing the uncertainties associated with extrapolation to very long term of corrosion data obtainable from laboratory tests on a relatively young spent nuclear fuel is a formidable challenge. In a geologic repository, spent nuclear fuel may come in contact with water tens or hundreds of thousands of years after repository closure. The corrosion behavior will depend on the fuel properties and on the conditions characterizing the near field surrounding the spent fuel at the time of water contact. This paper summarizes the main conclusions drawn from multiyear experimental campaigns performed at JRC-ITU to study corrosion behavior and radionuclide release from spent light water reactor fuel. The radionuclide release from the central region of a fuel pellet is higher than that from the radial periphery, in spite of the higher burnup and the corresponding structural modifications occurring at the pellet rim during irradiation. Studies on the extent and time boundaries of the radiolytic enhancement of the spent fuel corrosion rate indicate that after tens or hundreds of thousands of years have elapsed, very small or no contribution to the enhanced corrosion rate has to be expected from α radiolysis. A beneficial effect inhibiting spent fuel corrosion due to the hydrogen overpressure generated in the near field by iron corrosion is confirmed. The results obtained so far point toward a benign picture describing spent fuel corrosion in a deep geologic repository. More work is ongoing to further reduce uncertainties and to obtain a full description of the expected corrosion behavior of spent fuel.

  6. Test plan for reactions between spent fuel and J-13 well water under unsaturated conditions

    SciTech Connect

    Finn, P.A.; Wronkiewicz, D.J.; Hoh, J.C.; Emery, J.W.; Hafenrichter, L.D.; Bates, J.K.

    1993-01-01

    The Yucca Mountain Site Characterization Project is evaluating the long-term performance of a high-level nuclear waste form, spent fuel from commercial reactors. Permanent disposal of the spent fuel is possible in a potential repository to be located in the volcanic tuff beds near Yucca Mountain, Nevada. During the post-containment period the spent fuel could be exposed to water condensation since of the cladding is assumed to fail during this time. Spent fuel leach (SFL) tests are designed to simulate and monitor the release of radionuclides from the spent fuel under this condition. This Test Plan addresses the anticipated conditions whereby spent fuel is contacted by small amounts of water that trickle through the spent fuel container. Two complentary test plans are presented, one to examine the reaction of spent fuel and J-13 well water under unsaturated conditions and the second to examine the reaction of unirradiated UO{sub 2} pellets and J-13 well water under unsaturated conditions. The former test plan examines the importance of the water content, the oxygen content as affected by radiolysis, the fuel burnup, fuel surface area, and temperature. The latter test plant examines the effect of the non-presence of Teflon in the test vessel.

  7. Container materials in environments of corroded spent nuclear fuel

    NASA Astrophysics Data System (ADS)

    Huang, F. H.

    1996-07-01

    Efforts to remove corroded uranium metal fuel from the K Basins wet storage to long-term dry storage are underway. The multi-canister overpack (MCO) is used to load spent nuclear fuel for vacuum drying, staging, and hot conditioning; it will be used for interim dry storage until final disposition options are developed. Drying and conditioning of the corroded fuel will minimize the possibility of gas pressurization and runaway oxidation. During all phases of operations the MCO is subjected to radiation, temperature and pressure excursions, hydrogen, potential pyrophoric hazard, and corrosive environments. Material selection for the MCO applications is clearly vital for safe and efficient long-term interim storage. Austenitic stainless steels (SS) such as 304L SS or 316L SS appear to be suitable for the MCO. Of the two, Type 304L SS is recommended because it possesses good resistance to chemical corrosion, hydrogen embrittlement, and radiation-induced corrosive species. In addition, the material has adequate strength and ductility to withstand pressure and impact loading so that the containment boundary of the container is maintained under accident conditions without releasing radioactive materials.

  8. Physical and decay characteristics of commercial LWR spent fuel

    SciTech Connect

    Roddy, J.W.; Claiborne, H.C.; Ashline, R.C.; Johnson, P.J.; Rhyne, B.T.

    1986-01-01

    Information was collected from the literature and from major manufacturers that will be useful in the design and construction of a mined geologic repository for the disposal of light-water-reactor spent fuel. Pertinent data are included on mechanical design characteristics and materials of construction for fuel assemblies and fuel rods and computed values for heat generation rates, radioactivity, and photon and neutron emission rates as a function of time for four reference cases. Calculations were made with the ORIGEN2 computer code for burnups of 27,500 and 40,000 MWd for a typical boiling-water reactor and 33,000 and 60,000 MWd for a typical pressurized-water reactor. The results are presented in figures depicting the individual contributions per metric ton of initial heavy metal for the activation products, fission products, and actinides and their daughters to the radioactivity and thermal power as a function of time. Tables are also presented that list the contribution of each major nuclide to the radioactivity, thermal power, and photons and neutrons emitted for disposal emitted for disposal periods from 1 to 100,000 years.

  9. Physical and decay characteristics of commercial LWR spent fuel

    SciTech Connect

    Roddy, J.W.; Claiborne, H.C.; Ashline, R.C.; Johnson, P.J.; Rhyne, B.T.

    1985-10-01

    Information was collected from the literature and from major manufacturers that will be useful in the design and construction of a mined geologic repository for the disposal of light-water-reactor spent fuel. Pertinent data are included on mechanical design characteristics and materials of construction for fuel assemblies and fuel rods and computed values for heat generation rates, radioactivity, and photon and neutron emission rates as a function of time for four reference cases. Calculations were made with the ORIGEN2 computer code for burnups of 27,500 and 40,000 MWd for a typical boiling-water reactor and 33,000 and 60,000 MWd for a typical pressurized-water reactor. The results are presented in figures depicting the individual contributions per metric ton of initial heavy metal for the activation products, fission products, and actinides and their daughters to the radioactivity and thermal power as a function of time. Tables are also presented that list the contribution of each major nuclide to the radioactivity, thermal power, and photons and neutrons emitted for disposal periods from 1 to 100,000 years.

  10. ANL calculational methodologies for determining spent nuclear fuel source term

    SciTech Connect

    McKnight, R. D.

    2000-03-24

    Over the last decade Argonne National Laboratory has developed reactor depletion methods and models to determine radionuclide inventories of irradiated EBR-II fuels. Predicted masses based on these calculational methodologies have been validated using available data from destructive measurements--first from measurements of lead EBR-II experimental test assemblies and later using data obtained from processing irradiated EBR-II fuel assemblies in the Fuel Conditioning Facility. Details of these generic methodologies are described herein. Validation results demonstrate these methods meet the FCF operations and material control and accountancy requirements.

  11. Modelling the radiolytic corrosion of α-doped UO2 and spent nuclear fuel

    NASA Astrophysics Data System (ADS)

    Liu, Nazhen; Qin, Zack; Noël, James J.; Shoesmith, David W.

    2017-10-01

    A model previously developed to predict the corrosion rate of spent fuel (UO2) inside a failed waste container has been adapted to simulate the rates measured on a wide range of α-doped UO2 and spent fuel specimens. This simulation confirms the validity of the model and demonstrates that the steady-state corrosion rate is controlled by the radiolytic production of H2O2 (which has been shown to be the primary oxidant driving fuel corrosion), irrespective of the reactivity of the UO2 matrix. The model was then used to determine the consequences of corrosion inside a failed container resealed by steel corrosion products. The possible accumulation of O2, produced by H2O2 decomposition, was found to accelerate the corrosion rate in a closed system. However, the simultaneous accumulation of radiolytic H2, which is activated as a reductant on the noble metal (ε) particles in the spent fuel, rapidly overcame this acceleration leading to the eventual suppression of the corrosion rate to insignificant values. Calculations also showed that, while the radiation dose rate, the H2O2 decomposition ratio, and the surface coverage of ε particles all influenced the short term corrosion rate, the influence of the radiolytically produced H2 was the overwhelming influence in reducing the rate to negligible level (i.e., <10-20 mol m-2 s-1).

  12. Nuclear Forensics Attributing the Source of Spent Fuel Used in an RDD Event

    SciTech Connect

    Scott, Mark Robert

    2005-05-01

    An RDD attack against the U.S. is something America needs to prepare against. If such an event occurs the ability to quickly identify the source of the radiological material used in an RDD would aid investigators in identifying the perpetrators. Spent fuel is one of the most dangerous possible radiological sources for an RDD. In this work, a forensics methodology was developed and implemented to attribute spent fuel to a source reactor. The specific attributes determined are the spent fuel burnup, age from discharge, reactor type, and initial fuel enrichment. It is shown that by analyzing the post-event material, these attributes can be determined with enough accuracy to be useful for investigators. The burnup can be found within a 5% accuracy, enrichment with a 2% accuracy, and age with a 10% accuracy. Reactor type can be determined if specific nuclides are measured. The methodology developed was implemented into a code call NEMASYS. NEMASYS is easy to use and it takes a minimum amount of time to learn its basic functions. It will process data within a few minutes and provide detailed information about the results and conclusions.

  13. Testing and COBRA-SFS analysis of the VSC-17 ventilated concrete, spent fuel storage cask

    SciTech Connect

    McKinnon, M.A.; Dodge, R.E.; Schmitt, R.C.

    1992-04-01

    A performance test of a Pacific Sierra Nuclear VSC-17 ventilated concrete storage cask loaded with 17 canisters of consolidated PWR spent fuel generating approximately 15 kW was conducted. The performance test included measuring the cask surface, concrete, air channel surface, and fuel temperatures, as well as cask surface gamma and neutron dose rates. Testing was performed using vacuum, nitrogen, and helium backfill environments. Pretest predictions of cask thermal performance were made using the COBRA-SFS computer code. Analysis results were within 15{degrees}C of measured peak fuel temperature. Peak fuel temperature for normal operation was 321{degrees}C. In general, the surface dose rates were less than 30 mrem/h on the side of the cask and 40 mrem/h on the top of the cask.

