DOE Office of Scientific and Technical Information (OSTI.GOV)

Konzen, Kevin

Generally, plutonium has been manufactured to support commercial and military applications involving heat sources, weapons and reactor fuel. This work focuses on three typical plutonium mixtures, while observing the potential of 241Am ingrowth and its effect on internal dose. The term “ingrowth” is used to describe 241Am production due solely from the decay of 241Pu as part of a plutonium mixture, where it is initially absent or present in a smaller quantity. Dose calculation models do not account for 241Am ingrowth unless the 241Pu quantity is specified. This work suggested that 241Am ingrowth be considered in bioassay analysis when theremore » is a potential of a 10% increase to the individual’s committed effective dose. It was determined that plutonium fuel mixtures, initially absent of 241Am, would likely exceed 10% for typical reactor grade fuel aged less than 30 years; however, heat source grade and aged weapons grade fuel would normally fall below this threshold. In conclusion, although this work addresses typical plutonium mixtures following separation, it may be extended to irradiated commercial uranium fuel and is expected to be a concern in the recycling of spent fuel.« less

The Complete Burning of Weapons Grade Plutonium and Highly Enriched Uranium with (Laser Inertial Fusion-Fission Energy) LIFE Engine

DOE Office of Scientific and Technical Information (OSTI.GOV)

Farmer, J C; Diaz de la Rubia, T; Moses, E

2008-12-23

The National Ignition Facility (NIF) project, a laser-based Inertial Confinement Fusion (ICF) experiment designed to achieve thermonuclear fusion ignition and burn in the laboratory, is under construction at the Lawrence Livermore National Laboratory (LLNL) and will be completed in April of 2009. Experiments designed to accomplish the NIF's goal will commence in late FY2010 utilizing laser energies of 1 to 1.3 MJ. Fusion yields of the order of 10 to 20 MJ are expected soon thereafter. Laser initiated fusion-fission (LIFE) engines have now been designed to produce nuclear power from natural or depleted uranium without isotopic enrichment, and from spentmore » nuclear fuel from light water reactors without chemical separation into weapons-attractive actinide streams. A point-source of high-energy neutrons produced by laser-generated, thermonuclear fusion within a target is used to achieve ultra-deep burn-up of the fertile or fissile fuel in a sub-critical fission blanket. Fertile fuels including depleted uranium (DU), natural uranium (NatU), spent nuclear fuel (SNF), and thorium (Th) can be used. Fissile fuels such as low-enrichment uranium (LEU), excess weapons plutonium (WG-Pu), and excess highly-enriched uranium (HEU) may be used as well. Based upon preliminary analyses, it is believed that LIFE could help meet worldwide electricity needs in a safe and sustainable manner, while drastically shrinking the nation's and world's stockpile of spent nuclear fuel and excess weapons materials. LIFE takes advantage of the significant advances in laser-based inertial confinement fusion that are taking place at the NIF at LLNL where it is expected that thermonuclear ignition will be achieved in the 2010-2011 timeframe. Starting from as little as 300 to 500 MW of fusion power, a single LIFE engine will be able to generate 2000 to 3000 MWt in steady state for periods of years to decades, depending on the nuclear fuel and engine configuration. Because the fission blanket in a fusion-fission hybrid system is subcritical, a LIFE engine can burn any fertile or fissile nuclear material, including unenriched natural or depleted U and SNF, and can extract a very high percentage of the energy content of its fuel resulting in greatly enhanced energy generation per metric ton of nuclear fuel, as well as nuclear waste forms with vastly reduced concentrations of long-lived actinides. LIFE engines could thus provide the ability to generate vast amounts of electricity while greatly reducing the actinide content of any existing or future nuclear waste and extending the availability of low cost nuclear fuels for several thousand years. LIFE also provides an attractive pathway for burning excess weapons Pu to over 99% FIMA (fission of initial metal atoms) without the need for fabricating or reprocessing mixed oxide fuels (MOX). Because of all of these advantages, LIFE engines offer a pathway toward sustainable and safe nuclear power that significantly mitigates nuclear proliferation concerns and minimizes nuclear waste. An important aspect of a LIFE engine is the fact that there is no need to extract the fission fuel from the fission blanket before it is burned to the desired final level. Except for fuel inspection and maintenance process times, the nuclear fuel is always within the core of the reactor and no weapons-attractive materials are available outside at any point in time. However, an important consideration when discussing proliferation concerns associated with any nuclear fuel cycle is the ease with which reactor fuel can be converted to weapons usable materials, not just when it is extracted as waste, but at any point in the fuel cycle. Although the nuclear fuel remains in the core of the engine until ultra deep actinide burn up is achieved, soon after start up of the engine, once the system breeds up to full power, several tons of fissile material is present in the fission blanket. However, this fissile material is widely dispersed in millions of fuel pebbles, which can be tagged as individual accountable items, and thus made difficult to divert in large quantities. This report discusses the application of the LIFE concept to nonproliferation issues, initially looking at the LIFE (Laser Inertial Fusion-Fission Energy) engine as a means of completely burning WG Pu and HEU. By combining a neutron-rich inertial fusion point source with energy-rich fission, the once-through closed fuel-cycle LIFE concept has the following characteristics: it is capable of efficiently burning excess weapons or separated civilian plutonium and highly enriched uranium; the fission blanket is sub-critical at all times (keff < 0.95); because LIFE can operate well beyond the point at which light water reactors (LWRs) need to be refueled due to burn-up of fissile material and the resulting drop in system reactivity, fuel burn-up of 99% or more appears feasible. The objective of this work is to develop LIFE technology for burning of WG-Pu and HEU.« less

Physicochemical characterization of discrete weapons grade plutonium metal particles originating from the 1960 BOMARC incident

NASA Astrophysics Data System (ADS)

Bowen, James M.

The goal of this research was to investigate the physicochemical properties of weapons grade plutonium particles originating from the 1960 BOMARC incident for the purpose of predicting their fate in the environment and to address radiation protection and nuclear security concerns. Methods were developed to locate and isolate the particles in order to characterize them. Physical, chemical, and radiological characterization was performed using a variety of techniques. And finally, the particles were subjected to a sequential extraction procedure, a series of increasingly aggressive reagents, to simulate an accelerated environmental exposure. A link between the morphology of the particles and their partitioning amongst environmental mechanisms was established.

Why is weapons grade plutonium more hazardous to work with than highly enriched uranium?

DOE PAGES

Cournoyer, Michael E.; Costigan, Stephen A.; Schake, Bradley S.

2015-08-01

Highly Enriched Uranium and Weapons grade plutonium have assumed positions of dominant importance among the actinide elements because of their successful uses as explosive ingredients in nuclear weapons and the place they hold as key materials in the development of industrial use of nuclear power. While most chemists are familiar with the practical interest concerning HEU and WG Pu, fewer know the subtleties among their hazards. In this study, a primer is provided regarding the hazards associated with working with HEU and WG Pu metals and oxides. The care that must be taken to safely handle these materials is emphasizedmore » and the extent of the hazards is described. The controls needed to work with HEU and WG Pu metals and oxides are differentiated. Given the choice, one would rather work with HEU metal and oxides than WG Pu metal and oxides.« less

Why is weapons grade plutonium more hazardous to work with than highly enriched uranium?

DOE Office of Scientific and Technical Information (OSTI.GOV)

Cournoyer, Michael E.; Costigan, Stephen A.; Schake, Bradley S.

Highly Enriched Uranium and Weapons grade plutonium have assumed positions of dominant importance among the actinide elements because of their successful uses as explosive ingredients in nuclear weapons and the place they hold as key materials in the development of industrial use of nuclear power. While most chemists are familiar with the practical interest concerning HEU and WG Pu, fewer know the subtleties among their hazards. In this study, a primer is provided regarding the hazards associated with working with HEU and WG Pu metals and oxides. The care that must be taken to safely handle these materials is emphasizedmore » and the extent of the hazards is described. The controls needed to work with HEU and WG Pu metals and oxides are differentiated. Given the choice, one would rather work with HEU metal and oxides than WG Pu metal and oxides.« less

DOE Office of Scientific and Technical Information (OSTI.GOV)

Not Available

The Department of Energy (DOE) has contracted with Asea Brown Boveri-Combustion Engineering (ABB-CE) to provide information on the capability of ABB-CE`s System 80 + Advanced Light Water Reactor (ALWR) to transform, through reactor burnup, 100 metric tonnes (MT) of weapons grade plutonium (Pu) into a form which is not readily useable in weapons. This information is being developed as part of DOE`s Plutonium Disposition Study, initiated by DOE in response to Congressional action. This document, Volume 1, presents a technical description of the various elements of the System 80 + Standard Plant Design upon which the Plutonium Disposition Study wasmore » based. The System 80 + Standard Design is fully developed and directly suited to meeting the mission objectives for plutonium disposal. The bass U0{sub 2} plant design is discussed here.« less

Exploding the myths about the fast breeder reactor

DOE Office of Scientific and Technical Information (OSTI.GOV)

Burns, S.

1979-01-01

This paper discusses the facts and figures about the effects of conservation policies, the benefits of the Clinch River Breeder Reactor demonstration plant, the feasibility of nuclear weapons manufacture from reactor-grade plutonium, diversion of plutonium from nuclear plants, radioactive waste disposal, and the toxicity of plutonium. The paper concludes that the U.S. is not proceeding with a high confidence strategy for breeder development because of a variety of false assumptions.

Heterogeneity Effects in Plutonium Contaminated Soil

DTIC Science & Technology

2009-03-01

masses up to one kilogram once the ratio of Americium - 241 (Am- 241 ) and plutonium concentrations was established (Rademacher, 2001). Alpha...with a sample number and tared weight with a non-smearing marker. A standard control was then set using a point source of Americium - 241 on an aluminum...During the fire the weapons grade plutonium (Pu- 239, Pu-240, and Pu- 241 ) ignited and was released into the surrounding area, due to both

Radiation Detection and Classification of Heavy Oxide Inorganic Scintillator Crystals for Detection of Fast Neutrons

DTIC Science & Technology

2016-06-01

of these three pillars, yet current detectors for fast neutrons from nuclear weapons materials are bulky, expensive, and have low efficiencies, well...passive fast neutron emissions. Similarly, isotopes present in weapons grade Plutonium (which is predominantly Pu-239), especially Pu-240, are... weapons material, and the propensity of the neutrons resulting from their fission to inelastically scatter, defines the interactions of interest

Screening study for evaluation of the potential for system 80+ to consume excess plutonium - Volume 1. Final report

DOE Office of Scientific and Technical Information (OSTI.GOV)

Not Available

1994-04-30

As part of the U.S. effort to evaluate technologies offering solutions for the safe disposal or utilization of surplus nuclear materials, the fiscal year 1993 Energy and Water Appropriations legislation provided the Department of Energy (DOE) the necessary funds to conduct multi-phased studies to determine the technical feasibility of using reactor technologies for the triple mission of burning weapons grade plutonium, producing tritium for the existing smaller weapons stockpile, and generating commercial electricity. DOE limited the studies to five advanced reactor designs. Among the technologies selected is the ABB-Combustion Engineering (ABB-CE) System 80+. The DOE study, currently in Phase ID,more » is proceeding with a more detailed evaluation of the design`s capability for plutonium disposition.« less

The effect of the composition of plutonium loaded on the reactivity change and the isotopic composition of fuel produced in a fast reactor

NASA Astrophysics Data System (ADS)

Blandinskiy, V. Yu.

2014-12-01

This paper presents the results of a numerical investigation into burnup and breeding of nuclides in metallic fuel consisting of a mixture of plutonium and depleted uranium in a fast reactor with sodium coolant. The feasibility of using plutonium contained in spent nuclear fuel from domestic thermal reactors and weapons-grade plutonium is discussed. It is shown that the largest production of secondary fuel and the least change in the reactivity over the reactor lifetime can be achieved when employing plutonium contained in spent nuclear fuel from a reactor of the RBMK-1000 type.

Actinide Waste Forms and Radiation Effects

NASA Astrophysics Data System (ADS)

Ewing, R. C.; Weber, W. J.

Over the past few decades, many studies of actinides in glasses and ceramics have been conducted that have contributed substantially to the increased understanding of actinide incorporation in solids and radiation effects due to actinide decay. These studies have included fundamental research on actinides in solids and applied research and development related to the immobilization of the high level wastes (HLW) from commercial nuclear power plants and processing of nuclear weapons materials, environmental restoration in the nuclear weapons complex, and the immobilization of weapons-grade plutonium as a result of disarmament activities. Thus, the immobilization of actinides has become a pressing issue for the twenty-first century (Ewing, 1999), and plutonium immobilization, in particular, has received considerable attention in the USA (Muller et al., 2002; Muller and Weber, 2001). The investigation of actinides and

Safe disposal of surplus plutonium

NASA Astrophysics Data System (ADS)

Gong, W. L.; Naz, S.; Lutze, W.; Busch, R.; Prinja, A.; Stoll, W.

2001-06-01

About 150 tons of weapons grade and weapons usable plutonium (metal, oxide, and in residues) have been declared surplus in the USA and Russia. Both countries plan to convert the metal and oxide into mixed oxide fuel for nuclear power reactors. Russia has not yet decided what to do with the residues. The US will convert residues into a ceramic, which will then be over-poured with highly radioactive borosilicate glass. The radioactive glass is meant to provide a deterrent to recovery of plutonium, as required by a US standard. Here we show a waste form for plutonium residues, zirconia/boron carbide (ZrO 2/B 4C), with an unprecedented combination of properties: a single, radiation-resistant, and chemically durable phase contains the residues; billion-year-old natural analogs are available; and criticality safety is given under all conceivable disposal conditions. ZrO 2/B 4C can be disposed of directly, without further processing, making it attractive to all countries facing the task of plutonium disposal. The US standard for protection against recovery can be met by disposal of the waste form together with used reactor fuel.

Detection of Nuclear Weapons and Materials: Science, Technologies, Observations

DTIC Science & Technology

2010-06-04

extensive use of photons, packets of energy with no rest mass and no electrical charge. Electromagnetic radiation consists of photons, and may be measured...bulk property, expressed as mass per unit volume. In general, the densest materials are those of high Z. These properties may be used to detect...SNM by detecting the time pattern of neutron generation. A subcritical mass of highly enriched uranium or weapons-grade plutonium can support a

Assessment of Non-traditional Isotopic Ratios by Mass Spectrometry for Analysis of Nuclear Activities. Annual Report 2011

DOE Office of Scientific and Technical Information (OSTI.GOV)

Biegalski, Steven R.; Buchholz, Bruce A.

2011-08-24

The objective of this work is to identify isotopic ratios suitable for analysis via mass spectrometry that distinguish between commercial nuclear reactor fuel cycles, fuel cycles for weapons grade plutonium, and products from nuclear weapons explosions. Methods will also be determined to distinguish the above from medical and industrial radionuclide sources. Mass spectrometry systems will be identified that are suitable for field measurement of such isotopes in an expedient manner.

Characterization and source term assessments of radioactive particles from Marshall Islands using non-destructive analytical techniques

NASA Astrophysics Data System (ADS)

Jernström, J.; Eriksson, M.; Simon, R.; Tamborini, G.; Bildstein, O.; Marquez, R. Carlos; Kehl, S. R.; Hamilton, T. F.; Ranebo, Y.; Betti, M.

2006-08-01

Six plutonium-containing particles stemming from Runit Island soil (Marshall Islands) were characterized by non-destructive analytical and microanalytical methods. Composition and elemental distribution in the particles were studied with synchrotron radiation based micro X-ray fluorescence spectrometry. Scanning electron microscope equipped with energy dispersive X-ray detector and with wavelength dispersive system as well as a secondary ion mass spectrometer were used to examine particle surfaces. Based on the elemental composition the particles were divided into two groups: particles with pure Pu matrix, and particles where the plutonium is included in Si/O-rich matrix being more heterogenously distributed. All of the particles were identified as nuclear fuel fragments of exploded weapon components. As containing plutonium with low 240Pu/ 239Pu atomic ratio, less than 0.065, which corresponds to weapons-grade plutonium or a detonation with low fission yield, the particles were identified to originate from the safety test and low-yield tests conducted in the history of Runit Island. The Si/O-rich particles contained traces of 137Cs ( 239 + 240 Pu/ 137Cs activity ratio higher than 2500), which indicated that a minor fission process occurred during the explosion. The average 241Am/ 239Pu atomic ratio in the six particles was 3.7 × 10 - 3 ± 0.2 × 10 - 3 (February 2006), which indicated that plutonium in the different particles had similar age.

