Sample records for uranium mill-tailings sites

  1. Uranium and radium concentrations in plants growing on uranium mill tailings in South Dakota

    Treesearch

    Mark A. Rumble; Ardell J. Bjugstad

    1986-01-01

    Vegetation and soil samples were collected from a uranium mill tailings site and control sites in South Dakota. Uranium concentrations in soils from the mill tailings averaged 13.3 [micro]g g-1 compared to 5.1 [micro]g g-1 in soils from control sites. 226Ra concentrations in soils averaged 111.0 pCi g...

  2. 40 CFR 192.00 - Applicability.

    Code of Federal Regulations, 2012 CFR

    2012-07-01

    ... AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Standards for the Control of Residual Radioactive Materials from Inactive Uranium Processing Sites § 192.00 Applicability. This... sites under section 108 of the Uranium Mill Tailings Radiation Control Act of 1978 (henceforth...

  3. 40 CFR 192.00 - Applicability.

    Code of Federal Regulations, 2011 CFR

    2011-07-01

    ... AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Standards for the Control of Residual Radioactive Materials from Inactive Uranium Processing Sites § 192.00 Applicability. This... sites under section 108 of the Uranium Mill Tailings Radiation Control Act of 1978 (henceforth...

  4. 40 CFR 192.00 - Applicability.

    Code of Federal Regulations, 2013 CFR

    2013-07-01

    ... AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Standards for the Control of Residual Radioactive Materials from Inactive Uranium Processing Sites § 192.00 Applicability. This... sites under section 108 of the Uranium Mill Tailings Radiation Control Act of 1978 (henceforth...

  5. 40 CFR 192.00 - Applicability.

    Code of Federal Regulations, 2010 CFR

    2010-07-01

    ... AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Standards for the Control of Residual Radioactive Materials from Inactive Uranium Processing Sites § 192.00 Applicability. This... sites under section 108 of the Uranium Mill Tailings Radiation Control Act of 1978 (henceforth...

  6. Process for Transition of Uranium Mill Tailings Radiation Control Act Title II Disposal Sites to the U.S. Department of Energy Office of Legacy Management for Long-Term Surveillance and Maintenance

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    None

    This document presents guidance for implementing the process that the U.S. Department of Energy (DOE) Office of Legacy Management (LM) will use for assuming perpetual responsibility for a closed uranium mill tailings site. The transition process specifically addresses sites regulated under Title II of the Uranium Mill Tailings Radiation Control Act (UMTRCA) but is applicable in principle to the transition of sites under other regulatory structures, such as the Formerly Utilized Sites Remedial Action Program.

  7. Remedial action plan and site design for stabilization of the inactive uranium mill tailings sites at Rifle, Colorado

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1992-02-01

    This appendix assesses the present conditions and data gathered about the two inactive uranium mill tailings sites near Rifle, Colorado, and the designated disposal site six miles north of Rifle in the area of Estes Gulch. It consolidates available engineering, radiological, geotechnical, hydrological, meteorological, and other information pertinent to the design of the Remedial Action Plan (RAP). The data characterize conditions at the mill, tailings, and disposal site so that the Remedial Action Contractor (RAC) may complete final designs for the remedial actions.

  8. Biota of uranium mill tailings near the Black Hills

    Treesearch

    Mark A. Rumble

    1982-01-01

    Reclamation" often implies the enhancement of the land as wildlife habitat or for other productive uses. However, there are situations where revegetation to stabilize erosion is the only desired goal. Uranium mining and mill sites may fall into this later category. Data pertaining to plant and animal components on revegetated uranium mill tailings was collected....

  9. Remedial action plan and site design for stabilization of the inactive uranium mill tailings sites at Rifle, Colorado. Volume 2, Appendices D and E: Final report

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1992-02-01

    This appendix assesses the present conditions and data gathered about the two inactive uranium mill tailings sites near Rifle, Colorado, and the designated disposal site six miles north of Rifle in the area of Estes Gulch. It consolidates available engineering, radiological, geotechnical, hydrological, meteorological, and other information pertinent to the design of the Remedial Action Plan (RAP). The data characterize conditions at the mill, tailings, and disposal site so that the Remedial Action Contractor (RAC) may complete final designs for the remedial actions.

  10. Uptake of uranium by aquatic plants growing in fresh water ecosystem around uranium mill tailings pond at Jaduguda, India.

    PubMed

    Jha, V N; Tripathi, R M; Sethy, N K; Sahoo, S K

    2016-01-01

    Concentration of uranium was determined in aquatic plants and substrate (sediment or water) of fresh water ecosystem on and around uranium mill tailings pond at Jaduguda, India. Aquatic plant/substrate concentration ratios (CRs) of uranium were estimated for different sites on and around the uranium mill tailings disposal area. These sites include upstream and downstream side of surface water sources carrying the treated tailings effluent, a small pond inside tailings disposal area and residual water of this area. Three types of plant groups were investigated namely algae (filamentous and non-filamentous), other free floating & water submerged and sediment rooted plants. Wide variability in concentration ratio was observed for different groups of plants studied. The filamentous algae uranium concentration was significantly correlated with that of water (r=0.86, p<0.003). For sediment rooted plants significant correlation was found between uranium concentration in plant and the substrate (r=0.88, p<0.001). Both for other free floating species and sediment rooted plants, uranium concentration was significantly correlated with Mn, Fe, and Ni concentration of plants (p<0.01). Filamentous algae, Jussiaea and Pistia owing to their high bioproductivity, biomass, uranium accumulation and concentration ratio can be useful for prospecting phytoremediation of stream carrying treated or untreated uranium mill tailings effluent. Copyright © 2015 Elsevier B.V. All rights reserved.

  11. Remedial Action Plan and site design for stabilization of the inactive uranium mill tailings site at Durango, Colorado: Remedial action selection report. Revised final report

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1991-12-01

    The uranium mill tailings site near Durango, Colorado, was one of 24 inactive uranium mill sites designated to be remediated by the US Department of Energy (DOE) under the Uranium Mill Tailings Radiation Control Act of 1978 (UMTRCA). Part of the UMTRCA requires that the US Nuclear Regulatory Commission (NRC) concur with the DOE`s Remedial Action Plan (RAP) and certify that the remedial action conducted at the site complies with the standards promulgated by the US Environmental Protection Agency (EPA). Included in the RAP is this Remedial Action Selection Report (RAS), which has been developed to serve a two-fold purpose.more » First, it describes the activities that have been conducted by the DOE to accomplish remediation and long-term stabilization and control of the radioactive materials at the inactive uranium mill processing site near Durango, Colorado. Secondly, this document and the rest of the RAP, upon concurrence and execution by the DOE, the State of Colorado, and the NRC, become Appendix B of the Cooperative Agreement between the DOE and the State of Colorado.« less

  12. Remedial Action Plan and site design for stabilization of the inactive uranium mill tailings site at Durango, Colorado: Remedial action selection report

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1991-12-01

    The uranium mill tailings site near Durango, Colorado, was one of 24 inactive uranium mill sites designated to be remediated by the US Department of Energy (DOE) under the Uranium Mill Tailings Radiation Control Act of 1978 (UMTRCA). Part of the UMTRCA requires that the US Nuclear Regulatory Commission (NRC) concur with the DOE's Remedial Action Plan (RAP) and certify that the remedial action conducted at the site complies with the standards promulgated by the US Environmental Protection Agency (EPA). Included in the RAP is this Remedial Action Selection Report (RAS), which has been developed to serve a two-fold purpose.more » First, it describes the activities that have been conducted by the DOE to accomplish remediation and long-term stabilization and control of the radioactive materials at the inactive uranium mill processing site near Durango, Colorado. Secondly, this document and the rest of the RAP, upon concurrence and execution by the DOE, the State of Colorado, and the NRC, become Appendix B of the Cooperative Agreement between the DOE and the State of Colorado.« less

  13. UMTRA project water sampling and analysis plan, Durango, Colorado

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1994-01-01

    Surface remedial action has been completed at the Uranium Mill Tailings Remedial Action Project in Durango, Colorado. Contaminated soil and debris have been removed from the former processing site and placed in the Bodo Canyon disposal cell. Ground water at the former uranium mill/tailings site and raffinate pond area has been contaminated by the former milling operations. The ground water at the disposal site was not impacted by the former milling operations at the time of the cell`s construction. Activities for fiscal 1994 involve ground water sampling and site characterization of the disposal site.

  14. Engineering assessment of inactive uranium mill tailings: Maybell Site, Maybell, Colorado

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    None

    1981-09-01

    Ford, Bacon and Davis Utah Inc. has reevaluated the Maybell site in order to revise the October 1977 engineering assessment of the problems resulting from the existence of radioactive uranium mill tailings at Maybell, Colorado. This engineering assessment has included the preparation of topographic maps, the performance of core drillings and radiometric measurements sufficient to determine areas and volumes of tailings and radiation exposures of individuals and nearby populations, the investigations of site hydrology and meteorology, and the evaluation and costing of alternative corrective actions. Radon gas released from the 2.6 million dry tons of tailings at the Maybell sitemore » constitutes the most significant environmental impact, although windblown tailings and external gamma radiation also are factors. The two alternative actions presented in this engineering assessment range from millsite decontamination with the addition of 3 m of stabilization cover material (Option I), to disposal of the tailings in a nearby open pit mine and decontamination of the tailings site (Option II). Cost estimates for the two options are about $11,700,000 for stabilization in-place and about $22,700,000 for disposal within a distance of 2 mi. Three principal alternatives for the reprocessing of the Maybell tailings were examined: (a) heap leaching; (b) treatment at an existing mill; and (c) reprocessing at a new conventional mill constructed for tailings reprocessing. The cost of the uranium recovered would be about $125 and $165/lb of U/sub 3/O/sub 8/ by heap leach and conventional plant processes, respectively. The spot market price for uranium was $25/lb early in 1981. Therefore, reprocessing the tailings for uranium recovery is not economically attractive at present.« less

  15. Engineering assessment of inactive uranium mill tailings: Maybell Site, Maybell, Colorado. Summary

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    None

    1981-09-01

    Ford, Bacon and Davis Utah Inc. has reevaluated the Maybell site in order to revise the October 1977 engineering assessment of the problems resulting from the existence of radioactive uranium mill tailings at Maybell, Colorado. This engineering assessment has included the preparation of topographic maps, the performance of core drillings and radiometric measurements sufficient to determine areas and volumes of tailings and radiation exposures of individuals and nearby populations, the investigations of site hydrology and meteorology, and the evaluation and costing of alternative corrective actions. Radon gas released from the 2.6 million dry tons of tailings at the Maybell sitemore » constitutes the most significant environmental impact, although windblown tailings and external gamma radiation also are factors. The two alternative actions presented in this engineering assessment range from millsite decontamination with the addition of 3 m of stabilization cover material (Option I), to disposal of the tailings in a nearby open pit mine and decontamination of the tailings site (Option II). Cost estimates for the two options are about $11,700,000 for stabilization in-place and about $22,700,000 for disposal within a distance of 2 mi. Three principal alternatives for the reprocessing of the Maybell tailings were examined: (a) heap leaching; (b) treatment at an existing mill; and (c) reprocessing at a new conventional mill constructed for tailings reprocessing. The cost of the uranium recovered would be about $125 and $165/lb of U/sub 3/O/sub 8/ by heap leach and conventional plant processes, respectively. The spot market price for uranium was $25/lb early in 1981. Therefore, reprocessing the tailings for uranium recovery is not economically attractive at present.« less

  16. Environmental assessment of remedial action at the Slick Rock uranium mill tailings sites, Slick Rock, Colorado. Revision 1

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1994-09-01

    The Uranium Mill Tailings Radiation Control Act of 1978 (42 USC {section}7901 et seq.), hereafter referred to as the UMTRCA, authorized the US Department of Energy (DOE) to clean up two uranium mill tailings processing sites near Slick Rock, Colorado, in San Miquel County. Contaminated materials cover an estimated 63 acres of the Union Carbide (UC) processing site and 15 ac of the North Continent (NC) processing site. The sites are within 1 mile of each other and are adjacent to the Dolores River. The sites contain concrete foundations of mill buildings, tailings piles, and areas contaminated by windblown andmore » waterborne radioactive tailings materials. The total estimated volume of contaminated materials is approximately 621,300 cubic yards (yd{sup 3}). In addition to the contamination in the two processing site areas, four VPs were found to contain contamination. As a result of the tailings being exposed to the environment, contamination associated with the UC and NC sites has leached into shallow ground water. Surface water has not been affected. The closest residence is approximately 0.3 air mi from either site. The proposed action is to remediate the UC and NC sites by removing all contaminated materials within the designing site boundaries or otherwise associated with the sites, and relocating them to, and stabilizing them at, a location approximately 5 road mi northeast of the sites on land administered by the Bureau of Land Management (BLM).« less

  17. Environmental Assessment of remedial action at the Ambrosia Lake uranium mill tailings site, Ambrosia Lake, New Mexico

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1987-06-01

    This document assesses and compares the environmental impacts of various alternatives for remedial action at the Ambrosia Lake uranium mill tailings site located near Ambrosia Lake, New Mexico. The designated site covers 196 acres and contains 111 acres of tailings and some of the original mill structures. The Uranium Mill Tailings Radiation Control Act (UMTRCA), Public Law 95-604, authorizes the US Department of Energy to clean up the site to reduce the potential health impacts associated with the residual radioactive materials remaining at the site and at associated properties off the site. The US Environmental Protection Agency promulgated standards formore » th remedial action (40 CFR Part 192). Remedial action must be performed in accordance with these standards and with the concurrence of the Nuclear Regulatory Commission. The proposed action is to stabilize the tailings at their present location by consolidating the tailings and associated contaminated materials into a recontoured pile. A radon barrier would be constructed over the pile and various erosion protection measures would be taken to assure the long-term stability of the pile. Another alternative which would involve moving the tailings to a new location is also assessed in this document. This alternative would generally involve greater short-term impacts and costs but would result in stabilization of the tailings at an undeveloped location. The no action alternative is also assessed in this document.« less

  18. Remedial Action Plan and site design for stabilization of the inactive uranium mill tailings site at Durango, Colorado: Attachment 3, Groundwater hydrology report. Revised final report

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1991-12-01

    The US Environmental Protection Agency (EPA) has established health and environmental protection regulations to correct and prevent groundwater contamination resulting from processing activities at inactive uranium milling sites. According to the Uranium Mill Tailings Radiation Control Act of 1978, (UMTRCA) the US Department of Energy (DOE) is responsible for assessing the inactive uranium processing sites. The DOE has determined this assessment shall include information on hydrogeologic site characterization. The water resources protection strategy that describes how the proposed action will comply with the EPA groundwater protection standards is presented in Attachment 4. Site characterization activities discussed in this section include:more » Characterization of the hydrogeologic environment; characterization of existing groundwater quality; definition of physical and chemical characteristics of the potential contaminant source; and description of local water resources.« less

  19. 10 CFR 40.28 - General license for custody and long-term care of uranium or thorium byproduct materials disposal...

    Code of Federal Regulations, 2011 CFR

    2011-01-01

    ... 10 Energy 1 2011-01-01 2011-01-01 false General license for custody and long-term care of uranium... long-term care of uranium or thorium byproduct materials disposal sites. (a) A general license is... in this part for uranium or thorium mill tailings sites closed under title II of the Uranium Mill...

  20. 10 CFR 40.28 - General license for custody and long-term care of uranium or thorium byproduct materials disposal...

    Code of Federal Regulations, 2012 CFR

    2012-01-01

    ... 10 Energy 1 2012-01-01 2012-01-01 false General license for custody and long-term care of uranium... long-term care of uranium or thorium byproduct materials disposal sites. (a) A general license is... in this part for uranium or thorium mill tailings sites closed under title II of the Uranium Mill...

  1. 10 CFR 40.28 - General license for custody and long-term care of uranium or thorium byproduct materials disposal...

    Code of Federal Regulations, 2013 CFR

    2013-01-01

    ... 10 Energy 1 2013-01-01 2013-01-01 false General license for custody and long-term care of uranium... long-term care of uranium or thorium byproduct materials disposal sites. (a) A general license is... in this part for uranium or thorium mill tailings sites closed under title II of the Uranium Mill...

  2. 10 CFR 40.28 - General license for custody and long-term care of uranium or thorium byproduct materials disposal...

    Code of Federal Regulations, 2014 CFR

    2014-01-01

    ... 10 Energy 1 2014-01-01 2014-01-01 false General license for custody and long-term care of uranium... long-term care of uranium or thorium byproduct materials disposal sites. (a) A general license is... in this part for uranium or thorium mill tailings sites closed under title II of the Uranium Mill...

  3. 1996 monitoring report for the Gunnison, Colorado, wetlands mitigation plan

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    NONE

    1996-12-01

    The US Department of Energy (DOE) administers the Uranium Mill Tailings Remedial Action (UMTRA) Project to clean up uranium mill tailings and other surface contamination at 24 abandoned uranium mill sites in 10 states. One of these abandoned mill sites was near the town of Gunnison, Colorado. Surface remediation was completed at the Gunnison site in December 1995. Remedial action resulted in the elimination of 4.3 acres of wetlands and mitigation of this loss is through the enhancement of 17.8 acres of riparian plant communities in six spring-fed areas on US Bureau of Land Management mitigation sites. A five-year monitoringmore » program was then implemented to document the response of vegetation and wildlife to the exclusion of livestock. This report provides the results of the third year of the monitoring program.« less

  4. Engineering assessment of inactive uranium mill tailings, Durango Site, Durango, Colorado

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1981-06-01

    Ford, Bacon and Davis Utah Inc. has reevaluated the Durango site in order to revise the November 1977 engineering assessment of the problems resulting from the existence of radioactive uranium mill tailings at Durango, Colorado. This engineering assessment has included the preparation of topographic maps, the performance of core drillings and radiometric measurements sufficient to determine areas and volumes of tailings and radiation exposures of individuals and nearby populations, the investigations of site hydrology and meteorology, and the evaluation and costing of alternative corrective actions. Radon gas released from the nearly 1.6 million tons of tailings at the Durango sitemore » constitutes the most significant environmental impact, although windblown tailings and external gamma radiation also are factors. The four alternative actions presented in this engineering assessment range from millsite and off-site decontamination with the addition of 3 m of stabilization cover material (Option I), to removal of the tailings to remote disposal sites and decontamination of the tailings site (Options II through IV). Cost estimates for the seven options range from about $10,700,000 for stabilization in-place, to about $21,800,000 for disposal at a distance of about 10 mi. Three principal alternatives for the reprocessing of the Durango tailings were examined: (a) heap leaching; (b) treatment at an existing mill; and (c) reprocessing at a new conventional mill constructed for tailings reprocessing. The cost of the uranium recovered would be about $30/lb U/sub 3/O/sub 8/ by either heap leach or conventional plant processes.« less

  5. Nuclear facility decommissioning and site remedial actions: A selected bibliography, Volume 18. Part 1B: Citations with abstracts, sections 10 through 16

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    NONE

    1997-09-01

    This bibliography contains 3,638 citations with abstracts of documents relevant to environmental restoration, nuclear facility decontamination and decommissioning (D and D), uranium mill tailings management, and site remedial actions. The bibliography contains scientific, technical, financial, and regulatory information that pertains to DOE environmental restoration programs. The citations are separated by topic into 16 sections, including (1) DOE Environmental Restoration Program; (2) DOE D and D Program; (3) Nuclear Facilities Decommissioning; (4) DOE Formerly Utilized sites Remedial Action Program; (5) NORM-Contaminated Site Restoration; (6) DOE Uranium Mill Tailings Remedial Action Project; (7) Uranium Mill Tailings Management; (8) DOE Site-Wide Remedial Actions;more » (9) DOE Onsite Remedial Action Projects; (10) Contaminated Site Remedial Actions; (11) DOE Underground Storage Tank Remediation; (12) DOE Technology Development, Demonstration, and Evaluation; (13) Soil Remediation; (14) Groundwater Remediation; (15) Environmental Measurements, Analysis, and Decision-Making; and (16) Environmental Management Issues.« less

  6. Baseline risk assessment of ground water contamination at the uranium mill tailings site near Durango, Colorado

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1995-02-01

    This risk assessment evaluates the possibility of health and environmental risks from contaminated ground water at the uranium mill tailings site near Durango, Colorado. The former uranium processing site`s contaminated soil and material were removed and placed at a disposal site located in Body Canyon, Colorado, during 1986--1991 by the US Departments of Energy`s Uranium Mill Tailings Remedial Action (UMTRA) Project. Currently, the UMTRA Project is evaluating the nature and extent of ground water contamination at the site. This risk assessment follows an approach similar to that used by the US Environmental Protection Agency. The first step is to determinemore » what site-related contaminants are found in ground water samples. The next step in the risk assessment is to determine how much of these contaminants people might ingest if they got their drinking water from a well on the site. In accordance with standard practice for this type of risk assessment, the highest contaminant concentrations from the most contaminated wells are used. The risk assessment then explains the possible health problems that could result from this amount of contamination.« less

  7. Summary of the engineering assessment of inactive uranium mill tailings, Durango Site, Durango, Colorado

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1981-06-01

    Ford, Bacon and Davis Utah Inc. has reevaluated the Durango site in order to revise the November 1977 engineering assessment of the problems resulting from the existence of radioactive uranium mill tailings at Durango, Colorado. This engineering assessment has included the preparation of topographic measurements sufficient to determine areas and volumes of tailings and radiation exposures of individuals and nearby populations, the investigations of site hydrology and meteorology, and the evaluation and costing of alternative corrective actions. Radon gas released from the nearly 1.6 million tons of tailings at the Durango site constitutes the most significant environmental impact, although windblownmore » tailings and external gamma radiation also are factors. The four alternative actions presented in this engineering assessment range from millsite and off-site decontamination with the addition of 3 m of stabilization cover material (Option I), to removal of the tailings to remote disposal sites and decontamination of the tailings site (Options II through IV). Cost estimates for the seven options range from about $10,700,000 for stabilization in-place, to about $21,800,000 for disposal at a distance of about 10 mi. Three principal alternatives for the reprocessing of the Durango tailings were examined: (a) heap leaching; (b) treatment at an existing mill; and (c) reprocessing at a new conventional mill constructed for tailings reprocessing.« less

  8. Environmental assessment of remedial action at the Gunnison Uranium Mill Tailings Site, Gunnison, Colorado. [UMTRA Project

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Bachrach, A.; Hoopes, J.; Morycz, D.

    1984-12-01

    This document assesses and compares the environmental impacts of various alternatives for remedial action at the Gunnison uranium of mill tailings site located 0.5 miles south of Gunnison, Colorado. The site covers 56 acres and contains 35 acres of tailings, 2 of the original mill buildings and a water tower. The Uranium Mill Tailings Radiation Control of Act of 1978 (UMTRCA), Public Law 95-604, authorizes the US Department of Energy to clean up the site to reduce the potential health impacts associated with the residual radioactive materials remaining at the site and at associated (vicinity) properties off the site. Themore » US Environmental Protection Agency promulgated standards for the remedial actions (40 CFR 192). Remedial actions must be performed in accordance with these standards and with the occurrence of the Nuclear Regulatory Commission. Four alternatives have been addressed in this document. The first alternative is to consolidate the tailings and associated contaminated soils into a recontoured pile on the southern portion of the existing site. A radon barrier of silty clay would be constructed over the pile and various erosion control measures would be taken to assure the long-term integrity of the pile. Two other alternatives which involve moving the tailings to new locations are assessed in this document. These alternatives generally involve greater short-term impacts and are more costly but would result in the tailings being stabilized in a location farther from the city of Gunnison. The no action alternative is also assessed.« less

  9. Engineering assessment of inactive uranium mill tailings, Gunnison Site, Gunnison, Colorado. Phase II, Title I

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    None

    1977-11-01

    Ford, Bacon and Davis Utah Inc. has performed an engineering assessment of the problems resulting from the existence of radioactive uranium mill tailings at Gunnison, Colorado. The Phase II - Title I services include the preparation of topographic measurements sufficient to determine areas and volumes of tailings and other radium-contaminated materials, the evaluation of resulting radiation exposures of individuals and nearby populations, the investigation of site hydrology and meteorology, and the evaluation and costing of alternative corrective actions. Radon gas release from the 0.5 million tons of tailings at the Gunnison site constitutes the most significant environmental impact, although windblownmore » tailings and external gamma radiation are also factors. The nine alternative actions presented range from millsite decontamination (Option I), to adding various depths of stabilization cover material (Options II and III), to removal of the tailings to long-term storage sites and decontamination of the present site (Options IV through IX). Cost estimates for the nine options range from $480,000 to $5,890,000. Reprocessing the tailings for uranium does not appear to be economically attractive at present.« less

  10. Cleanup protocol for 226Ra-contaminated cobbly soil at UMTRA Project sites

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Gonzales, D.E.; Millard, J.B.; Miller, M.L.

    The nonuniform distribution of 226Ra and other radiological contamination of cobbly soil encountered on several Uranium Mill Tailings Remedial Action Project sites is presented and discussed, and the concomitant challenges to the intent and implementation of the U.S. Environmental Protection Agency's soil cleanup standards are noted. In response to technical assessments and information presented to the U.S. Nuclear Regulatory Commission by the U.S. Department of Energy, the Nuclear Regulatory Commission has recently resolved the dilemma by concluding that compliance with Environmental Protection Agency soil cleanup standards for cobby soil at Uranium Mill Tailings Remedial Action Project sites would be adequatelymore » attained using bulk radionuclide concentrations, instead of requiring that the radionuclide concentration of the finer soil fraction passing a No. 4 mesh sieve met the standards. A Nuclear Regulatory Commission-approved procedure developed for cobbly soil remediation is outlined and discussed. The site-specific implementation of this procedure at Uranium Mill Tailings Remedial Action Project sites containing cobbly soil is estimated to save millions of dollars.« less

  11. DOE Office of Scientific and Technical Information (OSTI.GOV)

    Peterson, Dave; Miller, David; Kautsky, Mark

    A uranium- and vanadium-ore-processing mill operated from 1954 to 1968 within the Navajo Nation near Shiprock, New Mexico. By September 1986, all tailings and structures on the former mill property were encapsulated in a disposal cell built on top of two existing tailings piles on the Shiprock site (the site) [1]. Local groundwater was contaminated by multiple inorganic constituents as a result of the milling operations. The U.S. Department of Energy (DOE) took over management of the site in 1978 as part of the Uranium Mill Tailings Remedial Action (UMTRA) Project. The DOE Office of Legacy Management currently manages ongoingmore » activities at the former mill facility, including groundwater remediation. Remediation activities are designed primarily to reduce the concentrations and total plume mass of the mill-related contaminants sulfate, uranium, and nitrate. In addition to contaminating groundwater in alluvial and bedrock sediments directly below the mill site, ore processing led to contamination of a nearby floodplain bordering the San Juan River. Groundwater in a shallow alluvial aquifer beneath the floodplain is strongly influenced by the morphology of the river channel as well as changing flows in the river, which provides drainage for regional runoff from the San Juan Mountains of Colorado. As part of a recent study of the floodplain hydrology, a revised conceptual model was developed for the alluvial aquifer along with an updated status of contaminant plumes that have been impacted by more than 10 years of groundwater pumping for site remediation purposes. Several findings from the recent study will be discussed here.« less

  12. DOE Office of Scientific and Technical Information (OSTI.GOV)

    Goins, L.F.; Webb, J.R.; Cravens, C.D.

    This publication contains 1035 abstracted references on environmental restoration, nuclear facility decommissioning, uranium mill tailings management, and site remedial actions. These citations constitute the thirteenth in a series of reports prepared annually for the US Department of Energy (DOE) Environmental Restoration programs. Citations to foreign and domestic literature of all types. There are 13 major sections of the publication, including: (1) DOE Decontamination and Decommissioning Program; (2) Nuclear Facilities Decommissioning; (3) DOE Formerly Utilized Sites Remedial Action Program; (4) DOE Uranium Mill Tailings Remedial Action Project; (5) Uranium Mill Tailings Management; (6) DOE Environmental Restoration Program; (7) DOE Site-Specific Remedialmore » Actions; (8) Contaminated Site Restoration; (9) Remediation of Contaminated Soil and Groundwater; (10) Environmental Data Measurements, Management, and Evaluation; (11) Remedial Action Assessment and Decision-Making; (12) Technology Development and Evaluation; and (13) Environmental and Waste Management Issues. Bibliographic references are arranged in nine subject categories by geographic location and then alphabetically by first author, corporate affiliation, or publication title. Indexes are provided for author, corporate affiliation, title word, publication description, geographic location, subject category, and key word.« less

  13. Uranium Mill Tailings Remedial Action Project Safety Advancement Field Effort (SAFE) Program

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1994-02-01

    In 1992, the Uranium Mill Tailings Remedial Action (UMTRA) Project experienced several health and safety related incidents at active remediation project sites. As a result, the U.S. Department of Energy (DOE) directed the Technical Assistance Contractor (TAC) to establish a program increasing the DOE`s overall presence at operational remediation sites to identify and minimize risks in operations to the fullest extent possible (Attachments A and B). In response, the TAC, in cooperation with the DOE and the Remedial Action Contractor (RAC), developed the Safety Advancement Field Effort (SAFE) Program.

  14. 40 CFR 192.03 - Monitoring.

    Code of Federal Regulations, 2012 CFR

    2012-07-01

    ... AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Standards for the Control of Residual Radioactive Materials from Inactive Uranium Processing Sites § 192.03 Monitoring. A...

  15. 40 CFR 192.03 - Monitoring.

    Code of Federal Regulations, 2011 CFR

    2011-07-01

    ... AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Standards for the Control of Residual Radioactive Materials from Inactive Uranium Processing Sites § 192.03 Monitoring. A...

  16. 40 CFR 192.03 - Monitoring.

    Code of Federal Regulations, 2013 CFR

    2013-07-01

    ... AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Standards for the Control of Residual Radioactive Materials from Inactive Uranium Processing Sites § 192.03 Monitoring. A...

  17. 40 CFR 192.03 - Monitoring.

    Code of Federal Regulations, 2010 CFR

    2010-07-01

    ... AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Standards for the Control of Residual Radioactive Materials from Inactive Uranium Processing Sites § 192.03 Monitoring. A...

  18. Nuclear facility decommissioning and site remedial actions: A selected bibliography, Volume 13: Part 1, Main text

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Goins, L.F.; Webb, J.R.; Cravens, C.D.

    1992-09-01

    This publication contains 1035 abstracted references on environmental restoration, nuclear facility decommissioning, uranium mill tailings management, and site remedial actions. These citations constitute the thirteenth in a series of reports prepared annually for the US Department of Energy (DOE) Environmental Restoration programs. Citations to foreign and domestic literature of all types. There are 13 major sections of the publication, including: (1) DOE Decontamination and Decommissioning Program; (2) Nuclear Facilities Decommissioning; (3) DOE Formerly Utilized Sites Remedial Action Program; (4) DOE Uranium Mill Tailings Remedial Action Project; (5) Uranium Mill Tailings Management; (6) DOE Environmental Restoration Program; (7) DOE Site-Specific Remedialmore » Actions; (8) Contaminated Site Restoration; (9) Remediation of Contaminated Soil and Groundwater; (10) Environmental Data Measurements, Management, and Evaluation; (11) Remedial Action Assessment and Decision-Making; (12) Technology Development and Evaluation; and (13) Environmental and Waste Management Issues. Bibliographic references are arranged in nine subject categories by geographic location and then alphabetically by first author, corporate affiliation, or publication title. Indexes are provided for author, corporate affiliation, title word, publication description, geographic location, subject category, and key word.« less

  19. Uranium association with iron-bearing phases in mill tailings from Gunnar, Canada.

    PubMed

    Othmane, Guillaume; Allard, Thierry; Morin, Guillaume; Sélo, Madeleine; Brest, Jessica; Llorens, Isabelle; Chen, Ning; Bargar, John R; Fayek, Mostafa; Calas, Georges

    2013-11-19

    The speciation of uranium was studied in the mill tailings of the Gunnar uranium mine (Saskatchewan, Canada), which operated in the 1950s and 1960s. The nature, quantification, and spatial distribution of uranium-bearing phases were investigated by chemical and mineralogical analyses, fission track mapping, electron microscopy, and X-ray absorption near edge structure (XANES) and extended X-ray absorption fine structure (EXAFS) spectroscopies at the U LIII-edge and Fe K-edge. In addition to uranium-containing phases from the ore, uranium is mostly associated with iron-bearing minerals in all tailing sites. XANES and EXAFS data and transmission electron microscopy analyses of the samples with the highest uranium concentrations (∼400-700 mg kg(-1) of U) demonstrate that uranium primarily occurs as monomeric uranyl ions (UO2(2+)), forming inner-sphere surface complexes bound to ferrihydrite (50-70% of the total U) and to a lesser extent to chlorite (30-40% of the total U). Thus, the stability and mobility of uranium at the Gunnar site are mainly influenced by sorption/desorption processes. In this context, acidic pH or alkaline pH with the presence of UO2(2+)- and/or Fe(3+)-complexing agents (e.g., carbonate) could potentially solubilize U in the tailings pore waters.

  20. Engineering assessment of inactive uranium mill tailings, Durango site, Durango, Colorado. A summary of the Phase II, Title I

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1977-11-01

    Ford, Bacon and Davis Utah Inc. has performed an engineering assessment of the problems resulting from the existence of radioactive uranium mill tailings at Durango, Colorado. The Phase II, Title I services include the preparation of topographic maps, the performance of core drillings and radiometric measurements sufficient to determine areas and volumes of tailings and other radium-contaminated materials, the evaluation of resulting radiation exposures of individuals and nearby populations, the investigation of site hydrology and meteorology and the evaluation and costing of alternative corrective actions. Radon gas release from the 1.555 million tons of tailings at the Durango site constitutesmore » the most significant environmental impact, although windblown tailings and external gamma radiation are also factors. The eight alternative actions presented range from vegetative stabilization (Option I), to contouring and stabilizing in-place with varying depths of cover material (Options II and III), to removal to an isolated long-term disposal site (Options V to VIII). All options include remedial action costs for offsite locations where tailings have been placed. Costs estimated for the eight options range from $4,340,000 to $13,590,000. Reprocessing the tailings for uranium is sufficiently economically attractive to justify reprocessing in conjunction with each of the options.« less

  1. Engineering assessment of inactive uranium mill tailings, Durango site, Durango, Colorado. Phase II, Title I

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1977-11-01

    Ford, Bacon and Davis Utah Inc. has performed an engineering assessment of the problems resulting from the existence of radioactive uranium mill tailings at Durango, Colorado. The Phase II, Title I services include the preparation of topographic maps, the performance of core drillings and radiometric measurements sufficient to determine areas and volumes of tailings and other radium-contaminated materials, the evaluation of resulting radiation exposures of individuals and nearby populations, the investigation of site hydrology and meteorology and the evaluation and costing of alternative corrective actions. Radon gas release from the 1.555 million tons of tailings at the Durango site constitutesmore » the most significant environmental impact, although windblown tailings and external gamma radiation are also factors. The eight alternative actions presented range from vegetative stabilization (Option I), to contouring and stabilizing in-place with varying depths of cover material (Options II and III), to removal to an isolated long-term disposal site (Options V to VIII). All options include remedial action costs for offsite locations where tailings have been placed. Costs estimated for the eight options range from $4,340,000 to $13,590,000. Reprocessing the tailings for uranium is sufficiently economically attractive to justify reprocessing in conjunction with each of the options.« less

  2. Nuclear facility decommissioning and site remedial actions: A selected bibliography: Volume 8

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Owen, P.T.; Michelson, D.C.; Knox, N.P.

    1987-09-01

    The 553 abstracted references on nuclear facility decommissioning, uranium mill tailings management, and site remedial actions constitute the eighth in a series of reports. Foreign and domestic literature of all types - technical reports, progress reports, journal articles, symposia proceedings, theses, books, patents, legislation, and research project descriptions - has been included. The bibliography contains scientific, technical, economic, regulatory, and legal information pertinent to the US Department of energy's remedial action program. Major chapters are Surplus Facilities Management Program, Nuclear Facilities Decommissioning, Formerly Utilized Sites Remedial Action Program, Facilities Contaminated with Naturally Occurring Radionuclides, Uranium Mill Tailings Remedial Action Program,more » Uranium Mill Tailings Management, Technical Measurements Center, and General Remedial Action Program Studies. Chapter sections for chapters 1, 2, 5, and 6 include Design, Planning, and Regulations; Environmental Studies and Site Surveys; Health, Safety, and Biomedical Studies; Decontamination Studies; Dismantlement and Demolition; Site Stabilization and Reclamation; Waste Disposal; Remedial Action Experience; and General Studies. Within these categories, references are arranged alphabetically by first author. Those references having no individual author are listed by corporate affiliation or by publication description. Indexes are provided for author, corporate affiliation, title word, publication description, geographic location, and keywords. The appendix contains a list of frequently used acronyms and abbreviations.« less

  3. 40 CFR 23.8 - Timing of Administrator's action under Uranium Mill Tailings Radiation Control Act of 1978.

    Code of Federal Regulations, 2010 CFR

    2010-07-01

    ... 40 Protection of Environment 1 2010-07-01 2010-07-01 false Timing of Administrator's action under Uranium Mill Tailings Radiation Control Act of 1978. 23.8 Section 23.8 Protection of Environment... Administrator's action under Uranium Mill Tailings Radiation Control Act of 1978. Unless the Administrator...

  4. 40 CFR 23.8 - Timing of Administrator's action under Uranium Mill Tailings Radiation Control Act of 1978.

    Code of Federal Regulations, 2013 CFR

    2013-07-01

    ... 40 Protection of Environment 1 2013-07-01 2013-07-01 false Timing of Administrator's action under Uranium Mill Tailings Radiation Control Act of 1978. 23.8 Section 23.8 Protection of Environment... Administrator's action under Uranium Mill Tailings Radiation Control Act of 1978. Unless the Administrator...

  5. 40 CFR 23.8 - Timing of Administrator's action under Uranium Mill Tailings Radiation Control Act of 1978.

    Code of Federal Regulations, 2014 CFR

    2014-07-01

    ... 40 Protection of Environment 1 2014-07-01 2014-07-01 false Timing of Administrator's action under Uranium Mill Tailings Radiation Control Act of 1978. 23.8 Section 23.8 Protection of Environment... Administrator's action under Uranium Mill Tailings Radiation Control Act of 1978. Unless the Administrator...

  6. 40 CFR 23.8 - Timing of Administrator's action under Uranium Mill Tailings Radiation Control Act of 1978.

    Code of Federal Regulations, 2012 CFR

    2012-07-01

    ... 40 Protection of Environment 1 2012-07-01 2012-07-01 false Timing of Administrator's action under Uranium Mill Tailings Radiation Control Act of 1978. 23.8 Section 23.8 Protection of Environment... Administrator's action under Uranium Mill Tailings Radiation Control Act of 1978. Unless the Administrator...

  7. 40 CFR 23.8 - Timing of Administrator's action under Uranium Mill Tailings Radiation Control Act of 1978.

    Code of Federal Regulations, 2011 CFR

    2011-07-01

    ... 40 Protection of Environment 1 2011-07-01 2011-07-01 false Timing of Administrator's action under Uranium Mill Tailings Radiation Control Act of 1978. 23.8 Section 23.8 Protection of Environment... Administrator's action under Uranium Mill Tailings Radiation Control Act of 1978. Unless the Administrator...

  8. Remedial Action Plan and site design for stabilization of the inactive uranium mill tailings site at Durango, Colorado: Attachment 4, Water resources protection strategy

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1991-12-01

    To achieve compliance with the proposed US Environmental Protection Agency (EPA) groundwater protection standards (Subpart A of 40 CFR 192), the US Department of Energy (DOE) proposes to meet background concentrations or the EPA maximum concentration limits (MCLS) for hazardous constituents in groundwater in the uppermost aquifer (Cliff House/Menefee aquifer) at the point of compliance (POC) at the Uranium Mill Tailings Remedial Action (UMTRA) Project disposal site in Bodo Canyon near Durango, Colorado (DOE, 1989). Details of hydrologic site characterization at the disposal site are provided in Attachment 3, Groundwater Hydrology Report. The principal features of the water resources protectionmore » strategy for the Bodo Canyon disposal site are presented in this document.« less

  9. Monticello Mill Tailings Site, Operable Unit lll, Annual Groundwater Report, May 2015 Through April 2016

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Nguyen, Jason; Smith, Fred

    This report provides the annual analysis of water quality restoration progress, cumulative through April 2016, for Operable Unit (OU) III, surface water and groundwater, of the U.S. Department of Energy (DOE) Office of Legacy Management (LM) Monticello Mill Tailings Site (MMTS). The MMTS is a Comprehensive Environmental Response, Compensation, and Liability Act National Priorities List site located in and near the city of Monticello, San Juan County, Utah. MMTS comprises the 110-acre site of a former uranium- and vanadium-ore-processing mill (mill site) and 1700 acres of surrounding private and municipal property. Milling operations generated 2.5 million cubic yards of wastemore » (tailings) from 1942 to 1960. The tailings were impounded at four locations on the mill site. Inorganic constituents in the tailings drained from the impoundments to contaminate local surface water (Montezuma Creek) and groundwater in the underlying alluvial aquifer. Mill tailings dispersed by wind and water also contaminated properties surrounding and downstream of the mill site. Remedial actions to remove and isolate radiologically contaminated soil, sediment, and debris from the former mill site, Operable Unit I (OU I), and surrounding properties (OU II) were completed in 1999 with the encapsulation of the wastes in an engineered repository located on DOE property 1 mile south of the former mill site. This effectively removed the primary source of groundwater contamination; however, contamination of groundwater and surface water remains within OU III at levels that exceed water quality protection standards. Uranium is the primary contaminant of concern (COC). LM implemented monitored natural attenuation with institutional controls as the OU III remedy in 2004. Because groundwater restoration proceeded more slowly than expected and did not meet performance criteria established in the OU III Record of Decision (June 2004), LM implemented a contingency action in 2009 by an Explanation of Significant Difference to include a pump-and­ treat system using a single extraction well and treatment by zero-valent iron (ex situ treatment system). The contingency action was optimized in 2015 with the installation of8 extraction wells and 16 monitoring wells in a focused area of the aquifer, the area of attainment (AOA). Contaminated water is treated by solar evaporation at an existing facility at the LM repository.« less

  10. Release behavior of uranium in uranium mill tailings under environmental conditions.

    PubMed

    Liu, Bo; Peng, Tongjiang; Sun, Hongjuan; Yue, Huanjuan

    2017-05-01

    Uranium contamination is observed in sedimentary geochemical environments, but the geochemical and mineralogical processes that control uranium release from sediment are not fully appreciated. Identification of how sediments and water influence the release and migration of uranium is critical to improve the prevention of uranium contamination in soil and groundwater. To understand the process of uranium release and migration from uranium mill tailings under water chemistry conditions, uranium mill tailing samples from northwest China were investigated with batch leaching experiments. Results showed that water played an important role in uranium release from the tailing minerals. The uranium release was clearly influenced by contact time, liquid-solid ratio, particle size, and pH under water chemistry conditions. Longer contact time, higher liquid content, and extreme pH were all not conducive to the stabilization of uranium and accelerated the uranium release from the tailing mineral to the solution. The values of pH were found to significantly influence the extent and mechanisms of uranium release from minerals to water. Uranium release was monitored by a number of interactive processes, including dissolution of uranium-bearing minerals, uranium desorption from mineral surfaces, and formation of aqueous uranium complexes. Considering the impact of contact time, liquid-solid ratio, particle size, and pH on uranium release from uranium mill tailings, reducing the water content, decreasing the porosity of tailing dumps and controlling the pH of tailings were the key factors for prevention and management of environmental pollution in areas near uranium mines. Copyright © 2017 Elsevier Ltd. All rights reserved.

  11. 76 FR 72920 - Notification of a Public Teleconference of the Chartered Science Advisory Board

    Federal Register 2010, 2011, 2012, 2013, 2014

    2011-11-28

    ... Document ``Considerations Related to Post-Closure Monitoring of Uranium In-Situ ISL/ISR Sites.'' DATES: The... Monitoring of Uranium In-Situ ISL/ISR Sites.'' The SAB will comply with the provisions of FACA and all... Environmental Protection Standards for Uranium and Thorium Mill Tailings in regard to underground In-Situ Leach...

  12. Remedial Action Plan and site design for stabilization of the inactive uranium mill tailings site at Durango, Colorado: Attachment 4, Water resources protection strategy. Revised final report

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1991-12-01

    To achieve compliance with the proposed US Environmental Protection Agency (EPA) groundwater protection standards (Subpart A of 40 CFR 192), the US Department of Energy (DOE) proposes to meet background concentrations or the EPA maximum concentration limits (MCLS) for hazardous constituents in groundwater in the uppermost aquifer (Cliff House/Menefee aquifer) at the point of compliance (POC) at the Uranium Mill Tailings Remedial Action (UMTRA) Project disposal site in Bodo Canyon near Durango, Colorado (DOE, 1989). Details of hydrologic site characterization at the disposal site are provided in Attachment 3, Groundwater Hydrology Report. The principal features of the water resources protectionmore » strategy for the Bodo Canyon disposal site are presented in this document.« less

  13. An aerial radiological survey of the Durango, Colorado uranium mill tailings site and surrounding area

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Hilton, L.K.

    1981-06-01

    An aerial radiological survey of Durango, Colorado, including the inactive uranium mill tailings piles located southwest of the town, was conducted during August 25--29, 1980, for the Department of Energy's Environmental and Safety Engineering Division. Areas of radiation exposure rates higher than the local background, which was about 15 microrentgens per hour ({mu}R/h), were observed directly over and to the south of the mill tailings piles, over a cemetery, and at two spots near the fairgrounds. The rapidly changing radiation exposure rates at the boundaries of the piles preclude accurate extrapolation of aerial radiological data to ground level exposure ratesmore » in their immediate vicinity. Estimated radiation exposure rates close to the piles, however, approached 30 times background, or about 450 {mu}R/h. Radiation exposure rates in a long area extending south from the tailings piles were about 25 {mu}R/h.« less

  14. 2013 Annual Site Inspection and Monitoring Report for Uranium Mill Tailings Radiation Control Act Title II Disposal Sites

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    None

    This report, in fulfillment of a license requirement, presents the results of long-term surveillance and maintenance activities conducted by the U.S. Department of Energy (DOE) Office of Legacy Management in 2013 at six uranium mill tailings disposal sites reclaimed under Title II of the Uranium Mill Tailings Radiation Control Act (UMTRCA) of 1978. These activities verified that the UMTRCA Title II disposal sites remain in compliance with license requirements. DOE manages six UMTRCA Title II disposal sites under a general license granted by the U.S. Nuclear Regulatory Commission (NRC) established at Title 10 Code of Federal Regulations Part 40.28. Reclamationmore » and site transition activities continue at other sites, and DOE ultimately expects to manage approximately 27 Title II disposal sites. Long-term surveillance and maintenance activities and services for these disposal sites include inspecting and maintaining the sites; monitoring environmental media and institutional controls; conducting any necessary corrective action; and performing administrative, records, stakeholder services, and other regulatory functions. Annual site inspections and monitoring are conducted in accordance with site-specific long-term surveillance plans (LTSPs) and procedures established by DOE to comply with license requirements. Each site inspection is performed to verify the integrity of visible features at the site; to identify changes or new conditions that may affect the long-term performance of the site; and to determine the need, if any, for maintenance, follow-up inspections, or corrective action. LTSPs and site compliance reports are available online at http://www.lm.doe.gov« less

  15. Nuclear facility decommissioning and site remedial actions. Volume 6. A selected bibliography

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Owen, P.T.; Michelson, D.C.; Knox, N.P.

    1985-09-01

    This bibliography of 683 references with abstracts on the subject of nuclear facility decommissioning, uranium mill tailings management, and site remedial actions is the sixth in a series of annual reports prepared for the US Department of Energy's Remedial Action Programs. Foreign as well as domestic literature of all types - technical reports, progress reports, journal articles, conference papers, symposium proceedings, theses, books, patents, legislation, and research project descriptions - has been included. The bibliography contains scientific (basic research as well as applied technology), economic, regulatory, and legal literature pertinent to the US Department of Energy's remedial action program. Majormore » chapters are: (1) Surplus Facilities Management Program; (2) Nuclear Facilities Decommissioning; (3) Formerly Utilized Sites Remedial Action Program; (4) Facilities Contaminated with Natural Radioactivity; (5) Uranium Mill Tailings Remedial Action Program; (6) Grand Junction Remedial Action Program; (7) Uranium Mill Tailings Management; (8) Technical Measurements Center; and (9) General Remedial Action Program Studies. Chapter sections for chapters 1, 2, 5, and 7 include Design, Planning, and Regulations; Environmental Studies and Site Surveys; Health, Safety, and Biomedical Studies; Decontamination Studies; Dismantlement and Demolition; Site Stabilization and Reclamation; Waste Disposal; Remedial Action Experience; and General Studies. The references within each chapter or section are arranged alphabetically by leading author. References having no individual author are arranged by corporate affiliation or by publication description.« less

  16. Radiologic characterization of the Mexican Hat, Utah, uranium mill tailings remedial action site: Appendix D, Addenda D1--D7

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Ludlam, J.R.

    1985-01-01

    This radiologic characterization of the inactive uranium millsite at Mexican Hat, Utah, was conducted by Bendix Field Engineering Corporation foe the US Department of Energy (DOE), Grand Junction Project Office, in response to and in accord with a Statement of Work prepared by the DOE Uranium Mill tailings Remedial Action Project (UMTRAP) Technical Assistance Contractor, Jacobs Engineering Group, Inc. the objective of this project was to determine the horizontal and vertical extent of contamination that exceeds the US Environmental Protection Agency (EPA) standards at the Mexican Hat site. The data presented in this report are required for characterization of themore » areas adjacent to the Mexican Hat tailings piles and for the subsequent design of cleanup activities. Some on-pile sampling was required to determine the depth of the 15-pCi/g Ra-226 interface in an area where wind and water erosion has taken place.« less

  17. Nuclear facility decommissioning and site remedial actions

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Knox, N.P.; Webb, J.R.; Ferguson, S.D.

    1990-09-01

    The 394 abstracted references on environmental restoration, nuclear facility decommissioning, uranium mill tailings management, and site remedial actions constitute the eleventh in a series of reports prepared annually for the US Department of Energy's Remedial Action Programs. Citations to foreign and domestic literature of all types -- technical reports, progress reports, journal articles, symposia proceedings, theses, books, patents, legislation, and research project descriptions -- have been included. The bibliography contains scientific, technical, economic, regulatory, and legal information pertinent to the US Department of Energy's Remedial Action Programs. Major sections are (1) Surplus Facilities Management Program, (2) Nuclear Facilities Decommissioning, (3)more » Formerly Utilized Sites Remedial Action Programs, (4) Facilities Contaminated with Naturally Occurring Radionuclides, (5) Uranium Mill Tailings Remedial Action Program, (6) Grand Junction Remedial Action Program, (7) Uranium Mill Tailings Management, (8) Technical Measurements Center, (9) Remedial Action Program, and (10) Environmental Restoration Program. Within these categories, references are arranged alphabetically by first author. Those references having no individual author are listed by corporate affiliation or by publication title. Indexes are provided for author, corporate affiliation, title word, publication description, geographic location, subject category, and keywords. This report is a product of the Remedial Action Program Information Center (RAPIC), which selects and analyzes information on remedial actions and relevant radioactive waste management technologies.« less

  18. Geochemical investigation of UMTRAP designated site at Durango, Colorado

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Markos, G.; Bush, K.J.

    1983-09-01

    This report is the result of a geochemical investigation of the former uranium mill and tailings site at Durango, Colorado. This is one in a series of site specific geochemical investigations performed on the inactive uranium mill tailings included in the UMTRA Project. The objectives of the investigation are to characterize the geochemistry, to determine the contaminant distribution resulting from the former milling activities and tailings, and to infer chemical pathways and transport mechanisms from the contaminant distribution. The results will be used to model contaminant migration and to develop criteria for long-term containment media such as a cover systemmore » which is impermeable to contaminant migration. This report assumes a familiarity with the hydrologic conditions of the site and the geochemical concepts underlying the investigation. The results reported are based on a one-time sampling of waters and solid material from the background, the area adjacent to the site, and the site. The solid samples are water extracted remove easily soluble salts and acids extracted to remove cabonates and hydroxides. The water extracts and solid samples were analyzed for the major and trace elements. A limited number of samples were analyzed for radiological components. The report includes the methods of sampling, sample processing, analysis, and data interpretation. Three major conclusions are: (1) carbonate salts and low TDS characterize the tailings; (2) the adjacent area and raffinate ponds contain contaminants deposited by a single event of fluid permeation of the soils; and (3) the Animas River adjacent to the site has elevated gross alpha activity attributed to /sup 226/Ra in the sediments derived from the tailings or milling activities.« less

  19. Field testing of fugitive dust control techniques at a uranium mill tailings pile - 1982 Field Test, Gas Hills, Wyoming.

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Elmore, M.R.; Hartley, J.N.

    A field test was conducted on a uranium tailings pile to evaluate the effectiveness of 15 chemical stabilizers for control of fugitive dust from uranium mill tailings. A tailings pile at the Federal American Partners (FAP) Uranium Mill, Gas Hills, Wyoming, was used for the field test. Preliminary laboratory tests using a wing tunnel were conducted to select the more promising stabilizers for field testing. Fourteen of the chemical stabilizers were applied with a field spray system pulled behind a tractor; one--Hydro Mulch--was applied with a hydroseeder. A portable weather station and data logger were installed to record the weathermore » conditions at the test site. After 1 year of monitoring (including three site visits), all of the stabilizers have degraded to some degree; but those applied at the manufacturers' recommended rate are still somewhat effective in reducing fugitive emissions. The following synthetic polymer emulsions appear to be the more effective stabilizers: Wallpol 40-133 from Reichold Chemicals, SP-400 from Johnson and March Corporation, and CPB-12 from Wen Don Corporation. Installed costs for the test plots ranged from $8400 to $11,300/ha; this range results from differences in stabilizer costs. Large-scale stabilization costs of the test materials are expected to range from $680 to $3600/ha based on FAP experience. Evaluation of the chemical stabilizers will continue for approximately 1 year. 2 references, 33 figures, 22 tables.« less

  20. Ecological aspects of microorganisms inhabiting uranium mill tailings

    USGS Publications Warehouse

    Miller, C.L.; Landa, E.R.; Updegraff, D.M.

    1987-01-01

    Numbers and types of microorganisms in uranium mill tailings were determined using culturing techniques. Arthrobacter were found to be the predominant microorganism inhabiting the sandy tailings, whereas Bacillus and fungi predominated in the slime tailings. Sulfate-reducing bacteria, capable of leaching radium, were isolated in low numbers from tailings samples but were isolated in significantly high numbers from topsoil in contact with the tailings. The results are placed in the context of the magnitude of uranium mill tailings in the United States, the hazards posed by the tailings, and how such hazards could be enhanced or diminished by microbial activities. Patterns in the composition of the microbial population are evaluated with respect to the ecological variables that influence microbial growth. ?? 1987 Springer-Verlag New York Inc.

  1. Assessment of a Hydroxyapatite Permeable Reactive Barrier to Remediate Uranium at the Old Rifle Site Colorado.

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Moore, Robert C.; Szecsody, James; Rigali, Mark J.

    We have performed an initial evaluation and testing program to assess the effectiveness of a hydroxyapatite (Ca10(PO4)6(OH)2) permeable reactive barrier and source area treatment to decrease uranium mobility at the Department of Energy (DOE) former Old Rifle uranium mill processing site in Rifle, western Colorado. Uranium ore was processed at the site from the 1940s to the 1970s. The mill facilities at the site as well as the uranium mill tailings previously stored there have all been removed. Groundwater in the alluvial aquifer beneath the site still contains elevated concentrations of uranium, and is currently used for field tests tomore » study uranium behavior in groundwater and investigate potential uranium remediation technologies. The technology investigated in this work is based on in situ formation of apatite in sediment to create a subsurface apatite PRB and also for source area treatment. The process is based on injecting a solution containing calcium citrate and sodium into the subsurface for constructing the PRB within the uranium plume. As the indigenous sediment micro-organisms biodegrade the injected citrate, the calcium is released and reacts with the phosphate to form hydroxyapatite (precipitate). This paper reports on proof-of-principle column tests with Old Rifle sediment and synthetic groundwater.« less

  2. Final programmatic environmental impact statement for the uranium mill tailings remedial action ground water project. Volume I

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    None

    1996-10-01

    This programmatic environmental impact statement (PElS) was prepared for the Uranium Mill Tailings Remedial Action (UMTRA) Ground Water Project to comply with the National Environmental Policy Act (NEPA). This PElS provides an analysis of the potential impacts of the alternatives and ground water compliance strategies as well as potential cumulative impacts. On November 8, 1978, Congress enacted the Uranium Mill Tailings Radiation Control Act (UMTRCA) of 1978, Public Law, codified at 42 USC §7901 et seq. Congress found that uranium mill tailings " ... may pose a potential and significant radiation health hazard to the public, and that every reasonablemore » effort should be made to provide for stabilization, disposal, and control in a safe, and environmentally sound manner of such tailings in order to prevent or minimize other environmental hazards from such tailings." Congress authorized the Secretary of Energy to designate inactive uranium processing sites for remedial action by the U.S. Department of Energy (DOE). Congress also directed the U.S. Environmental Protection Agency (EPA) to set the standards to be followed by the DOE for this process of stabilization, disposal, and control. On January 5, 1983, EPA published standards (40 CFR Part 192) for the disposal and cleanup of residual radioactive materials. On September 3, 1985, the U.S. Court of Appeals for the Tenth Circuit set aside and remanded to EPA the ground water provisions of the standards. The EPA proposed new standards to replace remanded sections and changed other sections of 40 CFR Part 192. These proposed standards were published in the Federal Register on September 24, 1987 (52 FR 36000). Section 108 of the UMTRCA requires that DOE comply with EPA's proposed standards in the absence of final standards. The Ground Water Project was planned under the proposed standards. On January 11, 1995, EPA published the final rule, with which the DOE must now comply. The PElS and the Ground Water Project are in accordance with the final standards. The EPA reserves the right to modify the ground water standards, if necessary, based on changes in EPA drinking water standards. Appendix A contains a copy of the 1983 EPA ground water compliance standards, the 1987 proposed changes to the standards, and the 1995 final rule. Under UMTRA, DOE is responsible for bringing the designated processing sites into compliance with the EPA ground water standards and complying with all other applicable standards and requirements. The U.S. Nuclear Regulatory Commission (NRC) must concur with DOE's actions. States are full participants in the process. The DOE also must consult with any affected Indian tribes and the Bureau of Indian Affairs. Uranium processing activities at most of the inactive mill sites resulted in the contamination of ground water beneath and, in some cases, downgradient of the sites. This contaminated ground water often has elevated levels of constituents such as but not limited to uranium and nitrates. The purpose of the UMTRA Ground Water Project is to eliminate or reduce to acceptable levels the potential health and environmental consequences of milling activities by meeting the EPA ground water standards.« less

  3. Nuclear facility decommissioning and site remedial actions: a selected bibliography. Volume 5

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Owen, P.T.; Knox, N.P.; Chilton, B.D.

    1984-09-01

    This bibliography of 756 references with abstracts on the subject of nuclear facility decommissioning, uranium mill tailings management, and site remedial actions is the fifth in a series of annual reports prepared for the US Department of Energy, Division of Remedial Action Projects. Foreign as well as domestic literature of all types - technical reports, progress reports, journal articles, conference papers, symposium proceedings, theses, books, patents, legislation, and research project descriptions - has been included in this publication. The bibliography contains scientific (basic research as well as applied technology), economic, regulatory, and legal literature pertinent to the US Department ofmore » Energy's Remedial Action Program. Major chapters are: (1) Surplus Facilities Management Program; (2) Nuclear Facilities Decommissioning; (3) Formerly Utilized Sites Remedial Action Program; (4) Uranium Mill Tailings Remedial Action Program; (5) Grand Junction Remedial Action Program; (6) Uranium Mill Tailings Management; and (7) Technical Measurements Center. Chapter sections for chapters 1, 2, 4, and 6 include Design, Planning, and Regulations; Environmental Studies and Site Surveys; Decontamination Studies; Dismantlement and Demolition; Site Stabilization and Reclamation; Waste Disposal; Remedial Action Experience; and General Studies. The references within each chapter or section are arranged alphabetically by leading author. References having no individual author are arranged by corporate author or by title. Indexes are provided for the categories of author, corporate affiliation, title, publication description, geographic location, and keywords. The Appendix contains a list of frequently used acronyms.« less

  4. TRANSPORT AND FATE OF AMMONIUM AND ITS IMPACT ON URANIUM AND OTHER TRACE ELEMENTS AT A FORMER URANIUM MILL TAILING SITE

    PubMed Central

    Miao, Ziheng; Nihat, Hakan; McMillan, Andrew Lee; Brusseau, Mark L.

    2013-01-01

    The remediation of ammonium-containing groundwater discharged from uranium mill tailing sites is a difficult problem facing the mining industry. The Monument Valley site is a former uranium mining site in the southwest US with both ammonium and nitrate contamination of groundwater. In this study, samples collected from 14 selected wells were analyzed for major cations and anions, trace elements, and isotopic composition of ammonium and nitrate. In addition, geochemical data from the U.S. Department of Energy (DOE) database were analyzed. Results showing oxic redox conditions and correspondence of isotopic compositions of ammonium and nitrate confirmed the natural attenuation of ammonium via nitrification. Moreover, it was observed that ammonium concentration within the plume area is closely related to concentrations of uranium and a series of other trace elements including chromium, selenium, vanadium, iron, and manganese. It is hypothesized that ammonium-nitrate transformation processes influence the disposition of the trace elements through mediation of redox potential, pH, and possibly aqueous complexation and solid-phase sorption. Despite the generally relatively low concentrations of trace elements present in groundwater, their transport and fate may be influenced by remediation of ammonium or nitrate at the site. PMID:24357895

  5. An aerial radiological survey of the Durango, Colorado uranium mill tailings site and surrounding area. Date of survey: August 1980

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Hilton, L.K.

    1981-06-01

    An aerial radiological survey of Durango, Colorado, including the inactive uranium mill tailings piles located southwest of the town, was conducted during August 25--29, 1980, for the Department of Energy`s Environmental and Safety Engineering Division. Areas of radiation exposure rates higher than the local background, which was about 15 microrentgens per hour ({mu}R/h), were observed directly over and to the south of the mill tailings piles, over a cemetery, and at two spots near the fairgrounds. The rapidly changing radiation exposure rates at the boundaries of the piles preclude accurate extrapolation of aerial radiological data to ground level exposure ratesmore » in their immediate vicinity. Estimated radiation exposure rates close to the piles, however, approached 30 times background, or about 450 {mu}R/h. Radiation exposure rates in a long area extending south from the tailings piles were about 25 {mu}R/h.« less

  6. 2015 Uranium Mill Tailings Radiation Control Act (UMTRCA) Title ll Annual Report, L-Bar, New Mexico Disposal Site

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Frazier, William; Johnson, Dick

    The L-Bar, New Mexico, Uranium Mill Tailings Radiation Control Act (UMTRCA) Title II Disposal Site was inspected on August 18, 2015. The tailings impoundment was in excellent condition. Erosion and vegetation measurements to monitor the condition of the impoundment cover indicated that no erosion is occurring, and perennial vegetation foliar cover at the measurement plots increased substantially compared to previous years due to above-average precipitation for the year. A short segment of the perimeter fence near the site entrance was realigned in spring 2015 because a gully was undermining the fence corner. Loose fence strands at another location were repairedmore » during the inspection, and a section of fence needs to be realigned to avoid areas affected by deep gullies and sediment deposition. Inspectors identified no other maintenance needs or cause for a follow-up inspection. Groundwater monitoring is required every 3 years. The next monitoring event will be in 2016.« less

  7. DOE Office of Scientific and Technical Information (OSTI.GOV)

    Owen, P. T.; Webb, J. R.; Knox, N. P.

    The 664 abstracted references on environmental restoration, nuclear facility decommissioning, uranium mill tailings management, and site remedial actions constitute the twelfth in a series of reports prepared annually for the US Department of Energy Remedial Action Programs. Citations to foreign and domestic literature of all types -- technical reports, progress reports, journal articles, symposia proceedings, theses, books, patents, legislation, and research project descriptions -- have been included. The bibliography contains scientific, technical, economic, regulatory, and legal information pertinent to the US Department of Energy Remedial Action Programs. Major sections are (1) Decontamination and Decommissioning Program, (2) Nuclear Facilities Decommissioning, (3)more » Formerly Utilized Sites Remedial Action Program, (4) Facilities Contaminated with Naturally Occurring Radionuclides, (5) Uranium Mill Tailings Remedial Action Program, (6) Uranium Mill Tailings Management, (7) Technical Measurements Center, and (8) Environmental Restoration Program. Within these categories, references are arranged alphabetically by first author. Those references having no individual author are listed by corporate affiliation or by publication title. Indexes are provided for author, corporate affiliation, title word, publication description, geographic location, subject category, and key word. This report is a product of the Remedial Action Program Information Center (RAPIC), which selects, analyzes, and disseminates information on environmental restoration and remedial actions. RAPIC staff and resources are available to meet a variety of information needs. Contact the center at FTS 624-7764 or (615) 574-7764.« less

  8. Nuclear facility decommissioning and site remedial actions: A selected bibliography, Vol. 18. Part 2. Indexes

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    NONE

    1997-09-01

    This bibliography contains 3638 citations with abstracts of documents relevant to environmental restoration, nuclear facility decontamination and decommissioning (D&D), uranium mill tailings management, and site remedial actions. This report is the eighteenth in a series of bibliographies prepared annually for the U.S. Department of Energy (DOE) Office of Environmental Restoration. Citations to foreign and domestic literature of all types - technical reports, progress reports, journal articles, symposia proceedings, theses, books, patents, legislation, and research project descriptions - have been included in Part 1 of the report. The bibliography contains scientific, technical, financial, and regulatory information that pertains to DOE environmentalmore » restoration programs. The citations are separated by topic into 16 sections, including (1) DOE Environmental Restoration Program; (2) DOE D&D Program; (3) Nuclear Facilities Decommissioning; (4) DOE Formerly Utilized Sites Remedial Action Programs; (5) NORM-Contaminated Site Restoration; (6) DOE Uranium Mill Tailings Remedial Action Project; (7) Uranium Mill Tailings Management; (8) DOE Site-Wide Remedial Actions; (9) DOE Onsite Remedial Action Projects; (10) Contaminated Site Remedial Actions; (11) DOE Underground Storage Tank Remediation; (12) DOE Technology Development, Demonstration, and Evaluations; (13) Soil Remediation; (14) Groundwater Remediation; (15) Environmental Measurements, Analysis, and Decision-Making; and (16) Environmental Management Issues. Within the 16 sections, the citations are sorted by geographic location. If a geographic location is not specified, the citations are sorted according to the document title. In Part 2 of the report, indexes are provided for author, author affiliation, selected title phrase, selected title word, publication description, geographic location, and keyword.« less

  9. Format and style for environmental documents prepared as part of the Uranium Mill Tailings Remedial Action Program. [Uranium Mill Tailings Remedial Action (UMTRA) Project

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1980-06-01

    The Uranium Mill Tailings Remedial Action Program will require the preparation of several environmental impact statements and several environmental assessments. This guide begins with a section describing in general terms the efforts required to make these documents readable. The sections describe the formats to be used for the pages, headings, front matter, footnotes, lists, figures, tables, references, glossaries, indexes, and appendixes in these documents. A final section presents some rules of style to be followed in writing the texts.

  10. 40 CFR 61.190 - Designation of facilities.

    Code of Federal Regulations, 2010 CFR

    2010-07-01

    ..., Lewiston, New York; the Weldon Spring Site, Weldon Spring, Missouri; the Middlesex Sampling Plant, Middlesex, New Jersey; the Monticello Uranium Mill Tailings Pile, Monticello, Utah. This subpart does not...

  11. Intense alpha-particle emitting crystallites in uranium mill wastes

    USGS Publications Warehouse

    Landa, E.R.; Stieff, L.R.; Germani, M.S.; Tanner, A.B.; Evans, J.R.

    1994-01-01

    Nuclear emulsion microscopy has demonstrated the presence of small, intense ??-particle emitting crystallites in laboratory-produced tailings derived from the sulfuric acid milling of uranium ores. The ??-particle activity is associated with the isotope pair 210Pb 210Po, and the host mineral appears to be PbSO4 occurring as inclusions in gypsum laths. These particles represent potential inhalation hazards at uranium mill tailings disposal areas. ?? 1994.

  12. Mobilization of radionuclides from uranium mill tailings and related waste materials in anaerobic environments

    USGS Publications Warehouse

    Landa, E.R.

    2003-01-01

    Specific extraction studies in our laboratory have shown that iron and manganese oxide- and alkaline earth sulfate minerals are important hosts of radium in uranium mill tailings. Iron- and sulfate-reducing bacteria may enhance the release of radium (and its analog barium) from uranium mill tailings, oil field pipe scale [a major technologically enhanced naturally occurring radioactive material (TENORM) waste], and jarosite (a common mineral in sulfuric acid processed-tailings). These research findings are reviewed and discussed in the context of nuclear waste forms (such as barium sulfate matrices), radioactive waste management practices, and geochemical environments in the Earth's surficial and shallow subsurface regions.

  13. Nuclear facility decommissioning and site remedial actions: a selected bibliography

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Owen, P.T.; Knox, N.P.; Fielden, J.M.

    This bibliography contains 693 references with abstracts on the subject of nuclear facility decommissioning, uranium mill tailings management, and site remedial actions. Foreign, as well as domestic, literature of all types - technical reports, progress reports, journal articles, conference papers, symposium proceedings, theses, books, patents, legislation, and research project descriptions - has been included in this publication. The bibliography contains scientific (basic research as well as applied technology), economic, regulatory, and legal literature pertinent to the US Department of Energy's Remedial Action Program. Major chapters are Surplus Facilities Management Program, Nuclear Facilities Decommissioning, Formerly Utilized Sites Remedial Action Program, Uraniummore » Mill Tailings Remedial Action Program, Grand Junction Remedial Action Program, and Uranium Mill Tailings Management. Chapter sections for chapters 1 and 2 include: Design, Planning, and Regulations; Site Surveys; Decontamination Studies; Dismantlement and Demolition; Land Decontamination and Reclamation; Waste Disposal; and General Studies. The references within each chapter are arranged alphabetically by leading author. References having no individual author are arranged by corporate author or by title. Indexes are provided for (1) author; (2) corporate affiliation; (3) title; (4) publication description; (5) geographic location; and (6) keywords. An appendix of 202 bibliographic references without abstracts or indexes has been included in this bibliography. This appendix represents literature identified but not abstracted due to time constraints.« less

  14. 40 CFR 61.222 - Standard.

    Code of Federal Regulations, 2010 CFR

    2010-07-01

    ... uranium mill tailings pile that are no longer operational shall not exceed 20 pCi/(m2-sec) (1.9 pCi/(ft2-sec)) of radon-222. (b) Once a uranium mill tailings pile or impoundment ceases to be operational it...

  15. Nuclear facility decommissioning and site remedial actions: A selected bibliography, volume 9

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Owen, P.T.; Knox, N.P.; Michelson, D.C.