  14. Spent nuclear fuel retrieval system fuel handling development testing. Final report

    SciTech Connect

    Jackson, D.R.; Meeuwsen, P.V.

    1997-09-01

    Fuel handling development testing was performed in support of the Fuel Retrieval System (FRS) Sub-Project, a subtask of the Spent Nuclear Fuel Project at the Hanford Site in Richland, Washington. The FRS will be used to retrieve and repackage K-Basin Spent Nuclear Fuel (SNF) currently stored in old K-Plant storage basins. The FRS is required to retrieve full fuel canisters from the basin, clean the fuel elements inside the canister to remove excessive uranium corrosion products (or sludge), remove the contents from the canisters and sort the resulting debris, scrap, and fuel for repackaging. The fuel elements and scrap will be collected in fuel storage and scrap baskets in preparation for loading into a multi canister overpack (MCO), while the debris is loaded into a debris bin and disposed of as solid waste. This report describes fuel handling development testing performed from May 1, 1997 through the end of August 1997. Testing during this period was mainly focused on performance of a Schilling Robotic Systems` Conan manipulator used to simulate a custom designed version, labeled Konan, being fabricated for K-Basin deployment. In addition to the manipulator, the camera viewing system, process table layout, and fuel handling processes were evaluated. The Conan test manipulator was installed and fully functional for testing in early 1997. Formal testing began May 1. The purposes of fuel handling development testing were to provide proof of concept and criteria, optimize equipment layout, initialize the process definition, and identify special needs/tools and required design changes to support development of the performance specification. The test program was set up to accomplish these objectives through cold (non-radiological) development testing using simulated and prototype equipment.

  15. Eddy Current Examination of Spent Nuclear Fuel Canister Closure Welds

    SciTech Connect

    Arthur D. Watkins; Dennis C. Kunerth; Timothy R. McJunkin

    2006-04-01

    The National Spent Nuclear Fuel Program (NSNFP) has developed standardized DOE SNF canisters for handling and interim storage of SNF at various DOE sites as well as SNF transport to and SNF handling and disposal at the repository. The final closure weld of the canister will be produced remotely in a hot cell after loading and must meet American Society of Mechanical Engineers (ASME) Section III, Division 3 code requirements thereby requiring volumetric and surface nondestructive evaluation to verify integrity. This paper discusses the use of eddy current testing (ET) to perform surface examination of the completed welds and repair cavities. Descriptions of integrated remote welding/inspection system and how the equipment is intended function will also be discussed.

  16. Fracture mapping at the Spent Fuel Test-Climax

    SciTech Connect

    Wilder, D.G.; Yow, J.L. Jr.

    1981-05-01

    Mapping of geologic discontinuities has been done in several phases at the Spent Fuel Test-Climax (SFT-C) in the granitic Climax stock at the Nevada Test Site. Mapping was carried out in the tail drift, access drift, canister drift, heater drifts, instrumentation alcove, and receiving room. The fractures mapped as intersecting a horizontal datum in the canister and heater drifts are shown on one figure. Fracture sketch maps have been compiled as additional figures. Geologic mapping efforts were scheduled around and significantly impacted by the excavation and construction schedules. Several people were involved in the mapping, and over 2500 geologic discontinuities were mapped, including joints, shears, and faults. Some variance between individuals` mapping efforts was noticed, and the effects of various magnetic influences upon a compass were examined. The examination of compass errors improved the credibility of the data. The compass analysis work is explained in Appendix A. Analysis of the fracture data will be presented in a future report.

  17. Air Transport of Spent Nuclear Fuel (SNF) Assemblies

    SciTech Connect

    Haire, M.J.; Moses, S.D.; Shapovalov, V.I.; Morenko, A.

    2007-07-01

    Sometimes the only feasible means of shipping research reactor spent nuclear fuel (SNF) among countries is via air transport because of location or political conditions. The International Atomic Energy Agency (IAEA) has established a regulatory framework to certify air transport Type C casks. However, no such cask has been designed, built, tested, and certified. In lieu of an air transport cask, research reactor SNF has been transported using a Type B cask under an exemption with special arrangements for administrative and security controls. This work indicates that it may be feasible to transport commercial power reactor SNF assemblies via air, and that the cost is only about three times that of shipping it by railway. Optimization (i.e., reduction) of this cost factor has yet to be done. (authors)

  18. Development of a Reliable Fuel Depletion Methodology for the HTR-10 Spent Fuel Analysis

    SciTech Connect

    Chung, Kiwhan; Beddingfield, David H.; Geist, William H.; Lee, Sang-Yoon

    2012-07-03

    A technical working group formed in 2007 between NNSA and CAEA to develop a reliable fuel depletion method for HTR-10 based on MCNPX and to analyze the isotopic inventory and radiation source terms of the HTR-10 spent fuel. Conclusions of this presentation are: (1) Established a fuel depletion methodology and demonstrated its safeguards application; (2) Proliferation resistant at high discharge burnup ({approx}80 GWD/MtHM) - Unfavorable isotopics, high number of pebbles needed, harder to reprocess pebbles; (3) SF should remain under safeguards comparable to that of LWR; and (4) Diversion scenarios not considered, but can be performed.

  19. Utilizing Divers in Support of Spent Fuel Basin Closure Subproject

    SciTech Connect

    Allen Nellesen

    2005-01-01

    A number of nuclear facilities in the world are aging and with this comes the fact that we have to either keep repairing them or decommission them. At the Department of Energy Idaho Site (DOEID) there are a number of facilities that are being decommissioned, but the facilities that pose the highest risk to the large aquifer that flows under the site are given highest priorities. Aging spent nuclear fuel pools at DOE-ID are among the facilities that pose the highest risk, therefore four pools were targeted for decommissioning in Fiscal Year 2004. To accomplish this task the Idaho Completion Project (ICP) of Bechtel BWXT Idaho, LLC, put together an integrated Basin Closure Subproject team. The team was assigned a goal to look beyond traditional practices at the Idaho National Engineering and Environmental Laboratory (INEEL) to find ways to get the basin closure work done safer and more efficiently. The Idaho Completion Project (ICP) was faced with a major challenge – cleaning and preparing aging spent nuclear fuel basins for closure by removing sludge and debris, as necessary, and removing water to eliminate a potential risk to the Snake River Plain Aquifer. The project included cleaning and removing water from four basins. Two of the main challenges to a project like this is the risk of contamination from the basin walls and floors becoming airborne as the water is removed and keeping personnel exposures ALARA. ICP’s baseline plan had workers standing at the edges of the basins and on rafts or bridge cranes and then using long-handled tools to manually scrub the walls of basin surfaces. This plan had significant risk of skin contamination events, workers falling into the water, or workers sustaining injuries from the awkward working position. Analysis of the safety and radiation dose risks presented by this approach drove the team to look for smarter ways to get the work done.

  20. Results from long-term dissolution tests using oxidized spent fuel

    SciTech Connect

    Wilson, C.N.

    1990-11-01

    Two semi-static dissolution tests using oxidized PWR spent fuel specimens are being conducted under ambient hot cell conditions in Nevada Test Site J-13 well water and unsealed fused silica vessels. The test specimens were oxidized at 250{degree}C in air to bulk oxygen-to-metal (O/M) values of 2.21 and 2.33. Following an initial 191-day test cycle, the specimens were restarted in fresh J-13 water for a second long-term test cycle. Results through the first 40 months of Cycle 2 are compared with results from similar tests at 25{degree}C and 85{degree}C using unoxidized spent fuel specimens. Increased concentrations of U, Am, Cm and NP were measured in 0.4-{mu}m filtered samples from the oxidized fuel tests compared to the unoxidized fuel tested at 25{degree}C; Pu concentrations were not affected by the fuel oxidation state. Most of the Am and Cm, and a portion of the Pu, measured in 0.4-{mu}m filtered samples was removed by 2-nm filtration. Fission product release results were normalized to specimen inventories and reported as fractional release. No attempt was made to normalize the data to surface area. Initial {sup 99}Tc release was greatly increased, and prolonged increases in the fractional release rates of {sup 99}Tc and {sup 129}I occurred as a result of fuel oxidation. Fractional release rates for {sup 137}Cs and {sup 90}Sr from oxidized fuel eventually decreased to levels similar to those observed with unoxidized fuel after equivalent testing times, suggesting that matrix dissolution rates normalized to fuel mass were not increased as a result of oxidation. 6 refs., 3 figs., 2 tabs.

  1. Direct Investigations of the Immobilization of Radionuclides in the Alteration Products of Spent Nuclear Fuel

    SciTech Connect

    Peter C. Burns; Robert J. Finch; David J. Wronkiewicz

    2004-12-27

    Safe disposal of the nation's nuclear waste in a geological repository involves unique scientific and engineering challenges owing to the very long-lived radioactivity of the waste. The repository must retain a variety of radionuclides that have vastly different chemical characters for several thousand years. Most of the radioactivity that will be housed in the proposed repository at Yucca Mountain will be associated with spent nuclear fuel, much of which is derived from commercial reactors. DOE is custodian of approximately 8000 tons of spent nuclear fuel that is also intended for eventual disposal in a geological repository. Unlike the spent fuel from commercial reactors, the DOE fuel is diverse in composition with more than 250 varieties. Safe disposal of spent fuel requires a detailed knowledge of its long-term behavior under repository conditions, as well as the fate of radionuclides released from the spent fuel as waste containers are breached.