New Organic Scintillators for Neutron Detection

DTIC Science & Technology

2016-03-01

highly enriched uranium and weapons grade plutonium. Neutrons and gamma rays are two signatures of these materials. Gamma ray detection techniques are...New Organic Scintillators for Neutron Detection Distribution Statement A. Approved for public release; distribution is unlimited. March...Title: New Organic Scintillators for Neutron Detection I. Abstract In this project, Radiation Monitoring Devices (RMD) proposes to develop novel

Long-term retrievability and safeguards for immobilized weapons plutonium in geologic storage

DOE Office of Scientific and Technical Information (OSTI.GOV)

Peterson, P.F.

1996-05-01

If plutonium is not ultimately used as an energy source, the quantity of excess weapons plutonium (w-Pu) that would go into a US repository will be small compared to the quantity of plutonium contained in the commercial spent fuel in the repository, and the US repository(ies) will likely be only one (or two) locations out of many around the world where commercial spent fuel will be stored. Therefore excess weapons plutonium creates a small perturbation to the long-term (over 200,000 yr) global safeguard requirements for spent fuel. There are details in the differences between spent fuel and immobilized w-Pu wastemore » forms (i.e. chemical separation methods, utility for weapons, nuclear testing requirements), but these are sufficiently small to be unlikely to play a significant role in any US political decision to rebuild weapons inventories, or to change the long-term risks of theft by subnational groups.« less

NCSP IER 422 CED-3b Documentation

DOE Office of Scientific and Technical Information (OSTI.GOV)

Hutchinson, Jesson D.; Cutler, Theresa Elizabeth; Bahran, Rian Mustafa

2017-11-22

A Subcritical Copper-Reflected α-phase Plutonium (SCRαP) integral benchmark experiment has been designed and measured. In this experiment, multiplication is approximated using correlated neutron data from a detector system consisting of 3He tubes inside high density polyethylene (HDPE). Measurements were performed on various subcritical experimental configurations consisting of a weapons-grade plutonium sphere surrounded by different Cu thicknesses. In addition to the proposed base experimental configurations with Cu, additional configurations were performed with the plutonium ball nested in various thicknesses of interleaved HDPE spherical shells mixed in with the Cu shells. The HDPE is intended to provide fast neutron moderation and reflection,more » resulting in additional measurements with differing multiplication, spectra, and nuclear data sensitivity.« less

Superconducting RF Linacs Driving Subcritical Reactors for Profitable Disposition of Surplus Weapons-grade Plutonium

NASA Astrophysics Data System (ADS)

Cummings, Mary Anne; Johnson, Rolland

Acceptable capital and operating costs of high-power proton accelerators suitable for profitable commercial electric-power and process-heat applications have been demonstrated. However, studies have pointed out that even a few hundred trips of an accelerator lasting a few seconds would lead to unacceptable thermal stresses as each trip causes fission to be turned off in solid fuel structures found in conventional reactors. The newest designs based on the GEM*STAR concept take such trips in stride by using molten-salt fuel, where fuel pin fatigue is not an issue. Other aspects of the GEM*STAR concept which address all historical reactor failures include an internal spallation neutron target and high temperature molten salt fuel with continuous purging of volatile radioactive fission products such that the reactor contains less than a critical mass and almost a million times fewer volatile radioactive fission products than conventional reactors. GEM*STAR is a reactor that without redesign will burn spent nuclear fuel, natural uranium, thorium, or surplus weapons material. It will operate without the need for a critical core, fuel enrichment, or reprocessing making it an excellent candidate for export. As a first application, the design for a pilot plant is described for the profitable disposition of surplus weapons-grade plutonium by using process heat to produce green diesel fuel for the Department of Defense (DOD) from natural gas and renewable carbon.

Effects of Aging on PuO2∙xH2O Particle Size in Alkaline Solution

DOE Office of Scientific and Technical Information (OSTI.GOV)

Delegard, Calvin H.

Between 1944 and 1989, 54.5 metric tons of the United States’ weapons-grade plutonium and an additional 12.9 metric tons of fuel-grade plutonium were produced and separated from irradiated fuel at the Hanford Site. Acidic high-activity wastes containing around 600 kg of plutonium were made alkaline and discharged to underground storage tanks from separations, isolation, and recycle processes to yield average plutonium concentration of about 0.003 grams per liter (or ~0.0002 wt%) in the ~200 million liter tank waste volume. The plutonium is largely associated with low-solubility metal hydroxide/oxide sludges where its low concentration and intimate mixture with neutron-absorbing elements (e.g.,more » iron) are credited in nuclear criticality safety. However, concerns have been expressed that plutonium, in the form of plutonium hydrous oxide, PuO2∙xH2O, could undergo sufficient crystal growth through dissolution and reprecipitation in the alkaline tank waste to potentially become separable from neutron absorbing constituents by settling or sedimentation. Thermodynamic considerations and laboratory studies of systems chemically analogous to tank waste show that the plutonium formed in the alkaline tank waste by precipitation through neutralization from acid solution probably entered as 2–4-nm PuO2∙xH2O crystallite particles that, because of their low solubility and opposition from radiolytic processes, grow from that point at exceedingly slow rates, thus posing no risk of physical segregation.« less

Leo Szilard Lectureship Award Talk: Controlling and eliminating nuclear-weapon materials

NASA Astrophysics Data System (ADS)

von Hippel, Frank

2010-02-01

Fissile material -- in practice plutonium and highly enriched uranium (HEU) -- is the essential ingredient in nuclear weapons. Controlling and eliminating fissile material and the means of its production is therefore the common denominator for nuclear disarmament, nuclear non-proliferation and the prevention of nuclear terrorism. From a fundamentalist anti-nuclear-weapon perspective, the less fissile material there is and the fewer locations where it can be found, the safer a world we will have. A comprehensive fissile-material policy therefore would have the following elements: *Consolidation of all nuclear-weapon-usable materials at a minimum number of high-security sites; *A verified ban on the production of HEU and plutonium for weapons; *Minimization of non-weapon uses of HEU and plutonium; and *Elimination of all excess stocks of plutonium and HEU. There is activity on all these fronts but it is not comprehensive and not all aspects are being pursued vigorously or competently. It is therefore worthwhile to review the situation. )

Stabilization and immobilization of military plutonium: A non-proliferation perspective

DOE Office of Scientific and Technical Information (OSTI.GOV)

Leventhal, P.

1996-05-01

The Nuclear Control Institute welcomes this DOE-sponsored technical workshop on stabilization and immobilization of weapons plutonium (W Pu) because of the significant contribution it can make toward the ultimate non-proliferation objective of eliminating weapons-usable nuclear material, plutonium and highly enriched uranium (HEU), from world commerce. The risk of theft or diversion of these materials warrants concern, as only a few kilograms in the hands of terrorists or threshold states would give them the capability to build nuclear weapons. Military plutonium disposition questions cannot be addressed in isolation from civilian plutonium issues. The National Academy of Sciences has urged that {open_quotes}furthermore » steps should be taken to reduce the proliferation risks posed by all of the world`s plutonium stocks, military and civilian, separated and unseparated...{close_quotes}. This report discusses vitrification and a mixed oxide fuels option, and the effects of disposition choices on civilian plutonium fuel cycles.« less

Fuzzy-probabilistic model for risk assessment of radioactive material railway transportation.

PubMed

Avramenko, M; Bolyatko, V; Kosterev, V

2005-01-01

Transportation of radioactive materials is obviously accompanied by a certain risk. A model for risk assessment of emergency situations and terrorist attacks may be useful for choosing possible routes and for comparing the various defence strategies. In particular, risk assessment is crucial for safe transportation of excess weapons-grade plutonium arising from the removal of plutonium from military employment. A fuzzy-probabilistic model for risk assessment of railway transportation has been developed taking into account the different natures of risk-affecting parameters (probabilistic and not probabilistic but fuzzy). Fuzzy set theory methods as well as standard methods of probability theory have been used for quantitative risk assessment. Information-preserving transformations are applied to realise the correct aggregation of probabilistic and fuzzy parameters. Estimations have also been made of the inhalation doses resulting from possible accidents during plutonium transportation. The obtained data show the scale of possible consequences that may arise from plutonium transportation accidents.

SHIELDING AND DETECTOR RESPONSE CALCULATIONS PERTAINING TO CATEGORY 1 QUANTITIES OF PLUTONIUM AND HAND-HELD PLASTIC SCINTILLATORS

DOE Office of Scientific and Technical Information (OSTI.GOV)

Couture, A.

2013-06-07

Nuclear facilities sometimes use hand-held plastic scintillator detectors to detect attempts to divert special nuclear material in situations where portal monitors are impractical. MCNP calculations have been performed to determine the neutron and gamma radiation field arising from a Category I quantity of weapons-grade plutonium in various shielding configurations. The shields considered were composed of combinations of lead and high-density polyethylene such that the mass of the plutonium plus shield was 22.7 kilograms. Monte-Carlo techniques were also used to determine the detector response to each of the shielding configurations. The detector response calculations were verified using field measurements of high-,more » medium-, and low- energy gamma-ray sources as well as a Cf-252 neutron source.« less

Neutronics calculations on the impact of burnable poisons to safety and non-proliferation aspects of inert matrix fuel

NASA Astrophysics Data System (ADS)

Pistner, C.; Liebert, W.; Fujara, F.

2006-06-01

Inert matrix fuels (IMF) with plutonium may play a significant role to dispose of stockpiles of separated plutonium from military or civilian origin. For reasons of reactivity control of such fuels, burnable poisons (BP) will have to be used. The impact of different possible BP candidates (B, Eu, Er and Gd) on the achievable burnup as well as on safety and non-proliferation aspects of IMF are analyzed. To this end, cell burnup calculations have been performed and burnup dependent reactivity coefficients (boron worth, fuel temperature and moderator void coefficient) were calculated. All BP candidates were analyzed for one initial BP concentration and a range of different initial plutonium-concentrations (0.4-1.0 g cm-3) for reactor-grade plutonium isotopic composition as well as for weapon-grade plutonium. For the two most promising BP candidates (Er and Gd), a range of different BP concentrations was investigated to study the impact of BP concentration on fuel burnup. A set of reference fuels was identified to compare the performance of uranium-fuels, MOX and IMF with respect to (1) the fraction of initial plutonium being burned, (2) the remaining absolute plutonium concentration in the spent fuel and (3) the shift in the isotopic composition of the remaining plutonium leading to differences in the heat and neutron rate produced. In the case of IMF, the remaining Pu in spent fuel is unattractive for a would be proliferator. This underlines the attractiveness of an IMF approach for disposal of Pu from a non-proliferation perspective.

11. VIEW OF A SITE RETURN WEAPONS COMPONENT. SITE RETURNS ...

Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

11. VIEW OF A SITE RETURN WEAPONS COMPONENT. SITE RETURNS WERE NUCLEAR WEAPONS SHIPPED TO THE ROCKY FLATS PLANT FROM THE NUCLEAR WEAPON STOCKPILE FOR RETIREMENT, TESTING, OR UPGRADING. FISSILE MATERIALS (PLUTONIUM, URANIUM, ETC.) AND RARE MATERIALS (BERYLLIUM) WERE RECOVERED FOR REUSE, AND THE REMAINDER WAS DISPOSED. (8/7/62) - Rocky Flats Plant, Plutonium Fabrication, Central section of Plant, Golden, Jefferson County, CO

Improving proliferation resistance of high breeding gain generation 4 reactors using blankets composed of light water reactor waste

DOE Office of Scientific and Technical Information (OSTI.GOV)

Hellesen, C.; Grape, S.; Haakanson, A.

2013-07-01

Fertile blankets can be used in fast reactors to enhance the breeding gain as well as the passive safety characteristics. However, such blankets typically result in the production of weapons grade plutonium. For this reason they are often excluded from Generation IV reactor designs. In this paper we demonstrate that using blankets manufactured directly from spent light water (LWR) reactor fuel it is possible to produce a plutonium product with non-proliferation characteristics on a par with spent LWR fuel of 30-50 MWd/kg burnup. The beneficial breeding and safety characteristics are retained. (authors)

Excess Weapons Plutonium Disposition: Plutonium Packaging, Storage and Transportation and Waste Treatment, Storage and Disposal Activities

DOE Office of Scientific and Technical Information (OSTI.GOV)

Jardine, L J; Borisov, G B

2004-07-21

A fifth annual Excess Weapons Plutonium Disposition meeting organized by Lawrence Livermore National Laboratory (LLNL) was held February 16-18, 2004, at the State Education Center (SEC), 4 Aerodromnya Drive, St. Petersburg, Russia. The meeting discussed Excess Weapons Plutonium Disposition topics for which LLNL has the US Technical Lead Organization responsibilities. The technical areas discussed included Radioactive Waste Treatment, Storage, and Disposal, Plutonium Oxide and Plutonium Metal Packaging, Storage and Transportation and Spent Fuel Packaging, Storage and Transportation. The meeting was conducted with a conference format using technical presentations of papers with simultaneous translation into English and Russian. There were 46more » Russian attendees from 14 different Russian organizations and six non-Russian attendees, four from the US and two from France. Forty technical presentations were made. The meeting agenda is given in Appendix B and the attendance list is in Appendix C.« less

Plutonium Isotopes in the Terrestrial Environment at the Savannah River Site, USA. A Long-Term Study

DOE PAGES

Armstrong, Christopher R.; Nuessle, Patterson R.; Brant, Heather A.; ...

2015-01-16

This work presents the findings of a long term plutonium study at Savannah River Site (SRS) conducted between 2003 and 2013. Terrestrial environmental samples were obtained at Savannah River National Laboratory (SRNL) in A-area. Plutonium content and isotopic abundances were measured over this time period by alpha spectrometry and three stage thermal ionization mass spectrometry (3STIMS). Here we detail the complete sample collection, radiochemical separation, and measurement procedure specifically targeted to trace plutonium in bulk environmental samples. Total plutonium activities were determined to be not significantly above atmospheric global fallout. However, the 238Pu/ 239+240Pu activity ratios attributed to SRS aremore » above atmospheric global fallout ranges. The 240Pu/ 239Pu atom ratios are reasonably consistent from year to year and are lower than fallout, while the 242Pu/ 239Pu atom ratios are higher than fallout values. Overall, the plutonium signatures obtained in this study reflect a mixture of weapons-grade, higher burn-up, and fallout material. This study provides a blue print for long term low level monitoring of plutonium in the environment.« less

Plutonium in the arctic marine environment--a short review.

PubMed

Skipperud, Lindis

2004-06-18

Anthropogenic plutonium has been introduced into the environment over the past 50 years as the result of the detonation of nuclear weapons and operational releases from the nuclear industry. In the Arctic environment, the main source of plutonium is from atmospheric weapons testing, which has resulted in a relatively uniform, underlying global distribution of plutonium. Previous studies of plutonium in the Kara Sea have shown that, at certain sites, other releases have given rise to enhanced local concentrations. Since different plutonium sources are characterised by distinctive plutonium-isotope ratios, evidence of a localised influence can be supported by clear perturbations in the plutonium-isotope ratio fingerprints as compared to the known ratio in global fallout. In Kara Sea sites, such perturbations have been observed as a result of underwater weapons tests at Chernaya Bay, dumped radioactive waste in Novaya Zemlya, and terrestrial runoff from the Ob and Yenisey Rivers. Measurement of the plutonium-isotope ratios offers both a means of identifying the origin of radionuclide contamination and the influence of the various nuclear installations on inputs to the Arctic, as well as a potential method for following the movement of water and sediment loads in the rivers.

Calorimetry of low mass Pu239 items

DOE Office of Scientific and Technical Information (OSTI.GOV)

Cremers, Teresa L; Sampson, Thomas E

2010-01-01

Calorimetric assay has the reputation of providing the highest precision and accuracy of all nondestructive assay measurements. Unfortunately, non-destructive assay practitioners and measurement consumers often extend, inappropriately, the high precision and accuracy of calorimetric assay to very low mass items. One purpose of this document is to present more realistic expectations for the random uncertainties associated with calorimetric assay for weapons grade plutonium items with masses of 200 grams or less.

Radiochemical determination of 237NP in soil samples contaminated with weapon grade plutonium

NASA Astrophysics Data System (ADS)

Antón, M. P.; Espinosa, A.; Aragón, A.

2006-01-01

The Palomares terrestrial ecosystem (Spain) constitutes a natural laboratory to study transuranics. This scenario is partially contaminated with weapon-grade plutonium since the burnout and fragmentation of two thermonuclear bombs accidentally dropped in 1966. While performing radiometric measurements in the field, the possible presence of 237Np was observed through its 29 keV gamma emission. To accomplish a detailed characterization of the source term in the contaminated area using the isotopic ratios Pu-Am-Np, the radiochemical isolation and quantification by alpha spectrometry of 237Np was initiated. The selected radiochemical procedure involves separation of Np from Am, U and Pu with ionic resins, given that in soil samples from Palomares 239+240Pu levels are several orders of magnitude higher than 237Np. Then neptunium is isolated using TEVA organic resins. After electrodeposition, quantification is performed by alpha spectrometry. Different tests were done with blank solutions spiked with 236Pu and 237Np, solutions resulting from the total dissolution of radioactive particles and soil samples. Results indicate that the optimal sequential radionuclide separation order is Pu-Np, with decontamination percentages obtained with the ionic resins ranging from 98% to 100%. Also, the addition of NaNO2 has proved to be necessary, acting as a stabilizer of Pu-Np valences.