    1988-09-01

    The 604 abstracted references on nuclear facility decommissioning, uranium mill tailings management, and site remedial actions constitute the ninth in a series of reports prepared annually for the US Department of Energy's Remedial Action Programs. Foreign and domestic literature of all types--technical reports, progress reports, journal articles, symposia proceedings, theses, books, patents, legislation, and research project descriptions--has been included. The bibliography contains scientific, technical, economic, regulatory, and legal information pertinent to the US Department of Energy's remedial action programs. Major sections are (1) Surplus Facilities Management Program, (2) Nuclear Facilities Decommissioning, (3) Formerly Utilized Sites Remedial Action Program, (4) Facilitiesmore » Contaminated with Naturally Occurring Radionuclides, (5) Uranium Mill Tailings Remedial Action Program, (6) Uranium Mill Tailings Management, (7) Technical Measurements Center, and (8) General Remedial Action Program Studies. Subsections for sections 1, 2, 5, and 6 include: Design, Planning, and Regulations; Environmental Studies and Site Surveys; Health, Safety, and Biomedical Studies; Decontamination Studies; Dismantlement and Demolition; Site Stabilization and Reclamation; Waste Disposal; Remedial Action Experience; and General Studies. Within these categories, references are arranged alphabetically by first author. Those references having no individual author are listed by corporate affiliation or by publication description. Indexes are provided for author, corporate affiliation, title word, publication description, geographic location, and keywords. This report is a product of the Remedial Action Program Information Center (RAPIC), which selects and analyzes information on remedial actions and relevant radioactive waste management technologies. RAPIC staff and resources are available to meet a variety of information needs. Contact the center at (615) 576-0568 or FTS 626-0568.« less

  16. Uptake of trace elements and radionuclides from uranium mill tailings by four-wing saltbush (Atriplex canescens) and alkali sacaton (Sporobolus airoides). [Radium 226; Uranium; Molybdenum; Selenium; Vanadium; Astatine

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Dreesen, D.R.; Marple, M.L.

    1979-01-01

    A greenhouse experiment was performed to determine the uptake of trace elements and radionuclides from uranium mill tailings by native plant species. Four-wing saltbush and alkali sacaton were grown in alkaline tailings covered with soil and in soil alone as controls. The tailings material was highly enriched in Ra-226, Mo, U, Se, V, and As compared with three local soils. The shrub grown in tailings had elevated concentrations of Mo, Se, Ra-226, U, As, and Na compared with the controls. Alkali sacaton contained high concentrations of Mo, Se, Ra-226, and Ni when grown on tailings. Molybdenum and selenium concentrations inmore » plants grown in tailings are above levels reported to be toxic to grazing animals. These results indicate that the bioavailability of Mo and Se in alkaline environments makes these elements among the most hazardous contaminants present in uranium mill wastes.« less

  17. Radiological survey of the inactive uranium-mill tailings at Durango, Colorado

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Haywood, F.F.; Perdue, P.T.; Shinpaugh, W.H.

    1980-03-01

    Results of a radiological survey of the inactive uranium-mill site at Durango, Colorado, conducted in April 1976, in cooperation with a team from Ford, Bacon and Davis Utah Inc., are presented together with descriptions of the instruments and techniques used to obtain the data. Direct above-ground gamma measurements and analysis of surface soil and sediment samples indicate movement of tailings from the piles toward Lightner Creek on the north and the Animas River on the east side of the piles. The concentration of /sup 226/Ra in the former raffinate pond area is only slightly above the background level. Two structuresmore » in Durango were found to contain high concentrations of airborne radon daughters, where tailings are known to have been utilized in construction. Near-background concentrations of radon daughters were found in a well-ventilated building close to the tailings.« less

  18. DOE Office of Scientific and Technical Information (OSTI.GOV)

    Dam, William; Gil, Dr. April; Johnson, Raymond H.

    The US Department of Energy Office of Legacy Management (LM) is responsible for maintaining protective public health and environmental conditions at former uranium mill tailings sites nationwide via long-term stewardship. One of these sites, a former uranium mill near Riverton, Wyoming, is within the boundary of the Wind River Indian Reservation and operated from 1958 to 1963. Tailings and contaminated material associated with mill operations were removed and transported to an offsite disposal cell in 1989. The remedial action was completed under Title I of the Uranium Mill Tailings Radiation Control Act of 1978. Milling operations, which included an unlinedmore » tailings impoundment and an unlined evaporation pond, contaminated the shallow groundwater, resulting in a downgradient groundwater plume that discharges to the Little Wind River. A natural flushing compliance strategy was implemented in 1998. This strategy allows contaminants of concern to naturally flush from the groundwater, provided that contaminants flush below US Environmental Protection Agency maximum concentration limits within 100 years. As part of the compliance strategy, LM has implemented a groundwater monitoring program along with institutional controls that include the installation of an alternate water supply, continued sampling of private wells, and restrictions on well drilling and gravel pit construction. LM works closely with local stakeholders and community members to ensure that these institutional controls are in place and maintained. The Riverton site provides an interesting case study where contaminant remobilization due to river flooding prompted a reevaluation of the conceptual site model to verify if the current compliance strategy would remain protective of human health and the environment. Concentrations of groundwater contaminants, which include sulfate, molybdenum, and uranium, were transiently elevated following flooding of the Little Wind River in 2010 and 2016. These flood events provided the impetus to investigate other aspects of the hydrologic system, including the unsaturated zone, naturally reduced (sulfidic) zones, and evaporite deposits. New site conceptual models, field and laboratory studies, and numerical models are being developed to explain how biogeochemical sediment–water interactions contribute to plume persistence and flood-related increases in groundwater concentrations. Updated human health and ecological risk assessments are progressing to evaluate the risk to human health and the environment based on current site conditions. Groundwater concentrations may remain above US Environmental Protection Agency maximum concentration limits beyond the 100-year natural flushing regulatory time frame. LM in its capacity as a long-term steward continues to monitor the site to ensure protectiveness is maintained and to determine the feasibility of alternative compliance and remediation strategies.« less

  19. Fractal and Chaos Analysis for Dynamics of Radon Exhalation from Uranium Mill Tailings

    NASA Astrophysics Data System (ADS)

    Li, Yongmei; Tan, Wanyu; Tan, Kaixuan; Liu, Zehua; Xie, Yanshi

    2016-08-01

    Tailings from mining and milling of uranium ores potentially are large volumes of low-level radioactive materials. A typical environmental problem associated with uranium tailings is radon exhalation, which can significantly pose risks to environment and human health. In order to reduce these risks, it is essential to study the dynamical nature and underlying mechanism of radon exhalation from uranium mill tailings. This motivates the conduction of this study, which is based on the fractal and chaotic methods (e.g. calculating the Hurst exponent, Lyapunov exponent and correlation dimension) and laboratory experiments of the radon exhalation rates. The experimental results show that the radon exhalation rate from uranium mill tailings is highly oscillated. In addition, the nonlinear analyses of the time series of radon exhalation rate demonstrate the following points: (1) the value of Hurst exponent much larger than 0.5 indicates non-random behavior of the radon time series; (2) the positive Lyapunov exponent and non-integer correlation dimension of the time series imply that the radon exhalation from uranium tailings is a chaotic dynamical process; (3) the required minimum number of variables should be five to describe the time evolution of radon exhalation. Therefore, it can be concluded that the internal factors, including heterogeneous distribution of radium, and randomness of radium decay, as well as the fractal characteristics of the tailings, can result in the chaotic evolution of radon exhalation from the tailings.

  20. Monticello Mill Tailings Site Operable Unit III Annual Groundwater Report May 2014 Through April 2015, October 2015

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Nguyen, Jason; Smith, Fred

    This report provides the annual analysis of water quality restoration progress, cumulative through April 2015, for Operable Unit (OU) III, surface water and groundwater, of the U.S. Department of Energy (DOE) Office of Legacy Management Monticello Mill Tailings Site (MMTS). The MMTS is a Comprehensive Environmental Response, Compensation, and Liability Act National Priorities List site located in and near the city of Monticello, San Juan County, Utah. MMTS comprises the 110-acre site of a former uranium- and vanadium-ore-processing mill (mill site) and 1,700 acres of surrounding private and municipal property. Milling operations generated 2.5 million cubic yards of waste (tailings)more » from 1942 to 1960. The tailings were impounded at four locations on the mill site. Inorganic constituents in the tailings drained from the impoundments to contaminate local surface water (Montezuma Creek) and groundwater in the underlying alluvial aquifer. Mill tailings dispersed by wind and water also contaminated properties surrounding and downstream of the mill site. Remedial actions to remove and isolate radiologically contaminated soil, sediment, and debris from the former mill site (OU I) and surrounding properties (OU II) were completed in 1999 with the encapsulation of the wastes in an engineered repository located on DOE property 1 mile south of the former mill site. Contamination of groundwater and surface water remains within OU III at levels that exceed water quality protection standards. Uranium is the primary contaminant of concern. LM implemented monitored natural attenuation with institutional controls as the OU III remedy in 2004. Because groundwater restoration proceeded more slowly than expected and did not meet performance criteria established in the OU III Record of Decision (June 2004), LM implemented a contingency action in 2009 by an Explanation of Significant Difference to include a pump-and-treat system using a single extraction well and treatment by zero-valent iron (ex-situ treatment system). The contingency action was optimized in 2015 with the installation of 8 extraction wells and 16 monitoring wells in a focused area of the aquifer (area of attainment). Contaminated water is treated by solar evaporation at an existing onsite LM facility. Environmental monitoring at OU III consists of twice-yearly (April and October) collection and analysis of hydrologic and water-quality data from an established network of observation wells, seeps, and surface water locations. The scope of monitoring was expanded in 2009 for the ex situ treatment system and in 2015 for the remedy optimization system. Operation and monitoring of the ex situ treatment system was discontinued in 2014 with the start-up of the remedy optimization system. No data anomalies for OU III water quality trending or restoration progress are identified for the May 2014 through April 2015 reporting period. Although some regions of the aquifer demonstrate decreasing concentration trends, such trending is not evident for the bulk of the aquifer and a prolonged restoration period is indicated. The groundwater contingency remedy optimization system captures significant contaminant mass (primarily uranium) from the area of attainment; however, because that system only became operational in 2015, a long-term forecast of restoration progress is premature.« less

  1. Effects of uranium development on erosion and associated sedimentation in southern San Juan Basin, New Mexico

    USGS Publications Warehouse

    Cooley, Maurice E.

    1979-01-01

    A reconnaissance was made of some of the effects of uranium development on erosion and associated sedimentation in the southern San Juan Basin, where uranium development is concentrated. In general, the effects of exploration on erosion are minor, although erosion may be accelerated by the building of access roads, by activities at the drilling sites, and by close concentration of drilling sites. Areas where the greatest effects on erosion and sedimentation from mining and milling operations have occurred are: (1) in the immediate vicinity of mines and mills, (2) near waste piles, and (3) in stream channels where modifications, such as changes in depth have been caused by discharge of excess mine and mill water. Collapse of tailings piles could result in localized but excessive erosion and sedimentation.

  2. Release of 226Ra from uranium mill tailings by microbial Fe(III) reduction

    USGS Publications Warehouse

    Landa, E.R.; Phillips, E.J.P.; Lovley, D.R.

    1991-01-01

    Uranium mill tailings were anaerobically incubated in the presence of H2 with Alteromonas putrefaciens, a bacterium known to couple the oxidation of H2 and organic compounds to the reduction of Fe(III) oxides. There was a direct correlation between the extent of Fe(III) reduction and the accumulation of dissolved 226Ra. In sterile tailings in which Fe(III) was not reduced, there was negligible leaching of 226Ra. The behavior of Ba was similar to that of Ra in inoculated and sterile systems. These results demonstrate that under anaerobic conditions, microbial reduction of Fe(III) may result in the release of dissolved 226Ra from uranium mill tailings. ?? 1991.

  3. Annual monitoring report for the Gunnison, Colorado, wetlands mitigation plan

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    NONE

    1995-10-01

    The US Department of Energy (DOE) administers the Uranium Mill Tailings Remedial Action (UMTRA) Project to clean up uranium mill tailings and other surface contamination at 24 abandoned uranium mill sites in 10 states. One of these abandoned mill sites is near the town of Gunnison, Colorado; surface remediation and the environmental impacts of remedial action are described in the Gunnison environmental assessment (EA) (DOE, 1992). Remedial action resulted in the elimination of 4.3 acres (ac) 1.7 hectares (ha) of wetlands and mitigation of this loss of wetlands is being accomplished through the enhance of 18.4 ac (7.5 ha) ofmore » riparian plant communities in six spring feed areas on Bureau of Land Management (BLM) land. The description of the impacted and mitigation wetlands is provided in the Mitigation and Monitoring Plan for Impacted Wetlands at the Gunnison UMTRA Project Site, Gunnison, Colorado (DOE, 1994), which is attached to the US Army corps of Engineers (USACE) Section 404 Permit. As part of the wetlands mitigation plan, the six mitigation wetlands were fenced in the fall of 1993 to exclude livestock grazing. Baseline of grazed conditions of the wetlands vegetation was determined during the summer of 1993 (DOE, 1994). A 5-year monitoring program of these six sites has been implemented to document the response of vegetation and wildlife to the exclusion of livestock. This annual monitoring report provides the results of the first year of the 5-year monitoring period.« less

  4. Biogeochemical aspects of uranium mineralization, mining, milling, and remediation

    USGS Publications Warehouse

    Campbell, Kate M.; Gallegos, Tanya J.; Landa, Edward R.

    2015-01-01

    Natural uranium (U) occurs as a mixture of three radioactive isotopes: 238U, 235U, and 234U. Only 235U is fissionable and makes up about 0.7% of natural U, while 238U is overwhelmingly the most abundant at greater than 99% of the total mass of U. Prior to the 1940s, U was predominantly used as a coloring agent, and U-bearing ores were mined mainly for their radium (Ra) and/or vanadium (V) content; the bulk of the U was discarded with the tailings (Finch et al., 1972). Once nuclear fission was discovered, the economic importance of U increased greatly. The mining and milling of U-bearing ores is the first step in the nuclear fuel cycle, and the contact of residual waste with natural water is a potential source of contamination of U and associated elements to the environment. Uranium is mined by three basic methods: surface (open pit), underground, and solution mining (in situ leaching or in situ recovery), depending on the deposit grade, size, location, geology and economic considerations (Abdelouas, 2006). Solid wastes at U mill tailings (UMT) sites can include both standard tailings (i.e., leached ore rock residues) and solids generated on site by waste treatment processes. The latter can include sludge or “mud” from neutralization of acidic mine/mill effluents, containing Fe and a range of coprecipitated constituents, or barium sulfate precipitates that selectively remove Ra (e.g., Carvalho et al., 2007). In this chapter, we review the hydrometallurgical processes by which U is extracted from ore, the biogeochemical processes that can affect the fate and transport of U and associated elements in the environment, and possible remediation strategies for site closure and aquifer restoration.This paper represents the fourth in a series of review papers from the U.S. Geological Survey (USGS) on geochemical aspects of UMT management that span more than three decades. The first paper (Landa, 1980) in this series is a primer on the nature of tailings and radionuclide mobilization from them. The second paper (Landa, 1999) includes coverage of research carried out under the U.S. Department of Energy’s Uranium Mill Tailings Remedial Action Program (UMTRA). The third paper (Landa, 2004) reflects the increased focus of researchers on biotic effects in UMT environs. This paper expands the focus to U mining, milling, and remedial actions, and includes extensive coverage of the increasingly important alkaline in situ recovery and groundwater restoration.

  5. In situ remediation of uranium contaminated groundwater

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Dwyer, B.P.; Marozas, D.C.

    1997-02-01

    In an effort to develop cost-efficient techniques for remediating uranium contaminated groundwater at DOE Uranium Mill Tailing Remedial Action (UMTRA) sites nationwide, Sandia National Laboratories (SNL) deployed a pilot scale research project at an UMTRA site in Durango, CO. Implementation included design, construction, and subsequent monitoring of an in situ passive reactive barrier to remove Uranium from the tailings pile effluent. A reactive subsurface barrier is produced by emplacing a reactant material (in this experiment various forms of metallic iron) in the flow path of the contaminated groundwater. Conceptually the iron media reduces and/or adsorbs uranium in situ to acceptablemore » regulatory levels. In addition, other metals such as Se, Mo, and As have been removed by the reductive/adsorptive process. The primary objective of the experiment was to eliminate the need for surface treatment of tailing pile effluent. Experimental design, and laboratory and field results are discussed with regard to other potential contaminated groundwater treatment applications.« less

  6. In situ remediation of uranium contaminated groundwater

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Dwyer, B.P.; Marozas, D.C.

    1997-12-31

    In an effort to develop cost-efficient techniques for remediating uranium contaminated groundwater at DOE Uranium Mill Tailing Remedial Action (UMTRA) sites nationwide, Sandia National Laboratories (SNL) deployed a pilot scale research project at an UMTRA site in Durango, CO. Implementation included design, construction, and subsequent monitoring of an in situ passive reactive barrier to remove Uranium from the tailings pile effluent. A reactive subsurface barrier is produced by emplacing a reactant material (in this experiment - various forms of metallic iron) in the flow path of the contaminated groundwater. Conceptually the iron media reduces and/or adsorbs uranium in situ tomore » acceptable regulatory levels. In addition, other metals such as Se, Mo, and As have been removed by the reductive/adsorptive process. The primary objective of the experiment was to eliminate the need for surface treatment of tailing pile effluent. Experimental design, and laboratory and field preliminary results are discussed with regard to other potential contaminated groundwater treatment applications.« less

  7. Uranium Mines and Mills | RadTown USA | US EPA

    EPA Pesticide Factsheets

    2017-08-07

    Uranium is used as nuclear fuel for electric power generation. U.S. mining industries can obtain uranium in two ways: mining or milling. Mining waste and mill tailings can contaminate water, soil and air if not disposed of properly.

  8. 2013 Annual Site Inspection and Monitoring Report for Uranium Mill Tailings Radiation Control Act Title I Disposal Sites

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    None, None

    This report, in fulfillment of a license requirement, presents the results of long-term surveillance and maintenance activities conducted by the U.S. Department of Energy (DOE) Office of Legacy Management (LM) in 2013 at 19 uranium mill tailings disposal sites established under Title I of the Uranium Mill Tailings Radiation Control Act (UMTRCA) of 1978.1 These activities verified that the UMTRCA Title I disposal sites remain in compliance with license requirements. DOE operates 18 UMTRCA Title I sites under a general license granted by the U.S. Nuclear Regulatory Commission (NRC) in accordance with Title 10 Code of Federal Regulations Part 40.27more » (10 CFR 40.27). As required under the general license, a long-term surveillance plan (LTSP) for each site was prepared by DOE and accepted by NRC. The Grand Junction, Colorado, Disposal Site, one of the 19 Title I sites, will not be included under the general license until the open, operating portion of the cell is closed. The open portion will be closed either when it is filled or in 2023. This site is inspected in accordance with an interim LTSP. Long-term surveillance and maintenance services for these disposal sites include inspecting and maintaining the sites; monitoring environmental media and institutional controls; conducting any necessary corrective actions; and performing administrative, records, stakeholder relations, and other regulatory stewardship functions. Annual site inspections and monitoring are conducted in accordance with site-specific LTSPs and procedures established by DOE to comply with license requirements. Each site inspection is performed to verify the integrity of visible features at the site; to identify changes or new conditions that may affect the long-term performance of the site; and to determine the need, if any, for maintenance, follow-up or contingency inspections, or corrective action in accordance with the LTSP. LTSPs and site compliance reports are available on the Internet at http://www.lm.doe.gov/.« less

  9. Remedial action plan and site design for stabilization of the inactive uranium mill tailings sites at Rifle, Colorado

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1990-02-01

    This volume contains appendices D6 through D8 containing laboratory test data: from MK-F investigation, 1987, Old Rifle and New Rifle sites; on bentonite amended radon barrier material; and from MK-F investigation, 1987, riprap tests.

  10. Leaching behavior of U, Mn, Sr, and Pb from different particle-size fractions of uranium mill tailings.

    PubMed

    Liu, Bo; Peng, Tongjiang; Sun, Hongjuan

    2017-06-01

    Pollution by the release of heavy metals from tailings constitutes a potential threat to the environment. To characterize the processes governing the release of Mn, Sr, Pb, and U from the uranium mill tailings, a dynamic leaching test was applied for different size of uranium mill tailings samples. Inductively coupled plasma atomic emission spectroscopy (ICP-AES) and inductively coupled plasma mass spectrometry (ICP-MS) were performed to determine the content of Mn, Sr, Pb, and U in the leachates. The release of mobile Mn, Sr, Pb, and U fraction was slow, being faster in the initial stage and then attained a near steady-state condition. The experimental results demonstrate that the release of Mn, Sr, Pb, and U from uranium mill tailings with different size fractions is controlled by a variety of mechanisms. Surface wash-off is the release mechanism for Mn. The main release mechanism of Sr and Pb is the dissolution in the initial leaching stage. For U, a mixed process of wash-off and diffusion is the controlling mechanism.

  11. Radiation dosimetry on revegetated uranium mill tailings in western South Dakota

    Treesearch

    Mark A. Rumble

    1986-01-01

    Measurement of gamma radiation using thermoluminescent dosimeters on three uranium mill tailings areas and a control area showed exposure rates below ground depended on the amount and type of soil covering. Covering tailings with 30 cm of shale and 60 cm of topsoil reduced gamma radiation exposure belowground to rates similar to the control area. Soil covering of 30 cm...

  12. 40 CFR 61.222 - Standard.

    Code of Federal Regulations, 2011 CFR

    2011-07-01

    ... EMISSION STANDARDS FOR HAZARDOUS AIR POLLUTANTS National Emission Standards for Radon Emissions From the Disposal of Uranium Mill Tailings § 61.222 Standard. (a) Radon-222 emissions to the ambient air from...-sec)) of radon-222. (b) Once a uranium mill tailings pile or impoundment ceases to be operational it...

  13. Diversity and Characterization of Sulfate-Reducing Bacteria in Groundwater at a Uranium Mill Tailings Site

    PubMed Central

    Chang, Yun-Juan; Peacock, Aaron D.; Long, Philip E.; Stephen, John R.; McKinley, James P.; Macnaughton, Sarah J.; Hussain, A. K. M. Anwar; Saxton, Arnold M.; White, David C.

    2001-01-01

    Microbially mediated reduction and immobilization of U(VI) to U(IV) plays a role in both natural attenuation and accelerated bioremediation of uranium-contaminated sites. To realize bioremediation potential and accurately predict natural attenuation, it is important to first understand the microbial diversity of such sites. In this paper, the distribution of sulfate-reducing bacteria (SRB) in contaminated groundwater associated with a uranium mill tailings disposal site at Shiprock, N.Mex., was investigated. Two culture-independent analyses were employed: sequencing of clone libraries of PCR-amplified dissimilatory sulfite reductase (DSR) gene fragments and phospholipid fatty acid (PLFA) biomarker analysis. A remarkable diversity among the DSR sequences was revealed, including sequences from δ-Proteobacteria, gram-positive organisms, and the Nitrospira division. PLFA analysis detected at least 52 different mid-chain-branched saturate PLFA and included a high proportion of 10me16:0. Desulfotomaculum and Desulfotomaculum-like sequences were the most dominant DSR genes detected. Those belonging to SRB within δ-Proteobacteria were mainly recovered from low-uranium (≤302 ppb) samples. One Desulfotomaculum-like sequence cluster overwhelmingly dominated high-U (>1,500 ppb) sites. Logistic regression showed a significant influence of uranium concentration over the dominance of this cluster of sequences (P = 0.0001). This strong association indicates that Desulfotomaculum has remarkable tolerance and adaptation to high levels of uranium and suggests the organism's possible involvement in natural attenuation of uranium. The in situ activity level of Desulfotomaculum in uranium-contaminated environments and its comparison to the activities of other SRB and other functional groups should be an important area for future research. PMID:11425735

  14. Bridging the gap between tribal risk perceptions and scientific decision-making for uranium legacy sites located in Native American communities

    NASA Astrophysics Data System (ADS)

    Joseph, C.; Waugh, W.; Glenn, E.; Chief, K.

    2017-12-01

    There are approximately 15,000 abandoned uranium mines (AUM) in the western United States, of which 500 AUMs are located in the Colorado Plateau Four-Corners region. Uranium mill tailings, referred to as legacy waste, compromise the largest volume of any category of radioactive waste in the nation. Today, the Department of Energy Legacy Management is responsible for long-term stewardship and maintenance of inactive uranium processing sites that have been remediated to prevent further migration and exposure of tailings to the environment and surrounding communities. In collaboration with the DOE-LM, I am investigating the impact of climate change and community adaptation on the long-term performance of disposal cell covers for uranium mill tailings located in Native American communities, as well as how these communities have adapted to and perceive these areas. I am interested in how abiotic engineered cell covers may be candidate sites for future conversion to vegetated evapotranspirative caps for arid to semi-arid climates. The objectives are to: 1) assess above-ground tissue of plants encroaching engineered cell covers for concentrations of uranium, radium, selenium, molybdenum, thorium, arsenic, lead, and manganese and compare them to control sites; 2) determine if above-cell plant tissue is accumulating to toxic levels that may create an exposure pathway, 3) identify climate scenarios for site locations and determine how short-and long-scale climate projections will influence spatial and temporal plant distribution for specific woody species; and 4) evaluate the risk perceptions of Hopi villages located five miles downstream of one site location. To date, risk perception and stakeholder outreach to the Hopi communities has been absent. This study will help inform how land use, water use, and sustenance practices may contribute to environmental health disparities for one of the few tribes that has maintained physical continuity within their ancestral homeland.

  15. DOE Office of Scientific and Technical Information (OSTI.GOV)

    Owen, P.T.; Knox, N.P.; Fielden, J.M.

    This bibliography of 657 references with abstracts on the subject of nuclear facility decommissioning, uranium mill tailings management, and site remedial actions is the fourth in a series of annual reports prepared for the US Department of Energy, Division of Remedial Action Projects. Foreign as well as domestic documents of all types - technical reports, progress reports, journal articles, conference papers, symposium proceedings, theses, books, patents, legislation, and research project descriptions - have been references in this publication. The bibliography contains scientific (basic research as well as applied technology), economic, regulatory, and legal literature pertinent to the US Department ofmore » Energy's Remedial Action Program. Major chapters are: (1) Surplus Facilities Management Program; (2) Nuclear Facilities Decommissioning; (3) Formerly Utilized Sites Remedial Action Program; (4) Uranium Mill Tailings Remedial Action Program; (5) Grand Junction Remedial Action Program; and (6) Uranium Mill Tailings Management. Chapter sections for chapters 1 and 2 include: Design, Planning, and Regulations; Site Surveys; Decontamination Studies; Dismantlement and Demolition; Land Decontamination and Reclamation; Waste Disposal; and General studies. The references within each chapter or section are arranged alphabetically by leading author. References having no individual author are arranged by corporate author, or by title. Indexes are provided for the categories of author, corporate affiliation, title, publication description, geographic location, and keywords. Appendix A lists 264 bibliographic references to literature identified during this reporting period but not abstracted due to time constraints. Title and publication description indexes are given for this appendix. Appendix B defines frequently used acronyms, and Appendix C lists the recipients of this report according to their corporate affiliation.« less

  16. DOE Office of Scientific and Technical Information (OSTI.GOV)

    Kautsky, Mark; Miller, David

    This annual report evaluates the performance of the groundwater remediation system at the Shiprock, New Mexico, Disposal Site (Shiprock site) for the period April 2015 through March 2016. The Shiprock site, a former uranium-ore processing facility remediated under the Uranium Mill Tailings Radiation Control Act, is managed by the U.S. Department of Energy (DOE) Office of Legacy Management. This annual report is based on an analysis of groundwater quality and groundwater level data obtained from site monitoring wells and the groundwater flow rates associated with the extraction wells, drains, and seeps. Background The Shiprock mill operated from 1954 to 1968more » on property leased from the Navajo Nation. Remediation of surface contamination, including stabilization of mill tailings in an engineered disposal cell, was completed in 1986. During mill operation, nitrate, sulfate, uranium, and other milling-related constituents leached into underlying sediments and contaminated groundwater in the area of the mill site. In March 2003, DOE initiated active remediation of groundwater at the site using extraction wells and interceptor drains. At that time, DOE developed a baseline performance report that established specific performance standards for the Shiprock site groundwater remediation system. The Shiprock site is divided into two distinct areas: the floodplain and the terrace. The floodplain remediation system consists of two groundwater extraction wells, a seep collection drain, and two collection trenches (Trench 1 and Trench 2). The terrace remediation system consists of nine groundwater extraction wells, two collection drains (Bob Lee Wash and Many Devils Wash), and a terrace drainage channel diversion structure. All extracted groundwater is pumped into a lined evaporation pond on the terrace. Compliance Strategy and Remediation Goals As documented in the Groundwater Compliance Action Plan, the U.S. Nuclear Regulatory Commission–approved compliance strategy for the floodplain is natural flushing supplemented by active remediation. The contaminants of concern (COCs) at the site are ammonia (total as nitrogen), manganese, nitrate (nitrate + nitrite as nitrogen), selenium, strontium, sulfate, and uranium. The compliance standards for nitrate, selenium, and uranium are listed in Title 40 Code of Federal Regulations Part 192. Regulatory standards are not available for ammonia, manganese, and sulfate; remediation goals for these constituents are either risk-based alternate cleanup standards or background levels. These standards and background levels apply only to the compliance strategy for the floodplain. The compliance strategy for the terrace is to eliminate exposure pathways at the washes and seeps and to apply supplemental standards in the western section.« less

  17. DOE Office of Scientific and Technical Information (OSTI.GOV)

    Metzler, D.; Gibb, J.P.; Glover, W.A.

    Compliance with the mandate of the Uranium Mill Tailings Radiation Control Act (UMTRCA) at Uranium Mill Tailings Remedial Action (UMTRA) Project sites requires implementation of a groundwater remedial action plan that meets the requirements of Subpart B of the US Environmental Protection Agency`s proposed groundwater protection standards (40 CFR 192). The UMTRA Groundwater Project will ensure that unacceptable current risk or potential risk to the public health, safety and the environment resulting from the groundwater contamination attributable to the UMTRA sites, is mitigated in a timely and cost-efficient manner. For each UMTRA processing site and vicinity property where contamination exists,more » a groundwater remedial action plan must be developed that identifies hazardous constituents and establishes acceptable concentration limits for the hazardous constituents as either (a) alternate concentration limits (ACL), (b) maximum concentration limits (MCLs), (c) supplemental standards, or (d) background groundwater quality levels. Project optimization is a strategy that will aggressively work within the current regulatory framework using all available options to meet regulatory requirements. This strategy is outlined within.« less

  18. Remedial action plan and site design for stabilization of the inactive Uranium Mill Tailing site Maybell, Colorado. Attachment 3, ground water hydrology report, Attachment 4, water resources protection strategy. Final report

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1994-06-01

    The U.S. Environmental Protection Agency (EPA) has established health and environmental regulations to correct and prevent ground water contamination resulting from former uranium processing activities at inactive uranium processing sites (40 CFR Part 192 (1993)) (52 FR 36000 (1978)). According to the Uranium Mill Tailings Radiation Control Act (UMTRCA) of 1978 (42 USC {section} 7901 et seq.), the U.S. Department of Energy (DOE) is responsible for assessing the inactive uranium processing sites. The DOE has decided that each assessment will include information on hydrogeologic site characterization. The water resources protection strategy that describes the proposed action compliance with the EPAmore » ground water protection standards is presented in Attachment 4, Water Resources Protection Strategy. Site characterization activities discussed in this section include the following: (1) Definition of the hydrogeologic characteristics of the environment, including hydrostratigraphy, aquifer parameters, areas of aquifer recharge and discharge, potentiometric surfaces, and ground water velocities. (2) Definition of background ground water quality and comparison with proposed EPA ground water protection standards. (3) Evaluation of the physical and chemical characteristics of the contaminant source and/or residual radioactive materials. (4) Definition of existing ground water contamination by comparison with the EPA ground water protection standards. (5) Description of the geochemical processes that affect the migration of the source contaminants at the processing site. (6) Description of water resource use, including availability, current and future use and value, and alternate water supplies.« less

  19. Remedial actions at the former Climax Uranium Company, Uranium Mill site, Grand Junction, Mesa County, Colorado. Volume 1, Text: Final environmental impact statement

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    None

    1986-12-01

    This statement evaluates and compares the environmental impacts associated with the remedial actions of the residual radioactive materials remaining at the inactive uranium processing site and associated vicinity properties at Grand Junction, Mesa County, Colorado. This statement is also intended to aid the BLM in amending their management framework plans and final resource management plan, as well as assisting in compliance with the withdrawal application as appropriate. The site is a 114-acre tract of private and state owned land which contains approximately 3.1 million cubic yards of tailings and associated contaminated soils. The vicinity properties are homes, businesses, public buildings,more » and vacant lots which may have been contaminated during construction by the use of tailings as building material. An estimated 3465 vicinity properties would be cleaned up during remedial action of the tailings pile. The tailings were produced by the former Climax Uranium Company which processed uranium ore, which it sold to the US Atomic Energy Commission from 1951 to 1966 and to private sources from 1966 to 1970. This statement evaluates six alternatives for stabilization and disposal of the tailings and other contaminated materials: (1) No action. (2) Stabilization at the Grand Junction site. (3) Disposal at the Cheney Reservoir site with truck transport. (4) Disposal at the Cheney Reservoir site with train and truck transport. (5) Disposal at the Two Road site with truck transport. (6) Disposal at the Two Road site with train and truck transport. All of the alternatives except no action include remedial action at an estimated 3465 vicinity properties. Alternative 3 is DOE`s preferred alternative.« less

  20. Innovative mathematical modeling in environmental remediation

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Yeh, Gour T.; National Central Univ.; Univ. of Central Florida

    2013-05-01

    There are two different ways to model reactive transport: ad hoc and innovative reaction-based approaches. The former, such as the Kd simplification of adsorption, has been widely employed by practitioners, while the latter has been mainly used in scientific communities for elucidating mechanisms of biogeochemical transport processes. It is believed that innovative mechanistic-based models could serve as protocols for environmental remediation as well. This paper reviews the development of a mechanistically coupled fluid flow, thermal transport, hydrologic transport, and reactive biogeochemical model and example-applications to environmental remediation problems. Theoretical bases are sufficiently described. Four example problems previously carried out aremore » used to demonstrate how numerical experimentation can be used to evaluate the feasibility of different remediation approaches. The first one involved the application of a 56-species uranium tailing problem to the Melton Branch Subwatershed at Oak Ridge National Laboratory (ORNL) using the parallel version of the model. Simulations were made to demonstrate the potential mobilization of uranium and other chelating agents in the proposed waste disposal site. The second problem simulated laboratory-scale system to investigate the role of natural attenuation in potential off-site migration of uranium from uranium mill tailings after restoration. It showed inadequacy of using a single Kd even for a homogeneous medium. The third example simulated laboratory experiments involving extremely high concentrations of uranium, technetium, aluminum, nitrate, and toxic metals (e.g.,Ni, Cr, Co).The fourth example modeled microbially-mediated immobilization of uranium in an unconfined aquifer using acetate amendment in a field-scale experiment. The purposes of these modeling studies were to simulate various mechanisms of mobilization and immobilization of radioactive wastes and to illustrate how to apply reactive transport models for environmental remediation.The second problem simulated laboratory-scale system to investigate the role of natural attenuation in potential off-site migration of uranium from uranium mill tailings after restoration. It showed inadequacy of using a single Kd even for a homogeneous medium.« less

  1. Surface complexation modeling of U(VI) adsorption by aquifer sediments from a former mill tailings site at Rifle, Colorado

    USGS Publications Warehouse

    Hyun, S.P.; Fox, P.M.; Davis, J.A.; Campbell, K.M.; Hayes, K.F.; Long, P.E.

    2009-01-01

    A study of U(VI) adsorption by aquifer sediment samples from a former uranium mill tailings site at Rifle, Colorado, was conducted under oxic conditions as a function of pH, U(VI), Ca, and dissolved carbonate concentration. Batch adsorption experiments were performed using <2mm size sediment fractions, a sand-sized fraction, and artificial groundwater solutions prepared to simulate the field groundwater composition. To encompass the geochemical conditions of the alluvial aquifer at the site, the experimental conditions ranged from 6.8 ?? 10-8 to 10-5 M in [U(VI)]tot, 7.2 to 8.0 in pH, 3.0 ?? 10-3 to 6.0 ?? 10 -3 M in [Ca2+], and 0.05 to 2.6% in partial pressure of carbon dioxide. Surface area normalized U(VI) adsorption Kd values for the sand and <2 mm sediment fraction were similar, suggesting a similar reactive surface coating on both fractions. A two-site two-reaction, nonelectrostatic generalized composite surface complexation model was developed and successfully simulated the U(VI) adsorption data. The model successfully predicted U(VI) adsorption observed from a multilevel sampling well installed at the site. A comparison of the model with the one developed previously for a uranium mill tailings site at Naturita, Colorado, indicated that possible calcite nonequilibrium of dissolved calcium concentration should be evaluated. The modeling results also illustrate the importance of the range of data used in deriving the best fit model parameters. ?? 2009 American Chemical Society.

  2. Ground water hydrology report: Revision 1, Attachment 3. Final

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    NONE

    1996-12-01

    This report presents ground water hydrogeologic activities for the Maybell, Colorado, Uranium Mill Tailings Remedial Action Project site. The Department of Energy has characterized the hydrogeology, water quality, and water resources at the site and determined that the proposed remedial action would comply with the requirements of the EPA ground water protection standards.

  3. Environmental Assessment of Ground Water Compliance at the Durango, Colorado, UMTRA Project Site

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    N /A

    2002-11-29

    The U.S. Department of Energy (DOE) is proposing a ground water compliance strategy for the Uranium Mill Tailings Remedial Action (UMTRA) Project site near Durango, Colorado. DOE has prepared this environmental assessment to provide the public with information concerning the potential effects of this proposed strategy.

  4. From rum jungle to Wismut-reducing the environmental impact of uranium mining and milling

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Zuk, W.M.; Jeffree, R.A.; Levins, D.M.

    1994-12-31

    Australia has a long history of uranium mining. In the early days, little attention was given to environmental matters and considerable pollution occurred. Ansto has been involved in rehabilitation of a number of the early uranium mining sites, from Rum Jungle in Australia`s Northern Territory to Wismut in Germany, and is working with current producers to minimise the environmental impact of their operations. Ansto`s expertise is extensive and includes, inter alia, amelioration of acid mine drainage, radon measurement and control, treatment of mill wastes, management of tailings, monitoring of seepage plumes, mathematical modelling of pollutant transport and biological impacts inmore » a tropical environment.« less

  5. Long-term surveillance plan for the Bodo Canyon Disposal Site, Durango, Colorado

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1994-03-01

    This long-term surveillance plan (LTSP) for the Durango, Colorado, Uranium Mill Tailings Remedial Action (UMTRA) Project disposal site describes the surveillance activities for the Durango (Bodo Canyon) disposal site, which will be referred to as the disposal site throughout this document. The US Department of Energy (DOE) will carry out these activities to ensure that the disposal site continues to function as designed. This LTSP was prepared as a requirement for acceptance under the US Nuclear Regulatory Commission (NRC) general license for custody and long-term care of residual radioactive materials (RRM). RRMs include tailings and other uranium ore processing wastesmore » still at the site, which the DOE determines to be radioactive. This LTSP is based on the DOE`s Guidance for Implementing the UMTRA Project Long-term Surveillance Program (DOE, 1992).« less

  6. Remedial action plan and site design for stabilization of the inactive uranium mill tailings sites at Rifle, Colorado. Volume 5, Addenda D6--D8 to Appendix D: Final report

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1990-02-01

    This volume contains appendices D6 through D8 containing laboratory test data: from MK-F investigation, 1987, Old Rifle and New Rifle sites; on bentonite amended radon barrier material; and from MK-F investigation, 1987, riprap tests.

  7. DOE Office of Scientific and Technical Information (OSTI.GOV)

    Kamboj, Sunita; Durham, Lisa A.

    A post-remediation radiological dose assessment was conducted for the Formerly Utilized Sites Remedial Action Program (FUSRAP) Linde Site by using the measured residual concentrations of the radionuclides of concern following the completion of the soils remedial action. The site’s FUSRAP-related contaminants of concern (COCs) are radionuclides associated with uranium processing activities conducted by the Manhattan Engineer District (MED) in support of the Nation’s early atomic energy and weapons program and include radium-226 (Ra-226), thorium-230 (Th-230), and total uranium (Utotal). Remedial actions to address Linde Site soils and structures were conducted in accordance with the Record of Decision for the Lindemore » Site, Tonawanda, New York (ROD) (USACE 2000a). In the ROD, the U.S. Army Corps of Engineers (USACE) determined that the cleanup standards found in Title 40, Part 192 of the Code of Federal Regulations (40 CFR Part 192), the standards for cleanup of uranium mill sites designated under the Uranium Mill Tailings Radiation Control Act (UMTRCA), and the Nuclear Regulatory Commission (NRC) standards for decommissioning of licensed uranium and thorium mills, found in 10 CFR Part 40, Appendix A, Criterion 6(6), are Applicable or Relevant and Appropriate Requirements (ARARs) for cleanup of MED-related contamination at the Linde Site. The major elements of this remedy will involve excavation of the soils with COCs above soil cleanup levels and placement of clean materials to meet the other criteria of 40 CFR Part 192.« less

  8. US Department of Energy response to standards for remedial actions at inactive uranium processing sites: Proposed rule

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1988-01-29

    The Title I groundwater standards for inactive uranium mill tailings sites, which were promulgated on January 5, 1983, by the US Environmental Protection Agency (EPA) for the Uranium Mill Tailings Remedial Action (UMTRA) Project, were remanded to the EPA on September 3, 1985, by the US Tenth Circuit Court of Appeals. The Court instructed the EPA to compile general groundwater standards for all Title I sites. On September 24, 1987, the EPA published proposed standards (52FR36000-36008) in response to the remand. This report includes an evaluation of the potential effects of the proposed EPA groundwater standards on the UMTRA Project,more » as well as a discussion of the DOE's position on the proposed standards. The report also contains and appendix which provides supporting information and cost analyses. In order to assess the impacts of the proposed EPA standards, this report summarizes the proposed EPA standards in Section 2.0. The next three sections assess the impacts of the three parts of the EPA standards: Subpart A considers disposal sites; Subpart B is concerned with restoration at processing sites; and Subpart C addresses supplemental standards. Section 6.0 integrates previous sections into a recommendations section. Section 7.0 contains the DOE response to questions posed by the EPA in the preamble to the proposed standards. 6 refs., 5 figs., 3 tabs.« less

  9. Atmospheric dispersion of radon around uranium mill tailings of the former Pridneprovsky Chemical Plant in Ukraine.

    PubMed

    Kovalets, Ivan V; Asker, Christian; Khalchenkov, Alexander V; Persson, Christer; Lavrova, Tatyana V

    2017-06-01

    Simulations of atmospheric dispersion of radon around the uranium mill tailings of the former Pridneprovsky Chemical Plant (PChP) in Ukraine were carried out with the aid of two atmospheric dispersion models: the Airviro Grid Model and the CALMET/CALPUFF model chain. The available measurement data of radon emission rates taken in the territories and the close vicinity of tailings were used in simulations. The results of simulations were compared to the yearly averaged measurements of concentration data. Both models were able to reasonably reproduce average radon concentration at the Sukhachivske site using averaged measured emission rates as input together with the measured meteorological data. At the same time, both models significantly underestimated concentrations as compared to measurements collected at the PChP industrial site. According to the results of both dispersion models, it was shown that only addition of significant radon emission rate from the whole territory of PChP in addition to emission rates from the tailings could explain the observed concentration measurements. With the aid of the uncertainty analysis, the radon emission rate from the whole territory of PChP was estimated to be between 1.5 and 3.5 Bq·m -2 s -1 . Copyright © 2017 Elsevier Ltd. All rights reserved.

  10. Contamination of the human food chain by uranium mill tailings piles

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Holtzman, R.B.; Urnezis, P.W.; Padova, A.

    A study is in progress to estimate the contamination of the human food chain by uranium, /sup 230/Th, /sup 226/Ra /sup 210/Pb, and /sup 210/Po originating from tailing piles associated with uranium ore processing mills. Rabbits, cattle, vegetables, and grass were collected on or near two uranium mill sites. For controls, similar samples were obtained from areas 20 km or more from the mining and mill operations. For the onsite rabbits the mean /sup 226/Ra concentrations in muscle, lung, and kidney of 5.5, 14, and 15 pCi/kg wet, respectively, were substantially higher than those in the respective tissues of controlmore » animals (0.4, 1.5, and 0.2 pCi/kg). The levels in liver did not differ significantly between the groups. The concentrations in bone (femur and vertebra) were about 9000 and 350 pCi/kg ash for the onsite and offsite animals, respectively. The levels of /sup 210/Pb and /sup 210/Po did not differ significantly for a given tissue between the two groups, except that the /sup 210/Pb level in the kidney was greater in the onsite group. For cattle, the concentrations in muscle, liver, and kidney do not differ greatly between those grazed near the pile and the controls. The levels of /sup 226/Ra, and possibly of /sup 210/Pb, appear to be greater in the femur of the animals near the piles. Vegetables from a residential area on a mill site contained substantially greater concentrations of /sup 226/Ra and /sup 210/Pb than those reported for standard New York City diets. Grass and cattle dung from land irrigated by water containing 60 pCi/L /sup 226/Ra from uranium mines had concentrations of /sup 226/Ra and /sup 210/Pb 50 and 8 times, respectively, those in control samples. It is estimated that doubling the normal concentrations in meat and vegetables of uranium and daughter products could increase the dose equivalent rates to the skeletons of persons consuming these foods by 30 or more mrem/yr.« less

  11. Ground-water contamination near a uranium tailings disposal site in Colorado

    USGS Publications Warehouse

    Goode, Daniel J.; Wilder, Russell J.

    1987-01-01

    Contaminants from uranium tailings disposed of at an active mill in Colorado have seeped into the shallow ground water onsite. This ground water discharges into the Arkansas River Valley through a superposed stream channel cut in the resistant sandstone ridge at the edge of a synclinal basin. In the river valley, seasonal surface-water irrigation has a significant impact on hydrodynamics. Water levels in residential wells fluctuate up to 20 ft and concentrations of uranium, molybdenum, and other contaminants also vary seasonally, with highest concentrations in the Spring, prior to irrigation, and lowest concentrations in the Fall. Results of a simple transient mixing cell model support the hypothesis that lateral ground-water inflow, and not irrigation recharge, is the source of ground-water contamination.

  12. THE INTERPLAY BETWEEN GEOCHEMICAL REACTIONS AND ADVECTION-DISPERSION IN CONTAMINANT TRANSPORT AT A URANIUM MILL TAILINGS SITE

    EPA Science Inventory

    It is well known that the fate and transport of contaminants in the subsurface are controlled by complex processes including advection, dispersion-diffusion, and chemical reactions. However, the interplay between the physical transport processes and chemical reactions, and their...

  13. Methods for Measuring Effects of Changes in Tamarisk Evapotranspiration on Groundwater at Southwestern Uranium Mill Tailings Sites

    NASA Astrophysics Data System (ADS)

    Waugh, W.; Nagler, P. L.; Vogel, J.; Glenn, E.; Nguyen, U.; Jarchow, C. J.

    2016-12-01

    Tamarisk (Tamarix spp.) is a non-native tree that competes with native species for water in riparian corridors of the southwestern U.S. The beetle, Diorhabda carinulata, which was released as a biocontrol agent, may be affecting tamarisk health. After several years of defoliation, tamarisk is now coming back along many southwestern rivers because of dwindling beetle numbers. We studied effects of changes in riparian plant communities dominated by tamarisk on evapotranspiration (ET) at uranium mill tailings sites. We used an unmanned aerial system (UAS) to acquire high resolution spectral data needed to estimate spatial and temporal variability in ET in riparian ecosystems at uranium mill tailings sites adjacent to the San Juan River near Shiprock, New Mexico, and the Colorado River near Moab, Utah. UAS imagery allowed us to monitor changes in phenology, fractional greenness, ET, and effects on water resources at these sites. We timed ground data and UAS image acquisition with an August 2016 Landsat image to assist with spatiotemporal scaling techniques. We measured leaf area index (LAI) and sampled biomass on tamarisk, cottonwood (Populus spp.), and willow (Salix spp.) within the UAS acquisition areas to scale leaf area on individual branches to LAI of whole trees. UAS cameras included a Sony Alpha A5100 for species-level vegetation mapping and a MicaSense Red Edge five-band multispectral camera to map Normalized Difference Vegetation Index (NDVI) and Enhanced Vegetation Index (EVI). The UAS products were correlated with satellite imagery. Our goal was to scale plant water use acquired from UAS imagery to Landsat and/or MODIS to provide a time-series documenting long-term trends and relationships of ET and groundwater elevation. NDVI and EVI were calibrated across UAS, MODIS and Landsat images using regression and ET was calculated using NDVI, EVI, ground meteorological data, and an existing empirical algorithm.

  14. 10 CFR 150.15a - Continued Commission authority pertaining to byproduct material.

    Code of Federal Regulations, 2010 CFR

    2010-01-01

    ... consistent with the provisions of the Uranium Mill Tailings Radiation Control Act of 1978, provided that the... Mill Tailings Radiation Control Act of 1978; and (6) The authority to enter into arrangements as may be...

  15. Microbiological, Geochemical and Hydrologic Processes Controlling Uranium Mobility: An Integrated Field-Scale Subsurface Research Challenge Site at Rifle, Colorado, Quality Assurance Project Plan

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Fix, N. J.

    The U.S. Department of Energy (DOE) is cleaning up and/or monitoring large, dilute plumes contaminated by metals, such as uranium and chromium, whose mobility and solubility change with redox status. Field-scale experiments with acetate as the electron donor have stimulated metal-reducing bacteria to effectively remove uranium [U(VI)] from groundwater at the Uranium Mill Tailings Site in Rifle, Colorado. The Pacific Northwest National Laboratory and a multidisciplinary team of national laboratory and academic collaborators has embarked on a research proposed for the Rifle site, the object of which is to gain a comprehensive and mechanistic understanding of the microbial factors andmore » associated geochemistry controlling uranium mobility so that DOE can confidently remediate uranium plumes as well as support stewardship of uranium-contaminated sites. This Quality Assurance Project Plan provides the quality assurance requirements and processes that will be followed by the Rifle Integrated Field-Scale Subsurface Research Challenge Project.« less

  16. Assessment and evaluation of engineering options at a low-level radioactive waste storage site

    NASA Astrophysics Data System (ADS)

    Kanehiro, B. Y.; Guvanasen, V.

    1982-09-01

    Solutions to hydrologic and geotechnical problems associated with existing disposal sites were sought and the efficiency of engineering options that were proposed to improve the integrity of such sites were evaluated. The Weldon Spring site is generally like other low-level nuclear waste sites, except that the wastes are primarily in the form of residues and contaminated rubble from the processing of uranium and thorium ores rather than industrial isotopes or mill tailings.

  17. The source of groundwater and solutes to Many Devils Wash at a former uranium mill site in Shiprock, New Mexico

    USGS Publications Warehouse

    Robertson, Andrew J.; Ranalli, Anthony J.; Austin, Stephen A.; Lawlis, Bryan R.

    2016-04-21

    The Shiprock Disposal Site is the location of the former Navajo Mill (Mill), a uranium ore-processing facility, located on a terrace overlooking the San Juan River in the town of Shiprock, New Mexico. Following the closure of the Mill, all tailings and associated materials were encapsulated in a disposal cell built on top of the former Mill and tailings piles. The milling operations, conducted at the site from 1954 to 1968, created radioactive tailings and process-related wastes that are now found in the groundwater. Elevated concentrations of constituents of concern—ammonium, manganese, nitrate, selenium, strontium, sulfate, and uranium—have also been measured in groundwater seeps in the nearby Many Devils Wash arroyo, leading to the inference that these constituents originated from the Mill. These constituents have also been reported in groundwater that is associated with Mancos Shale, the bedrock that underlies the site. The objective of this report is to increase understanding of the source of water and solutes to the groundwater beneath Many Devils Wash and to establish the background concentrations for groundwater that is in contact with the Mancos Shale at the site. This report presents evidence on three working hypotheses: (1) the water and solutes in Many Devils Wash originated from the operations at the former Mill, (2) groundwater in deep aquifers is upwelling under artesian pressure to recharge the shallow groundwater beneath Many Devils Wash, and (3) the groundwater beneath Many Devils Wash originates as precipitation that infiltrates into the shallow aquifer system and discharges to Many Devils Wash in a series of springs on the east side of the wash. The solute concentrations in the shallow groundwater of Many Devils Wash would result from the interaction of the water and the Mancos Shale if the source of water was upwelling from deep aquifers or precipitation.In order to compare the groundwater from various wells to groundwater that has been affected by Mill activities, a classification system was developed to determine which wells were most likely to have been affected. Affects to groundwater by the Mill were determined by using the reported uranium alpha activity ratios measured in groundwater samples, along with the concentration of the uranium and the location of the wells relative to the Mill. Activity ratios of 1.2 or less were determined to be the most reliable indicator of Mill-affected groundwater. Wells with samples that had a reported activity ratio of 1.2 or less were classified as Mill affected. To compare groundwater with background water-quality, data from groundwater seeps and springs in the Upper Eagle Nest Arroyo and Salt Creek Wash, located north of the San Juan River, are also presented and analyzed.Based on groundwater elevations and tritium concentrations measured in wells located between the disposal cell and Many Devils Wash, Mill water is not likely to reach Many Devils Wash. The tritium concentrations also indicate that groundwater from the Mill has not substantially affected Many Devils Wash in the past. Upwelling from deep aquifers was also determined to be an unlikely source, primarily by comparing the composition of the stable isotopes of water in the shallow groundwater with those reported in groundwater samples from the deeper aquifers. The stable-isotope compositions of the shallow groundwater around the site are enriched relative to the San Juan River and local meteoric lines, which suggests that most of the shallow groundwater has been influenced by evaporation and therefore was recharged at the surface. Several observations indicate that focused recharge is the likely source of groundwater in the area of Many Devils Wash. The visible erosional features in Many Devils Wash provide evidence of piping and groundwater sapping, and the distribution and type of vegetation in Many Devils Wash suggest that the focused recharge of precipitation is occurring. The estimated recharge from precipitation was calculated to be 0.0008 inches per year (in/yr) by using the mass-balance approach from reported seep discharge and 0.0011 in/yr using the chloride mass-balance approach.A conceptual model of groundwater quality beneath Many Devils Wash is presented to explain the source of solutes in the groundwater beneath Many Devils Wash. The major-ion concentrations and geochemical evolution in the groundwater beneath Many Devils Wash and across the study area support the conceptual model that the underlying Mancos Shale is the source of solutes. Differences in the major-ion composition between groundwater samples collected around the site, result from the degree of weathering to the Mancos Shale. The cation distribution appears to be an indicator of effects from the Mill, with samples from the Mill-affected wells largely having a calcium/magnesium-sulfate composition that resembles the reported compositions of more weathered shale; however, that composition could change if the Mill-processed water flowed into areas where the Mancos Shale was less weathered. On the basis of the widespread presence of uranium in the Mancos Shale and the distribution of aqueous uranium in the analog sites and other sites in the region, it appears likely that uranium in the groundwater of Many Devils Wash is naturally sourced from the Mancos Shale.

  18. A field experiment on Rn flux from reclaimed uranium mill tailings.

    PubMed

    Hinton, T G; Whicker, F W

    1985-04-01

    Design and construction techniques are described for a 1.6 ha experimental reclamation plot consisting of a 1-m-thick slab of uranium mill tailings covered with various depths of overburden. A passive, activated charcoal device was developed and used for measurements of Rn flux at the soil surface. Observations on Rn flux vs overburden depth indicated that tailings covered with 1.5 m of revegetated or 0.3 m of bare overburden had Rn exhalation rates comparable to background. Vegetated subplots exhibited a significantly higher (often an order of magnitude) flux than the bare subplots. A positive correlation was observed between precipitation quantities and Rn flux.

  19. Data Validation Package October 2015 Groundwater and Surface Water Sampling at the Monticello, Utah, Processing Site January 2016

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Nguyen, Jason; Smith, Fred

    Sampling Period: October 12–14, 2015. This semiannual event includes sampling groundwater and surface water at the Monticello Mill Tailings Site. Sampling and analyses were conducted as specified in the 2004 Monticello Mill Tailings Site Operable Unit III Post-Record of Decision Monitoring Plan, Draft Final and Sampling and Analysis Plan for U.S. Department of Energy Office of Legacy Management Sites (LMS/PRO/S04351, continually updated). Samples were collected from 52 of 61 planned locations (15 of 17 former mill site wells, 17 of 18 downgradient wells, 9 of 9 downgradient permeable reactive barrier wells, 2 of 7 seeps and wetlands, and 9 ofmore » 10 surface water locations). Locations MW00-07, Seep 1, Seep 2, Seep 3, Seep 5, Seep 6, SW00-01, T01-13, and T01-19 were not sampled because of insufficient water availability. All samples were filtered as specified in the monitoring plan. Duplicate samples were collected from surface water location W3-04 and from monitoring wells 82-08, 92-09, and 92-10. Water levels were measured at all but one sampled well and an additional set of wells. The contaminants of concern (COCs) for the Monticello Mill Tailings Site are arsenic, manganese, molybdenum, nitrate + nitrite as nitrogen (nitrate + nitrite as N), selenium, uranium, and vanadium. Time-concentration graphs of the COCs for all groundwater and surface water locations are included in this report. Locations with COCs that exceeded remediation goals are listed.« less

  20. Buffer zone monitoring plan for the Dos Rios subdivision, Gunnison, Colorado

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    NONE

    1996-02-01

    This report presents a plan for water quality monitoring at the Dos Rios subdivision (Units 2, 3, and the Island Unit) that is intended to satisfy the informational needs of residents who live southwest (downgradient) of the former Gunnison processing site. Water quality monitoring activities described in this report are designed to protect the public from residual contamination that entered the ground water as a result of previous uranium milling operations. Requirements presented in this monitoring plan are also included in the water sampling and analysis plan (WSAP) for the Gunnison Uranium Mill Tailings Remedial Action (UMTRA) Project site. Themore » Gunnison WSAP is a site-specific document prepared by the U.S. Department of Energy (DOE) that provides background, guidance, and justification for future ground water sampling and analysis activities for the UMTRA Project Gunnison processing and disposal sites. The WSAP will be updated annually, as additional water quality data are collected and interpreted, to provide ongoing protection for public health and the environment.« less

  1. Progress Toward Remediation of Uranium Tailings in Mailuu-Suu, Kyrgyzstan

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Buckley, P B; Ranville, J; Honeyman, B D

    2003-07-09

    The town of Mailuu-Suu in Kyrgyzstan inherited 23 distinct tailings deposits from Soviet-Era uranium mining operations. Mailuu-Suu is located in the narrow landslide-prone valley of the Mailuu-Suu River about 25 km from the Uzbekistan border. Large-scale release of the radioactive tailings, as a result of landslides, could lead to irreversible contamination of the river and downstream areas. The Mailuu-Suu River is a tributary to the Syr-Darya River, the Fergana valley's main source of irrigation water. The Fergana Valley is a key agricultural region and major population center that spans Kyrgyzstan, Tajikistan, and Uzbekistan. The trans-boundary nature of the Mailuu-Suu tailingsmore » issue presents an opportunity for collaboration among these Central Asian states. A cooperative approach to addressing environmental issues such as Mailuu-Suu may contribute to the region's stability by facilitating peaceful associations. Experience from remediation of sites in the US under the Uranium Mill Tailings Remediation Action Project (UMTRA) will be useful in progressing toward remediation at Mailuu-Suu.« less

  2. Subpart W: National Emission Standards for Radon Emissions From Operating Mill Tailings

    EPA Pesticide Factsheets

    Subpart W limits the radon-222 emissions rate from uranium tailings piles to 20 picocuries per square meter per second and requires that new tailings impoundments meet certain work practice standards.

  3. Uptake of Uranium and Other Elements of Concern by Plants Growing on Uranium Mill Tailings Disposal Cells

    NASA Astrophysics Data System (ADS)

    Joseph, C. N.; Waugh, W.; Glenn, E.

    2015-12-01

    The U.S. Department of Energy (DOE) is responsible for long-term stewardship of disposal cells for uranium mill tailings throughout the United States. Rock-armored disposal cell covers create favorable habitat for deep-rooted plants by reducing soil evaporation, increasing soil water storage, and trapping windblown dust, thereby providing water and nutrients for plant germination and establishment. DOE is studying the tradeoffs of potential detrimental and beneficial effects of plants growing on disposal cell covers to develop a rational and consistent vegetation management policy. Plant roots often extend vertically through disposal cell covers into underlying tailings, therefore, uptake of tailings contaminants and dissemination through animals foraging on stems and leaves is a possible exposure pathway. The literature shows that plant uptake of contaminants in uranium mill tailings occurs, but levels can vary widely depending on plant species, tailings and soil chemistry, and cover soil hydrology. Our empirical field study measured concentrations of uranium, radium, thorium, molybdenum, selenium, manganese, lead, and arsenic in above ground tissues harvested from plants growing on disposal cells near Native American communities in western states that represent a range of climates, cover designs, cover soil types, and vegetation types. For risk screening, contaminant levels in above ground tissues harvested from plants on disposal cells were compared to Maximum Tolerance Levels (MTLs) set for livestock by the National Research Council, and to tissue levels in the same plant species growing in reference areas near disposal cells. Although tailings were covered with uncontaminated soils, for 14 of 46 comparisons, levels of uranium and other contaminants were higher in plants growing on disposal cells compared to reference area plants, indicating possible mobilization of these elements from the tailing into plant tissues. However, with one exception, all plant levels were well below MTLs. Selenium, the only element that exceeded its MTL, likely originated in local seleniferous soil found both at reference areas and in disposal cell covers, and not in the underlying tailings. Our screening risk assessment suggests that allowing plants to grow on disposal cells appears to be safe.

  4. Department of Energy Programmatic Environmental Impact Statement (PEIS) scoping session

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1992-12-31

    The purpose of this programmatic environmental impact statement (PEIS) scoping meeting was: to present the ground water program so as to build some familiarity and understanding about the issue involved; and to get the Durango community`s input. This report contains the presentations made by the project manager for the uranium mill tailings program, site manager for the Durango UMTRA site, manager of ground water hydrology, and includes comments made by local residents.

  5. Comment and response document for the long-term surveillance plan for the Bodo Canyon Disposal Site, Durango, Colorado, Revision 0

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    NONE

    1995-11-01

    This report contains the comment and response document for the Draft Long-Term Surveillance Plan of the Bodo Canyon Site in Durango, California. This is a part of the Uranium Mill Tailings Remedial Action (UMTRA) Project. Questions and comments regarding specific sections or statements in the report are described and then a response to each review comment or question is provided.

  6. DOE Office of Scientific and Technical Information (OSTI.GOV)

    Muldoon, Joe; Yankovich, Tamara; Schramm, Laurier L.

    The Gunnar Mine and mill site was the largest of some 38 now-abandoned uranium mines that were developed and operated in Northern Saskatchewan, Canada, during the Cold War years. During their operating lifetimes these mines produced large quantities of ore and tailings. The Gunnar mine (open pit and underground) produced over 5 million tonnes of uranium ore and nearly 4.4 million tonnes of mine tailings during its operations from 1955 through 1963. An estimated 2.2 to 2.7 million m{sup 3} of waste rock that was generated during the processing of the ore abuts the shores of Lake Athabasca, the 22.more » largest lake in the world. After closure in the 1960's, the Gunnar site was abandoned with little to no decommissioning being done. The Saskatchewan Research Council has been contracted to manage the clean-up of these abandoned northern uranium mine and mill sites. The Gunnar Mine, because of the magnitude of tailings and waste rock, is subject to an environmental site assessment process regulated by both provincial and federal governments. This process requires a detailed study of the environmental impacts that have resulted from the mining activities and an analysis of projected impacts from remediation efforts. The environmental assessment process, specific site studies, and public involvement initiatives are all now well underway. Due to the many uncertainties associated with an abandoned site, an adaptive remediation approach, utilizing a decision tree, presented within the environmental assessment documents will be used as part of the site regulatory licensing. A critical early task was dealing with major public safety hazards on the site. The site originally included many buildings that were remnants of a community of approximately 800 people who once occupied the site. These buildings, many of which contained high levels of asbestos, had to be appropriately abated and demolished. Similarly, the original mine head frame and mill site buildings, many of which still contained the original machinery and equipment, also had to be dismantled. Remediation options for the accumulated demolition debris have been assessed, as have remediation options for the waste rock and tailings, all of which form part of the environmental assessment. The regulatory requirements include the environmental assessment processes, a complex public involvement strategy, and licensing from the Canadian Nuclear Safety Commission (CNSC) with the long-term goal of releasing the property in a remediated and stable state to the Province of Saskatchewan. Prescribed environmental and land use endpoints will be determined based on the environmental assessment studies and remediation options analyzed and implemented. Ultimately, the site will be released into an institutional controls program that will allow long-term government management and monitoring. (authors)« less

  7. Format and style for environmental documents prepared as part of the Uranium Mill Tailings Remedial Action Program

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1980-06-01

    The Uranium Mill Tailings Remedial Action Program will require the preparation of several environmental impact statements and several environmental assessments. This guide begins with a section describing in general terms the efforts required to make these documents readable. The sections describe the formats to be used for the pages, headings, front matter, footnotes, lists, figures, tables, references, glossaries, indexes, and appendixes in these documents. A final section presents some rules of style to be followed in writing the texts.

  8. Uranium mill tailings: nuclear waste and natural laboratory for geochemical and radioecological investigations

    USGS Publications Warehouse

    Landa, Edward R.

    2004-01-01

    Uranium mill tailings (UMT) are a high volume, low specific activity radioactive waste typically disposed in surface impoundments. This review focuses on research on UMT and related earth materials during the past decade relevant to the assessment of: (1) mineral hosts of radionuclides; (2) the use of soil analogs in predicting long-term fate of radionuclides; (3) microbial and diagenetic processes that may alter radionuclide mobility in the surficial environment; (4) waste-management technologies to limit radionuclide migration; and (5) the impact of UMT on biota.

  9. 40 CFR 61.252 - Standard.

    Code of Federal Regulations, 2011 CFR

    2011-07-01

    ... EMISSION STANDARDS FOR HAZARDOUS AIR POLLUTANTS National Emission Standards for Radon Emissions From Operating Mill Tailings § 61.252 Standard. (a) Radon-222 emissions to the ambient air from an existing uranium mill tailings pile shall not exceed 20 pCi/(m2-sec) (1.9 pCi/(ft2-sec)) of radon-222. (b) After...

  10. 10 CFR Appendix A to Part 40 - Criteria Relating to the Operation of Uranium Mills and the Disposition of Tailings or Wastes...

    Code of Federal Regulations, 2012 CFR

    2012-01-01

    ... itself. (6) The design requirements in this criterion for longevity and control of radon releases apply... radiological and nonradiological hazards associated with the sites, which is equivalent to, to the extent... “reasonably achievable” as equivalent terms. Decisions involved these terms will take into account the state...

  11. 10 CFR Appendix A to Part 40 - Criteria Relating to the Operation of Uranium Mills and the Disposition of Tailings or Wastes...

    Code of Federal Regulations, 2014 CFR

    2014-01-01

    ... associated with the sites, which is equivalent to, to the extent practicable, or more stringent than the... this appendix, the Commission will consider “practicable” and “reasonably achievable” as equivalent... formation, group of formations, or part of a formation capable of yielding a significant amount of ground...

  12. 30 CFR 875.16 - Exclusion of certain noncoal reclamation sites.

    Code of Federal Regulations, 2011 CFR

    2011-07-01

    ... moneys from the Fund or from prior balance replacement funds provided under § 872.29 of this chapter for... Radiation Control Act of 1978 (42 U.S.C. 7901 et seq.) or that have been listed for remedial action under... Uranium Mill Tailings Radiation Control Act of 1978 (42 U.S.C. 7901 et seq.) or that have been listed for...

  13. 30 CFR 875.16 - Exclusion of certain noncoal reclamation sites.

    Code of Federal Regulations, 2010 CFR

    2010-07-01

    ... Radiation Control Act of 1978 (42 U.S.C. 7901 et seq.) or that have been listed for remedial action under the Comprehensive Environmental Response Compensation and Liability Act of 1980 (42 U.S.C. 9601 et seq... Uranium Mill Tailings Radiation Control Act of 1978 (42 U.S.C. 7901 et seq.) or that have been listed for...

  14. Evolution of uranium distribution and speciation in mill tailings, COMINAK Mine, Niger.

    PubMed

    Déjeant, Adrien; Galoisy, Laurence; Roy, Régis; Calas, Georges; Boekhout, Flora; Phrommavanh, Vannapha; Descostes, Michael

    2016-03-01

    This study investigated the evolution of uranium distribution and speciation in mill tailings from the COMINAK mine (Niger), in production since 1978. A multi-scale approach was used, which combined high resolution remote sensing imagery, ICP-MS bulk rock analyses, powder X-ray diffraction, Scanning Electron Microscopy, Focused Ion Beam--Transmission Electron Microscopy and X-ray Absorption Near Edge Spectroscopy. Mineralogical analyses showed that some ore minerals, including residual uraninite and coffinite, undergo alteration and dissolution during tailings storage. The migration of uranium and other contaminants depends on (i) the chemical stability of secondary phases and sorbed species (dissolution and desorption processes), and (ii) the mechanical transport of fine particles bearing these elements. Uranium is stabilized after formation of secondary uranyl sulfates and phosphates, and adsorbed complexes on mineral surfaces (e.g. clay minerals). In particular, the stock of insoluble uranyl phosphates increases with time, thus contributing to the long-term stabilization of uranium. At the surface, a sulfate-cemented duricrust is formed after evaporation of pore water. This duricrust limits water infiltration and dust aerial dispersion, though it is enriched in uranium and many other elements, because of pore water rising from underlying levels by capillary action. Satellite images provided a detailed description of the tailings pile over time and allow monitoring of the chronology of successive tailings deposits. Satellite images suggest that uranium anomalies that occur at deep levels in the pile are most likely former surface duricrusts that have been buried under more recent tailings. Copyright © 2015 Elsevier B.V. All rights reserved.

  15. 40 CFR 192.34 - Effective date.

    Code of Federal Regulations, 2014 CFR

    2014-07-01

    ... AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Standards for Management of Uranium Byproduct Materials Pursuant to Section 84 of the Atomic Energy Act of 1954, as Amended...

  16. 40 CFR 192.34 - Effective date.

    Code of Federal Regulations, 2013 CFR

    2013-07-01

    ... AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Standards for Management of Uranium Byproduct Materials Pursuant to Section 84 of the Atomic Energy Act of 1954, as Amended...

  17. 40 CFR 192.10 - Applicability.

    Code of Federal Regulations, 2013 CFR

    2013-07-01

    ... AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Standards for Cleanup of Land and Buildings Contaminated with Residual Radioactive Materials from Inactive Uranium Processing... radioactive materials at which all or substantially all of the uranium was produced for sale to any Federal...

  18. 40 CFR 192.10 - Applicability.

    Code of Federal Regulations, 2014 CFR

    2014-07-01

    ... AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Standards for Cleanup of Land and Buildings Contaminated with Residual Radioactive Materials from Inactive Uranium Processing... radioactive materials at which all or substantially all of the uranium was produced for sale to any Federal...