  2. Preliminary study on direct recycling of spent BWR fuel in BWR system

    NASA Astrophysics Data System (ADS)

    Waris, A.; Sumbono, Prayudhatama, Dythia; Novitrian, Su'ud, Zaki

    2012-06-01

    Spent fuel management is considered to be one of the main problems in energy nuclear utilization. Recycling after reprocessing is one of the options for dealing with nuclear reactor spent fuel. Reprocessing is very costly and needs remote handling since spent fuel is very hazard high level waste. On top of that, only a small number of countries can manage a reprocessing plant. If country likes Indonesia decide to "go nuclear", it should find another way to deal with the nuclear spent fuel. Korea has proposed the DUPIC (Direct Utilization of Spent PWR fuel In CANDU) concept. Nevertheless, DUPIC concept requires two types of nuclear power plants, i.e., pressurized water reactor (PWR) and CANadian Deuterium Uranium reactor (CANDU). In this study, we evaluate a scheme of direct recycling of spent BWR fuel in BWR system, under the concept that we have called as a SUPEL (Straight Utilization of sPEnt LWR fuel in LWR system) scenario. Several spent BWR fuel compositions in loaded BWR fuel has been evaluated to achieve the criticality of reactor.

  3. Chemical reactivity testing for the National Spent Nuclear Fuel Program. Revision 2

    SciTech Connect

    Koester, L.W.

    2000-02-08

    This quality assurance project plan (QAPjP) summarizes requirements used by Lockheed Martin Energy Systems, Incorporated (LMES) Development Division at Y-12 for conducting chemical reactivity testing of Department of Energy (DOE) owned spent nuclear fuel, sponsored by the National Spent Nuclear Fuel Program (NSNFP). The requirements are based on the NSNFP Statement of work PRO-007 (Statement of Work for Laboratory Determination of Uranium Hydride Oxidation Reaction Kinetics.) This QAPjP will utilize the quality assurance program at Y-12, Y60-101PD, Quality Program Description, and existing implementing procedures for the most part in meeting the NSNFP Statement of Work PRO-007 requirements, exceptions will be noted. The project consists of conducting three separate series of related experiments, ''Passivation of Uranium Hydride Powder With Oxygen and Water'', '''Passivation of Uranium Hydride Powder with Surface Characterization'', and ''Electrochemical Measure of Uranium Hydride Corrosion Rate''.

  4. Electrochemical cell apparatus having axially distributed entry of a fuel-spent fuel mixture transverse to the cell lengths

    DOEpatents

    Reichner, P.; Dollard, W.J.

    1991-01-08

    An electrochemical apparatus is made having a generator section containing axially elongated electrochemical cells, a fresh gaseous feed fuel inlet, a gaseous feed oxidant inlet, and at least one gaseous spent fuel exit channel, where the spent fuel exit channel passes from the generator chamber to combine with the fresh feed fuel inlet at a mixing apparatus, reformable fuel mixture channel passes through the length of the generator chamber and connects with the mixing apparatus, that channel containing entry ports within the generator chamber, where the axis of the ports is transverse to the fuel electrode surfaces, where a catalytic reforming material is distributed near the reformable fuel mixture entry ports. 2 figures.

  5. Activity release from damaged fuel during the Paks-2 cleaning tank incident in the spent fuel storage pool

    NASA Astrophysics Data System (ADS)

    Hózer, Zoltán; Szabó, Emese; Pintér, Tamás; Varjú, Ilona Baracska; Bujtás, Tibor; Farkas, Gábor; Vajda, Nóra

    2009-07-01

    During crud removal operations the integrity of 30 fuel assemblies was lost at high temperature at the unit No. 2 of the Paks NPP. Part of the fission products was released from the damaged fuel into the coolant of the spent fuel storage pool. The gaseous fission products escaped through the chimney from the reactor hall. The volatile and non-volatile materials remained mainly in the coolant and were collected on the filters of water purification system. The activity release from damaged fuel rods during the Paks-2 cleaning tank incident was estimated on the basis of coolant activity concentration measurements and chimney activity data. The typical release rate of noble gases, iodine and caesium was 1-3%. The release of non-volatile fission products and actinides was also detected.

  6. Spent fuel disassembly hardware and other non-fuel bearing components: characterization, disposal cost estimates, and proposed repository acceptance requirements

    SciTech Connect

    Luksic, A.T.; McKee, R.W.; Daling, P.M.; Konzek, G.J.; Ludwick, J.D.; Purcell, W.L.

    1986-10-01

    There are two categories of waste considered in this report. The first is the spent fuel disassembly (SFD) hardware. This consists of the hardware remaining after the fuel pins have been removed from the fuel assembly. This includes end fittings, spacer grids, water rods (BWR) or guide tubes (PWR) as appropriate, and assorted springs, fasteners, etc. The second category is other non-fuel-bearing (NFB) components the DOE has agreed to accept for disposal, such as control rods, fuel channels, etc., under Appendix E of the standard utiltiy contract (10 CFR 961). It is estimated that there will be approximately 150 kg of SFD and NFB waste per average metric ton of uranium (MTU) of spent uranium. PWR fuel accounts for approximately two-thirds of the average spent-fuel mass but only 50 kg of the SFD and NFB waste, with most of that being spent fuel disassembly hardware. BWR fuel accounts for one-third of the average spent-fuel mass and the remaining 100 kg of the waste. The relatively large contribution of waste hardware in BWR fuel, will be non-fuel-bearing components, primarily consisting of the fuel channels. Chapters are devoted to a description of spent fuel disassembly hardware and non-fuel assembly components, characterization of activated components, disposal considerations (regulatory requirements, economic analysis, and projected annual waste quantities), and proposed acceptance requirements for spent fuel disassembly hardware and other non-fuel assembly components at a geologic repository. The economic analysis indicates that there is a large incentive for volume reduction.

  7. Impact analysis of stainless steel spent fuel canisters

    SciTech Connect

    Aramayo, G.A.; Turner, D.W.

    1998-04-01

    This paper presents the results of the numerical analysis performed to asses the structural integrity of spent nuclear fuel (SNF) stainless steel canisters when subjected to impact loads associated with free gravity drops from heights not exceeding 20 ft. The SNF canisters are to be used for the Shipment of radioactive material from the Oak Ridge National Laboratory (ORNL) Site to the Idaho National Engineering and Environmental Laboratory (INEEL) for storage. The Idaho chemical Processing Plant Fuel Receipt Criteria Questionnaire requires that the vertical drop accidents from two heights be analyze. These heights are those that are considered to be critical at the time of unloading the canisters from the shipping cask. The configurations analyzed include a maximum payload of 90 lbs dropping from heights of 20 and 3 ft. The nominal weight of the canister is 23.3 lbs. The analysis has been performed using finite element methods. Innovative analysis techniques are used to capture the effects of failure and separation of canister components. The structural integrity is evaluated in terms of physical deformation and separation of the canister components that may result from failure of components at selected interfaces.

  8. Safe Advantage on Dry Interim Spent Nuclear Fuel Storage

    SciTech Connect

    Romanato, L.S.

    2008-07-01

    This paper aims to present the advantages of dry cask storage in comparison with the wet storage (cooling water pools) for SNF. When the nuclear fuel is removed from the core reactor, it is moved to a storage unit and it wait for a final destination. Generally, the spent nuclear fuel (SNF) remains inside water pools within the reactors facility for the radioactive activity decay. After some period of time in pools, SNF can be sent to a definitive deposition in a geological repository and handled as radioactive waste or to reprocessing facilities, or still, wait for a future solution. Meanwhile, SNF remains stored for a period of time in dry or wet facilities, depending on the method adopted by the nuclear power plant or other plans of the country. Interim storage, up to 20 years ago, was exclusively wet and if the nuclear facility had to be decommissioned another storage solution had to be found. At the present time, after a preliminary cooling of the SNF elements inside the water pool, the elements can be stored in dry facilities. This kind of storage does not need complex radiation monitoring and it is safer then wet one. Casks, either concrete or metallic, are safer, especially on occurrence of earthquakes, like that occurred at Kashiwazaki-Kariwa nuclear power plant, in Japan on July 16, 2007. (authors)

  9. An analysis of plutonium immobilization versus the "spent fuel" standard

    SciTech Connect

    Gray, W L; McKibben, J M

    1998-06-16

    Safe Pu management is an important and urgent task with profound environmental, national, and international security implications. Presidential Policy Directive 13 and analyses by scientific, technical, and international policy organizations brought about a focused effort within the Department of Energy (DOE) to identify and implement long-term disposition paths for surplus Pu. The principal goal is to render surplus Pu as inaccessible and unattractive for reuse in nuclear weapons as Pu in spent reactor fuel. In the Programmatic Environmental Impact Statement and Record of Decision for the Storage and Disposition of Weapons- Usable Fissile Materials (1997), DOE announced pursuit of two disposition technologies: (1) irradiation of Pu as MOX fuel in existing reactors and (2) immobilization of Pu into solid forms containing fission products as a radiation barrier. DOE chose an immobilization approach that includes "use of the can-in-canister option.. . for a portion of the surplus, non-pit Pu material." In the can-in-canister approach, cans of glass or ceramic forms containing Pu are encapsulated within canisters of HLW glass. In support of the selection process, a technical evaluation of retrievability and recoverability of Pu from glass and ceramic forms by a host nation and by rogue nations or subnational groups was completed. The evaluation involved determining processes and flowsheets for Pu recovery, comparing these processes against criteria and metrics established by the Fissile Materials Disposition Program and then comparing the recovery processes against each other and against SNF processes.