A Plutonium-Contaminated Wound, 1985, USA

DOE Office of Scientific and Technical Information (OSTI.GOV)

Doran M. Christensen, DO, REAC /TS Associate Director and Staff Physician Eugene H. Carbaugh, CHP, Staff Scientist, Internal Dosimetry Manager, Pacific Northwest National Laboratory, Richland, Washington

2012-02-02

A hand injury occurred at a U.S. facility in 1985 involving a pointed shaft (similar to a meat thermometer) that a worker was using to remove scrap solid plutonium from a plastic bottle. The worker punctured his right index finger on the palm side at the metacarpal-phalangeal joint. The wound was not through-and- through, although it was deep. The puncture wound resulted in deposition of ~48 kBq of alpha activity from the weapons-grade plutonium mixture with a nominal 12 to 1 Pu-alpha to {sup 241}Am-alpha ratio. This case clearly showed that DTPA was very effective for decorporation of plutonium andmore » americium. The case is a model for management of wounds contaminated with transuranics: (1) a team approach for dealing with all of the issues surrounding the incident, including the psychological, (2) early surgical intervention for foreign-body removal, (3) wound irrigation with DTPA solution, and (4) early and prolonged DTPA administration based upon bioassay and in vivo dosimetry.« less

One perspective on stakeholder involvement at Hanford.

PubMed

Martin, Todd

2011-11-01

The Hanford nuclear site in Washington State had a major role in the production of nuclear weapons materials during the Manhattan Project in World War II and during the Cold War that followed. The production of weapons-grade radionuclides produced a large amount of radioactive byproducts that have been stored since the mid-1900s at the Hanford Site. These by-product radionuclides have leaked from containment facilities into the groundwater, contaminated buildings used for radionuclide processing, and also contaminated the nuclear reactors used to produce weapons-grade uranium and plutonium. This issue has been a major concern to Hanford stakeholders for several decades, and the U.S. Department of Energy, the U.S. Environmental Protection Agency, and the Washington State Department of Ecology established a Tri-Party Agreement in 1989, at which time Hanford ceased production of nuclear weapons materials and began a major effort to clean up and remediate the Hanford Site's contaminated groundwater, soil, and facilities. This paper describes the concerns of stakeholders in the production of nuclear weapons, the secrecy of Hanford operations, and the potential impacts to public health and the environment from the unintended releases of weapons-grade materials and by-products associated with their production at the Hanford Site. It also describes the involvement of public stakeholders in the development and oversight by the Hanford Advisory Board of the steps that have been taken in cleanup activities at the Hanford Site that began as a major effort about two decades ago. The importance of involvement of the general public and public interest organizations in developing and implementing the Hanford cleanup strategy are described in detail.

Radionuclide Basics: Plutonium

EPA Pesticide Factsheets

Plutonium (chemical symbol Pu) is a radioactive metal. Plutonium is considered a man-made element. Plutonium-239 is used to make nuclear weapons. Pu-239 and Pu-240 are byproducts of nuclear reactor operations and nuclear bomb explosions.

MOX fuel arrangement for nuclear core

DOEpatents

Kantrowitz, M.L.; Rosenstein, R.G.

1998-10-13

In order to use up a stockpile of weapons-grade plutonium, the plutonium is converted into a mixed oxide (MOX) fuel form wherein it can be disposed in a plurality of different fuel assembly types. Depending on the equilibrium cycle that is required, a predetermined number of one or more of the fuel assembly types are selected and arranged in the core of the reactor in accordance with a selected loading schedule. Each of the fuel assemblies is designed to produce different combustion characteristics whereby the appropriate selection and disposition in the core enables the resulting equilibrium cycle to closely resemble that which is produced using urania fuel. The arrangement of the MOX rods and burnable absorber rods within each of the fuel assemblies, in combination with a selective control of the amount of plutonium which is contained in each of the MOX rods, is used to tailor the combustion characteristics of the assembly. 38 figs.

Mox fuel arrangement for nuclear core

DOEpatents

Kantrowitz, Mark L.; Rosenstein, Richard G.

2001-05-15

In order to use up a stockpile of weapons-grade plutonium, the plutonium is converted into a mixed oxide (MOX) fuel form wherein it can be disposed in a plurality of different fuel assembly types. Depending on the equilibrium cycle that is required, a predetermined number of one or more of the fuel assembly types are selected and arranged in the core of the reactor in accordance with a selected loading schedule. Each of the fuel assemblies is designed to produce different combustion characteristics whereby the appropriate selection and disposition in the core enables the resulting equilibrium cycle to closely resemble that which is produced using urania fuel. The arrangement of the MOX rods and burnable absorber rods within each of the fuel assemblies, in combination with a selective control of the amount of plutonium which is contained in each of the MOX rods, is used to tailor the combustion. characteristics of the assembly.

MOX fuel arrangement for nuclear core

DOEpatents

Kantrowitz, Mark L.; Rosenstein, Richard G.

2001-07-17

In order to use up a stockpile of weapons-grade plutonium, the plutonium is converted into a mixed oxide (MOX) fuel form wherein it can be disposed in a plurality of different fuel assembly types. Depending on the equilibrium cycle that is required, a predetermined number of one or more of the fuel assembly types are selected and arranged in the core of the reactor in accordance with a selected loading schedule. Each of the fuel assemblies is designed to produce different combustion characteristics whereby the appropriate selection and disposition in the core enables the resulting equilibrium cycle to closely resemble that which is produced using urania fuel. The arrangement of the MOX rods and burnable absorber rods within each of the fuel assemblies, in combination with a selective control of the amount of plutonium which is contained in each of the MOX rods, is used to tailor the combustion characteristics of the assembly.

MOX fuel arrangement for nuclear core

DOEpatents

Kantrowitz, Mark L.; Rosenstein, Richard G.

1998-01-01

In order to use up a stockpile of weapons-grade plutonium, the plutonium is converted into a mixed oxide (MOX) fuel form wherein it can be disposed in a plurality of different fuel assembly types. Depending on the equilibrium cycle that is required, a predetermined number of one or more of the fuel assembly types are selected and arranged in the core of the reactor in accordance with a selected loading schedule. Each of the fuel assemblies is designed to produce different combustion characteristics whereby the appropriate selection and disposition in the core enables the resulting equilibrium cycle to closely resemble that which is produced using urania fuel. The arrangement of the MOX rods and burnable absorber rods within each of the fuel assemblies, in combination with a selective control of the amount of plutonium which is contained in each of the MOX rods, is used to tailor the combustion characteristics of the assembly.

12. VIEW OF A SITE RETURN WEAPONS COMPONENT. AFTER SEGREGATION, ...

Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

12. VIEW OF A SITE RETURN WEAPONS COMPONENT. AFTER SEGREGATION, PLUTONIUM MATERIALS WERE EITHER RETURNED TO THE BUILDING 776 FOUNDRY WHERE THEY WERE CAST INTO FEED INGOTS, OR UNDERWENT CHEMICAL RECOVERY FOR PURIFICATION. (8/7/62) - Rocky Flats Plant, Plutonium Fabrication, Central section of Plant, Golden, Jefferson County, CO

31. VIEW OF A WORKER HOLDING A PLUTONIUM 'BUTTON.' PLUTONIUM, ...

Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

31. VIEW OF A WORKER HOLDING A PLUTONIUM 'BUTTON.' PLUTONIUM, A MAN-MADE SUBSTANCE, WAS RARE. SCRAPS RESULTING FROM PRODUCTION AND PLUTONIUM RECOVERED FROM RETIRED NUCLEAR WEAPONS WERE REPROCESSED INTO VALUABLE PURE-PLUTONIUM METAL (9/19/73). - Rocky Flats Plant, Bounded by Indiana Street & Routes 93, 128 & 72, Golden, Jefferson County, CO

Determining Reactor Fuel Type from Continuous Antineutrino Monitoring

NASA Astrophysics Data System (ADS)

Jaffke, Patrick; Huber, Patrick

2017-09-01

We investigate the ability of an antineutrino detector to determine the fuel type of a reactor. A hypothetical 5-ton antineutrino detector is placed 25 m from the core and measures the spectral shape and rate of antineutrinos emitted by fission fragments in the core for a number of 90-d periods. Our results indicate that four major fuel types can be differentiated from the variation of fission fractions over the irradiation time with a true positive probability of detection at approximately 95%. In addition, we demonstrate that antineutrinos can identify the burnup at which weapons-grade mixed-oxide (MOX) fuel would be reduced to reactor-grade MOX, on average, providing assurance that plutonium-disposition goals are met. We also investigate removal scenarios where plutonium is purposefully diverted from a mixture of MOX and low-enriched uranium fuel. Finally, we discuss how our analysis is impacted by a spectral distortion around 6 MeV observed in the antineutrino spectrum measured from commercial power reactors.

Determination of the 240Pu/ 239Pu atomic ratio in soils from Palomares (Spain) by low-energy accelerator mass spectrometry

NASA Astrophysics Data System (ADS)

Chamizo, E.; García-León, M.; Synal, H.-A.; Suter, M.; Wacker, L.

2006-08-01

In 1966, the nuclear fuel of two thermonuclear bombs was released over the Spanish region of Palomares, due to a B52 bomber accident during a refuelling operation. Since then, much effort has been made to assess its impact to the different environmental compartments of this area in South-East Spain, mostly by measuring the 239+240Pu activity concentration and the 238Pu/239+240Pu activity ratio. Nevertheless, these measurements do not give enough information on the problem. In order to recognize unambiguously small traces of the weapon-grade plutonium released in the accident, the ratio of the two major isotopes of plutonium, 240Pu/239Pu, has to be determined. In this work, this ratio has been measured in low- and high-activity samples from Palomares by means of low-energy accelerator mass spectrometry (AMS). That way, we will show the potential of the new generation of compact AMS facilities in terms of plutonium characterization at ultra-trace levels.

The North Korean nuclear dilemma.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Hecker, Siegfried S.

2004-01-01

The current nuclear crisis, the second one in ten years, erupted when North Korea expelled international nuclear inspectors in December 2002, then withdrew from the Nuclear Nonproliferation Treaty (NPT), and claimed to be building more nuclear weapons with the plutonium extracted from the spent fuel rods heretofore stored under international inspection. These actions were triggered by a disagreement over U.S. assertions that North Korea had violated the Agreed Framework (which froze the plutonium path to nuclear weapons to end the first crisis in 1994) by clandestinely developing uranium enrichment capabilities providing an alternative path to nuclear weapons. With Stanford Universitymore » Professor John Lewis and three other Americans, I was allowed to visit the Yongbyon Nuclear Center on Jan. 8, 2004. We toured the 5 MWe reactor, the 50 MWe reactor construction site, the spent fuel pool storage building, and the radiochemical laboratory. We concluded that North Korea has restarted its 5 MWe reactor (which produces roughly 6 kg of plutonium annually), it removed the 8000 spent fuel rods that were previously stored under IAEA safeguards from the spent fuel pool, and that it most likely extracted the 25 to 30 kg of plutonium contained in these fuel rods. Although North Korean officials showed us what they claimed was their plutonium metal product from this reprocessing campaign, we were not able to conclude definitively that it was in fact plutonium metal and that it came from the most recent reprocessing campaign. Nevertheless, our North Korean hosts demonstrated that they had the capability, the facility and requisite capacity, and the technical expertise to produce plutonium metal. On the basis of our visit, we were not able to address the issue of whether or not North Korea had a 'deterrent' as claimed - that is, we were not able to conclude that North Korea can build a nuclear device and that it can integrate nuclear devices into suitable delivery systems. However, based on the capabilities we saw, we must assume that North Korea has the capability to produce a crude nuclear device. On the matter of uranium enrichment programs, our host categorically denied that North Korea has a uranium enrichment program - he said, 'we have no program, no equipment, and no technical expertise for uranium enrichment.' The denials were not convincing at the time and since then have proven to be quite hollow by the revelations of A.Q. Khan's nuclear black market activities. There is no easy solution to the nuclear crisis in North Korea. A military strike to eliminate the nuclear facilities was never very attractive and now has been overcome by events. The principal threat is posed by a stockpile of nuclear weapons and weapons-grade plutonium. We have no way of finding where either may be hidden. A diplomatic solution remains the only path forward, but it has proven elusive. All sides have proclaimed a nuclear weapons-free Korean Peninsula as the end goal. The U.S. Government has chosen to negotiate with North Korea by means of the six-party talks. It has very clearly outlined its position of insisting on complete, verifiable, irreversible dismantlement of all North Korean nuclear programs. North Korea has offered several versions of 're-freezing' its plutonium program while still denying a uranium enrichment program. It has insisted on simultaneous and reciprocal steps to a final solution. Regardless of which diplomatic path is chosen, the scientific challenges of eliminating the North Korean nuclear weapons programs (and its associated infrastructure) in a safe, secure, and verifiable manner are immense. The North Korean program is considerably more complex and developed than the fledgling Iraqi program of 1991 and Libyan program of 2004. It is more along the lines, but more complex than that of South Africa in the early 1990s. Actions taken or not taken by the North Koreans at their nuclear facilities during the course of the ongoing diplomatic discussions are key to whether or not the nuclear program can be eliminated safely and securely, and they will greatly influence the price tag for such operations. Moreover, they will determine whether or not one can verify complete elimination. Hence, cooperation of the North Koreans now and during the dismantlement and elimination stages is crucial. Technical discussions among specialists, perhaps within the framework of the working groups of the six-party talks, could be very productive in setting the stage for an effective, verifiable elimination of North Korea's nuclear weapons program.« less

69. INTERIOR, BUILDING 272 (PLUTONIUM STORAGE BUILDING) LOOKING SOUTHWEST THROUGH ...

Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

69. INTERIOR, BUILDING 272 (PLUTONIUM STORAGE BUILDING) LOOKING SOUTHWEST THROUGH DOOR-WAY INTO PLUTONIUM STORAGE AREA. - Loring Air Force Base, Weapons Storage Area, Northeastern corner of base at northern end of Maine Road, Limestone, Aroostook County, ME

Zirconia ceramics for excess weapons plutonium waste

NASA Astrophysics Data System (ADS)

Gong, W. L.; Lutze, W.; Ewing, R. C.

2000-01-01

We synthesized a zirconia (ZrO 2)-based single-phase ceramic containing simulated excess weapons plutonium waste. ZrO 2 has large solubility for other metallic oxides. More than 20 binary systems A xO y-ZrO 2 have been reported in the literature, including PuO 2, rare-earth oxides, and oxides of metals contained in weapons plutonium wastes. We show that significant amounts of gadolinium (neutron absorber) and yttrium (additional stabilizer of the cubic modification) can be dissolved in ZrO 2, together with plutonium (simulated by Ce 4+, U 4+ or Th 4+) and impurities (e.g., Ca, Mg, Fe, Si). Sol-gel and powder methods were applied to make homogeneous, single-phase zirconia solid solutions. Pu waste impurities were completely dissolved in the solid solutions. In contrast to other phases, e.g., zirconolite and pyrochlore, zirconia is extremely radiation resistant and does not undergo amorphization. Baddeleyite (ZrO 2) is suggested as the natural analogue to study long-term radiation resistance and chemical durability of zirconia-based waste forms.

Plutonium segregation in glassy aerodynamic fallout from a nuclear weapon test

DOE PAGES

Holliday, K. S.; Dierken, J. M.; Monroe, M. L.; ...