  19. Column Testing and 1D Reactive Transport Modeling to Evaluate Uranium Plume Persistence Processes

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Johnson, Raymond H.; Morrison, Stan; Morris, Sarah

    Motivation for Study: Natural flushing of contaminants at various U.S. Department of Energy Office of Legacy Management sites is not proceeding as quickly as predicted (plume persistence) Objectives: Help determine natural flushing rates using column tests. Use 1D reactive transport modeling to better understand the major processes that are creating plume persistence Approach: Core samples from under a former mill tailings area Tailings have been removed. Column leaching using lab-prepared water similar to nearby Gunnison River water. 1D reactive transport modeling to evaluate processes

  20. Final report of the decontamination and decommissioning of the exterior land areas at the Grand Junction Projects Office facility

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Widdop, M.R.

    1995-09-01

    The US Department of Energy (DOE) Grand Junction Projects Office (GJPO) facility occupies approximately 56.4 acres (22.8 hectares) along the Gunnison River near Grand Junction, Colorado. The site was contaminated with uranium ore and mill tailings during uranium-refining activities conducted by the Manhattan Engineer District and during pilot-milling experiments conducted for the US Atomic Energy Commission`s (AEC`s) domestic uranium procurement program. The GJPO facility was the collection and assay point for AEC uranium and vanadium oxide purchases until the early 1970s. The DOE Decontamination and Decommissioning Program sponsored the Grand Junction Projects Office Remedial Action Project (GJPORAP) to remediate themore » facility lands, site improvements, and the underlying aquifer. The site contractor, Rust Geotech, was the Remedial Action Contractor for GJPORAP. The exterior land areas of the facility assessed as contaminated have been remediated in accordance with identified standards and can be released for unrestricted use. Restoration of the aquifer will be accomplished through the natural flushing action of the aquifer during the next 50 to 80 years. The remediation of the DOE-GJPO facility buildings is ongoing and will be described in a separate report.« less

  1. Surface Water-Groundwater Interactions as a Critical Component of Uranium Plume Persistence

    NASA Astrophysics Data System (ADS)

    Williams, K. H.; Christensen, J. N.; Hobson, C.

    2015-12-01

    Residual contamination of soils, sediments and groundwater by uranium milling operations presents a lingering problem at former mill sites throughout the upper Colorado River Basin in the western USA. Remedial strategies predicated upon natural flushing by low uranium recharge waters have frequently failed to achieve target concentrations set by national and state regulators. Flushing times of tens of years have often yielded negligible decreases in groundwater uranium concentrations, with extrapolated trends suggesting multiple decades or longer may be required to achieve regulatory goals. The U.S. Department of Energy's Rifle, Colorado field site serves as a natural laboratory for investigating the underlying causes for uranium plume persistence, with recent studies there highlighting the important role that surface water-groundwater interactions play in sustaining uranium delivery to the aquifer. Annual snowmelt-driven increases in Colorado River discharge induce 1-2 m excursions in groundwater elevation at the Rifle site, which enables residual tailings-contaminated materials (so-called Supplemental Standards) to become hydrologically connected to the aquifer for short periods of time during peak discharge. The episodic contact between shallow groundwater and residual contamination leads to abrupt 20-fold increases in groundwater uranium concentration, which serve to seasonally replenish the plume given the location of the Supplemental Standards along the upgradient edge of the aquifer. Uranium isotope composition changes abruptly as uranium concentrations increase reflecting the contribution of a temporally distinct contaminant reservoir. The release of uranium serves to potentially replenish organic matter rich sediments located within the alluvial aquifer at downstream locations, which have been postulated to serve as a parallel contributor to plume persistence following the uptake, immobilization, and slow re-oxidation of uranium.

  2. 40 CFR 192.33 - Corrective action programs.

    Code of Federal Regulations, 2014 CFR

    2014-07-01

    ... PROGRAMS HEALTH AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Standards for Management of Uranium Byproduct Materials Pursuant to Section 84 of the Atomic Energy Act of 1954, as Amended...

  3. 40 CFR 192.33 - Corrective action programs.

    Code of Federal Regulations, 2013 CFR

    2013-07-01

    ... PROGRAMS HEALTH AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Standards for Management of Uranium Byproduct Materials Pursuant to Section 84 of the Atomic Energy Act of 1954, as Amended...

  4. Evaluation of liners for a uranium-mill tailings disposal site: a status report

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Buelt, J.L.; Hale, V.Q.; Barnes, S.M.

    1981-05-01

    The United States Department of Energy is conducting a program designed to reclaim or stabilize inactive uranium-mill tailings sites. This report presents the status of the Liner Evaluation Program. The purpose of the study was to identify eight prospective lining materials or composites for laboratory testing. The evaluation was performed by 1) reviewing proposed regulatory requirements to define the material performance criteria; 2) reviewing published literature and communicating with industrial and government experts experienced with lining materials and techniques; and 3) characterizing the tailings at three of the sites for calcium concentration, a selection of anions, radionuclides, organic solvents, andmore » acidity levels. The eight materials selected for laboratory testing are: natural soil amended with sodium-saturated montmorillonite (Volclay); locally available clay in conjunction with an asphalt emulsion radon suppression cover; locally available clay in conjunction with a multibarrier radon suppression cover; rubberized asphalt membrane; hydraulic asphalt concrete; chlorosulfonated polyethylene (hypalon) or high-density polyethylene; bentonite, sand and gravel mixture; and catalytic airblown asphalt membrane. The materials will be exposed in test units now being constructed to conditions such as wet/dry cycles, temperature cycles, oxidative environments, ion-exchange elements, etc. The results of the tests will identify the best material for field study. The status report also presents the information gathered during the field studies at Grand Junction, Colorado. Two liners, a bentonite, sand and gravel mixture, and a catalytic airblown asphalt membrane, were installed in a prepared trench and covered with tailings. The liners were instrumented and are being monitored for migration of moisture, radionuclides, and hazardous chemicals. The two liner materials will also be subjected to accelerated laboratory tests for a comparative assessment.« less

  5. Final report of the decontamination and decommissioning of Building 6 at the Grand Junction Projects Office Facility

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Widdop, M.R.

    1996-07-01

    The U.S. Department of Energy (DOE) Grand Junction Projects Office (GJPO) occupies a 61.7-acre facility along the Gunnison River near Grand Junction, Colorado. This site was contaminated with uranium ore and mill tailings during uranium refining activities of the Manhattan Engineer District and during pilot milling experiments conducted for the domestic uranium procurement program funded by the U.S. Atomic Energy Commission. The DOE Defense Decontamination and Decommissioning Program established the GJPO Remedial Action Project to clean up and restore the facility lands, improvements, and the underlying aquifer. The site contractor for the facility, Rust Geotech, is also the remedial actionmore » contractor. Radiological contamination was identified in Building 6, and the building was demolished in 1992. The soil area within the footprint of the building has been remediated in accordance with the identified standards and the area can be released for unlimited exposure and unrestricted use. This document was prepared in response to a DOE request for an individual final report for each contaminated GJPO building.« less

  6. Final report of the decontamination and decommissioning of Building 34 at the Grand Junction Projects Office Facility

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Widdop, M.R.

    1996-08-01

    The U.S. Department of Energy (DOE) Grand Junction Projects Office (GJPO) occupies a 61.7 acre facility along the Gunnison River near Grand Junction, Colorado. This site was contaminated with uranium ore and mill tailings during uranium refining activities of the Manhattan Engineer District and during pilot milling experiments conducted for the U.S. Atomic Energy Commission`s domestic uranium procurement program. The DOE Defense Decontamination and Decommissioning Program established the Grand Junction Projects Office Remedial Action Project to clean up and restore the facility lands, improvements, and the underlying aquifer. The site contractor for the facility, Rust Geotech, was also the remedialmore » action contractor. Building 34 was radiologically contaminated and the building was demolished in 1996. The soil area within the footprint of the building was analyzed and found to be not contaminated. The area can be released for unlimited exposure and unrestricted use. This document was prepared in response to a DOE request for an individual closeout report for each contaminated GJPO building.« less

  7. Final report of the decontamination and decommissioning of Building 39 at the Grand Junction Projects Office Facility

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Widdop, M.R.

    1996-07-01

    The U.S. Department of Energy (DOE) Grand Junction Projects Office (GJPO) occupies a 61.7-acre facility along the Gunnison River near Grand Junction, Colorado. This site was contaminated with uranium ore and mill tailings during uranium refining activities of the Manhattan Engineer District and during pilot milling experiments conducted for the U.S. Atomic Energy Commission`s domestic uranium procurement program. The DOE Defense Decontamination and Decommissioning Program established the GJPO Remedial Action Project to clean up and restore the facility lands, improvements, and the underlying aquifer. The site contractor for the facility, Rust Geotech, is also the remedial action contractor. The soilmore » beneath Building 39 was radiologically contaminated and the building was demolished in 1992. The soil area within the footprint of the building has been remediated in accordance with the identified standards and the area can be released for unlimited exposure and unrestricted use. This document was prepared in response to a DOE request for an individual final report for each contaminated GJPO building.« less

  8. Final report of the decontamination and decommissioning of Building 44 at the Grand Junction Projects Office Facility

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Widdop, M.R.

    1996-07-01

    The U.S. Department of Energy (DOE) Junction Projects Office (GJPO) occupies a 61.7 acre facility along the Gunnison River near Grand Junction, Colorado. This site was contaminated with uranium ore and mill tailings during uranium refining activities of the Manhattan Engineer District and during pilot milling experiments conducted for the U.S. Atomic Energy Commission`s domestic uranium procurement program. The DOE Defense Decontamination and Decommissioning Program established the Grand Junction Projects Office Remedial Action Project to clean up and restore the facility lands, improvements, and the underlying aquifer. The site contractor for the facility, Rust Geotech, is also the remedial actionmore » contractor. Building 44 was radiologically contaminated and the building was demolished in 1994. The soil area within the footprint of the building was not contaminated; it complies with the identified standards and the area can be released for unlimited exposure and unrestricted use. This document was prepared in response to a DOE request for an individual final report for each contaminated GJPO building.« less

  9. US Department of Energy Grand Junction Projects Office Remedial Action Project, final report of the decontamination and decommissioning of Building 36 at the Grand Junction Projects Office Facility

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Widdop, M.R.

    1996-08-01

    The U.S. Department of Energy (DOE) Grand Junction Projects Office (GJPO) occupies a 61.7-acre facility along the Gunnison River near Grand Junction, Colorado. This site was contaminated with uranium ore and mill tailings during uranium refining activities of the Manhattan Engineer District and during pilot milling experiments conducted for the U.S. Atomic Energy Commission`s domestic uranium procurement program. The DOE Defense Decontamination and Decommissioning Program established the GJPO Remedial Action Project to clean up and restore the facility lands, improvements, and the underlying aquifer. The site contractor for the facility, Rust Geotech, also is the remedial action contractor. Building 36more » was found to be radiologically contaminated and was demolished in 1996. The soil beneath the building was remediated in accordance with identified standards and can be released for unlimited exposure and unrestricted use. This document was prepared in response to a DOE request for an individual final report for each contaminated GJPO building.« less

  10. Final report of the decontamination and decommissioning of Building 18 at the Grand Junction Projects Office Facility

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Widdop, M.R.

    1996-08-01

    The U.S. Department of Energy (DOE) Grand Junction Projects Office (GJPO) occupies a 61.7-acre facility along the Gunnison River near Grand Junction, Colorado. This site was contaminated with uranium ore and mill tailings during uranium refining activities of the Manhattan Engineer District and during pilot milling experiments conducted for the U.S. Atomic Energy Commission`s domestic uranium procurement program. The DOE Defense Decontamination and Decommissioning Program established the GJPO Remedial Action Project to clean up and restore the facility lands, improvements, and the underlying aquifer. The site contractor for the facility, Rust Geotech, also is the remedial action contractor. The soilmore » beneath Building 18 was found to be radiologically contaminated; the building was not contaminated. The soil was remediated in accordance with identified standards. Building 18 and the underlying soil can be released for unlimited exposure and unrestricted use. This document was prepared in response to a DOE request for an individual final report for each contaminated GJPO building.« less

  11. Final report of the decontamination and decommissioning of Building 1 at the Grand Junction Projects Office Facility

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Widdop, M.R.

    1996-08-01

    The U.S. Department of Energy (DOE) Grand Junction Projects Office (GJPO) occupies a 61.7-acre facility along the Gunnison River near Grand Junction, Colorado. This site was contaminated with uranium ore and mill tailings during uranium refining activities of the Manhattan Engineer District and during pilot milling experiments conducted for the U.S. Atomic Energy Commission`s domestic uranium procurement program. The DOE Defense Decontamination and Decommissioning Program established the GJPO Remedial Action Project to clean up and restore the facility lands, improvements, and the underlying aquifer. The site contractor for the facility, Rust Geotech, also is the remedial action contractor. Building 1more » was found to be radiologically contaminated and was demolished in 1996. The soil beneath and adjacent to the building was remediated in accordance with identified standards and can be released for unlimited exposure and unrestricted use. This document was prepared in response to a DOE request for an individual final report for each contaminated GJPO building.« less

  12. Geochemical investigations by the U.S. Geological Survey on uranium mining, milling, and environmental restoration

    USGS Publications Warehouse

    Landa, Edward R.; Cravotta, Charles A.; Naftz, David L.; Verplanck, Philip L.; Nordstrom, D. Kirk; Zielinski, Robert A.

    2000-01-01

    Recent research by the U.S. Geological Survey has characterized contaminant sources and identified important geochemical processes that influence transport of radionuclides from uranium mining and milling wastes. 1) Selective extraction studies indicated that alkaline earth sulfates and hydrous ferric oxides are important hosts of 226Ra in uranium mill tailings. The action of sulfate-reducing and ironreducing bacteria on these phases was shown to enhance release of radium, and this adverse result may temper decisions to dispose of uranium mill tailings in anaerobic environments. 2) Field studies have shown that although surface-applied sewage sludge/wood chip amendments aid in revegetating pyritic spoil, the nitrogen in sludge leachate can enhance pyrite oxidation, acidification of groundwater, and the consequent mobilization of metals and radionuclides. 3) In a U.S. Environmental Protection Agencyfunded study, three permeable reactive barriers consisting of phosphate-rich material, zero-valent iron, or amorphous ferric oxyhydroxide have been installed at an abandoned uranium upgrader facility near Fry Canyon, UT. Preliminary results indicate that each of the permeable reactive barriers is removing the majority of the uranium from the groundwater. 4) Studies on the geochemistry of rare earth elements as analogues for actinides such as uranium and thorium in acid mine drainage environments indicate high mobility under acid-weathering conditions but measurable attenuation associated with iron and aluminum colloid formation. Mass balances from field and laboratory studies are being used to quantify the amount of attenuation. 5) A field study in Colorado demonstrated the use of 234U/238U isotopic ratio measurements to evaluate contamination of shallow groundwater with uranium mill effluent.

  13. Assessment of potential migration of radionuclides and trace elements from the White Mesa uranium mill to the Ute Mountain Ute Reservation and surrounding areas, southeastern Utah

    USGS Publications Warehouse

    Naftz, David L.; Ranalli, Anthony J.; Rowland, Ryan C.; Marston, Thomas M.

    2011-01-01

    In 2007, the Ute Mountain Ute Tribe requested that the U.S. Environmental Protection Agency and U.S. Geological Survey conduct an independent evaluation of potential offsite migration of radionuclides and selected trace elements associated with the ore storage and milling process at an active uranium mill site near White Mesa, Utah. Specific objectives of this study were (1) to determine recharge sources and residence times of groundwater surrounding the mill site, (2) to determine the current concentrations of uranium and associated trace elements in groundwater surrounding the mill site, (3) to differentiate natural and anthropogenic contaminant sources to groundwater resources surrounding the mill site, (4) to assess the solubility and potential for offsite transport of uranium-bearing minerals in groundwater surrounding the mill site, and (5) to use stream sediment and plant material samples from areas surrounding the mill site to identify potential areas of offsite contamination and likely contaminant sources.

  14. Uptake and speciation of uranium in synthetic gypsum (CaSO4•2H2O): Applications to radioactive mine tailings.

    PubMed

    Lin, Jinru; Sun, Wei; Desmarais, Jacques; Chen, Ning; Feng, Renfei; Zhang, Patrick; Li, Dien; Lieu, Arthur; Tse, John S; Pan, Yuanming

    2018-01-01

    Phosphogypsum formed from the production of phosphoric acid represents by far the biggest accumulation of gypsum-rich wastes in the world and commonly contains elevated radionuclides, including uranium, as well as other heavy metals and metalloids. Therefore, billions-of-tons of phosphogypsum stockpiled worldwide not only possess serious environmental problems but also represent a potential uranium resource. Gypsum is also a major solid constituent in many other types of radioactive mine tailings, which stems from the common usage of sulfuric acid in extraction processes. Therefore, management and remediation of radioactive mine tailings as well as future beneficiation of uranium from phosphogysum all require detailed knowledge about the nature and behavior of uranium in gypsum. However, little is known about the uptake mechanism or speciation of uranium in gypsum. In this study, synthesis experiments suggest an apparent pH control on the uptake of uranium in gypsum at ambient conditions: increase in U from 16 μg/g at pH = 6.5 to 339 μg/g at pH = 9.5. Uranium L 3 -edge synchrotron X-ray absorption spectroscopic analyses of synthetic gypsum show that uranyl (UO 2 ) 2+ at the Ca site is the dominant species. The EXAFS fitting results also indicate that uranyl in synthetic gypsum occurs most likely as carbonate complexes and yields an average U-O distance ∼0.25 Å shorter than the average Ca-O distance, signifying a marked local structural distortion. Applications to phosphogypsum from the New Wales phosphoric acid plant (Florida, USA) and uranium mine tailings from the Key Lake mill (Saskatchewan, Canada) show that gypsum is an important carrier of uranium over a wide range of pH and controls the fate of this radionuclide in mine tailings. Also, development of new technologies for recovering U from phosphogypsum in the future must consider lattice-bound uranyl in gypsum. Copyright © 2017 Elsevier Ltd. All rights reserved.

  15. Results of the independent verification of radiological remedial action at 397 East 3rd South Street, Monticello, Utah (MS00168)

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Wilson, M.J.; Crutcher, J.W.

    1991-07-01

    In 1980 the site of a vanadium and uranium mill at Monticello, Utah, was accepted into the US Department of Energy's (DOE's) Surplus Facilities Management Program, with the objectives of restoring the government-owned mill site to safe levels of radioactivity, disposing of or containing the tailings in an environmentally safe manner, and performing remedial actions on off-site (vicinity) properties that had been contaminated by radioactive material resulting from mill operations. During 1987 and 1988, UNC Geotech, the remedial action contractor designated by DOE, performed remedial action on the vicinity property at 397 East 3rd South Street, Monticello, Utah. The Pollutantmore » Assessments Group (PAG) of Oak Ridge National Laboratory was assigned the responsibility of verifying the data supporting the adequacy of remedial action and confirming the site's compliance with DOE guidelines. The PAG found that the site successfully meets the DOE remedial action objectives. Procedures used by PAG are described. 3 refs., 2 tabs.« less

  16. Results of the independent verification of radiological remedial action at 464 South 1st East Street, Monticello, Utah (MS00071)

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Wilson, M.J.; Crutcher, J.W.

    1991-07-01

    In 1980 the site of a vanadium and uranium mill at Monticello, Utah, was accepted into the US Department of Energy's (DOE's) Surplus Facilities Management Program, with the objectives of restoring the government-owned mill site to safe levels of radioactivity, disposing of or containing the tailings in an environmentally safe manner, and performing remedial actions on off-site (vicinity) properties that had been contaminated by radioactive material resulting from mill operations. During 1986 and 1987, UNC Geotech, the remedial action contractor designated by DOE, performed remedial action on the vicinity property at 464 South 1st East Street, Monticello, Utah. The Pollutantmore » Assessments Group (PAG) of Oak Ridge National Laboratory was assigned the responsibility of verifying the data supporting the adequacy of remedial action and confirming the site's compliance with DOE guidelines. The PAG found that the site successfully meets the DOE remedial action objectives. Procedures used by PAG are described. 3 refs., 2 tabs.« less

  17. Results of the independent verification of radiological remedial action at 16 East 5th South Street, Monticello, Utah (MS00075)

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Wilson, M.J.; Crutcher, J.W.

    1991-07-01

    In 1980 the site of a vanadium and uranium mill at Monticello, Utah, was accepted into the US Department of Energy's (DOE's) Surplus Facilities Management Program, with the objectives of restoring the government-owned mill site to safe levels of radioactivity, disposing of or containing the tailings in an environmentally safe manner, and performing remedial actions on off-site (vicinity) properties that had been contaminated by radioactive material resulting from mill operations. During 1984 UNC Geotech, the remedial action contractor designated by DOE, performed remedial action on the vicinity property at 16 East 5th South Street, Monticello, Utah. The Pollutant Assessments Groupmore » (PAG) of Oak Ridge National Laboratory was assigned the responsibility of verifying the data supporting the adequacy of remedial action and confirming the site's compliance with DOE guidelines. The PAG found that the site successfully meets the DOE remedial action objectives. Procedures used by PAG are described. 3 refs., 2 tabs.« less

  18. Evaluation of Permeable Reactive Barrier Performance

    DTIC Science & Technology

    2002-12-09

    and-fill operation, where the trench was initially stabilized using guar gum and subsequently broken down by circulating an enzyme through the trench...80 Peerless Reactive cell placed within gravel-filled capture trench, guar gum used during installation Uranium Mill Tailings Site...Regulatory Issues 5.3.1 Biostat. The use of guar gum (a natural food thickener) as a reactive medium or as a support for trench excavation, is gaining

  19. 2015 Advanced Site Investigation and Monitoring Report Riverton, Wyoming, Processing Site September 2016

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Frazier, William; Campbell, Sam

    The U.S. Department of Energy conducted initial groundwater characterization of the Riverton, Wyoming, Processing Site in the 1990s. The characterization culminated in a Site Observational Work Plan in 1998 that recommended a natural flushing compliance strategy. Results of verification monitoring indicated that natural flushing was generally progressing as expected until June 2010, when significant increases in contaminant concentrations were measured in several monitoring wells downgradient of the site after the area flooded. In response to the unexpected results following the flood, an enhanced characterization of the surficial aquifer was conducted in 2012, which included installation of 103 boreholes along ninemore » transects with a Geoprobe, collection of 103 water samples and 65 soil samples, laboratory tests on the soil samples, and additional groundwater modeling. This advanced site investigation report summarizes additional investigation in 2015 through the use of backhoe trenching, sonic drilling, multilevel monitoring wells, direct-push drilling, and temporary well points to collect soil and groundwater samples. Additional surface water measurements were made included the installation of a stilling well and the measurement of stream elevation along the Wind River to approximate upgradient groundwater heads. Groundwater sampling included the addition of geochemical constituents and isotopes that have not been sampled in the past to better understand post-flood conditions and the possibility of additional or ongoing contaminant sources. This sampling was performed to (1) better define the contaminant plumes, (2) verify the occurrence of persistent secondary contaminant sources, (3) better understand the reason for the contaminant spikes after a 2010 flood, and (4) assess contaminant plume stagnation near the Little Wind River. This report provides data analyses and interpretations for the 2015 site investigation that addresses these issues and provides recommendations for future efforts. Observations from trenches and sonic drilling indicate the general lithology of the shallow, unconsolidated sediments consists of a silt zone at the surface that ranges from 2.5 to 4.8 feet below ground surface, underlain by sand and gravel, underlain by the top of the weathered bedrock (Wind River Formation). Soil data from trenches and sonic drilling indicate (1) elevated concentrations of several constituents in the silt zone, likely due to the formation of evaporites, (2) uranium is the only measured element that appears to be concentrated in the silt over the groundwater contaminant plume, (3) in the former tailings impoundment area, there may be a thin unsaturated zone with elevated uranium in the native material just below the fill, (4) in the former tailings impoundment area, slightly higher uranium concentrations occur in the underlying saturated sand and gravel, and (5) several bedrock samples have a unique geochemical signature, generally related to a higher silt content. Assessment of groundwater flow included measuring river elevations along the Wind River and installing the temporary well points adjacent to the Little Wind River that provided additional data points to refine contours for water table elevations. These data confirm past interpretations of groundwater flow to the southeast across the site toward the Little Wind River. Hydraulic head elevations between paired surficial and semiconfined aquifer wells indicate variable vertical gradients across the site with the potential for upward and downward flow. Additional direct-push drilling and groundwater sampling confirmed the contaminant plume configuration, but it also revealed a low-sulfate-concentration zone at the edge of the former tailings impoundment. Temporary well points provided better definition of plume concentrations at the bank of the Little Wind River, and data from these wells indicate plume discharge to the river. Additional sampling in an area southwest of the plume that had elevated uranium groundwater concentrations in the past did not have any uranium concentrations above the U.S. Environmental Protection Agency maximum concentration limit for uranium. Results from multilevel monitoring wells indicate some geochemical differences with depth, but overall concentrations are similar to those in nearby conventional monitoring wells in the long-term monitoring program. Geochemistry data from these multilevel monitoring wells confirm the general increase in contaminant concentrations toward the river and toward the plume centerline for chloride, sulfate, and uranium but highlight geochemical controls on calcium. Iron data indicate slightly reducing conditions, especially near water table and bedrock surfaces, with more oxidizing conditions in the middle of the sand and gravel. Uranium activity ratios (234U/238U) confirm the uranium plume in the surficial aquifer as being mill related, and the area to the southwest outside the plume as natural, non-mill related. In the semiconfined aquifer, evidence of aquifer connection and impacts from the mill is inconclusive. Values of δD and δ 18O suggest water is derived from different sources and tritium data confirm that the semiconfined aquifer water is generally older than the surficial aquifer water. However, these data do indicate some groundwater communication from the surficial aquifer into the semiconfined aquifer, which resulted in δD and δ 18O and tritium values in the semiconfined aquifer that are more similar to those in the surficial aquifer. Values of δ 34S sulfate in the semiconfined aquifer combined with sulfate concentrations indicate the potential for some mill- related sulfate in the semiconfined aquifer, albeit limited to an area near and beneath the former tailings impoundment. Uranium and molybdenum concentrations in the semiconfined aquifer are below groundwater standards in all wells. However, the elevated molybdenum concentrations at one semiconfined aquifer well underneath the former tailings impoundment suggests a mill- derived source for the uranium and molybdenum in that well. It is possible that aquifer cross- communication occurred when the tailings impoundment was active and created a higher head. Current cross-communication appears unlikely given the large differences in tritium values and an upward hydraulic head at this location. Nine domestic wells are located within the institutional control boundary (eight in the confined aquifer and one in the semiconfined aquifer). Uranium and molybdenum concentrations in all samples collected from these wells were one or two orders of magnitude below the groundwater standards. Surface water flow in the Little Wind River in September 2015 was low compared to historical averages for that time of year. As a result, the uranium concentration measured in the Little Wind River was at a historical maximum at the sampling location upstream of the site. However, the impact of uranium discharge from the groundwater plume into the Little Wind River was not measureable. Elevated sulfate concentrations were observed in an outfall ditch related to an active sulfuric acid plant. Uranium concentrations in the oxbow lake remain at concentrations above the groundwater standard. Plume contaminant concentrations had returned to levels found prior to the 2010 flood by the end of 2015. However, these concentrations still exceed model predictions for natural flushing, and the current data indicate that natural flushing to achieve remediation goals within the 100-year time period is not likely, especially with the high potential for additional floods in the update to the conceptual site model (CSM), soil data indicate additional contaminant sources, specifically uranium, in evaporites within the silt layer over the uranium plume and in naturally reduced zones (NRZs). Additional zones of slightly elevated uranium concentration are in the native sediments just above the water table but below the fill layer in the former tailings impoundment area. This area also has slightly elevated uranium in the sand and gravel below the water table. Mass balance calculations indicate that small amounts of dissolution in any of these zones with increased uranium in the solid phase can produce groundwater uranium concentrations above the groundwater standard and could account for the post-flood uranium spike. The additional uranium near the former tailings impoundment provides a mechanism for a continuing source for the uranium plume that was not considered in earlier natural flushing models. In addition, uranium released from the silt layer or the NRZs seasonally and during flooding may add uranium to the groundwater plume near the Little Wind River. These mechanisms provide a possible explanation for plume persistence, along with spikes in concentrations during floods, that creates the current plume configuration. Additional updates to the CSM include (1) chloride flushes more rapidly than uranium beneath the former mill site, (2) chloride in the silt layer provides a scenario in which chloride cannot be used as a conservative tracer (especially in areas prone to flooding), (3) uranium concentrations with depth can be variable (especially below NRZs), and (4) calcite and gypsum solubility limits appear to provide important geochemical controls on groundwater geochemistry. The conclusion of this study provides several recommendations for additional work to refine the CSM and continue assessment of the natural flushing compliance strategy. Recommendations for additional work include targeted soil and groundwater sampling to assess geochemical conditions, distribution of contaminants, and groundwater/surface water interaction; additional column tests to provide data for geochemical modeling; and development of an updated groundwater flow model, which will be used in conjunction with a geochemical model to assess the viability of the natural flushing compliance strategy.« less

  20. Uranium ores and depleted uranium in the environment, with a reference to uranium in the biosphere from the Erzgebirge/Sachsen, Germany.

    PubMed

    Meinrath, A; Schneider, P; Meinrath, G

    2003-01-01

    The Erzgebirge ('Ore Mountains') area in the eastern part of Germany was a major source of uranium for Soviet nuclear programs between 1945 and 1989. During this time, the former German Democratic Republic became the third largest uranium producer in the world. The high abundance of uranium in the geological formations of the Erzgebirge are mirrored in the discovery of uranium by M. Klaproth close to Freiberg City in 1789 and the description of the so-called 'Schneeberg' disease, lung cancer caused in miners by the accumulation of the uranium decay product, radon, in the subsurfaces of shafts. Since 1991, remediation and mitigation of uranium at production facilities, rock piles and mill tailings has taken place. In parallel, efforts were initiated to assess the likely adverse effects of uranium mining to humans. The costs of these activities amount to about 6.5 10(9) Euro. A comparison with concentrations of depleted uranium at certain sites is given.

  1. BLENDING LOW ENRICHED URANIUM WITH DEPLETED URANIUM TO CREATE A SOURCE MATERIAL ORE THAT CAN BE PROCESSED FOR THE RECOVERY OF YELLOWCAKE AT A CONVENTIONAL URANIUM MILL

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Schutt, Stephen M.; Hochstein, Ron F.; Frydenlund, David C.

    2003-02-27

    Throughout the United States Department of Energy (DOE) complex, there are a number of streams of low enriched uranium (LEU) that contain various trace contaminants. These surplus nuclear materials require processing in order to meet commercial fuel cycle specifications. To date, they have not been designated as waste for disposal at the DOE's Nevada Test Site (NTS). Currently, with no commercial outlet available, the DOE is evaluating treatment and disposal as the ultimate disposition path for these materials. This paper will describe an innovative program that will provide a solution to DOE that will allow disposition of these materials atmore » a cost that will be competitive with treatment and disposal at the NTS, while at the same time recycling the material to recover a valuable energy resource (yellowcake) for reintroduction into the commercial nuclear fuel cycle. International Uranium (USA) Corporation (IUSA) and Nuclear Fuel Services, Inc. (NFS) have entered into a commercial relationship to pursue the development of this program. The program involves the design of a process and construction of a plant at NFS' site in Erwin, Tennessee, for the blending of contaminated LEU with depleted uranium (DU) to produce a uranium source material ore (USM Ore{trademark}). The USM Ore{trademark} will then be further processed at IUC's White Mesa Mill, located near Blanding, Utah, to produce conventional yellowcake, which can be delivered to conversion facilities, in the same manner as yellowcake that is produced from natural ores or other alternate feed materials. The primary source of feed for the business will be the significant sources of trace contaminated materials within the DOE complex. NFS has developed a dry blending process (DRYSM Process) to blend the surplus LEU material with DU at its Part 70 licensed facility, to produce USM Ore{trademark} with a U235 content within the range of U235 concentrations for source material. By reducing the U235 content to source material levels in this manner, the material will be suitable for processing at a conventional uranium mill under its existing Part 40 license to remove contaminants and enable the product to re-enter the commercial fuel cycle. The tailings from processing the USM Ore{trademark} at the mill will be permanently disposed of in the mill's tailings impoundment as 11e.(2) byproduct material. Blending LEU with DU to make a uranium source material ore that can be returned to the nuclear fuel cycle for processing to produce yellowcake, has never been accomplished before. This program will allow DOE to disposition its surplus LEU and DU in a cost effective manner, and at the same time provide for the recovery of valuable energy resources that would be lost through processing and disposal of the materials. This paper will discuss the nature of the surplus LEU and DU materials, the manner in which the LEU will be blended with DU to form a uranium source material ore, and the legal means by which this blending can be accomplished at a facility licensed under 10 CFR Part 70 to produce ore that can be processed at a conventional uranium mill licensed under 10 CFR Part 40.« less

  2. Microbial biogeochemistry of uranium mill tailings

    USGS Publications Warehouse

    Landa, Edward R.

    2005-01-01

    Uranium mill tailings (UMT) are the crushed ore residues from the extraction of uranium (U) from ores. Among the radioactive wastes associated with the nuclear fuel cycle, UMT are unique in terms of their volume and their limited isolation from the surficial environment. For this latter reason, their management and long-term fate has many interfaces with environmental microbial communities and processes. The interactions of microorganisms with UMT have been shown to be diverse and with significant consequences for radionuclide mobility and bioremediation. These radionuclides are associated with the U-decay series. The addition of organic carbon and phosphate is required to initiate the reduction of the U present in the groundwater down gradient of the mills. Investigations on sediment and water from the U-contaminated aquifer, indicates that the addition of a carbon source stimulates the rate of U removal by microbial reduction. Moreover, most attention with respect to passive or engineered removal of U from groundwaters focuses on iron-reducing and sulfate-reducing bacteria.

  3. Baseline risk assessment of ground water contamination at the uranium mill tailings site near Durango, Colorado. Revision 1

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    NONE

    1995-09-01

    For the UMTRA Project site located near Durango, Colorado (the Durango site), the Surface Project cleanup occurred from 1986 to 1991. An evaluation was made to determine whether exposure to ground water contaminated by uranium processing could affect people`s health. Exposure could occur from drinking water pumped from a hypothetical well drilled in the contaminated ground water area. In addition, environmental risks may result if plants or animals are exposed to contaminated ground water, or surface water that has mixed with contaminated ground water. This risk assessment report is the first site-specific document prepared for the UMTRA Ground Water Projectmore » at the Durango site. The results of this report and further site characterization of the Durango site will be used to determine what is necessary to protect public health and the environment, and to comply with the EPA standards.« less

  4. Wildlife mitigation and monitoring report Gunnison, Colorado, site

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    NONE

    1997-04-01

    The Uranium Mill Tailings Remedial Action (UMTRA) Project is administered by the U.S. Department of Energy (DOE); its purpose is to cleanup uranium mill tailings and other contaminated material at 24 UMTRA Project sites in 10 states. This report summarizes the wildlife mitigation and monitoring program under way at the Gunnison UMTRA Project, Gunnison, Colorado. Remedial action at the Gunnison site was completed in December 1995 and is described in detail in the Gunnison completion report. The impacts of this activity were analyzed in the Gunnison environmental assessment (EA). These impacts included two important game species: the pronghorn antelope (Antilocapramore » americans) and sage grouse (Wentrocerus urophasianus). Haul truck traffic was predicted to limit antelope access to water sources north of the Tenderfoot Mountain haul road and that truck traffic along this and other haul roads could result in antelope road kills. Clearing land at the disposal cell, haul road and borrow site activities, and the associated human activities also were predicted to negatively impact (directly and indirectly) sage grouse breeding, nesting, loafing, and wintering habitat. As a result, an extensive mitigation and monitoring plan began in 1992. Most of the monitoring studies are complete and the results of these studies, written by different authors, appear in numerous reports. This report will: (1) Analyze existing impacts and compare them to predicted impacts. (2) Summarize mitigation measures. (3) Summarize all existing monitoring data in one report. (4) Analyze the effectiveness of the mitigation measures.« less

  5. Health and Environmental Protection Standards for Uranium and Thorium Mill Tailings (40 CFR Part 192)

    EPA Pesticide Factsheets

    This regulation sets standards for the protection of public health, safety, and the environment from radiological and non-radiological hazards from uranium and thorium ore processing and disposal of associated wastes.

  6. Results of the independent verification of radiological remedial action at 87 East 500 South Street, Monticello, Utah (MS00153)

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Wilson, M.J.; Crutcher, J.W.

    1991-07-01

    In 1980 the iste of a vanadium and uranium mill at Monticello, Utah, was accepted into the US Department of Energy's (DOE's) Surplus Facilities Management Program, with the objectives of restoring the government-owned mill site to safe levels of radioactivity, disposing of or containing the tailings in an environmentally safe manner, and performing remedial actions on off-site (vicinity) properties that had been contaminated by radioactive material resulting from mill operations. During 1987 and 1988, UNC Geotech, the remedial action contractor designated by DOE, performed remedial action on the vicinity property at 87 East 500 South Street, Monticello, Utah. The Pollutantmore » Assessments Group (PAG) of Oak Ridge National Laboratory was assigned the responsibility of verifying the data supporting the adequacy of remedial action and confirming the site's compliance with DOE guidelines. The PAG found that the site successfully meets the DOE remedial action objectives. Procedures used by PAG are described. 3 refs., 2 tabs.« less

  7. Environmental radioactivity assessment around old uranium mining sites near Mangualde (Viseu), Portugal

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Carvalho, Fernando P.; Torres, Lubelia M.; Oliveira, Joao M.

    2007-07-01

    Uranium ore was extracted in the surroundings of Mangualde city, North of Portugal, in the mines of Cunha Baixa, Quinta do Bispo and Espinho until a few years ago. Mining waste, milling tailings and acid mine waters are the on site remains of this extractive activity. Environmental radioactivity measurements were performed in and around these sites in order to assess the dispersal of radionuclides from uranium mining waste and the spread of acidic waters resulting from the in situ uranium leaching with sulphuric acid. Results show migration of acid waters into groundwater around the Cunha Baixa mine. This groundwater ismore » tapped by irrigation wells in the agriculture area near the Cunha Baixa village. Water from wells displayed uranium ({sup 238}U) concentrations up to 19x10{sup 3} mBq L{sup -1} and sulphate ion concentrations up to 1070 mg L{sup -1}. These enhanced concentrations are positively correlated with low water pH, pointing to a common origin for radioactivity, dissolved sulphate, and acidity in underground mining works. Radionuclide concentrations were determined in horticulture and farm products from this area also and results suggest low soil to plant transfer of radionuclides and low food chain transfer of radionuclides to man. Analysis of aerosols in surface air showed re suspension of dust from mining and milling waste heaps. Therefore, it is recommended to maintain mine water treatment and to plan remediation of these mine sites in order to prevent waste dispersal in the environment. (authors)« less

  8. Summary of ground-water quality impacts of uranium mining and milling in the Grants mineral belt, New Mexico. Technical note (final)

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Kaufmann, R.F.; Eadie, G.G.; Russell, C.R.

    Ground-water contamination from uranium mining and milling results from the infiltration of radium-bearing mine, mill, and ion-exchange plant effluents. Radium, selenium, and nitrate were of most value as indicators of contamination. In recent years, mining has increased radium in mine effluents from several picocuries/liter (pCi/1) or less, to 100-150 pCi/1. The shallow aquifer in use in the vicinity of one mill was grossly contaminated with selenium, attributable to the mill tailings. Seepage from two other mill tailings ponds averaged 67,400,000 liters/year and, to date, has contributed an estimated 1.1 curies of radium to ground water. At one of these, anmore » injection well was used to dispose of over 3,400,000,000 liters of waste from 1960-1973. The wastes have not been properly monitored and have apparently migrated to more shallow, potable aquifers. No adverse impacts on municipal water quality in Paguate, Bluewater, Grants, Milan, and Gallup were observed. (GRA)« less

  9. Screening of bacterial strains isolated from uranium mill tailings porewaters for bioremediation purposes.

    PubMed

    Sánchez-Castro, Iván; Amador-García, Ahinara; Moreno-Romero, Cristina; López-Fernández, Margarita; Phrommavanh, Vannapha; Nos, Jeremy; Descostes, Michael; Merroun, Mohamed L

    2017-01-01

    The present work characterizes at different levels a number of bacterial strains isolated from porewaters sampled in the vicinity of two French uranium tailing repositories. The 16S rRNA gene from 33 bacterial isolates, corresponding to the different morphotypes recovered, was almost fully sequenced. The resulting sequences belonged to 13 bacterial genera comprised in the phyla Firmicutes, Actinobacteria and Proteobacteria. Further characterization at physiological level and metals/metalloid tolerance provided evidences for an appropriate selection of bacterial strains potentially useful for immobilization of uranium and other common contaminants. By using High Resolution Transmission Electron Microscope (HRTEM), this potential ability to immobilize uranium as U phosphate mineral phases was confirmed for the bacterial strains Br3 and Br5 corresponding to Arthrobacter sp. and Microbacterium oxydans, respectively. Scanning Transmission Electron Microscope- High-Angle Annular Dark-Field (STEM-HAADF) analysis showed U accumulates on the surface and within bacterial cytoplasm, in addition to the extracellular space. Energy Dispersive X-ray (EDX) element-distribution maps demonstrated the presence of U and P within these accumulates. These results indicate the potential of certain bacterial strains isolated from porewaters of U mill tailings for immobilizing uranium, likely as uranium phosphates. Some of these bacterial isolates might be considered as promising candidates in the design of uranium bioremediation strategies. Copyright © 2016 Elsevier Ltd. All rights reserved.

  10. Environmental assessment of remedial action at the Gunnison Uranium Mill Tailings Site near Gunnison, Colorado. Final

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1992-02-01

    The presence of contaminated uranium mill tailings adjacent to the city of Gunnison has been a local concern for many years. The following issues were identified during public meetings that were held by the DOE prior to distribution of an earlier version of this EA. Many of these issues will require mitigation. Groundwater contamination; in December 1989, a herd of 105 antelope were introduced in an area that includes the Landfill disposal site. There is concern that remedial action-related traffic in the area would result in antelope mortality. The proposed Tenderfoot Mountain haul road may restrict antelope access to theirmore » water supply; a second wildlife issue concerns the potential reduction in sage grouse use of breeding grounds (leks) and nesting habitat; the proposed Tenderfoot Mountain haul road would cross areas designated as wetlands by US Army Corps of Engineers (COE); the proposed disposal site is currently used for grazing by cattle six weeks a year in the spring. Additional concerns were stated in comments on a previous version of this EA. The proposed action is to consolidate and remove all contaminated materials associated with the Gunnison processing site to the Landfill disposal site six air miles east of Gunnison. All structures on the site (e.g., water tower, office buildings) were demolished in 1991. The debris is being stored on the site until it can be incorporated into the disposal cell at the disposal site. All contaminated materials would be trucked to the Landfill disposal site on a to-be-constructed haul road that crosses BLM-administered land.« less

  11. 40 CFR Table A to Subpart D of... - Table A to Subpart D of Part 192

    Code of Federal Regulations, 2013 CFR

    2013-07-01

    ...) RADIATION PROTECTION PROGRAMS HEALTH AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Standards for Management of Uranium Byproduct Materials Pursuant to Section 84 of the Atomic... Combined radium-226 and radium-228 5 Gross alpha-particle activity (excluding radon and uranium) 15 ...

  12. 40 CFR Table A to Subpart D of... - Table A to Subpart D of Part 192

    Code of Federal Regulations, 2014 CFR

    2014-07-01

    ...) RADIATION PROTECTION PROGRAMS HEALTH AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Standards for Management of Uranium Byproduct Materials Pursuant to Section 84 of the Atomic... Combined radium-226 and radium-228 5 Gross alpha-particle activity (excluding radon and uranium) 15 ...

  13. US Department of Energy Grand Junction Projects Office Remedial Action Project. Final report of the decontamination and decommissioning of Building 52 at the Grand Junction Projects Office Facility

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Krabacher, J.E.

    1996-08-01

    The U.S. Department of Energy (DOE) Grand Junction Projects Office (GJPO) occupies a 61.7-acre facility along the Gunnison River near Grand Junction, Colorado. This site was contaminated with uranium ore and mill tailings during uranium refining activities of the Manhattan Engineer District and during pilot milling experiments conducted for the U.S. Atomic Energy Commission`s domestic uranium procurement program. The DOE Defense Decontamination and Decommissioning Program established the GJPO Remedial Action Project to clean up and restore the facility lands, improvements, and the underlying aquifer. The site contractor for the facility, Rust Geotech, also was the remedial action contractor. Building 52more » was found to be radiologically contaminated and was demolished in 1994. The soil area within the footprint of the building has been remediated in accordance with the identified standards and the area can be released for unlimited exposure and unrestricted use. This document was prepared in response to a DOE request for an individual final report for each contaminated GJPO building.« less

  14. Final report of the decontamination and decommission of Building 31 at the Grand Junction Projects Office Facility

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Krabacher, J.E.

    1996-07-01

    The U.S. Department of Energy (DOE) Grand Junction Projects Office (GJPO) occupies a 61.7-acre facility along the Gunnison River near Grand Junction, Colorado. This site was contaminated with uranium ore and mill tailings during uranium refining activities of the Manhattan Engineer District and during pilot milling experiments conducted for the domestic uranium procurement program funded by the U.S. Atomic Energy Commission. The DOE Defense Decontamination and Decommissioning Program established the GJPO Remedial Action Project to clean up and restore the facility lands, improvements, and the underlying aquifer. The site contractor for the facility, Rust Geotech, also was the remedial actionmore » contractor. Radiological contamination was identified in Building 31 and the building was demolished in 1992. The soil area within the footprint of the building has been remediated in accordance with the identified standards and the area can be released for unlimited exposure and unrestricted use. This area was addressed in the summary final report of the remediation of the exterior areas of the GJPO facility. This document was prepared in response to a DOE request for an individual final report for each contaminated GJPO building.« less

  15. Synchrotron X-ray characterization of mackinawite and uraninite relevant to bio-remediation of groundwater contaminated with uranium

    NASA Astrophysics Data System (ADS)

    Carpenter, J.; Hyun, S.; Hayes, K. F.

    2010-12-01

    Uranium (U) originating from mining operations for weapon manufacturing and nuclear energy production is a significant radionuclide contaminant in groundwater local to uranium mining, uranium milling, and uranium mill tailing (UMT) storage sites. In the USA, the Department of Energy (DOE) is currently overseeing approximately 24 Uranium Mill Tailing Remediation Action (UMTRA) sites which have collectively processed over 27 million tons of uranium ore1,2. In-Situ microbial bio-reduction of the highly mobile U6+ ion into the dramatically less mobile U4+ ion has been demonstrated as an effective remedial process to inhibit uranium migration in the aqueous phase3. The resistance of this process to oxidization and possible remobilization of U when bioremediation stops (and oxidants such as oxygen from the air or nitrate in water diffuse into the formation) in the long term is not known. UMTRA site studies3 have shown that iron sulfide solids are produced by sulfate reducing bacteria (SRB) during U bioremediation, and some forms of these iron sulfide solids are known to be effective oxidant scavengers, potentially protecting against re-oxidation and thus remobilization of U. This work is investigating the role of iron sulfide solids in the long-term immobilization of reduced U compounds after bioremediation is completed in groundwater local to UMTRA sites. Re-oxidation tests are being performed in packed media columns loaded with both FeS and U solids. High quality mackinawite (FeS), and uraninite (UO2) have been synthesized in our laboratory via a wet chemistry approach. These synthetic materials are expected to mimic the naturally occurring and biogenic materials present in biologically stimulated UMTRA sites. In order to establish the initial conditions of the prepared experimental columns and to compare synthetic and biogenic FeS and UO2, these synthesized materials have been characterized with synchrotron radiation at the Stanford Synchrotron Radiation Lightsource using synchrotron x-ray powder diffraction (SXRD) and extended x-ray absorption fine structure (EXAFS). SXRD data were collected and analyzed with profile fitting to determine lattice parameters and crystallite size for comparison with published values for both biogenic and synthetic materials. This is particularly of interest for UO2, as there is very little information on particle size and lattice parameters for synthetic UO2 in the literature. Profile fitting of the SXRD data for FeS gives lattice parameters of a = b = 3.668 and a mean crystallite size of 5 to 8 nm. Both of these values are in good agreement with published values. For fresh UO2, lattice parameters were determined as a = b = c = 5.4 nm for both freshly synthesized and aged (3 months) UO2 and particle size was determined to be 3.5 nm for fresh UO2 and 5.83 nm for aged UO2. This suggests a growth mechanism for crystallites over time, and an inferred decrease in reactivity.

  16. Design, permitting, and construction issues associated with closure of the Panna Maria uranium tailings impoundment

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Strachan, C.L.; Raabe, K.L.

    1997-12-31

    In 1992, Panna Maria Uranium Operations (PMUO) initiated licensing and engineering activities for closure of the Panna Maria mill and 150-acre tailings impoundment located in southeast Texas. Closure of the tailings impoundment is permitted by license amendment through the Texas Natural Resources Conservation Commission (TNRCC), and based on closure criteria outlined in Texas regulations. The closure plan for the Panna Maria tailings impoundment was submitted for Texas regulatory agency review in April 1993, with details of the closure plan modified in 1994, 1995, and 1996. The closure plan included a multi-layered cover over the regraded tailings surface which was designedmore » for long-term isolation of tailings, reduction of radon emanation to regulated levels, and reduction of infiltration to TNRCC-accepted levels. The cover and embankment slope surfaces and surrounding areas were designed to provide acceptable erosional stability as compared to runoff velocities from the Probable Maximum Precipitation event. Cover materials were selected from on-site materials and evaluated for suitability based on permeability, radon attenuation, and soil dispersivity characteristics. Off-site materials were used when necessary. The cover over the tailings has a maximum slope of 0.5 percent, and the regraded embankment slopes outside the perimeter of the impoundment have a maximum slope of 20 percent. All reclaimed slopes are covered with topsoil and revegetated. A riprap-lined channel is to be used to convey runoff from within the perimeter of the reclaimed impoundment to the north of the impoundment.« less

  17. Reconnaissance soil geochemistry at the Riverton Uranium Mill Tailings Remedial Action Site, Fremont County, Wyoming

    USGS Publications Warehouse

    Smith, David B.; Sweat, Michael J.

    2012-01-01

    Soil samples were collected and chemically analyzed from the Riverton Uranium Mill Tailings Remedial Action Site, which lies within the Wind River Indian Reservation in Fremont County, Wyoming. Nineteen soil samples from a depth of 0 to 5 centimeters were collected in August 2011 from the site. The samples were sieved to less than 2 millimeters and analyzed for 44 major and trace elements following a near-total multi-acid extraction. Soil pH was also determined. The geochemical data were compared to a background dataset consisting of 160 soil samples previously collected from the same depth throughout the State of Wyoming as part of another ongoing study by the U.S. Geological Survey. Risk from potentially toxic elements in soil from the site to biologic receptors and humans was estimated by comparing the concentration of these elements with soil screening values established by the U.S. Environmental Protection Agency. All 19 samples exceeded the carcinogenic human health screening level for arsenic in residential soils of 0.39 milligrams per kilogram (mg/kg), which represents a one-in-one-million cancer risk (median arsenic concentration in the study area is 2.7 mg/kg). All 19 samples also exceeded the lead and vanadium screening levels for birds. Eighteen of the 19 samples exceeded the manganese screening level for plants, 13 of the 19 samples exceeded the antimony screening level for mammals, and 10 of 19 samples exceeded the zinc screening level for birds. However, these exceedances are also found in soils at most locations in the Wyoming Statewide soil database, and elevated concentrations alone are not necessarily cause for alarm. Uranium and thorium, two other elements of environmental concern, are elevated in soils at the site as compared to the Wyoming dataset, but no human or ecological soil screening levels have been established for these elements.

  18. Results of the independent verification of radiological remedial action at 600 South Clayhill Drive (AKA 600 South Cemetery Road), Monticello, Utah (MS00145)

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Wilson, M.J.; Crutcher, J.W.

    1991-07-01

    In 1980 the site of a vanadium and uranium mill at Monticello, Utah, was accepted into the US Department of Energy's (DOE's) Surplus Facilities Management Program, with the objectives of restoring the government-owned mill site to safe levels of radioactivity, disposing of or containing the tailings in an environmentally safe manner, and performing remedial actions on off-site (vicinity) properties that had been contaminated by radioactive material resulting from mill operations. During 1986 and 1987, UNC Geotech, the remedial action contractor designated by DOE, performed remedial action on the vicinity property at 600 South Cemetery Road (updated by San Juan Countymore » and the state of Utah to 600 South Clayhill Drive), Monticello, Utah. The Pollutant Assessments Group (PAG) of Oak Ridge National Laboratory was assigned the responsibility of verifying the data supporting the adequacy of remedial action and confirming the site's compliance with DOE guidelines. The PAG found that the site successfully meets the DOE remedial action objectives. Procedures used by PAG are described. 3 refs., 2 tabs.« less

  19. A Multifaceted Sampling Approach to Better Understanding Biogeochemical and Hydrogeological Controls on Uranium Mobility at a Former Uranium Mill Tailings Site in Riverton, Wyoming

    NASA Astrophysics Data System (ADS)

    Dam, W. L.; Johnson, R. H.; Campbell, S.; Bone, S. E.; Noel, V.; Bargar, J.

    2015-12-01

    Understanding uranium mobility in subsurface environments is not trivial. Obtaining sufficient data to accurately represent soil and aquifer characteristics can require unique approaches that evolve with added site knowledge. At Riverton, the primary source of uranium mill tailings remaining from ore processing was removed but contaminant plumes have persisted longer than predicted by groundwater modeling. What are the primary mechanisms controlling plume persistence? DOE is conducting new characterization studies to assist our understanding of underlying biogeochemical and hydrogeological mechanisms affecting secondary sources. A variety of field sampling techniques are being sequentially employed including augering, trenching, pore water sampling, and installing multi-level wells. In August 2012, vadose zone soil samples from 34 locations and groundwater from 103 boreholes were collected with Geoprobe ® direct push rods. Lower than expected uranium concentrations in composited shallow soils indicated the need for more focused and deeper samples. In May 2014, soil samples containing evaporites were collected along the bank of the Little Wind River; elevated uranium concentrations in evaporite minerals correlated with plume configurations and reflect contaminated groundwater discharge at the river. In September 2014, hand anger samples collected by the river and oxbow lake also indicated the presence of organic rich zones containing elevated uranium (>50 mg/kg). Subsequent samples collected from five backhoe trenches in May 2015 revealed a highly heterogeneous vadose zone composed of clay, silt, sand and cobbles containing evaporites and organic rich zones which may interact with groundwater plumes.Plans for August 2015 include sonic drilling to obtain continuous cores from the surface down to the base of the surficial aquifer with multi-level monitoring wells constructed in each borehole to assess vertical variation in groundwater chemistry. Temporary well-points will be installed adjacent to the river to assess geochemical and flow controls in the area of plume stagnation. Analyses include critical element speciation (C, S, Fe, and U), microbes, isotopes, diffusivity and flow characteristics. These activities support a dramatically improved understanding of plume persistence.

  20. Post Audit of a Field Scale Reactive Transport Model of Uranium at a Former Mill Site

    NASA Astrophysics Data System (ADS)

    Curtis, G. P.

    2015-12-01

    Reactive transport of hexavalent uranium (U(VI)) in a shallow alluvial aquifer at a former uranium mill tailings site near Naturita CO has been monitored for nearly 30 years by the US Department of Energy and the US Geological Survey. Groundwater at the site has high concentrations of chloride, alkalinity and U(VI) as a owing to ore processing at the site from 1941 to 1974. We previously calibrated a multicomponent reactive transport model to data collected at the site from 1986 to 2001. A two dimensional nonreactive transport model used a uniform hydraulic conductivity which was estimated from observed chloride concentrations and tritium helium age dates. A reactive transport model for the 2km long site was developed by including an equilibrium U(VI) surface complexation model calibrated to laboratory data and calcite equilibrium. The calibrated model reproduced both nonreactive tracers as well as the observed U(VI), pH and alkalinity. Forward simulations for the period 2002-2015 conducted with the calibrated model predict significantly faster natural attenuation of U(VI) concentrations than has been observed by the persistent high U(VI) concentrations at the site. Alternative modeling approaches are being evaluating evaluated using recent data to determine if the persistence can be explained by multirate mass transfer models developed from experimental observations at the column scale(~0.2m), the laboratory tank scale (~2m), the field tracer test scale (~1-4m) or geophysical observation scale (~1-5m). Results of this comparison should provide insight into the persistence of U(VI) plumes and improved management options.

  1. U.S. Geological Survey research in radioactive waste disposal - Fiscal years 1986-1990

    USGS Publications Warehouse

    Trask, N.J.; Stevens, P.R.

    1991-01-01

    The report summarizes progress on geologic and hydrologic research related to the disposal of radioactive wastes. The research efforts are categorized according to whether they are related most directly to: (1) high-level wastes, (2) transuranic wastes, (3) low-level and mixed low-level and hazardous wastes, or (4) uranium mill tailings. Included is research applicable to the identification and geohydrologic characterization of waste-disposal sites, to investigations of specific sites where wastes have been stored, to development of techniques and methods for characterizing disposal sites, and to studies of geologic and hydrologic processes related to the transport and/or retention of waste radionuclides.

  2. Department of Energy PEIS scoping session

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Badar, L

    1992-12-10

    This is the second programmatic environmental impact statement scoping session held in Durango, Colorado. The purpose was: to present the ground water program so as to build some familiarity and understanding about the issue involved; and to get Durango community's input. Scoping is the collection of information and getting everyone involved and really making a team out of coming up with a proposed action. This report contains the presentations made by the project manager for the Uranium Mill Tailings (UMTRA) program, site manager for the Durango UMTRA site, manager of ground water hydrology, and include comments made by local residents.

  3. Remediation strategy, capping construction and ongoing monitoring for the mill tailings pond, Ningyo-Toge uranium mine, Japan

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Hiroshi Saito; Tomihiro Taki

    2013-07-01

    Ningyo-toge Uranium Mine is subject to the environmental remediation. The main purposes are to take measures to ensure the radiation protection from the exposure pathways to humans in future, and to prevent the occurrence of mining pollution. The Yotsugi Mill Tailings Pond in the Ningyo-toge Uranium Mine has deposited mining waste and impounded water as a buffer reservoir before it is transferred to the Water Treatment Facility. It is located at the upstream of the water-source river and as the impact on its environment in case of earthquake is estimated significant, the highest priority has been put to it amongmore » mine-related facilities in the Mine. So far, basic concept has been examined and a great number of data has been acquired, and using the data, some remediation activities have already done, including capping construction for the upstream part of the Mill Tailings Pond. The capping is to reduce rainwater penetration to lower the burden of water treatment, and to reduce radon exhalation and dose rates. Only natural materials are used to alleviate the future maintenance. Data, including settlement amount and underground temperature is now being acquired and accumulated to verify the effectiveness of the capping, and used for the future remediation of the Downstream with revision of its specifications if necessary. (authors)« less

  4. An overview of Pennsylvania`s experience with NORM

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Yusko, J.G.

    1997-02-01

    Although Pennsylvania may be thought of as the state who brought you indoor radon, courtesy of a discovery of a residence with radon concentrations in excess of a few thousand picocuries per liter, this is not the states only claim to NORM fame. In the early years of the twentieth century, Pennsylvania was the largest producer of radium, utilizing its industrial base to produce large quantities of this {open_quotes}miracle cure{close_quotes} from ores mined in the West, and transported to a separation and purification facility in Western Pennsylvania. The company successfully held off foreign and political pressure, and generated large quantitiesmore » of uranium tailings as well, until a fire one New Year`s Eve destroyed the separation plant, and the company faded from view. The tailings were remediated as part of the Uranium Mill Tailings, Remedial Action Project, on the only site east of the Mississippi River. This article goes on to discuss the states experiences with NORM in various projects, coming in contact with human populations from different sources.« less

  5. DOE Office of Scientific and Technical Information (OSTI.GOV)

    Szescody, James E.; Moore, Robert C.; Rigali, Mark J.

    The Old Rifle Site is a former vanadium and uranium ore-processing facility located adjacent to the Colorado River and approximately 0.3 miles east of the city of Rifle, CO. The former processing facilities have been removed and the site uranium mill tailings are interned at a disposal cell north of the city of Rifle. However, some low level remnant uranium contamination still exists at the Old Rifle site. In 2002, the United States Nuclear Regulatory Commission (US NRC) concurred with United States Department of Energy (US DOE) on a groundwater compliance strategy of natural flushing with institutional controls to decreasemore » contaminant concentrations in the aquifer. In addition to active monitoring of contaminant concentrations, the site is also used for DOE Legacy Management (LM) and other DOE-funded small-scale field tests of remediation technologies. The purpose of this laboratory scale study was to evaluate the effectiveness of a hydroxyapatite (Ca 10(PO 4) 6(OH) 2) permeable reactive barrier and source area treatment in Old Rifle sediments. Phosphate treatment impact was evaluated by comparing uranium leaching and surface phase changes in untreated to PO 4-treated sediments. The impact of the amount of phosphate precipitation in the sediment on uranium mobility was evaluated with three different phosphate loadings. A range of flow velocity and uranium concentration conditions (i.e., uranium flux through the phosphate-treated sediment) was also evaluated to quantify the uranium uptake mass and rate by the phosphate precipitate.« less

  6. 40 CFR 61.226 - Reconsideration of rescission and reinstatement of this subpart.

    Code of Federal Regulations, 2010 CFR

    2010-07-01

    ... Emission Standards for Radon Emissions From the Disposal of Uranium Mill Tailings § 61.226 Reconsideration... by EPA and NRC or the tailings closure plan (radon) (i.e., contained in the license) requirements establishing milestones for the purpose of emplacing a permanent radon barrier that will achieve compliance...

  7. 40 CFR 61.226 - Reconsideration of rescission and reinstatement of this subpart.

    Code of Federal Regulations, 2011 CFR

    2011-07-01

    ... Emission Standards for Radon Emissions From the Disposal of Uranium Mill Tailings § 61.226 Reconsideration... by EPA and NRC or the tailings closure plan (radon) (i.e., contained in the license) requirements establishing milestones for the purpose of emplacing a permanent radon barrier that will achieve compliance...

  8. Geochemical hosts of solubilized radionuclides in uranium mill tailings

    USGS Publications Warehouse

    Landa, E.R.; Bush, C.A.

    1990-01-01

    The solubilization and subsequent resorption of radionuclides by ore components or by reaction products during the milling of uranium ores may have both economic and environmental consequences. Particle-size redistribution of radium during milling has been demonstrated by previous investigators; however, the identification of sorbing components in the tailings has received little experimental attention. In this study, uranium-bearing sandstone ore was milled, on a laboratory scale, with sulfuric acid. At regular intervals, filtrate from this suspension was placed in contact with mixtures of quartz sand and various potential sorbents which occur as gangue in uranium ores; the potential sorbents included clay minerals, iron and aluminum oxides, feldspar, fluorspar, barite, jarosite, coal, and volcanic glass. After equilibration, the quartz sand-sorbent mixtures were separated from the filtrate and radioassayed by gamma-spectrometry to determine the quantities of 238U, 230Th, 226Ra, and 210Pb sorbed, and the radon emanation coefficients. Sorption of 238U was low in all cases, with maximal sorptions of 1-2% by the bentonite- and coal-bearing samples. 230Th sorption also was generally less than 1%; maximal sorption here was observed in the fluorspar-bearing sample and appears to be associated with the formation of gypsum during milling. 226Ra and 210 Pb generally showed higher sorption than the other nuclides - more than 60% of the 26Ra solubilized from the ore was sorbed on the barite-bearing sample. The mechanism (s) for this sorption by a wide variety of substrates is not yet understood. Radon emanation coefficients of the samples ranged from about 5 to 30%, with the coal-bearing samples clearly demonstrating an emanating power higher than any of the other materials. ?? 1990.

  9. 1997 Monitoring report for the Gunnison, Colorado Wetlands Mitigation Plan

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    NONE

    1997-11-01

    Under the Uranium Mill Tailings Remedial Action (UMTRA) Project, the U.S. Department of Energy (DOE) cleaned up uranium mill tailings and other surface contamination near the town of Gunnison, Colorado. Remedial action resulted in the elimination of 4.3 acres (ac) (1.7 hectares [ha]) of wetlands. This loss is mitigated by the enhancement of six spring-fed areas on Bureau of Land Management (BLM) land (mitigation sites). Approximately 254 ac (1 03.3 ha) were fenced at the six sites to exclude grazing livestock. Of the 254 ac (103.3 ha), 17.8 ac (7.2 ha) are riparian plant communities; the rest are sagebrush communities.more » Baseline grazed conditions of the riparian plant communities at the mitigation sites were measured prior to fencing. This report discusses results of the fourth year of a monitoring program implemented to document the response of vegetation and wildlife to the exclusion of livestock. Three criteria for determining success of the mitigation were established: plant height, vegetation density (bare ground), and vegetation diversity. By 1996, Prospector Spring, Upper Long`s Gulch, and Camp Kettle met the criteria. The DOE requested transfer of these sites to BLM for long-term oversight. The 1997 evaluation of the three remaining sites, discussed in this report, showed two sites (Houston Gulch and Lower Long`s Gulch) meet the criteria. The DOE will request the transfer of these two sites to the BLM for long-term oversight. The last remaining site, Sage Hen Spring, has met only two of the criteria (percent bare ground and plant height). The third criterion, vegetation diversity, was not met. The vegetation appears to be changing from predominantly wet species to drier upland species, although the reason for this change is uncertain. It may be due to below-normal precipitation in recent years, diversion of water from the spring to the stock tank, or manipulation of the hydrology farther up gradient.« less

  10. Evaluation of impacts and mitigation assessments for the UMTRA Project: Gunnison and Durango pilot studies. Final report

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Beranich, S.J.

    1994-08-24

    This report evaluates the impacts assessment and proposed mitigations provided in environmental documents concerning the US Department of Energy`s (DOE) Uranium Mill Tailings Remedial Action (UMTRA) Project. The projected impacts and proposed mitigations identified in UMTRA Project environmental documents were evaluated for two UMTRA Project sites. These sites are Gunnison and Durango, which are representative of currently active and inactive UMTRA Project sites, respectively. National Environmental Policy Act (NEPA) documentation was prepared for the remedial action at Durango and Gunnison as well as for the provision of an alternate water supply system at Gunnison. Additionally, environmental analysis was completed formore » mill site demolition Gunnison, and for a new road related to the Durango remedial action. The results in this report pertain only to the impact assessments prepared by the Regulatory Compliance staff as a part of the NEPA compliance requirements. Similarly, the mitigative measures documented are those that were identified during the NEPA process.« less

  11. Column Testing and 1D Reactive Transport Modeling to Evaluate Uranium Plume Persistence Processes

    NASA Astrophysics Data System (ADS)

    Johnson, R. H.; Morrison, S.; Morris, S.; Tigar, A.; Dam, W. L.; Dayvault, J.

    2015-12-01

    At many U.S. Department of Energy Office of Legacy Management sites, 100 year natural flushing was selected as a remedial option for groundwater uranium plumes. However, current data indicate that natural flushing is not occurring as quickly as expected and solid-phase and aqueous uranium concentrations are persistent. At the Grand Junction, Colorado office site, column testing was completed on core collected below an area where uranium mill tailings have been removed. The total uranium concentration in this core was 13.2 mg/kg and the column was flushed with laboratory-created water with no uranium and chemistry similar to the nearby Gunnison River. The core was flushed for a total of 91 pore volumes producing a maximum effluent uranium concentration of 6,110 μg/L at 2.1 pore volumes and a minimum uranium concentration of 36.2 μg/L at the final pore volume. These results indicate complex geochemical reactions at small pore volumes and a long tailing affect at greater pore volumes. Stop flow data indicate the occurrence of non-equilibrium processes that create uranium concentration rebound. These data confirm the potential for plume persistence, which is occurring at the field scale. 1D reactive transport modeling was completed using PHREEQC (geochemical model) and calibrated to the column test data manually and using PEST (inverse modeling calibration routine). Processes of sorption, dual porosity with diffusion, mineral dissolution, dispersion, and cation exchange were evaluated separately and in combination. The calibration results indicate that sorption and dual porosity are major processes in explaining the column test data. These processes are also supported by fission track photographs that show solid-phase uranium residing in less mobile pore spaces. These procedures provide valuable information on plume persistence and secondary source processes that may be used to better inform and evaluate remedial strategies, including natural flushing.

  12. Data Validation Package: April 2016 Groundwater Sampling at the Falls City, Texas, Disposal Site

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Jasso, Tashina; Widdop, Michael

    Nine groundwater samples were collected at the Falls City, Texas, Disposal Site as specified in the March 2008 Long-Term Surveillance Plan for the US Department of Energy Falls City Uranium Mill Tailings Disposal Site, Falls City, Texas (DOE-LM/1602-2008). Sampling and analyses were conducted as specified in the Sampling and Analysis Plan for US Department of Energy Office of Legacy Management Sites (LMS/PRO/S04351, continually updated). The wells sampled included the cell performance monitoring wells (0709, 0858, 0880, 0906, and 0921) and the groundwater monitoring wells (0862, 0886, 0891, 0924, and 0963). A duplicate sample was collected from location 0891. Water levelsmore » were measured at each sampled well. Historically, cell performance monitoring wells 0908 and 0916 have not produced water and were confirmed as dry during this sampling event. These wells are completed above the saturated interval in the formation. Notable observations for time-concentration graphs in this report include: (1) uranium concentrations in well 0891 continue to increase; (2) the uranium concentration in well 0880 is higher than the 2015 value and lower than the 2014 value, and it remains within the range of historical values; and (3) uranium concentrations in the other sampled wells are below 2 mg/L and consistent with previous results.« less

  13. 10 CFR Appendix A to Part 40 - Criteria Relating to the Operation of Uranium Mills and the Disposition of Tailings or Wastes...

    Code of Federal Regulations, 2011 CFR

    2011-01-01

    ... to be relied upon for seepage control, tests must be conducted with representative tailings solutions... licensee shall control, minimize, or eliminate post-closure escape of nonradiological hazardous... beyond the control of the licensee. The phrase permits consideration of the cost of compliance only to...

  14. 10 CFR Appendix A to Part 40 - Criteria Relating to the Operation of Uranium Mills and the Disposition of Tailings or Wastes...

    Code of Federal Regulations, 2010 CFR

    2010-01-01

    ... to be relied upon for seepage control, tests must be conducted with representative tailings solutions... itself. (6) The design requirements in this criterion for longevity and control of radon releases apply... licensee shall control, minimize, or eliminate post-closure escape of nonradiological hazardous...