  10. SCALE Validation Experience Using an Expanded Isotopic Assay Database for Spent Nuclear Fuel

    SciTech Connect

    Gauld, Ian C; Radulescu, Georgeta; Ilas, Germina

    2009-01-01

    The availability of measured isotopic assay data to validate computer code predictions of spent fuel compositions applied in burnup-credit criticality calculations is an essential component for bias and uncertainty determination in safety and licensing analyses. In recent years, as many countries move closer to implementing or expanding the use of burnup credit in criticality safety for licensing, there has been growing interest in acquiring additional high-quality assay data. The well-known open sources of assay data are viewed as potentially limiting for validating depletion calculations for burnup credit due to the relatively small number of isotopes measured (primarily actinides with relatively few fission products), sometimes large measurement uncertainties, incomplete documentation, and the limited burnup and enrichment range of the fuel samples. Oak Ridge National Laboratory (ORNL) recently initiated an extensive isotopic validation study that includes most of the public data archived in the Organization for Economic Cooperation and Development/Nuclear Energy Agency (OECD/NEA) electronic database, SFCOMPO, and new datasets obtained through participation in commercial experimental programs. To date, ORNL has analyzed approximately 120 different spent fuel samples from pressurized-water reactors that span a wide enrichment and burnup range and represent a broad class of assembly designs. The validation studies, completed using SCALE 5.1, are being used to support a technical basis for expanded implementation of burnup credit for spent fuel storage facilities, and other spent fuel analyses including radiation source term, dose assessment, decay heat, and waste repository safety analyses. This paper summarizes the isotopic assay data selected for this study, presents validation results obtained with SCALE 5.1, and discusses some of the challenges and experience associated with evaluating the results. Preliminary results obtained using SCALE 6 and ENDF

  11. 75 FR 34181 - Connecticut Yankee Atomic Power Company, Haddam Neck Plant, Independent Spent Fuel Storage...

    Federal Register 2010, 2011, 2012, 2013, 2014

    2010-06-16

    ... COMMISSION Connecticut Yankee Atomic Power Company, Haddam Neck Plant, Independent Spent Fuel Storage... spent fuel storage installation (ISFSI) associated with the decommissioned Haddam Neck Plant, located in.... 4 will remain in effect for the casks at the CYAPCO ISFSI until the NRC expressly approves the...

  12. 77 FR 9515 - List of Approved Spent Fuel Storage Casks: HI-STORM 100, Revision 8

    Federal Register 2010, 2011, 2012, 2013, 2014

    2012-02-17

    ... RIN 3150-AJ05 List of Approved Spent Fuel Storage Casks: HI-STORM 100, Revision 8 AGENCY: Nuclear... Commission) is amending its spent fuel storage regulations by revising the Holtec International HI-STORM 100... and safety will be adequately protected. This direct final rule revises the HI-STORM 100 listing in 10...

  13. 10 CFR 72.230 - Procedures for spent fuel storage cask submittals.

    Code of Federal Regulations, 2010 CFR

    2010-01-01

    ... 10 Energy 2 2010-01-01 2010-01-01 false Procedures for spent fuel storage cask submittals. 72.230 Section 72.230 Energy NUCLEAR REGULATORY COMMISSION (CONTINUED) LICENSING REQUIREMENTS FOR THE INDEPENDENT STORAGE OF SPENT NUCLEAR FUEL, HIGH-LEVEL RADIOACTIVE WASTE, AND REACTOR-RELATED GREATER THAN CLASS...

  14. 10 CFR 72.236 - Specific requirements for spent fuel storage cask approval and fabrication.

    Code of Federal Regulations, 2011 CFR

    2011-01-01

    ... 10 Energy 2 2011-01-01 2011-01-01 false Specific requirements for spent fuel storage cask approval and fabrication. 72.236 Section 72.236 Energy NUCLEAR REGULATORY COMMISSION (CONTINUED) LICENSING REQUIREMENTS FOR THE INDEPENDENT STORAGE OF SPENT NUCLEAR FUEL, HIGH-LEVEL RADIOACTIVE WASTE, AND...

  15. 10 CFR 72.230 - Procedures for spent fuel storage cask submittals.

    Code of Federal Regulations, 2011 CFR

    2011-01-01

    ... 10 Energy 2 2011-01-01 2011-01-01 false Procedures for spent fuel storage cask submittals. 72.230 Section 72.230 Energy NUCLEAR REGULATORY COMMISSION (CONTINUED) LICENSING REQUIREMENTS FOR THE INDEPENDENT STORAGE OF SPENT NUCLEAR FUEL, HIGH-LEVEL RADIOACTIVE WASTE, AND REACTOR-RELATED GREATER THAN CLASS...

  16. 76 FR 9381 - Notice of Availability of Interim Staff Guidance Documents for Spent Fuel Storage Casks

    Federal Register 2010, 2011, 2012, 2013, 2014

    2011-02-17

    ... Gordon, Structural Mechanics and Materials Branch, Division of Spent Fuel Storage and Transportation... ISG-23 should be directed to Matthew Gordon, Structural Mechanics and Materials Branch, Division of.... Michele Sampson, Acting Chief, Structural Mechanics and Materials Branch, Division of Spent Fuel Storage...

  17. Electrometallurgical treatment of metal, oxide, and aluminum-alloy spent nuclear fuel types.

    SciTech Connect

    McPheeters, C. C.; Gay, E. C.; Karell, E. J.; Ackerman, J. P.; Chemical Engineering

    1997-01-01

    Electrorefining uranium in a molten salt bath is the key step in the electrometallurgical treatment of spent nuclear fuels. The versatility of the electrometallurgical treatment suggests its use for a variety of spent fuel types, as well as for nonnuclear metal-separation applications.

  18. 10 CFR 72.240 - Conditions for spent fuel storage cask renewal.

    Code of Federal Regulations, 2013 CFR

    2013-01-01

    ... 10 Energy 2 2013-01-01 2013-01-01 false Conditions for spent fuel storage cask renewal. 72.240 Section 72.240 Energy NUCLEAR REGULATORY COMMISSION (CONTINUED) LICENSING REQUIREMENTS FOR THE INDEPENDENT STORAGE OF SPENT NUCLEAR FUEL, HIGH-LEVEL RADIOACTIVE WASTE, AND REACTOR-RELATED GREATER THAN CLASS C...

  19. 10 CFR 72.230 - Procedures for spent fuel storage cask submittals.

    Code of Federal Regulations, 2012 CFR

    2012-01-01

    ... 10 Energy 2 2012-01-01 2012-01-01 false Procedures for spent fuel storage cask submittals. 72.230 Section 72.230 Energy NUCLEAR REGULATORY COMMISSION (CONTINUED) LICENSING REQUIREMENTS FOR THE INDEPENDENT STORAGE OF SPENT NUCLEAR FUEL, HIGH-LEVEL RADIOACTIVE WASTE, AND REACTOR-RELATED GREATER THAN CLASS C...

  20. 10 CFR 72.240 - Conditions for spent fuel storage cask renewal.

    Code of Federal Regulations, 2014 CFR

    2014-01-01

    ... 10 Energy 2 2014-01-01 2014-01-01 false Conditions for spent fuel storage cask renewal. 72.240 Section 72.240 Energy NUCLEAR REGULATORY COMMISSION (CONTINUED) LICENSING REQUIREMENTS FOR THE INDEPENDENT STORAGE OF SPENT NUCLEAR FUEL, HIGH-LEVEL RADIOACTIVE WASTE, AND REACTOR-RELATED GREATER THAN CLASS C...

  1. 10 CFR 72.236 - Specific requirements for spent fuel storage cask approval and fabrication.

    Code of Federal Regulations, 2014 CFR

    2014-01-01

    ... 10 Energy 2 2014-01-01 2014-01-01 false Specific requirements for spent fuel storage cask approval and fabrication. 72.236 Section 72.236 Energy NUCLEAR REGULATORY COMMISSION (CONTINUED) LICENSING REQUIREMENTS FOR THE INDEPENDENT STORAGE OF SPENT NUCLEAR FUEL, HIGH-LEVEL RADIOACTIVE WASTE, AND REACTOR...

  2. 10 CFR 72.240 - Conditions for spent fuel storage cask renewal.

    Code of Federal Regulations, 2012 CFR

    2012-01-01

    ... 10 Energy 2 2012-01-01 2012-01-01 false Conditions for spent fuel storage cask renewal. 72.240 Section 72.240 Energy NUCLEAR REGULATORY COMMISSION (CONTINUED) LICENSING REQUIREMENTS FOR THE INDEPENDENT STORAGE OF SPENT NUCLEAR FUEL, HIGH-LEVEL RADIOACTIVE WASTE, AND REACTOR-RELATED GREATER THAN CLASS C...

  3. 10 CFR 72.230 - Procedures for spent fuel storage cask submittals.

    Code of Federal Regulations, 2013 CFR

    2013-01-01

    ... 10 Energy 2 2013-01-01 2013-01-01 false Procedures for spent fuel storage cask submittals. 72.230 Section 72.230 Energy NUCLEAR REGULATORY COMMISSION (CONTINUED) LICENSING REQUIREMENTS FOR THE INDEPENDENT STORAGE OF SPENT NUCLEAR FUEL, HIGH-LEVEL RADIOACTIVE WASTE, AND REACTOR-RELATED GREATER THAN CLASS C...

  4. 10 CFR 72.236 - Specific requirements for spent fuel storage cask approval and fabrication.

    Code of Federal Regulations, 2013 CFR

    2013-01-01

    ... 10 Energy 2 2013-01-01 2013-01-01 false Specific requirements for spent fuel storage cask approval and fabrication. 72.236 Section 72.236 Energy NUCLEAR REGULATORY COMMISSION (CONTINUED) LICENSING REQUIREMENTS FOR THE INDEPENDENT STORAGE OF SPENT NUCLEAR FUEL, HIGH-LEVEL RADIOACTIVE WASTE, AND REACTOR...

  5. 10 CFR 72.236 - Specific requirements for spent fuel storage cask approval and fabrication.

    Code of Federal Regulations, 2012 CFR

    2012-01-01

    ... 10 Energy 2 2012-01-01 2012-01-01 false Specific requirements for spent fuel storage cask approval and fabrication. 72.236 Section 72.236 Energy NUCLEAR REGULATORY COMMISSION (CONTINUED) LICENSING REQUIREMENTS FOR THE INDEPENDENT STORAGE OF SPENT NUCLEAR FUEL, HIGH-LEVEL RADIOACTIVE WASTE, AND REACTOR...