2017-01-11

Our study combines electron microscopy equipped with energy dispersive spectroscopy to probe major element composition and autoradiography to map plutonium in order to examine the spatial relationships between plutonium and fallout composition in aerodynamic glassy fallout from a nuclear weapon test. We interrogated a sample set of 48 individual fallout specimens in order to reveal that the significant chemical heterogeneity of this sample set could be described compositionally with a relatively small number of compositional endmembers. Furthermore, high concentrations of plutonium were never associated with several endmember compositions and concentrated with the so-called mafic glass endmember. Our result suggests thatmore » it is the physical characteristics of the compositional endmembers and not the chemical characteristics of the individual component elements that govern the un-burnt plutonium distribution with respect to major element composition in fallout.« less

71. INTERIOR, BUILDING 272 (PLUTONIUM STORAGE BUILDING) LOOKING NORTHEAST INTO ...

Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

71. INTERIOR, BUILDING 272 (PLUTONIUM STORAGE BUILDING) LOOKING NORTHEAST INTO PLUTONIUM STORAGE ROOM SHOWING CUBICLES FOR STORAGE. - Loring Air Force Base, Weapons Storage Area, Northeastern corner of base at northern end of Maine Road, Limestone, Aroostook County, ME

Advanced Quantification of Plutonium Ionization Potential to Support Nuclear Forensic Evaluations by Resonance Ionization Mass Spectrometry

DTIC Science & Technology

2015-06-01

Research Committee nm Nanometer Np Neptunium NPT Treaty of Non-proliferation of Nuclear Weapons ns Nanosecond ps Picosecond Pu Plutonium RIMS...discovery—credited also to Fritz Strassman— scientists realized these reactions also emitted secondary neutrons . These secondary neutrons could in...destructive capabilities of nuclear fission and atomic weapons . Figure 1. Uranium-235 Fission chain reaction, from [1

A Stochastic Imaging Technique for Spatio-Spectral Characterization of Special Nuclear Material

NASA Astrophysics Data System (ADS)

Hamel, Michael C.

Radiation imaging is advantageous for detecting, locating and characterizing special nuclear material (SNM) in complex environments. A dual-particle imager (DPI) has been designed that is capable of detecting gamma-ray and neutron signatures from shielded SNM. The system combines liquid organic and NaI(Tl) scintillators to form a combined Compton and neutron scatter camera. Effective image reconstruction of detected particles is a crucial component for maximizing the performance of the system; however, a key deficiency exists in the widely used list-mode maximum-likelihood estimation-maximization (MLEM) image reconstruction technique. The steady-state solution produced by this iterative method will have poor quality compared to solutions produced with fewer iterations. A stopping condition is required to achieve a better solution but these conditions fail to achieve maximum image quality. Stochastic origin ensembles (SOE) imaging is a good candidate to address this problem as it uses Markov chain Monte Carlo to reach a stochastic steady-state solution that has image quality comparable to the best MLEM solution. The application of SOE to the DPI is presented in this work. SOE was originally applied in medical imaging applications with no mechanism to isolate spectral information based on location. This capability is critical for non-proliferation applications as complex radiation environments with multiple sources are often encountered. This dissertation extends the SOE algorithm to produce spatially dependent spectra and presents experimental result showing that the technique was effective for isolating a 4.1-kg mass of weapons grade plutonium (WGPu) when other neutron and gamma-ray sources were present. This work also demonstrates the DPI as an effective tool for localizing and characterizing highly enriched uranium (HEU). A series of experiments were performed with the DPI using a deuterium-deuterium (DD) and deuterium-tritium (DT) neutron generator, as well as AmLi, to interrogate a 13.7-kg sphere of HEU. In all cases, the neutrons and gamma rays produced from induced fission were successfully discriminated from the interrogating particles to localize the HEU. For characterization, the fast neutron and gamma-ray spectra were recorded from multiple HEU configurations with low-Z and high-Z moderation. Further characterization of the configurations used the measured neutron lifetime to show that the DPI can be used to infer multiplication.

Nuclear Weapons: Comprehensive Test Ban Treaty

DTIC Science & Technology

2006-07-10

continued...) The complex could contain explosions up to 500 pounds of explosive and associated plutonium. Another SCE, “ Unicorn ,” is to be conducted...scheduled for FY2006, as noted below. SCEs try to determine if radioactive decay of aged plutonium would degrade weapon performance. Several SCEs...Richardson called SCEs “a key part of our scientific program to provide new tools and data that assess age -related complications and maintain the reliability

Ceramics: Durability and radiation effects

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ewing, R.C.; Lutze, W.; Weber, W.J.

1996-05-01

At present, there are three seriously considered options for the disposition of excess weapons plutonium: (1) incorporation, partial burn-up and direct disposal of MOX-fuel; (2) vitrification with defense waste and disposal as glass {open_quotes}logs{close_quotes}; (3) deep borehole disposal. The first two options provide a safeguard due to the high activity of fission products in the irradiated fuel and the defense waste. The latter option has only been examined in a preliminary manner, and the exact form of the plutonium has not been identified. In this paper, we review the potential for the immobilization of plutonium in highly durable crystalline ceramicsmore » apatite, pyrochlore, zirconolite, monazite and zircon. Based on available data, we propose zircon as the preferred crystalline ceramic for the permanent disposition of excess weapons plutonium.« less

Excess Weapons Plutonium Immobilization in Russia

DOE Office of Scientific and Technical Information (OSTI.GOV)

Jardine, L.; Borisov, G.B.

2000-04-15

The joint goal of the Russian work is to establish a full-scale plutonium immobilization facility at a Russian industrial site by 2005. To achieve this requires that the necessary engineering and technical basis be developed in these Russian projects and the needed Russian approvals be obtained to conduct industrial-scale immobilization of plutonium-containing materials at a Russian industrial site by the 2005 date. This meeting and future work will provide the basis for joint decisions. Supporting R&D projects are being carried out at Russian Institutes that directly support the technical needs of Russian industrial sites to immobilize plutonium-containing materials. Special R&Dmore » on plutonium materials is also being carried out to support excess weapons disposition in Russia and the US, including nonproliferation studies of plutonium recovery from immobilization forms and accelerated radiation damage studies of the US-specified plutonium ceramic for immobilizing plutonium. This intriguing and extraordinary cooperation on certain aspects of the weapons plutonium problem is now progressing well and much work with plutonium has been completed in the past two years. Because much excellent and unique scientific and engineering technical work has now been completed in Russia in many aspects of plutonium immobilization, this meeting in St. Petersburg was both timely and necessary to summarize, review, and discuss these efforts among those who performed the actual work. The results of this meeting will help the US and Russia jointly define the future direction of the Russian plutonium immobilization program, and make it an even stronger and more integrated Russian program. The two objectives for the meeting were to: (1) Bring together the Russian organizations, experts, and managers performing the work into one place for four days to review and discuss their work with each other; and (2) Publish a meeting summary and a proceedings to compile reports of all the excellent Russian plutonium immobilization contract work. This proceedings document presents the wide extent of Russian immobilization activities, provides a reference for their work, and makes it available to others.« less

Preserving Plutonium-244 as a National Asset

DOE Office of Scientific and Technical Information (OSTI.GOV)

Patton, Bradley D; Alexander, Charles W; Benker, Dennis

Plutonium-244 (244 Pu) is an extremely rare and long-lived isotope of plutonium with a half-life of 80 million years. Measureable amounts of 244 Pu are found in neither reactor-grade nor weapons-grade plutonium. Production of this isotope requires a very high thermal flux to permit the two successive neutron captures that convert 242 Pu to 243 Pu to 244 Pu, particularly given the short (about 5 hour) half-life of 243 Pu. Such conditions simply do not exist in plutonium production processes. Therefore, 244 Pu is ideal for precise radiochemical analyses measuring plutonium material properties and isotopic concentrations in items containing plutonium.more » Isotope dilution mass spectrometry is about ten times more sensitive when using 244 Pu rather than 242 Pu for determining plutonium isotopic content. The isotope can also be irradiated in small quantities to produce superheavy elements. The majority of the existing global inventory of 244 Pu is contained in the outer housing of Mark-18A targets at the Savannah River Site (SRS). The total inventory is about 20 grams of 244 Pu in about 400 grams of plutonium distributed among the 65 targets. Currently, there are no specific plans to preserve these targets. Although the cost of separating and preserving this material would be considerable, it is trivial in comparison to new production costs. For all practical purposes, the material is irreplaceable, because new production would cost billions of dollars and require a series of irradiation and chemical separation cycles spanning up to 50 years. This paper will discuss a set of options for overcoming the significant challenges to preserve the 244 Pu as a National Asset: (1) the need to relocate the material from SRS in a timely manner, (2) the need to reduce the volume of material to the extent possible for storage, and (3) the need to establish an operational capability to enrich the 244 Pu in significant quantities. This paper suggests that if all the Mark-18A plutonium is separated, it would occupy a small volume and would be inexpensive to store while an enrichment capability is developed. Very small quantities could be enriched in existing mass separators to support critical needs.« less

Radioactive waste management and plutonium recovery within the context of the development of nuclear energy in Russia

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kushnikov, V.

1996-05-01

The Russian strategy for radioactive waste and plutonium management is based on the concept of the closed fuel cycle that has been adopted in Russia, and, to a great degree, falls under the jurisdiction of the existing Russian nuclear energy structures. From its very beginning, Russian atomic energy policy was based on finding the most effective method of developing the new fuel direction with the maximum possible utilization of the energy potential from the fission of heavy atoms and the achievement of fuel self-sufficiency through the recycling of secondary fuel. Although there can be no doubt about the importance ofmore » economic considerations (for the future), concerns for the safety of the environment are currently of the utmost importance. In this context, spent NPP fuel can be viewed as a waste to be buried only if there is persuasive evidence that such an approach is both economically and environmentally sound. The production of I GW of energy per year is accompanied by the accumulation of up to 800-1000 kg of highly radioactive fission products and approximately 250 kg of plutonium. Currently, spent fuel from the VVER 100 and the RBNK reactors contains approximately 25 tons of plutonium. There is an additional 30 tons of fuel-grade plutonium in the form of purified oxide, separated from spent fuels used in VVER440 reactors and other power production facilities, as well as approximately 100 tons of weapons-grade plutonium from dismantled warheads. The spent fuel accumulates significant amounts of small actinoids - neptunium americium, and curium. Science and technology have not yet found technical solutions for safe and secure burial of non-reprocessed spent fuel with such a broad range of products, which are typically highly radioactive and will continue to pose a threat for hundreds of thousands of years.« less

The Task of Detecting Illicit Nuclear Material: Status and Challenges

NASA Astrophysics Data System (ADS)

Kouzes, Richard

2006-04-01

In August 1994, police at the Munich airport intercepted a suitcase from Moscow with half a kilogram of nuclear-reactor fuel, of which 363 grams was weapons- grade plutonium. A few months later police seized 2.7 kilograms of highly enriched uranium from a former worker at a Russian nuclear institute and his accomplices in Prague. These are just two of 18 incidents involving the smuggling of weapons grade nuclear materials between 1993 and 2004 reported by the International Atomic Energy Agency. The consequences of a stolen or improvised nuclear device being exploded in a U.S. city would be world changing. The concern over the possibility of a nuclear weapon, or the material for a weapon or a radiological dispersion device, being smuggled across U.S. borders has led to the deployment of radiation detection equipment at the borders. Related efforts are occurring around the world. Radiation portal monitors are used as the main screening tool, supplemented by handheld detectors, personal radiation detectors, and x-ray imaging systems. Passive detection techniques combined with imaging, and possibly active techniques, are the current available tools for screening cargo for items of concern. There are a number of physics limitations to what is possible with each technology given the presence of naturally occurring radioactive materials, commercial sources, and medical radionuclides in the stream of commerce. There have been a number of lessons learned to date from the various efforts in the U.S. and internationally about the capability for interdicting illicit nuclear material.

The Manhattan Project; A very brief introduction to the physics of nuclear weapons

NASA Astrophysics Data System (ADS)

Reed, B. Cameron

2017-05-01

The development of nuclear weapons by the Manhattan Project during World War II was one of the most dramatic scientific/technological episodes in human history. This book, prepared by a recognized expert on the Manhattan Project, offers a concise survey of the essential physics concepts underlying fission weapons. The text describes the energetics and timescales of fast-neutron chain reactions, why only certain isotopes of uranium and plutonium are suitable for use in fission weapons, how critical mass and bomb yield can be estimated, how the efficiency of nuclear weapons can be enhanced, how the fissile forms of uranium and plutonium were obtained, some of the design details of the 'Little Boy' and 'Fat Man' bombs, and some of the thermal, shock, and radiation effects of nuclear weapons. Calculation exercises are provided, and a Bibliography lists authoritative print and online sources of information for readers who wish to pursue more detailed study of this fascinating topic.

Radioisotope contaminations from releases of the Tomsk-Seversk nuclear facility (Siberia, Russia).

PubMed

Gauthier-Lafaye, F; Pourcelot, L; Eikenberg, J; Beer, H; Le Roux, G; Rhikvanov, L P; Stille, P; Renaud, Ph; Mezhibor, A

2008-04-01

Soils have been sampled in the vicinity of the Tomsk-Seversk facility (Siberia, Russia) that allows us to measure radioactive contaminations due to atmospheric and aquatic releases. Indeed soils exhibit large inventories of man-made fission products including 137Cs (ranging from 33,000 to 68,500 Bq m(-2)) and actinides such as plutonium (i.e. 239+240Pu from 420 to 5900 Bq m(-2)) or 241Am (160-1220 Bq m(-2)). Among all sampling sites, the bank of the Romashka channel exhibits the highest radioisotope concentrations. At this site, some short half-life gamma emitters were detected as well indicating recent aquatic discharge in the channel. In comparison, soils that underwent atmospheric depositions like peat and forest soils exhibit lower activities of actinides and 137Cs. Soil activities are too high to be related solely to global fallout and thus the source of plutonium must be discharges from the Siberian Chemical Combine (SCC) plant. This is confirmed by plutonium isotopic ratios measured by ICP-MS; the low 241Pu/239Pu and 240Pu/239Pu atomic ratios with respect to global fallout ratio or civil nuclear fuel are consistent with weapons grade signatures. Up to now, the influence of Tomsk-Seversk plutonium discharges was speculated in the Ob River and its estuary. Isotopic data from the present study show that plutonium measured in SCC probably constitutes a significant source of plutonium in the aquatic environment, together with plutonium from global fallout and other contaminated sites including Tomsk, Mayak (Russia) and Semipalatinsk (Republic of Kazakhstan). It is estimated that the proportion of plutonium from SCC source can reach 45% for 239Pu and 60% for 241Pu in the sediments.

Plutonium isotopes and 241Am in the atmosphere of Lithuania: A comparison of different source terms

NASA Astrophysics Data System (ADS)

Lujanienė, G.; Valiulis, D.; Byčenkienė, S.; Šakalys, J.; Povinec, P. P.

2012-12-01

137Cs, 241Am and Pu isotopes collected in aerosol samples during 1994-2011 were analyzed with special emphasis on better understanding of Pu and Am behavior in the atmosphere. The results from long-term measurements of 240Pu/239Pu atom ratios showed a bimodal frequency distribution with median values of 0.195 and 0.253, indicating two main sources contributing to the Pu activities at the Vilnius sampling station. The low Pu atom ratio of 0.141 could be attributed to the weapon-grade plutonium derived from the nuclear weapon test sites. The frequency of air masses arriving from the North-West and North-East correlated with the Pu atom ratio indicating the input from the sources located in these regions (the Novaya Zemlya test site, Siberian nuclear plants), while no correlation with the Chernobyl region was observed. Measurements carried out during the Fukushima accident showed a negligible impact of this source with Pu activities by four orders of magnitude lower as compared to the Chernobyl accident. The activity concentration of actinides measured in the integrated sample collected in March-April, 2011 showed a small contribution of Pu with unusual activity and atom ratios indicating the presence of the spent fuel of different origin than that of the Chernobyl accident.

The 871 keV gamma ray from 17O and the identification of plutonium oxide

NASA Astrophysics Data System (ADS)

Peurrung, Anthony; Arthur, Richard; Elovich, Robert; Geelhood, Bruce; Kouzes, Richard; Pratt, Sharon; Scheele, Randy; Sell, Richard

2001-12-01

Disarmament agreements and discussions between the United States and the Russian Federation for reducing the number of stockpiled nuclear weapons require verification of the origin of materials as having come from disassembled weapons. This has resulted in the identification of measurable "attributes" that characterize such materials. It has been proposed that the 871 keV gamma ray of 17O can be observed as an indicator of the unexpected presence of plutonium oxide, as opposed to plutonium metal, in such materials. We have shown that the observation of the 871 keV gamma ray is not a specific indicator of the presence of the oxide, but rather indicates the presence of nitrogen.