  15. Innovative mathematical modeling in environmental remediation.

    PubMed

    Yeh, Gour-Tsyh; Gwo, Jin-Ping; Siegel, Malcolm D; Li, Ming-Hsu; Fang, Yilin; Zhang, Fan; Luo, Wensui; Yabusaki, Steve B

    2013-05-01

    There are two different ways to model reactive transport: ad hoc and innovative reaction-based approaches. The former, such as the Kd simplification of adsorption, has been widely employed by practitioners, while the latter has been mainly used in scientific communities for elucidating mechanisms of biogeochemical transport processes. It is believed that innovative mechanistic-based models could serve as protocols for environmental remediation as well. This paper reviews the development of a mechanistically coupled fluid flow, thermal transport, hydrologic transport, and reactive biogeochemical model and example-applications to environmental remediation problems. Theoretical bases are sufficiently described. Four example problems previously carried out are used to demonstrate how numerical experimentation can be used to evaluate the feasibility of different remediation approaches. The first one involved the application of a 56-species uranium tailing problem to the Melton Branch Subwatershed at Oak Ridge National Laboratory (ORNL) using the parallel version of the model. Simulations were made to demonstrate the potential mobilization of uranium and other chelating agents in the proposed waste disposal site. The second problem simulated laboratory-scale system to investigate the role of natural attenuation in potential off-site migration of uranium from uranium mill tailings after restoration. It showed inadequacy of using a single Kd even for a homogeneous medium. The third example simulated laboratory experiments involving extremely high concentrations of uranium, technetium, aluminum, nitrate, and toxic metals (e.g., Ni, Cr, Co). The fourth example modeled microbially-mediated immobilization of uranium in an unconfined aquifer using acetate amendment in a field-scale experiment. The purposes of these modeling studies were to simulate various mechanisms of mobilization and immobilization of radioactive wastes and to illustrate how to apply reactive transport models for environmental remediation. Copyright © 2011 Elsevier Ltd. All rights reserved.

  16. U.S. Geological Survey research in radioactive waste disposal - Fiscal years 1983, 1984, and 1985

    USGS Publications Warehouse

    Dinwiddie, G.A.; Trask, N.J.

    1986-01-01

    The report summarizes progress on geologic and hydrologic research related to the disposal of radioactive wastes. The research is described according to whether it is related most directly to: (1) high-level and transuranic wastes, (2) low-level wastes, or (3) uranium mill tailings. Included is research applicable to the identification and geohydrologic characterization of waste-disposal sites, to investigations of specific sites where wastes have been stored, and to studies of regions or environments where waste-disposal sites might be located. A significant part of the activity is concerned with techniques and methods for characterizing disposal sites and studies of geologic and hydrologic processes related to the transport and (or) retention of waste radionuclides.

  17. Assessment of the quality of groundwater and the Little Wind River in the area of a former uranium processing facility on the Wind River Reservation, Wyoming, 1987 through 2010

    USGS Publications Warehouse

    Ranalli, Anthony J.; Naftz, David L.

    2014-01-01

    In 2010, the U.S Geological Survey (USGS), in cooperation with the Wind River Environmental Quality Commission (WREQC), began an assessment of the effectiveness of the existing monitoring network at the Riverton, Wyoming, Uranium Mill Tailings Remedial Action (UMTRA) site. The USGS used existing data supplied by the U.S. Department of Energy (DOE). The study was to determine (1) seasonal variations in the direction of groundwater flow in the area of the former uranium processing facility toward the Little Wind River, (2) the extent of contaminated groundwater among the aquifers and between the aquifers and the Little Wind River, (3) whether current monitoring is adequate to establish the effectiveness of natural attenuation for the contaminants of concern, and (4) the influence of groundwater discharged from the sulfuric-acid plant on water quality in the Little Wind River.

  18. Guidance for implementing the long-term surveillance program for UMTRA Project Title I Disposal Sites

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    NONE

    1996-02-01

    This guidance document has two purposes: it provides guidance for writing site-specific long-term surveillance plans (LTSP) and it describes site surveillance, monitoring, and long-term care techniques for Title I disposal sites of the Uranium Mill Tailings Radiation Control Act (UMTRCA) (42 USC Section 7901 et seq.). Long-term care includes monitoring, maintenance, and emergency measures needed to protect public health and safety and the environment after remedial action is completed. This document applies to the UMTRCA-designated Title I disposal sites. The requirements for long-term care of the Title I sites and the contents of the LTSPs are provided in U.S. Nuclearmore » Regulatory Commission (NRC) regulations (10 CFR Section 40.27) provided in Attachment 1.« less

  19. Geology, geochemistry, and geophysics of the Fry Canyon uranium/copper project site, southeastern Utah - Indications of contaminant migration

    USGS Publications Warehouse

    Otton, James K.; Zielinski, Robert A.; Horton, Robert J.

    2010-01-01

    The Fry Canyon uranium/copper project site in San Juan County, southeastern Utah, was affected by the historical (1957-68) processing of uranium and copper-uranium ores. Relict uranium tailings and related ponds, and a large copper heap-leach pile at the site represent point sources of uranium and copper to local soils, surface water, and groundwater. This study was designed to establish the nature, extent, and pathways of contaminant dispersion. The methods used in this study are applicable at other sites of uranium mining, milling, or processing. The uranium tailings and associated ponds sit on a bench that is as much as 4.25 meters above the level of the adjacent modern channel of Fry Creek. The copper heap leach pile sits on bedrock just south of this bench. Contaminated groundwater from the ponds and other nearby sites moves downvalley and enters the modern alluvium of adjacent Fry Creek, its surface water, and also a broader, deeper paleochannel that underlies the modern creek channel and adjacent benches and stream terraces. The northern extent of contaminated groundwater is uncertain from geochemical data beyond an area of monitoring wells about 300 meters north of the site. Contaminated surface water extends to the State highway bridge. Some uranium-contaminated groundwater may also enter underlying bedrock of the Permian Cedar Mesa Sandstone along fracture zones. Four dc-resistivity surveys perpendicular to the valley trend were run across the channel and its adjacent stream terraces north of the heap-leach pile and ponds. Two surveys were done in a small field of monitoring wells and two in areas untested by borings to the north of the well field. Bedrock intercepts, salt distribution, and lithologic information from the wells and surface observations in the well field aided interpretation of the geophysical profiles there and allowed interpretation of the two profiles not tested by wells. The geophysical data for the two profiles to the north of the well field suggest that the paleochannel persists at least 900 m to the north of the heap leach and pond sites. Contamination of groundwater beneath the stream terraces may extend at least that far. Fry Creek surface water (six samples), seeps and springs (six samples), and wells (eight samples) were collected during a dry period of April 16-19, 2007. The most uranium-rich (18.7 milligrams per liter) well water on the site displays distinctive Ca-Mg-SO4-dominant chemistry indicating the legacy of heap leaching copper-uranium ores with sulfuric acid. This same water has strongly negative d34S of sulfate (-13.3 per mil) compared to most local waters of -2.4 to -5.4 per mil. Dissolved uranium species in all sampled waters are dominantly U(VI)-carbonate complexes. All waters are undersaturated with respect to U(VI) minerals. The average 234U/238U activity ratio (AR) in four well waters from the site (0.939 + or ? 0.011) is different from that of seven upstream waters (1.235 + or ? 0.069). This isotopic contrast permits quantitative estimates of mixing of site-derived uranium with natural uranium in waters collected downstream. At the time of sampling, uranium in downstream surface water was mostly (about 67 percent) site-derived and subject to further concentration by evaporation. Three monitoring wells located approximately 0.4 kilometer downstream contained dominantly (78-87 percent) site-derived uranium. Distinctive particles of chalcopyrite (CuFeS) and variably weathered pyrite (FeS2) are present in tailings at the stream edge on the site and are identified in stream sediments 1.3 kilometers downstream, based on inspection of polished grain mounts of magnetic mineral separates.

  20. Field analyses of (238)U and (226)Ra in two uranium mill tailings piles from Niger using portable HPGe detector.

    PubMed

    Déjeant, Adrien; Bourva, Ludovic; Sia, Radia; Galoisy, Laurence; Calas, Georges; Phrommavanh, Vannapha; Descostes, Michael

    2014-11-01

    The radioactivities of (238)U and (226)Ra in mill tailings from the U mines of COMINAK and SOMAÏR in Niger were measured and quantified using a portable High-Purity Germanium (HPGe) detector. The (238)U and (226)Ra activities were measured under field conditions on drilling cores with 600s measurements and without any sample preparation. Field results were compared with those obtained by Inductive Coupled Plasma Atomic Emission Spectroscopy (ICP-AES) and emanometry techniques. This comparison indicates that gamma-ray absorption by such geological samples does not cause significant deviations. This work shows the feasibility of using portable HPGe detector in the field as a preliminary method to observe variations of radionuclides concentration with the aim of identifying samples of interest. The HPGe is particularly useful for samples with strong secular disequilibrium such as mill tailings. Copyright © 2014 Elsevier Ltd. All rights reserved.

  1. 10 CFR 40.2a - Coverage of inactive tailings sites.

    Code of Federal Regulations, 2011 CFR

    2011-01-01

    ... materials as defined in this part that are located at a site where milling operations are no longer active... defined in this part that is located at a site where milling operations are no longer active, if such site... 10 Energy 1 2011-01-01 2011-01-01 false Coverage of inactive tailings sites. 40.2a Section 40.2a...

  2. 10 CFR 40.2a - Coverage of inactive tailings sites.

    Code of Federal Regulations, 2012 CFR

    2012-01-01

    ... materials as defined in this part that are located at a site where milling operations are no longer active... defined in this part that is located at a site where milling operations are no longer active, if such site... 10 Energy 1 2012-01-01 2012-01-01 false Coverage of inactive tailings sites. 40.2a Section 40.2a...

  3. 10 CFR 40.2a - Coverage of inactive tailings sites.

    Code of Federal Regulations, 2014 CFR

    2014-01-01

    ... materials as defined in this part that are located at a site where milling operations are no longer active... defined in this part that is located at a site where milling operations are no longer active, if such site... 10 Energy 1 2014-01-01 2014-01-01 false Coverage of inactive tailings sites. 40.2a Section 40.2a...

  4. 10 CFR 40.2a - Coverage of inactive tailings sites.

    Code of Federal Regulations, 2013 CFR

    2013-01-01

    ... materials as defined in this part that are located at a site where milling operations are no longer active... defined in this part that is located at a site where milling operations are no longer active, if such site... 10 Energy 1 2013-01-01 2013-01-01 false Coverage of inactive tailings sites. 40.2a Section 40.2a...

  5. Lessons Learned from Radioactive Waste Storage and Disposal Facilities

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Esh, David W.; Bradford, Anna H.

    2008-01-15

    The safety of radioactive waste disposal facilities and the decommissioning of complex sites may be predicated on the performance of engineered and natural barriers. For assessing the safety of a waste disposal facility or a decommissioned site, a performance assessment or similar analysis is often completed. The analysis is typically based on a site conceptual model that is developed from site characterization information, observations, and, in many cases, expert judgment. Because waste disposal facilities are sited, constructed, monitored, and maintained, a fair amount of data has been generated at a variety of sites in a variety of natural systems. Thismore » paper provides select examples of lessons learned from the observations developed from the monitoring of various radioactive waste facilities (storage and disposal), and discusses the implications for modeling of future waste disposal facilities that are yet to be constructed or for the development of dose assessments for the release of decommissioning sites. Monitoring has been and continues to be performed at a variety of different facilities for the disposal of radioactive waste. These include facilities for the disposal of commercial low-level waste (LLW), reprocessing wastes, and uranium mill tailings. Many of the lessons learned and problems encountered provide a unique opportunity to improve future designs of waste disposal facilities, to improve dose modeling for decommissioning sites, and to be proactive in identifying future problems. Typically, an initial conceptual model was developed and the siting and design of the disposal facility was based on the conceptual model. After facility construction and operation, monitoring data was collected and evaluated. In many cases the monitoring data did not comport with the original site conceptual model, leading to additional investigation and changes to the site conceptual model and modifications to the design of the facility. The following cases are discussed: commercial LLW disposal facilities; uranium mill tailings disposal facilities; and reprocessing waste storage and disposal facilities. The observations developed from the monitoring and maintenance of waste disposal and storage facilities provide valuable lessons learned for the design and modeling of future waste disposal facilities and the decommissioning of complex sites.« less

  6. Transfer and Transition: Interagency Coordination for Managing Public Lands at UMTRCA Title II Sites in Wyoming – 16614

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Shafer, David S.; Vanek, Tim; Ribeiro, Tracy

    By the end of fiscal year 2025, the U.S. Department of Energy (DOE) Office of Legacy Management (LM) is anticipating adding 17 sites remediated under Title II of the Uranium Mill Tailings Radiation Control Act (UMTRCA) to the current inventory of 90 sites that it manages. Among the new sites are ones where federal public lands occur within the proposed long-term care boundary, the boundary determined by the Nuclear Regulatory Commission and LM as necessary to maintain site protectiveness for the entombed uranium mill tailings and residual groundwater contamination. For these sites, public land withdrawals for land and minerals willmore » need to be established. LM’s primary mission at UMTRCA sites is to protect the public and the environment from exposure to contamination at the sites. For the sites with public lands or federally controlled minerals that will be transferring to LM, the Office will apply to the Department of the Interior (DOI) Bureau of Land Management (BLM) for new, public land and mineral withdrawals. At most current LM UMTRCA sites that involved public lands and minerals, DOI granted DOE “full administrative jurisdiction” and permanent withdrawals. Hence, these withdrawals are, permanently, no longer subject to public land, mining, and mineral-leasing laws and regulations. LM is coordinating with DOI/BLM in Wyoming to permanently withdraw full and partial jurisdiction at future UMTRCA Title II sites in that state. This approach would allow LM to fully administer surface lands and minerals, where necessary, and DOI and LM to administer surface lands and leasable minerals where it would not jeopardize sites’ radiological safety and long-term public and environmental protection. This “shared-jurisdiction approach” will meet LM’s strategic goal of protecting human health and the environment but also allow BLM to fulfill their mission to “manage and conserve the lands under the mandate of multiple-use and sustained yield.” In addition, LM could also fulfill the fourth goal of its Strategic Plan, to optimize land use and assets.« less

  7. 40 CFR 192.22 - Supplemental standards.

    Code of Federal Regulations, 2013 CFR

    2013-07-01

    ... 40 Protection of Environment 26 2013-07-01 2013-07-01 false Supplemental standards. 192.22 Section 192.22 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) RADIATION PROTECTION PROGRAMS HEALTH AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Implementation...

  8. 40 CFR 192.22 - Supplemental standards.

    Code of Federal Regulations, 2012 CFR

    2012-07-01

    ... 40 Protection of Environment 26 2012-07-01 2011-07-01 true Supplemental standards. 192.22 Section 192.22 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) RADIATION PROTECTION PROGRAMS HEALTH AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Implementation...

  9. 40 CFR 192.22 - Supplemental standards.

    Code of Federal Regulations, 2014 CFR

    2014-07-01

    ... 40 Protection of Environment 25 2014-07-01 2014-07-01 false Supplemental standards. 192.22 Section 192.22 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) RADIATION PROTECTION PROGRAMS HEALTH AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Implementation...

  10. 40 CFR 192.22 - Supplemental standards.

    Code of Federal Regulations, 2010 CFR

    2010-07-01

    ... 40 Protection of Environment 24 2010-07-01 2010-07-01 false Supplemental standards. 192.22 Section 192.22 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) RADIATION PROTECTION PROGRAMS HEALTH AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Implementation...

  11. 40 CFR 192.22 - Supplemental standards.

    Code of Federal Regulations, 2011 CFR

    2011-07-01

    ... 40 Protection of Environment 25 2011-07-01 2011-07-01 false Supplemental standards. 192.22 Section 192.22 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) RADIATION PROTECTION PROGRAMS HEALTH AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Implementation...

  12. Evapotranspiration And Geochemical Controls On Groundwater Plumes At Arid Sites: Toward Innovative Alternate End-States For Uranium Processing And Tailings Facilities

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Looney, Brian B.; Denham, Miles E.; Eddy-Dilek, Carol A.

    2014-01-08

    Management of legacy tailings/waste and groundwater contamination are ongoing at the former uranium milling site in Tuba City AZ. The tailings have been consolidated and effectively isolated using an engineered cover system. For the existing groundwater plume, a system of recovery wells extracts contaminated groundwater for treatment using an advanced distillation process. The ten years of pump and treat (P&T) operations have had minimal impact on the contaminant plume – primarily due to geochemical and hydrological limits. A flow net analysis demonstrates that groundwater contamination beneath the former processing site flows in the uppermost portion of the aquifer and exitsmore » the groundwater as the plume transits into and beneath a lower terrace in the landscape. The evaluation indicates that contaminated water will not reach Moenkopi Wash, a locally important stream. Instead, shallow groundwater in arid settings such as Tuba City is transferred into the vadose zone and atmosphere via evaporation, transpiration and diffuse seepage. The dissolved constituents are projected to precipitate and accumulate as minerals such as calcite and gypsum in the deep vadose zone (near the capillary fringe), around the roots of phreatophyte plants, and near seeps. The natural hydrologic and geochemical controls common in arid environments such as Tuba City work together to limit the size of the groundwater plume, to naturally attenuate and detoxify groundwater contaminants, and to reduce risks to humans, livestock and the environment. The technical evaluation supports an alternative beneficial reuse (“brownfield”) scenario for Tuba City. This alternative approach would have low risks, similar to the current P&T scenario, but would eliminate the energy and expense associated with the active treatment and convert the former uranium processing site into a resource for future employment of local citizens and ongoing benefit to the Native American Nations.« less

  13. 76 FR 60941 - Policy Regarding Submittal of Amendments for Processing of Equivalent Feed at Licensed Uranium...

    Federal Register 2010, 2011, 2012, 2013, 2014

    2011-09-30

    ... State-licensed uranium recovery site, either conventional, heap leach, or in situ recovery. DATES... types of new uranium recovery facilities (conventional mills, heap leach facilities, and in situ... from the ground for processing at a mill. Rather, the ore is processed in-situ with the resulting...

  14. Superfund Record of Decision (EPA Region 9): Coalinga Asbestos Mine, Fresno County, CA. (Second remedial action), September 1990. Final report

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    The 557-acre Coalinga Asbestos Mine site, a former asbestos processing area and chromite mine, comprises part of the Johns Manville Coalinga Asbestos Mill site in western Fresno County, California. This rural mountainous area is used primarily for recreational purposes. From 1962 to 1974, asbestos ore from several local mines was processed and sorted onsite, and the resulting asbestos mill tailings were periodically bulldozed into an intermittent stream channel. Subsequently, from 1975 to 1977, a chromite milling operation was conducted onsite. Tailings were often washed downstream during periods of stream flow, and the resuspension of asbestos fibers from the tailings intomore » the air produced a significant inhalation hazard. As a result of these activities, approximately 450,000 cubic yards of mill tailings and asbestos ore remain onsite within a large tailing pile. In 1980 and 1987, State investigations indicated that the site was contributing a significant amount of asbestos into the surface water. The site will be remediated as two Operable Units (OU). The Record of Decision (ROD) addresses the remedial action for OU2, the Johns Manville Coalinga Asbestos Mill Area. The primary contaminant of concern affecting the surface water is asbestos.« less

  15. 40 CFR 192.10 - Applicability.

    Code of Federal Regulations, 2010 CFR

    2010-07-01

    ... 40 Protection of Environment 24 2010-07-01 2010-07-01 false Applicability. 192.10 Section 192.10 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) RADIATION PROTECTION PROGRAMS HEALTH AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Standards for Cleanup of...

  16. 40 CFR 192.43 - Effective date.

    Code of Federal Regulations, 2010 CFR

    2010-07-01

    ... 40 Protection of Environment 24 2010-07-01 2010-07-01 false Effective date. 192.43 Section 192.43 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) RADIATION PROTECTION PROGRAMS HEALTH AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Standards for Management...

  17. 40 CFR 192.42 - Substitute provisions.

    Code of Federal Regulations, 2010 CFR

    2010-07-01

    ... 40 Protection of Environment 24 2010-07-01 2010-07-01 false Substitute provisions. 192.42 Section 192.42 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) RADIATION PROTECTION PROGRAMS HEALTH AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Standards for...

  18. 40 CFR 192.34 - Effective date.

    Code of Federal Regulations, 2010 CFR

    2010-07-01

    ... 40 Protection of Environment 24 2010-07-01 2010-07-01 false Effective date. 192.34 Section 192.34 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) RADIATION PROTECTION PROGRAMS HEALTH AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Standards for Management...

  19. 40 CFR 61.252 - Standard.

    Code of Federal Regulations, 2010 CFR

    2010-07-01

    ... uranium mill tailings pile shall not exceed 20 pCi/(m2-sec) (1.9 pCi/(ft2-sec)) of radon-222. (b) After... piles, the exemption for existing piles in 40 CFR 192.32(a) notwithstanding. [54 FR 51703, Dec. 15, 1989...

  20. 40 CFR 192.04 - Corrective action.

    Code of Federal Regulations, 2014 CFR

    2014-07-01

    ... 40 Protection of Environment 25 2014-07-01 2014-07-01 false Corrective action. 192.04 Section 192.04 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) RADIATION PROTECTION PROGRAMS HEALTH AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Standards for...

  1. 40 CFR 192.03 - Monitoring.

    Code of Federal Regulations, 2014 CFR

    2014-07-01

    ... 40 Protection of Environment 25 2014-07-01 2014-07-01 false Monitoring. 192.03 Section 192.03 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) RADIATION PROTECTION PROGRAMS HEALTH AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Standards for the Control...

  2. 40 CFR 192.00 - Applicability.

    Code of Federal Regulations, 2014 CFR

    2014-07-01

    ... 40 Protection of Environment 25 2014-07-01 2014-07-01 false Applicability. 192.00 Section 192.00 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) RADIATION PROTECTION PROGRAMS HEALTH AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Standards for the Control...

  3. Long-term surveillance plan for the Bodo Canyon Disposal Site, Durango, Colorado. Revision 1

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    NONE

    1995-11-01

    This long-term surveillance plan (LTSP) for the Uranium Mill Tailings Remedial Act on (UMTRA) Project Bodo Canyon disposal site at Durango, Colorado, describes the surveillance activities for the disposal site. The US Department of Energy (DOE) will carry out these activities to ensure that the disposal call continues to function as designed This LTSP was prepared as a requirement for DOE acceptance under the US Nuclear Regulatory Commission (NRC) general license for custody and long-term care of residual radioactive materials (RRM) from processing uranium ore. This LTSP documents that the land and interests are owned by the United States andmore » details how long-term care of the disposal site will be carried out. It is based on the DOE`s Guidance for Implementing the UMTRA Project Long-term Surveillance Program (DOE, 1992a). Following the introduction, contents of this report include the following: site final condition; site drawings and photographs; permanent site surveillance features; ground water monitoring; annual site inspections; unscheduled inspections; custodial maintenance; corrective action; record keeping and reporting requirements; emergency notification and reporting; quality assurance; personal health and safety; list of contributions; and references.« less

  4. Radon emanation from backfilled mill tailings in underground uranium mine.

    PubMed

    Sahu, Patitapaban; Mishra, Devi Prasad; Panigrahi, Durga Charan; Jha, Vivekananda; Patnaik, R Lokeswara; Sethy, Narendra Kumar

    2014-04-01

    Coarser mill tailings used as backfill to stabilize the stoped out areas in underground uranium mines is a potential source of radon contamination. This paper presents the quantitative assessment of radon emanation from the backfilled tailings in Jaduguda mine, India using a cylindrical accumulator. Some of the important parameters such as (226)Ra activity concentration, bulk density, bulk porosity, moisture content and radon emanation factor of the tailings affecting radon emanation were determined in the laboratory. The study revealed that the radon emanation rate of the tailings varied in the range of 0.12-7.03 Bq m(-2) s(-1) with geometric mean of 1.01 Bq m(-2) s(-1) and geometric standard deviation of 3.39. An increase in radon emanation rate was noticed up to a moisture saturation of 0.09 in the tailings, after which the emanation rate gradually started declining with saturation due to low diffusion coefficient of radon in the saturated tailings. Radon emanation factor of the tailings varied in the range of 0.08-0.23 with the mean value of 0.21. The emanation factor of the tailings with moisture saturation level over 0.09 was found to be about three times higher than that of the absolutely dry tailings. The empirical relationship obtained between (222)Rn emanation rate and (226)Ra activity concentration of the tailings indicated a significant positive linear correlation (r = 0.95, p < 0.001). This relationship may be useful for quick prediction of radon emanation rate from the backfill material of similar nature. Copyright © 2014 Elsevier Ltd. All rights reserved.

  5. 43 CFR 3832.34 - How may I use my mill site?

    Code of Federal Regulations, 2011 CFR

    2011-10-01

    ... MANAGEMENT, DEPARTMENT OF THE INTERIOR MINERALS MANAGEMENT (3000) LOCATING MINING CLAIMS OR SITES Mill Sites... plants and substations; (3) Tailings ponds and leach pads; (4) Rock and soil dumps; (5) Water and process... independent mill sites for processing metallic minerals from lode claims using: (1) Quartz or stamp mills; or...

  6. 43 CFR 3832.34 - How may I use my mill site?

    Code of Federal Regulations, 2013 CFR

    2013-10-01

    ... MANAGEMENT, DEPARTMENT OF THE INTERIOR MINERALS MANAGEMENT (3000) LOCATING MINING CLAIMS OR SITES Mill Sites... plants and substations; (3) Tailings ponds and leach pads; (4) Rock and soil dumps; (5) Water and process... independent mill sites for processing metallic minerals from lode claims using: (1) Quartz or stamp mills; or...

  7. 43 CFR 3832.34 - How may I use my mill site?

    Code of Federal Regulations, 2012 CFR

    2012-10-01

    ... MANAGEMENT, DEPARTMENT OF THE INTERIOR MINERALS MANAGEMENT (3000) LOCATING MINING CLAIMS OR SITES Mill Sites... plants and substations; (3) Tailings ponds and leach pads; (4) Rock and soil dumps; (5) Water and process... independent mill sites for processing metallic minerals from lode claims using: (1) Quartz or stamp mills; or...

  8. 40 CFR 192.33 - Corrective action programs.

    Code of Federal Regulations, 2010 CFR

    2010-07-01

    ... 40 Protection of Environment 24 2010-07-01 2010-07-01 false Corrective action programs. 192.33 Section 192.33 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) RADIATION PROTECTION PROGRAMS HEALTH AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Standards for...

  9. 40 CFR 192.23 - Effective date.

    Code of Federal Regulations, 2014 CFR

    2014-07-01

    ... 40 Protection of Environment 25 2014-07-01 2014-07-01 false Effective date. 192.23 Section 192.23 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) RADIATION PROTECTION PROGRAMS HEALTH AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Implementation § 192.23...

  10. 40 CFR 192.23 - Effective date.

    Code of Federal Regulations, 2011 CFR

    2011-07-01

    ... 40 Protection of Environment 25 2011-07-01 2011-07-01 false Effective date. 192.23 Section 192.23 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) RADIATION PROTECTION PROGRAMS HEALTH AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Implementation § 192.23...

  11. 40 CFR 192.23 - Effective date.

    Code of Federal Regulations, 2012 CFR

    2012-07-01

    ... 40 Protection of Environment 26 2012-07-01 2011-07-01 true Effective date. 192.23 Section 192.23 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) RADIATION PROTECTION PROGRAMS HEALTH AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Implementation § 192.23...

  12. 40 CFR 192.23 - Effective date.

    Code of Federal Regulations, 2013 CFR

    2013-07-01

    ... 40 Protection of Environment 26 2013-07-01 2013-07-01 false Effective date. 192.23 Section 192.23 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) RADIATION PROTECTION PROGRAMS HEALTH AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL TAILINGS Implementation § 192.23...

  13. Mineralogical controls on aluminum and magnesium in uranium mill tailings: Key Lake, Saskatchewan, Canada.

    PubMed

    Gomez, M A; Hendry, M J; Koshinsky, J; Essilfie-Dughan, J; Paikaray, S; Chen, J

    2013-07-16

    The mineralogy and evolution of Al and Mg in U mill tailings are poorly understood. Elemental analyses (ICP-MS) of both solid and aqueous phases show that precipitation of large masses of secondary Al and Mg mineral phases occurs throughout the raffinate neutralization process (pH 1-11) at the Key Lake U mill, Saskatchewan, Canada. Data from a suite of analytical methods (ICP-MS, EMPA, laboratory- and synchrotron-based XRD, ATR-IR, Raman, TEM, EDX, ED) and equilibrium thermodynamic modeling showed that nanoparticle-sized, spongy, porous, Mg-Al hydrotalcite is the dominant mineralogical control on Al and Mg in the neutralized raffinate (pH ≥ 6.7). The presence of this secondary Mg-Al hydrotalcite in mineral samples of both fresh and 15-year-old tailings indicates that the Mg-Al hydrotalcite is geochemically stable, even after >16 years in the oxic tailings body. Data shows an association between the Mg-Al hydrotalcite and both As and Ni and point to this Mg-Al hydrotalcite exerting a mineralogical control on the solubility of these contaminants.

  14. Historic mills and mill tailings as potential sources of contamination in and near the Humboldt River basin, northern Nevada. Chapter D.

    USGS Publications Warehouse

    Nash, J. Thomas; Stillings, Lisa L.

    2003-01-01

    Reconnaissance field studies of 40 mining districts in and near the Humboldt River basin have identified 83 mills and associated tailings impoundments and several other kinds of mineral-processing facilities (smelters, mercury retorts, heap-leach pads) related to historic mining. The majority of the mills and tailings sites are not recorded in the literature. All tailings impoundments show evidence of substantial amounts of erosion. At least 11 tailings dams were breached by flood waters, carrying fluvial tailings 1 to 15 km down canyons and across alluvial fans. Most of the tailings sites are dry most of the year, but some are near streams. Tailings that are wet for part of the year do not appear to be reacting significantly with those waters because physical factors such as clay layers and hard-pan cement appear to limit permeability and release of metals to surface waters. The major impact of mill tailings on surface- water quality may be brief flushes of runoff during storm events that carry acid and metals released from soluble mineral crusts. Small ephemeral ponds and puddles that tend to collect in trenches and low areas on tailings impoundments tend to be acidic and extremely enriched in metals, in part through cycles of evaporation. Ponded water that is rich in salts and metals could be acutely toxic to unsuspecting animals. Rare extreme storms have the potential to cause catastrophic failure of tailings impoundments, carry away metals in stormwaters, and transport tailings as debris flows for 1 to 15 km. In most situations these stormwaters and transported tailings could impact wildlife but probably would impact few or no people or domes-tic water wells. Because all identified historic tailings sites are several kilometers or more from the Humboldt River and major tributaries, tailings probably have no measurable impact on water quality in the main stem of the Humboldt River.

  15. Geochemistry of Mine Waste and Mill Tailings, Meadow Deposits, Streambed Sediment, and General Hydrology and Water Quality for the Frohner Meadows Area, Upper Lump Gulch, Jefferson County, Montana

    USGS Publications Warehouse

    Klein, Terry L.; Cannon, Michael R.; Fey, David L.

    2004-01-01

    Frohner Meadows, an area of low-topographic gradient subalpine ponds and wetlands in glaciated terrane near the headwaters of Lump Gulch (a tributary of Prickly Pear Creek), is located about 15 miles west of the town of Clancy, Montana, in the Helena National Forest. Mining and ore treatment of lead-zinc-silver veins in granitic rocks of the Boulder batholith over the last 120 years from two sites (Frohner mine and the Nellie Grant mine) has resulted in accumulations of mine waste and mill tailings that have been distributed downslope and downstream by anthropogenic and natural processes. This report presents the results of an investigation of the geochemistry of the wetlands, streams, and unconsolidated-sediment deposits and the hydrology, hydrogeology, and water quality of the area affected by these sources of ore-related metals. Ground water sampled from most shallow wells in the meadow system contained high concentrations of arsenic, exceeding the Montana numeric water-quality standard for human health. Transport of cadmium and zinc in ground water is indicated at one site near Nellie Grant Creek based on water-quality data from one well near the creek. Mill tailings deposited in upper Frohner Meadow contribute large arsenic loads to Frohner Meadows Creek; Nellie Grant Creek contributes large arsenic, cadmium, and zinc loads to upper Frohner Meadows. Concentrations of total-recoverable cadmium, copper, lead, and zinc in most surface-water sites downstream from the Nellie Grant mine area exceeded Montana aquatic-life standards. Nearly all samples of surface water and ground water had neutral to slightly alkaline pH values. Concentrations of arsenic, cadmium, lead, and zinc in streambed sediment in the entire meadow below the mine waste and mill tailings accumulations are highly enriched relative to regional watershed-background concentrations and exceed consensus-based, probable-effects concentrations for streambed sediment at most sites. Cadmium, copper, and zinc typically are adsorbed to the surface coatings of streambed-sediment grains. Mine waste and mill tailings contain high concentrations of arsenic, cadmium, copper, lead, and zinc in a quartz-rich matrix. Most of the waste sites that were sampled had low acid-generating capacity, although one site (fine-grained mill tailings from the Nellie Grant mine deposited in the upper part of lower Frohner Meadows) had extremely high acid-generating potential because of abundant fine-grained pyrite. Two distinct sites were identified as metal sources based on streambed-sediment samples, cores in the meadow substrate, and mine and mill-tailings samples. The Frohner mine and mill site contribute material rich in arsenic and lead; similar material from the Nellie Grant mine and mill site is rich in cadmium and zinc.

  16. Réduction des nitrates et de l'uranium par les bactéries indigènes

    NASA Astrophysics Data System (ADS)

    Abdelouas, Abdesselam; Lutze, Werner; Nuttall, Eric

    1998-07-01

    A bioremediation concept has been developed to clean up ground water contaminated with nitrate (1200 mg·L -1) and uranium (0.25 mg·L -1). We studied the Tuba City mill tailings site, Arizona, USA. Indigenous bacteria capable of catalyzing the reduction of NO 3- and U(VI) were identified in the ground water and in the host rock, the Navajo sandstone. After complete reduction of O 2 and NO 3- within one week, U(VI) was reduced and precipitated as uraninite. Final uranium concentrations < 15 μg·L -1 were reached after a few weeks at 24 °C. Iron sulfide also precipitated as a result of reduction of Fe(III) on the sand surface and sulfate in the ground water. U(VI) was not reduced by sulfide. It was found that enzymatic reduction of U(VI) is faster than abiotic reduction under the conditions given by the composition of the ground water.

  17. Long-term biobarriers to plant and animal intrusions of uranium tailings. [24% trifluralin, 18% carbon black, and 58% polymer

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Cline, J.F.; Burton, F.G.; Cataldo, D.A.

    1982-09-01

    The objective of this project was to develop and evaluate the effectiveness of physical and chemical barriers designed to prevent plant and animal breachment of uranium mill tailings containment systems for an extended period of time. A polymeric carrier/biocide delivery system was developed and tested in the laboratory, greenhouse and field. A continuous flow technique was established to determine the release rates of the biocides from the PCD systems; polymeric carrier specifications were established. Studies were conducted to determine effective biocide concentrations required to produce a phytotoxic response and the relative rates of phytotoxin degradation resulting from chemical and biologicalmore » breakdown in soils. The final PCD system developed was a pelletized system containing 24% trifluralin, 18% carbon black and 58% polymer. Pellets were placed in the soil at the Grand Junction U-tailings site at one in. and two in. intervals. Data obtained in the field determined that the pellets released enough herbicide to the soil layer to stop root elongation past the barrier. Physical barriers to subsurface movement of burrowing animals were investigated. Small crushed stone (1 to 1 1/2 in. diameter) placed over asphalt emulsion and multilayer soil seals proved effective as barriers to a small mammal (ground squirrels) but were not of sufficient size to stop a larger animal (the prairie dog). No penetrations were made through the asphalt emulsion or the clay layer of the multilayer soil seals by either of the two mammals tested. A literature survey was prepared and published on the burrowing habits of the animals that may be found at U-tailings sites.« less

  18. Phytoremediation of a nitrogen-contaminated desert soil by native shrubs and microbial processes

    DOE PAGES

    Glenn, Edward P.; Jordan, Fiona; Waugh, W. Joseph

    2016-02-24

    Here, we combined phytoremediation and soil microbial nitrification and denitrification cycles to reduce nitrate and ammonium levels at a former uranium mill site near Monument Valley, Arizona. Ammonia used in uranium extraction was present throughout the soil profile. Sulfate,applied as sulfuric acid to solubilize uranium, was also present in the soil. These contaminants were leaching from a denuded area where a tailings pile had been removed and were migrating away from the site in groundwater. We planted the source area with two deep-rooted native shrubs, Atriplex cansescens and Sarcobatus vermiculatus, and irrigated transplants for 11 years at 20% the ratemore » of potential evapotranspiration to stimulate growth, then discontinued irrigation for 4 years. Over 15 years, total nitrogen levels dropped 82%, from 347 to 64 mg kg –1. Analysis of δ 15N supported our hypothesis that coupled microbial nitrification and denitrification processes were responsible for the loss of N. Soil sulfate levels changed little; however, evapotranspiration reduced sulfate leaching into the aquifer. For arid sites where traditional pump-and-treat methods are problematic, the Monument Valley data suggest that alternatives that incorporate native plants and rely on vadose zone biogeochemistry and hydrology could be a sustainable remediation for nitrogen contaminated soil.« less

  19. Phytoremediation of a nitrogen-contaminated desert soil by native shrubs and microbial processes

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Glenn, Edward P.; Jordan, Fiona; Waugh, W. Joseph

    Here, we combined phytoremediation and soil microbial nitrification and denitrification cycles to reduce nitrate and ammonium levels at a former uranium mill site near Monument Valley, Arizona. Ammonia used in uranium extraction was present throughout the soil profile. Sulfate,applied as sulfuric acid to solubilize uranium, was also present in the soil. These contaminants were leaching from a denuded area where a tailings pile had been removed and were migrating away from the site in groundwater. We planted the source area with two deep-rooted native shrubs, Atriplex cansescens and Sarcobatus vermiculatus, and irrigated transplants for 11 years at 20% the ratemore » of potential evapotranspiration to stimulate growth, then discontinued irrigation for 4 years. Over 15 years, total nitrogen levels dropped 82%, from 347 to 64 mg kg –1. Analysis of δ 15N supported our hypothesis that coupled microbial nitrification and denitrification processes were responsible for the loss of N. Soil sulfate levels changed little; however, evapotranspiration reduced sulfate leaching into the aquifer. For arid sites where traditional pump-and-treat methods are problematic, the Monument Valley data suggest that alternatives that incorporate native plants and rely on vadose zone biogeochemistry and hydrology could be a sustainable remediation for nitrogen contaminated soil.« less

  20. UMTRA Project water sampling and analysis plan, Durango, Colorado. Revision 1

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    NONE

    1995-09-01

    Planned, routine ground water sampling activities at the US Department of Energy (DOE) Uranium Mill Tailings Remedial Action (UMTRA) Project site in Durango, Colorado, are described in this water sampling and analysis plan. The plan identifies and justifies the sampling locations, analytical parameters, detection limits, and sampling frequency for the routine monitoring stations at the site. The ground water data are used to characterize the site ground water compliance strategies and to monitor contaminants of potential concern identified in the baseline risk assessment (DOE, 1995a). Regulatory basis for routine ground water monitoring at UMTRA Project sites is derived from themore » US EPA regulations in 40 CFR Part 192 (1994) and EPA standards of 1995 (60 FR 2854). Sampling procedures are guided by the UMTRA Project standard operating procedures (SOP) (JEG, n.d.), the Technical Approach Document (TAD) (DOE, 1989), and the most effective technical approach for the site.« less

  1. 40 CFR 61.223 - Compliance procedures.

    Code of Federal Regulations, 2010 CFR

    2010-07-01

    ... completion of covering the pile to limit radon emissions but prior to the long term stabilization of the pile, the owners or operators of uranium mill tailings shall conduct testing for all piles within the... the following information: (1) The name and location of the facility. (2) A list of the piles at the...

  2. Bioremediation of Uranium-Contaminated Groundwater using Engineered Injection and Extraction

    NASA Astrophysics Data System (ADS)

    Greene, J. A.; Neupauer, R.; Ye, M.; Kasprzyk, J. R.; Mays, D. C.; Curtis, G. P.

    2017-12-01

    During in-situ remediation of contaminated groundwater, a treatment chemical is injected into the contaminated groundwater to react with and degrade the contaminant, with reactions occurring where the treatment chemical contacts the contaminant. Traditional in-situ groundwater remediation relies on background groundwater flow for spreading of treatment chemicals into contaminant plumes. Engineered Injection and Extraction (EIE), in which time-varying induced flow fields are used to actively spread the treatment chemical into the contaminant plume, has been developed to increase contact between the contaminant and treatment chemical, thereby enhancing contaminant degradation. EIE has been investigated for contaminants that degrade through irreversible bimolecular reaction with a treatment chemical, but has not been investigated for a contaminant governed by reversible reactions. Uranium primarily occurs in its aqueous, mobile form, U(VI), in the environment but can be bioreduced to its sparingly soluble, immobile form, U(IV), by iron reducing bacteria stimulated by an acetate amendment. In this study, we investigate the ability of EIE to facilitate and sustain favorable conditions to immobilize uranium during remediation, and to prevent re-mobilization of uranium into the aqueous phase after active remediation has ended. Simulations in this investigation are conducted using a semi-synthetic model based on physical and chemical conditions at the Naturita Uranium Mill Tailings Remedial Action (UMTRA) site in southwestern Colorado and the Old Rifle UMTRA site in western Colorado. The EIE design is optimized for the synthetic model using the Borg multi-objective evolutionary algorithm.

  3. Psychosocial and health impacts of uranium mining and milling on Navajo lands.

    PubMed

    Dawson, Susan E; Madsen, Gary E

    2011-11-01

    The uranium industry in the American Southwest has had profoundly negative impacts on American Indian communities. Navajo workers experienced significant health problems, including lung cancer and nonmalignant respiratory diseases, and psychosocial problems, such as depression and anxiety. There were four uranium processing mills and approximately 1,200 uranium mines on the Navajo Nation's over 27,000 square miles. In this paper, a chronology is presented of how uranium mining and milling impacted the lives of Navajo workers and their families. Local community leaders organized meetings across the reservation to inform workers and their families about the relationship between worker exposures and possible health problems. A reservation-wide effort resulted in activists working with political leaders and attorneys to write radiation compensation legislation, which was passed in 1990 as the Radiation Exposure Compensation Act (RECA) and included underground uranium miners, atomic downwinders, and nuclear test-site workers. Later efforts resulted in the inclusion of surface miners, ore truck haulers, and millworkers in the RECA Amendments of 2000. On the Navajo Nation, the Office of Navajo Uranium Workers was created to assist workers and their families to apply for RECA funds. Present issues concerning the Navajo and other uranium-impacted groups include those who worked in mining and milling after 1971 and are excluded from RECA. Perceptions about uranium health impacts have contributed recently to the Navajo people rejecting a resumption of uranium mining and milling on Navajo lands.

  4. Refining the site conceptual model at a former uranium mill site in Riverton, Wyoming, USA

    DOE PAGES

    Dam, William; Campbell, Sam; Johnson, Ray; ...

    2015-07-07

    Milling activities at a former uranium mill site near Riverton, Wyoming, USA, contaminated the shallow groundwater beneath and downgradient of the site. Although the mill operated for <6 years (1958-1963), its impact remains an environmental liability. Groundwater modeling predicted that contaminant concentrations were declining steadily, which confirmed the conceptual site model (CSM). However, local flooding in 2010 mobilized contaminants that migrated downgradient from the Riverton site and resulted in a dramatic increase in groundwater contaminant concentrations. This observation indicated that the original CSM was inadequate to explain site conditions and needed to be refined. In response to the new observationsmore » after the flood, a collaborative investigation to better understand site conditions and processes commenced. This investigation included installing 103 boreholes to collect soil and groundwater samples, sampling and analysis of evaporite minerals along the bank of the Little Wind River, an analysis of evaportranspiration in the shallow aquifer, and sampling naturally organic-rich sediments near groundwater discharge areas. The enhanced characterization revealed that the existing CSM did not account for high uranium concentrations in groundwater remaining on the former mill site and groundwater plume stagnation near the Little Wind River. Observations from the flood and subsequent investigations indicate that additional characterization is still needed to continue refining the CSM and determine the viability of the natural flushing compliance strategy. Additional sampling, analysis, and testing of soil and groundwater are necessary to investigate secondary contaminant sources, mobilization of contaminants during floods, geochemical processes, contaminant plume stagnation, distribution of evaporite minerals and organic-rich sediments, and mechanisms and rates of contaminant transfer from soil to groundwater. Future data collection will be used to continually revise the CSM and evaluate the compliance strategy at the site.« less

  5. Abandoned Rayrock uranium mill tailings in the Northwest Territories: Environmental conditions and radiological impact

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Veska, E.; Eaton, R.S.

    Field and laboratory investigations were undertaken of the environment surrounding abandoned U mill tailings at Rayrock, Northwest Territories, Canada, to examine the extent of 226Ra and U contamination. Samples of ground water, surface water, and unconsolidated geological material from the Rayrock area were collected for chemical and radiochemical analyses. Results indicated that the surface waters contained levels of 226Ra as high as 20 Bq L-1, 210Pb as high as 1.1 Bq L-1, and ground water U as high as 2800 micrograms L-1. Lower levels of 226Ra, 210Pb, and U, 3.6 Bq L-1, 0.5 Bq L-1, and 4 micrograms L-1, respectively,more » were found in a small lake adjacent to the tailings area. Analysis of tailings and soil in the immediate vicinity indicates that the radionuclides and U are mobilized and can move within the tailings. Some of the mobilized radionuclides will be bound by the surrounding peat. The remainder may move to Lake Alpha in ground water. Surface water flow also transports some contaminants both in the water of Alpha Creek and by washing tailings into Lake Alpha. The potential annual external and internal dose equivalents to a hypothetical resident were calculated based on exposure from the abandoned U mill tailings, drinking water, and fish caught in the lakes in the vicinity of the tailings. While Alpha Creek and Lake Alpha water showed evidence of contamination, the rest of the water system and the fish were at natural background levels of radioactivity.« less

  6. Long-term surveillance plan for the Green River, Utah, disposal site

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    NONE

    1997-06-01

    The long-term surveillance plan (LTSP) for the Green River, Utah, Uranium Mill Tailings Remedial Action (UMTRA) Project disposal site describes the surveillance activities for the Green River disposal cell. The U.S. Department of Energy (DOE) will carry out these activities to ensure that the disposal cell continues to function as designed. This final LTSP was prepared as a requirement for acceptance under the U.S. Nuclear Regulatory Commission (NRC) general license for custody and long-term care of residual radioactive materials (RRM). This LTSP documents whether the land and interests are owned by the United States or an Indian tribe and detailsmore » how the long-term care of the disposal site will be carried out. The Green River, Utah, LTSP is based on the DOE`s Guidance for Implementing the UMTRA Project Long-term Surveillance Program (DOE, 1992a).« less

  7. Radio-Ecological Conditions of Groundwater in the Area of Uranium Mining and Milling Facility - 13525

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Titov, A.V.; Semenova, M.P.; Seregin, V.A.

    2013-07-01

    Manmade chemical and radioactive contamination of groundwater is one of damaging effects of the uranium mining and milling facilities. Groundwater contamination is of special importance for the area of Priargun Production Mining and Chemical Association, JSC 'PPMCA', because groundwater is the only source of drinking water. The paper describes natural conditions of the site, provides information on changes of near-surface area since the beginning of the company, illustrates the main trends of contaminators migration and assesses manmade impact on the quality and mode of near-surface and ground waters. The paper also provides the results of chemical and radioactive measurements inmore » groundwater at various distances from the sources of manmade contamination to the drinking water supply areas. We show that development of deposits, mine water discharge, leakages from tailing dams and cinder storage facility changed general hydro-chemical balance of the area, contributed to new (overlaid) aureoles and flows of scattering paragenetic uranium elements, which are much smaller in comparison with natural ones. However, increasing flow of groundwater stream at the mouth of Sukhoi Urulyungui due to technological water infiltration, mixing of natural water with filtration streams from industrial reservoirs and sites, containing elevated (relative to natural background) levels of sulfate-, hydro-carbonate and carbonate- ions, led to the development and moving of the uranium contamination aureole from the undeveloped field 'Polevoye' to the water inlet area. The aureole front crossed the southern border of water inlet of drinking purpose. The qualitative composition of groundwater, especially in the southern part of water inlet, steadily changes for the worse. The current Russian intervention levels of gross alpha activity and of some natural radionuclides including {sup 222}Rn are in excess in drinking water; regulations for fluorine and manganese concentrations are also in excess. Possible ways to improve the situation are considered. (authors)« less

  8. Radium-226 whole-body gamma counting and 222Rn breath analysis: report on a subject exposed to uranium mill tailings.

    PubMed

    Lucas, H F

    1991-02-01

    One of two boys born in September 1949 who played on U mill tailings between age 8 and 12 was diagnosed as having leukemia at age 15.5. The exposed and control subjects were well matched; they were approximately the same age and both were 1.85 m (6' 1") in height and weighed 75.2 kg (165 pounds). The result obtained by gamma spectrometric method for the exposed subject was 0 +/- 17 Bq (0 +/- 470 pCi), while that for the control subject was 4 +/- 15 Bq (100 +/- 400 pCi). The result obtained by the Rn breath method for the exposed subject was 4.4 +/- 0.7 Bq (120 +/- 20 pCi), while that for the control was 5.4 +/- 1.4 Bq (150 +/- 38 pCi). These results suggest that the 226Ra body burden of the exposed subject is within the range of those observed in subjects exposed only through normal food sources, which have a mean 226Ra content of 1.5 Bq (range: 0.4-4.4 Bq) so that no significant mill-tailing intake is indicated. The best estimate of alpha particle dose to the red marrow from 226Ra and its decay products was 0.05 mGy at age 14 and 0.10 mGy at age 38. This dose, when compared to that observed in the dial painters, suggests that the leukemia was not caused by uptake of Ra from the mill tailings.

  9. Contribution of Uranium-Bearing Evaporites to Plume Persistence Issues at a Former Uranium Mill Site Riverton, Wyoming, USA

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Johnson, Raymond; Dam, William; Campbell, Sam

    2016-08-01

    • Evaporites occur in an unsaturated silt layer, which is underlain by a sand and gravel aquifer. • These evaporites are rich in chloride across the site. • Uranium concentrations are higher in the evaporites that overlie the uranium contaminant plume. • Flooding can solubilize the evaporites in the silt layer and release chloride, sulfate (not shown), and uranium into the underlyingsand and gravel aquifer. • The uranium-rich evaporites can delay natural flushing, creating plume persistence near the Little Wind River.

  10. Time-Series Radiocarbon Measurements Indicate Carbon Turnover Across Soil Fractions is Correlated With Productivity in a Long-Term Agricultural Experiment

    NASA Astrophysics Data System (ADS)

    Sanderman, J.; Baisden, W. T.; Creamer, C.; Farrell, M.; Fallon, S.

    2016-12-01

    Carbonatites and alkaline intrusions are important sources of REEs. Environmental risks related to these deposit types have been assessed through literature review and evaluation of the geochemical properties of representative samples of mill tailings and their leachates. The main ore mineral in carbonatite deposits is bastnasite [(Ce,La)(CO3)F], which is found with dolomite and calcite ( 65 %), barite (20 - 25 %), plus a number of minor accessory minerals including sulfides such as galena and pyrite. Generally, alkaline intrusion-related REE deposits either occur in layered complexes or with dikes and veins cutting alkaline intrusions. Such intrusions have a more diverse group of REE ore minerals that include fluorcarbonates, oxides, silicates, and phosphates. Ore also can include minor calcite and iron (Fe), lead (Pb), and zinc (Zn) sulfides. The acid-generating potential of both deposit types is low because of a predominance of carbonate minerals in the carbonatite deposits, the presence of feldspars and minor calcite in alkaline intrusion-related deposits, and to only minor to trace occurrence of potentially acid-generating sulfide minerals. Both deposit types, however, are produced by igneous and hydrothermal processes that enrich high-field strength, incompatible elements, which typically are excluded from common rock-forming minerals. Elements such as yttrium (Y), niobium Nb), zirconium (Zr), hafnium (Hf), tungsten (W), titanium (Ti), tantalum (Ta), scandium (Sc), thorium (Th), and uranium (U) can be characteristic of these deposits and may be of environmental concern. Most of these elements, including the REEs, but with the exception of U, have low solubilities in water at the near-neutral pH values expected around these deposits. Mill tailings from carbonatite deposits can exceed residential soil and sediment criteria for Pb, and leachates from mill tailings can exceed drinking water guidelines for Pb. The greatest environmental challenges, however, are linked to the presence of Th and U, although mineral hosts for these elements are moderately unreactive in the environment. Both deposit types can have mill tailings that exceed residential soil criteria for U. Uranium can be recovered as a byproduct to mitigate its environmental effects, but Th remains a waste product that requires management.

  11. Environmental Characteristics of Carbonatite and Alkaline Intrusion-related Rare Earth Element (REE) Deposits

    NASA Astrophysics Data System (ADS)

    Seal, R. R., II; Piatak, N. M.

    2017-12-01

    Carbonatites and alkaline intrusions are important sources of REEs. Environmental risks related to these deposit types have been assessed through literature review and evaluation of the geochemical properties of representative samples of mill tailings and their leachates. The main ore mineral in carbonatite deposits is bastnasite [(Ce,La)(CO3)F], which is found with dolomite and calcite ( 65 %), barite (20 - 25 %), plus a number of minor accessory minerals including sulfides such as galena and pyrite. Generally, alkaline intrusion-related REE deposits either occur in layered complexes or with dikes and veins cutting alkaline intrusions. Such intrusions have a more diverse group of REE ore minerals that include fluorcarbonates, oxides, silicates, and phosphates. Ore also can include minor calcite and iron (Fe), lead (Pb), and zinc (Zn) sulfides. The acid-generating potential of both deposit types is low because of a predominance of carbonate minerals in the carbonatite deposits, the presence of feldspars and minor calcite in alkaline intrusion-related deposits, and to only minor to trace occurrence of potentially acid-generating sulfide minerals. Both deposit types, however, are produced by igneous and hydrothermal processes that enrich high-field strength, incompatible elements, which typically are excluded from common rock-forming minerals. Elements such as yttrium (Y), niobium Nb), zirconium (Zr), hafnium (Hf), tungsten (W), titanium (Ti), tantalum (Ta), scandium (Sc), thorium (Th), and uranium (U) can be characteristic of these deposits and may be of environmental concern. Most of these elements, including the REEs, but with the exception of U, have low solubilities in water at the near-neutral pH values expected around these deposits. Mill tailings from carbonatite deposits can exceed residential soil and sediment criteria for Pb, and leachates from mill tailings can exceed drinking water guidelines for Pb. The greatest environmental challenges, however, are linked to the presence of Th and U, although mineral hosts for these elements are moderately unreactive in the environment. Both deposit types can have mill tailings that exceed residential soil criteria for U. Uranium can be recovered as a byproduct to mitigate its environmental effects, but Th remains a waste product that requires management.

  12. Assessment of (222)Rn emanation from ore body and backfill tailings in low-grade underground uranium mine.

    PubMed

    Mishra, Devi Prasad; Sahu, Patitapaban; Panigrahi, Durga Charan; Jha, Vivekanand; Patnaik, R Lokeswara

    2014-02-01

    This paper presents a comparative study of (222)Rn emanation from the ore and backfill tailings in an underground uranium mine located at Jaduguda, India. The effects of surface area, porosity, (226)Ra and moisture contents on (222)Rn emanation rate were examined. The study revealed that the bulk porosity of backfill tailings is more than two orders of magnitude than that of the ore. The geometric mean radon emanation rates from the ore body and backfill tailings were found to be 10.01 × 10(-3) and 1.03 Bq m(-2) s(-1), respectively. Significant positive linear correlations between (222)Rn emanation rate and the (226)Ra content of ore and tailings were observed. For normalised (226)Ra content, the (222)Rn emanation rate from tailings was found to be 283 times higher than the ore due to higher bulk porosity and surface area. The relative radon emanation from the tailings with moisture fraction of 0.14 was found to be 2.4 times higher than the oven-dried tailings. The study suggested that the mill tailings used as a backfill material significantly contributes to radon emanation as compared to the ore body itself and the (226)Ra content and bulk porosity are the dominant factors for radon emanation into the mine atmosphere.

  13. In-Well Sediment Incubators to Evaluate Microbial Community Stability and Dynamics following Bioimmobilization of Uranium

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Baldwin, Brett R.; Peacock, Aaron D.; Gan, M.

    2009-09-23

    An in-situ incubation device (ISI) was developed in order to investigate the stability and dynamics of sediment associated microbial communities to prevailing subsurface oxidizing or reducing conditions. Here we describe the use of these devices at the Old Rifle Uranium Mill Tailings Remedial Action (UMTRA) site. During the 7 month deployment oxidized Rifle aquifer background sediments (RABS) were deployed in previously biostimulated wells under iron reducing conditions, cell densities of known iron reducing bacteria including Geobacteraceae increased significantly showing the microbial community response to local subsurface conditions. PLFA profiles of RABS following in situ deployment were strikingly similar to thosemore » of adjacent sediment cores suggesting ISI results could be extrapolated to the native material of the test plots. Results for ISI deployed reduced sediments showed only slight changes in community composition and pointed toward the ability of the ISIs to monitor microbial community stability and response to subsurface conditions.« less

  14. 10 CFR Appendix A to Part 40 - Criteria Relating to the Operation of Uranium Mills and the Disposition of Tailings or Wastes...

    Code of Federal Regulations, 2013 CFR

    2013-01-01

    ... relatively thin, in-situ clay soils are to be relied upon for seepage control, tests must be conducted with... itself. (6) The design requirements in this criterion for longevity and control of radon releases apply... licensee shall control, minimize, or eliminate post-closure escape of nonradiological hazardous...

  15. Remedial Action Plan and site design for stabilization of the inactive uranium mill tailings site at Durango, Colorado: Attachment 2, Geology report. Revised final report

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1991-12-01

    Detailed investigations of geologic, geomorphic, and seismic conditions at the Bodo Canyon disposal site were conducted. The purpose of these investigations was basic site characterization and identification of potential geologic hazards that could affect long-term site stability. Subsequent engineering studies, such as analyses of hydrologic and liquefaction hazards, used the data developed in these studies. The geomorphic analysis was employed in the design of effective erosion protection. Studies of the regional and local seismotectonic setting, which included a detailed search for possible capable faults within a 65 kilometer radius of the site, provided the basis for seismic design parameters. Themore » scope of work performed included the following: Compilation and analysis of previous published and unpublished geologic literature and maps; Review of historical and instrumental earthquake data; Review of site-specific subsurface geologic data, including lithologic and geophysical logs of exploratory boreholes advanced in the site area; Photogeologic interpretations of existing conventional aerial photographs; and, Ground reconnaissance and mapping of the site region.« less

  16. DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    The site observational work plan (SOWP) for the Riverton, Wyoming, Uranium Mill Tailings Remedial Action (UMTRA) Project Site is the first document for the UMTRA Ground Water Project to address site-specific activities to meet compliance with the U.S. Environmental Protection Agency (EPA) proposed ground water standards (52 FR 36000 (1987)). In support of the activities the regulatory framework and drivers are presented along with a discussion of the relationship of this SOWP to other UMTRA Ground Water Project programmatic documents. A combination of the two compliance strategies that will be recommended for this site are no remediation with the applicationmore » of alternate concentration levels (ACL) and natural flushing in conjunction with institutional controls. ACLs are to be applied to constituents that occur at concentrations above background levels but which are essential nutrients and occur within nutritional ranges and/or have very low toxicity and high dietary intake rates compared to the levels detected in the ground water. The essential premise of natural flushing is that ground water movement and natural attenuation processes will reduce the detected contamination to background levels within 1 00 years. These two recommended compliance strategies were evaluated by applying Riverton site-specific data to the compliance framework developed in the UMTRA Ground Water programmatic environmental impact statement. There are three aquifers beneath the site: a surficial unconfined aquifer, a middle semiconfined aquifer, and a deeper confined aquifer. The milling-related contamination at the site has affected both the surficial and semiconfined aquifers, although the leaky shale aquifers separating these units limits the downward migration of contamination into the semiconfined aquifer. A shale aquitard separates the semiconfined aquifer from the underlying confined aquifer which has not been contaminated by milling-related constituents.« less

  17. Russian Experience in the Regulatory Supervision of the Uranium Legacy Sites - 12441

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Kiselev, M.F.; Romanov, V.V.; Shandala, N.K.

    2012-07-01

    Management of the uranium legacy is accompanied with environmental impact intensity of which depends on the amount of the waste generated, the extent of that waste localization and environmental spreading. The question is: how hazardous is such impact on the environment and human health? The criterion for safety assurance is adequate regulation of the uranium legacy. Since the establishment of the uranium industry, the well done regulatory system operates in the FMBA of Russia. Such system covers inter alia, the uranium legacy. This system includes the extent laboratory network of independent control and supervision, scientific researches, regulative practices. The currentmore » Russian normative and legal basis of the regulation and its application practice has a number of problems relating to the uranium legacy, connected firstly with the environmental remediation. To improve the regulatory system, the urgent tasks are: -To introduce the existing exposure situation into the national laws and standards in compliance with the ICRP system. - To develop criteria for site remediation and return, by stages, to uncontrolled uses. The similar criteria have been developed within the Russian-Norwegian cooperation for the purpose of remediation of the sites for temporary storage of SNF and RW. - To consider possibilities and methods of optimization for the remediation strategies under development. - To separate the special category - RW resulted from uranium ore mining and dressing. The current Russian RW classification is based on the waste subdivision in terms of the specific activities. Having in mind the new RW-specific law, we receive the opportunity to separate some special category - RW originated from the uranium mining and milling. Introduction of such category can simplify significantly the situation with management of waste of uranium mining and milling processes. Such approach is implemented in many countries and approved by IAEA. The category of 'RW originated from uranium mining and milling' is to be introduced as the legal acts and regulatory documents. The recent ICRP recommendations provide the flexible approaches for solving of such tasks. The FMBA of Russia recognizes the problems of radiation safety assurance related to the legacy of the former USSR in the uranium mining industry. Some part of the regulatory problems assumes to be solved within the EurAsEC inter-state target program 'Reclamation of the territories of the EurAsEC member states affected by the uranium mining and milling facilities'. Using the example of the uranium legacy sites in Kyrgyz and Tajikistan which could result in the tran-boundary disasters and require urgent reclamation, the experience will be gained to be used in other states as well. Harmonization of the national legislations and regulative documents on radiation safety assurance is envisaged. (authors)« less

  18. Feasibility Study of Economics and Performance of Geothermal Power Generation at the Lakeview Uranium Mill Site in Lakeview, Oregon. A Study Prepared in Partnership with the Environmental Protection Agency for the RE-Powering America's Land Initiative: Siting Renewable Energy on Potentially Contaminated Land and Mine Sites

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Hillesheim, M.; Mosey, G.

    2013-11-01

    The U.S. Environmental Protection Agency (EPA), in accordance with the RE-Powering America's Land initiative, selected the Lakeview Uranium Mill site in Lakeview, Oregon, for a feasibility study of renewable energy production. The EPA contracted with the National Renewable Energy Laboratory (NREL) to provide technical assistance for the project. The purpose of this report is to describe an assessment of the site for possible development of a geothermal power generation facility and to estimate the cost, performance, and site impacts for the facility. In addition, the report recommends development pathways that could assist in the implementation of a geothermal power systemmore » at the site.« less

  19. Integrated data base report--1996: US spent nuclear fuel and radioactive waste inventories, projections, and characteristics

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    NONE

    1997-12-01

    The Integrated Data Base Program has compiled historic data on inventories and characteristics of both commercial and U.S. Department of Energy (DOE) spent nuclear fuel (SNF) and commercial and U.S. government-owned radioactive wastes. Inventories of most of these materials are reported as of the end of fiscal year (FY) 1996, which is September 30, 1996. Commercial SNF and commercial uranium mill tailings inventories are reported on an end-of-calendar year (CY) basis. All SNF and radioactive waste data reported are based on the most reliable information available from government sources, the open literature, technical reports, and direct contacts. The information forecastedmore » is consistent with the latest DOE/Energy Information Administration (EIA) projections of U.S. commercial nuclear power growth and the expected DOE-related and private industrial and institutional activities. The radioactive materials considered, on a chapter-by-chapter basis, are SNF, high-level waste, transuranic waste, low-level waste, uranium mill tailings, DOE Environmental Restoration Program contaminated environmental media, naturally occurring and accelerator-produced radioactive material, and mixed (hazardous and radioactive) low-level waste. For most of these categories, current and projected inventories are given through FY 2030, and the radioactivity and thermal power are calculated based on reported or estimated isotopic compositions.« less

  20. Remedial Action Plan and site design for stabilization of the inactive uranium mill tailings site at Durango, Colorado: Attachment 6, Supplemental standard for Durango processing site. Revised final report

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1991-12-01

    Excavation control to the 15 pCi/g radium-226 (Ra-226) standard at certain areas along the Animas River on the Durango Site would require extensive engineering and construction support. Elevated Ra-226 concentrations have been encountered immediately adjacent to the river at depths in excess of 7 feet below the present river stage. Decontamination to such depths to ensure compliance with the EPA standards will, in our opinion, become unreasonable. This work does not appear to be in keeping with the intent of the standards. Because the principal reason for radium removal is reduction of radon daughter concentrations (RDC) in homes to bemore » built onsite, and because radon produced at depth will be attenuated in clean fill cover before entering such homes, it is appropriate to calculate the depth of excavation needed under a home to reduce RDC to acceptable levels. Potential impact was assessed through radon emanation estimation, using the RAECOM computer model. Elevated Ra-226 concentrations were encountered during final radium excavation of the flood plain below the large tailings pile, adjacent to the slag area. Data from 7 test pits excavated across the area were analyzed to provide an estimate of the Ra-226 concentration profile. Results are given in this report.« less

  1. Regulatory Oversight of the Legacy Gunner Uranium Mine and Mill Site in Northern Saskatchewan, Canada - 13434

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Stenson, Ron; Howard, Don

    2013-07-01

    As Canada's nuclear regulator, the Canadian Nuclear Safety Commission (CNSC) is responsible for licensing all aspects of uranium mining, including remediation activities at legacy sites. Since these sites already existed when the current legislation came into force in 2000, and the previous legislation did not apply, they present a special case. The Nuclear Safety and Control Act (NSCA), was written with cradle-to- grave oversight in mind. Applying the NSCA at the end of a 'facilities' life-cycle poses some challenges to both the regulator and the proponent. When the proponent is the public sector, even more challenges can present themselves. Althoughmore » the licensing process for legacy sites is no different than for any other CNSC license, assuring regulatory compliance can be more complicated. To demonstrate how the CNSC has approached the oversight of legacy sites the history of the Commission's involvement with the Gunnar uranium mine and mill site provides a good case study. The lessons learned from the CNSC's experience regulating the Gunnar site will benefit those in the future who will need to regulate legacy sites under existing or new legislation. (authors)« less

  2. Microbial Functional Gene Diversity with a Shift of Subsurface Redox Conditions during In Situ Uranium Reduction

    PubMed Central

    Liang, Yuting; Van Nostrand, Joy D.; N′Guessan, Lucie A.; Peacock, Aaron D.; Deng, Ye; Long, Philip E.; Resch, C. Tom; Wu, Liyou; He, Zhili; Li, Guanghe; Hazen, Terry C.; Lovley, Derek R.

    2012-01-01

    To better understand the microbial functional diversity changes with subsurface redox conditions during in situ uranium bioremediation, key functional genes were studied with GeoChip, a comprehensive functional gene microarray, in field experiments at a uranium mill tailings remedial action (UMTRA) site (Rifle, CO). The results indicated that functional microbial communities altered with a shift in the dominant metabolic process, as documented by hierarchical cluster and ordination analyses of all detected functional genes. The abundance of dsrAB genes (dissimilatory sulfite reductase genes) and methane generation-related mcr genes (methyl coenzyme M reductase coding genes) increased when redox conditions shifted from Fe-reducing to sulfate-reducing conditions. The cytochrome genes detected were primarily from Geobacter sp. and decreased with lower subsurface redox conditions. Statistical analysis of environmental parameters and functional genes indicated that acetate, U(VI), and redox potential (Eh) were the most significant geochemical variables linked to microbial functional gene structures, and changes in microbial functional diversity were strongly related to the dominant terminal electron-accepting process following acetate addition. The study indicates that the microbial functional genes clearly reflect the in situ redox conditions and the dominant microbial processes, which in turn influence uranium bioreduction. Microbial functional genes thus could be very useful for tracking microbial community structure and dynamics during bioremediation. PMID:22327592

  3. Uranium-Bearing Evaporite Mineralization Influencing Plume Persistence. Literature Review and DOE-LM Site Surveys

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    None, None

    This report on evaporite mineralization was completed as an Ancillary Work Plan for the Applied Studies and Technology program under the U.S. Department of Energy (DOE) Office of Legacy Management (LM). This study reviews all LM sites under Title I and Title II of the Uranium Mill Tailings Radiation Control Act (UMTRCA) and one Decontamination and Decommissioning site to provide (1) a summary of which sites have evaporite deposits, (2) any available quantitative geochemical and mineralogical analyses, and (3) references to relevant reports. In this study, “evaporite” refers to any secondary mineral precipitate that occurs due to a loss ofmore » water through evaporative processes. This includes efflorescent salt crusts, where this term refers to a migration of dissolved constituents to the surface with a resulting salt crust, where “salt” can refer to any secondary precipitate, regardless of constituents. The potential for the formation of evaporites at LM sites has been identified, and may have relevance to plume persistence issues. Evaporite deposits have the potential to concentrate and store contaminants at LM sites that could later be re-released. These deposits can also provide a temporary storage mechanism for carbonate, chloride, and sulfate salts along with uranium and other contaminants of concern (COCs). Identification of sites with evaporites will be used in a new technical task plan (TTP), Persistent Secondary Contaminant Sources (PeSCS), for any proposed additional sampling and analyses. This additional study is currently under development and will focus on determining if the dissolution of evaporites has the potential to hinder natural flushing strategies and impact plume persistence. This report provides an initial literature review on evaporites followed by details for each site with identified evaporites. The final summary includes a table listing of all relevant LM sites regardless of evaporite identification.« less

  4. An industry perspective on commercial radioactive waste disposal conditions and trends.

    PubMed

    Romano, Stephen A

    2006-11-01

    The United States is presently served by Class-A, -B and -C low-level radioactive waste and naturally-occurring and accelerator-produced radioactive material disposal sites in Washington and South Carolina; a Class-A and mixed waste disposal site in Utah that also accepts naturally-occurring radioactive material; and hazardous and solid waste facilities and uranium mill tailings sites that accept certain radioactive materials on a site-specific basis. The Washington site only accepts low-level radioactive waste from 11 western states due to interstate Compact restrictions on waste importation. The South Carolina site will be subject to geographic service area restrictions beginning 1 July 2008, after which only three states will have continued access. The Utah site dominates the commercial Class-A and mixed waste disposal market due to generally lower state fees than apply in South Carolina. To expand existing commercial services, an existing hazardous waste site in western Texas is seeking a Class-A, -B and -C and mixed waste disposal license. With that exception, no new Compact facilities are proposed. This fluid, uncertain situation has inspired national level rulemaking initiatives and policy studies, as well as alternative disposal practices for certain low-activity materials.

  5. Predicting arsenic concentrations in porewaters of buried uranium mill tailings

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Langmuir, D.; Mahoney, J.; MacDonald, A.