  6. 10 CFR 72.230 - Procedures for spent fuel storage cask submittals.

    Code of Federal Regulations, 2014 CFR

    2014-01-01

    ... 10 Energy 2 2014-01-01 2014-01-01 false Procedures for spent fuel storage cask submittals. 72.230 Section 72.230 Energy NUCLEAR REGULATORY COMMISSION (CONTINUED) LICENSING REQUIREMENTS FOR THE INDEPENDENT STORAGE OF SPENT NUCLEAR FUEL, HIGH-LEVEL RADIOACTIVE WASTE, AND REACTOR-RELATED GREATER THAN CLASS C...

  7. A study on the expulsion of iodine from spent-fuel solutions

    SciTech Connect

    Sakurai, Tsutomu; Takahashi, Akira; Ishikawa, Niroh

    1995-02-01

    During dissolution of spent nuclear fuels, some radioiodine remains in spent-fuel solutions. Its expulsion to dissolver off-gas is important to minimize iodine escape to the environment. In our current work, the iodine remaining in spent-fuel solutions varied from 0 to 10% after dissolution of spent PWR-fuel specimens (approximately 3 g each). The amount remaining probably was dependent upon the dissolution time required. The cause is ascribable to the increased nitrous acid concentration that results from NOx generated during dissolution. The presence of nitrous acid was confirmed spectrophotometrically in an NO-HNO{sub 3} system at 100{degrees}C. Experiments examining NOx concentration versus the quantity of iodine in a simulated spent-fuel solution indicate that iodine (I{minus}) in spent fuels is subjected to the following three reactions: (1) oxidation into I{sub 2} by nitric acid, (2) oxidation into I{sub 2} by nitrous acid arising from NOx, and (3) formation of colloidal iodine (AgI, PdI{sub 2}), the major iodine species in a spent-fuel solution. Reaction (2) competes with reaction (3) to control the quantity of iodine remaining in solution. The following two-step expulsion process to remove iodine from a spent-fuel solution was derived from these experiments: Step One - Heat spent-fuel solutions without NOx sparging. When aged colloidal iodine is present, an excess amount of iodate should be added to the solution. Step Two - Sparge the fuel solution with NOx while heating. Effect of this new method was confirmed by use of a spent PWR-fuel solution.

  8. REACTOR PHYSICS MODELING OF SPENT RESEARCH REACTOR FUEL FOR TECHNICAL NUCLEAR FORENSICS

    SciTech Connect

    Nichols, T.; Beals, D.; Sternat, M.

    2011-07-18

    Technical nuclear forensics (TNF) refers to the collection, analysis and evaluation of pre- and post-detonation radiological or nuclear materials, devices, and/or debris. TNF is an integral component, complementing traditional forensics and investigative work, to help enable the attribution of discovered radiological or nuclear material. Research is needed to improve the capabilities of TNF. One research area of interest is determining the isotopic signatures of research reactors. Research reactors are a potential source of both radiological and nuclear material. Research reactors are often the least safeguarded type of reactor; they vary greatly in size, fuel type, enrichment, power, and burn-up. Many research reactors are fueled with highly-enriched uranium (HEU), up to {approx}93% {sup 235}U, which could potentially be used as weapons material. All of them have significant amounts of radiological material with which a radioactive dispersal device (RDD) could be built. Therefore, the ability to attribute if material originated from or was produced in a specific research reactor is an important tool in providing for the security of the United States. Currently there are approximately 237 operating research reactors worldwide, another 12 are in temporary shutdown and 224 research reactors are reported as shut down. Little is currently known about the isotopic signatures of spent research reactor fuel. An effort is underway at Savannah River National Laboratory (SRNL) to analyze spent research reactor fuel to determine these signatures. Computer models, using reactor physics codes, are being compared to the measured analytes in the spent fuel. This allows for improving the reactor physics codes in modeling research reactors for the purpose of nuclear forensics. Currently the Oak Ridge Research reactor (ORR) is being modeled and fuel samples are being analyzed for comparison. Samples of an ORR spent fuel assembly were taken by SRNL for analytical and radiochemical

  9. Interim report spent nuclear fuel retrieval system fuel handling development testing

    SciTech Connect

    Ketner, G.L.; Meeuwsen, P.V.; Potter, J.D.; Smalley, J.T.; Baker, C.P.; Jaquish, W.R.

    1997-06-01

    Fuel handling development testing was performed in support of the Fuel Retrieval System (FRS) Sub-Project at the Hanford Site. The project will retrieve spent nuclear fuel, clean and remove fuel from canisters, repackage fuel into baskets, and load fuel into a multi-canister overpack (MCO) for vacuum drying and interim dry storage. The FRS is required to retrieve basin fuel canisters, clean fuel elements sufficiently of uranium corrosion products (or sludge), empty fuel from canisters, sort debris and scrap from whole elements, and repackage fuel in baskets in preparation for MCO loading. The purpose of fuel handling development testing was to examine the systems ability to accomplish mission activities, optimization of equipment layouts for initial process definition, identification of special needs/tools, verification of required design changes to support performance specification development, and validation of estimated activity times/throughput. The test program was set up to accomplish this purpose through cold development testing using simulated and prototype equipment; cold demonstration testing using vendor expertise and systems; and graphical computer modeling to confirm feasibility and throughput. To test the fuel handling process, a test mockup that represented the process table was fabricated and installed. The test mockup included a Schilling HV series manipulator that was prototypic of the Schilling Hydra manipulator. The process table mockup included the tipping station, sorting area, disassembly and inspection zones, fuel staging areas, and basket loading stations. The test results clearly indicate that the Schilling Hydra arm cannot effectively perform the fuel handling tasks required unless it is attached to some device that can impart vertical translation, azimuth rotation, and X-Y translation. Other test results indicate the importance of camera locations and capabilities, and of the jaw and end effector tool design. 5 refs., 35 figs., 3 tabs.

  10. Utilization of spent activated carbon to enhance the combustion efficiency of organic sludge derived fuel.

    PubMed

    Chen, Wei-Sheng; Lin, Chang-Wen; Chang, Fang-Chih; Lee, Wen-Jhy; Wu, Jhong-Lin

    2012-06-01

    This study examines the heating value and combustion efficiency of organic sludge derived fuel, spent activated carbon derived fuel, and derived fuel from a mixture of organic sludge and spent activated carbon. Spent activated carbon was sampled from an air pollution control device of an incinerator and characterized by XRD, XRF, TG/DTA, and SEM. The spent activated carbon was washed with deionized water and solvent (1N sulfuric acid) and then processed by the organic sludge derived fuel manufacturing process. After washing, the salt (chloride) and sulfide content could be reduced to 99% and 97%, respectively; in addition the carbon content and heating value were increased. Different ratios of spent activated carbon have been applied to the organic sludge derived fuel to reduce the NO(x) emission of the combustion.

  11. Simulation of differential die-away instrument’s response to asymmetrically burned spent nuclear fuel

    DOE PAGES

    Martinik, Tomas; Henzl, Vladimir; Grape, Sophie; ...

    2015-03-04

    Here, previous simulation studies of Differential Die–Away (DDA) instrument’s response to active interrogation of spent nuclear fuel from a pressurized water reactor (PWR) yielded promising results in terms of its capability to accurately measure or estimate basic spent fuel assembly (SFA) characteristics, such as multiplication, initial enrichment (IE) and burn-up (BU) as well as the total plutonium content. These studies were however performed only for a subset of idealized SFAs with a symmetric BU with respect to its longitudinal axis. Therefore, to complement the previous results, additional simulations have been performed of the DDA instrument’s response to interrogation of asymmetricallymore » burned spent nuclear fuel in order to determine whether detailed assay of SFAs from all 4 sides will be necessary in real life applications or whether a cost and time saving single sided assay could be used to achieve results of similar quality as previously reported in case of symmetrically burned SFAs.« less

  12. Analyses of the transportation of spent research reactor fuel in the United States

    SciTech Connect

    Cashwell, J.W.; Neuhauser, K.S.

    1989-01-01

    We analyzed the impacts of transportation of research reactor spent fuel from US and foreign reactors for the US Department of Energy's (DOE) Office of Defense Programs. Two separate shipment programs were analyzed. The shipment of research reactor spent fuel from Taiwan to the US (Fuel Movement Program), and the return of research reactor spent fuels of US origin from foreign and domestic reactors (Research Reactor Fuel Return Program). To perform these analyses, a comprehensive methodology for analyzing the probabilities and consequences of transportation in coastal waters and port facilities, handling at the port, and shipment by truck to reprocessing facilities was developed. The Taiwanese fuel consists of low-burnup aluminum-clad metallic uranium research reactor spent fuel; the other fuels are primarily aluminum-clad oxide fuels. The Fuel Movement Program is ongoing, while the Fuel Return Program addresses future shipments over a ten-year period. The operational aspects of the Taiwanese shipments have been uniform, but several possible shipping configurations are possible for the Fuel Return Program shipments. The risks of transporting spent nuclear fuel and other radioactive materials by all modes have been analyzed extensively. Comprehensive assessments, which bound the impacts of spent fuel transport, demonstrate that when shipments are made in compliance with applicable regulations, the risks for all such transport are low. For comparison with previously licensed transport activities and to provide continuity with earlier analyses, the results for shipment of 150-day-old commercial pressurized water reactor (PWR) spent fuel are presented as part of this study.

  13. Instrumentation Report No. 2: identification, evaluation, and remedial actions related to transducer failures at the spent fuel test-climax

    SciTech Connect

    Patrick, W.C.; Carlson, R.C.; Rector, N.L.

    1981-11-30

    The Spent Fuel Test-Climax (SFT-C) is a test of the feasibility of safe and reliable short-term storage and retrieval of spent fuel from commercial nuclear reactors. In support of operational and technical goals of the test, about 850 channels of instrumentation have been installed at the SFT-C. Failure of several near-field instruments began less than six months after emplacement of 11 canisters of spent fuel and activation of six thermally similar simulators. The failed units were linear potentiometers (used to make displacement measurements) and vibrating wire stressmeters (used to make change-in-stress measurements). This report discusses the observed problems and remedial actions taken to date.