DOUBLE TRACKS Test Site interim corrective action plan

DOE Office of Scientific and Technical Information (OSTI.GOV)

NONE

The DOUBLE TRACKS site is located on Range 71 north of the Nellis Air Force Range, northwest of the Nevada Test Site (NTS). DOUBLE TRACKS was the first of four experiments that constituted Operation ROLLER COASTER. On May 15, 1963, weapons-grade plutonium and depleted uranium were dispersed using 54 kilograms of trinitrotoluene (TNT) explosive. The explosion occurred in the open, 0.3 m above the steel plate. No fission yield was detected from the test, and the total amount of plutonium deposited on the ground surface was estimated to be between 980 and 1,600 grams. The test device was composed primarilymore » of uranium-238 and plutonium-239. The mass ratio of uranium to plutonium was 4.35. The objective of the corrective action is to reduce the potential risk to human health and the environment and to demonstrate technically viable and cost-effective excavation, transportation, and disposal. To achieve these objectives, Bechtel Nevada (BN) will remove soil with a total transuranic activity greater then 200 pCI/g, containerize the soil in ``supersacks,`` transport the filled ``supersacks`` to the NTS, and dispose of them in the Area 3 Radioactive Waste Management Site. During this interim corrective action, BN will also conduct a limited demonstration of an alternative method for excavation of radioactive near-surface soil contamination.« less

Risk Assessment for Emergency Planning Related to Nuclear Weapons Accidents

DTIC Science & Technology

1985-09-25

accidents is higher than many of the other accidents, several reviewers thought it appropriate to evaluate these accidents in more detail. In particular, it...consequences is presented in Table 2-5. The plutonium releases in the 1F-3F gram range are due to plutonium burning in Type A weapons, while the higher ...explosion given a tanker casualty varies from 0.05 (in harbor) to 0.16 (at pier) to 0.19 (at sea). Although these numbers are somewhat higher than the

68. INTERIOR SHOT OF ENTRANCE TO BUILDING 272 (PLUTONIUM STORAGE ...

Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

68. INTERIOR SHOT OF ENTRANCE TO BUILDING 272 (PLUTONIUM STORAGE BUILDING) LOOKING WEST. - Loring Air Force Base, Weapons Storage Area, Northeastern corner of base at northern end of Maine Road, Limestone, Aroostook County, ME

Control of a laser inertial confinement fusion-fission power plant

DOEpatents

Moses, Edward I.; Latkowski, Jeffery F.; Kramer, Kevin J.

2015-10-27

A laser inertial-confinement fusion-fission energy power plant is described. The fusion-fission hybrid system uses inertial confinement fusion to produce neutrons from a fusion reaction of deuterium and tritium. The fusion neutrons drive a sub-critical blanket of fissile or fertile fuel. A coolant circulated through the fuel extracts heat from the fuel that is used to generate electricity. The inertial confinement fusion reaction can be implemented using central hot spot or fast ignition fusion, and direct or indirect drive. The fusion neutrons result in ultra-deep burn-up of the fuel in the fission blanket, thus enabling the burning of nuclear waste. Fuels include depleted uranium, natural uranium, enriched uranium, spent nuclear fuel, thorium, and weapons grade plutonium. LIFE engines can meet worldwide electricity needs in a safe and sustainable manner, while drastically shrinking the highly undesirable stockpiles of depleted uranium, spent nuclear fuel and excess weapons materials.

Study of plutonium disposition using the GE Advanced Boiling Water Reactor (ABWR)

DOE Office of Scientific and Technical Information (OSTI.GOV)

NONE

1994-04-30

The end of the cold war and the resulting dismantlement of nuclear weapons has resulted in the need for the U.S. to disposition 50 to 100 metric tons of excess of plutonium in parallel with a similar program in Russia. A number of studies, including the recently released National Academy of Sciences (NAS) study, have recommended conversion of plutonium into spent nuclear fuel with its high radiation barrier as the best means of providing long-term diversion resistance to this material. The NAS study {open_quotes}Management and Disposition of Excess Weapons Plutonium{close_quotes} identified light water reactor spent fuel as the most readilymore » achievable and proven form for the disposition of excess weapons plutonium. The study also stressed the need for a U.S. disposition program which would enhance the prospects for a timely reciprocal program agreement with Russia. This summary provides the key findings of a GE study where plutonium is converted into Mixed Oxide (MOX) fuel and a 1350 MWe GE Advanced Boiling Water Reactor (ABWR) is utilized to convert the plutonium to spent fuel. The ABWR represents the integration of over 30 years of experience gained worldwide in the design, construction and operation of BWRs. It incorporates advanced features to enhance reliability and safety, minimize waste and reduce worker exposure. For example, the core is never uncovered nor is any operator action required for 72 hours after any design basis accident. Phase 1 of this study was documented in a GE report dated May 13, 1993. DOE`s Phase 1 evaluations cited the ABWR as a proven technical approach for the disposition of plutonium. This Phase 2 study addresses specific areas which the DOE authorized as appropriate for more in-depth evaluations. A separate report addresses the findings relative to the use of existing BWRs to achieve the same goal.« less

The nuclear arsenals and nuclear disarmament.

PubMed

Barnaby, F

1998-01-01

Current world stockpiles of nuclear weapons and the status of treaties for nuclear disarmament and the ultimate elimination of nuclear weapons are summarised. The need for including stockpiles of civil plutonium in a programme for ending production and disposing of fissile materials is emphasized, and the ultimate difficulty of disposing of the last few nuclear weapons discussed.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Adamov, E.O.; Lebedev, V.A.; Kuznetsov, Yu.N.

Zheleznogorsk is situated near the territorial center -- Krasnoyarsk on the Yenisei river. Mining and chemical complex is the main industrial enterprise of the town, which has been constructed for generation and used for isolation of weapons-grade plutonium. Heat supply to the chemical complex and town at the moment is largely provided by nuclear co-generation plant (NCGP) on the basis of the ADEh-2 dual-purpose reactor, generating 430 Gcal/h of heat and, partially, by coal backup peak-load boiler houses. NCGP also provides 73% of electric power consumed. In line with agreements between Russia and USA on strategic arms reduction and phasingmore » out of weapons-grade plutonium production, decommissioning of the ADEh-2 reactor by 2000 is planned. Thus, a problem arises relative to compensation for electric and thermal power generation for the needs of the town and industrial enterprises, which is now supplied by the reactor. A nuclear power plant constructed on the same site as a substituting power source should be considered as the most practical option. Basic requirements to the reactor of substituting nuclear power plant are as follows. It is to be a new generation reactor on the basis of verified technologies, having an operating prototype optimal for underground siting and permitting utmost utilization of the available mining workings and those being disengaged. NCGP with the reactor is to be constructed in the time period required and is to become competitive with other possible power sources. Analysis has shown that the VK-300 simplified vessel-type boiling reactor meets the requirements made in the maximum extent. Its design is based on the experience of the VK-50 reactor operation for a period of 30 years in Dimitrovgrad (Russia) and allows for experience in the development of the SBWR type reactors. The design of the reactor is discussed.« less

70. INTERIOR, BUILDING 272 (PLUTONIUM STORAGE BUILDING) LOOKING WEST INTO ...

Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

70. INTERIOR, BUILDING 272 (PLUTONIUM STORAGE BUILDING) LOOKING WEST INTO STORAGE AREA SHOWING THE FOUR STORAGE ROOM ENTRANCES. - Loring Air Force Base, Weapons Storage Area, Northeastern corner of base at northern end of Maine Road, Limestone, Aroostook County, ME

FMDP reactor alternative summary report. Volume 1 - existing LWR alternative

DOE Office of Scientific and Technical Information (OSTI.GOV)

Greene, S.R.; Bevard, B.B.

1996-10-07

Significant quantities of weapons-usable fissile materials [primarily plutonium and highly enriched uranium (HEU)] are becoming surplus to national defense needs in both the United States and Russia. These stocks of fissile materials pose significant dangers to national and international security. The dangers exist not only in the potential proliferation of nuclear weapons but also in the potential for environmental, safety, and health (ES&H) consequences if surplus fissile materials are not properly managed. This document summarizes the results of analysis concerned with existing light water reactor plutonium disposition alternatives.

Plutonium

NASA Astrophysics Data System (ADS)

Clark, David L.; Hecker, Siegfried S.; Jarvinen, Gordon D.; Neu, Mary P.

The element plutonium occupies a unique place in the history of chemistry, physics, technology, and international relations. After the initial discovery based on submicrogram amounts, it is now generated by transmutation of uranium in nuclear reactors on a large scale, and has been separated in ton quantities in large industrial facilities. The intense interest in plutonium resulted fromthe dual-use scenario of domestic power production and nuclear weapons - drawing energy from an atomic nucleus that can produce a factor of millions in energy output relative to chemical energy sources. Indeed, within 5 years of its original synthesis, the primary use of plutonium was for the release of nuclear energy in weapons of unprecedented power, and it seemed that the new element might lead the human race to the brink of self-annihilation. Instead, it has forced the human race to govern itself without resorting to nuclear war over the past 60 years. Plutonium evokes the entire gamut of human emotions, from good to evil, from hope to despair, from the salvation of humanity to its utter destruction. There is no other element in the periodic table that has had such a profound impact on the consciousness of mankind.

PLUTONIUM PROCESSING OPTIMIZATION IN SUPPORT OF THE MOX FUEL PROGRAM

DOE Office of Scientific and Technical Information (OSTI.GOV)

GRAY, DEVIN W.; COSTA, DAVID A.

2007-02-02

After Los Alamos National Laboratory (LANL) personnel completed polishing 125 Kg of plutonium as highly purified PuO{sub 2} from surplus nuclear weapons, Duke, COGEMA, Stone, and Webster (DCS) required as the next process stage, the validation and optimization of all phases of the plutonium polishing flow sheet. Personnel will develop the optimized parameters for use in the upcoming 330 kg production mission.

Plutonium Isotopes (239-241Pu) Dissolved in Pacific Ocean Waters Detected by Accelerator Mass Spectrometry: No Effects of the Fukushima Accident Observed.

PubMed

Hain, Karin; Faestermann, Thomas; Fimiani, Leticia; Golser, Robin; Gómez-Guzmán, José Manuel; Korschinek, Gunther; Kortmann, Florian; Lierse von Gostomski, Christoph; Ludwig, Peter; Steier, Peter; Tazoe, Hirofumi; Yamada, Masatoshi

2017-02-21

The concentration of plutonium (Pu) and the isotopic ratios of 240 Pu to 239 Pu and 241 Pu to 239 Pu were determined by accelerator mass spectrometry (AMS) in Pacific Ocean water samples (20 L each) collected in late 2012. The isotopic Pu ratios are important indicators of different contamination sources and were used to identify a possible release of Pu into the ocean by the Fukushima Daiichi Nuclear Power Plant (FDNPP) accident. In particular, 241 Pu is a well-suited indicator for a recent entry of Pu because 241 Pu from fallout of nuclear weapon testings has already significantly decayed. A total of 10 ocean water samples were prepared at the Radiochemie München of the TUM and analyzed at the Vienna Environmental Research Laboratory (VERA). Several samples showed a slightly elevated 240 Pu/ 239 Pu ratio of up to 0.22 ± 0.02 compared to global fallout ( 240 Pu/ 239 Pu = 0.180 ± 0.007), whereas all measured 241 Pu-to- 239 Pu ratios were consistent with nuclear weapon fallout ( 241 Pu/ 239 Pu < 2.4 × 10 -3 ), which means that no impact from the Fukushima accident was detected. From the average 241 Pu-to- 239 Pu ratio of 8 -2 +3 ×10 -4 at a sampling station located at a distance of 39.6 km to FDNPP, the 1-σ upper limit for the FDNPP contribution to the 239 Pu inventory in the water column was estimated to be 0.2%. Pu, with the signature of weapon-grade Pu was found in a single sample collected around 770 km off the west coast of the United States.

High-temperature Gas Reactor (HTGR)

NASA Astrophysics Data System (ADS)

Abedi, Sajad

2011-05-01

General Atomics (GA) has over 35 years experience in prismatic block High-temperature Gas Reactor (HTGR) technology design. During this period, the design has recently involved into a modular have been performed to demonstrate its versatility. This versatility is directly related to refractory TRISO coated - particle fuel that can contain any type of fuel. This paper summarized GA's fuel cycle studies individually and compares each based upon its cycle sustainability, proliferation-resistance capabilities, and other performance data against pressurized water reactor (PWR) fuel cycle data. Fuel cycle studies LEU-NV;commercial HEU-Th;commercial LEU-Th;weapons-grade plutonium consumption; and burning of LWR waste including plutonium and minor actinides in the MHR. results show that all commercial MHR options, with the exception of HEU-TH, are more sustainable than a PWR fuel cycle. With LEU-NV being the most sustainable commercial options. In addition, all commercial MHR options out perform the PWR with regards to its proliferation-resistance, with thorium fuel cycle having the best proliferation-resistance characteristics.

An analysis of the background and development of regulations for the air transport of plutonium in the USA

DOE Office of Scientific and Technical Information (OSTI.GOV)

McClure, J.D.; Luna, R.E.

1989-01-01

Several aspects of special packagings of plutonium for air transport should be recognized. The accident cases cited by Congressman Scheuer were incidents of local plutonium contamination in military aircraft accidents that had nuclear weapons on board. There is no disputing the occurrence of these military accidents but military weapon shipments were exempted from the provisions of the Scheuer amendment. There have been no recorded civilian aircraft crashes involving plutonium dispersal although there have been civilian aircraft crashes that were severe. Shortly after the introduction of the amendment by Mr. Scheuer on June 20, 1975, there was a serious aircraft crashmore » at JFK International. In his remarks to the House on July 24, 1975 Mr. Scheuer called attention to this event. The NRC originally opposed the provisions of the Scheuer amendment but with the passing of the amendment NRC compiled with its provisions. This led to the development of the plutonium air transport package PAT-1 in the US. The introduction of special rules for the air transport of plutonium into the US packaging regulations has been made them more severe than the provision of the international regulations, IAEA Safety Series 6. The IAEA is now discussing proposed regulations related to the air transport of plutonium. An additional legislative action was introduced the US in December 1987 which would require actual crash tests of packages intended for the air transport of plutonium, the Murkowski amendment. 13 refs.« less

Plutonium Immobilization Project System Design Description for Can Loading System

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kriikku, E.

2001-02-15

The purpose of this System Design Description (SDD) is to specify the system and component functions and requirements for the Can Loading System and provide a complete description of the system (design features, boundaries, and interfaces), principles of operation (including upsets and recovery), and the system maintenance approach. The Plutonium Immobilization Project (PIP) will immobilize up to 13 metric tons (MT) of U.S. surplus weapons usable plutonium materials.

Method of immobilizing weapons plutonium to provide a durable, disposable waste product

DOEpatents

Ewing, Rodney C.; Lutze, Werner; Weber, William J.

1996-01-01

A method of atomic scale fixation and immobilization of plutonium to provide a durable waste product. Plutonium is provided in the form of either PuO.sub.2 or Pu(NO.sub.3).sub.4 and is mixed with and SiO.sub.2. The resulting mixture is cold pressed and then heated under pressure to form (Zr,Pu)SiO.sub.4 as the waste product.

Transportation and storage of MOX and LEU assemblies at the Balakovo Nuclear Power Plant

DOT National Transportation Integrated Search

2001-01-01

The VVER-1000-type Balakovo Nuclear Power Plant has been chosen to dispose of the : plutonium created as part of Russian weapons program. The plutonium will be converted to mixed-oxide : (MOX), fabricated into assemblies and loaded into the reactor. ...

Dealing With Russian Tactical Nuclear Weapons

DTIC Science & Technology

2004-01-01

the plants, facilities, and equipment necessary to safely secure and store weapons pits (the plutonium “triggers” at the center of a thermonuclear ... bomb , and hence the most critical piece) proffered by either party. Furthermore, the statute requires the IAEA to establish control over the pits until

A Clear Success for International Transport of Plutonium and MOX Fuels

DOE Office of Scientific and Technical Information (OSTI.GOV)

Blachet, L.; Jacot, P.; Bariteau, J.P.

2006-07-01

An Agreement between the United States and Russia to eliminate 68 metric tons of surplus weapons-grade plutonium provided the basis for the United States government and its agency, the Department of Energy (DOE), to enter into contracts with industry leaders to fabricate mixed oxide (MOX) fuels (a blend of uranium oxide and plutonium oxide) for use in existing domestic commercial reactors. DOE contracted with Duke, COGEMA, Stone and Webster (DCS), a limited liability company comprised of Duke Energy, COGEMA Inc. and Stone and Webster to design a Mixed Oxide Fuel Fabrication Facility (MFFF) which would be built and operated atmore » the DOE Savannah River Site (SRS) near Aiken, South Carolina. During this same time frame, DOE commissioned fabrication and irradiation of lead test assemblies in one of the Mission Reactors to assist in obtaining NRC approval for batch implementation of MOX fuel prior to the operations phase of the MFFF facility. On February 2001, DOE directed DCS to initiate a pre-decisional investigation to determine means to obtain lead assemblies including all international options for manufacturing MOX fuels. This lead to implementation of the EUROFAB project and work was initiated in earnest on EUROFAB by DCS on November 7, 2003. (authors)« less

A Graphical Examination of Uranium and Plutonium Fissility

ERIC Educational Resources Information Center

Reed, B. Cameron

2008-01-01

The issue of why only particular isotopes of uranium and plutonium are suitable for use in nuclear weapons is analyzed with the aid of graphs and semiquantitative discussions of parameters such as excitation energies, fission barriers, reaction cross-sections, and the role of processes such as [alpha]-decay and spontaneous fission. The goal is to…

Introduction to Pits and Weapons Systems (U)

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kautz, D.