    The proposed JEB Tailings Management Facility (TMF) to be emplaced below the groundwater table in northern Saskatchewan, Canada, will contain uranium mill tailings from McClean Lake, Midwest and Cigar Lake ore bodies, which are high in arsenic (up to 10%) and nickel (up to 5%). A serious concern is the possibility that high arsenic and nickel concentrations may be released from the buried tailings, contaminating adjacent groundwaters and a nearby lake. Laboratory tests and geochemical modeling were performed to examine ways to reduce the arsenic and nickel concentrations in TMF porewaters so as to minimize such contamination from tailings buriedmore » for 50 years and longer. The tests were designed to mimic conditions in the mill neutralization circuit (3 hr tests at 25 C), and in the TMF after burial (5--49 day aging tests). The aging tests were run at 50, 25 and 4 C (the temperature in the TMF). In order to optimize the removal of arsenic by adsorption and precipitation, ferric sulfate was added to tailings raffinates having Fe/As ratios of less than 3--5. The acid raffinates were then neutralized by addition of slaked lime to nominal pH values of 7, 8, or 9. Analysis and modeling of the test results showed that with slaked lime addition to acid tailings raffinates, relatively amorphous scorodite (ferric arsenate) precipitates near pH 1, and is the dominant form of arsenate in slake limed tailings solids except those high in Ni and As and low in Fe, in which cabrerite-annabergite (Ni, Mg, Fe(II) arsenate) may also precipitate near pH 5--6. In addition to the arsenate precipitates, smaller amounts of arsenate are also adsorbed onto tailings solids. The aging tests showed that after burial of the tailings, arsenic concentrations may increase with time from the breakdown of the arsenate phases (chiefly scorodite). However, the tests indicate that the rate of change decreases and approaches zero after 72 hrs at 25 C, and may equal zero at all times in the TMF at 4 C. Consistent with a kinetic model that describes the rate of breakdown of scorodite to form hydrous ferric oxide, the rate of release of dissolved arsenate to tailings porewaters from slake limed tailings: (1) is proportional to pH above pH 6--7; (2) decreases exponentially as the total molar Fe/As ratio of tailings raffinates is increased from 1/1 to greater than 5/1; and (3) is proportional to temperature with an average Arrhenius activation energy of 13.4 {+-} 4.2 kcal/mol. Study results suggest that if ferric sulfate and slaked lime are added in the tailings neutralization circuit to give a raffinate Fe/As molar ratio of at least 3--5 and a nominal (initial) pH of 8 (final pH of 7--8), arsenic and nickel concentrations of 2 mg/L or less, are probable in porewaters of individual tailings in the TMF for 50 to 10,000 yrs after tailings disposal. However, the tailings will be mixed in the TMF, which will contain about 35% tailings with Fe/As = 3.0, and 65% tailings with Fe/As = 5.0--7.7. Thus, it seems likely that average arsenic pore water concentrations in the TMF may not exceed 1 mg/L.« less

  6. Groundwater contamination from an inactive uranium mill tailings pile: 2. Application of a dynamic mixing model

    NASA Astrophysics Data System (ADS)

    Narasimhan, T. N.; White, A. F.; Tokunaga, T.

    1986-12-01

    At Riverton, Wyoming, low pH process waters from an abandoned uranium mill tailings pile have been infiltrating into and contaminating the shallow water table aquifer. The contamination process has been governed by transient infiltration rates, saturated-unsaturated flow, as well as transient chemical reactions between the many chemical species present in the mixing waters and the sediments. In the first part of this two-part series [White et al., 1984] we presented field data as well as an interpretation based on a static mixing model. As an upper bound, we estimated that 1.7% of the tailings water had mixed with the native groundwater. In the present work we present the results of numerical investigation of the dynamic mixing process. The model, DYNAMIX (DYNAmic MIXing), couples a chemical speciation algorithm, PHREEQE, with a modified form of the transport algorithm, TRUMP, specifically designed to handle the simultaneous migration of several chemical constituents. The overall problem of simulating the evolution and migration of the contaminant plume was divided into three sub problems that were solved in sequential stages. These were the infiltration problem, the reactive mixing problem, and the plume-migration problem. The results of the application agree reasonably with the detailed field data. The methodology developed in the present study demonstrates the feasibility of analyzing the evolution of natural hydrogeochemical systems through a coupled analysis of transient fluid flow as well as chemical reactions. It seems worthwhile to devote further effort toward improving the physicochemical capabilities of the model as well as to enhance its computational efficiency.

  7. Groundwater contamination from an inactive uranium mill tailings pile. 2. Application of a dynamic mixing model

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Narashimhan, T.N.; White, A.F.; Tokunaga, T.

    1986-12-01

    At Riverton, Wyoming, low pH process waters from an abandoned uranium mill tailings pile have been infiltrating into and contaminating the shallow water table aquifer. The contamination process has been governed by transient infiltration rates, saturated-unsaturated flow, as well as transient chemical reactions between the many chemical species present in the mixing waters and the sediments. In the first part of this two-part series the authors presented field data as well as an interpretation based on a static mixing models. As an upper bound, the authors estimated that 1.7% of the tailings water had mixed with the native groundwater. Inmore » the present work they present the results of numerical investigation of the dynamic mixing process. The model, DYNAMIX (DYNamic MIXing), couples a chemical speciation algorithm, PHREEQE, with a modified form of the transport algorithm, TRUMP, specifically designed to handle the simultaneous migration of several chemical constituents. The overall problem of simulating the evolution and migration of the contaminant plume was divided into three sub problems that were solved in sequential stages. These were the infiltration problem, the reactive mixing problem, and the plume-migration problem. The results of the application agree reasonably with the detailed field data. The methodology developed in the present study demonstrates the feasibility of analyzing the evolution of natural hydrogeochemical systems through a coupled analysis of transient fluid flow as well as chemical reactions. It seems worthwhile to devote further effort toward improving the physicochemical capabilities of the model as well as to enhance its computational efficiency.« less

  8. DOE Office of Scientific and Technical Information (OSTI.GOV)

    Kautsky, Mark; Ranalli, Tony; Dander, David

    The objective of this investigation was to identify and differentiate potential non- mill-related water inputs to a shallow terrace groundwater system through the use of aqueous chemical and isotopic tracers at a former uranium- and vanadium-ore processing facility. Terrace groundwater in the vicinity of the Shiprock, New Mexico, site is hypothesized to be largely anthropogenic because natural rates of recharge in the terrace are likely insufficient to sustain a continuous water table in the terrace alluvial system, as observed in several analogue terrace locations east of the site and in response to post-mill dewatering efforts across the site. The terracemore » is composed of alluvial sand and gravel and weathered and unweathered Mancos Shale. Terrace groundwater exists and flows in the alluvium and to a much less extent in the Mancos Shale. Historical data established that in both the terrace and floodplain below the terrace, mill-derived uranium and sulfate is found primarily in the alluvium and the upper portion of the weathered Mancos Shale. Groundwater extraction is being conducted in the vicinity of former mill operations and in washes and seeps to dewater the formation and remove contamination, thus eliminating these exposure pathways and minimizing movement to the floodplain. However, past and present contribution of non-mill anthropogenic water sources may be hindering the dewatering effort, resulting in reduced remedy effectiveness. Groundwater source signatures can be determined based on chemical and isotopic ratios and are used to help identify and delineate both mill and non-mill water contributions. Aqueous chemical and isotopic tracers, such as 234U/238U activity ratios and uranium concentrations, δ34S sulfate and sulfate concentrations, tritium concentrations, and δ2Hwater and δ18O water are being used in this Phase I study. The aqueous chemical and isotopic analysis has identified areas on the terrace where groundwater is derived from mill-related activities and areas where the groundwater is associated with non-mill activities. A separate field effort of Phase II work will follow, including investigating additional locations for these isotopes and examination of δ18Osulfate , δ34Ssulfate , and chlorofluorocarbon signatures.« less

  9. Using proteomic data to assess a genome-scale "in silico" model of metal reducing bacteria in the simulation of field-scale uranium bioremediation

    NASA Astrophysics Data System (ADS)

    Yabusaki, S.; Fang, Y.; Wilkins, M. J.; Long, P.; Rifle IFRC Science Team

    2011-12-01

    A series of field experiments in a shallow alluvial aquifer at a former uranium mill tailings site have demonstrated that indigenous bacteria can be stimulated with acetate to catalyze the conversion of hexavalent uranium in a groundwater plume to immobile solid-associated uranium in the +4 oxidation state. While this bioreduction of uranium has been shown to lower groundwater concentrations below actionable standards, a viable remediation methodology will need a mechanistic, predictive and quantitative understanding of the microbially-mediated reactions that catalyze the reduction of uranium in the context of site-specific processes, properties, and conditions. At the Rifle IFRC site, we are investigating the impacts on uranium behavior of pulsed acetate amendment, acetate-oxidizing iron and sulfate reducing bacteria, seasonal water table variation, spatially-variable physical (hydraulic conductivity, porosity) and geochemical (reactive surface area) material properties. The simulation of three-dimensional, variably saturated flow and biogeochemical reactive transport during a uranium bioremediation field experiment includes a genome-scale in silico model of Geobacter sp. to represent the Fe(III) terminal electron accepting process (TEAP). The Geobacter in silico model of cell-scale physiological metabolic pathways is comprised of hundreds of intra-cellular and environmental exchange reactions. One advantage of this approach is that the TEAP reaction stoichiometry and rate are now functions of the metabolic status of the microorganism. The linkage of in silico model reactions to specific Geobacter proteins has enabled the use of groundwater proteomic analyses to assess the accuracy of the model under evolving hydrologic and biogeochemical conditions. In this case, the largest predicted fluxes through in silico model reactions generally correspond to high abundances of proteins linked to those reactions (e.g. the condensation reaction catalyzed by the protein citrate synthase that generates citrate from acetyl-CoA and oxaloacetate). Model discrepancies with the proteomic data, such as the prediction of shifts associated with nitrogen limitation, revealed pathways in the in silico code that could be modified to more accurately predict metabolic processes that occur in the subsurface. The potential outcome of this approach is the engineering of electron donor (e.g., acetate), terminal electron acceptor [e.g., U(VI)], and biogeochemical conditions that enhance the desired metabolic pathways of the target microorganism(s) to effect cost-effective uranium bioreduction.

  10. Natural and Enhanced Attenuation of Soil and Groundwater at the Monument Valley, Arizona, DOE Legacy Waste Site—10281

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Waugh, W.J.; Miller, D.E.; Morris, S.A.

    2010-03-07

    The U.S. Department of Energy (DOE), the Navajo Nation, and the University of Arizona are exploring natural and enhanced attenuation remedies for groundwater contamination at a former uranium-ore processing site near Monument Valley, Arizona. DOE removed radioactive tailings from the Monument Valley site in 1994. Nitrate and ammonium, waste products of the milling process, remain in an alluvial groundwater plume spreading from the soil source where tailings were removed. Planting and irrigating two native shrubs, fourwing saltbush and black greasewood, markedly reduced both nitrate and ammonium in the source area over an 8-year period. Total nitrogen dropped from 350 mg/kgmore » in 2000 to less than 200 mg/kg in 2008. Most of the reduction is attributable to irrigation-enhanced microbial denitrification rather than plant uptake. However, soil moisture and percolation flux monitoring show that the plantings control the soil water balance in the source area, preventing additional leaching of nitrogen compounds. Enhanced denitrification and phytoremediation also look promising for plume remediation. Microcosm experiments, nitrogen isotopic fractionation analysis, and solute transport modeling results suggest that (1) up to 70 percent of nitrate in the plume has been lost through natural denitrification since the mill was closed in 1968, and (2) injection of ethanol may accelerate microbial denitrification in plume hot spots. A field-scale ethanol injection pilot study is underway. Landscape-scale remote sensing methods developed for the project suggest that transpiration from restored native phreatophyte populations rooted in the aquifer could limit further expansion of the plume. An evaluation of landfarm phytoremediation, the irrigation of native shrub plantings with high nitrate water pumped from the alluvial aquifer, is also underway.« less

  11. A Uranium Bioremediation Reactive Transport Benchmark

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Yabusaki, Steven B.; Sengor, Sevinc; Fang, Yilin

    A reactive transport benchmark problem set has been developed based on in situ uranium bio-immobilization experiments that have been performed at a former uranium mill tailings site in Rifle, Colorado, USA. Acetate-amended groundwater stimulates indigenous microorganisms to catalyze the reduction of U(VI) to a sparingly soluble U(IV) mineral. The interplay between the flow, acetate loading periods and rates, microbially-mediated and geochemical reactions leads to dynamic behavior in metal- and sulfate-reducing bacteria, pH, alkalinity, and reactive mineral surfaces. The benchmark is based on an 8.5 m long one-dimensional model domain with constant saturated flow and uniform porosity. The 159-day simulation introducesmore » acetate and bromide through the upgradient boundary in 14-day and 85-day pulses separated by a 10 day interruption. Acetate loading is tripled during the second pulse, which is followed by a 50 day recovery period. Terminal electron accepting processes for goethite, phyllosilicate Fe(III), U(VI), and sulfate are modeled using Monod-type rate laws. Major ion geochemistry modeled includes mineral reactions, as well as aqueous and surface complexation reactions for UO2++, Fe++, and H+. In addition to the dynamics imparted by the transport of the acetate pulses, U(VI) behavior involves the interplay between bioreduction, which is dependent on acetate availability, and speciation-controlled surface complexation, which is dependent on pH, alkalinity and available surface complexation sites. The general difficulty of this benchmark is the large number of reactions (74), multiple rate law formulations, a multisite uranium surface complexation model, and the strong interdependency and sensitivity of the reaction processes. Results are presented for three simulators: HYDROGEOCHEM, PHT3D, and PHREEQC.« less

  12. Natural radionuclides in trees grown on a uranium mill tailings waste pile.

    PubMed

    Strok, Marko; Smodiš, Borut; Eler, Klemen

    2011-06-01

    The purpose of the study was to investigate natural radionuclide uptake and allocation by trees. Samples from six Scots pines (P. sylvestris), six Norway spruces (Picea abies) and one sycamore maple (Acer pseudoplatanus) tree, growing on the Boršt uranium mill tailings waste pile in Slovenia were collected. (238)U, (230)Th, (226)Ra and (210)Pb activity concentrations in wood, shoots and 1-year-old needles or leaves were determined. Particular radionuclides were separated from the samples by appropriate radiochemical procedures and their activity concentrations measured with an alpha spectrometry system. In addition, concentration ratios for different plant parts were calculated. Results showed that for all radionuclides, the highest activity concentrations were found in foliage, followed by shoots and wood. The activity concentrations in trees were from 0.01 to 5.4 Bq kg(-1) for (238)U, 0.03-11.3 Bq kg(-1) for (230)Th, 2.7-2,728 Bq kg(-1) for (226)Ra and 5.1-321 Bq kg(-1) for (210)Pb. All activity concentrations were calculated on dry weight basis. The calculated concentration ratios were from 1.05E-5 to 5.39E-3 for (238)U, 7.65E-6-2.88E-3 for (230)Th, 3.10E-4-3.16E-1 for (226)Ra and 6.70E-4-4.22E-2 for (210)Pb.

  13. Effects of grazing on leaf area index, fractional cover and evapotranspiration by a desert phreatophyte community at a former uranium mill site on the Colorado Plateau

    USGS Publications Warehouse

    Bresloff, Cynthia J.; Nguyen, Uyen; Glenn, Edward P.; Waugh, Jody; Nagler, Pamela L.

    2013-01-01

    This study employed ground and remote sensing methods to monitor the effects of grazing on leaf area index (LAI), fractional cover (fc) and evapotranspiration (ET) of a desert phreatophyte community over an 11 year period at a former uranium mill site on the Colorado Plateau, U.S. Nitrate, ammonium and sulfate are migrating away from the mill site in a shallow alluvial aquifer. The phreatophyte community, consisting of Atriplex canescens (ATCA) and Sarcobatus vermiculatus (SAVE) shrubs, intercepts groundwater and could potentially slow the movement of the contaminant plume through evapotranspiration (ET). However, the site has been heavily grazed by livestock, reducing plant cover and LAI. We used livestock exclosures and revegetation plots to determine the effects of grazing on LAI, fc and ET, then projected the findings over the whole site using multi-platform remote sensing methods. We show that ET is approximately equal to annual precipitation at the site, but when ATCA and SAVE are protected from grazing they can develop high fc and LAI values, and ET can exceed annual precipitation, with the excess coming from groundwater discharge. Therefore, control of grazing could be an effective method to slow migration of contaminants at this and similar sites in the western U.S.

  14. Site observational work plan for the UMTRA Project site at Monument Valley, Arizona

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    NONE

    1995-09-01

    The site observational work plan (SOWP) for the Monument Valley, Arizona, US Department of Energy (DOE) Uranium Mill Tailings Remedial Action (UMTRA) Project site is one of the first site-specific documents developed to achieve ground water compliance at the site. This SOWP applies information about the Monument Valley site to a regulatory compliance framework that identifies strategies that could be used to meet ground water compliance. The compliance framework was developed in the UMTRA Ground Water programmatic environmental impact statement (DOE, 1995). The DOE`s goal is to implement a cost-effective site strategy that complies with the US Environmental Protection Agencymore » (EPA) ground water standards and protects human health and the environment. The compliance strategy that emerges in the final version of the SOWP will assess potential environmental impacts and provide stakeholder a forum for review and comment. When the compliance strategy is acceptable, it will be detailed in a remedial action plan that will be subject to review by the state and/or tribe and concurrence by the US Nuclear Regulatory Commission (NRC). Information available for the preparation of this SOWP indicates active remediation is the most likely compliance strategy for the Monument Valley site. Additional data are needed to determine the most effective remediation technology.« less

  15. UMTRA project list of reportable occurrences

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1994-04-01

    This UMTRA Project List of Reportable occurrences is provided to facilitate efficient categorization of reportable occurrences. These guidelines have been established in compliance with DOE minimum reporting requirements under DOE Order 5000.3B. Occurrences are arranged into nine groups relating to US Department of Energy (DOE) Uranium Mill Tailings Remedial Action (UMTRA) Project operations for active sites. These nine groupings are provided for reference to determined whether an occurrence meets reporting requirement criteria in accordance with the minimum reporting requirements. Event groups and significance categories that cannot or will not occur, and that do not apply to UMTRA Project operations, aremore » omitted. Occurrence categorization shall be as follows: Group 1. Facility Condition; Group 2. Environmental; Group 3. Personnel Safety; Group 4. Personnel Radiation Protection; Group 5. Safeguards and Security; Group 6. Transportation; Group 7. Value Basis Reporting; Group 8. Facility Status; and Group 9. Cross-Category Items.« less

  16. 76 FR 70170 - Proposed Alternative Soils Standards for the Uravan, Colorado Uranium Mill

    Federal Register 2010, 2011, 2012, 2013, 2014

    2011-11-10

    ... identified four discrete areas that are not in full compliance with the soil remediation standards. The... State of Colorado and the EPA to proceed with delisting the Uravan site from the NPL. Four discrete... four discrete areas are referred to as: the Mill Hillside Area; A-Plant North Area; River Ponds Area...

  17. Biogeochemical behaviour and bioremediation of uranium in waters of abandoned mines.

    PubMed

    Mkandawire, Martin

    2013-11-01

    The discharges of uranium and associated radionuclides as well as heavy metals and metalloids from waste and tailing dumps in abandoned uranium mining and processing sites pose contamination risks to surface and groundwater. Although many more are being planned for nuclear energy purposes, most of the abandoned uranium mines are a legacy of uranium production that fuelled arms race during the cold war of the last century. Since the end of cold war, there have been efforts to rehabilitate the mining sites, initially, using classical remediation techniques based on high chemical and civil engineering. Recently, bioremediation technology has been sought as alternatives to the classical approach due to reasons, which include: (a) high demand of sites requiring remediation; (b) the economic implication of running and maintaining the facilities due to high energy and work force demand; and (c) the pattern and characteristics of contaminant discharges in most of the former uranium mining and processing sites prevents the use of classical methods. This review discusses risks of uranium contamination from abandoned uranium mines from the biogeochemical point of view and the potential and limitation of uranium bioremediation technique as alternative to classical approach in abandoned uranium mining and processing sites.

  18. The new nuclear west: Uranium milling as community on Colorado's western slope

    NASA Astrophysics Data System (ADS)

    Tidwell, Abraham S. D.

    In mid-2007, Energy Fuels, a Toronto-based uranium mining and milling company, announced their intent to build Piñon Ridge, the first new conventional uranium mill in the United States in 30 years. The prospect of a return to uranium milling has mobilized community support to bring back an industry some see as both familiar and capable of supporting and growing their communities. Using transcripts generated during the Colorado Department of Public Health and Environment's public meetings and hearings during 2010 and 2012, this study examines how proponents of the mill frame the socioeconomic advantages of bringing the industry back. Applying Kinsella's bounded constitutive model of communication, this study shows that the community and the uranium mill are bound in a "sorge-enframing" duality where the care generated by each binds the other to the recalcitrant nature of the uranium industry and preconceived notions of socioeconomic development, respectively.

  19. Microbial transformations of uranium in wastes and implication on its mobility

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Suzuki,Y.; Nankawa, T.; Ozaki, T.

    2008-09-14

    Uranium exists in several chemical forms in mining and mill tailings and in nuclear and weapons production wastes. Under appropriate conditions, microorganisms can affect the stability and mobility of U in wastes by altering the chemical speciation, solubility and sorption properties and thus could increase or decrease the concentrations of U in solution and the bioavailability. Dissolution or immobilization of U is brought about by direct enzymatic action or indirect nonenzymatic action of microorganisms. Although the physical, chemical, and geochemical processes affecting dissolution, precipitation, and mobilization of U have been extensively investigated, we have only limited information on the mechanismsmore » of microbial transformations of various chemical forms of U in the presence of electron donors and acceptors.« less

  20. Superfund Record of Decision (EPA Region 6): Cimarron Mining Corporation site, Operable Unit 1, Lincoln County, Carrizozo, NM. (First remedial action), September 1990

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1990-09-21

    The 10.6-acre Cimarron Mining site, Lincoln County, New Mexico, is an inactive milling facility used to recover iron from ores transported to the site. A shallow aquifer, which is not a potential drinking water source, and a deeper primary drinking water aquifer lie beneath the site. Cyanide was used until 1982 to recover precious metals. The operation of the mill resulted in the discharge of contaminated liquids onsite. The sources of environmental cyanide contamination at the site are the processed waste materials, including tailings piles and cinder block trench sediment piles, the cyanide solution and tailings spillage areas, and themore » cyanide solution recycling and disposal areas, including cinder block trenches and an unlined discharge pit. The major sources of ground water contamination by cyanide are the cinder block trenches and the discharge pit. These areas of prolonged contact between cyanide solution and underlying soil led to cyanide contamination in the shallow aquifer. The ROD addresses contaminated shallow ground water at the Cimarron Mining mill area as Operable Unit 1 (OU1). The primary contaminants of concern affecting the ground water are inorganics including cyanide.« less

  1. Technical approach to groundwater restoration. Final report

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1993-11-01

    The Technical Approach to Groundwater Restoration (TAGR) provides general technical guidance to implement the groundwater restoration phase of the Uranium Mill Tailings Remedial Action (UMTRA) Project. The TAGR includes a brief overview of the surface remediation and groundwater restoration phases of the UMTRA Project and describes the regulatory requirements, the National Environmental Policy Act (NEPA) process, and regulatory compliance. A section on program strategy discusses program optimization, the role of risk assessment, the observational approach, strategies for meeting groundwater cleanup standards, and remedial action decision-making. A section on data requirements for groundwater restoration evaluates the data quality objectives (DQO) andmore » minimum data required to implement the options and comply with the standards. A section on sits implementation explores the development of a conceptual site model, approaches to site characterization, development of remedial action alternatives, selection of the groundwater restoration method, and remedial design and implementation in the context of site-specific documentation in the site observational work plan (SOWP) and the remedial action plan (RAP). Finally, the TAGR elaborates on groundwater monitoring necessary to evaluate compliance with the groundwater cleanup standards and protection of human health and the environment, and outlines licensing procedures.« less

  2. Effects of grazing on leaf area index, fractional cover and evapotranspiration by a desert phreatophyte community at a former uranium mill site on the Colorado Plateau.

    PubMed

    Bresloff, Cynthia J; Nguyen, Uyen; Glenn, Edward P; Waugh, Jody; Nagler, Pamela L

    2013-01-15

    This study employed ground and remote sensing methods to monitor the effects of grazing on leaf area index (LAI), fractional cover (f(c)) and evapotranspiration (ET) of a desert phreatophyte community over an 11 year period at a former uranium mill site on the Colorado Plateau, U.S. Nitrate, ammonium and sulfate are migrating away from the mill site in a shallow alluvial aquifer. The phreatophyte community, consisting of Atriplex canescens (ATCA) and Sarcobatus vermiculatus (SAVE) shrubs, intercepts groundwater and could potentially slow the movement of the contaminant plume through evapotranspiration (ET). However, the site has been heavily grazed by livestock, reducing plant cover and LAI. We used livestock exclosures and revegetation plots to determine the effects of grazing on LAI, f(c) and ET, then projected the findings over the whole site using multi-platform remote sensing methods. We show that ET is approximately equal to annual precipitation at the site, but when ATCA and SAVE are protected from grazing they can develop high f(c) and LAI values, and ET can exceed annual precipitation, with the excess coming from groundwater discharge. Therefore, control of grazing could be an effective method to slow migration of contaminants at this and similar sites in the western U.S. Copyright © 2012 Elsevier Ltd. All rights reserved.

  3. Sensitivity of geological, geochemical and hydrologic parameters in complex reactive transport systems for in-situ uranium bioremediation

    NASA Astrophysics Data System (ADS)

    Yang, G.; Maher, K.; Caers, J.

    2015-12-01

    Groundwater contamination associated with remediated uranium mill tailings is a challenging environmental problem, particularly within the Colorado River Basin. To examine the effectiveness of in-situ bioremediation of U(VI), acetate injection has been proposed and tested at the Rifle pilot site. There have been several geologic modeling and simulated contaminant transport investigations, to evaluate the potential outcomes of the process and identify crucial factors for successful uranium reduction. Ultimately, findings from these studies would contribute to accurate predictions of the efficacy of uranium reduction. However, all these previous studies have considered limited model complexities, either because of the concern that data is too sparse to resolve such complex systems or because some parameters are assumed to be less important. Such simplified initial modeling, however, limits the predictive power of the model. Moreover, previous studies have not yet focused on spatial heterogeneity of various modeling components and its impact on the spatial distribution of the immobilized uranium (U(IV)). In this study, we study the impact of uncertainty on 21 parameters on model responses by means of recently developed distance-based global sensitivity analysis (DGSA), to study the main effects and interactions of parameters of various types. The 21 parameters include, for example, spatial variability of initial uranium concentration, mean hydraulic conductivity, and variogram structures of hydraulic conductivity. DGSA allows for studying multi-variate model responses based on spatial and non-spatial model parameters. When calculating the distances between model responses, in addition to the overall uranium reduction efficacy, we also considered the spatial profiles of the immobilized uranium concentration as target response. Results show that the mean hydraulic conductivity and the mineral reaction rate are the two most sensitive parameters with regard to the overall uranium reduction. But in terms of spatial distribution of immobilized uranium, initial conditions of uranium concentration and spatial uncertainty in hydraulic conductivity also become important. These analyses serve as the first step of further prediction practices of the complex uranium transport and reaction systems.

  4. Capacity of Lemna gibba L. (duckweed) for uranium and arsenic phytoremediation in mine tailing waters.

    PubMed

    Mkandawire, Martin; Taubert, Barbara; Dudel, E Gert

    2004-01-01

    The potential of Lemna gibba L. to clean uranium and arsenic contamination from mine surface waters was investigated in wetlands of two former uranium mines in eastern Germany and in laboratory hydroponic culture. Water and plants were sampled and L gibba growth and yield were monitored in tailing ponds from the field study sites. Contaminant accumulation, growth and yield experiments were conducted in the laboratory using synthetic tailing water. Mean background concentrations of the surface waters were 186.0+/-81.2 microg l(-1) uranium and 47.0+/-21.3 microg l(-1) arsenic in Site one and 293.7+/-121.3 microg l(-1) uranium and 41.37+/-24.7 microg l(-1) arsenic in Site two. The initial concentration of both uranium and arsenic in the culture solutions was 100 microg l(-1). The plant samples were either not leached, leached with deionized H2O or ethylenediaminetetracetic (EDTA). The results revealed high bioaccumulation coefficients for both uranium and arsenic. Uranium and arsenic content of L gibba dry biomass of the field samples were as follows: nonleached samples > deionized H2O leached (insignificant ANOVA p = 0.05) > EDTA leached. The difference in both arsenic and uranium enrichment were significantly high between the nonleached and the other two lead samples tested at ANOVA p > 0.001. Estimated mean L gibba density in surface water was 85,344.8+/-1843.4 fronds m(-2) (approximately 1319.7 g m(-2)). The maximum specific growth rate was 0.47+/-0.2 d(-1), which exceeded reported specific growth rates for L gibba in the literature. Average yield was estimated at 20.2+/-6.7 g m(-2) d(-1), giving approximately 73.6+/-21.4 t ha(-1) y(-1) as the annual yield. The highest accumulations observed were 896.9+/-203.8 mg kg(-1) uranium and 1021.7+/-250.8 mg kg(-1) arsenic dry biomass for a 21-d test period in the laboratory steady-state experiments. The potential extractions from surface waters with L gibba L. were estimated to be 662.7 kg uranium ha(-1) yr(-1) and 751.9 kg arsenic ha(-1) yr(-1) under the above conditions.

  5. DOE Office of Scientific and Technical Information (OSTI.GOV)

    Dam, William; Campbell, Sam; Johnson, Ray

    Milling activities at a former uranium mill site near Riverton, Wyoming, USA, contaminated the shallow groundwater beneath and downgradient of the site. Although the mill operated for <6 years (1958-1963), its impact remains an environmental liability. Groundwater modeling predicted that contaminant concentrations were declining steadily, which confirmed the conceptual site model (CSM). However, local flooding in 2010 mobilized contaminants that migrated downgradient from the Riverton site and resulted in a dramatic increase in groundwater contaminant concentrations. This observation indicated that the original CSM was inadequate to explain site conditions and needed to be refined. In response to the new observationsmore » after the flood, a collaborative investigation to better understand site conditions and processes commenced. This investigation included installing 103 boreholes to collect soil and groundwater samples, sampling and analysis of evaporite minerals along the bank of the Little Wind River, an analysis of evaportranspiration in the shallow aquifer, and sampling naturally organic-rich sediments near groundwater discharge areas. The enhanced characterization revealed that the existing CSM did not account for high uranium concentrations in groundwater remaining on the former mill site and groundwater plume stagnation near the Little Wind River. Observations from the flood and subsequent investigations indicate that additional characterization is still needed to continue refining the CSM and determine the viability of the natural flushing compliance strategy. Additional sampling, analysis, and testing of soil and groundwater are necessary to investigate secondary contaminant sources, mobilization of contaminants during floods, geochemical processes, contaminant plume stagnation, distribution of evaporite minerals and organic-rich sediments, and mechanisms and rates of contaminant transfer from soil to groundwater. Future data collection will be used to continually revise the CSM and evaluate the compliance strategy at the site.« less

  6. Review of samples of tailings, soils and stream sediment adjacent to and downstream from the Ruth Mine, Inyo County, California

    USGS Publications Warehouse

    Rytuba, James J.; Kim, Christopher S.; Goldstein, Daniel N.

    2011-01-01

    The Ruth Mine and mill are located in the western Mojave Desert in Inyo County, California (fig. 1). The mill processed gold-silver (Au-Ag) ores mined from the Ruth Au-Ag deposit, which is adjacent to the mill site. The Ruth Au-Ag deposit is hosted in Mesozoic intrusive rocks and is similar to other Au-Ag deposits in the western Mojave Desert that are associated with Miocene volcanic centers that formed on a basement of Mesozoic granitic rocks (Bateman, 1907; Gardner, 1954; Rytuba, 1996). The volcanic rocks consist of silicic domes and associated flows, pyroclastic rocks, and subvolcanic intrusions (fig. 2) that were emplaced into Mesozoic silicic intrusive rocks (Troxel and Morton, 1962). The Ruth Mine is on Federal land managed by the U.S. Bureau of Land Management (BLM). Tailings from the mine have been eroded and transported downstream into Homewood Canyon and then into Searles Valley (figs. 3, 4, 5, and 6). The BLM provided recreational facilities at the mine site for day-use hikers and restored and maintained the original mine buildings in collaboration with local citizen groups for use by visitors (fig. 7). The BLM requested that the U.S. Geological Survey (USGS), in collaboration with Chapman University, measure arsenic (As) and other geochemical constituents in soils and tailings at the mine site and in stream sediments downstream from the mine in Homewood Canyon and in Searles Valley (fig. 3). The request was made because initial sampling of the site by BLM staff indicated high concentrations of As in tailings and soils adjacent to the Ruth Mine. This report summarizes data obtained from field sampling of mine tailings and soils adjacent to the Ruth Mine and stream sediments downstream from the mine on June 7, 2009. Our results permit a preliminary assessment of the sources of As and associated chemical constituents that could potentially impact humans and biota.

  7. Utilizing hydrologic, statistical, and geochemical tools to assess uranium mobility in surface and near-surface environments

    NASA Astrophysics Data System (ADS)

    Naftz, D. L.; Walton-Day, K. E.; Fuller, C.; Dam, W. L.; Briggs, M. A.; Snyder, T.

    2015-12-01

    Legacy uranium (U) mining and processing activities have resulted in soil and water contamination on Federal, state, and tribal lands in the western United States. Sites include legacy mill sites associated with U extraction now managed by the Department of Energy and thousands of waste dumps associated with U exploration, mining, and processing. Recently (2012), over 400,000 hectares of federally managed land in northern Arizona was withdrawn from consideration of mining for a 20-year period to protect the Grand Canyon watershed from potentially adverse effects of U mineral exploration and development. Ore from active and recently active U mines in the Colorado Plateau, the Henry Mountains Complex, and the Arizona Strip is transported to the only currently (2015) active conventional mill site in the western United States, located in Utah. Previous and ongoing U.S. Geological Survey assessments to examine U mobility at a variety of legacy and active sites associated with ore exploration, extraction, and processing will be presented as field-scale examples. Topics associated with site investigations will include: (1) offsite migration of radionuclides associated with the operation of the White Mesa U mill; (2) long-term contaminant transport from legacy U waste dumps on Bureau of Land Management regulated land in Utah; (3) application of incremental soil sampling techniques to determine pre- and post-mining radionuclide levels associated with planned and operating U mines in northern Arizona; (4) application of fiber optic digital temperature sensing equipment to identify areas where shallow groundwater containing elevated U levels may be discharging to a river adjacent to a reclaimed mill site in central Wyoming; and (5) field-scale manipulation of groundwater chemistry to limit U migration from a legacy upgrader site in southeastern Utah.

  8. Lessons Learned: Tribal Community Engagement, Remediation and Restoration of a Uranium Mine Tailings Site, Navajo Nation - 12484

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Wadsworth, Donald K.; Hicks, Allison H.

    2012-07-01

    In May, 2011 New World Environmental Inc. was awarded a contract by the Navajo Nation Environmental Protection Agency to remediate an illegal radioactive waste disposal site located in the Navajo Nation. The initial scope included the excavation and shipment of an estimated 3,000 cubic yards of Uranium mine tailings and associated industrial waste. In this instance Stakeholders were supportive of the project, remediation and restoration, yet the movement of residual radioactive materials through tribal communities was a controversial issue. Other Stakeholder issues included site security, water sources for remediation activities, local residents' temporary re-location and care of livestock, right ofmore » way permissions and local workforce development. This presentation recaps the technical and non-technical issues encountered in the remediation and restoration the seven acre site and the outreach to surrounding communities. Cultural and equity issues resulting from historical problems associated with this and other sites in the immediate area and education and training. (authors)« less

  9. Source identification of uranium-containing materials at mine legacy sites in Portugal.

    PubMed

    Keatley, A C; Martin, P G; Hallam, K R; Payton, O D; Awbery, R; Carvalho, F P; Oliveira, J M; Silva, L; Malta, M; Scott, T B

    2018-03-01

    Whilst prior nuclear forensic studies have focused on identifying signatures to distinguish between different uranium deposit types, this paper focuses on providing a scientific basis for source identification of materials from different uranium mine sites within a single region, which can then be potentially used within nuclear forensics. A number of different tools, including gamma spectrometry, alpha spectrometry, mineralogy and major and minor elemental analysis, have been utilised to determine the provenance of uranium mineral samples collected at eight mine sites, located within three different uranium provinces, in Portugal. A radiation survey was initially conducted by foot and/or unmanned aerial vehicle at each site to assist sample collection. The results from each mine site were then compared to determine if individual mine sites could be distinguished based on characteristic elemental and isotopic signatures. Gamma and alpha spectrometry were used to differentiate between samples from different sites and also give an indication of past milling and mining activities. Ore samples from the different mine sites were found to be very similar in terms of gangue and uranium mineralogy. However, rarer minerals or specific impurity elements, such as calcium and copper, did permit some separation of the sites examined. In addition, classification rates using linear discriminant analysis were comparable to those in the literature. Crown Copyright © 2018. Published by Elsevier Ltd. All rights reserved.

  10. New Technique for Speciation of Uranium in Sediments Following Acetate-Stimulated Bioremediation

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    2011-06-22

    Acetate-stimulated bioremediation is a promising new technique for sequestering toxic uranium contamination from groundwater. The speciation of uranium in sediments after such bioremediation attempts remains unknown as a result of low uranium concentration, and is important to analyzing the stability of sequestered uranium. A new technique was developed for investigating the oxidation state and local molecular structure of uranium from field site sediments using X-Ray Absorption Spectroscopy (XAS), and was implemented at the site of a former uranium mill in Rifle, CO. Glass columns filled with bioactive Rifle sediments were deployed in wells in the contaminated Rifle aquifer and amendedmore » with a hexavalent uranium (U(VI)) stock solution to increase uranium concentration while maintaining field conditions. This sediment was harvested and XAS was utilized to analyze the oxidation state and local molecular structure of the uranium in sediment samples. Extended X-Ray Absorption Fine Structure (EXAFS) data was collected and compared to known uranium spectra to determine the local molecular structure of the uranium in the sediment. Fitting was used to determine that the field site sediments did not contain uraninite (UO{sub 2}), indicating that models based on bioreduction using pure bacterial cultures are not accurate for bioremediation in the field. Stability tests on the monomeric tetravalent uranium (U(IV)) produced by bioremediation are needed in order to assess the efficacy of acetate-stimulation bioremediation.« less

  11. Study on immobilization and migration of nuclide u in superficial soil of uranium tailings pond

    NASA Astrophysics Data System (ADS)

    Chang, Zhe; Zhou, Shukui

    2017-05-01

    The uranium tailings in southern China was used as the object of study to study the fixation and migration characteristics of nuclide U in shallow tailings. The results showed that the precipitation of tailings in the tailings soil was not linearly related to the depth during the acid rain leaching process. Tailings soil in the role of fixatives, when the lime as a fixative, the tailings of different soil uranium in 20 days after the re-precipitation. However, when lime and ammonium phosphate were used as fixing agents, the cumulative precipitation of U had a significant effect, and the migration of uranium was inhibited.

  12. In situ effects of metal contamination from former uranium mining sites on the health of the three-spined stickleback (Gasterosteus aculeatus, L.).

    PubMed

    Le Guernic, Antoine; Sanchez, Wilfried; Bado-Nilles, Anne; Palluel, Olivier; Turies, Cyril; Chadili, Edith; Cavalié, Isabelle; Delahaut, Laurence; Adam-Guillermin, Christelle; Porcher, Jean-Marc; Geffard, Alain; Betoulle, Stéphane; Gagnaire, Béatrice

    2016-08-01

    Human activities have led to increased levels of various pollutants including metals in aquatic ecosystems. Increase of metallic concentrations in aquatic environments represents a potential risk to exposed organisms, including fish. The aim of this study was to characterize the environmental risk to fish health linked to a polymetallic contamination from former uranium mines in France. This contamination is characterized by metals naturally present in the areas (manganese and iron), uranium, and metals (aluminum and barium) added to precipitate uranium and its decay products. Effects from mine releases in two contaminated ponds (Pontabrier for Haute-Vienne Department and Saint-Pierre for Cantal Department) were compared to those assessed at four other ponds outside the influence of mine tailings (two reference ponds/department). In this way, 360 adult three-spined sticklebacks (Gasterosteus aculeatus) were caged for 28 days in these six ponds before biomarker analyses (immune system, antioxidant system, biometry, histology, DNA integrity, etc.). Ponds receiving uranium mine tailings presented higher concentrations of uranium, manganese and aluminum, especially for the Haute-Vienne Department. This uranium contamination could explain the higher bioaccumulation of this metal in fish caged in Pontabrier and Saint-Pierre Ponds. In the same way, many fish biomarkers (antioxidant and immune systems, acetylcholinesterase activity and biometric parameters) were impacted by this environmental exposure to mine tailings. This study shows the interest of caging and the use of a multi-biomarker approach in the study of a complex metallic contamination.

  13. The paradox of uranium development: A Polanyian analysis of social movements surrounding the Pinon Ridge Uranium Mill

    NASA Astrophysics Data System (ADS)

    Malin, Stephanie A.

    Renewal of nuclear energy development has been proposed as one viable solution for reducing greenhouse gas emissions and impacts of climate change. This discussion became concrete as the first uranium mill proposed since the end of the Cold War, the Pinon Ridge Uranium Mill, received state permits in January 2011 to process uranium in southwest Colorado's Paradox Valley. Though environmental contamination from previous uranium activity caused one local community to be bulldozed to the ground, local support for renewed uranium activity emerges among local residents in communities like Nucla, Naturita, and Bedrock, Colorado. Regionally, however, a coalition of organized, oppositionbased grassroots groups fights the decision to permit the mill. Combined, these events allow social scientists a natural laboratory through which to view social repercussions of nuclear energy development. In this dissertation, I use a Polanyian theoretical framework to analyze social, political-economic, and environmental contexts of social movements surrounding PR Mill. My overarching research problem is: How might Polanyian double movement theory be applied to and made empirically testable within the social and environmental context of uranium development? I intended this analysis to inform energy policy debates regarding renewable energy. In Chapter 1, I found various forms of social dislocation lead to two divergent social movement outcomes. Economic social dislocation led to strong mill support among most local residents, according to archival, in-depth interview, and survey data. On the other hand, residents in regional communities experienced two other types of social dislocation -- another kind of economic dislocation, related to concern over boom-bust economies, and environmental health dislocations related to uranium exposure, creating conditions for a regional movement in opposition to PR Mill. In Chapter 2, I focus on regulations and find that two divergent social movements -- a support movement locally and a countermovement against the mill regionally -- emerge also as a result of strong faith in regulations, regulators, and Energy Fuels countered by marked distrust in regulations, regulators, and Energy Fuels, respectively. In Chapter 3, I advance Polanyi's double movement theory by comparing different emergent social movements surrounding uranium, showing that historically different circumstances surrounding uranium can help create conditions for divergent social movements.

  14. U.S.-Australia Civilian Nuclear Cooperation: Issues for Congress

    DTIC Science & Technology

    2010-09-30

    7 Uranium Mining and Milling ................................................................................................8...cycle begins with mining uranium ore and upgrading it to yellowcake. Because naturally occurring uranium lacks sufficient fissile 235U to make fuel for...enrichment, and finally fabrication into fuel elements. Australia exports its uranium after the mining and milling stage. Commercial enrichment services

  15. Compilation of data on the uranium and equivalent uranium content of samples analyzed by U.S. Geological Survey during a program of sampling mine, mill, and smelter products

    USGS Publications Warehouse

    Hall, Marlene Louise; Butler, Arthur Pierce

    1952-01-01

    In 1942 the Geological Survey began to collect, in response to a request made by the War Production Board, samples of mine, mill, and smelter products. About 1,400 such samples were collected and analyzed spectrographically for about 20 elements that were of strategic importance, in order to determine whether any of the products analyzed might be possible sources of some of the needed elements. When attention was directed to radioactive elements in 1943, most of the samples were scanned for radioactivity. Part of the work was done on behalf of the Division of Raw Materials of the Atomic Energy Commission. The sources, mine mill, smelter, or prospect, from which these samples were collected, the kind of material sampled, i.e. ores, concentrates, middlings, tailings, flue dusts, and so forth, and the radioactivity of the samples are listed in this report. Samples of the materials collected in the course of the Geological Survey’s investigations for uranium are excluded, but about 500 such samples were analyzed spectrographically for some or all of the same 20 elements sought in the samples that are the subject of this report. Most of the samples were tested only for their radioactivity, but a few were analyzed chemically for uranium. The radioactivity of many of the samples tested in the early screening was determined only qualitatively. Several samples were tested at one time, and if the count obtained did not exceed a predetermined minimum above background, the samples were not tested individually. If the count was more than this minimum, the samples were tested individually to identify the radioactive sample or samples and to obtain a quantitative value for the radioactivity. In general, the rough screening served as a basis for separating samples in which the radioactivity amount to less than 0.003 percent equivalent uranium from those in which it exceeded that amount. Some aspects of various phases of the investigation of radioactivity in these samples have been reported in various other reports, as follows.

  16. Comprehensive Evaluation of Soil Near Uranium Tailings, Beishan City, China.

    PubMed

    Xun, Yan; Zhang, Xinjia; Chaoliang, Chen; Luo, Xuegang; Zhang, Yu

    2018-06-01

    To evaluate the impact of uranium tailings on soil composition and soil microbial, six soil samples at different distance from the uranium tailings (Beishan City, China) were collected for further analysis. Concentrations of radionuclides ( 238 U and 232 Th), heavy metals (Mn, Cd, Cr, Ni, Zn, and Pb) and organochlorine pesticide were determined by ICP-MS and GC, they were significantly higher than those of the control. And the Average Well Color Development as well as the Shannon, the Evenness, and the Simpson index were calculated to evaluate the soil microbial diversity. The carbon utilization model of soil microbial community was also analyzed by Biolog-eco. All results indicated that uranium tailings leaded to excessive radionuclides and heavy metals, and decreased the diversity of the soil microbial community. Our study will provide a valuable basis for soil quality evaluation around uranium tailing repositories and lay a foundation for the management and recovery of uranium tailings.

  17. Biological pathways of exposure and ecotoxicity values for uranium and associated radionuclides: Chapter D in Hydrological, geological, and biological site characterization of breccia pipe uranium deposits in Northern Arizona

    USGS Publications Warehouse

    Hinck, Jo E.; Linder, Greg L.; Finger, Susan E.; Little, Edward E.; Tillitt, Donald E.; Kuhne, Wendy

    2010-01-01

    This chapter compiles available chemical and radiation toxicity information for plants and animals from the scientific literature on naturally occurring uranium and associated radionuclides. Specifically, chemical and radiation hazards associated with radionuclides in the uranium decay series including uranium, thallium, thorium, bismuth, radium, radon, protactinium, polonium, actinium, and francium were the focus of the literature compilation. In addition, exposure pathways and a food web specific to the segregation areas were developed. Major biological exposure pathways considered were ingestion, inhalation, absorption, and bioaccumulation, and biota categories included microbes, invertebrates, plants, fishes, amphibians, reptiles, birds, and mammals. These data were developed for incorporation into a risk assessment to be conducted as part of an environmental impact statement for the Bureau of Land Management, which would identify representative plants and animals and their relative sensitivities to exposure of uranium and associated radionuclides. This chapter provides pertinent information to aid in the development of such an ecological risk assessment but does not estimate or derive guidance thresholds for radionuclides associated with uranium. Previous studies have not attempted to quantify the risks to biota caused directly by the chemical or radiation releases at uranium mining sites, although some information is available for uranium mill tailings and uranium mine closure activities. Research into the biological impacts of uranium exposure is strongly biased towards human health and exposure related to enriched or depleted uranium associated with the nuclear energy industry rather than naturally occurring uranium associated with uranium mining. Nevertheless, studies have reported that uranium and other radionuclides can affect the survival, growth, and reproduction of plants and animals. Exposure to chemical and radiation hazards is influenced by a plant’s or an animal’s life history and surrounding environment. Various species of plants, invertebrates, fishes, amphibians, reptiles, birds, and mammals found in the segregation areas that are considered species of concern by State and Federal agencies were included in the development of the site-specific food web. The utilization of subterranean habitats (burrows in uranium-rich areas, burrows in waste rock piles or reclaimed mining areas, mine tunnels) in the seasonally variable but consistently hot, arid environment is of particular concern in the segregation areas. Certain species of reptiles, amphibians, birds, and mammals in the segregation areas spend significant amounts of time in burrows where they can inhale or ingest uranium and other radionuclides through digging, eating, preening, and hibernating. Herbivores may also be exposed though the ingestion of radionuclides that have been aerially deposited on vegetation. Measured tissues concentrations of uranium and other radionuclides are not available for any species of concern in the segregation areas. The sensitivity of these animals to uranium exposure is unknown based on the existing scientific literature, and species-specific uranium presumptive effects levels were only available for two endangered fish species known to inhabit the segregation areas. Overall, the chemical toxicity data available for biological receptors of concern were limited, although chemical and radiation toxicity guidance values are available from several sources. However, caution should be used when directly applying these values to northern Arizona given the unique habitat and life history strategies of biological receptors in the segregation areas and the fact that some guidance values are based on models rather than empirical (laboratory or field) data. No chemical toxicity information based on empirical data is available for reptiles, birds, or wild mammals; therefore, the risks associated with uranium and other radionuclides are unknown for these biota.

  18. Comparison of Grab, Air, and Surface Results for Radiation Site Characterization

    NASA Astrophysics Data System (ADS)

    Glassford, Eric Keith

    2011-12-01

    The use of proper sampling methods and sample types for evaluating sites believed to be contaminated with radioactive materials is necessary to avoid misrepresenting conditions at the site. This study was designed to investigate if the site characterization, based upon uranium contamination measured in different types of samples, is dependent upon the mass of the sample collected. A bulk sample of potentially contaminated interior dirt was collected from an abandoned metal processing mill that rolled uranium between 1948 and 1956. The original mill dates from 1910 and has a dirt floor. The bulk sample was a mixture of dirt, black and yellow particles of metal dust, and small fragments of natural debris. Small mass (approximately 0.75 grams (g)) and large mass (approximately 70g) grab samples were prepared from the bulk sample material to simulate collection of a "grab" type sample. Air sampling was performed by re-suspending a portion of the bulk sample material using a vibration table to simulate airborne contamination that might be present during site remediation. Additionally, samples of removable contaminated surface dust were collected on 47 mm diameter filter paper by wiping the surfaces of the exposure chamber used to resuspend the bulk material. Certified reference materials, one containing a precisely known quantity of U 3O8 and one containing a known quantity of natural uranium, were utilized to calibrate the gamma spectrometry measurement system. Non-destructive gamma spectrometry measurements were used to determine the content of uranium-235 (235U) at 185 keV and 143 keV, thorium-234 (234Th) at 63 keV, and protactinium-234m (234mPa) at 1001 keV in each sample. Measurement of natural uranium in small, 1 g samples is usually accomplished by radiochemical analysis in order to measure alpha particles emitted by 238U, 235U, and 234U. However, uranium in larger bulk samples can also be measured non-destructively using gamma spectrometry to detect the low energy photons from 234Th and 234mPa, the short-lived decay products of 238U, and 235U. Two sided t-tests and coefficient of variation were used to compare sampling types. The large grab samples had the lowest calculated coefficient of variation results for activity and atom percentage. The wipe samples had the highest calculated coefficient of variation of mean specific activity (dis/sec/g) for all three energies. The air filter samples had the highest coefficient of variation calculation for mean atom percentage, for both uranium isotopes examined. The data indicated that the large mass sample was the most effective at characterizing the rolling mill radioactive site conditions, since this would indicate which samples had the smallest variations compared to the mean. Additionally, measurement results of natural uranium in the samples indicate that the distribution of radioactive contamination at the sampling location is most likely non-homogeneous and that the size of the sample collected and analyzed must be sufficiently large to insure that the analytical results are truly representative of the activity present.

  19. U.S. Department of Energy Office of Legacy Management's Tribal Interactions - 12513

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Gil, April; Shafer, David; Elmer, John

    2012-07-01

    Effective government-to-government interactions with tribal nations and maintaining stakeholder relations with members of tribes are increasingly important to the U.S. Department of Energy (DOE) Office of Legacy Management (LM). As of October 2011, LM was responsible for long-term surveillance and maintenance of 87 sites and facilities in the continental U.S. and Puerto Rico, including some sites on tribal lands. The sites on tribal lands can affect natural resources that are managed or used by tribes, or the sites can potentially affect areas of cultural significance to tribal nations in Alaska, Arizona, Colorado, New Mexico, Utah, Washington, and Wyoming. Tribes aremore » separate sovereign governments recognized in the U.S. Constitution and are significant stakeholders for LM sites. The tribes are individual nations with diverse histories, cultures, customs, religions, and laws. LM has regular communication with the affected tribes to inform members of issues, to allow the tribe to participate in decision making, to provide technical reviews, and to ensure tribal concerns are addressed. Four LM sites are in the Navajo Nation. Three of those sites contain uranium mill tailings disposal cells regulated under long-term surveillance and maintenance programs that require monitoring and annual inspections. The fourth site was remediated but still has a groundwater plume that LM is responsible for. DOE and LM have worked with the Navajo Nation for almost 30 years on technical issues and to ensure tribal concerns are addressed. (authors)« less

  20. Uranium and its decay products in samples contaminated with uranium mine and mill waste

    NASA Astrophysics Data System (ADS)

    Benedik, L.; Klemencic, H.; Repinc, U.; Vrecek, P.

    2003-05-01

    The routine determination of the activity concentrations of uranium isotopes (^{238}U, ^{235}U and ^{234}U), thorium isotopes (^{212}Th, ^{230}TI, and ^{228}Th), ^{231}Pa, ^{226}Ra, ^{210}Pb and ^{210}Po in the environment is one of the most important tasks in uranium mining areas. Natural radionuclides contribute negligibly to the extemal radiation dose, but in the case of ingestion or inhalation can represent a very serious hazard. The objective of this study was to determine the activities of uranium and its decay products ^{230}Th, ^{231}Pa, ^{226}Ra, ^{210}Pb and ^{210}Po in sediments and water below sources of contamination (uranium mine, disposal sites and individual inflows) using gamma and alpha spectrometry, beta counting, the liquid scintillation technique and radiochemical neutron activation analysis.

  1. U.S.-Australia Civilian Nuclear Cooperation: Issues for Congress

    DTIC Science & Technology

    2010-12-01

    Enrichment.......................................................................................................7 Uranium Mining and Milling...Issues for Congress Congressional Research Service 7 The nuclear fuel cycle begins with mining uranium ore and upgrading it to yellowcake. Because...uranium after the mining and milling stage. Commercial enrichment services are available in the United States, Europe, Russia, and Japan. Fuel

  2. 1. VIEW NORTH OF PARADISE MILL FOUNDATION AND TAILINGS (FEATURE ...

    Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

    1. VIEW NORTH OF PARADISE MILL FOUNDATION AND TAILINGS (FEATURE P-7). PHOTO TAKEN FROM MERCURY RETORT. (OCTOBER, 1995) - McCormick Group Mine, Paradise Mill, East slope of Buckskin Mountain, Paradise Valley, Humboldt County, NV

  3. Evaluation of residual uranium contamination in the dirt floor of an abandoned metal rolling mill.

    PubMed

    Glassford, Eric; Spitz, Henry; Lobaugh, Megan; Spitler, Grant; Succop, Paul; Rice, Carol

    2013-02-01

    A single, large, bulk sample of uranium-contaminated material from the dirt floor of an abandoned metal rolling mill was separated into different types and sizes of aliquots to simulate samples that would be collected during site remediation. The facility rolled approximately 11,000 tons of hot-forged ingots of uranium metal approximately 60 y ago, and it has not been used since that time. Thirty small mass (≈ 0.7 g) and 15 large mass (≈ 70 g) samples were prepared from the heterogeneously contaminated bulk material to determine how measurements of the uranium contamination vary with sample size. Aliquots of bulk material were also resuspended in an exposure chamber to produce six samples of respirable particles that were obtained using a cascade impactor. Samples of removable surface contamination were collected by wiping 100 cm of the interior surfaces of the exposure chamber with 47-mm-diameter fiber filters. Uranium contamination in each of the samples was measured directly using high-resolution gamma ray spectrometry. As expected, results for isotopic uranium (i.e., U and U) measured with the large-mass and small-mass samples are significantly different (p < 0.001), and the coefficient of variation (COV) for the small-mass samples was greater than for the large-mass samples. The uranium isotopic concentrations measured in the air and on the wipe samples were not significantly different and were also not significantly different (p > 0.05) from results for the large- or small-mass samples. Large-mass samples are more reliable for characterizing heterogeneously distributed radiological contamination than small-mass samples since they exhibit the least variation compared to the mean. Thus, samples should be sufficiently large in mass to insure that the results are truly representative of the heterogeneously distributed uranium contamination present at the facility. Monitoring exposure of workers and the public as a result of uranium contamination resuspended during site remediation should be evaluated using samples of sufficient size and type to accommodate the heterogeneous distribution of uranium in the bulk material.

  4. 76 FR 45300 - Notice of Issuance of Materials License SUA-1597 and Record of Decision for Uranerz Energy...

    Federal Register 2010, 2011, 2012, 2013, 2014

    2011-07-28

    ... considered but eliminated from detailed analysis include conventional uranium mining and milling, conventional mining and heap leach processing, alternative site location, alternate lixiviants, and alternate...'s Agencywide Document Access and Management System (ADAMS), which provides text and image files of...

  5. Plant/soil concentration ratios of SSWRa for contrasting sites around an active U mine-mill

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Ibrahim, S.A.; Whicker, F.W.

    Concentrations of 226Ra were determined in native vegetation and underlying substrate (soil and tailings) at various sites around a conventional open-pit, acid leach U production operation in Wyoming. Plant/soil concentration ratios (CRs) for 226Ra were estimated for various sites, including weathered tailings; a tailings impoundment shoreline; downwind from exposed tailings; a mine overburden reclamation area; and several background locations. Radium-226 concentrations for vegetation and substrate and CR values from the perturbed sites were elevated above background. The highest vegetation concentration (1.3 Bq g-1) was found in a grass which had invaded exposed, weathered tailings. Levels of 226Ra in soil andmore » vegetation and CR values decreased with distance from the tailings impoundment edge. CR values varied significantly among sites, but few differences were found between plant species groups. The observed CR values ranged from 0.07 at the background and reclamation areas to 0.4 downwind from the tailings area. Average CR values for plants growing on exposed tailings and within one meter from the impoundment edge were 0.15 and 0.3, respectively. CR values of 226Ra for plants on tailings substrates were comparatively low in contrast to other radionuclides in the U chain. We speculate that in the case of sulfuric acid leached tailings-derived material, 226Ra is sequestered as sulfate, which is highly insoluble relative to the sulfates of the other elements (e.g., U and Th) resulting in reduced availability for plant uptake.« less

  6. Bacterial diversity and composition of an alkaline uranium mine tailings-water interface.

    PubMed

    Khan, Nurul H; Bondici, Viorica F; Medihala, Prabhakara G; Lawrence, John R; Wolfaardt, Gideon M; Warner, Jeff; Korber, Darren R

    2013-10-01

    The microbial diversity and biogeochemical potential associated with a northern Saskatchewan uranium mine water-tailings interface was examined using culture-dependent and -independent techniques. Morphologically-distinct colonies from uranium mine water-tailings and a reference lake (MC) obtained using selective and non-selective media were selected for 16S rRNA gene sequencing and identification, revealing that culturable organisms from the uranium tailings interface were dominated by Firmicutes and Betaproteobacteria; whereas, MC organisms mainly consisted of Bacteroidetes and Gammaproteobacteria. Ion Torrent (IT) 16S rRNA metagenomic analysis carried out on extracted DNA from tailings and MC interfaces demonstrated the dominance of Firmicutes in both of the systems. Overall, the tailings-water interface environment harbored a distinct bacterial community relative to the MC, reflective of the ambient conditions (i.e., total dissolved solids, pH, salinity, conductivity, heavy metals) dominating the uranium tailings system. Significant correlations among the physicochemical data and the major bacterial groups present in the tailings and MC were also observed. Presence of sulfate reducing bacteria demonstrated by culture-dependent analyses and the dominance of Desulfosporosinus spp. indicated by Ion Torrent analyses within the tailings-water interface suggests the existence of anaerobic microenvironments along with the potential for reductive metabolic processes.

  7. Extraction of uranium from tailings by sulfuric acid leaching with oxidants

    NASA Astrophysics Data System (ADS)

    Huang, Jing; Li, Mi; Zhang, Xiaowen; Huang, Chunmei; Wu, Xiaoyan

    2017-06-01

    Recovery of uranium have been performed by leaching uranium-containing tailings in sulfuric acid system with the assistance of HF, HClO4, H2O2 and MnO2. The effect of reagent dosage, sulfuric acid concentration, Liquid/solid ratio, reaction temperature and particle size on the leaching of uranium were investigated. The results show that addiction of HF, HClO4, H2O2 and MnO2 significantly increased the extraction of uranium under 1M sulphuric acid condition and under the optimum reaction conditions a dissolution fraction of 85% by HClO4, 90% by HF, 95% by H2O2 can be reached respectively. The variation of technological mineralogy properites of tailings during leaching process show that the assistants can break gangue effectively. These observations suggest that optimum oxidants could potentially influence the extraction of uranium from tailings even under dilute acid condition.

  8. Safeguards on uranium ore concentrate? the impact of modern mining and milling process

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Francis, Stephen

    2013-07-01

    Increased purity in uranium ore concentrate not only raises the question as to whether Safeguards should be applied to the entirety of uranium conversion facilities, but also as to whether some degree of coverage should be moved back to uranium ore concentrate production at uranium mining and milling facilities. This paper looks at uranium ore concentrate production across the globe and explores the extent to which increased purity is evident and the underlying reasons. Potential issues this increase in purity raises for IAEA's strategy on the Starting Point of Safeguards are also discussed.

  9. 25. VIEW OF MILL FROM UPPER TAILINGS POND. SHOWS ROASTER ...

    Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

    25. VIEW OF MILL FROM UPPER TAILINGS POND. SHOWS ROASTER ON LEFT EDGE OF VIEW. THE SECONDARY THICKENER No. 7 IS OFF VIEW TO THE RIGHT. - Bald Mountain Gold Mill, Nevada Gulch at head of False Bottom Creek, Lead, Lawrence County, SD

  10. OVERVIEW OF CYANIDE PLANT FOUNDATIONS, ZINC BOXES, TANKS, AND TAILINGS ...

    Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

    OVERVIEW OF CYANIDE PLANT FOUNDATIONS, ZINC BOXES, TANKS, AND TAILINGS PILES, LOOKING NORTHEAST. THE LOWER TRAM TERMINAL AND MILL SITE IS AT TOP CENTER IN THE DISTANCE. THE DARK SPOT JUST BELOW THE TRAM TERMINAL ARE REMAINS OF THE DEWATERING BUILDING. THE MAIN ACCESS ROAD IS AT UPPER LEFT. THE FOUNDATIONS AT CENTER SUPPORTED SIX 25 FT. OR GREATER DIAMETER SETTLING TANKS WHERE TAILINGS FROM THE MILL SETTLED IN A CYANIDE SOLUTION IN ORDER TO RECLAIM ANY GOLD CONTENT. THE PREGNANT SOLUTION WAS THEN RUN THROUGH THE ZINC BOXES ON THE GROUND AT CENTER RIGHT, WHERE ZINC SHAVINGS WERE INTRODUCED, CAUSING THE GOLD TO PRECIPITATE OUT OF THE CYANIDE SOLUTION, WHICH COULD BE USED AGAIN. THE FLAT AREA IN THE FOREGROUND WITH THE TANK AND TANK HOOPS IS THE FOOTPRINT OF A LARGE BUILDING WHERE THE PRECIPITATION AND FURTHER FILTERING AND FINAL CASTING TOOK PLACE. - Keane Wonder Mine, Park Route 4 (Daylight Pass Cutoff), Death Valley Junction, Inyo County, CA

  11. Radiochronological Age of a Uranium Metal Sample from an Abandoned Facility

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Meyers, L A; Williams, R W; Glover, S E

    2012-03-16

    A piece of scrap uranium metal bar buried in the dirt floor of an old, abandoned metal rolling mill was analyzed using multi-collector inductively coupled plasma mass spectroscopy (MC-ICP-MS). The mill rolled uranium rods in the 1940s and 1950s. Samples of the contaminated dirt in which the bar was buried were also analyzed. The isotopic composition of uranium in the bar and dirt samples were both the same as natural uranium, though a few samples of dirt also contained recycled uranium; likely a result of contamination with other material rolled at the mill. The time elapsed since the uranium metalmore » bar was last purified can be determined by the in-growth of the isotope {sup 230}Th from the decay of {sup 234}U, assuming that only uranium isotopes were present in the bar after purification. The age of the metal bar was determined to be 61 years at the time of this analysis and corresponds to a purification date of July 1950 {+-} 1.5 years.« less

  12. The yellowed archives of yellowcake.

    PubMed Central

    Silver, K

    1996-01-01

    Extensive historical documentation of exposures and releases at government-owned energy facilities is a unique and valuable resource for analyzing and communicating health risks. Facilities at all stages of the atomic fuel cycle were the subject of numerous industrial hygiene, occupational health, and environmental assessments during the Cold War period. Uranium mines and mills on the Colorado Plateau were investigated as early as the 1940s. One such facility was the mill in Monticello, Utah, which began operation as a vanadium extraction plant in 1943 and was later adapted to recover uranium from carnotite ores. The mill ceased operation in 1960. The site was added to the federal Superfund list in 1986. ATSDR held public availability sessions in 1993 as part of its public health assessment process, at which several former mill workers voiced health concerns. An extensive literature search yielded several industrial hygiene evaluations of the Monticello mill and health studies that included Monticello workers, only two of which had been published in the peer-reviewed literature. In combination with the broader scientific literature, these historical reports provide a partial basis for responding to mill workers' contemporary health concerns. The strengths and limitations of the available exposure data for analytical epidemiologic studies and dose reconstruction are discussed. As an interim measure, the available historical documentation may be especially helpful in communicating about health risks with workers and communities in ways that acknowledge the historical context of their experience. Images p116-a p117-a p118-a PMID:8606907

  13. DETAIL VIEW OF CLASSIFIER, TAILINGS LAUNDER TROUGH, LINE SHAFTS, AND ...

    Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

    DETAIL VIEW OF CLASSIFIER, TAILINGS LAUNDER TROUGH, LINE SHAFTS, AND CONCENTRATION TABLES, LOOKING SOUTHWEST. SLURRY EXITING THE BALL MILL WAS COLLECTED IN AN AMALGAMATION BOX (MISSING) FROM THE END OF THE MILL, AND INTRODUCED INTO THE CLASSIFIER. THE TAILINGS LAUDER IS ON THE GROUND AT LOWER RIGHT. THE LINE SHAFTING ABOVE PROVIDED POWER TO THE CONCENTRATION TABLES BELOW AT CENTER RIGHT. - Gold Hill Mill, Warm Spring Canyon Road, Death Valley Junction, Inyo County, CA

  14. 2010 Five-Year Plan: Assessment of Health and Environmental Impacts of Uranium Mining and Milling

    EPA Pesticide Factsheets

    The five-year plan is intended to compile all activities contributing to the identification and cleanup of legacy uranium milling and mining activities in the Grants Mining District in the State of New Mexico.

  15. Remedial Action Plan and site design for stabilization of the inactive uranium mill tailings site at Durango, Colorado: Attachment 5, Dewatering report. Revised final report

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1991-12-01

    This report provides an update on dewatering activities at the Durango disposal embankment and presents recommendations for the work required to complete the closure of the cell in 1990 (Section 2). In October 1989, test pit investigations were performed and a toe trench was excavated at the eastern slope of the disposal embankment. A description and results of the test pit investigations along with the implications . of the results relative to the over . all dewatering effort are discussed in Sections 3 through 5. Installation and performance of the 17-well dewatering system were previously described in` the ``StatusReport onmore » Dewatering of Disposal Embankment`` issued in September, 1989. Additional studies are still on-going and are described in Section 6. Laboratory analysis continues on samples taken from the test pits. TAC`s characterization of the hydrogeological conditions at the Durango site is also proceeding. Results of these studies will be presented in subsequent reports. Appendices A and B present construction details of the well point system, toe trench and holding pond. Appendix C summarizes the performance-of the 17 pumping wells prior to winter shutdown and provides information on pumping rates, drawdowns, and disposition of the wells. Appendix D outlines the chronology of the dewatering effort to date.« less

  16. Nuclear regulatory legislation: 102d Congress. Volume 1, No. 2

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1993-10-01

    This document is a compilation of nuclear regulatory legislation and other relevant material through the 102d Congress, 2d Session. This compilation has been prepared for use as a resource document, which the NRC intends to update at the end of every Congress. The contents of NUREG-0980 include: The Atomic Energy Act of 1954, as amended; Energy Reorganization Act of 1974, as amended, Uranium Mill Tailings Radiation Control Act of 1978; Low-Level Radioactive Waste Policy Act; Nuclear Waste Policy Act of 1982; and NRC Authorization and Appropriations Acts. Other materials included are statutes and treaties on export licensing, nuclear non-proliferation, andmore » environmental protection.« less

  17. Nuclear regulatory legislation, 102d Congress. Volume 2, No. 2

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1993-10-01

    This document is a compilation of nuclear regulatory legislation and other relevant material through the 102d Congress, 2d Session. This compilation has been prepared for use as a resource document, which the NRC intends to update at the end of every Congress. The contents of NUREG-0980 include The Atomic Energy Act of 1954, as amended; Energy Reorganization Act of 1974, as amended, Uranium Mill Tailings Radiation Control Act of 1978; Low-Level Radioactive Waste Policy Act; Nuclear Waste Policy Act of 1982; and NRC Authorization and Appropriations Acts. Other materials included are statutes and treaties on export licensing, nuclear non-proliferation, andmore » environmental protection.« less

  18. 24. VIEW OF MILL FROM UPPER TAILINGS POND (NORTH). ROASTER ...

    Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

    24. VIEW OF MILL FROM UPPER TAILINGS POND (NORTH). ROASTER ON LEFT WITH ELEVATOR/CRUSHED ORE BIN TOWER TO RIGHT. MAIN MILL BUILDING IN CENTER WITH THICKENER ADDITION TO RIGHT. MACHINE SHOP ON CRUDE ORE BIN TERRACE ABOVE ROASTER. THE LOCATION OF THE 100,000 GALLON MILL WATER TANK CAN BE SEEN AT THE CENTER RIGHT NEAR THE TOP OF THE MOUNTAIN. - Bald Mountain Gold Mill, Nevada Gulch at head of False Bottom Creek, Lead, Lawrence County, SD

  19. 165. VIEW OF MILL FROM UPPER TAILINGS POND (NORTH). ROASTER ...

    Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

    165. VIEW OF MILL FROM UPPER TAILINGS POND (NORTH). ROASTER ON LEFT WITH ELEVATOR/CRUSHED ORE BIN TOWER TO RIGHT. MAIN MILL BUILDING IN CENTER WITH THICKENER ADDITION TO RIGHT. MACHINE SHOP ON CRUDE ORE BIN TERRACE ABOVE ROASTER. THE LOCATION OF THE 100,000 GALLON MILL WATER TANK CAN BE SEEN AT THE CENTER RIGHT NEAR THE TOP OF THE MOUNTAIN - Bald Mountain Gold Mill, Nevada Gulch at head of False Bottom Creek, Lead, Lawrence County, SD

  20. Results of the survey activities and mobile gamma scanning in Monticello, Utah

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Little, C.A.; Berven, B.A.