  14. Method for computing the maximum water temperature in a fuel pool containing spent nuclear fuel

    SciTech Connect

    Singh, K.P.; Soler, A.I.; Gupta, J.P.

    1986-01-01

    A method is proposed for computing the upper bound on the local water temperature rise with respect to the bulk temperature in a spent fuel pool. The solution involves casting the continuity and momentum relationships in integral form in terms of the unknown velocity functions. The method of collocation is used to solve the problem. Computer application of this method shows it to be an efficient and cost-effective design tool.

  15. Monte Carlo simulations of a differential die-away instrument for determination of fissile content in spent fuel assemblies

    SciTech Connect

    Lee, Taehoon; Menlove, Howard O; Swinhoe, Martyn T; Tobin, Stephen J

    2010-01-01

    The differential die-away (DDA) technique has been simulated by using the MCNPX code to quantify its capability to measure the fissile content in spent fuel assemblies, For 64 different spent fuel cases of various initial enrichment, burnup and cooling time, the count rate and signal to background ratios of the DDA system were obtained, where neutron backgrounds are mainly coming from the {sup 244}Cm of the spent fuel. To quantify the total fissile mass of spent fuel, a concept of the effective {sup 239}Pu mass was introduced by weighting the relative contribution to the signal of {sup 235}U and {sup 241}Pu compared to {sup 239}Pu and the calibration curves of DDA count rate vs. {sup 239}Pu{sub eff} were obtained by using the MCNPX code. With a deuterium-tritium (DT) neutron generator of 10{sup 9} n/s strength, signal to background ratios of sufficient magnitude are acquired for a DDA system with the spent fuel assembly in water.

  16. 78 FR 78285 - List of Approved Spent Fuel Storage Casks: HI-STORM 100 Cask System; Amendment No. 9

    Federal Register 2010, 2011, 2012, 2013, 2014

    2013-12-26

    ...; ] NUCLEAR REGULATORY COMMISSION 10 CFR Part 72 RIN 3150-AJ12 List of Approved Spent Fuel Storage Casks: HI... revising the Holtec International HI-STORM 100 Cask System listing within the ``List of Approved Spent Fuel...

  17. 78 FR 78165 - List of Approved Spent Fuel Storage Casks: HI-STORM 100 Cask System; Amendment No. 9

    Federal Register 2010, 2011, 2012, 2013, 2014

    2013-12-26

    ... RIN 3150-AJ12 List of Approved Spent Fuel Storage Casks: HI-STORM 100 Cask System; Amendment No. 9... amends the NRC's spent fuel storage regulations by revising the Holtec International HI-STORM 100 Cask...

  18. Plasma processing of spent nuclear fuel by two-frequency ion cyclotron resonance heating

    SciTech Connect

    Timofeev, A. V.

    2009-11-15

    A previously developed method for analyzing the plasma processing of spent nuclear fuel is generalized to a plasma containing multicharged fuel ions. In such a plasma, ion cyclotron resonance heating of nuclear ash ions should be carried out in two monochromatic RF fields of different frequencies, provided that the fraction of {xi} multicharged ions is small, {xi} {<=} 0.1, a condition that substantially restricts the productivity of systems for processing spent nuclear fuel. Ways of overcoming this difficulty are discussed.

  19. Spent nuclear fuel integrity during dry storage - performance tests and demonstrations

    SciTech Connect

    McKinnon, M.A.; Doherty, A.L.

    1997-06-01

    This report summarizes the results of fuel integrity surveillance determined from gas sampling during and after performance tests and demonstrations conducted from 1983 through 1996 by or in cooperation with the US DOE Office of Commercial Radioactive Waste Management (OCRWM). The cask performance tests were conducted at Idaho National Engineering Laboratory (INEL) between 1984 and 1991 and included visual observation and ultrasonic examination of the condition of the cladding, fuel rods, and fuel assembly hardware before dry storage and consolidation of fuel, and a qualitative determination of the effects of dry storage and fuel consolidation on fission gas release from the spent fuel rods. The performance tests consisted of 6 to 14 runs involving one or two loading, usually three backfill environments (helium, nitrogen, and vacuum backfills), and one or two storage system orientations. The nitrogen and helium backfills were sampled and analyzed to detect leaking spent fuel rods. At the end of each performance test, periodic gas sampling was conducted on each cask. A spent fuel behavior project (i.e., enhanced surveillance, monitoring, and gas sampling activities) was initiated by DOE in 1994 for intact fuel in a CASTOR V/21 cask and for consolidated fuel in a VSC-17 cask. The results of the gas sampling activities are included in this report. Information on spent fuel integrity is of interest in evaluating the impact of long-term dry storage on the behavior of spent fuel rods. Spent fuel used during cask performance tests at INEL offers significant opportunities for confirmation of the benign nature of long-term dry storage. Supporting cask demonstration included licensing and operation of an independent spent fuel storage installation (ISFSI) at the Virginia Power (VP) Surry reactor site. A CASTOR V/21, an MC-10, and a Nuclear Assurance NAC-I28 have been loaded and placed at the VP ISFSI as part of the demonstration program. 13 refs., 14 figs., 9 tabs.

  20. Multi-Pack Disposal Concepts for Spent Fuel (Revision 1)

    SciTech Connect

    Hardin, Ernest; Matteo, Edward N.; Hadgu, Teklu

    2016-01-01

    At the initiation of the Used Fuel Disposition (UFD) R&D campaign, international geologic disposal programs and past work in the U.S. were surveyed to identify viable disposal concepts for crystalline, clay/shale, and salt host media. Concepts for disposal of commercial spent nuclear fuel (SNF) and high-level waste (HLW) from reprocessing are relatively advanced in countries such as Finland, France, and Sweden. The UFD work quickly showed that these international concepts are all “enclosed,” whereby waste packages are emplaced in direct or close contact with natural or engineered materials . Alternative “open” modes (emplacement tunnels are kept open after emplacement for extended ventilation) have been limited to the Yucca Mountain License Application Design. Thermal analysis showed that if “enclosed” concepts are constrained by peak package/buffer temperature, that waste package capacity is limited to 4 PWR assemblies (or 9 BWR) in all media except salt. This information motivated separate studies: 1) extend the peak temperature tolerance of backfill materials, which is ongoing; and 2) develop small canisters (up to 4-PWR size) that can be grouped in larger multi-pack units for convenience of storage, transportation, and possibly disposal (should the disposal concept permit larger packages). A recent result from the second line of investigation is the Task Order 18 report: Generic Design for Small Standardized Transportation, Aging and Disposal Canister Systems. This report identifies disposal concepts for the small canisters (4-PWR size) drawing heavily on previous work, and for the multi-pack (16-PWR or 36-BWR).

  1. Multi-pack Disposal Concepts for Spent Fuel (Rev. 0)

    SciTech Connect

    Hadgu, Teklu; Hardin, Ernest; Matteo, Edward N.

    2015-12-01

    At the initiation of the Used Fuel Disposition (UFD) R&D campaign, international geologic disposal programs and past work in the U.S. were surveyed to identify viable disposal concepts for crystalline, clay/shale, and salt host media (Hardin et al., 2012). Concepts for disposal of commercial spent nuclear fuel (SNF) and high-level waste (HLW) from reprocessing are relatively advanced in countries such as Finland, France, and Sweden. The UFD work quickly showed that these international concepts are all “enclosed,” whereby waste packages are emplaced in direct or close contact with natural or engineered materials . Alternative “open” modes (emplacement tunnels are kept open after emplacement for extended ventilation) have been limited to the Yucca Mountain License Application Design (CRWMS M&O, 1999). Thermal analysis showed that, if “enclosed” concepts are constrained by peak package/buffer temperature, waste package capacity is limited to 4 PWR assemblies (or 9-BWR) in all media except salt. This information motivated separate studies: 1) extend the peak temperature tolerance of backfill materials, which is ongoing; and 2) develop small canisters (up to 4-PWR size) that can be grouped in larger multi-pack units for convenience of storage, transportation, and possibly disposal (should the disposal concept permit larger packages). A recent result from the second line of investigation is the Task Order 18 report: Generic Design for Small Standardized Transportation, Aging and Disposal Canister Systems (EnergySolution, 2015). This report identifies disposal concepts for the small canisters (4-PWR size) drawing heavily on previous work, and for the multi-pack (16-PWR or 36-BWR).

  2. Efficient regeneration of partially spent ammonia borane fuel

    SciTech Connect

    Davis, Benjamin Lee; Gordon, John C; Stephens, Frances; Dixon, David A; Matus, Myrna H

    2008-01-01

    A necessary target in realizing a hydrogen (H{sub 2}) economy, especially for the transportation sector, is its storage for controlled delivery, presumably to an energy producing fuel cell. In this vein, the U.S. Department of Energy's (DOE) Centers of Excellence (CoE) in Hydrogen Storage have pursued different methodologies, including metal hydrides, chemical hydrides, and sorbents, for the expressed purpose of supplanting gasoline's current > 300 mile driving range. Chemical hydrogen storage has been dominated by one appealing material, ammonia borane (H{sub 3}B-NH{sub 3}, AB), due to its high gravimetric capacity of hydrogen (19.6 wt %) and low molecular weight (30.7 g mol{sup -1}). In addition, AB has both hydridic and protic moieties, yielding a material from which H2 can be readily released. As such, a number of publications have described H{sub 2} release from amine boranes, yielding various rates depending on the method applied. Even though the viability of any chemical hydrogen storage system is critically dependent on efficient recyclability, reports on the latter subject are sparse, invoke the use of high energy reducing agents, and suffer from low yields. For example, the DOE recently decided to no longer pursue the use of NaBH{sub 4} as a H{sub 2} storage material, in part because of inefficient regeneration. We thus endeavored to find an energy efficient regeneration process for the spent fuel from H{sub 2} depleted AB with a minimum number of steps.