2012-07-02

A Nuclear Explosive Package includes the Primary, Secondary, Radiation Case and related components. This is the part of the weapon that produces nuclear yield and it converts mechanical energy into nuclear energy. The pit is composed of materials that allow mechanical energy to be converted to electromagnetic energy. Fabrication processes used are typical of any metal fabrication facility: casting, forming, machining and welding. Some of the materials used in pits include: Plutonium, Uranium, Stainless Steel, Beryllium, Titanium, and Aluminum. Gloveboxes are used for three reasons: (1) Protect workers and public from easily transported, finely divided plutonium oxides - (a) Plutoniummore » is very reactive and produces very fine particulate oxides, (b) While not the 'Most dangerous material in the world' of Manhattan Project lore, plutonium is hazardous to health of workers if not properly controlled; (2) Protect plutonium from reactive materials - (a) Plutonium is extremely reactive at ambient conditions with several components found in air: oxygen, water, hydrogen, (b) As with most reactive metals, reactions with these materials may be violent and difficult to control, (c) As with most fabricated metal products, corrosion may significantly affect the mechanical, chemical, and physical properties of the product; and (3) Provide shielding from radioactive decay products: {alpha}, {gamma}, and {eta} are commonly associated with plutonium decay, as well as highly radioactive materials such as {sup 241}Am and {sup 238}Pu.« less

Generalized Rate Theory for Void and Bubble Swelling and its Application to Delta-Plutonium

DOE Office of Scientific and Technical Information (OSTI.GOV)

Allen, P. G.; Wall, M. A.; Wolfer, W. G.

2016-10-04

A rate theory for void and bubble swelling is derived that allows both vacancies and self-interstitial atoms to be generated by thermal activation at all sinks. In addition, they can also be produced by displacement damage from external and internal radiation. This generalized rate theory (GRT) is applied to swelling of gallium-stabilized δ-plutonium in which α-decay causes the displacement damage. Since the helium atoms produced also become trapped in vacancies, a distinction is made between empty and occupied vacancies. The growth of helium bubbles observed by transmission electron microscopy (TEM) in weapons-grade and in material enriched with Pu238 is analyzed,more » using different values for the formation energy of self-interstitial atoms (SIA) and two different sets of relaxation volumes for the vacancy and for the SIA. One set allows preferential capture of SIA at dislocations, while the other set gives equal preference to both vacancy and SIA. It is found that the helium bubble diameters observed are in better agreement with GRT predictions if no preferential capture occurs at dislocations. Therefore, helium bubbles in δ-plutonium will not evolve into voids. The helium density within the bubbles remains sufficiently high to cause thermal emission of SIA. Based on a helium density between two to three helium atoms per vacant site, the sum of formation and migration energies must be around 2.0 eV for SIA in δ-plutonium.« less

Status of plutonium ceramic immobilization processes and immobilization forms

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ebbinghaus, B.B.; Van Konynenburg, R.A.; Vance, E.R.

1996-05-01

Immobilization in a ceramic followed by permanent emplacement in a repository or borehole is one of the alternatives currently being considered by the Fissile Materials Disposition Program for the ultimate disposal of excess weapons-grade plutonium. To make Pu recovery more difficult, radioactive cesium may also be incorporated into the immobilization form. Valuable data are already available for ceramics form R&D efforts to immobilize high-level and mixed wastes. Ceramics have a high capacity for actinides, cesium, and some neutron absorbers. A unique characteristic of ceramics is the existence of mineral analogues found in nature that have demonstrated actinide immobilization over geologicmore » time periods. The ceramic form currently being considered for plutonium disposition is a synthetic rock (SYNROC) material composed primarily of zirconolite (CaZrTi{sub 2}O{sub 7}), the desired actinide host phase, with lesser amounts of hollandite (BaAl{sub 2}Ti{sub 6}O{sub 16}) and rutile (TiO{sub 2}). Alternative actinide host phases are also being considered. These include pyrochlore (Gd{sub 2}Ti{sub 2}O{sub 7}), zircon (ZrSiO{sub 4}), and monazite (CePO{sub 4}), to name a few of the most promising. R&D activities to address important technical issues are discussed. Primarily these include moderate scale hot press fabrications with plutonium, direct loading of PuO{sub 2} powder, cold press and sinter fabrication methods, and immobilization form formulation issues.« less

Upward movement of plutonium to surface sediments during an 11-year field study.

PubMed

Kaplan, D I; Demirkanli, D I; Molz, F J; Beals, D M; Cadieux, J R; Halverson, J E

2010-05-01

An 11-year lysimeter study was established to monitor the movement of Pu through vadose zone sediments. Sediment Pu concentrations as a function of depth indicated that some Pu moved upward from the buried source material. Subsequent numerical modeling suggested that the upward movement was largely the result of invading grasses taking up the Pu and translocating it upward. The objective of this study was to determine if the Pu of surface sediments originated from atmosphere fallout or from the buried lysimeter source material (weapons-grade Pu), providing additional evidence that plants were involved in the upward migration of Pu. The (240)Pu/(239)Pu and (242)Pu/(239)Pu atomic fraction ratios of the lysimeter surface sediments, as determined by Thermal Ionization Mass Spectroscopy (TIMS), were 0.063 and 0.00045, respectively; consistent with the signatures of the weapons-grade Pu. Our numerical simulations indicate that because plants create a large water flux, small concentrations over multiple years may result in a measurable accumulation of Pu on the ground surface. These results may have implications on the conceptual model for calculating risk associated with long-term stewardship and monitored natural attenuation management of Pu contaminated subsurface and surface sediments. Copyright (c) 2010 Elsevier Ltd. All rights reserved.

A perspective on the proliferation risks of plutonium mines

DOE Office of Scientific and Technical Information (OSTI.GOV)

Lyman, E.S.

1996-05-01

The program of geologic disposal of spent fuel and other plutonium-containing materials is increasingly becoming the target of criticism by individuals who argue that in the future, repositories may become low-cost sources of fissile material for nuclear weapons. This paper attempts to outline a consistent framework for analyzing the proliferation risks of these so-called {open_quotes}plutonium mines{close_quotes} and putting them into perspective. First, it is emphasized that the attractiveness of plutonium in a repository as a source of weapons material depends on its accessibility relative to other sources of fissile material. Then, the notion of a {open_quotes}material production standard{close_quotes} (MPS) ismore » proposed: namely, that the proliferation risks posed by geologic disposal will be acceptable if one can demonstrate, under a number of reasonable scenarios, that the recovery of plutonium from a repository is likely to be as difficult as new production of fissile material. A preliminary analysis suggests that the range of circumstances under which current mined repository concepts would fail to meet this standard is fairly narrow. Nevertheless, a broad application of the MPS may impose severe restrictions on repository design. In this context, the relationship of repository design parameters to easy of recovery is discussed.« less

Multiplication and Presence of Shielding Material from Time-Correlated Pulse-Height Measurements of Subcritical Plutonium Assemblies

DOE PAGES

Monterial, Mateusz; Marleau, Peter; Paff, Marc; ...

2017-01-20

Here, we present the results from the first measurements of the Time-Correlated Pulse-Height (TCPH) distributions from 4.5 kg sphere of α-phase weapons-grade plutonium metal in five configurations: bare, reflected by 1.27 cm and 2.54 cm of tungsten, and 2.54 cm and 7.62 cm of polyethylene. A new method for characterizing source multiplication and shielding configuration is also demonstrated. The method relies on solving for the underlying fission chain timing distribution that drives the spreading of the measured TCPH distribution. We found that a gamma distribution fits the fission chain timing distribution well and that the fit parameters correlate with bothmore » multiplication (rate parameter) and shielding material types (shape parameter). The source-to-detector distance was another free parameter that we were able to optimize, and proved to be the most well constrained parameter. MCNPX-PoliMi simulations were used to complement the measurements and help illustrate trends in these parameters and their relation to multiplication and the amount and type of material coupled to the subcritical assembly.« less

Multiplication and Presence of Shielding Material from Time-Correlated Pulse-Height Measurements of Subcritical Plutonium Assemblies

NASA Astrophysics Data System (ADS)

Monterial, Mateusz; Marleau, Peter; Paff, Marc; Clarke, Shaun; Pozzi, Sara

2017-04-01

We present the results from the first measurements of the Time-Correlated Pulse-Height (TCPH) distributions from 4.5 kg sphere of α-phase weapons-grade plutonium metal in five configurations: bare, reflected by 1.27 cm and 2.54 cm of tungsten, and 2.54 cm and 7.62 cm of polyethylene. A new method for characterizing source multiplication and shielding configuration is also demonstrated. The method relies on solving for the underlying fission chain timing distribution that drives the spreading of the measured TCPH distribution. We found that a gamma distribution fits the fission chain timing distribution well and that the fit parameters correlate with both multiplication (rate parameter) and shielding material types (shape parameter). The source-to-detector distance was another free parameter that we were able to optimize, and proved to be the most well constrained parameter. MCNPX-PoliMi simulations were used to complement the measurements and help illustrate trends in these parameters and their relation to multiplication and the amount and type of material coupled to the subcritical assembly.

Sources of plutonium in the atmosphere and stratosphere-troposphere mixing

PubMed Central

Hirose, Katsumi; Povinec, Pavel P.

2015-01-01

Plutonium isotopes have primarily been injected to the stratosphere by the atmospheric nuclear weapon tests and the burn-up of the SNAP-9A satellite. Here we show by using published data that the stratospheric plutonium exponentially decreased with apparent residence time of 1.5 ± 0.5 years, and that the temporal variations of plutonium in surface air followed the stratospheric trends until the early 1980s. In the 2000s, plutonium and its isotope ratios in the atmosphere varied dynamically, and sporadic high concentrations of 239,240Pu reported for the lower stratospheric and upper tropospheric aerosols may be due to environmental events such as the global dust outbreaks and biomass burning. PMID:26508010

Selection of Russian Plutonium Beryllium Sources for Inclusion in the Nuclear Mateirals Information Program Archive

DOE Office of Scientific and Technical Information (OSTI.GOV)

Narlesky, Joshua E; Padilla, Dennis D; Watts, Joe

2009-01-01

Throughout the 1960s and 1970s, the former Soviet Union produced and exported Plutonium-Beryllium (PuBe) neutron sources to various Eastern European countries. The Russian sources consist of an intermetallic compound of plutonium and beryllium encapsulated in an inner welded, sealed capsule and consisting of a body and one or more covers. The amount of plutonium in the sources ranges from 0.002 g up to 15 g. A portion of the sources was originally exported to East Germany. A portion of these sources were acquired by Los Alamos National Laboratory (LANL) in the late 1990s for destruction in the Offsite Source Recoverymore » Program. When the OSRP was canceled, the remaining 88 PuBe neutron sources were packaged and stored in a 55-gal drum at T A-55. This storage configuration is no longer acceptable for PuBe sources, and the sources must either be repackaged or disposed of. Repackaging would place the sources into Hagan container, and depending on the dose rates, some sources may be packaged individually increasing the footprint and cost of storage. In addition, each source will be subject to leak-checking every six months. Leaks have already been detected in some of the sources, and due to the age of these sources, it is likely that additional leaks may be detected over time, which will increase the overall complexity of handling and storage. Therefore, it was decided that the sources would be disposed of at the Waste Isolation Pilot Plant (WIPP) due to the cost and labor associated with continued storage at TA-55. However, the plutonium in the sources is of Russian origin and needs to be preserved for research purposes. Therefore, it is important that a representative sample of the sources retained and archived for future studies. This report describes the criteria used to obtain a representative sample of the sources. Nine Russian PuBe neutron sources have been selected out of a collection of 77 sources for inclusion in the NMIP archive. Selection criteria were developed so that the largest sources that are representative of the collection are included. One representative source was chosen for every 20 sources in the collection, and effort was made to preserve sources unique to the collection. In total, four representative sources and five unique sources were selected for the archive. The archive samples contain 40 grams of plutonium with an isotopic composition similar to that of weapon grade material and three grams of plutonium with an isotopic composition similar to that of reactor grade plutonium.« less

Assessment of plutonium in the Savannah River Site environment. Revision 1

DOE Office of Scientific and Technical Information (OSTI.GOV)

Carlton, W.H.; Evans, A.G.; Geary, L.A.

1992-12-31

Plutonium in the Savannah River Site Environment is published as a part of the Radiological Assessment Program (RAP). It is the fifth in a series of eight documents on individual radioisotopes released to the environment as a result of Savannah River Site (SRS) operations. These are living documents, each to be revised and updated on a two-year schedule. This document describes the sources of plutonium in the environment, its release from SRS, environmental transport and ecological concentration of plutonium, and the radiological impact of SRS releases to the environment. Plutonium exists in the environment as a result of above-ground nuclearmore » weapons tests, the Chernobyl accident, the destruction of satellite SNAP 9-A, plane crashes involving nuclear weapons, and small releases from reactors and reprocessing plants. Plutonium has been produced at SRS during the operation of five production reactors and released in small quantities during the processing of fuel and targets in chemical separations facilities. Approximately 0.6 Ci of plutonium was released into streams and about 12 Ci was released to seepage basins, where it was tightly bound by clay in the soil. A smaller quantity, about 3.8 Ci, was released to the atmosphere. Virtually all releases have occurred in F- and H-Area separation facilities. Plutonium concentration and transport mechanisms for the atmosphere, surface water, and ground water releases have been extensively studied by Savannah River Technology Center (SRTC) and ecological mechanisms have been studied by Savannah River Ecology Laboratory (SREL). The overall radiological impact of SRS releases to the offsite maximum individual can be characterized by a total dose of 15 mrem (atmospheric) and 0.18 mrem (liquid), compared with the dose of 12,960 mrem from non-SRS sources during the same period of time (1954--1989). Plutonium releases from SRS facilities have resulted in a negligible impact to the environment and the population it supports.« less

Minimizing Glovebox Glove Breaches, Part III: Deriving Service Lifetimes

DOE Office of Scientific and Technical Information (OSTI.GOV)

Cournoyer, M.E.; Wilson, K.V.; Maestas, M.M.

At the Los Alamos Plutonium Facility, various isotopes of plutonium along with other actinides are handled in a glove box environment. Weapons-grade plutonium consists mainly in Pu-239. Pu-238 is another isotope used for heat sources. The Pu-238 is more aggressive regarding gloves due to its higher alpha-emitting characteristic ({approx}300 times more active than Pu-239), which modifies the change-out intervals for gloves. Optimization of the change-out intervals for gloves is fundamental since Nuclear Materials Technology (NMT) Division generates approximately 4 m{sup 3}/yr of TRU waste from the disposal of glovebox gloves. To reduce the number of glovebox glove failures, the NMTmore » Division pro-actively investigates processes and procedures that minimize glove failures. Aging studies have been conducted that correlate changes in mechanical (physical) properties with degradation chemistry. This present work derives glovebox glove change intervals based on mechanical data of thermally aged Hypalon{sup R}, and Butasol{sup R} glove samples. Information from this study represent an important baseline in gauging the acceptable standards for polymeric gloves used in a laboratory glovebox environment and will be used later to account for possible presence of dose-rate or synergistic effects in 'combined-environment'. In addition, excursions of contaminants into the operator's breathing zone and excess exposure to the radiological sources associated with unplanned breaches in the glovebox are reduced. (authors)« less

DOE Office of Scientific and Technical Information (OSTI.GOV)

CHARBONEAU, S.L.

The Plutonium Finishing Plant (PFP) consists of a number of process and support buildings for handling plutonium. Building construction began in the late 1940's to meet national priorities and became operational in 1950 producing refined plutonium salts and metal for the United States nuclear weapons program. The primary mission of the PFP was to provide plutonium used as special nuclear material for fabrication into a nuclear device for the war effort. Subsequent to the end of World War II, the PFP's mission expanded to support the Cold War effort through plutonium production during the nuclear arms race. PFP has nowmore » completed its mission and is fully engaged in deactivation, decontamination and decommissioning (D&D). At this time the PFP buildings are planned to be reduced to ground level (slab-on-grade) and the site remediated to satisfy national, Department of Energy (DOE) and Washington state requirements. The D&D of a highly contaminated plutonium processing facility presents a plethora of challenges. PFP personnel approached the D&D mission with a can-do attitude. They went into D&D knowing they were facing a lot of challenges and unknowns. There were concerns about the configuration control associated with drawings of these old process facilities. There were unknowns regarding the location of electrical lines and process piping containing chemical residues such as strong acids and caustics. The gloveboxes were highly contaminated with plutonium and chemical residues. Most of the glovebox windows were opaque with splashed process chemicals that coated the windows or etched them, reducing visibility to near zero. Visibility into the glovebox was a serious worker concern. Additionally, all the gloves in the gloveboxes were degraded and unusable. Replacing gloves in gloveboxes was necessary to even begin glovebox cleanout. The sheer volume of breathing air needed was also an issue. These and other challenges and PFP's approach to overcome these challengers are described. Many of the challenges to the D&D work at PFP were met with innovative approaches based on new science and/or technology and many were also based on the creativity and motivation of the work force personnel.« less

DOE Office of Scientific and Technical Information (OSTI.GOV)

Charboneau, S.; Klos, B.; Heineman, R.