    The town of Monticello, Utah, was once the site of an active mill which processed vanadium ore (1942 to 1948), and uranium ore (1948 to 1960). Properties in the vicinity of that mill have become contaminated with radioactive material from ore processing. The Radiological Survey Activities (RASA) group at Oak Ridge National Laboratory (ORNL) was requested by the Division of Remedial Action Projects (DRAP) in the Department of Energy (DOE) to: (1) identify potentially contaminated properties; (2) assess natural background radiation levels; and (3) rapidly assess the magnitude, extent, and type (i.e. ore, tailings, etc.) of contamination present on thesemore » properties (if any). This survey was conducted by RASA during April 1983. In addition to the 114 properties previously identified from historical information, the ORNL mobile gamma scanning van located 36 new properties exhibiting anomalous gamma radiation levels. Onsite surveys were conducted on 145 of the 150 total properties identified either historically or with the gamma scanning van. Of these 145 properties, 122 of them appeared to have some type of contaminated material present on them; however, only 48 appeared to be contaminated to the extent where they were in excess of Environmental Protection Agency (EPA) criteria (40 CFR 192). Twenty-one other properties were recommended for additional investigation (indoor gamma scanning and radon daughter measurements); of these, only ten required further analysis. This report provides the detailed data and analyses related to the radiological survey efforts performed by ORNL in Monticello, Utah.« less

  1. Process for producing enriched uranium having a .sup.235 U content of at least 4 wt. % via combination of a gaseous diffusion process and an atomic vapor laser isotope separation process to eliminate uranium hexafluoride tails storage

    DOEpatents

    Horton, James A.; Hayden, Jr., Howard W.

    1995-01-01

    An uranium enrichment process capable of producing an enriched uranium, having a .sup.235 U content greater than about 4 wt. %, is disclosed which will consume less energy and produce metallic uranium tails having a lower .sup.235 U content than the tails normally produced in a gaseous diffusion separation process and, therefore, eliminate UF.sub.6 tails storage and sharply reduce fluorine use. The uranium enrichment process comprises feeding metallic uranium into an atomic vapor laser isotope separation process to produce an enriched metallic uranium isotopic mixture having a .sup.235 U content of at least about 2 wt. % and a metallic uranium residue containing from about 0.1 wt. % to about 0.2 wt. % .sup.235 U; fluorinating this enriched metallic uranium isotopic mixture to form UF.sub.6 ; processing the resultant isotopic mixture of UF.sub.6 in a gaseous diffusion process to produce a final enriched uranium product having a .sup.235 U content of at least 4 wt. %, and up to 93.5 wt. % or higher, of the total uranium content of the product, and a low .sup.235 U content UF.sub.6 having a .sup.235 U content of about 0.71 wt. % of the total uranium content of the low .sup.235 U content UF.sub.6 ; and converting this low .sup.235 U content UF.sub.6 to metallic uranium for recycle to the atomic vapor laser isotope separation process.

  2. Process for producing enriched uranium having a {sup 235}U content of at least 4 wt. % via combination of a gaseous diffusion process and an atomic vapor laser isotope separation process to eliminate uranium hexafluoride tails storage

    DOEpatents

    Horton, J.A.; Hayden, H.W. Jr.

    1995-05-30

    An uranium enrichment process capable of producing an enriched uranium, having a {sup 235}U content greater than about 4 wt. %, is disclosed which will consume less energy and produce metallic uranium tails having a lower {sup 235}U content than the tails normally produced in a gaseous diffusion separation process and, therefore, eliminate UF{sub 6} tails storage and sharply reduce fluorine use. The uranium enrichment process comprises feeding metallic uranium into an atomic vapor laser isotope separation process to produce an enriched metallic uranium isotopic mixture having a {sup 235} U content of at least about 2 wt. % and a metallic uranium residue containing from about 0.1 wt. % to about 0.2 wt. % {sup 235} U; fluorinating this enriched metallic uranium isotopic mixture to form UF{sub 6}; processing the resultant isotopic mixture of UF{sub 6} in a gaseous diffusion process to produce a final enriched uranium product having a {sup 235}U content of at least 4 wt. %, and up to 93.5 wt. % or higher, of the total uranium content of the product, and a low {sup 235}U content UF{sub 6} having a {sup 235}U content of about 0.71 wt. % of the total uranium content of the low {sup 235}U content UF{sub 6}; and converting this low {sup 235}U content UF{sub 6} to metallic uranium for recycle to the atomic vapor laser isotope separation process. 4 figs.

  3. 28 CFR 79.51 - Definitions.

    Code of Federal Regulations, 2011 CFR

    2011-07-01

    ... includes in situ lung cancers. (m) Readily available documentation means documents in the possession... or functional damage to the kidney tubules that results in renal disease and dysfunction. (g) Miller or uranium mill worker means a person who operated or otherwise worked in a uranium mill. (h...

  4. 28 CFR 79.51 - Definitions.

    Code of Federal Regulations, 2014 CFR

    2014-07-01

    ... includes in situ lung cancers. (m) Readily available documentation means documents in the possession... or functional damage to the kidney tubules that results in renal disease and dysfunction. (g) Miller or uranium mill worker means a person who operated or otherwise worked in a uranium mill. (h...

  5. Sustainability of uranium mining and milling: toward quantifying resources and eco-efficiency.

    PubMed

    Mudd, Gavin M; Diesendorf, Mark

    2008-04-01

    The mining of uranium has long been a controversial public issue, and a renewed debate has emerged on the potential for nuclear power to help mitigate against climate change. The central thesis of pro-nuclear advocates is the lower carbon intensity of nuclear energy compared to fossil fuels, although there remains very little detailed analysis of the true carbon costs of nuclear energy. In this paper, we compile and analyze a range of data on uranium mining and milling, including uranium resources as well as sustainability metrics such as energy and water consumption and carbon emissions with respect to uranium production-arguably the first time for modern projects. The extent of economically recoverable uranium resources is clearly linked to exploration, technology, and economics but also inextricably to environmental costs such as energy/water/chemicals consumption, greenhouse gas emissions, and social issues. Overall, the data clearly show the sensitivity of sustainability assessments to the ore grade of the uranium deposit being mined and that significant gaps remain in complete sustainability reporting and accounting. This paper is a case study of the energy, water, and carbon costs of uranium mining and milling within the context of the nuclear energy chain.

  6. Anaerobic bioremediation of hexavalent uranium in groundwater by reductive precipitation with methanogenic granular sludge.

    PubMed

    Tapia-Rodriguez, Aida; Luna-Velasco, Antonia; Field, Jim A; Sierra-Alvarez, Reyes

    2010-04-01

    Uranium has been responsible for extensive contamination of groundwater due to releases from mill tailings and other uranium processing waste. Past evidence has confirmed that certain bacteria can enzymatically reduce soluble hexavalent uranium (U(VI)) to insoluble tetravalent uranium (U(IV)) under anaerobic conditions in the presence of appropriate electron donors. This paper focuses on the evaluation of anaerobic granular sludge as a source of inoculum for the bioremediation of uranium in water. Batch experiments were performed with several methanogenic anaerobic granular sludge samples and different electron donors. Abiotic controls consisting of heat-killed inoculum and non-inoculated treatments confirmed the biological removal process. In this study, unadapted anaerobic granular sludge immediately reduced U(VI), suggesting an intrinsic capacity of the sludge to support this process. The high biodiversity of anaerobic granular sludge most likely accounts for the presence of specific microorganisms capable of reducing U(VI). Oxidation by O(2) was shown to resolubilize the uranium. This observation combined with X-ray diffraction evidence of uraninite confirmed that the removal during anaerobic treatment was due to reductive precipitation. The anaerobic removal activity could be sustained after several respikes of U(VI). The U(VI) removal was feasible without addition of electron donors, indicating that the decay of endogenous biomass substrates was contributing electron equivalents to the process. Addition of electron donors, such as H(2) stimulated the removal of U(VI) to varying degrees. The stimulation was greater in sludge samples with lower endogenous substrate levels. The present work reveals the potential application of anaerobic granular sludge for continuous bioremediation schemes to treat uranium-contaminated water. Copyright (c) 2009 Elsevier Ltd. All rights reserved.

  7. Analytical Results for 35 Mine-Waste Tailings Cores and Six Bed-Sediment Samples, and An Estimate of the Volume of Contaminated Material at Buckeye Meadow on Upper Basin Creek, Northern Jefferson County, Montana

    USGS Publications Warehouse

    Fey, David L.; Church, Stan E.; Finney, Christopher J.

    1999-01-01

    Metal-mining related wastes in the Boulder River basin study area in northern Jefferson County, Montana have been implicated in their detrimental effects on water quality with regard to acid-generation and toxic-metal solubilization. Flotation-mill tailings in the meadow below the Buckeye mine, hereafter referred to as the Buckeye mill-tailings site, have been identified as significant contributors to water quality degradation of Basin Creek, Montana. Basin Creek is one of three tributaries to the Boulder River in the study area; bed sediments and waters draining from the Buckeye mine have also been implicated. Geochemical analysis of 35 tailings cores and six bed-sediment samples was undertaken to determine the concentrations of Ag, As, Cd, Cu, Pb,and Zn present in these materials. These elements are environmentally significant, in that they can be toxic to fish and/or the invertebrate organisms that constitute their food. A suite of one-inch cores of dispersed flotation-mill tailings and underlying premining material was taken from a large, flat area north of Basin Creek near the site of the Buckeye mine. Thirty-five core samples were taken and divided into 204 subsamples. The samples were analyzed by ICP-AES (inductively coupled plasma-atomic emission spectroscopy) using a mixed-acid digestion. Results of the core analyses show that the elements listed above are present at moderate to very high concentrations (arsenic to 63,000 ppm, silver to 290 ppm, cadmium to 370 ppm, copper to 4,800 ppm, lead to 93,000 ppm, and zinc to 23,000 ppm). Volume calculations indicate that an estimated 8,400 metric tons of contaminated material are present at the site. Six bed-sediment samples were also subjected to the mixed-acid total digestion, and a warm (50°C) 2M HCl-1% H2O2 leach and analyzed by ICP-AES. Results indicate that bed sediments of Basin Creek are only slightly impacted by past mining above the Buckeye-Enterprise complex, moderately impacted at the upper (eastern) end of the tailings area, and heavily impacted at the lower (western) end of the area and downstream. The metals are mostly contained in the 2M HCl-1% H2O2 leachable phase, which are the hydrous amorphous iron- and manganese-hydroxide coatings on detrital sediment particles.

  8. Impact of Environmentally Based Chemical Hardness on Uranium Speciation and Toxicity in Six Aquatic Species

    PubMed Central

    Goulet, Richard R; Thompson, Patsy A; Serben, Kerrie C; Eickhoff, Curtis V

    2015-01-01

    Treated effluent discharge from uranium (U) mines and mills elevates the concentrations of U, calcium (Ca), magnesium (Mg), and sulfate (SO42–) above natural levels in receiving waters. Many investigations on the effect of hardness on U toxicity have been experiments on the combined effects of changes in hardness, pH, and alkalinity, which do not represent water chemistry downstream of U mines and mills. Therefore, more toxicity studies with water chemistry encountered downstream of U mines and mills are necessary to support predictive assessments of impacts of U discharge to the environment. Acute and chronic U toxicity laboratory bioassays were realized with 6 freshwater species in waters of low alkalinity, circumneutral pH, and a range of chemical hardness as found in field samples collected downstream of U mines and mills. In laboratory-tested waters, speciation calculations suggested that free uranyl ion concentrations remained constant despite increasing chemical hardness. When hardness increased while pH remained circumneutral and alkalinity low, U toxicity decreased only to Hyalella azteca and Pseudokirchneriella subcapitata. Also, Ca and Mg did not compete with U for the same uptake sites. The present study confirms that the majority of studies concluding that hardness affected U toxicity were in fact studies in which alkalinity and pH were the stronger influence. The results thus confirm that studies predicting impacts of U downstream of mines and mills should not consider chemical hardness. PMID:25475484

  9. Uranium Fate and Transport Modeling, Guterl Specialty Steel Site, New York - 13545

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Frederick, Bill; Tandon, Vikas

    2013-07-01

    The Former Guterl Specialty Steel Corporation Site (Guterl Site) is located 32 kilometers (20 miles) northeast of Buffalo, New York, in Lockport, Niagara County, New York. Between 1948 and 1952, up to 15,875 metric tons (35 million pounds) of natural uranium metal (U) were processed at the former Guterl Specialty Steel Corporation site in Lockport, New York. The resulting dust, thermal scale, mill shavings and associated land disposal contaminated both the facility and on-site soils. Uranium subsequently impacted groundwater and a fully developed plume exists below the site. Uranium transport from the site involves legacy on-site pickling fluid handling, themore » leaching of uranium from soil to groundwater, and the groundwater transport of dissolved uranium to the Erie Canal. Groundwater fate and transport modeling was performed to assess the transfer of dissolved uranium from the contaminated soils and buildings to groundwater and subsequently to the nearby Erie Canal. The modeling provides a tool to determine if the uranium contamination could potentially affect human receptors in the vicinity of the site. Groundwater underlying the site and in the surrounding area generally flows southeasterly towards the Erie Canal; locally, groundwater is not used as a drinking water resource. The risk to human health was evaluated outside the Guterl Site boundary from the possibility of impacted groundwater discharging to and mixing with the Erie Canal waters. This condition was evaluated because canal water is infrequently used as an emergency water supply for the City of Lockport via an intake located approximately 122 meters (m) (400 feet [ft]) southeast of the Guterl Site. Modeling was performed to assess whether mixing of groundwater with surface water in the Erie Canal could result in levels of uranium exceeding the U.S. Environmental Protection Agency (USEPA) established drinking water standard for total uranium; the Maximum Concentration Limit (MCL). Geotechnical test data indicate that the major portion of uranium in the soil will adsorb or remain bound to soil, yet leaching to groundwater appears as an on-site source. Soil leaching was modeled using low adsorption factors to replicate worst-case conditions where the uranium leaches to the groundwater. Results indicate that even after several decades, which is the period of time since uranium was processed at the Guterl Site, leaching from soil does not fully account for the currently observed levels of groundwater contamination. Modeling results suggest that there were historic releases of uranium from processing operations directly to the shallow fractured rock and possibly other geochemical conditions that have produced the current groundwater contamination. Groundwater data collected at the site between 1997 and 2011 do not indicate an increasing level of uranium in the main plume, thus the uranium adsorbed to the soil is in equilibrium with the groundwater geochemistry and transport conditions. Consequently, increases in the overall plume concentration or size are not expected. Groundwater flowing through fractures under the Guterl Site transports dissolved uranium from the site to the Erie Canal, where the groundwater has been observed to seep from the northern canal wall at some locations. The seeps discharge uranium at concentrations near or below the MCL to the Erie Canal. Conservative mixing calculations were performed using two worst-case assumptions: 1) the seeps were calculated as contiguous discharges from the Erie Canal wall and 2) the uranium concentration of the seepage is 274 micrograms per liter (μg/L) of uranium, which is the highest on-site uranium concentration in groundwater and nearly ten-fold the actual seep concentrations. The results indicate that uranium concentrations in the seep water would have to be more than 200 times greater than the highest observed on-site groundwater concentrations (or nearly 55,000 μg/L) to potentially exceed the drinking water standard (the MCL) for total uranium in the Erie Canal. (authors)« less

  10. Radioactivity Risk Assessment of Radon and Gamma Dose at One Uranium Tailings Pond in China

    NASA Astrophysics Data System (ADS)

    Lou, Yalong; Liu, Yong; Peng, Guowen; Zhao, Guodong; Zhang, Yan; Yang, Zhu

    2018-01-01

    A year-long monitoring of gamma radiation effective dose rate and radon concentration had been done in the reservoir area of one uranium tailings pond in Hunan province (The monitoring area included indoor and outdoor area of residential buildings and workshops, tailings dam slope). Afterwards, the annual effective radiation dose of the people in that radiation environment had been calculated based on the results of monitoring, as well as a radiation risk assessment. According to the assessment, gamma radiation effective dose rate and radon concentration in the monitoring area were low, and the annual effective radiation dose was far below the international standard (30mSv), which showed that the radiation would not put the people’s health at risk. However, the annual effective radiation dose of gamma was far above that of radon in the area of uranium tailings pond; therefore, it’s advisable to take quarantine measures in in the area of uranium tailings pond to keep the surrounding residents away from unnecessary ionizing radiation.

  11. Quantifying uranium transport rates and storage of fluvially eroded mine tailings from a historic mine site in the Grand Canyon Region

    NASA Astrophysics Data System (ADS)

    Skalak, K.; Benthem, A. J.; Walton-Day, K. E.; Jolly, G.

    2015-12-01

    The Grand Canyon region contains a large number of breccia pipes with economically viable uranium, copper, and silver concentrations. Mining in this region has occurred since the late 19th century and has produced ore and waste rock having elevated levels of uranium and other contaminants. Fluvial transport of these contaminants from mine sites is a possibility, as this arid region is susceptible to violent storms and flash flooding which might erode and mobilize ore or waste rock. In order to assess and manage the risks associated with uranium mining, it is important to understand the transport and storage rates of sediment and uranium within the ephemeral streams of this region. We are developing a 1-dimensional sediment transportation model to examine uranium transport and storage through a typical canyon system in this region. Our study site is Hack Canyon Mine, a uranium and copper mine site, which operated in the 1980's and is currently experiencing fluvial erosion of its waste rock repository. The mine is located approximately 40km upstream from the Colorado River and is in a deep, narrow canyon with a small watershed. The stream is ephemeral for the upper half of its length and sediment is primarily mobilized during flash flood events. We collected sediment samples at 110 locations longitudinally through the river system to examine the distribution of uranium in the stream. Samples were sieved to the sand size and below fraction (<2mm) and uranium was measured by gamma-ray spectroscopy. Sediment storage zones were also examined in the upper 8km of the system to determine where uranium is preferentially stored in canyon systems. This information will quantify the downstream transport of constituents associated with the Hack Canyon waste rock and contribute to understanding the risks associated with fluvial mobilization of uranium mine waste.

  12. Determination of the elemental concentration of uranium and thorium in the products and by-products of amang tin tailings process

    NASA Astrophysics Data System (ADS)

    Alnour, I. A.; Wagiran, H.; Ibrahim, N.; Hamzah, S.; Elias, M. S.

    2017-01-01

    Amang or tin tailing is processed into concentrated ores and other economical valuable minerals such as monazite, zircon, xenotime, ilmenite etc. Besides that, the tailings from these ores may have a significant potential source of radiation exposure to amang plants' workers. This study was conducted to determine the elemental concentration of uranium and thorium in mineral samples collected from five amang tailing factories. The concentration of uranium and thorium was carried out by using instrumental neutron activation analysis (INAA) relative technique. The concentration of uranium and thorium in ppm obtained in this study are as follows: raw (189-1064) and (622-4965); monazite (1076-1988) and (3467-33578); xenotime 4053 and 5540; zircon (309-3090) and (387-6339); ilmenite (104-583) and (88-1205); rutile (212-889) and (44-1119); pyrite (7-43) and (9-132); and waste (5-338) and (9-1218) respectively. The analysis results shows that the monazite, xenotime and zircon have high content of uranium and thorium, whereas ilmenite, rutile, pyrite and waste have lower concentration compare with raw materials after tailing process. The highest values of uranium and thorium concentrations (4053 ± 428 ppm and 33578 ± 873 ppm, respectively) were observed in xenotime and monazite; whereas the lowest value was 5.48 ± 0.86 ppm of uranium recorded in waste (sand) and 9 ± 0.32 ppm of thorium for waste (sand) and pyrite.

  13. U.S.-Australia Civilian Nuclear Cooperation: Issues for Congress

    DTIC Science & Technology

    2010-07-07

    Mining and Milling ................................................................................................7 Uranium Sales to India...carried out at Lucas Heights (see below). The nuclear fuel cycle begins with mining uranium ore and upgrading it to yellowcake. Because naturally... mining and milling stage. Commercial enrichment services are available in the United States, Europe, Russia, and Japan. Fuel fabrication services are

  14. 76 FR 37160 - Notice of Availability of Final Supplemental Environmental Impact Statement for the Lost Creek In...

    Federal Register 2010, 2011, 2012, 2013, 2014

    2011-06-24

    ... Environmental Impact Statement for the Lost Creek In-Situ Recovery (ISR) Project in Sweetwater County, WY; Supplement to the Generic Environmental Impact Statement for In-Situ Leach Uranium Milling Facilities AGENCY... Statement (SEIS) to the Generic Environmental Impact Statement for In- Situ Leach Uranium Milling Facilities...

  15. An Evaluation of a Networked Radiation Detection System

    DTIC Science & Technology

    2010-03-01

    conducted at the site using RAT (Cooper, 2008a): “Beginning in the 1940’ s , widespread mining and milling of uranium ore for national defense and energy...contamination…” in order to determine future sampling points (Cooper, 2007). 2. 4 May 2005, conducted mobile air monitoring during the removal of 30...provide site-wide estimates of emissions…” at Warren (OH) Recycling Inc.®’ s 85 acre landfill emitting hydrogen sulfide (H2S) (Cooper, 2007). 4. 7 July

  16. Ammonium Sulfate Evaporites Associated With Uranium Mill Tailings Disposal Cells

    NASA Astrophysics Data System (ADS)

    Wendlandt, R. F.; Harrison, W. J.

    2006-12-01

    The waste products of uranium mill operations are complex and dependent on the ore mineralogy, milling process (e.g., low pH vs. high pH), and operational status of the mill among other things. The White Mesa Mill, Utah, was visited during both quiescent (July 2004) and operational phases (August 2005) to collect liquid and solid samples from the active evaporation and storage ponds environments (Cells 1 and 3). Cell 4, which was unused and being excavated at the times of both samplings, yielded solids accumulated through the history of that cell's use. Raffinate samples are concentrated Na-Mg-Al-Fe-SO4-NO3(-NH4) brines characterized by extreme enrichments in REE and transition elements. Ionic strengths, calculated using the Pitzer activity coefficient model varied from 25M (pH = 1 at 25°C) in Cell 1 and 12M (pH = 2.7) in Cell 3 during July 2004, to 5M (pH = 1.5) in Cell 1 and 1.2M (pH = 2.9) in Cell 3 during August 2005. At the first sampling, the dominant anion was sulfate in Cell 1 and nitrate in Cell 3. At the time of the second sampling, both cells were dominated by sulfate. During July 2004, there was significant evaporative drawdown in the ponds, resulting in 3 variably colored zones (~7m) of mineralogically complex evaporites at the cell margins. During August 2005, the operational nature of the mill and the addition of fresh water had produced high water levels in Cells 1 and 3. Evaporation crusts were recognized around the margins of the cells but they were <2m in extent. XRD analyses document the presence of boussingaultite, (NH4)2Mg(SO4)2.6H2O, which was actively precipitating from Cell 1 during 2004, tschermigite, (NH4)Al(SO4)2.12H2O, gypsum, and polymorphs of Na2SO4 including thenardite. ESEM imaging and EDS analyses of crusts reveal complex parageneses involving the above-mentioned phases and NH4-bearing metavoltine, K2Na6Fe^{+2}Fe6^{+3}(SO4)12O2.18H2O, among others. Ksp calculations and field relations are consistent with a precipitation sequence of tschermigite followed by boussingaultite and metavoltine.

  17. Chemical quality of ground water in Salt Lake Valley, Utah, 1969-85

    USGS Publications Warehouse

    Waddell, K.M.; Seiler, R.L.; Solomon, D.K.

    1986-01-01

    During 1979-84, 35 wells completed in the principal aquifer in the Salt Lake Valley, Utah, that had been sampled during 1962-67 were resampled to determine if water quality changes had occurred. The dissolved solids concentration of the water from 13 of the wells has increased by more than 10% since 1962-67. Much of the ground water between the mouth of Bingham Canyon and the Jordan River about 10 mi to the east has been contaminated by seepage from reservoirs and evaporation ponds associated with mining activities. Many domestic and irrigation wells yield water with concentrations of dissolved solids that exceed 2,000 mg/L. A reservoir in the mouth of Bingham Canyon contains acidic waters with a pH of 3 to 4 and concentrations of dissolved solids ranging from 43,000 to 68,000 mg/L. Seepage from evaporation ponds, which are about 4.5 mi east of the reservoir, also is acidic and contains similar concentrations of dissolved solids. East of the reservoir, where a steep hydraulic gradient exists along the mountain front, the velocities of contaminant movement were estimated to range from about 680-1,000 ft/yr. Groundwater underlying part of the community of South Salt Lake near the Jordan River has been contaminated by leachate from uranium-mill tailings. The major effect of the leachate from the tailings of the Vitro Chemical Co. on the shallow unconfined aquifer downgradient from the tailings was the contribution of measurable quantities of dissolved solids, chloride, sulfate, iron, and uranium. The concentration of dissolved solids in uncontaminated water was 1,650 mg/L, whereas downgradient from the tailings area, the concentrations ranged from 2,320-21,000 mg/L. The maximum volume of contaminated water was estimated to be 7,800 acre-ft. The major effect of the leachate from the Vitro tailings on the confined aquifer was the contribution of measurable quantities of dissolved solids, chloride, sulfate, and iron. The concentration of dissolved solids upgradient from the tailings was 330 mg/L, and beneath and downgradient from the tailings the concentrations were 864 and 1,240 mg/L. The minimum volume of contaminated water in the confined aquifer was estimated to be about 12,000 acre-ft. (Lantz-PTT)

  18. Effects of Prescribed Burning and Cattle Grazing on Deer Diets in Louisiana

    Treesearch

    Ronald E. Thill; Alton Martin; Hershel F. Morris; Austin T. Harrel

    1995-01-01

    A study was conducted on the dietary and nutritional effects of cattle grazing and rotational prescribed burning on the diets of three to five captive white-tailed deer (Odocoileus virginianus) on longleaf pine (Pinus palustris Mill.) bluestem (Andropogon spp. and Schizachyriumspp.) sites in central Louisiana from October 1980 through February 1987. Deer diets were...

  19. Uptake of /sup 226/Ra by established vegetation and black cutworm larvae, Agrotis ipsilon (class Insecta: order Lepidoptera), on U mill tailings at Elliot Lake, Canada

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Clulow, F.V.; Dave, N.K.; Lim, T.P.

    1988-07-01

    Radium-226 levels in samples from an inactive U tailings site at Elliot Lake, Ontario, Canada, were: 9140 +/- 500 mBq g-1 dry weight in the substrate; 62 +/- 1 mBq g-1 dry weight in rye, Secale cereale, and less than 3.7 mBq g-1 dry weight in oats, Avena sativa, the dominant species established by revegetation of the tailings; and 117 +/- 7 mBq g-1 dry weight in washed and unwashed black cutworm larvae. Concentration ratios were: vegetation to tailings 0.001-0.007; black cutworms to vegetation 3.6 and black cutworms to tailings 0.01. The values are considered too low to be consideredmore » a hazard to herring gulls, Larus argentatus, which occasionally feed on cutworms.« less

  20. Chemical data and lead isotopic compositions of geochemical baseline samples from streambed sediments and smelter slag, lead isotopic compositions in fluvial tailings, and dendrochronology results from the Boulder River watershed, Jefferson County, Montana

    USGS Publications Warehouse

    Unruh, Daniel M.; Fey, David L.; Church, Stan E.

    2000-01-01

    IntroductionAs a part of the U.S. Geological Survey Abandoned Mine Lands Initiative, metal-mining related wastes in the Boulder River study area in northern Jefferson County, Montana, have been evaluated for their environmental effects. The study area includes a 24-km segment of the Boulder River in and around Basin, Montana and three principal tributaries to the Boulder River: Basin Creek, Cataract Creek, and High Ore Creek. Mine and prospect waste dumps and mill wastes are located throughout the drainage basins of these tributaries and in the Boulder River. Mine-waste material has been transported into and down streams, where it has mixed with and become incorporated into the streambed sediments. In some localities, mine waste material was placed directly in stream channels and was transported downstream forming fluvial tailings deposits along the stream banks. Water quality and aquatic habitat have been affected by trace-element-contaminated sediment that moves from mine wastes into and down streams during snowmelt and storm runoff events within the Boulder River watershed.Present-day trace element concentrations in the streambed sediments and fluvial tailings have been extensively studied. However, in order to accurately evaluate the impact of mining on the stream environments, it is also necessary to evaluate the pre-mining trace-element concentrations in the streambed sediments. Three types of samples have been collected for estimation of pre-mining concentrations: 1) streambed sediment samples from the Boulder River and its tributaries located upstream from historical mining activity, 2) stream terrace deposits located both upstream and downstream of the major tributaries along the Boulder River, and 3) cores through sediment in overbank deposits, in abandoned stream channels, or beneath fluvial tailings deposits. In this report, we present geochemical data for six stream-terrace samples and twelve sediment-core samples and lead isotopic data for six terrace and thirteen core samples. Sample localities are in table 1 and figures 1 and 2, and site and sample descriptions are in table 2.Geochemical data have been presented for cores through fluvial tailings on High Ore Creek, on upper Basin Creek, and on Jack Creek and Uncle Sam Gulch. Geochemical and lead isotopic data for modern streambed-sediment samples have been presented by Fey and others.Lead isotopic determinations in bed sediments have been shown to be an effective tool for evaluating the contributions from various sources to the metals in bed sediments. However, in order to make these calculations, the lead isotopic compositions of the contaminant sources must also be known. Consequently, we have determined the lead isotopic compositions of five streambed-sediment samples heavily contaminated with fluvial mine waste immediately downstream from large mines in the Boulder River watershed in order to determine the lead isotopic signatures of the contaminants. Summary geochemical data for the contaminants are presented here and geochemical data for the streambed-sediment samples are given by Fey and others.Downstream from the Katie mill site and Jib tailings, fluvial deposits of mill tailings are present on a 10-m by 50-m bar in the Boulder River below the confluence with Basin Creek. The source of these tailings is not known, but fluvial tailings are also present immediately downstream from the Katie mill site, which is immediately upstream from the confluence with Basin Creek. Nine cores of fluvial tailings from this bar were analyzed.Dendrochronology samples were taken at several stream terrace localities to provide age control on the stream terrace deposits. Trees growing on the surfaces of stream terraces provide a minimum age for the terrace deposits, although floods subsequent to the trees' growth could have deposited post-mining overbank deposits around the trees. Historical data were also used to provide estimates of minimum ages of cultural features and to bracket the age of events.

  1. Alteration, adsorption and nucleation processes on clay-water interfaces: Mechanisms for the retention of uranium by altered clay surfaces on the nanometer scale

    NASA Astrophysics Data System (ADS)

    Schindler, Michael; Legrand, Christine A.; Hochella, Michael F.

    2015-03-01

    Nano-scale processes on the solid-water interface of clay minerals control the mobility of metals in the environment. These processes can occur in confined pore spaces of clay buffers and barriers as well as in contaminated sediments and involve a combination of alteration, adsorption and nucleation processes of multiple species and phases. This study characterizes nano-scale processes on the interface between clay minerals and uranyl-bearing solution near neutral pH. Samples of clay minerals with a contact pH of ∼6.7 are collected from a U mill and mine tailings at Key Lake, Saskatchewan, Canada. The tailings material contains Cu-, As-, Co-, Mo-, Ni-, Se-bearing polymetallic phases and has been deposited with a surplus of Ca(OH)2 and Na2CO3 slaked lime. Small volumes of mill-process solutions containing sulfuric acid and U are occasionally discharged onto the surface of the tailings and are neutralized after discharge by reactions with the slaked lime. Transmission electron microscopy (TEM) in combination with the focused ion beam (FIB) technique and other analytical methods (SEM, XRD, XRF and ICP-OES) are used to characterize the chemical and mineralogical composition of phases within confined pore spaces of the clay minerals montmorillonite and kaolinite and in the surrounding tailings material. Alteration zones around the clay minerals are characterized by different generations of secondary silicates containing variable proportions of adsorbed uranyl- and arsenate-species and by the intergrowth of the silicates with the uranyl-minerals cuprosklodowskite, Cu[(UO2)2(SiO3OH)2](H2O)6 and metazeunerite, Cu[(UO2)(AsO4)2](H2O)8. The majority of alteration phases such as illite, illite-smectite, kaolinite and vermiculite have been most likely formed in the sedimentary basin of the U-ore deposit and contain low amounts of Fe (<5 at.%). Iron-enriched Al-silicates or illite-smectites (Fe >10 at.%) formed most likely in the limed tailings at high contact pH (∼10.5) and their structure is characterized by a low degree of long-range order. Adsorption of U and nucleation of metazeunerite and cuprosklodowskite are strongly controlled by the presence of the adsorbed oxy-anion species arsenate and silica on the Fe-enriched silicates. Heterogeneous nucleation of nano-crystals of the uranyl minerals occurs most likely on adsorption sites of binary uranyl-, arsenate- and silica-complexes as well as on ternary uranyl-arsenate or uranyl-silicate complexes. The uranyl minerals occur as aggregates of misoriented nano-size crystals and are the result of supersaturated solutions and a high number of nucleation sites that prevented the formation of larger crystals through Oswald ripening. The results of this study provide an understanding of interfacial nano-scale processes between uranyl species and altered clay buffers in a potential Nuclear Waste repository as similar alteration conditions of clays may occur in a multi-barrier system.

  2. Evidence of Geobacter-associated phage in a uranium-contaminated aquifer

    PubMed Central

    Holmes, Dawn E; Giloteaux, Ludovic; Chaurasia, Akhilesh K; Williams, Kenneth H; Luef, Birgit; Wilkins, Michael J; Wrighton, Kelly C; Thompson, Courtney A; Comolli, Luis R; Lovley, Derek R

    2015-01-01

    Geobacter species may be important agents in the bioremediation of organic and metal contaminants in the subsurface, but as yet unknown factors limit the in situ growth of subsurface Geobacter well below rates predicted by analysis of gene expression or in silico metabolic modeling. Analysis of the genomes of five different Geobacter species recovered from contaminated subsurface sites indicated that each of the isolates had been infected with phage. Geobacter-associated phage sequences were also detected by metagenomic and proteomic analysis of samples from a uranium-contaminated aquifer undergoing in situ bioremediation, and phage particles were detected by microscopic analysis in groundwater collected from sediment enrichment cultures. Transcript abundance for genes from the Geobacter-associated phage structural proteins, tail tube Gp19 and baseplate J, increased in the groundwater in response to the growth of Geobacter species when acetate was added, and then declined as the number of Geobacter decreased. Western blot analysis of a Geobacter-associated tail tube protein Gp19 in the groundwater demonstrated that its abundance tracked with the abundance of Geobacter species. These results suggest that the enhanced growth of Geobacter species in the subsurface associated with in situ uranium bioremediation increased the abundance and activity of Geobacter-associated phage and show that future studies should focus on how these phages might be influencing the ecology of this site. PMID:25083935

  3. Innovative Approach to Prevent Acid Drainage from Uranium Mill Tailings Based on the Application of Na-Ferrate (VI)

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Fernandes, H.M.; Reinhart, D.; Lettie, L.

    2006-07-01

    The operation of uranium mining and milling plants gives rise to huge amounts of wastes from both mining and milling operations. When pyrite is present in these materials, the generation of acid drainage can take place and result in the contamination of underground and surface waters through the leaching of heavy metals and radionuclides. To solve this problem, many studies have been conducted to find cost-effective solutions to manage acid mine drainage; however, no adequate strategy to deal with sulfide-ric h wastes is currently available. Ferrate (VI) is a powerful oxidizing agent in aqueous media. Under acidic conditions, the redoxmore » potential of the Ferrate (VI) ion is the highest of any other oxidant used in wastewater treatment processes. The standard half cell reduction potential of ferrate (VI) has been determined as +2.20 V to + 0.72 V in acidic and basic solutions, respectively. Ferrate (VI) exhibits a multitude of advantageous properties, including higher reactivity and selectivity than traditional oxidant alternatives, as well as disinfectant, flocculating, and coagulant properties. Despite numerous beneficial properties in environmental applications, ferrate (VI) has remained commercially unavailable. Starting in 1953, different methods for producing a high purity, powdered ferrate (VI) product were developed. However, producing this dry, stabilized ferrate (VI) product required numerous process steps which led to excessive synthesis costs (over $20/lb) thereby preventing bulk industrial use. Recently a novel synthesis method for the production of a liquid ferrate (VI) based on hypochlorite oxidation of ferric ion in strongly alkaline solutions has been discovered (USPTO 6,790,428; September 14, 2004). This on-site synthesis process dramatically reduces manufacturing cost for the production of ferrate (VI) by utilizing common commodity feedstocks. This breakthrough means that for the first time ferrate (VI) can be an economical alternative to treating acid mining drainage generating materials. The objective of the present study was to investigate a methodology of preventing the generation of acid drainage by applying ferrate (VI) to acid generating materials prior to the disposal in impoundments or piles. Oxidizing the pyritic material in mining waste could diminish the potential for acid generation and its related environmental risks and long-term costs at disposal sites. The effectiveness of toxic metals removal from acid mine drainage by applying ferrate (VI) is also examined. Preliminary results presented in this paper show that the oxidation of pyrite by ferrate is a first-order rate reaction in Fe(VI) with a half-life of about six hours. The stability of Fe(VI) in water solutions will not influence the reaction rate in a significant manner. New low-cost production methods for making liquid ferrate on-site makes this technology a very attractive option to mitigate one of the most pressing environmental problems in the mining industry. (authors)« less

  4. Exposure pathways and health effects associated with chemical and radiological toxicity of natural uranium: a review.

    PubMed

    Brugge, Doug; de Lemos, Jamie L; Oldmixon, Beth

    2005-01-01

    Natural uranium exposure derives from the mining, milling, and processing of uranium ore, as well as from ingestion of groundwater that is naturally contaminated with uranium. Ingestion and inhalation are the primary routes of entry into the body. Absorption of uranium from the lungs or digestive track is typically low but can vary depending on compound specific solubility. From the blood, two-thirds of the uranium is excreted in urine over the first 24 hours and up to 80% to 90% of uranium deposited in the bone leaves the body within 1.5 years. The primary health outcomes of concern documented with respect to uranium are renal, developmental, reproductive, diminished bone growth, and DNA damage. The reported health effects derive from experimental animal studies and human epidemiology. The Lowest Observed Adverse Effect Level (LOAEL) derived from animal studies is 50 microg/m3 for inhalation and 60 ug/kg body weight/day for ingestion. The current respiratory standard of the Occupational Safety and Health Administration (OSHA), 50 microg/m3, affords no margin of safety. Considering the safety factors for species and individual variation, the ingestion LOAEL corresponds to the daily consumption set by the World Health Organization Drinking Water Standard at 2 microg/L. Based on economic considerations, the United States Environmental Protection Agency maximum contaminant level is 30 microg/L. Further research is needed, with particular attention on the impact of uranium on indigenous populations, on routes of exposure in communities near uranium sites, on the combined exposures present at many uranium sites, on human developmental defects, and on health effects at or below established exposure standards.

  5. Effects of uranium mining, Puerco River, New Mexico

    USGS Publications Warehouse

    Lopes, Thomas J.

    1991-01-01

    Effluent from uranium-mine dewatering and acidic water released by a tailings-pond dike failure increased radionuclide activities in streamflow in the Puerco River in New Mexico and Arizona. Median dissolved gross-alpha activity in the streamflow was 1,130 picocuries per liter from 1975 to 1986 when mine discharges ceased and 6.2 picocuries per liter from 1986 to 1989. From 1975 to July 1979, major ions in streamflow at the Puerco River at Gallup streamflow-gaging station were sodium, bicarbonate, and sulfate. On July 16, 1979, the day of the tailing spill, major ions in streamflow were magnesium, calcium, and sulfate. From 1979 to 1984, major ions in streamflow had a greater proportion of calcium and sulfate than prior to the spill, indicating flushing of residual tailings solution. Geochemical modeling of mine effluent indicates that uranium was unlikely to precipitate from effluent between the mines and Gallup or when mixed with wastewater downstream from Gallup. Geochemical modeling of acidic-tailings solution indicates that uranium was in solution as far downstream as Gallup. When the acidic-tailings solution mixed with 10- to 40-percent wastewater, uranium may have precipitated from solution as carnotite [K2(UO2)2(VO4)2] and tyuyamunite [Ca(UO2)2(VO4)2].

  6. Uranium Bio-accumulation and Cycling as revealed by Uranium Isotopes in Naturally Reduced Sediments from the Upper Colorado River Basin

    NASA Astrophysics Data System (ADS)

    Lefebvre, Pierre; Noël, Vincent; Jemison, Noah; Weaver, Karrie; Bargar, John; Maher, Kate

    2016-04-01

    Uranium (U) groundwater contamination following oxidized U(VI) releases from weathering of mine tailings is a major concern at numerous sites across the Upper Colorado River Basin (CRB), USA. Uranium(IV)-bearing solids accumulated within naturally reduced zones (NRZs) characterized by elevated organic carbon and iron sulfide compounds. Subsequent re-oxidation of U(IV)solid to U(VI)aqueous then controls the release to groundwater and surface water, resulting in plume persistence and raising public health concerns. Thus, understanding the extent of uranium oxidation and reduction within NRZs is critical for assessing the persistence of the groundwater contamination. In this study, we measured solid-phase uranium isotope fractionation (δ238/235U) of sedimentary core samples from four study sites (Shiprock, NM, Grand Junction, Rifle and Naturita, CO) using a multi-collector inductively coupled plasma mass spectrometer (MC-ICP-MS). We observe a strong correlation between U accumulation and the extent of isotopic fractionation, with Δ238U up to +1.8 ‰ between uranium-enriched and low concentration zones. The enrichment in the heavy isotopes within the NRZs appears to be especially important in the vadose zone, which is subject to variations in water table depth. According to previous studies, this isotopic signature is consistent with biotic reduction processes associated with metal-reducing bacteria. Positive correlations between the amount of iron sulfides and the accumulation of reduced uranium underline the importance of sulfate-reducing conditions for U(IV) retention. Furthermore, the positive fractionation associated with U reduction observed across all sites despite some variations in magnitude due to site characteristics, shows a regional trend across the Colorado River Basin. The maximum extent of 238U enrichment observed in the NRZ proximal to the water table further suggests that the redox cycling of uranium, with net release of U(VI) to the groundwater by non-fractionating oxidation, is occurring within this zone. Thus, release of uranium from the NRZs may play a critical role in the persistence of groundwater contamination at these sites.

  7. Process for the removal of radium from acidic solutions containing same

    DOEpatents

    Scheitlin, F.M.

    The invention is a process for the removal of radium from acidic aqueous solutions. In one aspect, the invention is a process for removing radium from an inorganic-acid solution. The process comprises contacting the solution with coal fly ash to effect adsorption of the radium on the ash. The radium-containing ash then is separated from the solution. The process is simple, comparatively inexpensive, and efficient. High radium-distribution coefficients are obtained even at room temperature. Coal fly ash is an inexpensive, acid-resistant, high-surface-area material which is available in large quantities throughout the United States. The invention is applicable, for example, to the recovery of /sup 226/Ra from nitric acid solutions which have been used to leach radium from uranium-mill tailings.

  8. Removal of radium from acidic solutions containing same by adsorption on coal fly ash

    DOEpatents

    Scheitlin, Frank M.

    1984-01-01

    The invention is a process for the removal of radium from acidic aqueous solutions. In one aspect, the invention is a process for removing radium from an inorganic-acid solution. The process comprises contacting the solution with coal fly ash to effect adsorption of the radium on the ash. The radium-containing ash then is separated from the solution. The process is simple, comparatively inexpensive, and efficient. High radium-distribution coefficients are obtained even at room temperature. Coal fly ash is an inexpensive, acid-resistant, high-surface-area material which is available in large quantities throughout the United States. The invention is applicable, for example, to the recovery of .sup.226 Ra from nitric acid solutions which have been used to leach radium from uranium-mill tailings.

  9. 10 CFR 51.60 - Environmental report-materials licenses.

    Code of Federal Regulations, 2011 CFR

    2011-01-01

    ... oil and gas recovery. (vii) Construction and operation of a uranium enrichment facility. (2) Issuance... conversion of uranium hexafluoride pursuant to part 70 of this chapter. (ii) Possession and use of source material for uranium milling or production of uranium hexafluoride pursuant to part 40 of this chapter...

  10. 10 CFR 51.60 - Environmental report-materials licenses.

    Code of Federal Regulations, 2010 CFR

    2010-01-01

    ... oil and gas recovery. (vii) Construction and operation of a uranium enrichment facility. (2) Issuance... conversion of uranium hexafluoride pursuant to part 70 of this chapter. (ii) Possession and use of source material for uranium milling or production of uranium hexafluoride pursuant to part 40 of this chapter...

  11. 10 CFR 51.60 - Environmental report-materials licenses.

    Code of Federal Regulations, 2013 CFR

    2013-01-01

    ... oil and gas recovery. (vii) Construction and operation of a uranium enrichment facility. (2) Issuance... conversion of uranium hexafluoride pursuant to part 70 of this chapter. (ii) Possession and use of source material for uranium milling or production of uranium hexafluoride pursuant to part 40 of this chapter...

  12. 10 CFR 51.60 - Environmental report-materials licenses.

    Code of Federal Regulations, 2014 CFR

    2014-01-01

    ... oil and gas recovery. (vii) Construction and operation of a uranium enrichment facility. (2) Issuance... conversion of uranium hexafluoride pursuant to part 70 of this chapter. (ii) Possession and use of source material for uranium milling or production of uranium hexafluoride pursuant to part 40 of this chapter...

  13. 10 CFR 51.60 - Environmental report-materials licenses.

    Code of Federal Regulations, 2012 CFR

    2012-01-01

    ... oil and gas recovery. (vii) Construction and operation of a uranium enrichment facility. (2) Issuance... conversion of uranium hexafluoride pursuant to part 70 of this chapter. (ii) Possession and use of source material for uranium milling or production of uranium hexafluoride pursuant to part 40 of this chapter...

  14. 77 FR 70486 - Supplemental Environmental Impact Statement for Proposed Dewey-Burdock In-Situ Uranium Recovery...

    Federal Register 2010, 2011, 2012, 2013, 2014

    2012-11-26

    ... Proposed Dewey- Burdock In-Situ Uranium Recovery Project in Custer and Fall River Counties, SD AGENCY... draft Supplemental Environmental Impact Statement (Draft SEIS) for the Dewey-Burdock In-Situ Uranium... NUREG-1910, ``Generic Environmental Impact Statement for In-Situ Leach Uranium Milling Facilities,'' May...

  15. Impact of environmentally based chemical hardness on uranium speciation and toxicity in six aquatic species.

    PubMed

    Goulet, Richard R; Thompson, Patsy A; Serben, Kerrie C; Eickhoff, Curtis V

    2015-03-01

    Treated effluent discharge from uranium (U) mines and mills elevates the concentrations of U, calcium (Ca), magnesium (Mg), and sulfate (SO4 (2-) ) above natural levels in receiving waters. Many investigations on the effect of hardness on U toxicity have been experiments on the combined effects of changes in hardness, pH, and alkalinity, which do not represent water chemistry downstream of U mines and mills. Therefore, more toxicity studies with water chemistry encountered downstream of U mines and mills are necessary to support predictive assessments of impacts of U discharge to the environment. Acute and chronic U toxicity laboratory bioassays were realized with 6 freshwater species in waters of low alkalinity, circumneutral pH, and a range of chemical hardness as found in field samples collected downstream of U mines and mills. In laboratory-tested waters, speciation calculations suggested that free uranyl ion concentrations remained constant despite increasing chemical hardness. When hardness increased while pH remained circumneutral and alkalinity low, U toxicity decreased only to Hyalella azteca and Pseudokirchneriella subcapitata. Also, Ca and Mg did not compete with U for the same uptake sites. The present study confirms that the majority of studies concluding that hardness affected U toxicity were in fact studies in which alkalinity and pH were the stronger influence. The results thus confirm that studies predicting impacts of U downstream of mines and mills should not consider chemical hardness. Environ Toxicol Chem 2015;34:562-574. © 2014 The Authors. Published by Wiley Periodicals, Inc. on behalf of SETAC. © 2014 The Authors. Published by Wiley Periodicals, Inc. on behalf of SETAC.

  16. Improvement of the Uranium Sequestration Ability of a Chlamydomonas sp. (ChlSP Strain) Isolated From Extreme Uranium Mine Tailings Through Selection for Potential Bioremediation Application.

    PubMed

    Baselga-Cervera, Beatriz; Romero-López, Julia; García-Balboa, Camino; Costas, Eduardo; López-Rodas, Victoria

    2018-01-01

    The extraction and processing of uranium (U) have polluted large areas worldwide, rendering anthropogenic extreme environments inhospitable to most species. Noticeably, these sites are of great interest for taxonomical and applied bioprospection of extremotolerant species successfully adapted to U tailings contamination. As an example, in this work we have studied a microalgae species that inhabits extreme U tailings ponds at the Saelices mining site (Salamanca, Spain), characterized as acidic (pH between 3 and 4), radioactive (around 4 μSv h -1 ) and contaminated with metals, mainly U (from 25 to 48 mg L -1 ) and zinc (from 17 to 87 mg L -1 ). After isolation of the extremotolerant ChlSP strain, morphological characterization and internal transcribed spacer (ITS)-5.8S gene sequences placed it in the Chlamydomonadaceae , but BLAST analyses identity values, against the nucleotide datasets at the NCBI database, were very low (<92%). We subjected the ChlSP strain to an artificial selection protocol to increase the U uptake and investigated its response to selection. The ancestral strain ChlSP showed a U-uptake capacity of ≈4.30 mg U g -1 of dry biomass (DB). However, the artificially selected strain ChlSG was able to take up a total of ≈6.34 mg U g -1 DB, close to the theoretical maximum response (≈7.9 mg U g -1 DB). The selected ChlSG strain showed two possible U-uptake mechanisms: the greatest proportion by biosorption onto cell walls (ca. 90%), and only a very small quantity, ~0.46 mg g -1 DB, irreversibly bound by bioaccumulation. Additionally, the kinetics of the U-uptake process were characterized during a microalgae growth curve; ChlSG cells removed close to 4 mg L -1 of U in 24 days. These findings open up promising prospects for sustainable management of U tailings waters based on newly evolved extremotolerants and outline the potential of artificial selection in the improvement of desired features in microalgae by experimental adaptation and selection.

  17. Improvement of the Uranium Sequestration Ability of a Chlamydomonas sp. (ChlSP Strain) Isolated From Extreme Uranium Mine Tailings Through Selection for Potential Bioremediation Application

    PubMed Central

    Baselga-Cervera, Beatriz; Romero-López, Julia; García-Balboa, Camino; Costas, Eduardo; López-Rodas, Victoria

    2018-01-01

    The extraction and processing of uranium (U) have polluted large areas worldwide, rendering anthropogenic extreme environments inhospitable to most species. Noticeably, these sites are of great interest for taxonomical and applied bioprospection of extremotolerant species successfully adapted to U tailings contamination. As an example, in this work we have studied a microalgae species that inhabits extreme U tailings ponds at the Saelices mining site (Salamanca, Spain), characterized as acidic (pH between 3 and 4), radioactive (around 4 μSv h−1) and contaminated with metals, mainly U (from 25 to 48 mg L−1) and zinc (from 17 to 87 mg L−1). After isolation of the extremotolerant ChlSP strain, morphological characterization and internal transcribed spacer (ITS)-5.8S gene sequences placed it in the Chlamydomonadaceae, but BLAST analyses identity values, against the nucleotide datasets at the NCBI database, were very low (<92%). We subjected the ChlSP strain to an artificial selection protocol to increase the U uptake and investigated its response to selection. The ancestral strain ChlSP showed a U-uptake capacity of ≈4.30 mg U g−1 of dry biomass (DB). However, the artificially selected strain ChlSG was able to take up a total of ≈6.34 mg U g−1 DB, close to the theoretical maximum response (≈7.9 mg U g−1 DB). The selected ChlSG strain showed two possible U-uptake mechanisms: the greatest proportion by biosorption onto cell walls (ca. 90%), and only a very small quantity, ~0.46 mg g−1 DB, irreversibly bound by bioaccumulation. Additionally, the kinetics of the U-uptake process were characterized during a microalgae growth curve; ChlSG cells removed close to 4 mg L−1 of U in 24 days. These findings open up promising prospects for sustainable management of U tailings waters based on newly evolved extremotolerants and outline the potential of artificial selection in the improvement of desired features in microalgae by experimental adaptation and selection. PMID:29662476

  18. 78 FR 20146 - Lost Creek ISR, LLC, Lost Creek Uranium In-Situ Recovery Project, Sweetwater County, Wyoming

    Federal Register 2010, 2011, 2012, 2013, 2014

    2013-04-03

    ... ISR, LLC, Lost Creek Uranium In-Situ Recovery Project, Sweetwater County, Wyoming AGENCY: Nuclear... to Source Materials License SUA-1598 for continued uranium production operations and in-situ recovery... identified in NUREG-1910, ``Generic Environmental Impact Statement for In-Situ Leach Uranium Milling...

  19. Environmental guidance for public participation in environmental restoration activities

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1991-11-01

    The US Department of Energy (DOE) is issuing this document, entitled Guidance on Public Participation for US Department of Energy Environmental Restoration Activities, to summarize policy and provide guidance for public participation in environmental restoration activities at DOE Headquarters, Field Offices, facilities, and laboratories. While the Office of Environmental Restoration and Waste Management (EM) has environmental restoration responsibility for the majority of DOE sites and facilities, other DOE Project Offices have similar responsibilities at their sites and facilities. This guidance is applicable to all environment restoration activities conducted by or for DOE under the Comprehensive Environmental Response, Compensation, and Liabilitymore » Act of 1980 (CERCLA) as amended by the Superfund Amendments and Reauthorization Act of 1986 (SARA); the Resource Conservation and Recovery Act of 1976 (RCRA) as amended by the Hazardous and Solid Waste Amendments of 1984 (HSWA) (corrective actions only); and the National Environmental Policy Act of 1969 (NEPA). This guidance also is applicable to CERCLA remedial action programs under the Uranium Mill Tailings Radiation Control Act of 1978 and the Formerly Utilized Sites Remedial Action Program, where DOE is the designated lead. The primary objectives of this guidance document are as follows: acclimate DOE staff to a changing culture that emphasizes the importance of public participation activities; provide direction on implementing these public participation activities; and, provide consistent guidance for all DOE Field Offices and facilities. The purpose of this document is to provide guidance on conducting effective public participation activities for environmental restoration activities under CERCLA; RCRA corrective actions under sections 3004(u), 3004(v), and 3008(h); and NEPA public participation activities.« less

  20. Recycling/Disposal Alternatives for Depleted Uranium Wastes

    DTIC Science & Technology

    1981-01-01

    could pass before new sites are available. Recent experi- ence with attempts to dispose of wastes generated by cleanup of the Three Mile Island...commercial sector. Nonordnance uses include counterweights, Lallast, shielding , and special appli- cations machinery. Although the purity requirements...Refer- ence 11). Since the activity of the tailings is higher than allow- able for unrestricted access, large earth -dam retention systems, known as

  1. Ramie (Boehmeria nivea)'s uranium bioconcentration and tolerance attributes.

    PubMed

    Wang, Wei-Hong; Luo, Xue-Gang; Liu, Lai; Zhang, Yan; Zhao, Hao-Zhou

    2018-04-01

    The authors sampled and analyzed 15 species of dominant wild plants in Huanan uranium tailings pond in China, whose tailings' uranium contents were 3.21-120.52 μg/g. Among the 15 species of wild plants, ramie (Boehmeria nivea) had the strongest uranium bioconcentration and transfer capacities. In order to study the uranium bioconcentration and tolerance attributes of ramie in detail, and provide a reference for the screening remediation plants to phytoremedy on a large scale in uranium tailings pond, a ramie cultivar Xiangzhu No. 7 pot experiment was carried out. We found that both wild ramie and Xiangzhu No. 7 could bioconcentrate uranium, but there were two differences. One was wild ramie's shoots bioconcentrated uranium up to 20 μg/g (which can be regarded as the critical content value of the shoot of uranium hyperaccumulator) even the soil uranium content was as low as 5.874 μg/g while Xiangzhu No. 7's shoots could reach 20 μg/g only when the uranium treatment concentrations were 275 μg/g or more; the other was that all the transfer factors of 3 wild samples were >1, and the transfer factors of 27 out of 28 pot experiment samples were <1. Probably wild ramie was a uranium hyperaccumulator. Xiangzhu No. 7 satisfied the needs of uranium hyperaccumulator on accumulation capability, tolerance capability, bioconcentration factor, but not transfer capability, so Xiangzhu No. 7 was not a uranium hyperaccumulator. We analyzed the possible reasons why there were differences in the uranium bioconcentration and transfer attributes between wild ramie and Xiangzhu No. 7., and proposed the direction for further research. In our opinion, both the plants which bioconcentrate contaminants in the shoots and roots can act as phytoextractors. Although Xiangzhu No. 7's biomass and accumulation of uranium were concentrated on the roots, the roots were small in volume and easy to harvest. And Xiangzhu No. 7's cultivating skills and protection measures had been developed very well. Xiangzhu No. 7's whole bioconcentration factors and the roots' bioconcentration factors, which were 1.200-1.834 and 1.460-2.341, respectively, increased with the increases of uranium contents of pot soil when the soil's uranium contents are 25-175 μg/g, so it can act as a potential phytoextractor when Huanan uranium tailings pond is phytoremediated. Copyright © 2018. Published by Elsevier Ltd.

  2. 2. VIEW OF LOWER MILL FLOOR FOUNDATION, SHOWING, LEFT TO ...

    Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

    2. VIEW OF LOWER MILL FLOOR FOUNDATION, SHOWING, LEFT TO RIGHT, EDGE OF MILLING FLOOR, TABLE FLOOR, VANNING FLOOR, LOADING LEVEL, TAILINGS POND IN RIGHT BACKGROUND. VIEW IS LOOKING FROM THE NORTHWEST - Mountain King Gold Mine & Mill, 4.3 Air miles Northwest of Copperopolis, Copperopolis, Calaveras County, CA

  3. Bioassays with caged hyalella azteca to determine in situ toxicity downstream of two Saskatchewan, Canada, uranium operations.

    PubMed

    Robertson, Erin L; Liber, Karsten

    2007-11-01

    The main objectives of this in situ study were to evaluate the usefulness of an in situ bioassay to determine if downstream water bodies at the Key Lake and Rabbit Lake uranium operations (Saskatchewan, Canada) were toxic to Hyalella azteca and, if toxicity was observed, to differentiate between the contribution of surface water and sediment contamination to in situ toxicity. These objectives were achieved by performing 4-d in situ bioassays with laboratory-reared H. azteca confined in specially designed, paired, surface water and sediment exposure chambers. Results from the in situ bioassays revealed significant mortality, relative to the respective reference site, at the exposure sites at both Key Lake (p

  4. 10 CFR 40.65 - Effluent monitoring reporting requirements.

    Code of Federal Regulations, 2010 CFR

    2010-01-01

    ... 10 Energy 1 2010-01-01 2010-01-01 false Effluent monitoring reporting requirements. 40.65 Section 40.65 Energy NUCLEAR REGULATORY COMMISSION DOMESTIC LICENSING OF SOURCE MATERIAL Records, Reports... possess and use source material in uranium milling, in production of uranium hexafluoride, or in a uranium...

  5. 9. VIEW OF MILLING AND LATHE MACHINES, MILLING AND LATHE ...

    Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

    9. VIEW OF MILLING AND LATHE MACHINES, MILLING AND LATHE MACHINES WERE USED TO FORM COMPONENTS INTO THEIR FINAL SHAPE. IN THE FOUNDRY, ENRICHED URANIUM WAS CAST INTO SPHERICAL SHAPES OR INGOT FROM WHICH WEAPONS COMPONENTS WERE FABRICATED. (4/4/66) - Rocky Flats Plant, General Manufacturing, Support, Records-Central Computing, Southern portion of Plant, Golden, Jefferson County, CO

  6. A review and overview of nuclear waste management

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Murray, R.L.

    1984-12-31

    An understanding of the status and issues in the management of radioactive wastes is based on technical information on radioactivity, radiation, biological hazard of radiation exposure, radiation standards, and methods of protection. The fission process gives rise to radioactive fission products and neutron bombardment gives activation products. Radioactive wastes are classified according to source: defense, commercial, industrial, and institutional; and according to physical features: uranium mill tailings, high-level, transuranic, and low-level. The nuclear fuel cycle, which contributes a large fraction of annual radioactive waste, starts with uranium ore, includes nuclear reactor use for electrical power generation, and ends with ultimatemore » disposal of residues. The relation of spent fuel storage and reprocessing is governed by technical, economic, and political considerations. Waste has been successfully solidified in glass and other forms and choices of the containers for the waste form are available. Methods of disposal of high-level waste that have been investigated are transmutation by neutron bombardment, shipment to Antartica, deep-hole insertion, subseabed placement, transfer by rocket to an orbit in space, and disposal in a mined cavity. The latter is the favored method. The choices of host geological media are salt, basalt, tuff, and granite.« less

  7. Effect of desliming of sulphide-rich mill tailings on the long-term strength of cemented paste backfill.

    PubMed

    Ercikdi, Bayram; Baki, Hakan; İzki, Muhammet

    2013-01-30

    This paper presents the effect of desliming on the short- and long-term strength, stability and rheological properties of cemented paste backfill (CPB) produced from two different mill tailings. A 28-day unconfined compressive strength (UCS) of ≥1.0 MPa and the maintenance of stability over 224 days of curing were selected as the design criteria for the evaluation of paste backfill performance. Desliming induced some changes in the physical, chemical, mineralogical and rheological properties of the tailings. CPB mixture of the deslimed tailings achieved the required consistency at a lower water to cement ratio. The short-term UCSs of CPB samples of the deslimed tailings were found to be 30-100% higher than those samples of the reference tailings at all the binder dosages and curing times. CPB samples of the deslimed tailings achieved the long-term stability at relatively low binder dosages (e.g. 5 wt% c.f. ≥6.1% for the reference tailings). It was also estimated that desliming could allow a 13.4-23.1% reduction in the binder consumption depending apparently on the inherent characteristics of the tailings. Over the curing period, generation of sulphate and acid by the oxidation of pyrite present in the tailings was also monitored to correlate with the strength losses observed in the long term. Scanning electron microscope (SEM) and Mercury Intrusion Porosimetry (MIP) analyses provided an insight into the microstructure of CPB and the formation of secondary mineral phases (i.e. gypsum) confirming the beneficial effect of desliming. These findings suggest that desliming can be suitably exploited for CPB of sulphide-rich mill tailings to improve the strength and stability particularly in the long term and to reduce binder consumption. Copyright © 2012 Elsevier Ltd. All rights reserved.

  8. Microbial communities in low permeability, high pH uranium mine tailings: characterization and potential effects.

    PubMed

    Bondici, V F; Lawrence, J R; Khan, N H; Hill, J E; Yergeau, E; Wolfaardt, G M; Warner, J; Korber, D R

    2013-06-01

    To describe the diversity and metabolic potential of microbial communities in uranium mine tailings characterized by high pH, high metal concentration and low permeability. To assess microbial diversity and their potential to influence the geochemistry of uranium mine tailings using aerobic and anaerobic culture-based methods, in conjunction with next generation sequencing and clone library sequencing targeting two universal bacterial markers (the 16S rRNA and cpn60 genes). Growth assays revealed that 69% of the 59 distinct culturable isolates evaluated were multiple-metal resistant, with 15% exhibiting dual-metal hypertolerance. There was a moderately positive correlation coefficient (R = 0·43, P < 0·05) between multiple-metal resistance of the isolates and their enzyme expression profile. Of the isolates tested, 17 reduced amorphous iron, 22 reduced molybdate and seven oxidized arsenite. Based on next generation sequencing, tailings depth was shown to influence bacterial community composition, with the difference in the microbial diversity of the upper (0-20 m) and middle (20-40 m) tailings zones being highly significant (P < 0·01) from the lower zone (40-60 m) and the difference in diversity of the upper and middle tailings zone being significant (P < 0·05). Phylotypes closely related to well-known sulfate-reducing and iron-reducing bacteria were identified with low abundance, yet relatively high diversity. The presence of a population of metabolically-diverse, metal-resistant micro-organisms within the tailings environment, along with their demonstrated capacity for transforming metal elements, suggests that these organisms have the potential to influence the long-term geochemistry of the tailings. This study is the first investigation of the diversity and functional potential of micro-organisms present in low permeability, high pH uranium mine tailings. © 2013 The Society for Applied Microbiology.

  9. Uranium production in Romania

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    NONE

    1994-12-01

    This article reviews uranium production in Romania. Geological aspects of the country are discussed, and known uranium deposits are noted. Uranium mining and milling activities are also covered. Utilization of Romania`s uranium production industry will primarily be to supply the country`s nuclear power program, and with the present adequate supplies and the operation of their recently revamped fuel production facility, Romania should be self-reliant in the front end of the nuclear fuel cycle.

  10. Dissolution of alkaline earth sulfates in the presence of montmorillonite

    USGS Publications Warehouse

    Eberl, D.D.; Landa, E.R.

    1985-01-01

    In a study of the effect of montmorillonite on the dissolution of BaSO4 (barite), SrSO4 (celestite), and 226Ra from U mill tailings, it was found that: (1) More of these substances dissolve in an aqueous system that contains montmorillonite than dissolve in a similar system without clay, due to the ion exchange properties of the clay; (2) Na-montmorillonite is more effective in aiding dissolution than is Ca-montmorillonite; (3) the amount of Ra that moves from mill tailings to an exchanger increases as solution sulfate activity decreases. Leaching experiments suggest that 226Ra from H2SO4-circuit U mill tailings from Edgemont, South Dakota, is not present as pure Ra sulfate or as an impurity in anhydrite or gypsum; it is less soluble, and probably occurs as a trace constituent in barite.

  11. Estimated water requirements for the conventional flotation of copper ores

    USGS Publications Warehouse

    Bleiwas, Donald I.

    2012-01-01

    This report provides a perspective on the amount of water used by a conventional copper flotation plant. Water is required for many activities at a mine-mill site, including ore production and beneficiation, dust and fire suppression, drinking and sanitation, and minesite reclamation. The water required to operate a flotation plant may outweigh all of the other uses of water at a mine site, [however,] and the need to maintain a water balance is critical for the plant to operate efficiently. Process water may be irretrievably lost or not immediately available for reuse in the beneficiation plant because it has been used in the production of backfill slurry from tailings to provide underground mine support; because it has been entrapped in the tailings stored in the TSF, evaporated from the TSF, or leaked from pipes and (or) the TSF; and because it has been retained as moisture in the concentrate. Water retained in the interstices of the tailings and the evaporation of water from the surface of the TSF are the two most significant contributors to water loss at a conventional flotation circuit facility.

  12. Uranium Mines and Mills Location Database

    EPA Pesticide Factsheets

    EPA has compiled mine location information from federal, state, and Tribal agencies into a single database as part of its investigation into the potential environmental hazards of wastes from abandoned uranium mines in the western United States.

  13. 40 CFR 190.12 - Effective date.

    Code of Federal Regulations, 2010 CFR

    2010-07-01

    ... Uranium Fuel Cycle § 190.12 Effective date. (a) The standards in § 190.10(a) shall be effective December 1, 1979, except that for doses arising from operations associated with the milling of uranium ore the...

  14. A coupled modelling effort to study the fate of contaminated sediments downstream of the Coles Hill deposit, Virginia, USA

    NASA Astrophysics Data System (ADS)

    Castro-Bolinaga, C. F.; Zavaleta, E. R.; Diplas, P.

    2015-03-01

    This paper presents the preliminary results of a coupled modelling effort to study the fate of tailings (radioactive waste-by product) downstream of the Coles Hill uranium deposit located in Virginia, USA. The implementation of the overall modelling process includes a one-dimensional hydraulic model to qualitatively characterize the sediment transport process under severe flooding conditions downstream of the potential mining site, a two-dimensional ANSYS Fluent model to simulate the release of tailings from a containment cell located partially above the local ground surface into the nearby streams, and a one-dimensional finite-volume sediment transport model to examine the propagation of a tailings sediment pulse in the river network located downstream. The findings of this investigation aim to assist in estimating the potential impacts that tailings would have if they were transported into rivers and reservoirs located downstream of the Coles Hill deposit that serve as municipal drinking water supplies.

  15. 40 CFR 440.30 - Applicability; description of the uranium, radium and vanadium ores subcategory.

    Code of Federal Regulations, 2014 CFR

    2014-07-01

    ... vanadium ores are produced; and (b) mills using the acid leach, alkaline leach, or combined acid and alkaline leach process for the extraction of uranium, radium and vanadium. Only vanadium byproduct...

  16. 40 CFR 440.30 - Applicability; description of the uranium, radium and vanadium ores subcategory.

    Code of Federal Regulations, 2012 CFR

    2012-07-01

    ... vanadium ores are produced; and (b) mills using the acid leach, alkaline leach, or combined acid and alkaline leach process for the extraction of uranium, radium and vanadium. Only vanadium byproduct...

  17. 40 CFR 440.30 - Applicability; description of the uranium, radium and vanadium ores subcategory.

    Code of Federal Regulations, 2013 CFR

    2013-07-01

    ... vanadium ores are produced; and (b) mills using the acid leach, alkaline leach, or combined acid and alkaline leach process for the extraction of uranium, radium and vanadium. Only vanadium byproduct...

  18. Radium-226 dose to a boy from playing on mill tailings

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Mays, C.W.; Lucas, H.F.; Lloyd, R.D.

    Two boys born in September 1949 played on uranium mill tailings from about ages 8 to 12. One of these boys was diagnosed as having leukemia at age 15.5. The 226Ra body burden of the survivor was measured at age 38. The whole-body 226Ra content measured by counting in vivo was 0 {plus minus} 17 Bq and independently by Rn breath analysis as 4.3 {plus minus} 2.1 Bq. At the same time, a control subject with no known exposure to 226Ra, matched in age, height, and weight, was also measured. The whole-body content was estimated as 4 {plus minus} 15more » Bq and independently by Rn breath analysis as 5.5 {plus minus} 3.7 Bq. The body burden of the control subject was not significantly different from that of the exposed person. The radiation dose to the marrow-free skeleton assuming a constant 226Ra:Ca ratio since birth was 0.49 and 1.33 mGy at ages 14 and 38, respectively. The radiation dose to the marrow-free skeleton assuming 226Ra intake only between ages 8 to 12 was 1.4 and 2.8 mGy at ages 14 and 38, respectively. The best estimate is the mean of these two estimates: 0.9 and 2.1 mGy at ages 14 and 38, respectively. The alpha-particle dose to the red marrow from 226Ra and its decay products was 0.05 mGy at age 14 and 0.10 mGy at age 38. Since no excess was found for the radium dial painters whose doses were much higher, the induction of leukemia by doses of this magnitude would seem quite unlikely.« less

  19. Removal of As, Mn, Mo, Se, U, V and Zn from groundwater by zero-valent iron in a passive treatment cell: reaction progress modeling.