  3. 76 FR 20722 - In the Matter of Indiana Michigan Power Company; DC Cook Nuclear Plant Independent Spent Fuel...

    Federal Register 2010, 2011, 2012, 2013, 2014

    2011-04-13

    ...: Issuance of Order for Implementation of Additional Security Measures and Fingerprinting for Unescorted... Project Manager, Licensing and Inspection Directorate, Division of Spent Fuel Storage and Transportation... determined these measures to be prudent. Comparable Orders have been issued to all licensees that currently...

  4. Progress on High Energy Delayed Gamma Spectroscopy for Direct Assay of Pu in Spent Fuel

    SciTech Connect

    Campbell, Luke W.; Smith, Leon E.

    2010-08-11

    The direct, nondestructive measurement of fissile and fissionable isotopes in spent fuel is not yet possible. Current methods which infer plutonium content through proxy measurements and confirmatory burnup calculations have relatively large uncertainty and do not satisfy the desire for a measurement that is independent of operator declarations. We are currently exploring the High Energy Delayed Gamma Spectroscopy (HEDGS) technique for direct, independent Pu measurement in light-water reactor fuels. HEDGS exploits the unique distribution of fission-product nuclei from each of the fissile isotopes. Fission is stimulated in the sample with a source of interrogating neutrons, and delayed gamma rays from the decay of the short-lived fission-product nuclei are measured. The measured gamma spectrum from the unknown sample is then fit with a linear combination of gamma spectra from pure U-235, Pu-239, and Pu-241, as deduced from the known fission-product yield curves and decay properties of the fission-product nuclei, to determine the original proportions of these fissile isotopes. In previous work, we performed preliminary modeling studies of HEDGS on idealized single fuel pins of various burnups. Here, we report progress on extending our GEANT-based modeling tools to efficiently model full pressurized water reactor (PWR) fuel assemblies using variance reduction techniques specific to the background emissions and induced signal, as appropriate. Predicted performance for a nominal HEDGS instrument design, is reported for the assay of U-235, Pu-239 and Pu-241 in spent fuel assemblies ranging from fresh to 60 GWd/MTU in burnup.

  5. REACTOR PHYSICS MODELING OF SPENT NUCLEAR RESEARCH REACTOR FUEL FOR SNM ATTRIBUTION AND NUCLEAR FORENSICS

    SciTech Connect

    Sternat, M.; Beals, D.; Webb, R.; Nichols, T.

    2010-06-09

    Nuclear research reactors are the least safeguarded type of reactor; in some cases this may be attributed to low risk and in most cases it is due to difficulty from dynamic operation. Research reactors vary greatly in size, fuel type, enrichment, power and burnup providing a significant challenge to any standardized safeguard system. If a whole fuel assembly was interdicted, based on geometry and other traditional forensics work, one could identify the material's origin fairly accurately. If the material has been dispersed or reprocessed, in-depth reactor physics models may be used to help with the identification. Should there be a need to attribute research reactor fuel material, the Savannah River National Laboratory would perform radiochemical analysis of samples of the material as well as other non-destructive measurements. In depth reactor physics modeling would then be performed to compare to these measured results in an attempt to associate the measured results with various reactor parameters. Several reactor physics codes are being used and considered for this purpose, including: MONTEBURNS/ORIGEN/MCNP5, CINDER/MCNPX and WIMS. In attempt to identify reactor characteristics, such as time since shutdown, burnup, or power, various isotopes are used. Complexities arise when the inherent assumptions embedded in different reactor physics codes handle the isotopes differently and may quantify them to different levels of accuracy. A technical approach to modeling spent research reactor fuel begins at the assembly level upon acquiring detailed information of the reactor to be modeled. A single assembly is run using periodic boundary conditions to simulate an infinite lattice which may be repeatedly burned to produce input fuel isotopic vectors of various burnups for a core level model. A core level model will then be constructed using the assembly level results as inputs for the specific fuel shuffling pattern in an attempt to establish an equilibrium cycle. The

  6. Shipping and storage cask data for spent nuclear fuel

    SciTech Connect

    Johnson, E.R.; Notz, K.J.

    1988-11-01

    This document is a compilation of data on casks used for the storage and/or transport of commercially generated spent fuel in the US based on publicly available information. In using the information contained in the following data sheets, it should be understood that the data have been assembled from published information, which in some instances was not internally consistent. Moreover, it was sometimes necessary to calculate or infer the values of some attributes from available information. Nor was there always a uniform method of reporting the values of some attributes; for example, an outside surface dose of the loaded cask was sometimes reported to be the maximum acceptable by NRC, while in other cases the maximum actual dose rate expected was reported, and in still other cases the expected average dose rate was reported. A summary comparison of the principal attributes of storage and transportable storage casks is provided and a similar comparison for shipping casks is also shown. References to source data are provided on the individual data sheets for each cask.

  7. Irradiation of Microbes from Spent Nuclear Fuel Storage Pool Environments

    SciTech Connect

    Breckenridge, C.R.; Watkins, C.S.; Bruhn, D.F.; Roberto, F.F.; Tsang, M.N.; Pinhero, P.J.; Brey, R.F.; Wright, R.N.; Windes, W.F.

    1999-09-03

    Microbes have been isolated and identified from spent nuclear fuel storage pools at the Idaho National Engineering and Environmental Laboratory (INEEL). Included among these are Corynebacterium aquaticum, Pseudomonas putida, Comamonas acidovorans, Gluconobacter cerinus, Micrococcus diversus, Rhodococcus rhodochrous, and two strains of sulfate-reducing bacteria (SRB). We examined the sensitivity of these microbes to a variety of total exposures of radiation generated by a 6-MeV linear accelerator (LINAC). The advantage of using a LINAC is that it provides a relatively quick screen of radiation tolerance. In the first set of experiments, we exposed each of the aforementioned microbes along with four additional microbes, pseudomonas aeruginosa, Micrococcus luteus, Escherchia coli, and Deinococcus radiodurans to exposures of 5 x 10{sup 3} and 6 x 10{sup 4} rad. All microbial specimens withstood the lower exposure with little or no reduction in cell population. Upon exposing the microbes to the larger dose of 6 x 10{sup 4} rad, we observed two distinct groupings: microbes that demonstrate resistance to radiation, and microbes that display intolerance through a dramatic reduction from their initial population. Microbes in the radiation tolerant grouping were exposed to 1.1 x 10{sup 5} rad to examine the extent of their resistance. We observe a correlation between radiation resistance and gram stain. The gram-positive species we examined seem to demonstrate a greater radiation resistance.

  8. 5.0. Depletion, activation, and spent fuel source terms

    SciTech Connect

    Wieselquist, William A.

    2016-04-01

    SCALE’s general depletion, activation, and spent fuel source terms analysis capabilities are enabled through a family of modules related to the main ORIGEN depletion/irradiation/decay solver. The nuclide tracking in ORIGEN is based on the principle of explicitly modeling all available nuclides and transitions in the current fundamental nuclear data for decay and neutron-induced transmutation and relies on fundamental cross section and decay data in ENDF/B VII. Cross section data for materials and reaction processes not available in ENDF/B-VII are obtained from the JEFF-3.0/A special purpose European activation library containing 774 materials and 23 reaction channels with 12,617 neutron-induced reactions below 20 MeV. Resonance cross section corrections in the resolved and unresolved range are performed using a continuous-energy treatment by data modules in SCALE. All nuclear decay data, fission product yields, and gamma-ray emission data are developed from ENDF/B-VII.1 evaluations. Decay data include all ground and metastable state nuclides with half-lives greater than 1 millisecond. Using these data sources, ORIGEN currently tracks 174 actinides, 1149 fission products, and 974 activation products. The purpose of this chapter is to describe the stand-alone capabilities and underlying methodology of ORIGEN—as opposed to the integrated depletion capability it provides in all coupled neutron transport/depletion sequences in SCALE, as described in other chapters.

  9. Uncanistered Spent Nuclear fuel Disposal Container System Description Document

    SciTech Connect

    N. E. Pettit

    2001-07-13

    The Uncanistered Spent Nuclear Fuel (SNF) Disposal Container System supports the confinement and isolation of waste within the Engineered Barrier System of the Monitored Geologic Repository (MGR). Disposal containers are loaded with intact uncanistered assemblies and/or individually canistered SNF assemblies and sealed in the surface waste handling facilities, transferred to the underground through the access drifts, and emplaced in emplacement drifts. The Uncanistered SNF Disposal Container provides long-term confinement of the commercial SNF placed inside, and withstands the loading, transfer, emplacement, and retrieval loads and environments. The Uncanistered SNF Disposal Container System provides containment of waste for a designated period of time, and limits radionuclide release. The disposal container maintains the waste in a designated configuration, withstands maximum handling and rockfall loads, limits the individual SNF assembly temperatures after emplacement, limits the introduction of moderator into the disposal container during the criticality control period, resists corrosion in the expected handling and repository environments, and provides containment of waste in the event of an accident.