The Plutonium Finishing Plant (PFP) consists of a number of process and support buildings for handling plutonium. Building construction began in the late 1940's to meet national priorities and became operational in 1950 producing refined plutonium salts and metal for the United States nuclear weapons program The primary mission of the PFP was to provide plutonium used as special nuclear material for fabrication into a nuclear device for the war effort. Subsequent to the end of World War II, the PFP's mission expanded to support the Cold War effort through plutonium production during the nuclear arms race. PFP has nowmore » completed its mission and is fully engaged in deactivation, decontamination and decommissioning (D and D). At this time the PFP buildings are planned to be reduced to ground level (slab-on-grade) and the site remediated to satisfy national, Department of Energy (DOE) and Washington state requirements. The D and D of a highly contaminated plutonium processing facility presents a plethora of challenges. PFP personnel approached the D and D mission with a can-do attitude. They went into D and D knowing they were facing a lot of challenges and unknowns. There were concerns about the configuration control associated with drawings of these old process facilities. There were unknowns regarding the location of electrical lines and the condition and contents of process piping containing chemical residues such as strong acids and caustics. The gloveboxes were highly contaminated with plutonium and chemical residues. Most of the glovebox windows were opaque with splashed process chemicals that coated the windows or etched them, reducing visibility to near zero. Visibility into the glovebox was a serious worker concern. Additionally, all the gloves in the gloveboxes were degraded and unusable. Replacing gloves in gloveboxes was necessary to even begin glovebox clean-out. The sheer volume of breathing air needed was also an issue. These and other challenges and PFP's approach to overcome these challengers are described. Many of the challenges to the D and D work at PFP were met with innovative approaches based on new science and/or technology and many were also based on the creativity and motivation of the work force personnel. (authors)« less

Physics overview of AVLIS

NASA Astrophysics Data System (ADS)

Solarz, R. W.

1985-02-01

Atomic vapor laster isotope separation (AVLIS) represents the largest-scale potential application of tunable lasers that has received serious attention. The underlying physical principles were identified and optimized, the major technology components were developed, and the integrated enrichment performance of the process was tested. The central physical processes are outlined, progress to date on the technology elements is reviewed, and scaling laws are fomulated. Two primary applications are the production of light-water reactor fuel and the conversion of fuel-grade plutonium to weapons-grade material. A variety of applications exist that all potentially use a common base of AVLIS technology. These include missions such as the enrichment of mercury isotopes to improve fluorescent lamp efficiency, the enrichment of iodine isotopes for medical isotope use, and the cleanup of strontium from defense waste for recovering strontium isotopes for radiothermal mechanical generators. The ability to radidly assess the economic and technical feasibility of each mission is derived from the general applicability of AVLIS physics and AVLIS technology.

Mortality among workers with chronic radiation sickness

DOE Office of Scientific and Technical Information (OSTI.GOV)

Shilnikova, N.S.; Koshurnikova, N.A.; Bolotnikova, M.G.

1996-07-01

This study is based on a registry containing medical and dosimetric data of the employees who began working at different plants of the Mayak nuclear complex between 1948 and 1958 who developed chronic radiation sickness. Mayak is the first nuclear weapons plutonium production enterprise built in Russia and includes nuclear reactors, a radiochemical plant for plutonium separation, and a plutonium production enterprise built in Russia and includes nuclear reactors, a radiochemical plant for plutonium separation, and a plutonium production plant.Workers whose employment began between 1948 and 1958 exhibited a 6-28% incidence of chronic radiation sickness at the different facilities. Theremore » were no cases of chronic radiation sickness among those who began working after 1958. Data on doses of external whole-body gamma-irradiation and mortality in workers with chronic radiation sickness are presented. 6 refs., 5 tabs.« less

The UK Government's global partnership programme - Its achievements over the past five years and challenges ahead

DOE Office of Scientific and Technical Information (OSTI.GOV)

Heyes, Alan

2007-07-01

Through the Global Partnership the UK continues to make a significant contribution to improve national and global security. Over the past year the UK has continued to implement a wide range of projects across the breadth of its Global Partnership Programme. As well as ensuring the Programme is robust and capable of dealing with new challenges, the UK has cooperated with other donor countries to help them progress projects associated with submarine dismantling, scientist redirection, enhancing nuclear security and Chemical Weapons Destruction. The Global Partnership, although only five years old, has already achieved a great deal. Some 23 states, plusmore » the European Union, are now working closer together under the Global Partnership, and collectively have enhanced global regional and national security by reducing the availability of Weapons of Mass Destruction (WMD) materials and expertise to both states of concern and terrorists. Considerable progress has already been made in, for example: - Improving the security of fissile materials, dangerous biological agents and chemical weapons stocks; - Reducing the number of sites containing radioactive materials; - Working towards closure of reactors still producing weapon-grade plutonium; - Improving nuclear safety to reduce the risks of further, Chernobyl style accidents; - Constructing facilities for destroying Chemical Weapons stocks, and starting actual destruction; - Providing sustainable employment for former WMD scientists to reduce the risk that their expertise will be misused by states or terrorists. By contributing to many of these activities, the UK has helped to make the world safer. This paper reports on the UK's practical and sustainable contribution to the Global Partnership and identifies a number of challenges that remain if it is to have a wider impact on reducing the threats from WMD material. (authors)« less

Detecting special nuclear material using a neutron time projection chamber

NASA Astrophysics Data System (ADS)

Carosi, G.; Bernstein, A.; Bowden, N.; Burke, J.; Carter, D.; Foxe, M.; Heffner, M.; Jovanovic, I.; Mintz, J.; O'Malley, P.

2010-02-01

Time projection chambers are 3-dimensional charged particle cameras based on drifting ionization tracks at a known velocity onto an electronic readout plane. These instruments are capable of detecting fast neutrons which are unique signatures of special nuclear material with low natural background rates. Here we describe a neutron Time Projection Chamber (nTPC) developed at Lawrence Livermore National Laboratory (LLNL) which has demonstrated directional sensitivity to fission neutrons along with high rejection of background gamma-ray and electron events. Using a combination hydrogen/methane drift gas at several atmospheres we've demonstrated the ability to point to a Cf-252 source simulating 6kg of weapons grade plutonium at 10's of meters with one hour integration time. Plans for future field deployable devices will also be outlined. )

KSC-97PC1537

NASA Image and Video Library

1997-10-10

At Launch Complex 40 on Cape Canaveral Air Station, workers are installing three Radioisotope Thermoelectric Generators (RTGs) on the Cassini spacecraft. RTGs are lightweight, compact spacecraft electrical power systems that have flown successfully on 23 previous U.S. missions over the past 37 years. These generators produce power by converting heat into electrical energy; the heat is provided by the natural radioactive decay of plutonium-238 dioxide, a non-weapons-grade material. RTGs enable spacecraft to operate at significant distances from the Sun where solar power systems would not be feasible. Cassini will travel two billion miles to reach Saturn and another 1.1 billion miles while in orbit around Saturn. Cassini is undergoing final preparations for liftoff on a Titan IVB/Centaur launch vehicle, with the launch window opening at 4:55 a.m. EDT, Oct. 13

KSC-97PC1535

NASA Image and Video Library

1997-10-10

At Launch Complex 40 on Cape Canaveral Air Station, workers are installing three Radioisotope Thermoelectric Generators (RTGs) on the Cassini spacecraft. RTGs are lightweight, compact spacecraft electrical power systems that have flown successfully on 23 previous U.S. missions over the past 37 years. These generators produce power by converting heat into electrical energy; the heat is provided by the natural radioactive decay of plutonium-238 dioxide, a non-weapons-grade material. RTGs enable spacecraft to operate at significant distances from the Sun where solar power systems would not be feasible. Cassini will travel two billion miles to reach Saturn and another 1.1 billion miles while in orbit around Saturn. Cassini is undergoing final preparations for liftoff on a Titan IVB/Centaur launch vehicle, with the launch window opening at 4:55 a.m. EDT, Oct. 13

KSC-97PC1533

NASA Image and Video Library

1997-10-10

At Launch Complex 40 on Cape Canaveral Air Station, workers are installing three Radioisotope Thermoelectric Generators (RTGs) on the Cassini spacecraft. RTGs are lightweight, compact spacecraft electrical power systems that have flown successfully on 23 previous U.S. missions over the past 37 years. These generators produce power by converting heat into electrical energy; the heat is provided by the natural radioactive decay of plutonium-238 dioxide, a non-weapons-grade material. RTGs enable spacecraft to operate at significant distances from the Sun where solar power systems would not be feasible. Cassini will travel two billion miles to reach Saturn and another 1.1 billion miles while in orbit around Saturn. Cassini is undergoing final preparations for liftoff on a Titan IVB/Centaur launch vehicle, with the launch window opening at 4:55 a.m. EDT, Oct. 13

KSC-97PC1538

NASA Image and Video Library

1997-10-10

At Launch Complex 40 on Cape Canaveral Air Station, workers are installing three Radioisotope Thermoelectric Generators (RTGs) on the Cassini spacecraft. RTGs are lightweight, compact spacecraft electrical power systems that have flown successfully on 23 previous U.S. missions over the past 37 years. These generators produce power by converting heat into electrical energy; the heat is provided by the natural radioactive decay of plutonium-238 dioxide, a non-weapons-grade material. RTGs enable spacecraft to operate at significant distances from the Sun where solar power systems would not be feasible. Cassini will travel two billion miles to reach Saturn and another 1.1 billion miles while in orbit around Saturn. Cassini is undergoing final preparations for liftoff on a Titan IVB/Centaur launch vehicle, with the launch window opening at 4:55 a.m. EDT, Oct. 13

Proliferation resistance of small modular reactors fuels

DOE Office of Scientific and Technical Information (OSTI.GOV)

Polidoro, F.; Parozzi, F.; Fassnacht, F.

2013-07-01

In this paper the proliferation resistance of different types of Small Modular Reactors (SMRs) has been examined and classified with criteria available in the literature. In the first part of the study, the level of proliferation attractiveness of traditional low-enriched UO{sub 2} and MOX fuels to be used in SMRs based on pressurized water technology has been analyzed. On the basis of numerical simulations both cores show significant proliferation risks. Although the MOX core is less proliferation prone in comparison to the UO{sub 2} core, it still can be highly attractive for diversion or undeclared production of nuclear material. Inmore » the second part of the paper, calculations to assess the proliferation attractiveness of fuel in typical small sodium cooled fast reactor show that proliferation risks from spent fuel cannot be neglected. The core contains a highly attractive plutonium composition during the whole life cycle. Despite some aspects of the design like the sealed core that enables easy detection of unauthorized withdrawal of fissile material and enhances proliferation resistance, in case of open Non-Proliferation Treaty break-out, weapon-grade plutonium in sufficient quantities could be extracted from the reactor core.« less

Chemical interaction matrix between reagents in a Purex based process

DOE Office of Scientific and Technical Information (OSTI.GOV)

Brahman, R.K.; Hennessy, W.P.; Paviet-Hartmann, P.

2008-07-01

The United States Department of Energy (DOE) is the responsible entity for the disposal of the United States excess weapons grade plutonium. DOE selected a PUREX-based process to convert plutonium to low-enriched mixed oxide fuel for use in commercial nuclear power plants. To initiate this process in the United States, a Mixed Oxide (MOX) Fuel Fabrication Facility (MFFF) is under construction and will be operated by Shaw AREVA MOX Services at the Savannah River Site. This facility will be licensed and regulated by the U.S. Nuclear Regulatory Commission (NRC). A PUREX process, similar to the one used at La Hague,more » France, will purify plutonium feedstock through solvent extraction. MFFF employs two major process operations to manufacture MOX fuel assemblies: (1) the Aqueous Polishing (AP) process to remove gallium and other impurities from plutonium feedstock and (2) the MOX fuel fabrication process (MP), which processes the oxides into pellets and manufactures the MOX fuel assemblies. The AP process consists of three major steps, dissolution, purification, and conversion, and is the center of the primary chemical processing. A study of process hazards controls has been initiated that will provide knowledge and protection against the chemical risks associated from mixing of reagents over the life time of the process. This paper presents a comprehensive chemical interaction matrix evaluation for the reagents used in the PUREX-based process. Chemical interaction matrix supplements the process conditions by providing a checklist of any potential inadvertent chemical reactions that may take place. It also identifies the chemical compatibility/incompatibility of the reagents if mixed by failure of operations or equipment within the process itself or mixed inadvertently by a technician in the laboratories. (aut0010ho.« less

Scope and verification of a Fissile Material (Cutoff) Treaty

DOE PAGES

von Hippel, Frank N.

2014-01-01

A Fissile Material Cutoff Treaty (FMCT) would ban the production of fissile material – in practice highly-enriched uranium and separated plutonium – for weapons. It has been supported by strong majorities in the United Nations. After it comes into force, newly produced fissile materials could only be produced under international – most likely International Atomic Energy Agency – monitoring. There are many non-weapon states that argue the treaty should also place under safeguards pre-existing stocks of fissile material in civilian use or declared excess for weapons so as to make nuclear-weapons reductions irreversible. Our paper discusses the scope of themore » FMCT, the ability to detect clandestine production and verification challenges in the nuclear-weapons states.« less

In search of plutonium: A nonproliferation journey

NASA Astrophysics Data System (ADS)

Hecker, Siegfried

2010-02-01

In February 1992, I landed in the formerly secret city of Sarov, the Russian Los Alamos, followed a few days later by a visit to Snezhinsk, their Livermore. The briefings we received of the Russian nuclear weapons program and tours of their plutonium, reactor, explosives, and laser facilities were mind boggling considering the Soviet Union was dissolved only two months earlier. This visit began a 17-year, 41 journey relationship with the Russian nuclear complex dedicated to working with them in partnership to protect and safeguard their weapons and fissile materials, while addressing the plight of their scientists and engineers. In the process, we solved a forty-year disagreement about the plutonium-gallium phase diagram and began a series of fundamental plutonium science workshops that are now in their tenth year. At the Yonbyon reprocessing facility in January 2004, my North Korean hosts had hoped to convince me that they have a nuclear deterrent. When I expressed skepticism, they asked if I wanted to see their ``product.'' I asked if they meant the plutonium; they replied, ``Well, yes.'' Thus, I wound up holding 200 grams of North Korean plutonium (in a sealed glass jar) to make sure it was heavy and warm. So began the first of my six journeys to North Korea to provide technical input to the continuing North Korean nuclear puzzle. In Trombay and Kalpakkam a few years later I visited the Indian nuclear research centers to try to understand how India's ambitious plans for nuclear power expansion can be accomplished safely and securely. I will describe these and other attempts to deal with the nonproliferation legacy of the cold war and the new challenges ahead. )

Source Book on Plutonium and Its Decontamination

DTIC Science & Technology

1973-09-24

Energy Commisjsion Policy The AEC is the foremoacst regulator of the use of radioactive materials in this country. It derives this power from the...Congress and furthers Its responsibilities in two ways; first, through its licensin~g power and second, by regulation of the activities of its contractors...biological hazard. Plutonium- 239 is of interest because of its abundance in weapons and Pu-238 because of its use in power sources. Half lives for the two

Plutonium release from Fukushima Daiichi fosters the need for more detailed investigations

NASA Astrophysics Data System (ADS)

Schneider, Stephanie; Walther, Clemens; Bister, Stefan; Schauer, Viktoria; Christl, Marcus; Synal, Hans-Arno; Shozugawa, Katsumi; Steinhauser, Georg

2013-10-01

The contamination of Japan after the Fukushima accident has been investigated mainly for volatile fission products, but only sparsely for actinides such as plutonium. Only small releases of actinides were estimated in Fukushima. Plutonium is still omnipresent in the environment from previous atmospheric nuclear weapons tests. We investigated soil and plants sampled at different hot spots in Japan, searching for reactor-borne plutonium using its isotopic ratio 240Pu/239Pu. By using accelerator mass spectrometry, we clearly demonstrated the release of Pu from the Fukushima Daiichi power plant: While most samples contained only the radionuclide signature of fallout plutonium, there is at least one vegetation sample whose isotope ratio (0.381 +/- 0.046) evidences that the Pu originates from a nuclear reactor (239+240Pu activity concentration 0.49 Bq/kg). Plutonium content and isotope ratios differ considerably even for very close sampling locations, e.g. the soil and the plants growing on it. This strong localization indicates a particulate Pu release, which is of high radiological risk if incorporated.