    PubMed

    Morrison, Stan J; Metzler, Donald R; Dwyer, Brian P

    2002-05-01

    Three treatment cells were operated at a site near Durango, CO. One treatment cell operated for more than 3 years. The treatment cells were used for passive removal of contamination from groundwater at a uranium mill tailings repository site. Zero-valent iron [Fe(0)] that had been powdered, bound with aluminosilicate and molded into plates was used as a reactive material in one treatment cell. The others used granular Fe(0) and steel wool. The treatment cells significantly reduced concentrations of As, Mn, Mo, Se, U, V and Zn in groundwater that flowed through it. Zero-valent iron [Fe(0)], magnetite (Fe3O4), calcite (CaCO3), goethite (FeOOH) and mixtures of contaminant-bearing phases were identified in the solid fraction of one treatment cell. A reaction progress approach was used to model chemical evolution of water chemistry as it reacted with the Fe(0). Precipitation of calcite, ferrous hydroxide [Fe(OH)2] and ferrous sulfide (FeS) were used to simulate observed changes in major-ion aqueous chemistry. The amount of reaction progress differed for each treatment cell. Changes in contaminant concentrations were consistent with precipitation of reduced oxides (UO2, V2O3), sulfides (As2S3, ZnS), iron minerals (FeSe2, FeMoO4) and carbonate (MnCO3). Formation of a free gas phase and precipitation of minerals contributed to loss of hydraulic conductivity in one treatment cell.

  20. Drinking Water with Uranium below the U.S. EPA Water Standard Causes Estrogen Receptor–Dependent Responses in Female Mice

    PubMed Central

    Raymond-Whish, Stefanie; Mayer, Loretta P.; O’Neal, Tamara; Martinez, Alisyn; Sellers, Marilee A.; Christian, Patricia J.; Marion, Samuel L.; Begay, Carlyle; Propper, Catherine R.; Hoyer, Patricia B.; Dyer, Cheryl A.

    2007-01-01

    Background The deleterious impact of uranium on human health has been linked to its radioactive and heavy metal–chemical properties. Decades of research has defined the causal relationship between uranium mining/milling and onset of kidney and respiratory diseases 25 years later. Objective We investigated the hypothesis that uranium, similar to other heavy metals such as cadmium, acts like estrogen. Methods In several experiments, we exposed intact, ovariectomized, or pregnant mice to depleted uranium in drinking water [ranging from 0.5 μg/L (0.001 μM) to 28 mg/L (120 μM). Results Mice that drank uranium-containing water exhibited estrogenic responses including selective reduction of primary follicles, increased uterine weight, greater uterine luminal epithelial cell height, accelerated vaginal opening, and persistent presence of cornified vaginal cells. Coincident treatment with the antiestrogen ICI 182,780 blocked these responses to uranium or the synthetic estrogen diethylstilbestrol. In addition, mouse dams that drank uranium-containing water delivered grossly normal pups, but they had significantly fewer primordial follicles than pups whose dams drank control tap water. Conclusions Because of the decades of uranium mining/milling in the Colorado plateau in the Four Corners region of the American Southwest, the uranium concentration and the route of exposure used in these studies are environmentally relevant. Our data support the conclusion that uranium is an endocrine-disrupting chemical and populations exposed to environmental uranium should be followed for increased risk of fertility problems and reproductive cancers. PMID:18087588

  1. Observational studies as human experimentation: the uranium mining experience in the Navajo Nation (1947-66).

    PubMed

    Moure-Eraso, R

    1999-01-01

    This article evaluates how an observational epidemiologic study of federal agencies in uranium miners became an experiment of opportunity for radiation effects. Navajo miners and communities suffered environmental exposures caused by the practices of uranium mining and milling in the Navajo reservation during the 1947 to 1966 period. A historical review of the state-of-the-art knowledge of the health effects of uranium mining and milling during the years prior to 1947 was conducted. Contemporary prevention and remediation practices also were assessed. An appraisal of the summary of findings of a comprehensive evaluation of radiation human experimentation conducted by the U.S. federal government in 1995-96 (ACHRE) demonstrates that uranium miners, including Navajo miners, were the single group that was put more seriously at risk of harm from radiation exposures, with inadequate disclosure and often with fatal consequences. Uranium miners were unwilling and unaware victims of human experimentation to evaluate the health effects of radiation. The failure of the State and U.S. Governments to issue regulations or demand installation of known mine-dust exposure control measures caused widespread environmental damage in the Navajo Nation.

  2. A top-down assessment of energy, water and land use in uranium mining, milling, and refining

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    E. Schneider; B. Carlsen; E. Tavrides

    2013-11-01

    Land, water and energy use are key measures of the sustainability of uranium production into the future. As the most attractive, accessible deposits are mined out, future discoveries may prove to be significantly, perhaps unsustainably, more intensive consumers of environmental resources. A number of previous attempts have been made to provide empirical relationships connecting these environmental impact metrics to process variables such as stripping ratio and ore grade. These earlier attempts were often constrained by a lack of real world data and perform poorly when compared against data from modern operations. This paper conditions new empirical models of energy, watermore » and land use in uranium mining, milling, and refining on contemporary data reported by operating mines. It shows that, at present, direct energy use from uranium production represents less than 1% of the electrical energy produced by the once-through fuel cycle. Projections of future energy intensity from uranium production are also possible by coupling the empirical models with estimates of uranium crustal abundance, characteristics of new discoveries, and demand. The projections show that even for the most pessimistic of scenarios considered, by 2100, the direct energy use from uranium production represents less than 3% of the electrical energy produced by the contemporary once-through fuel cycle.« less

  3. 37. VIEW NORTH FROM EAST CRUDE ORE BIN TO CRUSHER ...

    Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

    37. VIEW NORTH FROM EAST CRUDE ORE BIN TO CRUSHER ADDITION AND CRUSHED OXIDIZED ORE BIN. VISIBLE ARE DINGS MAGNETIC PULLEY (CENTER), THE 100-TON STEEL CRUSHED UNOXIDIZED ORE BIN, AND UPPER PORTION OF THE STEPHENS-ADAMSON 25 TON/HR BUCKET ELEVATOR. THE UPPER TAILINGS POND LIES BEYOND THE MILL WITH THE UPPER TAILINGS DAM UNDER THE GRAVEL ROAD IN THE UPPER RIGHT CORNER. - Bald Mountain Gold Mill, Nevada Gulch at head of False Bottom Creek, Lead, Lawrence County, SD

  4. Map showing radon potential of rocks and soils in Fairfax County, Virginia

    USGS Publications Warehouse

    Otton, James K.; Schumann, R. Randall; Owen, Douglass E.; Thurman, Nelson; Duval, Joseph S.

    1988-01-01

    Since 1984, indoor radon has gained national attention as a significant health hazard in the United States. Radon is a colorless, odorless, radioactive gas derived from uranium by radioactive decay. The U.S. Environmental Protection Agency (EPA) now projects that 5,000 to 20,000 lung-cancer deaths per year may be attributed to the long-term exposure to indoor radon and its radioactive decay products. Indoor radon has been previously recognized as a health hazard associated with uranium-bearing mill tailings or building materials, but it was not until December 1984 that some natural soils and rocks were found to be sources of indoor radon at levels comparable to those in uranium mines. It is now suspected that elevated indoor radon levels are far more widespread than initially though. The EPA considers 4 picoCuries of radon per liter of air (pCi/L) as the level (in a year-round measurement) at which actions ought to be taken to lower the concentration of indoor radon. All soils and rocks contain measurable amounts of uranium, which generate measurable amounts of radon. Certain soils and rocks, however, have a greater potential to cause indoor radon problems than others because (1) they have a higher uranium content and thus can generate higher levels of radon in soil gas (gas that occupies the pores of the soil), and (2) the permeability of the sol or rack is sufficiently high that radon-bearing soil gas can flow freely and move indoors through the foundation of the structure. This study was designed to demonstrate the correlation between the geologic environment and indoor radon levels and to demonstrate a method of assessment that could be used by other informed workers in areas of their interest. A parallel study by Gundersen and others (1988) of the radon potential of rocks and soils in Montgomery County, Md., used somewhat different methods of assessment because the data available for and assessment of Montgomery County differed.

  5. 16. VIEW OF A ROLLING MILL THAT WAS USED TO ...

    Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

    16. VIEW OF A ROLLING MILL THAT WAS USED TO CREATE A METAL SHEET (SHOWN). (4/16/57) - Rocky Flats Plant, Uranium Rolling & Forming Operations, Southeast section of plant, southeast quadrant of intersection of Central Avenue & Eighth Street, Golden, Jefferson County, CO

  6. Office of Legacy Management Decision Tree for Solar Photovoltaic Projects - 13317

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Elmer, John; Butherus, Michael; Barr, Deborah L.

    2013-07-01

    To support consideration of renewable energy power development as a land reuse option, the DOE Office of Legacy Management (LM) and the National Renewable Energy Laboratory (NREL) established a partnership to conduct an assessment of wind and solar renewable energy resources on LM lands. From a solar capacity perspective, the larger sites in the western United States present opportunities for constructing solar photovoltaic (PV) projects. A detailed analysis and preliminary plan was developed for three large sites in New Mexico, assessing the costs, the conceptual layout of a PV system, and the electric utility interconnection process. As a result ofmore » the study, a 1,214-hectare (3,000-acre) site near Grants, New Mexico, was chosen for further study. The state incentives, utility connection process, and transmission line capacity were key factors in assessing the feasibility of the project. LM's Durango, Colorado, Disposal Site was also chosen for consideration because the uranium mill tailings disposal cell is on a hillside facing south, transmission lines cross the property, and the community was very supportive of the project. LM worked with the regulators to demonstrate that the disposal cell's long-term performance would not be impacted by the installation of a PV solar system. A number of LM-unique issues were resolved in making the site available for a private party to lease a portion of the site for a solar PV project. A lease was awarded in September 2012. Using a solar decision tree that was developed and launched by the EPA and NREL, LM has modified and expanded the decision tree structure to address the unique aspects and challenges faced by LM on its multiple sites. The LM solar decision tree covers factors such as land ownership, usable acreage, financial viability of the project, stakeholder involvement, and transmission line capacity. As additional sites are transferred to LM in the future, the decision tree will assist in determining whether a solar PV project is feasible on the new sites. (authors)« less

  7. Uranium mining wastes, garden exhibition and health risks

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Schmidt, Gerhard; Schmidt, Peter; Hinz, Wilko

    2007-07-01

    Available in abstract form only. Full text of publication follows: For more than 40 years the Soviet-German stockholding company SDAG WISMUT mined and milled Uranium in the East of Germany and became up to 1990 the world's third largest Uranium producer. After reunification of Germany, the new found state own company Wismut GmbH was faced with the task of decommissioning and rehabilitation of the mining and milling sites. One of the largest mining areas in the world, that had to be cleaned up, was located close to the municipality of Ronneburg near the City of Gera in Thuringia. After closingmore » the operations of the Ronneburg underground mine and at the 160 m deep open pit mine with a free volume of 84 Mio.m{sup 3}, the open pit and 7 large piles of mine waste, together 112 Mio.m{sup 3} of material, had to be cleaned up. As a result of an optimisation procedure it was chosen to relocate the waste rock piles back into the open pit. After taking this decision and approval of the plan the disposal operation was started. Even though the transport task was done by large trucks, this took 16 years. The work will be finished in 2007, a cover consisting of 40 cm of uncontaminated material will be placed on top of the material, and the re-vegetation of the former open pit area will be established. When in 2002 the City of Gera applied to host the largest garden exhibition in Germany, Bundesgartenschau (BUGA), in 2007, Wismut GmbH supported this plan by offering parts of the territory of the former mining site as an exhibition ground. Finally, it was decided by the BUGA organizers to arrange its 2007 exhibition on grounds in Gera and in the valley adjacent to the former open pit mine, with parts of the remediated area within the fence of the exhibition. (authors)« less

  8. OVERVIEW OF CYANIDE PLANT REMAINS, TAILINGS PILES, PARKING LOT, AND ...

    Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

    OVERVIEW OF CYANIDE PLANT REMAINS, TAILINGS PILES, PARKING LOT, AND MINE MANAGER'S HOME, LOOKING SOUTH SOUTHEAST. RIGHT, TAILINGS PILES ARE AT CENTER WITH CYANIDE PLANT FOUNDATIONS TO THE LEFT OF THE PILES. PARKING LOT IS AT UPPER LEFT. THE AREA BETWEEN THE COLLAPSED TANK AT CENTER LEFT AND THE REMAINS OF THE MANAGER'S HOUSE AT LOWER RIGHT IS A TAILINGS HOLDING AREA. TAILINGS FROM THE MILL WERE HELD HERE. THE LARGE SETTLING TANKS WERE CHARGED FROM THIS HOLDING AREA BY A TRAM ON RAILS AND BY A SLUICEWAY SEEN AS THE DARK SPOT ON THE CENTER LEFT EDGE OF THE FRAME. AFTER THE TAILINGS WERE LEACHED, THEY WERE DEPOSITED ON THE LARGE WASTE PILE AT CENTER RIGHT. THE TANK AT CENTER RIGHT EDGE IS WHERE THE WATER PIPELINE ENTERED THE WORKS. A STRAIGHT LINE OF POSTS IN THE GROUND GO ACROSS THE CENTER FROM LEFT TO RIGHT, WHICH ORIGINALLY SUSPENDED THE WATER PIPELINE GOING FROM THE WATER HOLDING TANK AT RIGHT UP TO THE SECONDARY WATER TANKS ABOVE THE MILL. - Keane Wonder Mine, Park Route 4 (Daylight Pass Cutoff), Death Valley Junction, Inyo County, CA

  9. 77 FR 14837 - Bioassay at Uranium Mills

    Federal Register 2010, 2011, 2012, 2013, 2014

    2012-03-13

    ..., Revision 1 was issued. Comments related to the operation of in-situ recovery mills and associated... received on or before this date. Although a time limit is given, comments and suggestions in connection with items for inclusion in guides currently being developed or improvements in all published guides...

  10. Simplified behaviors from increased heterogeneity: I. 2-D uranium transport experiments at the decimeter scale.

    PubMed

    Miller, Andrew W; Rodriguez, Derrick R; Honeyman, Bruce D

    2013-05-01

    Intermediate scale tank studies were conducted to examine the effects of physical heterogeneity of aquifer material on uranium desorption and subsequent transport in order to bridge the scaling gap between bench and field scale systems. Uranium contaminated sediment from a former uranium mill field site was packed into two 2-D tanks with internal dimensions of 2.44×1.22×0.076 m (tank 1) and 2.44×0.61×0.076 m (tank 2). Tank 1 was packed in a physically homogenous manner, and tank 2 was packed with long lenses of high and low conductivities resulting in different flow fields within the tanks. Chemical gradients within the flow domain were altered by temporal changes in influent water chemistry. The uranium source was desorption from the sediment. Despite the physical differences in the flow fields, there were minimal differences in global uranium leaching behavior between the two tanks. The dominant uranium species in both tanks over time and space was Ca2UO2(CO3)3(0). However, the uranium/alkalinity relationships varied as a function of time in tank 1 and were independent of time in tank 2. After planned stop-flow events, small, short-lived rebounds were observed in tank 1 while no rebound of uranium concentrations was observed in tank 2. Despite appearing to be in local equilibrium with respect to uranium desorption, a previously derived surface complexation model was insufficient to describe uranium partitioning within the flow domain. This is the first in a pair of papers; the companion paper presents an intermediate scale 3-D tank experiment and inter-tank comparisons. For these systems, physical heterogeneity at or above the decimeter scale does not affect global scale uranium desorption and transport. Instead, uranium fluxes are controlled by chemistry dependent desorption patterns induced by changing the influent ionic composition. Published by Elsevier B.V.

  11. Simplified behaviors from increased heterogeneity: I. 2-D uranium transport experiments at the decimeter scale

    NASA Astrophysics Data System (ADS)

    Miller, Andrew W.; Rodriguez, Derrick R.; Honeyman, Bruce D.

    2013-05-01

    Intermediate scale tank studies were conducted to examine the effects of physical heterogeneity of aquifer material on uranium desorption and subsequent transport in order to bridge the scaling gap between bench and field scale systems. Uranium contaminated sediment from a former uranium mill field site was packed into two 2-D tanks with internal dimensions of 2.44 × 1.22 × 0.076 m (tank 1) and 2.44 × 0.61 × 0.076 m (tank 2). Tank 1 was packed in a physically homogenous manner, and tank 2 was packed with long lenses of high and low conductivities resulting in different flow fields within the tanks. Chemical gradients within the flow domain were altered by temporal changes in influent water chemistry. The uranium source was desorption from the sediment. Despite the physical differences in the flow fields, there were minimal differences in global uranium leaching behavior between the two tanks. The dominant uranium species in both tanks over time and space was Ca2UO2(CO3)30. However, the uranium/alkalinity relationships varied as a function of time in tank 1 and were independent of time in tank 2. After planned stop-flow events, small, short-lived rebounds were observed in tank 1 while no rebound of uranium concentrations was observed in tank 2. Despite appearing to be in local equilibrium with respect to uranium desorption, a previously derived surface complexation model was insufficient to describe uranium partitioning within the flow domain. This is the first in a pair of papers; the companion paper presents an intermediate scale 3-D tank experiment and inter-tank comparisons. For these systems, physical heterogeneity at or above the decimeter scale does not affect global scale uranium desorption and transport. Instead, uranium fluxes are controlled by chemistry dependent desorption patterns induced by changing the influent ionic composition.

  12. Integrated Geophysical Measurements for Bioremediation Monitoring: Combining Spectral Induced Polarization, Nuclear Magnetic Resonance and Magnetic Methods

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Keating, Kristina; Slater, Lee; Ntarlagiannis, Dimitris

    2015-02-24

    This documents contains the final report for the project "Integrated Geophysical Measurements for Bioremediation Monitoring: Combining Spectral Induced Polarization, Nuclear Magnetic Resonance and Magnetic Methods" (DE-SC0007049) Executive Summary: Our research aimed to develop borehole measurement techniques capable of monitoring subsurface processes, such as changes in pore geometry and iron/sulfur geochemistry, associated with remediation of heavy metals and radionuclides. Previous work has demonstrated that geophysical method spectral induced polarization (SIP) can be used to assess subsurface contaminant remediation; however, SIP signals can be generated from multiple sources limiting their interpretation value. Integrating multiple geophysical methods, such as nuclear magnetic resonance (NMR)more » and magnetic susceptibility (MS), with SIP, could reduce the ambiguity of interpretation that might result from a single method. Our research efforts entails combining measurements from these methods, each sensitive to different mineral forms and/or mineral-fluid interfaces, providing better constraints on changes in subsurface biogeochemical processes and pore geometries significantly improving our understanding of processes impacting contaminant remediation. The Rifle Integrated Field Research Challenge (IFRC) site was used as a test location for our measurements. The Rifle IFRC site is located at a former uranium ore-processing facility in Rifle, Colorado. Leachate from spent mill tailings has resulted in residual uranium contamination of both groundwater and sediments within the local aquifer. Studies at the site include an ongoing acetate amendment strategy, native microbial populations are stimulated by introduction of carbon intended to alter redox conditions and immobilize uranium. To test the geophysical methods in the field, NMR and MS logging measurements were collected before, during, and after acetate amendment. Next, laboratory NMR, MS, and SIP measurements were collected on columns of Rifle sediments during acetate amendment. The laboratory experiments were designed to simulate the field experiments; changes in geophysical signals were expected to correlate with changes in redox conditions and iron speciation. Field MS logging measurements revealed vertically stratified magnetic mineralization, likely the result of detrital magnetic fraction within the bulk alluvium. Little to no change was observed in the MS data suggesting negligible production of magnetic phases (e.g. magnetite, pyrrhotite) as a result of sulfidogenesis. Borehole NMR measurements contained high levels of noise contamination requiring significant signal processing, and analysis suggests that any changes may be difficult to differentiate from simultaneous changes in water content. Laboratory MS and NMR measurements remained relatively stable throughout the course of the acetate amendment experiment, consistent with field measurements. However, SIP measurements changed during the acetate amendment associated with the formation of iron-sulfide mineral phases; a finding that is consistent with chemical analysis of the solid phase materials in the columns.« less

  13. Transfer coefficient of 226Ra from vegetation to meadow voles, Microtus pennsylvanicus, on U mill tailings

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Cloutier, N.R.; Clulow, F.V.; Lim, T.P.

    The 226Ra level in vegetation growing on U mine tailings in Elliot Lake, Ontario, Canada, was 211 + 22 mBq g-1 (dry weight) compared to less than 7 mBq g-1 (dry weight) in material from a control site. Skeletons of meadow voles (Microtus pennsylvanicus) established on the tailings had concentrations of 226Ra of 6083 +/- 673 mBq per animal in winter; 7163 +/- 1077 mBq per animal in spring; 1506 +/- 625 mBq per animal in summer; and 703 +/- 59 mBq per animal in fall, compared to less than 7 mBq per animal in controls. The /sup 226/Ra transfermore » coefficient from vegetation to voles (defined as total millibecquerels of /sup 226/Ra in adult vole per total millibecquerels of 226Ra consumed by the vole in its lifetime) was calculated as 4.6 +/- 2.9 X 10(-2) in summer and 2.8 +/- 0.6 X 10(-2) in fall.« less

  14. 5. VIEW OF BERYLLIUM PROCESSING AREA, ROLLING MILL. BERYLLIUM FORMING ...

    Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

    5. VIEW OF BERYLLIUM PROCESSING AREA, ROLLING MILL. BERYLLIUM FORMING BEGAN IN SIDE A OF THE BUILDING IN 1962. (11/5/73) - Rocky Flats Plant, Uranium Rolling & Forming Operations, Southeast section of plant, southeast quadrant of intersection of Central Avenue & Eighth Street, Golden, Jefferson County, CO

  15. Variably Saturated Flow and Multicomponent Biogeochemical Reactive Transport Modeling of a Uranium Bioremediation Field Experiment

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Yabusaki, Steven B.; Fang, Yilin; Williams, Kenneth H.

    2011-11-01

    Field experiments at a former uranium mill tailings site have identified the potential for stimulating indigenous bacteria to catalyze the conversion of aqueous uranium in the +6 oxidation state to immobile solid-associated uranium in the +4 oxidation state. This effectively removes uranium from solution resulting in groundwater concentrations below actionable standards. Three-dimensional, coupled variably-saturated flow and biogeochemical reactive transport modeling of a 2008 in situ uranium bioremediation field experiment is used to better understand the interplay of transport rates and biogeochemical reaction rates that determine the location and magnitude of key reaction products. A comprehensive reaction network, developed largely throughmore » previous 1-D modeling studies, was used to simulate the impacts on uranium behavior of pulsed acetate amendment, seasonal water table variation, spatially-variable physical (hydraulic conductivity, porosity) and geochemical (reactive surface area) material properties. A principal challenge is the mechanistic representation of biologically-mediated terminal electron acceptor process (TEAP) reactions whose products significantly alter geochemical controls on uranium mobility through increases in pH, alkalinity, exchangeable cations, and highly reactive reduction products. In general, these simulations of the 2008 Big Rusty acetate biostimulation field experiment in Rifle, Colorado confirmed previously identified behaviors including (1) initial dominance by iron reducing bacteria that concomitantly reduce aqueous U(VI), (2) sulfate reducing bacteria that become dominant after {approx}30 days and outcompete iron reducers for the acetate electron donor, (3) continuing iron-reducer activity and U(VI) bioreduction during dominantly sulfate reducing conditions, and (4) lower apparent U(VI) removal from groundwater during dominantly sulfate reducing conditions. New knowledge on simultaneously active metal and sulfate reducers has been incorporated into the modeling. In this case, an initially small population of slow growing sulfate reducers is active from the initiation of biostimulation. Three-dimensional, variably saturated flow modeling was used to address impacts of a falling water table during acetate injection. These impacts included a significant reduction in aquifer saturated thickness and isolation of residual reactants and products, as well as unmitigated uranium, in the newly unsaturated vadose zone. High permeability sandy gravel structures resulted in locally high flow rates in the vicinity of injection wells that increased acetate dilution. In downgradient locations, these structures created preferential flow paths for acetate delivery that enhanced local zones of TEAP reactivity and subsidiary reactions. Conversely, smaller transport rates associated with the lower permeability lithofacies (e.g., fine) and vadose zone were shown to limit acetate access and reaction. Once accessed by acetate, however, these same zones limited subsequent acetate dilution and provided longer residence times that resulted in higher concentrations of TEAP products when terminal electron donors and acceptors were not limiting. Finally, facies-based porosity and reactive surface area variations were shown to affect aqueous uranium concentration distributions; however, the ranges were sufficiently small to preserve general trends. Large computer memory and high computational performance were required to simulate the detailed coupled process models for multiple biogeochemical components in highly resolved heterogeneous materials for the 110-day field experiment and 50 days of post-biostimulation behavior. In this case, a highly-scalable subsurface simulator operating on 128 processor cores for 12 hours was used to simulate each realization. An equivalent simulation without parallel processing would have taken 60 days, assuming sufficient memory was available.« less

  16. Profile of a Rural Area Work Force: The Wyoming Uranium Industry.

    ERIC Educational Resources Information Center

    Dobbs, Thomas L.; Kiner, Phil E.

    1974-01-01

    Designed to provide insights into policies relative to human resource investments and employment information channels, the study's objectives were to: (1) relate types of employment in Wyoming's uranium mines and mills to work force participants; (2) determine employee earnings and relate those earnings to employment categories and…

  17. 40 CFR 440.34 - New source performance standards (NSPS).

    Code of Federal Regulations, 2011 CFR

    2011-07-01

    ... uranium ore, excluding mines using in situ leach methods, shall not exceed: Effluent characteristic... for the extraction of uranium or from mines and mills using in situ leach methods. The Agency... Subcategory § 440.34 New source performance standards (NSPS). Except as provided in subpart L of this part any...

  18. 40 CFR 440.34 - New source performance standards (NSPS).

    Code of Federal Regulations, 2010 CFR

    2010-07-01

    ... uranium ore, excluding mines using in situ leach methods, shall not exceed: Effluent characteristic... for the extraction of uranium or from mines and mills using in situ leach methods. The Agency... Subcategory § 440.34 New source performance standards (NSPS). Except as provided in subpart L of this part any...

  19. Development of Triad approach based system for ecological risk assessment for contaminated areas of Kyrgyzstan

    NASA Astrophysics Data System (ADS)

    Kydralieva, Kamilia; Uzbekov, Beksultan; Khudaibergenova, Bermet; Terekhova, Vera; Jorobekova, Sharipa

    2014-05-01

    This research is aimed to develop a high-effective system of an ecological risk assessment and risk-based decision making for anthropogenic ecosystems, with particular focus on the soils of the Kyrgyz Republic. The study is focused on the integration of Triad data including chemical, biological and ecotoxicological soil markers to estimate the potential risk from soils of highly anthropized areas impacted by deposition of different pollutants from mining operation. We focus on technogenic areas of Kyrgyzstan, the former uranium-producing province. Triad-based ecological risk assessment for technogenic sites are not currently used in Kyrgyzstan. However, the vitality of such research is self-evident. There are about 50 tailing dumps and more than 80 tips of radioactive waste which are formed as a result of uranium and complex ores (mercury, antimony, lead, cadmium and etc) mining around the unfavorable aforementioned places. According to the Mining Wastes' Tailings and Fills Rehabilitation Centre established in 1999 by a special Government's Resolution, one of the most ecologically dangerous uranium tailings resides in Kadzhi-Say. Although uranium processing is no longer practiced in Kadzhi-Say, a large number of open landfills and uranium ore storages still remain abandoned at the vicinity of this settlement. These neglected sites have enormous problems associated with soil erosion known as "technogenic deserts". The upper soil horizons are deprived of humus and vegetation, which favor the formation of low-buffer landscapes in the zones of maximum contamination. As a result, most of these areas are not re-cultivated and remain in critical environmental condition (Bykovchenko, et al., 2005; Tukhvatshin, 2005; Suranova, 2006). Triad data for assessing environmental risk and biological vulnerability at contaminated sites will be integrated. The following Triad-based parameters will be employed: 1) chemical soil analyses (revealing the presence of potentially dangerous substances), 2) ecological parameters (assessing changes in microorganism's community structure and functions, bioindication); and 3) toxicological bioassays (utilizing classical endpoints such as survival and reproduction rates, genotoxicity). The output will be consisted of 3 indexes: 1) Environmental Risk Index, quantifying the level of biological damage at population-community level, 2) Biological Vulnerability Index, assessing the potential threats to biological equilibria, and 3) Genotoxicity Index, screening genotoxic effects. Multi-criteria Decision Analysis (MCDA) will be used to integrate a set of environmental Triad data to be obtained during the project, which will be carried out in order to estimate the potential risk from soil contamination of the highly anthropized areas of Kadzhi-Say, which have been impacted by deposition of heavy metals. The basis of the development under this research is studies with a particular focus concerning the biocenosis mapping of Kyrgyz soils (Mamytova et al., 2003, 2010), investigations on interaction of humic substances with soil contaminants (Jorobekova, Kydralieva, Khudaibergenova, 2004; Khudaibergenova, 2005, 2007), and in addition, technical approach for ecotoxicological assessment of soils (Terekhova, 2007, 2011). Soil ecotoxicological estimation has been studied with a battery of tests using test-organisms of many trophic levels. Currently, bioindication of soils with various humus states is under study (Senesi, Yakimenko 2007; Yakimenko, et al., 2008).

  20. Study on the Classification of the Uranium Mineral of Venta de Cardena; ESTUDIO SOBRE LA CLASIFICACION DEL MINERAL DE VENTA DE CARDENA

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Otero, A.R.

    1959-01-01

    The behavior of uranium mineral from Venta de Cardena in a spiral classifier which operates in a closed system with a ball mill was studied to obtain data for the design of a milling-classification system with a production capacity of 200 tons per day with a particle size less than 0.417 mm. The characteristics of such a system, the problems in normal operation, the inconveriences which these cause, and their solution were investigated. Correlations between these tests and the results obtained with long glass tubes are presented. (J.S.R.)

  1. The Sequoyah corporation fuels release and the Church Rock spill: unpublicized nuclear releases in American Indian communities.

    PubMed

    Brugge, Doug; deLemos, Jamie L; Bui, Cat

    2007-09-01

    The Three Mile Island nuclear release exemplifies why there is public and policy interest in the high-technology, highly visible end of the nuclear cycle. The environmental and health consequences of the early steps in the cycle--mining, milling, and processing of uranium ore--may be less appreciated. We examined 2 large unintended acute releases of uranium--at Kerr McGee's Sequoyah Fuels Corporation in Oklahoma and United Nuclear Corporation's Church Rock uranium mill in New Mexico, which were incidents with comparable magnitude to the Three Mile Island release. We urge exploration of whether there is limited national interest and concern for the primarily rural, low-income, and American Indian communities affected by these releases. More attention should be given to the early stages of the nuclear cycle and their impacts on health and the environment.

  2. Heavy metal contamination of a Greenland Fjord system by mine wastes

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Loring, D.H.; Asmund, G.

    Since 1973, about 500,000 tons/yr of metal-rich particulate tailings from a lead/zinc flotation mill have been discharged through a submarine outfall into a two-fjord system on the west coast of Greenland. Differential solubilization of particulate metals by seawater, seasonal water mixing, and sill exchange tailings dispersal processes have resulted in high, but seasonally variable, Zn, Cd, and Pb contamination of the water and suspended particulate matter (SPM). Chemical partition of the SPM shows that most of the Pb, but relatively low proportions of Zn and Cd are weakly bound to the SPM. Such particulate metal characteristics allow the real timemore » effects of tailings discharges and dispersal on the system to be traced even in the sediments where tailings accumulation is very slow. Fjord seaweeds and blue mussels also contain varying amounts of Zn, Pb, and Cd, depending on the metal and their location relative to the tailings outfall. They apparently responded almost instantly to the metal contamination as did the water and SPM. High Pb concentrations in the fjord mussels most likely derive from the preferential uptake of available particulate Pb, whereas the seaweeds appear to derive most of their heavy metal concentrations from the dissolved phase. The evidence from this and other sites, and from experimental work, indicates that any discharge of Pb-particles into the marine environment, either directly as mine wastes or indirectly from natural runoff from current and former lead mining sites, results in immediate lead contamination of the in situ mussel population. 20 refs., 4 figs., 5 tab.« less

  3. Geochemical Analyses of Rock, Sediment, and Water from the Region In and Around the Tuba City Landfill, Tuba City, Arizona

    USGS Publications Warehouse

    Johnson, Raymond H.; Wirt, Laurie

    2009-01-01

    The Tuba City Landfill (TCL) started as an unregulated waste disposal site in the 1940s and was administratively closed in 1997. Since the TCL closure, radionuclides have been detected in the shallow ground water. In 2006, the Bureau of Indian Affairs (BIA) contracted with the U.S. Geological Survey (USGS) to better understand the source of radionuclides in the ground water at the TCL compared to the surrounding region. This report summarizes those data and presents interpretations that focus on the geochemistry in the rocks and water from the Tuba City region. The TCL is sited on Navajo Sandstone above the contact with the Kayenta Formation. These formations are not rich in uranium but generally are below average crustal abundance values for uranium. Uranium ores in the area were mined nearby in the Chinle Formation and processed at the Rare Metals mill (RMM). Regional samples of rock, sediment, leachates, and water were collected in and around the TCL site and analyzed for major and minor elements, 18O, 2H, 3H, 13C, 14C,34S, 87Sr, and 234U/238U, as appropriate. Results of whole rock and sediment samples, along with leachates, suggest the Chinle Formation is a major source of uranium and other trace elements in the area. Regional water samples indicate that some of the wells within the TCL site have geochemical signatures that are different from the regional springs and surface water. The geochemistry from these TCL wells is most similar to leachates from the Chinle Formation rocks and sediments. Isotope samples do not uniquely identify TCL-derived waters, but they do provide a useful indicator for shallow compared to deep ground-water flow paths and general rock/water interaction times. Information in this report provides a comparison between the geochemistry within the TCL and in the region as a whole.

  4. Navajo Uranium Education Programs: The Search for Environmental Justice

    ERIC Educational Resources Information Center

    Charley, Perry H.; Dawson, Susan E.; Madsen, Gary E.; Spykerman, Bryan R.

    2004-01-01

    Uranium mining and milling in the Four Corners' area of the American Southwest has had serious negative impacts on American Indian workers, their families, and their communities. In this article, we will examine Navajo education programs which inform citizens about risks and health impacts associated with radiation exposures. Because the Navajo…

  5. 40 CFR 440.34 - New source performance standards (NSPS).

    Code of Federal Regulations, 2013 CFR

    2013-07-01

    ... underground, that produce uranium ore, excluding mines using in situ leach methods, shall not exceed: Effluent... leach process for the extraction of uranium or from mines and mills using in situ leach methods. The... Vanadium Ores Subcategory § 440.34 New source performance standards (NSPS). Except as provided in subpart L...

  6. 40 CFR 440.34 - New source performance standards (NSPS).

    Code of Federal Regulations, 2012 CFR

    2012-07-01

    ... underground, that produce uranium ore, excluding mines using in situ leach methods, shall not exceed: Effluent... leach process for the extraction of uranium or from mines and mills using in situ leach methods. The... Vanadium Ores Subcategory § 440.34 New source performance standards (NSPS). Except as provided in subpart L...

  7. 40 CFR 440.34 - New source performance standards (NSPS).

    Code of Federal Regulations, 2014 CFR

    2014-07-01

    ... underground, that produce uranium ore, excluding mines using in situ leach methods, shall not exceed: Effluent... leach process for the extraction of uranium or from mines and mills using in situ leach methods. The... Vanadium Ores Subcategory § 440.34 New source performance standards (NSPS). Except as provided in subpart L...

  8. Outdoor (222)Rn-concentrations in Germany - part 2 - former mining areas.

    PubMed

    Kümmel, M; Dushe, C; Müller, S; Gehrcke, K

    2014-06-01

    In the German Federal States of Saxony, Saxony-Anhalt and Thuringia, centuries of mining and milling activities resulted in numerous residues with increased levels of natural radioactivity such as waste rock dumps and tailings ponds. These may have altered potential radiation exposures of the population significantly. Especially waste rock dumps from old mining activities as well as 20th century uranium mining may, due to their radon ((222)Rn) exhalation capacity, lead to significant radiation exposures. They often lie close to or within residential areas. In order to study the impact on the natural radon level, the Federal Office for Radiation Protection (BfS) has run networks of radon measurement points in 16 former mining areas, together with 2 networks in regions not influenced by mining for comparison purposes. Representative overviews of the long-term outdoor radon concentrations could be established including estimates of regional background concentrations. Former mining and milling activities did not result in large-area impacts on the outdoor radon level. However, significantly increased radon concentrations were observed in close vicinity of shafts and large waste rock dumps. They are partly located in residential areas and need to be considered under radiation protection aspects. Examples are given that illustrate the consequences of the Wismut Ltd. Company's reclamation activities on the radon situation. Copyright © 2014 Elsevier Ltd. All rights reserved.

  9. Investigation of background radiation levels and geologic unit profiles in Durango, Colorado

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Triplett, G.H.; Foutz, W.L.; Lesperance, L.R.

    1989-11-01

    As part of the Uranium Mill Tailings Remedial Action (UMTRA) Project, Oak Ridge National Laboratory (ORNL) has performed radiological surveys on 435 vicinity properties (VPs) in the Durango area. This study was undertaken to establish the background radiation levels and geologic unit profiles in the Durango VP area. During the months of May through June, 1986, extensive radiometric measurements and surface soil samples were collected in the Durango VP area by personnel from ORNL's Grand Junction Office. A majority of the Durango VP surveys were conducted at sites underlain by Quaternary alluvium, older Quaternary gravels, and Cretaceous Lewis and Mancosmore » shales. These four geologic units were selected to be evaluated. The data indicated no formation anomalies and established regional background radiation levels. Durango background radionuclide concentrations in surface soil were determined to be 20.3 {plus minus} 3.4 pCi/g for {sup 40}K, 1.6 {plus minus} 0.5 pCi/g for {sup 226}Ra, and 1.2 {plus minus} 0.3 pCi/g for {sup 232}Th. The Durango background gamma exposure rate was found to be 16.5 {plus minus} 1.3 {mu}R/h. Average gamma spectral count rate measurements for {sup 40}K, {sup 226}Ra and {sup 232}Th were determined to be 553, 150, and 98 counts per minute (cpm), respectively. Geologic unit profiles and Durango background radiation measurements are presented and compared with other areas. 19 refs., 15 figs., 5 tabs.« less

  10. Mitigation and Monitoring Plan for impacted wetlands at the Gunnison UMTRA Project site, Gunnison, Colorado. Revision 1

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1994-12-01

    The Gunnison, Colorado, abandoned uranium mill site is one site being cleaned up by the DOE under UMTRCA authority. This site`s contaminated material is being transported to a disposal site on US Bureau of Land Management (BLM) land east of Gunnison. Remedial action activities have temporarily disturbed 0.8 acre (ac) (0.3 hectares [ha]) of wetlands and permanently eliminated 4.3 ac (1.7 ha). As required by the Clean Water Act, the US Army Corps of Engineers (USACE) prepared a Section 404 Permit that addresses the loss of wetlands as a result of remedial action at the Gunnison UMTRA Project site. Themore » 404 permit includes this report as an attachment and it describes the wetland mitigation and monitoring plan. The DOE formulated this plan in consultation with the BLM and the USACE. This report represents a revised version of the mitigation and monitoring plan (DOE, 1992b).« less

  11. Temporal Chemical Data for Sediment, Water, and Biological Samples from the Lava Cap Mine Superfund Site, Nevada County, California-2006-2008

    USGS Publications Warehouse

    Foster, Andrea L.; Ona-Nguema, Georges; Tufano, Kate; White, Richard III

    2010-01-01

    The Lava Cap Mine is located about 6 km east of the city of Grass Valley, Nevada County, California, at an elevation of about 900 m. Gold was hosted in quartz-carbonate veins typical of the Sierran Gold Belt, but the gold grain size was smaller and the abundance of sulfide minerals higher than in typical deposits. The vein system was discovered in 1860, but production was sporadic until the 1930s when two smaller operations on the site were consolidated, a flotation mill was built, and a 100-foot deep adit was driven to facilitate drainage and removal of water from the mine workings, which extended to 366 m. Peak production at the Lava Cap occurred between 1934 and 1943, when about 90,000 tons of ore per year were processed. To facilitate removal of the gold and accessory sulfide minerals, the ore was crushed to a very fine sand or silt grain size for processing. Mining operations at Lava Cap ceased in June 1943 due to War Production Board Order L-208 and did not resume after the end of World War II. Two tailings retention structures were built at the Lava Cap Mine. The first was a log dam located about 0.4 km below the flotation mill on Little Clipper Creek, and the second, built in 1938, was a larger earth fill and rip-rap structure constructed about 2 km downstream, which formed the water body now called Lost Lake. The log dam failed during a storm that began on December 31, 1996, and continued into January 1997; an estimated 8,000-10,000 m3 of tailings were released into Little Clipper Creek during this event. Most of the fine tailings were deposited in Lost Lake, dramatically increasing its turbidity and resulting in a temporary 1-1.5 m rise in lake level due to debris blocking the dam spillway. When the blockage was cleared, the lake level quickly lowered, leaving a ?bathtub ring? of very fine tailings deposited substantially above the water line. The U.S. Environmental Protection Agency (EPA) initiated emergency action in late 1997 at the mine site to reduce the possibility of future movement of tailings, and began an assessment of the risks posed by physical and chemical hazards at the site. The EPA's assessment identified arsenic (As) as the primary hazard of concern. Three main exposure routes were identified: inhalation/ingestion of mine tailings, dermal absorption/ingestion of As in lake water from swimming, and ingestion of As-contaminated ground water or surface water. Lost Lake is a private lake which is completely surrounded by low-density residential development. Prior to the dam failure, the lake was used by the local residents for swimming and boating. An estimated 1,776 people reside within one mile of the lake, and almost all residents of the area use potable groundwater for domestic use. Risk factors for human exposure to As derived from mine wastes were high enough to merit placement of the mine site and surrounding area on the National Priority List (commonly called ?Superfund?). The Lava Cap Mine Superfund site (LCMS) encompasses approximately 33 acres that include the mine site, the stretch of Little Clipper Creek between the mine and Lost Lake, the lake itself, and the area between the lake and the confluence of Little Clipper Creek with its parent stream, Clipper Creek. The area between the two creeks is named the ?deposition area? due to the estimated 24 m thick layer of tailings that were laid down there during and after active mining. The lobate structure of Lost Lake is also due to deposition in this area. The deposition area and Lost Lake are together estimated to contain 382,277 m3 of tailings. The primary goals of the EPA have been to minimize tailings movement downstream of Lost Lake and to ensure that residents in the area have drinking water that meets national water quality standards. EPA has officially decided to construct a public water supply line to deliver safe water to affected residences, since some residential wells in the area have As concentrations above the curr

  12. Site Area Boundaries

    EPA Pesticide Factsheets

    This dataset consists of site boundaries from multiple Superfund sites in U.S. EPA Region 8. These data were acquired from multiple sources at different times and were combined into one region-wide layer. Thus far the sources include:1. California Gulch (Irrigated Meadows) - ESAT Contractor.2. Manning Canyon - U.S. EPA Region 8; ESAT Contractor.3. Rapid City Small Arms Range - U.S. EPA Region 8; ESAT Contractor.4. Animas River/Cement Creek - U.S. EPA Region 8; ESAT Contractor.5. Monticello Mill Tailings (USDOE) - USDOE; ESAT Contractor.6. Pinon Canyon - USDOD.7. Rock Flats Industrial Park - U.S. EPA Region 8.8. Bountiful/Woods Cross - U.S. EPA Region 8.9. Lincoln Park - U.S. EPA Region 8.10. Marshall Landfill - U.S. EPA Region 8.11. U.S. Magnesium - Pacific Western Technologies Inc.

  13. DOE Office of Scientific and Technical Information (OSTI.GOV)

    Curtis, Michael M.

    As a result of NSG restrictions, India cannot import the natural uranium required to fuel its Pressurized Heavy Water Reactors (PHWRs); consequently, it is forced to rely on the expediency of domestic uranium production. However, domestic production from mines and byproduct sources has not kept pace with demand from commercial reactors. This shortage has been officially confirmed by the Indian Planning Commission’s Mid-Term Appraisal of the country’s current Five Year Plan. The report stresses that as a result of the uranium shortage, Indian PHWR load factors have been continually decreasing. The Uranium Corporation of India Ltd (UCIL) operates a numbermore » of underground mines in the Singhbhum Shear Zone of Jharkhand, and it is all processed at a single mill in Jaduguda. UCIL is attempting to aggrandize operations by establishing new mines and mills in other states, but the requisite permit-gathering and development time will defer production until at least 2009. A significant portion of India’s uranium comes from byproduct sources, but a number of these are derived from accumulated stores that are nearing exhaustion. A current maximum estimate of indigenous uranium production is 430t/yr (230t from mines and 200t from byproduct sources); whereas, the current uranium requirement for Indian PHWRs is 455t/yr (depending on plant capacity factor). This deficit is exacerbated by the additional requirements of the Indian weapons program. Present power generation capacity of Indian nuclear plants is 4350 MWe. The power generation target set by the Indian Department of Atomic Energy (DAE) is 20,000 MWe by the year 2020. It is expected that around half of this total will be provided by PHWRs using indigenously supplied uranium with the bulk of the remainder provided by breeder reactors or pressurized water reactors using imported low-enriched uranium.« less

  14. DISPOSAL OF LIQUID WASTE IN THE DURANGO-TYPE URANIUM MILLING FLOWSHEET

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Tame, K.E.; Valdez, E.G.; Rosenbaum, J.B.

    1961-01-01

    Possible modifications were studied in conventional uraniuum ore- processing steps to confine and permit controlled disposal of radioactive wastes. Surveys of Ra/sup 226/ contamination of liquid wastes from uranium mills indicated that the Vanadium Corporation of America plant at Durango, Colo., had one of the more urgent problems. A possible procedure for minimizing the waste disposal problem was to reuse the waste solution in the mill-in effect, erasing the need for disposal of liquid waste. In examining this possibility, interlocked bench-scale leaching and solvent extraction tests simulating the Durango fiowsheet were made. The simulated reuse of barren raffinate for leachingmore » and washing was carried through three separate campaigns of 9, 12, and 35 cycles each. An attempt to expedite the test work by using agitation leaching during the first campaign resulted in pregnant solutions of varying turbidity, giving a discordant pattern of radioactivity analyses. Percolation leaching and washing patterned more nearly after the Durango flowsheet was used in the second and third campaigns and consistently gave solutions of satisfactory clarity. The radioactivity was somewhat variable but did not build up with prolonged recycling of the raffinate. The buildup of other impurities in the pregnant solution had little noticeabIe effect on the operation of the percolation leach column. Operational difficulties from slow phase disengagement and entrainment in the solvent extraction stripping and scrubbing units occurred during the first two campaigns. In the third campaign slow phase disengagement and aqueous entrainment in the strippers were practically eliminated by heating the last stage to about 40 deg C and operating with the aqueous phase continuous. Increased mixing time in the scrubbing section was successful in reducing entrainment of aqueous in the organic from the settlers. Also, the concentrations of active reagents in the solvent extraction system were increased during the third campaign to correspond to an increase made at the Durango plant. The recovery of uranium and vanadium from the acid leach solution was excellent, averaging 99.7 and 95.6%, respectively. During the test work the Durango plant made several changes in tailing disposal procedures to minimize the waste problem. The most important comprised impounding all barren raffinate in two large lagoons. This was a successful temporary solution to the problem. However, as evaporation is relied upon to eliminate the water, it is estimated that 40 acres of area will be needed. The use of barren raffinate for washing in the Durango process would greatly diminish the quantity of solution to be disposed of by solar evaporation and the conjunctive need for a large disposal area. (auth)« less

  15. Assessing Natural Radionuclide Migration in the Legacy Tailings of Uranium Production

    NASA Astrophysics Data System (ADS)

    Bondarenko, G.; Koliabina, I.; Marinich, O.

    2011-12-01

    The former Prydniprovsky Chemical Plant in Dniprodzerzhynsk, Ukraine, processed uranium ore from 1949 until 1991. Multiple tailing ponds containing solid residual waste products from the uranium leaching and processing of uranium were accumulated along the Dnieper River, including the largest, adjacent to the Dnieper Reservoir, containing over 12 million tons of tailings. Samples for this study were selected from a core recovered from the Dnieper tailing pit in 2009, and used to assess radionuclide migration from tailing ponds. Samples were selected from different depths of the tailing pit core, analyzed for total radionuclide concentrations [Marinich et al., 2009], and successively leached using distilled water, followed by 1N ammonium acetate solution, and finally by 1N HCl solution. Leaching times were ~24 h at 15.17 °C. 238U, 230Th and 226Ra leachate activities were measured by γ-spectrometry with a Ge(Li) detector. 210Pb activity was measured using a SEB-01 scintillation β-spectrometer. Errors depended on measuring method, radionuclide, activity and exposure time: 238U, 11.9%; 230Th, 10.9%; 226Ra, 9.3%; 210Pb ~30%. The average total 238U activity in the tailing profile was 4 Bq/g. The concentration of 238U in the water leachates increased with depth from 14.5% (7-7.5 m), to 43% (11-11.5 m). The concentration of 238U in the acid leachates behaved similarly, increasing from 5.5 % to 15.5% with depth. While the total 230Th activity in increased from 30 Bq/g (7-7.5 m) to 540 Bq/g (11-11.5 m), the 230Th concentration in ammonium acetate leachates decreased from ˜15% to ˜1%. The concentration of 226Ra in all leachates was <1%, indicating that, under conditions of the Dnieper tailing pit, 226Ra is essentially immobile. The concentration of 210Pb in the leachates was as high as 10%. In general, the magnitude of mobile activity from the Dnieper tailing pit core samples decreases in the order 238U>230Th≥210Pb> 226Ra. Secular radioactive equilibrium in the 238U - 230Th - 226Ra - 210Pb decay chain, typical for closed systems, has been disturbed during selective chemical uranium extraction from the parent ore. We calculated the migration of 210Pb, assuming constant 226Ra activity. The results of these calculations show that over 50 years, ~18% of the initial (unknown) 210Pb(0) activity was removed. If we assume removal of 226Ra decay products will continue at the current level, we expect the future annual activity loss of 210Pb to be about 0.36% per year, or 0.072 Bq/g. Assuming the examined core sample is representative of all 12 million tons of tails, the total annual activity loss is estimated to be ~1012 Bq/year. These results allow us to conclude that the loss of activity from the tailing pit by water migration is mainly associated with the 226Ra decay products: 222Rn, 210Pb, 210Po.
    Activity ratios, Dnieper tailings

  16. Removal of heavy metals from Missouri lead mill tailings by froth flotation

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Benn, F.W.; Cornell, W.L.

    Froth flotation techniques to remove heavy metals (Pb, Cu, and Zn) from southeast Missouri lead mill tailings were investigated. It has been estimated that southeast Missouri contains between 200 and 300 million st of Pb tailings stored above ground. The tailings were classified as two distinct types: (1) pre-1968 tailings from the Old Lead Belt (some more than 100 years old) and (2) post-1968 tailings from the New Lead Belt. The objectives of the investigation were to reduce the Pb remaining in the tailings to < 500 ppm (< 0.05 pct Pb) and to attempt to recover a marketable concentratemore » to offset a portion of the remediation costs. The remaining dolomite-limestone would then be used as mining backfill or agricultural limestone. Bench-scale froth flotation removed, in percent, 95 Pb, 84 Cu, and 54 Zn, leaving 94 pct of the original weight containing, in parts per million, 400 Pb, 40 Cu, and 300 Zn from the Old Lead Belt tailings. Separate flotation tests also removed, in percent, 85 Pb, 84 Cu, and 80 Zn, leaving 75 pct of the original weight containing, in parts per million, 400 Pb, 200 Cu, and 500 Zn from the New Lead Belt tailings. Concentrates recovered from the Old Lead Belt were retreated to produce a final Pb concentrate containing 72 pct Pb with a cleaner flotation recovery of 79 pct. Froth flotation proved to be a viable method to remove the heavy metals.« less

  17. White sand potentially suppresses radon emission from uranium tailings

    NASA Astrophysics Data System (ADS)

    Abdel Ghany, H. A.; El Aassy, Ibrahim E.; Ibrahim, Eman M.; Gamil, S. H.

    2018-03-01

    Uranium tailings represent a huge radioactive waste contaminant, where radon emanation is considered a major health hazard. Many trials have been conducted to minimize radon exhalation rate by using different covering materials. In the present work, three covering materials, commonly available in the local environment, (kaolin, white sand and bentonite) have been used with different thickness 10, 15, and 20 mm). 238U, 232Th, 40K and the radon exhalation rate were measured by using gamma spectrometry with a Hyper Pure Germanium (HPGe) detector and solid state nuclear track detectors (CR-39). Radon exhalation rate, calculated before and after covering, ranged from 2.80 ± 0.14 to 4.20 ± 0.21 Bq m-2 h-1, and from 0.30 ± 0.01 to 4.00 ± 0.20 Bq m-2 h-1, respectively. Also, the attenuation coefficients of different covering materials and radon emanation were calculated. The obtained results demonstrate that covering of uranium tailings by kaolin, white sand and bentonite has potentially minimized both the radon exhalation rate and the corresponding internal doses.

  18. Rolling Process Modeling Report. Finite-Element Model Validation and Parametric Study on various Rolling Process parameters

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Soulami, Ayoub; Lavender, Curt A.; Paxton, Dean M.

    2015-06-15

    Pacific Northwest National Laboratory (PNNL) has been investigating manufacturing processes for the uranium-10% molybdenum alloy plate-type fuel for high-performance research reactors in the United States. This work supports the U.S. Department of Energy National Nuclear Security Administration’s Office of Material Management and Minimization Reactor Conversion Program. This report documents modeling results of PNNL’s efforts to perform finite-element simulations to predict roll-separating forces for various rolling mill geometries for PNNL, Babcock & Wilcox Co., Y-12 National Security Complex, Los Alamos National Laboratory, and Idaho National Laboratory. The model developed and presented in a previous report has been subjected to further validationmore » study using new sets of experimental data generated from a rolling mill at PNNL. Simulation results of both hot rolling and cold rolling of uranium-10% molybdenum coupons have been compared with experimental results. The model was used to predict roll-separating forces at different temperatures and reductions for five rolling mills within the National Nuclear Security Administration Fuel Fabrication Capability project. This report also presents initial results of a finite-element model microstructure-based approach to study the surface roughness at the interface between zirconium and uranium-10% molybdenum.« less

  19. Metal loading in Soda Butte Creek upstream of Yellowstone National Park, Montana and Wyoming; a retrospective analysis of previous research; and quantification of metal loading, August 1999

    USGS Publications Warehouse

    Boughton, G.K.

    2001-01-01

    Acid drainage from historic mining activities has affected the water quality and aquatic biota of Soda Butte Creek upstream of Yellowstone National Park. Numerous investigations focusing on metals contamination have been conducted in the Soda Butte Creek basin, but interpretations of how metals contamination is currently impacting Soda Butte Creek differ greatly. A retrospective analysis of previous research on metal loading in Soda Butte Creek was completed to provide summaries of studies pertinent to metal loading in Soda Butte Creek and to identify data gaps warranting further investigation. Identification and quantification of the sources of metal loading to Soda Butte Creek was recognized as a significant data gap. The McLaren Mine tailings impoundment and mill site has long been identified as a source of metals but its contribution relative to the total metal load entering Yellowstone National Park was unknown. A tracer-injection and synoptic-sampling study was designed to determine metal loads upstream of Yellowstone National Park.A tracer-injection and synoptic-sampling study was conducted on an 8,511-meter reach of Soda Butte Creek from upstream of the McLaren Mine tailings impoundment and mill site downstream to the Yellowstone National Park boundary in August 1999. Synoptic-sampling sites were selected to divide the creek into discrete segments. A lithium bromide tracer was injected continuously into Soda Butte Creek for 24.5 hours. Downstream dilution of the tracer and current-meter measurements were used to calculate the stream discharge. Stream discharge values, combined with constituent concentrations obtained by synoptic sampling, were used to quantify constituent loading in each segment of Soda Butte Creek.Loads were calculated for dissolved calcium, silica, and sulfate, as well as for dissolved and total-recoverable iron, aluminum, and manganese. Loads were not calculated for cadmium, copper, lead, and zinc because these elements were infrequently detected in mainstem synoptic samples. All of these elements were detected at high concentrations in the seeps draining the McLaren Mine tailings impoundment. The lack of detection of these elements in the downstream mainstem synoptic samples is probably because of sorption (coprecipitation and adsorption) to metal colloids in the stream.Most of the metal load that entered Soda Butte Creek was contributed by the inflows draining the McLaren Mine tailings impoundment (between 505 meters and 760 meters downstream from the tracer-injection site), Republic Creek (1,859 meters), and Unnamed Tributary (8,267 meters). Results indicate that treatment or removal of the McLaren Mine tailings impoundment would greatly reduce metal loading in Soda Butte Creek upstream of Yellowstone National Park. However, removing only that single source may not reduce metal loads to acceptable levels. The sources of metal loading in Republic Creek and Unnamed Tributary merit further investigation.

  20. Beneficiation of Stillwater Complex Rock for the Production of Lunar Simulants

    NASA Technical Reports Server (NTRS)

    Rickman, D. L.; Young, C.; Stoeser, D.; Edmunson, J.

    2014-01-01

    The availability of pure, high calcium plagioclase would be a significant asset in any attempt to manufacture high-quality lunar simulants. A suitable plagioclase product can be obtained from materials obtained from the Stillwater Complex of Montana. The access, geology, petrology, and mineralogy of the relevant rocks and the mill tailings are described here. This study demonstrates successful plagioclase recovery from mill tailings produced by the Stillwater Mine Company. Hydrogen peroxide was used to remove carboxymethyl cellulose from the tailing. The characteristics of the plagioclase products are shown and locked grains are identified as a limit to achievable purity. Based on the experimental results, flowsheets were developed showing how these resources could be processed and made into 'separates' of (1) high calcium plagioclase and (2) orthopyroxene/clinopyroxene with the thought that they would be combined later to make simulant.

  1. Annotated bibliography of environmentally relevant investigations of uranium mining and milling in the Grants Mineral Belt, northwestern New Mexico

    USGS Publications Warehouse

    Otton, James K.

    2011-01-01

    Studies of the natural environment in the Grants Mineral Belt in northwestern New Mexico have been conducted since the 1930s; however, few such investigations predate uranium mining and milling operations, which began in the early 1950s. This report provides an annotated bibliography of reports that describe the hydrology and geochemistry of groundwaters and surface waters and the geochemistry of soils and sediments in the Grants Mineral Belt and contiguous areas. The reports referenced and discussed provide a large volume of information about the environmental conditions in the area after mining started. Data presented in many of these studies, if evaluated carefully, may provide much basic information about the baseline conditions that existed over large parts of the Grants Mineral Belt prior to mining. Other data may provide information that can direct new work in efforts to discriminate between baseline conditions and the effects of the mining and milling on the natural environment.

  2. Hydrogeochemical investigations of some historic mining areas in the western Humboldt River basin, Nevada

    USGS Publications Warehouse

    Nash, J.T.

    2001-01-01

    Productive historic mines in 13 mining districts, of many geochemical types, were investigated in May of 1998. Reconnaissance field observations were made and samples of mine dumps, mine drainage waters, and mill tailings have been collected to characterize the geochemical signature of these materials and to determine their actual or potential contamination of surface or ground waters. Field observations suggest that visible indicators of acidic mine drainage are rare, and field measurements of pH and chemical analyses of several kinds of materials indicate that only a few sites release acid or significant concentrations of metals.

  3. 76 FR 60935 - Notice of Application from ExxonMobil Corporation, Highland Uranium Mine and Millsite, To Amend...

    Federal Register 2010, 2011, 2012, 2013, 2014

    2011-09-30

    ... and Extend the NRC Long-Term Surveillance Boundary With Respect to Materials License SUA-1139 AGENCY... concentration limits and to extend the NRC Long-Term Surveillance Boundary at its Highland Uranium Mine and Mill... wells and at the proposed POC well. The amendment also proposes to expand the Long-Term Surveillance...

  4. 75 FR 3261 - Powertech (USA) Inc.; Dewey-Burdock Project; New Source Material License Application; Notice of...

    Federal Register 2010, 2011, 2012, 2013, 2014

    2010-01-20

    ... in-situ uranium recovery (ISR, also known as in-situ leach) facilities, and would require restoration... Environmental Impact Statement for In-Situ Leach Uranium Milling Facilities (ISR GEIS) that was published in... published in the Federal Register on January 05, 2010 (75 FR 467-471). The purpose of this notice of intent...

  5. Uranium interaction with soil minerals in the presence of co-contaminants: Case Study- subsurface sediments at or below the water table

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Gartman, Brandy N.; Qafoku, Nikolla

    2016-03-09

    Uranium (U) contaminated subsurface systems are common on a global scale mainly because of its essential role in the production of plutonium for nuclear weapons and other nuclear energy and research activities. Studying the behavior and fate of U in these systems is challenging because of heterogeneities of different types (i.e., physical, chemical and mineralogical) and a complex network of often time-dependent hydrological, biological and chemical reactions and processes that occur sequentially or simultaneously, affecting and/or controlling U mobility. A U contaminated site, i.e., the Integrated Field Research Challenge site in Rifle, CO, USA (a former U mill site) ismore » the focus of this discussion. The overall objectives of this chapter are to 1) provide an overview of the contamination levels (U and other co-contaminants) at this field site; 2) review and discuss different aspects of mineral-U contaminant interactions in reduced and oxidized environments, and in the presence of co-contaminants; 3) present results from a systematic macroscopic, microscopic, and spectroscopic study as an example of the current research efforts and the state-of-knowledge in this important research area; and 4) offer insightful conclusive remarks and future research needs about reactions and processes that control U and other contaminants’ fate and behavior under hydraulically saturated conditions. The implications and applications presented in this chapter are valid for U contaminated sites across the world.« less

  6. Monitoring of uranium concentrations in water samples collected near potentially hazardous objects in North-West Tajikistan.

    PubMed

    Zoriy, P; Schläger, M; Murtazaev, K; Pillath, J; Zoriy, M; Heuel-Fabianek, B

    2018-01-01

    The water contamination near ecologically problematic objects was investigated between 2009 and 2014 in North-West Tajikistan as a part of a joint project between Forschungszentrum Jülich and Khujand State University. The main part of this work was the determination of uranium in water samples collected near the Degmay tailings dump, the Taboshar pit lake and the Syr Darya river. More than 130 water samples were collected and analyzed to monitor the uranium concentration near the investigated areas. Two different mass spectrometers and an ion chromatograph were used for element concentration measurements. Based on the results obtained, the uranium influence of the Degmay tailings on the rivers Khoja-Bakyrgan-Say and Syr Darya and surrounding water was not found. The uranium concentration in water samples was monitored for a lengthy period at seven locations Great differences in the uranium concentration in waters collected in 2010, 2011, 2012, 2013 for each location were not observed. Drinking water samples from the region of North-West Tajikistan were analyzed and compared with the World Health Organization's guidelines. Seven out of nine drinking water samples near Taboshar exceeded the WHO guideline value for uranium concentrations (30 μg/L). The average uranium concentration of water samples from Syr Darya for the period from 2009 to 2014 was determined to be 20.1 (±5.2) μg/L. The uranium contamination of the Syr Darya was determined from the western border to the eastern border and the results are shown in this paper. Copyright © 2017 Elsevier Ltd. All rights reserved.

  7. 76 FR 59173 - Standard Format and Content of License Applications for Conventional Uranium Mills

    Federal Register 2010, 2011, 2012, 2013, 2014

    2011-09-23

    ...On May 30, 2008 (73 FR 31152), the U.S. Nuclear Regulatory Commission (NRC) published for public comment a notice of issuance and availability of Draft Regulatory Guide (DG)-3024, ``Standard Format and Content of License Applications for Conventional Uranium Mills.'' DG- 3024 was a proposed Revision 2 of Regulatory Guide (RG) 3.5. However, upon further consideration the NRC has decided not to revise RG 3.5 at this time. For this reason, DG-3024 will be withdrawn. The comment period closed on August 4, 2008, and 6 comments were received. The comments received will be considered and incorporated as appropriate if the NRC decides to revise RG 3.5 in the future.

  8. The History of Uranium Mining and the Navajo People

    PubMed Central

    Brugge, Doug; Goble, Rob

    2002-01-01

    From World War II until 1971, the government was the sole purchaser of uranium ore in the United States. Uranium mining occurred mostly in the southwestern United States and drew many Native Americans and others into work in the mines and mills. Despite a long and well-developed understanding, based on the European experience earlier in the century, that uranium mining led to high rates of lung cancer, few protections were provided for US miners before 1962 and their adoption after that time was slow and incomplete. The resulting high rates of illness among miners led in 1990 to passage of the Radiation Exposure Compensation Act. PMID:12197966

  9. Uranium bioreduction rates across scales: biogeochemical hot moments and hot spots during a biostimulation experiment at Rifle, Colorado.

    PubMed

    Bao, Chen; Wu, Hongfei; Li, Li; Newcomer, Darrell; Long, Philip E; Williams, Kenneth H

    2014-09-02

    We aim to understand the scale-dependent evolution of uranium bioreduction during a field experiment at a former uranium mill site near Rifle, Colorado. Acetate was injected to stimulate Fe-reducing bacteria (FeRB) and to immobilize aqueous U(VI) to insoluble U(IV). Bicarbonate was coinjected in half of the domain to mobilize sorbed U(VI). We used reactive transport modeling to integrate hydraulic and geochemical data and to quantify rates at the grid block (0.25 m) and experimental field scale (tens of meters). Although local rates varied by orders of magnitude in conjunction with biostimulation fronts propagating downstream, field-scale rates were dominated by those orders of magnitude higher rates at a few selected hot spots where Fe(III), U(VI), and FeRB were at their maxima in the vicinity of the injection wells. At particular locations, the hot moments with maximum rates negatively corresponded to their distance from the injection wells. Although bicarbonate injection enhanced local rates near the injection wells by a maximum of 39.4%, its effect at the field scale was limited to a maximum of 10.0%. We propose a rate-versus-measurement-length relationship (log R' = -0.63 log L - 2.20, with R' in μmol/mg cell protein/day and L in meters) for orders-of-magnitude estimation of uranium bioreduction rates across scales.

  10. Simplified behaviors from increased heterogeneity: II. 3-D uranium transport at the decimeter scale and intertank comparisons.

    PubMed

    Miller, Andrew W; Rodriguez, Derrick R; Honeyman, Bruce D

    2013-05-01

    Upscaling from bench scale systems to field scale systems incorporates physical and chemical heterogeneities from atomistic up to field scales. Heterogeneities of intermediate scale (~10(-1) m) are impossible to incorporate in a bench scale experiment. To transcend these scale discrepancies, this second in a pair of papers presents results from an intermediate scale, 3-D tank experiment completed using five different particle sizes of uranium contaminated sediment from a former uranium mill field site. The external dimensions of the tank were 2.44 m×0.61 m×0.61 m (L×H×W). The five particle sizes were packed in a heterogeneous manner using roughly 11 cm cubes. Small groundwater wells were installed for spatial characterization of chemical gradients and flow parameters. An approximately six month long bromide tracer test was used for flow field characterization. Within the flow domain, local uranium breakthrough curves exhibited a wide range of behaviors. However, the global effluent breakthrough curve was smooth, and not unlike breakthrough curves observed in column scale experiments. This paper concludes with an inter-tank comparison of all three experimental systems presented in this pair of papers. Although there is a wide range of chemical and physical variability between the three tanks, major chemical constituent behaviors are often quite similar or even identical. Copyright © 2013 Elsevier B.V. All rights reserved.

  11. Radionuclides from past uranium mining in rivers of Portugal.

    PubMed

    Carvalho, Fernando P; Oliveira, João M; Lopes, Irene; Batista, Aleluia

    2007-01-01

    During several decades and until a few years ago, uranium mines were exploited in the Centre of Portugal and wastewaters from uranium ore milling facilities were discharged into river basins. To investigate enhancement of radioactivity in freshwater ecosystems, radionuclides of uranium and thorium series were measured in water, sediments, suspended matter, and fish samples from the rivers Vouga, Dão, Távora and Mondego. The results show that these rivers carry sediments with relatively high naturally occurring radioactivity, and display relatively high concentrations of radon dissolved in water, which is typical of a uranium rich region. Riverbed sediments show enhanced concentrations of radionuclides in the mid-section of the Mondego River, a sign of past wastewater discharges from mining and milling works at Urgeiriça confirmed by the enhanced values of (238)U/(232)Th radionuclide ratios in sediments. Radionuclide concentrations in water, suspended matter and freshwater fish from that section of Mondego are also enhanced in comparison with concentrations measured in other rivers. Based on current radionuclide concentrations in fish, regular consumption of freshwater species by local populations would add 0.032 mSv a(-1) of dose equivalent (1%) to the average background radiation dose. Therefore, it is concluded that current levels of enhanced radioactivity do not pose a significant radiological risk either to aquatic fauna or to freshwater fish consumers.

  12. Elemental mobility in sulfidic mine tailings reclaimed with paper mill by-products as sealing materials.

    PubMed

    Jia, Yu; Stahre, Nanna; Mäkitalo, Maria; Maurice, Christian; Öhlander, Björn

    2017-09-01

    Sealing layers made of two alkaline paper mill by-products, fly ash and green liquor dregs, were placed on top of 50-year-old sulfide-containing tailings as a full-scale remediation approach. The performance and effectiveness of the sealing layers with high water content for an oxygen barrier and low hydraulic conductivity for a sealing layer in preventing the formation of acid rock drainage were evaluated 5 years after the remediation. The leaching behavior of the covered tailings was studied using batch leaching tests (L/S ratio 10 L/kg). The leaching results revealed that, in general, the dregs- and ash-covered tailings released relatively lower concentrations of many elements contained in acid rock drainage compared to those from the uncovered tailings. A change in the chemical composition and mineralogical state of the tailings was observed for the tailings beneath the covers. The increase in pH caused by the alkaline materials promoted metal precipitation. Geochemical modeling using PHREEQC confirmed most of the geochemical changes of the covered tailings. Both the ash and dregs showed potential to function as sealing materials in terms of their geochemical properties. However, mobilization of Zn and Ni from the lower part of the dregs-covered tailings was observed. The same phenomenon was observed for the lower part of the ash-covered tailings. Ash showed advantages over dregs as a cover material; based on geochemical studies, the ash immobilized more elements than the dregs did. Lysimeters were installed below the sealing layers, and infiltrating water chemistry and hydrology were studied to monitor the amount and quality of the leachate percolating through.

  13. Initial-phase investigation of multi-dimensional streamflow simulations in the Colorado River, Moab Valley, Grand County, Utah, 2004

    USGS Publications Warehouse

    Kenney, Terry A.