  10. A NOVEL APPROACH TO SPENT FUEL POOL DECOMMISSIONING

    SciTech Connect

    R. L. Demmer

    2011-04-01

    The Idaho National Laboratory (INL) has been at the forefront of developing methods to reduce the cost and schedule of deactivating spent fuel pools (SFP). Several pools have been deactivated at the INL using an underwater approach with divers. These projects provided a basis for the INL cooperation with the Dresden Nuclear Power Station Unit 1 SFP (Exelon Generation Company) deactivation. It represents the first time that a commercial nuclear power plant (NPP) SFP was decommissioned using this underwater coating process. This approach has advantages in many aspects, particularly in reducing airborne contamination and allowing safer, more cost effective deactivation. The INL pioneered underwater coating process was used to decommission three SFPs with a total combined pool volume of over 900,000 gallons. INL provided engineering support and shared project plans to successfully initiate the Dresden project. This report outlines the steps taken by INL and Exelon to decommission SFPs using the underwater coating process. The rationale used to select the underwater coating process and the advantages and disadvantages are described. Special circumstances are also discussed, such as the use of a remotely-operated underwater vehicle to visually and radiologically map the pool areas that were not readily accessible. A larger project, the INTEC-603 SFP in-situ (grouting) deactivation, is reviewed. Several specific areas where special equipment was employed are discussed and a Lessons Learned evaluation is included.

  11. Packaging and transportation system for K-Basin spent fuel

    SciTech Connect

    Kee, A.T.

    1998-03-03

    This paper describes the cask/transportation system that was designed, procured and delivered to the Hanford K-Basin site at Richland, Washington. The performance requirements and design of the various components -- cask, trailer with cask tie-down system, and the cask operation equipment for the load-out pit -- will be discussed. The presentation will include the details of the factory acceptance testing and its results. The performance requirements for the cask/transportation system was dictated by the constraints imposed by the large number of high priority shipments and the spent fuel pool environment, and the complex interface requirements with other equipment and facility designs. The results of the testing form the basis for the conclusion that the system satisfies the site performance requirements. The cask/transportation system design was driven by the existing facility constraints and the limitations imposed by the large number of shipments over a short two-year period. This system may be useful information for other DOE facilities that may be or will be in a similar situation.

  12. Technology development program for Idaho Chemical Processing Plant spent fuel and waste management

    SciTech Connect

    Ermold, L.F.; Knecht, D.A.; Hogg, G.W.; Olson, A.L.

    1993-08-01

    Acidic high-level radioactive waste (HLW) resulting from fuel reprocessing at the Idaho Chemical Processing Plant (ICPP) for the U.S. Department of Energy (DOE) has been solidified to a calcine since 1963 and stored in stainless steel bins enclosed by concrete vaults. Several different types of unprocessed irradiated DOE-owned fuels are also in storage at the ICPP. In April, 1992, DOE announced that spent fuel would no longer be reprocessed to recover enriched uranium and called for a shutdown of the reprocessing facilities at the ICPP. A new Spent Fuel and HLW Technology Development program was subsequently initiated to develop technologies for immobilizing ICPP spent fuels and HLW for disposal, in accordance with the Nuclear Waste Policy Act. The Program elements include Systems Analysis, Graphite Fuel Disposal, Other Spent Fuel Disposal, Sodium-Bearing Liquid Waste Processing, Calcine Immobilization, and Metal Recycle/Waste Minimization. This paper presents an overview of the ICPP radioactive wastes and current spent fuels, and describes the Spent Fuel and HLW Technology program in more detail.

  13. Disposal of defense spent fuel and HLW from the Idaho Chemical Processing Plant

    SciTech Connect

    Ermold, L.F.; Loo, H.H.; Klingler, R.D.; Herzog, J.D.; Knecht, D.A.

    1992-12-01

    Acid high-level radioactive waste (HLW) resulting from fuel reprocessing at the Idaho Chemical Processing Plant (ICPP) for the US Department of Energy (DOE) has been solidified to a calcine since 1963 and stored in stainless steel bins enclosed by concrete vaults. Several different types of unprocessed irradiated DOE-owned fuels are also in storage ate the ICPP. In April, 1992, DOE announced that spent fuel would no longer be reprocessed to recover enriched uranium and called for a shutdown of the reprocessing facilities at the ICPP. A new Spent Fuel and HLW Technology Development program was subsequently initiated to develop technologies for immobilizing ICPP spent fuels and HLW for disposal, in accordance with the Nuclear Waste Policy Act. The Program elements include Systems Analysis, Graphite Fuel Disposal, Other Spent Fuel Disposal, Sodium-Bearing Liquid Waste Processing, Calcine Immobilization, and Metal Recycle/Waste Minimization. This paper presents an overview of the ICPP radioactive wastes and current spent fuels, with an emphasis on the description of HLW and spent fuels requiring repository disposal.

  14. Oxidation of spent fuel in air at 175 degree to 195 degree C

    SciTech Connect

    Einziger, R.E.; Buchanan, H.C.; Thomas, L.E. ); Stout, R.B. )

    1992-04-01

    Oxidation tests in dry air were conducted on four LWR spent fuels at 175{degrees} and 195{degrees}C to determine the effect of the fuel characteristics on the oxidation state likely to exist at the time leaching occurs in a potential repository. Weight changes were measured and samples were examined by XRD, ceramography, TEM, and TGA. Despite local variations in the grain boundary susceptibility to oxidation, all four fuels progressed toward an apparent endpoint at an oxygen-to-metal (O/M) ratio of 2.4. The sole oxidation product was U{sub 4}O{sub 9+x,} a cubic phase structurally related to UO{sub 2} but with a slightly smaller lattice constant. The growth of the U{sub 4}O{sub 9+x} from the grain boundaries into the UO{sub 2} grains followed parabolic kinetics and had an activation energy of 26.6 kcal/mol. Based on the kinetics, the time required at 95{degrees}C to completely oxidize LWR spent fuel to U{sub 4}O{sub 9+x} would be at least 2000 yr. The next oxidation product to form after the U{sub 4}O{sub 9+x} phase may be U{sub 3}O{sub 8,} but no U{sub 3}O{sub 8} or other dilatational oxidation product has been detected in these accelerated tests conducted up to 25,000 h.

  15. Oxidation of spent fuel in air at 175{degree} to 195{degree}C

    SciTech Connect

    Einziger, R.E.; Buchanan, H.C.; Thomas, L.E.; Stout, R.B.

    1992-04-01

    Oxidation tests in dry air were conducted on four LWR spent fuels at 175{degrees} and 195{degrees}C to determine the effect of the fuel characteristics on the oxidation state likely to exist at the time leaching occurs in a potential repository. Weight changes were measured and samples were examined by XRD, ceramography, TEM, and TGA. Despite local variations in the grain boundary susceptibility to oxidation, all four fuels progressed toward an apparent endpoint at an oxygen-to-metal (O/M) ratio of 2.4. The sole oxidation product was U{sub 4}O{sub 9+x,} a cubic phase structurally related to UO{sub 2} but with a slightly smaller lattice constant. The growth of the U{sub 4}O{sub 9+x} from the grain boundaries into the UO{sub 2} grains followed parabolic kinetics and had an activation energy of 26.6 kcal/mol. Based on the kinetics, the time required at 95{degrees}C to completely oxidize LWR spent fuel to U{sub 4}O{sub 9+x} would be at least 2000 yr. The next oxidation product to form after the U{sub 4}O{sub 9+x} phase may be U{sub 3}O{sub 8,} but no U{sub 3}O{sub 8} or other dilatational oxidation product has been detected in these accelerated tests conducted up to 25,000 h.

  16. 10 CFR 51.23 - Temporary storage of spent fuel after cessation of reactor operation-generic determination of no...

    Code of Federal Regulations, 2010 CFR

    2010-01-01

    ... 10 Energy 2 2010-01-01 2010-01-01 false Temporary storage of spent fuel after cessation of reactor... Procedures § 51.23 Temporary storage of spent fuel after cessation of reactor operation—generic determination... necessary, spent fuel generated in any reactor can be stored safely and without significant...

  17. 10 CFR 51.23 - Temporary storage of spent fuel after cessation of reactor operation-generic determination of no...

    Code of Federal Regulations, 2011 CFR

    2011-01-01

    ... 10 Energy 2 2011-01-01 2011-01-01 false Temporary storage of spent fuel after cessation of reactor... Procedures § 51.23 Temporary storage of spent fuel after cessation of reactor operation—generic determination... necessary, spent fuel generated in any reactor can be stored safely and without significant...

  18. 76 FR 33121 - List of Approved Spent Fuel Storage Casks: HI-STORM Flood/Wind Addition

    Federal Register 2010, 2011, 2012, 2013, 2014

    2011-06-08

    ... 3150-AI90 List of Approved Spent Fuel Storage Casks: HI-STORM Flood/Wind Addition AGENCY: Nuclear... the NRC's spent fuel storage regulations to add the Holtec HI-STORM Flood/Wind cask system to the... Holtec HI- STORM Flood/Wind cask system to the ``List of Approved Spent Fuel Storage Casks'' as...

  19. 76 FR 35137 - Vulnerability and Threat Information for Facilities Storing Spent Nuclear Fuel and High-Level...

    Federal Register 2010, 2011, 2012, 2013, 2014

    2011-06-16

    ... Storing Spent Nuclear Fuel and High-Level Radioactive Waste AGENCY: U.S. Nuclear Regulatory Commission... Independent Storage of Spent Nuclear Fuel, High-Level Radioactive Waste, and Reactor-Related Greater Than...-based security regulations for Spent Nuclear Fuel (SNF) and High-Level Radioactive Waste (HLW)...

  20. Spent Nuclear Fuel Project (SNFP) gas generation from N-Fuel in multi-canister overpacks

    SciTech Connect

    Cooper, T.D.

    1996-08-01

    During the conversion from wet pool storage for spent nuclear fuel at Hanford, gases will be generated from both radiolysis and chemical reactions. The gas generation phenomenon needs to be understood as it applies to safety and design issues,specifically over pressurization of sealed storage containers,and detonation/deflagration of flammable gases. This study provides an initial basis to predict the implications of gas generation on the proposed functional processes for spent nuclear fuel conversion from wet to dry storage. These projections are based upon examination of the history of fuel manufacture at Hanford, irradiation in the reactors, corrosion during wet pool storage, available fuel characterization data and available information from literature. Gas generation via radiolysis and metal corrosion are addressed. The study examines gas generation, the boundary conditio