    2005-01-01

    A multi-dimensional hydrodynamic model was applied to aid in the assessment of the potential hazard posed to the uranium mill tailings near Moab, Utah, by flooding in the Colorado River as it flows through Moab Valley. Discharge estimates for the 100- and 500-year recurrence interval and for the Probable Maximum Flood (PMF) were evaluated with the model for the existing channel geometry. These discharges also were modeled for three other channel-deepening configurations representing hypothetical scour of the channel at the downstream portal of Moab Valley. Water-surface elevation, velocity distribution, and shear-stress distribution were predicted for each simulation.The hydrodynamic model was developed from measured channel topography and over-bank topographic data acquired from several sources. A limited calibration of the hydrodynamic model was conducted. The extensive presence of tamarisk or salt cedar in the over-bank regions of the study reach presented challenges for determining roughness coefficients.Predicted water-surface elevations for the current channel geometry indicated that the toe of the tailings pile would be inundated by about 4 feet by the 100-year discharge and 25 feet by the PMF discharge. A small area at the toe of the tailings pile was characterized by velocities of about 1 to 2 feet per second for the 100-year discharge. Predicted velocities near the toe for the PMF discharge increased to between 2 and 4 feet per second over a somewhat larger area. The manner to which velocities progress from the 100-year discharge to the PMF discharge in the area of the tailings pile indicates that the tailings pile obstructs the over-bank flow of flood discharges. The predicted path of flow for all simulations along the existing Colorado River channel indicates that the current distribution of tamarisk in the over-bank region affects how flood-flow velocities are spatially distributed. Shear-stress distributions were predicted throughout the study reach for each discharge and channel geometry examined. Material transport was evaluated by applying these shear-stress values to empirically determined critical shear-stress values for grain sizes ranging from very fine sands to very coarse gravels.

  14. 10. VIEW OF THE ADDITION TO BUILDING 883, REFERRED TO ...

    Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

    10. VIEW OF THE ADDITION TO BUILDING 883, REFERRED TO AS SIDE C. ARMOR PLATE MADE WITH DEPLETED URANIUM WAS HEATED IN A MOLTEN SALT BATH, THEN PROCESSED THROUGH THE ROLLING MILL TO FORM LARGE SHEETS. (9/16/85) - Rocky Flats Plant, Uranium Rolling & Forming Operations, Southeast section of plant, southeast quadrant of intersection of Central Avenue & Eighth Street, Golden, Jefferson County, CO

  15. Calculations of the Electron Energy Distribution Function in a Uranium Plasma by Analytic and Monte Carlo Techniques. Ph.D. Thesis

    NASA Technical Reports Server (NTRS)

    Bathke, C. G.

    1976-01-01

    Electron energy distribution functions were calculated in a U235 plasma at 1 atmosphere for various plasma temperatures and neutron fluxes. The distributions are assumed to be a summation of a high energy tail and a Maxwellian distribution. The sources of energetic electrons considered are the fission-fragment induced ionization of uranium and the electron induced ionization of uranium. The calculation of the high energy tail is reduced to an electron slowing down calculation, from the most energetic source to the energy where the electron is assumed to be incorporated into the Maxwellian distribution. The pertinent collisional processes are electron-electron scattering and electron induced ionization and excitation of uranium. Two distinct methods were employed in the calculation of the distributions. One method is based upon the assumption of continuous slowing and yields a distribution inversely proportional to the stopping power. An iteration scheme is utilized to include the secondary electron avalanche. In the other method, a governing equation is derived without assuming continuous electron slowing. This equation is solved by a Monte Carlo technique.

  16. Uranium mining wastes: The use of the Fish Embryo Acute Toxicity Test (FET) test to evaluate toxicity and risk of environmental discharge.

    PubMed

    Lourenço, J; Marques, S; Carvalho, F P; Oliveira, J; Malta, M; Santos, M; Gonçalves, F; Pereira, R; Mendo, S

    2017-12-15

    Active and abandoned uranium mining sites often create environmentally problematic situations, since they cause the contamination of all environmental matrices (air, soil and water) with stable metals and radionuclides. Due to their cytotoxic, genotoxic and teratogenic properties, the exposure to these contaminants may cause several harmful effects in living organisms. The Fish Embryo Acute Toxicity Test (FET) test was employed to evaluate the genotoxic and teratogenic potential of mine liquid effluents and sludge elutriates from a deactivated uranium mine. The aims were: a) to determine the risk of discharge of such wastes in the environment; b) the effectiveness of the chemical treatment applied to the uranium mine water, which is a standard procedure generally applied to liquid effluents from uranium mines and mills, to reduce its toxicological potential; c) the suitability of the FET test for the evaluation the toxicity of such wastes and the added value of including the evaluation of genotoxicity. Results showed that through the FET test it was possible to determine that both elutriates and effluents are genotoxic and also that the mine effluent is teratogenic at low concentrations. Additionally, liquid effluents and sludge elutriates affect other parameters namely, growth and hatching and that water pH alone played an important role in the hatching process. The inclusion of genotoxicity evaluation in the FET test was crucial to prevent the underestimation of the risks posed by some of the tested effluents/elutriates. Finally, it was possible to conclude that care should be taken when using benchmark values calculated for specific stressors to evaluate the risk posed by uranium mining wastes to freshwater ecosystems, due to their chemical complexity. Copyright © 2017 Elsevier B.V. All rights reserved.

  17. Health assessment for Cimarron Mining Corporation, Carrizozo, Lincoln County, New Mexico, Region 6. CERCLIS No. NMD980749378. Preliminary report

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1990-05-09

    The Cimarron Mining Corporation, an Update 7 National Priorities List site, is located in the southeastern section of Carrizozo, Lincoln County, New Mexico. From 1979 to 1982 the site was operated as a milling operation where precious metals were extracted from crushed iron ore by using either sodium cyanide or potassium cyanide mixed with a metal stripper in a leaching process. Currently the site is inactive; however, drums of sodium/potassium cyanide and solid metal stripping and recovery compounds remain on-site. Preliminary environmental monitoring data indicate chromium, cyanide, lead, and nitrate contamination of on-site groundwater, and cyanide contamination of on-site soil,more » tailings, and wastes. The most likely pathways for contaminant transport to off-site areas appear to be those associated with groundwater and soil. Pathways for human exposure to site-associated contaminants include ingestion of contaminated groundwater and soil and inhalation of contaminated dusts. The site is of potential public health concern because of possible human exposure to site contaminants.« less

  18. Bioaccumulation and Toxicity of Uranium, Arsenic and Nickel to Juveniles and Adults Hyalella azteca in Spiked Sediment Bioassays.

    PubMed

    Goulet, Richard R; Thompson, Patsy-A

    2018-05-26

    Uranium mining and milling release arsenic (As), nickel (Ni) and uranium (U) to receiving waters, which accumulate in sediments. The objective of this study was to investigate if As, Ni and U concentrations in tissue residue of Hyalella azteca, overlying water, sediment pore water and solids could predict juvenile and adult survival and growth in similar conditions to lake sediments downstream of Uranium mines and mills. We conducted 14 day, static sediment toxicity tests spiked with uranium, arsenic and nickel salts. For uranium, we spiked uranyl nitrate with sodium bicarbonate to limit U precipitation once in contact with circumneutral sediment. LC 50 for As, Ni and U of juveniles and adults based on measured concentrations in sediments were 1.8 and 2.2 µmol As/g dw, 6.3 and 13.4 µmol Ni/g dw and 0.2 and 0.9 µmol U/g dw, respectively. Adult survival and growth linearly decreased with increasing bioaccumulation. For juveniles, metal accumulation linearly predicted survival. We calculated lethal body concentrations (LBC 50 ) for juveniles and adults of 70 and 485 nmol As/g dw, 246 and 832 nmol Ni/g dw and 1.7 and 4.4 nmol U/g dw, respectively. The concentrations of As, Ni and U in tissue residue leading to a 20% decrease in growth were 427 nmol As/g, 755 nmol Ni/g and 5 nmol U/g. Overall, this study showed that Uranium was the most toxic element followed by As and Ni, that juveniles were more sensitive to the three metals tested than adults and that threshold body concentrations can support assessment of benthic invertebrate community impairment. This article is protected by copyright. All rights reserved. This article is protected by copyright. All rights reserved.

  19. Micro-PIXE mapping of elemental distribution in arbuscular mycorrhizal roots of the grass, Cynodon dactylon, from gold and uranium mine tailings

    NASA Astrophysics Data System (ADS)

    Weiersbye, I. M.; Straker, C. J.; Przybylowicz, W. J.

    1999-10-01

    A combination of PIXE, proton back-scattering (BS) spectrometry and confocal laser scanning microscopy (CLSM) was used to determine in situ elemental concentrations in arbuscular mycorrhizal (AM) grass roots and AM fungal spores from gold and uranium mine tailings in South Africa. AM regions of roots were characterised by locally elevated P and vesicles were defined by distinctive transition metal and radionuclide distributions. Vesicles (AM structures responsible for nutrient storage), accumulated Mn, Cu, Ni and U, whereas Fe and Zn were present at lower levels than in host tissue. AM spores from mine tailings accumulated Ca, Cr, Fe, Ni, Cu, Br, Y, Th and U, but were deficient in P and K. The sequestration of excess metals and radionuclides in vesicles may limit metal availability, and thus toxicity, to the host.

  20. Remote Sensing and GIS Methods to Detect Uranium Contamination in Watersheds on the Navajo Nation: A NASA/AIHEC Summer Research Experience

    NASA Astrophysics Data System (ADS)

    Chaco, E.; Robinson, D. K.; Carlson, M.; Rock, B. N.

    2010-12-01

    Using ground-based mapping of private drinking water wells contaminated with uranium, we developed Landsat Thematic Mapper (TM) band combinations which indicate possible contamination of extensive areas along the Polacca Wash, the Cottonwood Wash and the Balakai Wash below Black Mesa on the Navajo Nation. The project built on water quality samples taken on unregulated wells by a Field Research Water Quality Team from Dine’ College. The Nevada State Health Laboratory analyzed twenty-six samples, and of those, 12 wells showed uranium in exceedance of 13 μR/hr, the equivalent of 114 mrem per year, greater than the Nuclear Regulatory Commission’s exposure limit of 100 mrem per year. This project hypothesized that point locations of contaminated wells could be compared with US Geologic Survey National Uranium Resource Evaluation (NURE) measures of high uranium levels in soil to identify other possible areas of contamination. We used Cluster Analysis remote sensing methods from MultiSpec© with data acquired by Landsat 5-TM satellite to produce a false color composite band combination, (7 4 2/R G B). Overlaid with a geological map, the Landsat classification correlated sections of sediment with pixilated colored minerals in the NURE data. This map shows possible high levels of uranium in the soil in the watersheds below mine and mill locations. Ground truth studies are needed to confirm the presence of uranium at these suspected sites. The larger goal of this study is to help solve the uranium contamination problem for the Navajo Nation. Chaco was one of 21 TCU (Tribal Colleges and Universities) students who participated in the 2010 NASA/AIHEC (National Aeronautics and Space Administration/American Indian Higher Education Council) Summer Research Experience program. Robinson was his TCU faculty mentor, and Carlson and Rock were Summer Research Experience instructors.

  1. Simultaneous estimation of local-scale and flow path-scale dual-domain mass transfer parameters using geoelectrical monitoring

    USGS Publications Warehouse

    Briggs, Martin A.; Day-Lewis, Frederick D.; Ong, John B.; Curtis, Gary P.; Lane, John W.

    2013-01-01

    Anomalous solute transport, modeled as rate-limited mass transfer, has an observable geoelectrical signature that can be exploited to infer the controlling parameters. Previous experiments indicate the combination of time-lapse geoelectrical and fluid conductivity measurements collected during ionic tracer experiments provides valuable insight into the exchange of solute between mobile and immobile porosity. Here, we use geoelectrical measurements to monitor tracer experiments at a former uranium mill tailings site in Naturita, Colorado. We use nonlinear regression to calibrate dual-domain mass transfer solute-transport models to field data. This method differs from previous approaches by calibrating the model simultaneously to observed fluid conductivity and geoelectrical tracer signals using two parameter scales: effective parameters for the flow path upgradient of the monitoring point and the parameters local to the monitoring point. We use regression statistics to rigorously evaluate the information content and sensitivity of fluid conductivity and geophysical data, demonstrating multiple scales of mass transfer parameters can simultaneously be estimated. Our results show, for the first time, field-scale spatial variability of mass transfer parameters (i.e., exchange-rate coefficient, porosity) between local and upgradient effective parameters; hence our approach provides insight into spatial variability and scaling behavior. Additional synthetic modeling is used to evaluate the scope of applicability of our approach, indicating greater range than earlier work using temporal moments and a Lagrangian-based Damköhler number. The introduced Eulerian-based Damköhler is useful for estimating tracer injection duration needed to evaluate mass transfer exchange rates that range over several orders of magnitude.

  2. Methods for Estimating Adsorbed Uranium(VI) and Distribution Coefficients of Contaminated Sediments

    USGS Publications Warehouse

    Kohler, M.; Curtis, G.P.; Meece, D.E.; Davis, J.A.

    2004-01-01

    Assessing the quantity of U(VI) that participates in sorption/desorption processes in a contaminated aquifer is an important task when investigating U migration behavior. U-contaminated aquifer sediments were obtained from 16 different locations at a former U mill tailings site at Naturita, CO (U.S.A.) and were extracted with an artificial groundwater, a high pH sodium bicarbonate solution, hydroxylamine hydrochloride solution, and concentrated nitric acid. With an isotopic exchange method, both a KD value for the specific experimental conditions as well as the total exchangeable mass of U(VI) was determined. Except for one sample, KD values determined by isotopic exchange with U-contaminated sediments that were in equilibrium with atmospheric CO2 agreed within a factor of 2 with KD values predicted from a nonelectrostatic surface complexation model (NEM) developed from U(VI) adsorption experiments with uncontaminated sediments. The labile fraction of U(VI) and U extracted by the bicarbonate solution were highly correlated (r2 = 0.997), with a slope of 0.96 ?? 0.01. The proximity of the slope to one suggests that both methods likely access the same reservoir of U(VI) associated with the sediments. The results indicate that the bicarbonate extraction method is useful for estimating the mass of labile U(VI) in sediments that do not contain U(IV). In-situ KD values calculated from the measured labile U(VI) and the dissolved U(VI) in the Naturita alluvial aquifer agreed within a factor of 3 with in-situ K D values predicted with the NEM and groundwater chemistry at each well.

  3. A statistical approach for generating synthetic tip stress data from limited CPT soundings

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Basalams, M.K.

    CPT tip stress data obtained from a Uranium mill tailings impoundment are treated as time series. A statistical class of models that was developed to model time series is explored to investigate its applicability in modeling the tip stress series. These models were developed by Box and Jenkins (1970) and are known as Autoregressive Moving Average (ARMA) models. This research demonstrates how to apply the ARMA models to tip stress series. Generation of synthetic tip stress series that preserve the main statistical characteristics of the measured series is also investigated. Multiple regression analysis is used to model the regional variationmore » of the ARMA model parameters as well as the regional variation of the mean and the standard deviation of the measured tip stress series. The reliability of the generated series is investigated from a geotechnical point of view as well as from a statistical point of view. Estimation of the total settlement using the measured and the generated series subjected to the same loading condition are performed. The variation of friction angle with depth of the impoundment materials is also investigated. This research shows that these series can be modeled by the Box and Jenkins ARMA models. A third degree Autoregressive model AR(3) is selected to represent these series. A theoretical double exponential density function is fitted to the AR(3) model residuals. Synthetic tip stress series are generated at nearby locations. The generated series are shown to be reliable in estimating the total settlement and the friction angle variation with depth for this particular site.« less

  4. Improved detector for the measurement of gamma radiation

    NASA Astrophysics Data System (ADS)

    Zelt, F. B.

    1985-07-01

    The present invention lies in the field of gamma ray spectrometry of geologic deposits and other materials, such as building materials (cement, asphalt, etc.) More specifically, the invention is an improved device for the gamma ray spetcrometery of gelogical deposits as a tool for petroleum exploration, geologic research and monitoring of radio-active materials such as in uranium mill tailings and the like. Improvement consists in enlarging the area of the receptor face and without any necessarily substantial increase in the volume of the receptor crystal over the current cylindrical shapes. The invention also provides, as a corollary of the increase in area receptor crystal face, a reduction in the weight of the amount of material necessary to provide effective shielding of the crystal from atmospheric radiation and radiation from deposits not under examination. The area of the receptor crystal face is increased by forming the crystal as a truncated cone with the shielding shaped as a hollow frustrum of a cone. A photomultiplier device is secured to the smaller face of the crystal. The improved detector shape can also be used in scintillometers which measure total gamma radiation.

  5. Health and Safety Research Division: Progress report, October 1, 1985-March 31, 1987

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Walsh, P.J.

    1987-09-01

    This report summarizes the progress in our programs for the period October 1, 1985, through March 31, 1987. The division's presentations and publications represented important contributions on the forefronts of many fields. Eleven invention disclosures were filed, two patent applications submitted, and one patent issued. The company's transfers new technologies to the private sector more efficiently than in the past. The division's responsibilities to DOE under the Uranium Mill Tailings Remedial Action (UMTRA) program includes inclusion recommendations for 3100 properties. The nuclear medicine program developed new radiopharmaceuticals and radionuclide generators through clinical trials with some of our medical cooperatives. Twomore » major collaborative indoor air quality studies and a large epidemiological study of drinking water quality and human health were completed. ORNL's first scanning tunneling microscope (STM) has achieved single atom resolution and has produced some of the world's best images of single atoms on the surface of a silicon crystal. The Biological and Radiation Physics Section, designed and constructed a soft x-ray spectrometer which has exhibited a measuring efficiency that is 10,000 times higher than other equipment. 1164 refs.« less

  6. Technical Report on the Behavior of Trace Elements, Stable Isotopes, and Radiogenic Isotopes During the Processing of Uranium Ore to Uranium Ore Concentrate

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Marks, N. E.; Borg, L. E.; Eppich, G. R.

    2015-07-09

    The goals of this SP-1 effort were to understand how isotopic and elemental signatures behave during mining, milling, and concentration and to identify analytes that might preserve geologic signatures of the protolith ores. The impurities that are preserved through the concentration process could provide useful forensic signatures and perhaps prove diagnostic of sample origin.

  7. Effect of biogas generation on radon emissions from landfills receiving radium-bearing waste from shale gas development.

    PubMed

    Walter, Gary R; Benke, Roland R; Pickett, David A

    2012-09-01

    Dramatic increases in the development of oil and natural gas from shale formations will result in large quantities of drill cuttings, flowback water, and produced water. These organic-rich shale gas formations often contain elevated concentrations of naturally occurring radioactive materials (NORM), such as uranium, thorium, and radium. Production of oil and gas from these formations will also lead to the development of technologically enhanced NORM (TENORM) in production equipment. Disposal of these potentially radium-bearing materials in municipal solid waste (MSW) landfills could release radon to the atmosphere. Risk analyses of disposal of radium-bearing TENORM in MSW landfills sponsored by the Department of Energy did not consider the effect of landfill gas (LFG) generation or LFG control systems on radon emissions. Simulation of radon emissions from landfills with LFG generation indicates that LFG generation can significantly increase radon emissions relative to emissions without LFG generation, where the radon emissions are largely controlled by vapor-phase diffusion. Although the operation of LFG control systems at landfills with radon source materials can result in point-source atmospheric radon plumes, the LFG control systems tend to reduce overall radon emissions by reducing advective gas flow through the landfill surface, and increasing the radon residence time in the subsurface, thus allowing more time for radon to decay. In some of the disposal scenarios considered, the radon flux from the landfill and off-site atmospheric activities exceed levels that would be allowed for radon emissions from uranium mill tailings. Increased development of hydrocarbons from organic-rich shale formations has raised public concern that wastes from these activities containing naturally occurring radioactive materials, particularly radium, may be disposed in municipal solid waste landfills and endanger public health by releasing radon to the atmosphere. This paper analyses the processes by which radon may be emitted from a landfill to the atmosphere. The analyses indicate that landfill gas generation can significantly increase radon emissions, but that the actual level of radon emissions depend on the place of the waste, construction of the landfill cover, and nature of the landfill gas control system.

  8. Psychological effects of technological/human-caused environmental disasters: examination of the Navajo and uranium.

    PubMed

    Markstrom, Carol A; Charley, Perry H

    2003-01-01

    Disasters can be defined as catastrophic events that challenge the normal range of human coping ability. The technological/human-caused disaster, a classification of interest in this article, is attributable to human error or misjudgment. Lower socioeconomic status and race intersect in the heightened risk for technological/human-caused disasters among people of color. The experience of the Navajo with the uranium industry is argued to specifically be this type of a disaster with associated long-standing psychological impacts. The history of the Navajo with uranium mining and milling is reviewed with a discussion of the arduous efforts for compensation. The psychological impacts of this long-standing disaster among the Navajo are organized around major themes of: (a) human losses and bereavement, (b) environmental losses and contamination, (c) feelings of betrayal by government and mining and milling companies, (d) fears about current and future effects, (e) prolonged duration of psychological effects, (f) anxiety and depression, and (g) complicating factors of poverty and racism. The paper concludes with suggestions for culturally-appropriate education and intervention.

  9. Changes in the substrate of rivers in historic mining districts

    USGS Publications Warehouse

    Milhous, R.T.

    2004-01-01

    The restoration of rivers in watersheds with historic mining districts has become a topic of interest during the last decade. Rivers restoration in these areas is difficult because the mines and mills can be scattered over a wide area and often small. Many have also been abandoned. This paper presents two substrate related factors that are important in the evaluation of river restoration alternatives in watersheds with significance impacts from mines and mills most of which are old and abandoned. The two factors are 1) changes in the size distribution and specific weights of the substrate, and 2) the changes in quality of the interstecial waters caused by metals associated with the tailings in the substrate. The most important impacts of tailings from mills may be on the physical characteristics of the substrate (porosity) and on the quality of the pore waters. The measurements presented in this paper do show significant variation in the porosity in gravel bed rivers and in the quality of the pore waters. Copyright ASCE 2004.

  10. Uranium Bioreduction Rates across Scales: Biogeochemical Hot Moments and Hot Spots during a Biostimulation Experiment at Rifle, Colorado

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Bao, Chen; Wu, Hongfei; Li, Li

    2014-09-02

    We aim to understand the scale-dependent evolution of uranium bioreduction during a field experiment at a former uranium mill site near Rifle, Colorado. Acetate was injected to stimulate Fe-reducing bacteria (FeRB) and to immobilize aqueous U(VI) to insoluble U(IV). Bicarbonate was coinjected in half of the domain to mobilize sorbed U(VI). We used reactive transport modeling to integrate hydraulic and geochemical data and to quantify rates at the grid block (0.25 m) and experimental field scale (tens of meters). Although local rates varied by orders of magnitude in conjunction with biostimulation fronts propagating downstream, field-scale rates were dominated by thosemore » orders of magnitude higher rates at a few selected hot spots where Fe(III), U(VI), and FeRB were at their maxima in the vicinity of the injection wells. At particular locations, the hot moments with maximum rates negatively corresponded to their distance from the injection wells. Although bicarbonate injection enhanced local rates near the injection wells by a maximum of 39.4%, its effect at the field scale was limited to a maximum of 10.0%. We propose a rate-versus-measurement-length relationship (log R' = -0.63« less

  11. 7. THE BEGINNING OF A PANORAMIC SERIES VIEW LOOKING WEST ...

    Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

    7. THE BEGINNING OF A PANORAMIC SERIES VIEW LOOKING WEST NORTHWEST FROM THE UPHILL SIDE OF THE MILL. THE ORE RECEIVING HOUSE IS IN THE IMAGE CENTER, THE ORE DELIVERY TRESTLE EXTENDS FROM THE RECEIVING HOUSE TO THE MILL BUILDING IN THE BACKGROUND LEFT. IN THE MID-GROUND LEFT IS A CYLINDRICAL STRUCTURE BELIEVE TO BE A SETTLING TANK FROM A LATER CHEMICAL RETREATMENT OF THE TAILINGS IN THE FOREGROUND RIGHT IS AN EXTANT ORE BUCKET. - Standard Gold Mill, East of Bodie Creek, Northeast of Bodie, Bodie, Mono County, CA

  12. Cancer deaths and occupational exposure in a group of plutonium workers.

    PubMed

    Fallahian, Naz Afarin; Brey, Richard R; Tivis, Rick D; Piland, Neill F; Simpson, David R

    2012-04-01

    An exploratory epidemiological study was conducted for 319 deceased nuclear workers who had intakes of transuranic radionuclides and histories of employment during the time period from 1943 to 1995. The workers were employed at various facilities throughout the United States, including the Department of Energy defense facilities and uranium mining and milling sites. The majority of individuals were involved in documented radiological incidents during their careers. All had voluntarily agreed to donate their organs or whole body to the United States Transuranium and Uranium Registries. External and internal dose assessments were performed using occupational exposure histories and postmortem concentrations of transuranic radionuclides in critical organs. Statistical data analyses were performed to investigate the potential relationship between radiation exposure and causes of death within this population due to cancers of the lungs, liver, and all sites combined while controlling for the effects of other confounders. No association was found between radiation exposure and death due to cancer (α = 0.05). However, statistically significant associations were found between death due to any type of cancer and smoking (yes or no) (odds ratio = 5.41; 95% CI: 1.42 to 20.67) and rate of cigarette smoking (packs per day) (odds ratio = 2.70; 95% CI: 1.37 to 5.30).

  13. Mortality among a cohort of uranium mill workers: an update

    PubMed Central

    Pinkerton, L; Bloom, T; Hein, M; Ward, E

    2004-01-01

    Aims: To evaluate the mortality experience of 1484 men employed in seven uranium mills in the Colorado Plateau for at least one year on or after 1 January 1940. Methods: Vital status was updated through 1998, and life table analyses were conducted. Results: Mortality from all causes and all cancers was less than expected based on US mortality rates. A statistically significant increase in non-malignant respiratory disease mortality and non-significant increases in mortality from lymphatic and haematopoietic malignancies other than leukaemia, lung cancer, and chronic renal disease were observed. The excess in lymphatic and haematopoietic cancer mortality was due to an increase in mortality from lymphosarcoma and reticulosarcoma and Hodgkin's disease. Within the category of non-malignant respiratory disease, mortality from emphysema and pneumoconioses and other respiratory disease was increased. Mortality from lung cancer and emphysema was higher among workers hired prior to 1955 when exposures to uranium, silica, and vanadium were presumably higher. Mortality from these causes of death did not increase with employment duration. Conclusions: Although the observed excesses were consistent with our a priori hypotheses, positive trends with employment duration were not observed. Limitations included the small cohort size and limited power to detect a moderately increased risk for some outcomes of interest, the inability to estimate individual exposures, and the lack of smoking data. Because of these limitations, firm conclusions about the relation of the observed excesses in mortality and mill exposures are not possible. PMID:14691274

  14. 2. VIEW OF INTERIOR, EAST SIDE (SIDE A) OF BUILDING ...

    Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

    2. VIEW OF INTERIOR, EAST SIDE (SIDE A) OF BUILDING 883. INSTALLATION OF ROLLING MILLS AND MOLTEN SALT BATH EQUIPMENT FOR DEPLETED URANIUM FABRICATION. THE CRANE NEAR THE CEILING WAS USED TO INSTALL THE EQUIPMENT. BOXES ON THE FLOOR CONTAINED EQUIPMENT TO BE INSTALLED. (1/23/57) - Rocky Flats Plant, Uranium Rolling & Forming Operations, Southeast section of plant, southeast quadrant of intersection of Central Avenue & Eighth Street, Golden, Jefferson County, CO

  15. DOE Office of Scientific and Technical Information (OSTI.GOV)

    Chambers, Doug; Wiatzka, Gerd; Brown, Steve

    This paper provides the life story of Canada's original radium/uranium mine. In addition to the history of operations, it discusses the unique and successful approach used to identify the key issues and concerns associated with the former radium, uranium and silver mining property and the activities undertaken to define the remedial actions and subsequent remedial plan. The Port Radium Mine site, situated approximately 275 km north of Yellowknife on the east shore of Great Bear Lake, Northwest Territories, was discovered in 1930 and underground mining began in 1932. The mine operated almost continuously from 1932 to 1982, initially for recoverymore » of radium, then uranium and finally, for recovery of silver. Tailings production totaled an estimated 900,000 tons and 800,000 tons from uranium and silver processing operations respectively. In the early days of mining, Port Radium miners were exposed to radon and associated decay product levels (in Working Level Months of exposure - WLM) hundreds of times greater than modern standards. The experience of the Port Radium miners provides important contribution to understanding the risks from radon. While the uranium mine was originally decommissioned in the early 1960's, to the standards of the day, the community of Deline (formerly Fort Franklin) had concerns about residual contamination at the mine site and the potential effects arising from use of traditional lands. The Deline people were also concerned about the possible risks to Deline Dene arising from their work as ore carriers. In the late 1990's, the community of Deline brought these concerns to national attention and consequently, the Government of Canada and the community of Deline agreed to move forward in a collaborative manner to address these concerns. The approach agreed to was to establish the Canada-Deline Uranium Table (CDUT) to provide a joint process by which the people of Deline could have their concerns expressed and addressed. A great deal of work was done through the CDUT, including efforts to assess site environment and safety issues in the context of modern reclamation standards. In addition to the environmental and remediation studies, an assessment of historic exposures of Deline ore carriers to radiation and a follow-up epidemiological feasibility study were performed. SENES Consultants Limited (SENES) carried out the dose reconstruction for the Port Radium miners in the 1990's, was the environmental consultant to the CDUT from 2000 to 2005, developed the Remedial Action Plan (RAP), engineering plans and specifications for decommissioning the Port Radium mine and vicinity sites in 2005/6, supervised the remedial works in 2007 and carried out the long term post closure monitoring from 2008 to 2012. Our firsthand experience from working cooperatively with the CDUT provides insights into effective decommissioning of historic contaminated sites. (authors)« less

  16. Occupational safety data and casualty rates for the uranium fuel cycle. [Glossaries

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    O'Donnell, F.R.; Hoy, H.C.

    1981-10-01

    Occupational casualty (injuries, illnesses, fatalities, and lost workdays) and production data are presented and used to calculate occupational casualty incidence rates for technologies that make up the uranium fuel cycle, including: mining, milling, conversion, and enrichment of uranium; fabrication of reactor fuel; transportation of uranium and fuel elements; generation of electric power; and transmission of electric power. Each technology is treated in a separate chapter. All data sources are referenced. All steps used to calculate normalized occupational casualty incidence rates from the data are presented. Rates given include fatalities, serious cases, and lost workdays per 100 man-years worked, per 10/supmore » 12/ Btu of energy output, and per other appropriate units of output.« less

  17. Cryo-FIB-SEM serial milling and block face imaging: Large volume structural analysis of biological tissues preserved close to their native state.

    PubMed

    Vidavsky, Netta; Akiva, Anat; Kaplan-Ashiri, Ifat; Rechav, Katya; Addadi, Lia; Weiner, Steve; Schertel, Andreas

    2016-12-01

    Many important biological questions can be addressed by studying in 3D large volumes of intact, cryo fixed hydrated tissues (⩾10,000μm 3 ) at high resolution (5-20nm). This can be achieved using serial FIB milling and block face surface imaging under cryo conditions. Here we demonstrate the unique potential of the cryo-FIB-SEM approach using two extensively studied model systems; sea urchin embryos and the tail fin of zebrafish larvae. We focus in particular on the environment of mineral deposition sites. The cellular organelles, including mitochondria, Golgi, ER, nuclei and nuclear pores are made visible by the image contrast created by differences in surface potential of different biochemical components. Auto segmentation and/or volume rendering of the image stacks and 3D reconstruction of the skeleton and the cellular environment, provides a detailed view of the relative distribution in space of the tissue/cellular components, and thus of their interactions. Simultaneous acquisition of secondary and back-scattered electron images adds additional information. For example, a serial view of the zebrafish tail reveals the presence of electron dense mineral particles inside mitochondrial networks extending more than 20μm in depth in the block. Large volume imaging using cryo FIB SEM, as demonstrated here, can contribute significantly to the understanding of the structures and functions of diverse biological tissues. Copyright © 2016 Elsevier Inc. All rights reserved.

  18. Cyanide and migratory birds at gold mines in Nevada, USA

    USGS Publications Warehouse

    Henny, C.J.; Hallock, R.J.; Hill, E.F.

    1994-01-01

    Since the mid-1980s, cyanide in heap leach solutions and mill tailings ponds at gold mines in Nevada has killed a large but incompletely documented number of wildlife ( gt 9,500 individuals, primarily migratory birds). This field investigation documents the availability of cyanide at a variety of 'typical' Nevada gold mines during 1990 and 1991, describes wildlife reactions to cyanide solutions, and discusses procedures for eliminating wildlife loss from cyanide poisoning. Substantial progress has been made to reduce wildlife loss. About half of the mill tailings ponds (some up to 150 ha) in Nevada have been chemically treated to reduce cyanide concentrations (the number needing treatment is uncertain) and many of the smaller heap leach solution ponds and channels are now covered with netting to exclude birds and most mammals. The discovery of a cyanide gradient in mill tailings ponds (concentration usually 2-3 times higher at the inflow point than at reclaim point) provides new insight into wildlife responses (mortality) observed in different portions of the ponds. Finding dead birds on the tops of ore heaps and associated with solution puddling is a new problem, but management procedures for eliminating this source of mortality are available. A safe threshold concentration of cyanide to eliminate wildlife loss could not be determined from the field data and initial laboratory studies. New analytical methods may be required to assess further the wildlife hazard of cyanide in mining solutions.

  19. Health implications of radionuclide levels in cattle raised near U mining and milling facilities in Ambrosia Lake, New Mexico

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Lapham, S.C.; Millard, J.B.; Samet, J.M.

    1989-03-01

    This study was conducted to determine radionuclide tissue levels in cattle raised near U mining and milling facilities. Ambrosia Lake, New Mexico, has been the site of extensive U mining for 30 y and contains several underground U mines, a processing mill, and two large U tailings piles. Ten cows were purchased from two grazing areas in Ambrosia Lake and ten control animals were purchased from Crownpoint, New Mexico. Muscle, liver, kidney, and bone tissue taken from these animals, and environmental samples, including water, grasses and soil collected from the animals' grazing areas, were analyzed for /sup 238/U, /sup 234/U,more » /sup 230/Th, /sup 226/Ra, /sup 210/Pb, and /sup 210/Po. Mean radionuclide levels in cattle tissue and environmental samples from Ambrosia Lake were higher in almost every comparison than those found in respective controls. Liver and kidney tissues were particularly elevated in /sup 226/Ra and /sup 210/Po. Radiation dose commitments from eating cattle tissue with these radionuclide concentrations were calculated. We concluded that the health risk to the public from eating exposed cattle is minimal, unless large amounts of this tissue, especially liver and kidney, are ingested.« less

  20. 75 FR 8346 - Proposed CERCLA Administrative Settlement; Anderson-Calhoun Mine and Mill Site, Leadpoint, WA

    Federal Register 2010, 2011, 2012, 2013, 2014

    2010-02-24

    ...-Calhoun Mine and Mill Site, Leadpoint, WA AGENCY: Environmental Protection Agency (EPA). ACTION: Notice...-Calhoun Mine and Mill Site in Leadpoint, Washington, with settling party Blue Tee Corporation. The... Anderson-Calhoun Mine and Mill Site in Leadpoint, Washington, EPA Docket No. CERCLA-10-2010-0105 and should...

  1. IN-SITU DUOX™ CHEMICAL OXIDATION TECHNOLOGY TO TREAT CHLORINATED ORGANICS AT THE ROOSEVELT MILLS SITE, VERNON, CT: SITE CHARACTERIZATION AND TREATABILITY STUDY

    EPA Science Inventory

    A study was performed investigating the feasibility of applying the DUOX™ chemical oxidation technology to chlorinated solvent contaminated media at the Roosevelt Mills site in Vernon, Connecticut. The Roosevelt Mills site is a former woolen mill that included dry cleaning operat...

  2. Monitoring Physical and Biogeochemical Dynamics of Uranium Bioremediation at the Intermediate Scale

    NASA Astrophysics Data System (ADS)

    Tarrell, A. N.; Figueroa, L. A.; Rodriguez, D.; Haas, A.; Revil, A.

    2011-12-01

    Subsurface uranium above desired levels for aquifer use categories exists naturally and from historic mining and milling practices. In situ bioimmobilization offers a cost effective alternative to conventional pump and treat methods by stimulating growth of microorganisms that lead to the reduction and precipitation of uranium. Vital to the long-term success of in situ bioimmobilization is the ability to successfully predict and demonstrate treatment effectiveness to assure that regulatory goals are met. However, successfully monitoring the progress over time is difficult and requires long-term stewardship to ensure effective treatment due to complex physical and biogeochemical heterogeneity. In order to better understand these complexities and the resultant effect on uranium immobilization, innovative systematic monitoring approaches with multiple performance indicators must be investigated. A key issue for uranium bioremediation is the long term stability of solid-phase reduction products. It has been shown that a combination of data from electrode-based monitoring, self-potential monitoring, oxidation reduction potential (ORP), and water level sensors provides insight for identifying and localizing bioremediation activity and can provide better predictions of deleterious biogeochemical change such as pore clogging. In order to test the proof-of-concept of these sensing techniques and to deconvolve redox activity from other electric potential changing events, an intermediate scale 3D tank experiment has been developed. Well-characterized materials will be packed into the tank and an artificial groundwater will flow across the tank through a constant-head boundary. The experiment will utilize these sensing methods to image the electrical current produced by bacteria as well as indications of when and where electrical activity is occurring, such as with the reduction of radionuclides. This work will expand upon current knowledge by exploring the behavior of uranium bioremediation at an intermediate scale, as well as examining the effects from introducing a flow field in a laboratory setting. Data collected from this experiment will help further characterize which factors are contributing to current increases. Additional information concerning the effect of geochemical changes in porosity may also be observed. The results of this work will allow the creation of a new data set collected from a more comprehensive laboratory monitoring network and will allow stakeholders to develop effective decision-making tools on the long-term remediation management at uranium contaminated sites. The data will also aid in the long-term prediction abilities of a reactive transport models. As in situ bioremediation offers a low cost alternative to ex situ treatment methods, the results of this work will help to both reduce cost at existing sites and enable treatment of sites that otherwise have no clear solution.

  3. The Sequoyah Corporation Fuels Release and the Church Rock Spill: Unpublicized Nuclear Releases in American Indian Communities

    PubMed Central

    Brugge, Doug; deLemos, Jamie L.; Bui, Cat

    2007-01-01

    The Three Mile Island nuclear release exemplifies why there is public and policy interest in the high-technology, highly visible end of the nuclear cycle. The environmental and health consequences of the early steps in the cycle—mining, milling, and processing of uranium ore—may be less appreciated. We examined 2 large unintended acute releases of uranium—at Kerr McGee’s Sequoyah Fuels Corporation in Oklahoma and United Nuclear Corporation’s Church Rock uranium mill in New Mexico, which were incidents with comparable magnitude to the Three Mile Island release. We urge exploration of whether there is limited national interest and concern for the primarily rural, low-income, and American Indian communities affected by these releases. More attention should be given to the early stages of the nuclear cycle and their impacts on health and the environment. PMID:17666688

  4. 77 FR 4559 - Ecusta Mill Site, Pisgah Forest, Transylvania County, NC; Notice of Amended Settlement

    Federal Register 2010, 2011, 2012, 2013, 2014

    2012-01-30

    ... ENVIRONMENTAL PROTECTION AGENCY [EPA-R4-SFUND 2012-; FRL-9624-1] Ecusta Mill Site, Pisgah Forest... settlement for resolution of past response and future costs concerning the Ecusta Mill Superfund Site located... settlement are available from Ms. Paula V. Painter. Submit your comments by Site name Ecusta Mill Superfund...

  5. Chemical composition of samples collected from waste rock dumps and other mining-related features at selected phosphate mines in southeastern Idaho, western Wyoming, and northern Utah

    USGS Publications Warehouse

    Moyle, Phillip R.; Causey, J. Douglas

    2001-01-01

    This report provides chemical analyses for 31 samples collected from various phosphate mine sites in southeastern Idaho (25), northern Utah (2), and western Wyoming (4). The sampling effort was undertaken as a reconnaissance and does not constitute a characterization of mine wastes. Twenty-five samples were collected from waste rock dumps, 2 from stockpiles, and 1 each from slag, tailings, mill shale, and an outcrop. All samples were analyzed for a suite of major, minor, and trace elements. Although the analytical data set for the 31 samples is too small for detailed statistical analysis, a summary of general observations is made.

  6. The use of field-based mesocosm systems to assess the effects of uranium milling effluent on fathead minnow (Pimephales promelas) reproduction.

    PubMed

    Driessnack, Melissa K; Dubé, Monique G; Rozon-Ramilo, Lisa D; Jones, Paul D; Wiramanaden, Cheryl I E; Pickering, Ingrid J

    2011-08-01

    Northern Saskatchewan, Canada is home to a uranium milling operation that discharges a complex milling effluent containing nutrients, cations and anions, and many metals including selenium (Se). Se has the potential to accumulate in a system even when water concentrations are low. This study evaluated the effects of treated uranium milling effluent and contaminated sediment in combination and in isolation to determine the contribution and importance of each source to fathead minnow (Pimephales promelas) reproduction and survival. Trios of fathead minnows were allocated to one of four treatments for 21-days where the following were evaluated; survival (adult and 5 day larval), larval deformities, reproductive effects (egg production, spawning events) and metal tissue burdens (muscle, gonad, eggs and larvae). In addition Se speciation analysis was conducted on fish tissues. Effects were solely effluent-mediated with little contribution observed due to the presence of contaminated sediments. The contaminated sediments tested were taken from the actual receiving environment and represented the sediment composition found in greatest abundance. Results showed egg production significantly increased in the effluent treatments compared to the reference water treatments. Although egg production increased following effluent exposure, there was reduced hatching and larval survival and a significant increase in skeletal deformities in 5 day old larvae. Despite these effects on the offspring, when examined in an integrated manner relative to increased egg production, the mean number of normal larvae did not differ among treatments. Total selenium significantly increased in the effluent exposed, algae, female muscle, gonad, eggs and larvae in addition to other metals. A shift in the proportion of species of selenium was evident with changing exposure conditions. Biofilm/algae was key in the transfer of available Se into the food chain from the water and a source of direct dietary exposure in fish and possibly invertebrates.

  7. General View of Kinckley Knitting Mill site, east end of ...

    Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

    General View of Kinckley Knitting Mill site, east end of site along Wister Street, looking north, showing ruin of stone mill building and smoke stack of the Germantown Dyeworks in background - Hinckley Knitting Mills, 21-35 East Wister Street, Philadelphia, Philadelphia County, PA

  8. DOE Office of Scientific and Technical Information (OSTI.GOV)

    Linard, Joshua; Hall, Steve

    9.1 Compliance Summary The Lakeview, Oregon, Uranium Mill Tailings Radiation Control Act (UMTRCA) Title I Disposal Site was inspected September 16 and 17, 2015. Other than some ongoing concern with erosion-control rock riprap degradation, the disposal cell was in good condition. Some minor fence repairs and vegetation removal, and minor erosion repair work along the west site fence is planned. Inspectors identified no other maintenance needs or cause for a follow-up or contingency inspection. Disposal cell riprap is evaluated annually to ensure continued long-term protection of the cell from erosion during a severe precipitation event. Degradation of the rock riprapmore » was first observed at the site in the mid-1990s. Rock gradation monitoring of the riprap on the west side slope has been performed as part of the annual inspection since 1997 to determine the mean diameter (D 50) value. As prescribed by the monitoring procedure, the rock monitoring is routinely conducted at random locations. However, at the U.S. Nuclear Regulatory Commission’s (NRC’s) request, the 2015 rock monitoring approach deviated from the normal procedure by using a pre-established monitoring grid in a subset area of the west side slope. This changed the monitoring approach from random sampling to biased sampling. The D 50 value measured during the 2015 gradation monitoring is 2.39 inches, which falls below the original D 50 design size range of 2.7–3.9 inches for the Type B size side slope riprap. At NRC’s request, rock durability monitoring was added to the gradation monitoring in 2009 to monitor durability by rock type. Results of the 2015 durability monitoring showed that74 percent of the total rock sampled is durability class code A rock with an assigned durability class of “highly durable” or durability class code B “durable” rock, and that over 90 percent of the 3-inch or larger rock is durability class code A or B. The rock durability classifications are further explained in Section 9.4.2.2.« less

  9. An Assessment of Radiological Hazards from Gold Mine Tailings in the Province of Gauteng in South Africa

    PubMed Central

    Kamunda, Caspah; Mathuthu, Manny; Madhuku, Morgan

    2016-01-01

    Radiological hazards associated with exposure to Naturally Occurring Radionuclides Materials from gold mine tailings in the province of Gauteng in South Africa were evaluated. A comparison was made with soil samples from a control area. In this study, gamma spectroscopy was used to measure the activity concentrations of these radionuclides in 56 soil samples from the mine tailings and 10 soil samples from the control area. The average activity concentrations in Bq∙kg−1 for Uranium-238, Thorium-232, and Potassium-40 from the mine tailings were found to be 785.3 ± 13.7, 43.9 ± 1.0 and 427.0 ± 13.1, respectively. On the other hand, the average activity concentrations in Bq∙kg−1 for Uranium-238, Thorium-232, and Potassium-40 from the control area were found to be 17.0.1 ± 0.4, 22.2 ± 0.5 and 496.8 ± 15.2, respectively. Radiological hazard parameters calculated from these activity concentrations were higher than recommended safe limits. In particular, calculated average values for the external hazard (Hex) and the internal hazard (Hin) from the mine tailings were found to be 2.4 and 4.5. Both these values were higher than unity, posing a significant health risk to the population in the area. PMID:26797624

  10. 10 CFR 765.3 - Definitions.

    Code of Federal Regulations, 2013 CFR

    2013-01-01

    ... ENERGY REIMBURSEMENT FOR COSTS OF REMEDIAL ACTION AT ACTIVE URANIUM AND THORIUM PROCESSING SITES General... uranium or thorium processing site or active processing site means: (1) Any uranium or thorium processing... an Agreement State, for the production at a site of any uranium or thorium derived from ore— (i) Was...

  11. 10 CFR 765.3 - Definitions.

    Code of Federal Regulations, 2012 CFR

    2012-01-01

    ... ENERGY REIMBURSEMENT FOR COSTS OF REMEDIAL ACTION AT ACTIVE URANIUM AND THORIUM PROCESSING SITES General... uranium or thorium processing site or active processing site means: (1) Any uranium or thorium processing... an Agreement State, for the production at a site of any uranium or thorium derived from ore— (i) Was...

  12. 10 CFR 765.3 - Definitions.

    Code of Federal Regulations, 2014 CFR

    2014-01-01

    ... ENERGY REIMBURSEMENT FOR COSTS OF REMEDIAL ACTION AT ACTIVE URANIUM AND THORIUM PROCESSING SITES General... uranium or thorium processing site or active processing site means: (1) Any uranium or thorium processing... an Agreement State, for the production at a site of any uranium or thorium derived from ore— (i) Was...

  13. DOE Office of Scientific and Technical Information (OSTI.GOV)

    Harmon, K.M.; Lakey, L.T.; Leigh, I.W.

    Worldwide activities related to nuclear fuel cycle and radioactive waste management programs are summarized. Several trends have developed in waste management strategy: All countries having to dispose of reprocessing wastes plan on conversion of the high-level waste (HLW) stream to a borosilicate glass and eventual emplacement of the glass logs, suitably packaged, in a deep geologic repository. Countries that must deal with plutonium-contaminated waste emphasize pluonium recovery, volume reduction and fixation in cement or bitumen in their treatment plans and expect to use deep geologic repositories for final disposal. Commercially available, classical engineering processing are being used worldwide to treatmore » and immobilize low- and intermediate-level wastes (LLW, ILW); disposal to surface structures, shallow-land burial and deep-underground repositories, such as played-out mines, is being done widely with no obvious technical problems. Many countries have established extensive programs to prepare for construction and operation of geologic repositories. Geologic media being studied fall into three main classes: argillites (clay or shale); crystalline rock (granite, basalt, gneiss or gabbro); and evaporates (salt formations). Most nations plan to allow 30 years or longer between discharge of fuel from the reactor and emplacement of HLW or spent fuel is a repository to permit thermal and radioactive decay. Most repository designs are based on the mined-gallery concept, placing waste or spent fuel packages into shallow holes in the floor of the gallery. Many countries have established extensive and costly programs of site evaluation, repository development and safety assessment. Two other waste management problems are the subject of major R and D programs in several countries: stabilization of uranium mill tailing piles; and immobilization or disposal of contaminated nuclear facilities, namely reactors, fuel cycle plants and R and D laboratories.« less

  14. Comparison of in situ uranium KD values with a laboratory determined surface complexation model

    USGS Publications Warehouse

    Curtis, G.P.; Fox, P.; Kohler, M.; Davis, J.A.

    2004-01-01

    Reactive solute transport simulations in groundwater require a large number of parameters to describe hydrologic and chemical reaction processes. Appropriate methods for determining chemical reaction parameters required for reactive solute transport simulations are still under investigation. This work compares U(VI) distribution coefficients (i.e. KD values) measured under field conditions with KD values calculated from a surface complexation model developed in the laboratory. Field studies were conducted in an alluvial aquifer at a former U mill tailings site near the town of Naturita, CO, USA, by suspending approximately 10 g samples of Naturita aquifer background sediments (NABS) in 17-5.1-cm diameter wells for periods of 3 to 15 months. Adsorbed U(VI) on these samples was determined by extraction with a pH 9.45 NaHCO3/Na2CO3 solution. In wells where the chemical conditions in groundwater were nearly constant, adsorbed U concentrations for samples taken after 3 months of exposure to groundwater were indistinguishable from samples taken after 15 months. Measured in situ K D values calculated from the measurements of adsorbed and dissolved U(VI) ranged from 0.50 to 10.6 mL/g and the KD values decreased with increasing groundwater alkalinity, consistent with increased formation of soluble U(VI)-carbonate complexes at higher alkalinities. The in situ K D values were compared with KD values predicted from a surface complexation model (SCM) developed under laboratory conditions in a separate study. A good agreement between the predicted and measured in situ KD values was observed. The demonstration that the laboratory derived SCM can predict U(VI) adsorption in the field provides a critical independent test of a submodel used in a reactive transport model. ?? 2004 Elsevier Ltd. All rights reserved.

  15. Environmental geochemical studies of selected mineral deposits in Wrangell-St. Elias National Park and Preserve, Alaska

    USGS Publications Warehouse

    Eppinger, Robert G.; Briggs, Paul H.; Rosenkrans, Danny; Ballestrazze, Vanessa

    2000-01-01

    Environmental geochemical investigations at Wrangell-St. Elias National Park and Preserve, Alaska, between 1994 and 1997 included studies of the Kennecott stratabound copper mines and mill area; historic mines and mill in the Bremner District, gold placer mines at Gold Hill; the undisturbed porphyry, Cu-Mo deposits at Orange Hill and Bond Creek, and the historic mines and mill at Nabesna, The study was in cooperation with the National Park Service and focused on sample media including surface water, bedload sediment, rock, mine waste, and mill tailings samples. Results demonstrate that bedrock geology and mineral deposit type must be considered when environmental geochemical effects of historic or active mine areas are evaluated.

  16. 76 FR 2145 - International Paper Company, Franklin Pulp & Paper Mill, Including On-Site Leased Workers From...

    Federal Register 2010, 2011, 2012, 2013, 2014

    2011-01-12

    ... Company, Franklin Pulp & Paper Mill, Including On-Site Leased Workers From Railserve, Franklin, VA..., applicable to workers and former workers of International Paper Company, Franklin Pulp & Paper Mill, Franklin... follows: All workers International Paper Company, Franklin Pulp & Paper Mill, including on-site leased...

  17. Hydrogeochemical Investigations of Historic Mining Districts, Central Western Slope of Colorado, Including Influence on Surface-Water Quality

    USGS Publications Warehouse

    Nash, J. Thomas

    2002-01-01

    This report describes reconnaissance hydrogeochemical investigations of 22 mining districts on the Western Slope of Colorado in the Gunnison and Uncompahgre National Forests and adjacent public lands administered by the Bureau of Land Management. Sources and fates of contaminants from historic mines, mine waste, and mill tailings are interpreted from chemical analyses for 190 samples of surface waters; 185 samples of mined rocks, mill tailings, and altered rocks; and passive leach analyses of 116 samples of those mineralized materials. Short reaches of several headwater streams show relatively low level effects of historic mining; the headwaters of the Uncompahgre River are highly contaminated by mines and unmined altered rocks in the Red Mountain district. There is encouraging evidence that natural processes attenuate mine-related contamination in most districts.

  18. 40 CFR 192.21 - Criteria for applying supplemental standards.

    Code of Federal Regulations, 2010 CFR

    2010-07-01

    ... standards. 192.21 Section 192.21 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) RADIATION PROTECTION PROGRAMS HEALTH AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL... a clear and present risk of injury to workers or to members of the public, notwithstanding...

  19. 40 CFR 192.21 - Criteria for applying supplemental standards.

    Code of Federal Regulations, 2011 CFR

    2011-07-01

    ... 40 Protection of Environment 25 2011-07-01 2011-07-01 false Criteria for applying supplemental standards. 192.21 Section 192.21 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) RADIATION PROTECTION PROGRAMS HEALTH AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL...

  20. 40 CFR 192.21 - Criteria for applying supplemental standards.

    Code of Federal Regulations, 2012 CFR

    2012-07-01

    ... 40 Protection of Environment 26 2012-07-01 2011-07-01 true Criteria for applying supplemental standards. 192.21 Section 192.21 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) RADIATION PROTECTION PROGRAMS HEALTH AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL...

  1. 40 CFR 192.21 - Criteria for applying supplemental standards.

    Code of Federal Regulations, 2013 CFR

    2013-07-01

    ... 40 Protection of Environment 26 2013-07-01 2013-07-01 false Criteria for applying supplemental standards. 192.21 Section 192.21 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) RADIATION PROTECTION PROGRAMS HEALTH AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL...

  2. 40 CFR 192.21 - Criteria for applying supplemental standards.

    Code of Federal Regulations, 2014 CFR

    2014-07-01

    ... 40 Protection of Environment 25 2014-07-01 2014-07-01 false Criteria for applying supplemental standards. 192.21 Section 192.21 Protection of Environment ENVIRONMENTAL PROTECTION AGENCY (CONTINUED) RADIATION PROTECTION PROGRAMS HEALTH AND ENVIRONMENTAL PROTECTION STANDARDS FOR URANIUM AND THORIUM MILL...

  3. 75 FR 81675 - Notice of Issuance of Regulatory Guide

    Federal Register 2010, 2011, 2012, 2013, 2014

    2010-12-28

    ... Fuel Cycle Facilities.'' FOR FURTHER INFORMATION CONTACT: Mekonen M. Bayssie, Regulatory Guide... Materials in Liquid and Gaseous Effluents from Nuclear Fuel Cycle Facilities,'' was published as Draft... guidance is applicable to nuclear fuel cycle facilities, with the exception of uranium milling facilities...

  4. Uranium content and leachable fraction of fluorspars

    USGS Publications Warehouse

    Landa, E.R.; Councell, T.B.

    2000-01-01

    Much attention in the radiological health community has recently focused on the management and regulation of naturally occurring radioactive materials. Although uranium-bearing minerals are present in a variety of fluorspar deposits, their potential consideration as naturally occurring radioactive materials has received only limited recognition. The uranium content of 28 samples of acid- and cryolite-grade (>97% CaF2) fluorspar from the National Defense Stockpile was found to range from 120 to 24,200 ??g kg-1, with a mean of 2,145 ??g kg-1. As a point of comparison, the average concentration of uranium in the upper crust of the earth is about 2,500 ??g kg-1. Leachability of this uranium was assessed by means of the Toxicity Characteristic Leaching Procedure (TCLP). The TCLP extractable fraction ranged from 1 to 98%, with a mean of 24% of the total uranium. The typically low concentrations of uranium seen in these materials probably reflects the removal of uranium-bearing mineral phases during the beneficiation of the crude fluorspar ore to achieve industrial specifications. Future NORM studies should examine crude fluorspar ores and flotation tailings.

  5. 78 FR 46948 - Proposed Agreement Regarding Site Costs and Covenants Not To Sue for American Lead and Zinc Mill...

    Federal Register 2010, 2011, 2012, 2013, 2014

    2013-08-02

    ... Not To Sue for American Lead and Zinc Mill Site, Ouray County, Colorado AGENCY: Environmental... provides for Settling Party's payment of certain response costs incurred at the American Lead and Zinc Mill... reference the American Lead and Zinc Mill Site, the EPA Docket No. CERCLA-08-2013- 0004. The Agency's...

  6. Pillsbury Mills LLC Removal Site

    EPA Pesticide Factsheets

    The Pillsbury Mills LLC removal site is located at 1525 E. Phillips St., Springfield, IL. Residential properties are located immediately across the street on the north and east perimeters. The site is a former Pillsbury grain mill on about 18 acres.

  7. Acclimation capacity of the three-spined stickleback (Gasterosteus aculeatus, L.) to a sudden biological stress following a polymetallic exposure.

    PubMed

    Le Guernic, Antoine; Sanchez, Wilfried; Palluel, Olivier; Bado-Nilles, Anne; Floriani, Magali; Turies, Cyril; Chadili, Edith; Vedova, Claire Della; Cavalié, Isabelle; Adam-Guillermin, Christelle; Porcher, Jean-Marc; Geffard, Alain; Betoulle, Stéphane; Gagnaire, Béatrice

    2016-10-01

    To get closer to the environmental reality, ecotoxicological studies should no longer consider the evaluation of a single pollutant, but rather combination of stress and their interaction. The aim of this study was to determine if responses of a fish to a sudden biological stress could be modified by a prior exposure to a chemical stress (a polymetallic contamination). For this purpose, in situ experiment was conducted in three ponds in the Haute-Vienne department (France). One pond was chosen for its high uranium concentration due to uranium mine tailings, and the two other ponds, which were not submitted to these tailings. Three-spined sticklebacks (Gasterosteus aculeatus) were caged in these ponds for 14 days. After this period, fish were submitted to a biological stress, exerted by lipopolysaccharides injection after anesthesia, and were sacrificed 4 days after these injections for multi-biomarkers analyses (leucocyte viability, phagocytic capacity and reactive oxygen species production, antioxidant peptide and enzymes, lipid peroxidation and DNA damage). The pond which received uranium mine tailings had higher metallic concentrations. Without biological stress, sticklebacks caged in this pond presented an oxidative stress, with increasing of reactive oxygen species levels, modification of some parts of the antioxidant system, and lipid peroxidation. Caging in the two most metal-contaminated ponds resulted in an increase of susceptibility of sticklebacks to the biological stress, preventing their phagocytic responses to lipopolysaccharides and modifying their glutathione contents and glutathione-S-transferase activity.

  8. A Non-Proliferating Fuel Cycle: No Enrichment, Reprocessing or Accessible Spent Fuel - 12375

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Parker, Frank L.

    2012-07-01

    Current fuel cycles offer a number of opportunities for access to plutonium, opportunities to create highly enriched uranium and access highly radioactive wastes to create nuclear weapons and 'dirty' bombs. The non-proliferating fuel cycle however eliminates or reduces such opportunities and access by eliminating the mining, milling and enrichment of uranium. The non-proliferating fuel cycle also reduces the production of plutonium per unit of energy created, eliminates reprocessing and the separation of plutonium from the spent fuel and the creation of a stream of high-level waste. It further simplifies the search for land based deep geologic repositories and interim storagemore » sites for spent fuel in the USA by disposing of the spent fuel in deep sub-seabed sediments after storing the spent fuel at U.S. Navy Nuclear Shipyards that have the space and all of the necessary equipment and security already in place. The non-proliferating fuel cycle also reduces transportation risks by utilizing barges for the collection of spent fuel and transport to the Navy shipyards and specially designed ships to take the spent fuel to designated disposal sites at sea and to dispose of them there in deep sub-seabed sediments. Disposal in the sub-seabed sediments practically eliminates human intrusion. Potential disposal sites include Great Meteor East and Southern Nares Abyssal Plain. Such sites then could easily become international disposal sites since they occur in the open ocean. It also reduces the level of human exposure in case of failure because of the large physical and chemical dilution and the elimination of a major pathway to man-seawater is not potable. Of course, the recovery of uranium from sea water and the disposal of spent fuel in sub-seabed sediments must be proven on an industrial scale. All other technologies are already operating on an industrial scale. If externalities, such as reduced terrorist threats, environmental damage (including embedded emissions), long term care, reduced access to 'dirty' bomb materials, the social and political costs of siting new facilities and the psychological impact of no solution to the nuclear waste problem, were taken into account, the costs would be far lower than those of the present fuel cycle. (authors)« less

  9. THE MARY KATHLEEN URANIUM PROJECT

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Nelson, A.

    1960-02-01

    A description is given of uranium mining and milling methods at the Mary Kathleen Mine in the Cloncurry-Mt. Isa district of Queensland, Australia. The discovery of this property and its development are outlined. The deposit cecurs in highly altered meta-sediments in the corella beds of lower proterozoic age. Because of the considerable internal waste in the deposit, it was necessary to devise a selective mining method which would keep dilution to the lowest possible level. The mining, haulage and handling, premilling program, drilling, and blasting are discussed. (M.C.G.)

  10. Process for converting magnesium fluoride to calcium fluoride

    DOEpatents

    Kreuzmann, A.B.; Palmer, D.A.

    1984-12-21

    This invention is a process for the conversion of magnesium fluoride to calcium fluoride whereby magnesium fluoride is decomposed by heating in the presence of calcium carbonate, calcium oxide or calcium hydroxide. Magnesium fluoride is a by-product of the reduction of uranium tetrafluoride to form uranium metal and has no known commercial use, thus its production creates a significant storage problem. The advantage of this invention is that the quality of calcium fluoride produced is sufficient to be used in the industrial manufacture of anhydrous hydrogen fluoride, steel mill flux or ceramic applications.

  11. 76 FR 30696 - Reimbursement for Costs of Remedial Action at Active Uranium and Thorium Processing Sites

    Federal Register 2010, 2011, 2012, 2013, 2014

    2011-05-26

    ... DEPARTMENT OF ENERGY Reimbursement for Costs of Remedial Action at Active Uranium and Thorium...) acceptance of claims in FY 2011 from eligible active uranium and thorium processing site licensees for... incurred by licensees at active uranium and thorium processing sites to remediate byproduct material...

  12. MONTHLY REPORT OF DEVELOPMENT, SEPTEMBER 1963

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    None

    1964-10-31

    Methods for separating germanium from Taiga carbonaceous shale by flotation and salt roasting are described. The recovery of vanadium from Beaverlodge mill tailings by carbonate leaching is briefly discussed. Methods of chemical analysis are also discussed. (N.W.R.)

  13. Thermal Stability of Milled Nanocrystalline Tungsten Powders

    DTIC Science & Technology

    2011-05-01

    v Acknowledgments This research is supported by mission funding from the Depleted Uranium Replacement Program and is the result of collaborative...L.; Reddy, R. G. Synthesis of Titanium Carbide Nano-powders by Thermal Plasma. Scripta Materialia 2005, 52 (12), 1253–1258. 4. Karagedov, G. R

  14. Bioaccessibility of U, Th and Pb in particulate matter from an abandoned uranium mine

    NASA Astrophysics Data System (ADS)

    Millward, Geoffrey; Foulkes, Michael; Henderson, Sam; Blake, William

    2016-04-01

    Currently, there are approximately 150 uranium mines in Europe at various stages of either operation, development, decommissioning, restoration or abandonment (wise-uranium.com). The particulate matter comprising the mounds of waste rock and mill tailings poses a risk to human health through the inadvertent ingestion of particles contaminated with uranium and thorium, and their decay products, which exposes recipients to the dual toxicity of heavy elements and their radioactive emissions. We investigated the bioaccessibility of 238U, 232Th and 206,214,210Pb in particulate samples taken from a contaminated, abandoned uranium mine in South West England. Sampling included a mine shaft, dressing floor and waste heap, as well as soils from a field used for grazing. The contaminants were extracted using the in-vitro Unified Bioaccessibility Research Group of Europe Method (UBM) in order to mimic the digestion processes in the human stomach (STOM) and the combined stomach and gastrointestinal tract (STOM+INT). Analyses of concentrations of U, Th and Pb in the extracts were by ICP-MS and the activity concentrations of radionuclides were determined on the same particles, before and after extraction, using gamma spectroscopy. 'Total' concentrations of U, Th and Pb for all samples were in the range 57 to 16,200, 0.28 to 3.8 and 69 to 4750 mg kg-1, respectively. For U and Pb the concentrations in the STOM fraction were lower than the total and STOM+INT fractions were even lower. However, for Th the STOM+INT fractions were higher than the STOM due to the presence of Th carbonate species within the gastrointestinal fluid. Activity concentrations for 214Pb and 210Pb, including total, STOM and STOM+INT, were in the range 180 to <1 Bq g-1 for the dressing floor and waste heap and 18 to <1 Bq g-1 for the grazing land. Estimates of the bioaccessible fractions (BAFs) of 238U in the most contaminated samples were 39% and 8% in the STOM and STOM+INT, respectively, whereas the respective BAFs for 232Th were 3% and 9%. For stable 206Pb the STOM and STOM+INT BAFs were 16% and 3% for the most contaminated samples, whereas those from the field had 44% in the STOM fraction and 17% in the STOM+INT fraction. The BAFs for 214Pb and 210Pb were the same as 206Pb. Dose estimates were made for the contaminants together with radioactive doses in order to assess potential risk to human health.

  15. 75 FR 69471 - Smurfit-Stone Container Corporation, Containerboard Mill, Including On-Site Leased Workers From...

    Federal Register 2010, 2011, 2012, 2013, 2014

    2010-11-12

    ... Corporation, Containerboard Mill, Including On-Site Leased Workers From KMW Enterprises, Ontonagon, MI... to workers of Smurfit-Stone Container Corporation, Containerboard Mill, Ontonagon, Michigan. The... Ontonagon, Michigan location of Smurfit-Stone Container Corporation, Containerboard Mill. The Department has...

  16. The ultimate disposition of depleted uranium

    DOE Office of Scientific and Technical Information (OSTI.GOV)

    Not Available

    1990-12-01

    Significant amounts of the depleted uranium (DU) created by past uranium enrichment activities have been sold, disposed of commercially, or utilized by defense programs. In recent years, however, the demand for DU has become quite small compared to quantities available, and within the US Department of Energy (DOE) there is concern for any risks and/or cost liabilities that might be associated with the ever-growing inventory of this material. As a result, Martin Marietta Energy Systems, Inc. (Energy Systems), was asked to review options and to develop a comprehensive plan for inventory management and the ultimate disposition of DU accumulated atmore » the gaseous diffusion plants (GDPs). An Energy Systems task team, under the chairmanship of T. R. Lemons, was formed in late 1989 to provide advice and guidance for this task. This report reviews options and recommends actions and objectives in the management of working inventories of partially depleted feed (PDF) materials and for the ultimate disposition of fully depleted uranium (FDU). Actions that should be considered are as follows. (1) Inspect UF{sub 6} cylinders on a semiannual basis. (2) Upgrade cylinder maintenance and storage yards. (3) Convert FDU to U{sub 3}O{sub 8} for long-term storage or disposal. This will include provisions for partial recovery of costs to offset those associated with DU inventory management and the ultimate disposal of FDU. Another recommendation is to drop the term tails'' in favor of depleted uranium'' or DU'' because the tails'' label implies that it is waste.'' 13 refs.« less

  17. OVERVIEW OF REMAINS OF DEWATERING BUILDING, LOOKING SOUTH TOWARD CYANIDE ...

    Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

    OVERVIEW OF REMAINS OF DEWATERING BUILDING, LOOKING SOUTH TOWARD CYANIDE PROCESSING AREA. WATER USED IN PROCESSING AT THE STAMP MILL WAS CIRCULATED HERE FOR RECLAMATION. SANDS WERE SETTLED OUT AND DEPOSITED IN ONE OF TWO TAILINGS HOLDING AREAS. CLEARED WATER WAS PUMPED BACK TO THE MILL FOR REUSE. THIS PROCESS WAS ACCOMPLISHED BY THE USE OF SETTLING CONES, EIGHT FEET IN DIAMETER AND SIX FEET HIGH. THE REMAINS OF FOUR CONES ARE AT CENTER, BEHIND THE TANK IN THE FOREGROUND. TO THE LEFT IS THE MAIN ACCESS ROAD BETWEEN THE MILL AND THE PARKING LOT. - Keane Wonder Mine, Park Route 4 (Daylight Pass Cutoff), Death Valley Junction, Inyo County, CA

  18. 77 FR 40637 - Smurfit-Stone Container Corporation, Containerboard Mill, Including On-Site Leased Workers From...

    Federal Register 2010, 2011, 2012, 2013, 2014

    2012-07-10

    ... Corporation, Containerboard Mill, Including On-Site Leased Workers From KMW Enterprises and General Security... Assistance on May 6, 2010, applicable to workers of Smurfit-Stone Container Corporation, Containerboard Mill... Ontonagon, Michigan location of Smurfit-Stone Container Corporation, Containerboard Mill, Ontonagon...

  19. Nesting habitat relationships of sympatric Crested Caracaras, Red-tailed Hawks, and White-tailed Hawks in South Texas

    USGS Publications Warehouse

    Actkinson, M.A.; Kuvlesky, W.P.; Boal, C.W.; Brennan, L.A.; Hernandez, F.

    2007-01-01

    We quantified nesting-site habitats for sympatric White-tailed Hawks (Buteo albicaudatus) (n = 40), Red-tailed Hawks (B. jamaicensis) (n = 39), and Crested Caracaras (Caracara cheriway) (n = 24) in the Coastal Sand Plain of south Texas. White-tailed Hawks and Crested Caracara nest sites occurred in savannas, whereas Red-tailed Hawk nest sites occurred in woodlands on the edge of savannas. White-tailed Hawk nest sites were in shrubs and trees that were shorter (3.5 ?? 1.0 m) and had smaller canopy diameters (5.5 ?? 2.1 m) than those of Red-tailed Hawks (10.1 ?? 2.0 m, 13.7 ?? 5.8 m) and Crested Caracaras (5.6 ?? 1.7 m, 8.5 ?? 3.5 m). Red-tailed Hawk nest sites had higher woody densities (15.7 ?? 9.6 plants) and more woody cover (84 ?? 19%) than those of White-tailed Hawks (5.6 ?? 5.8 plants, 20 ?? 21%) and Crested Caracaras (9.9 ?? 6.7 plants, 55 ?? 34%). Crested Caracara nest sites were in dense, multi-branched shrubs composed of more living material (97 ?? 3%) than those of White-tailed (88 ?? 18%) and Red-tailed hawks (88 ?? 18%). Nest sites of White-tailed Hawks, Red-tailed Hawks, and Crested Caracaras were similar to random samples from the surrounding habitat indicating that preferred nesting habitat was available for each of these species at least within 60 m of active nest sites. Nest tree height, along with woody plant and native grass cover best discriminated nest sites among the three raptor species. There was no overlap at Red-tailed and White-tailed hawk nest sites in vegetation structure, while Crested Caracara nests were in habitat intermediate between the two other species. Partitioning of nesting habitat may be how these raptor species co-exist at the broader landscape scale of our study area in the Coastal Sand Plain of Texas.

  20. 75 FR 6068 - Extension of Public Comment Period on the Draft Environmental Impact Statement for the Lost Creek...

    Federal Register 2010, 2011, 2012, 2013, 2014

    2010-02-05

    ... Environmental Impact Statement for the Lost Creek In-Situ Recovery Project in Sweetwater County, WY; Supplement to the Generic Environmental Impact Statement for In-Situ Leach Uranium Milling Facilities AGENCY... SEIS) for the Lost Creek [[Page 6069

Top