Plutonium release from the 903 pad at Rocky Flats.

PubMed

Mongan, T R; Ripple, S R; Winges, K D

1996-10-01

The Colorado Department of Public Health and Environment (CDH) sponsored a study to reconstruct contaminant doses to the public from operations at the Rocky Flats nuclear weapons plant. This analysis of the accidental release of plutonium from the area known as the 903 Pad is part of the CDH study. In the 1950's and 1960's, 55-gallon drums of waste oil contaminated with plutonium, and uranium were stored outdoors at the 903 Pad. The drums corroded, leaking contaminated oil onto soil subsequently carried off-site by the wind. The plutonium release is estimated using environmental data from the 1960's and 1970's and an atmospheric transport model for fugitive dust. The best estimate of total plutonium release to areas beyond plant-owned property is about 0.26 TBq (7 Ci). Off-site airborne concentrations and deposition of plutonium are estimated for dose calculation purposes. The best estimate of the highest predicted off-site effective dose is approximately 72 microSv (7.2 mrem).

Nuclear energy and security

DOE Office of Scientific and Technical Information (OSTI.GOV)

BLEJWAS,THOMAS E.; SANDERS,THOMAS L.; EAGAN,ROBERT J.

2000-01-01

Nuclear power is an important and, the authors believe, essential component of a secure nuclear future. Although nuclear fuel cycles create materials that have some potential for use in nuclear weapons, with appropriate fuel cycles, nuclear power could reduce rather than increase real proliferation risk worldwide. Future fuel cycles could be designed to avoid plutonium production, generate minimal amounts of plutonium in proliferation-resistant amounts or configurations, and/or transparently and efficiently consume plutonium already created. Furthermore, a strong and viable US nuclear infrastructure, of which nuclear power is a large element, is essential if the US is to maintain a leadershipmore » or even participatory role in defining the global nuclear infrastructure and controlling the proliferation of nuclear weapons. By focusing on new fuel cycles and new reactor technologies, it is possible to advantageously burn and reduce nuclear materials that could be used for nuclear weapons rather than increase and/or dispose of these materials. Thus, the authors suggest that planners for a secure nuclear future use technology to design an ideal future. In this future, nuclear power creates large amounts of virtually atmospherically clean energy while significantly lowering the threat of proliferation through the thoughtful use, physical security, and agreed-upon transparency of nuclear materials. The authors must develop options for policy makers that bring them as close as practical to this ideal. Just as Atoms for Peace became the ideal for the first nuclear century, they see a potential nuclear future that contributes significantly to power for peace and prosperity.« less

JOWOG 22/2 - Actinide Chemical Technology (July 9-13, 2012)

DOE Office of Scientific and Technical Information (OSTI.GOV)

Jackson, Jay M.; Lopez, Jacquelyn C.; Wayne, David M.

2012-07-05

The Plutonium Science and Manufacturing Directorate provides world-class, safe, secure, and reliable special nuclear material research, process development, technology demonstration, and manufacturing capabilities that support the nation's defense, energy, and environmental needs. We safely and efficiently process plutonium, uranium, and other actinide materials to meet national program requirements, while expanding the scientific and engineering basis of nuclear weapons-based manufacturing, and while producing the next generation of nuclear engineers and scientists. Actinide Process Chemistry (NCO-2) safely and efficiently processes plutonium and other actinide compounds to meet the nation's nuclear defense program needs. All of our processing activities are done in amore » world class and highly regulated nuclear facility. NCO-2's plutonium processing activities consist of direct oxide reduction, metal chlorination, americium extraction, and electrorefining. In addition, NCO-2 uses hydrochloric and nitric acid dissolutions for both plutonium processing and reduction of hazardous components in the waste streams. Finally, NCO-2 is a key team member in the processing of plutonium oxide from disassembled pits and the subsequent stabilization of plutonium oxide for safe and stable long-term storage.« less

Amarillo National Resource Center for plutonium. Work plan progress report, November 1, 1995--January 31, 1996

DOE Office of Scientific and Technical Information (OSTI.GOV)

Cluff, D.

1996-04-01

The Center operates under a cooperative agreement between DOE and the State of Texas and is directed and administered by an education consortium. Its programs include developing peaceful uses for the materials removed from dismantled weapons, studying effects of nuclear materials on environment and public health, remedying contaminated soils and water, studying storage, disposition, and transport of Pu, HE, and other hazardous materials removed from weapons, providing research and counsel to US in carrying out weapons reductions in cooperation with Russia, and conducting a variety of education and training programs.

Limiting Regret: Building the Army We Will Need

DTIC Science & Technology

2015-08-18

Recently, U.S. and Chinese experts have estimated that the North Koreans may be able to produce enough fissionable plutonium and uranium to build up...long-range missiles, but their recently revealed ability to separate uranium could give them the ability to build gun-assembled fission weapons similar...weapons programs and living up to their international obligations.” 36North Korea has had a uranium enrichment capacity since at least November 2010

Detection Technology in the 21st Century: The Case of Nuclear Weapons of Mass Destruction

DTIC Science & Technology

2008-03-26

Weapons of Mass Destruction FORMAT : Strategy Research Project DATE: 26 March 2008 WORD COUNT: 6,764 PAGES: 25 KEY TERMS: National Security, Deterrence...stocks remaining in Ukraine, Belarus, Uzbekistan, and other former Soviet and Eastern European states, and the unknown amounts of highly enriched uranium ...detect emissions from the decay of radioactive nuclides, which can occur naturally, such as uranium and thorium, or are manmade, such as plutonium

KSC-97PC1534

NASA Image and Video Library

1997-10-10

At Launch Complex 40 on Cape Canaveral Air Station, one of three Radioisotope Thermoelectric Generators (RTGs) is being installed on the Cassini spacecraft. RTGs are lightweight, compact spacecraft electrical power systems that have flown successfully on 23 previous U.S. missions over the past 37 years. These generators produce power by converting heat into electrical energy; the heat is provided by the natural radioactive decay of plutonium-238 dioxide, a non-weapons-grade material. RTGs enable spacecraft to operate at significant distances from the Sun where solar power systems would not be feasible. Cassini will travel two billion miles to reach Saturn and another 1.1 billion miles while in orbit around Saturn. Cassini is undergoing final preparations for liftoff on a Titan IVB/Centaur launch vehicle, with the launch window opening at 4:55 a.m. EDT, Oct. 13

KSC-97PC1532

NASA Image and Video Library

1997-10-10

KENNEDY SPACE CENTER, FLA. -- At Launch Complex 40 on Cape Canaveral Air Station, workers are installing three Radioisotope Thermoelectric Generators (RTGs) on the Cassini spacecraft. RTGs are lightweight, compact spacecraft electrical power systems that have flown successfully on 23 previous U.S. missions over the past 37 years. These generators produce power by converting heat into electrical energy; the heat is provided by the natural radioactive decay of plutonium-238 dioxide, a non-weapons-grade material. RTGs enable spacecraft to operate at significant distances from the Sun where solar power systems would not be feasible. Cassini will travel two billion miles to reach Saturn and another 1.1 billion miles while in orbit around Saturn. Cassini is undergoing final preparations for liftoff on a Titan IVB/Centaur launch vehicle, with the launch window opening at 4:55 a.m. EDT, Oct. 13

KSC-97PC1536

NASA Image and Video Library

1997-10-10

KENNEDY SPACE CENTER, FLA. -- At Launch Complex 40 on Cape Canaveral Air Station, workers are installing three Radioisotope Thermoelectric Generators (RTGs) on the Cassini spacecraft. RTGs are lightweight, compact spacecraft electrical power systems that have flown successfully on 23 previous U.S. missions over the past 37 years. These generators produce power by converting heat into electrical energy; the heat is provided by the natural radioactive decay of plutonium-238 dioxide, a non-weapons-grade material. RTGs enable spacecraft to operate at significant distances from the Sun where solar power systems would not be feasible. Cassini will travel two billion miles to reach Saturn and another 1.1 billion miles while in orbit around Saturn. Cassini is undergoing final preparations for liftoff on a Titan IVB/Centaur launch vehicle, with the launch window opening at 4:55 a.m. EDT, Oct. 13

Workers install the RTGs on the Cassini spacecraft at LC 40, CCAS

NASA Technical Reports Server (NTRS)

1997-01-01

At Launch Complex 40 on Cape Canaveral Air Station, workers are installing three Radioisotope Thermoelectric Generators (RTGs) on the Cassini spacecraft. RTGs are lightweight, compact spacecraft electrical power systems that have flown successfully on 23 previous U.S. missions over the past 37 years. These generators produce power by converting heat into electrical energy; the heat is provided by the natural radioactive decay of plutonium-238 dioxide, a non-weapons-grade material. RTGs enable spacecraft to operate at significant distances from the Sun where solar power systems would not be feasible. Cassini will travel two billion miles to reach Saturn and another 1.1 billion miles while in orbit around Saturn. Cassini is undergoing final preparations for liftoff on a Titan IVB/Centaur launch vehicle, with the launch window opening at 4:55 a.m. EDT, Oct. 13.

Accelerator-based conversion (ABC) of weapons plutonium: Plant layout study and related design issues

DOE Office of Scientific and Technical Information (OSTI.GOV)

Cowell, B.S.; Fontana, M.H.; Krakowski, R.A.

1995-04-01

In preparation for and in support of a detailed R and D Plan for the Accelerator-Based Conversion (ABC) of weapons plutonium, an ABC Plant Layout Study was conducted at the level of a pre-conceptual engineering design. The plant layout is based on an adaptation of the Molten-Salt Breeder Reactor (MSBR) detailed conceptual design that was completed in the early 1070s. Although the ABC Plant Layout Study included the Accelerator Equipment as an essential element, the engineering assessment focused primarily on the Target; Primary System (blanket and all systems containing plutonium-bearing fuel salt); the Heat-Removal System (secondary-coolant-salt and supercritical-steam systems); Chemicalmore » Processing; Operation and Maintenance; Containment and Safety; and Instrumentation and Control systems. Although constrained primarily to a reflection of an accelerator-driven (subcritical) variant of MSBR system, unique features and added flexibilities of the ABC suggest improved or alternative approaches to each of the above-listed subsystems; these, along with the key technical issues in need of resolution through a detailed R&D plan for ABC are described on the bases of the ``strawman`` or ``point-of-departure`` plant layout that resulted from this study.« less

Modeling and Comparison of Options for the Disposal of Excess Weapons Plutonium in Russia

DTIC Science & Technology

2002-04-01

fuel LWR cooling time LWR Pu load rate LWR net destruction frac ~ LWR reactors op life mox core frac Excess Separated Pu HTGR Cycle Pu in Waste LWR MOX...reflecting the cycle used in this type of reactor. For the HTGR , the entire core consists of plutonium fuel , therefore a core fraction is not specified...cooling time Time spent fuel unloaded from HTGR reactor must cool before permanently stored 3 years Mox core fraction Fraction of

Nuclear Weapons: Comprehensive Test Ban Treaty

DTIC Science & Technology

2006-08-16

Unicorn ,” is to be conducted in a “down-hole” or vertical shaft configuration similar to an underground nuclear test, not in a tunnel, to exercise...operational readiness.42 It is scheduled for FY2006, as noted below. SCEs try to determine if radioactive decay of aged plutonium would degrade weapon...Secretary of Energy Bill Richardson called SCEs “a key part of our scientific program to provide new tools and data that assess age -related complications

Nuclear Weapons: Comprehensive Test Ban Treaty

DTIC Science & Technology

2006-11-15

Unicorn ,” was conducted in a “down-hole” or vertical CRS-18 58 “Nanos Tours Nevada Test Site,” Daily Newsbulletin, Los Alamos National Laboratory...radioactive decay of aged plutonium would degrade weapon performance. Several SCEs have been used to support certification of the W88 pit. (A pit is the...tools and data that assess age -related complications and maintain the reliability and safety of the nation’s nuclear deterrent.”59 As they produce no

Environmental Information Document: L-reactor reactivation

DOE Office of Scientific and Technical Information (OSTI.GOV)

Mackey, H.E. Jr.

1982-04-01

Purpose of this Environmental Information Document is to provide background for assessing environmental impacts associated with the renovation, restartup, and operation of L Reactor at the Savannah River Plant (SRP). SRP is a major US Department of Energy installation for the production of nuclear materials for national defense. The purpose of the restart of L Reactor is to increase the production of nuclear weapons materials, such as plutonium and tritium, to meet projected needs in the nuclear weapons program.

Comparative safety assessment of surface versus submarine plutonium shipments

DOE Office of Scientific and Technical Information (OSTI.GOV)

Knepper, D.S.; Feltus, M.A.

1993-01-01

The recent shipment of plutonium from France to Japan aboard the freighter Akatsuki Maru touched off protests from environmental and antinuclear organizations. These protests arose from the fear of an accidental sinking of the vessel that would release its cargo to the sea, as well as the threat of a terrorist nation highjacking the ship for its cargo to produce atomic weapons. The sinking of a merchant ship is not uncommon, as illustrated by the famous losses of the tankers Amoco Cadiz and Exxon Valdez. The highjacking of a lightly armed freighter such as the Akatsuki Maru is possible andmore » would not be unduly difficult for a well-equipped terrorist nation. The combined threats of weapons proliferation and environmental damage arising from the diversion or destruction of a sea vessel carrying plutonium will continue to abound as the reprocessing of spent nuclear fuel increases. An alternate method for the transportation with reduced risks of both diversion and destruction needs to be developed. The shipment aboard the Akatsuki Maru was originally proposed to be flown from France to Japan over the continental United States. This proposal was rejected by the Reagan administration in 1988. A third alternative to the current ideas of air transport and surface transport is subsurface transport. This research project investigates the transportation of plutonium by submarine and compares it to the current method of transportation by freighter. This analysis involves a study of the military threat to a submarine by a terrorist nation and comparable threat to a surface vessel. To study the nonmilitary aspects of plutonium shipping, a fault-tree evaluation is performed for transportation by submarine and compared with the current risk analysis performed for surface vessels.« less

On the public perception of the risks from nuclear weapons: Would oralloy be more acceptable than plutonium

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kunsman, D.M.

We technologists generally only address risk magnitudes in our analyses, although other studies have found nineteen additional dimensions for the way the public perceives risk. These include controllability, voluntariness, catastrophic potential, and trust in the institution putting forth the risk. We and the geneml public use two different languages, and to understand what their concerns are, we need to realize that the culture surrounding nuclear weapons is completely alien to the general public. Ultimately, the acceptability of a risk is a values question, not a technical question. For most of the risk dimensions, the public would perceive no significant differencemore » between using oralloy and plutonium. This does not mean that the suggested design change should not be proposed, only that the case for, or against, it be made comprehensively using the best information available today. The world has changed: the ending of the cold war has decreased the benefit of nuclear weapons in the minds of the public and the specter of Chernobyl has increased the perceived risks of processes that use radioactive materials. Our analyses need to incorporate the lessons pertinent to this newer world.« less

On the public perception of the risks from nuclear weapons: Would oralloy be more acceptable than plutonium?

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kunsman, D.M.

We technologists generally only address risk magnitudes in our analyses, although other studies have found nineteen additional dimensions for the way the public perceives risk. These include controllability, voluntariness, catastrophic potential, and trust in the institution putting forth the risk. We and the geneml public use two different languages, and to understand what their concerns are, we need to realize that the culture surrounding nuclear weapons is completely alien to the general public. Ultimately, the acceptability of a risk is a values question, not a technical question. For most of the risk dimensions, the public would perceive no significant differencemore » between using oralloy and plutonium. This does not mean that the suggested design change should not be proposed, only that the case for, or against, it be made comprehensively using the best information available today. The world has changed: the ending of the cold war has decreased the benefit of nuclear weapons in the minds of the public and the specter of Chernobyl has increased the perceived risks of processes that use radioactive materials. Our analyses need to incorporate the lessons pertinent to this newer world.« less

Testing three explanations of the emergence of weapon carrying in peer context: the roles of aggression, victimization, and the social network.

PubMed

Dijkstra, Jan Kornelis; Gest, Scott D; Lindenberg, Siegwart; Veenstra, René; Cillessen, Antonius H N

2012-04-01

To examine the relative contribution of weapon carrying of peers, aggression, and victimization to weapon carrying of male and female adolescents over time. Data were derived from a population-based sample of male (N = 224) and female (N = 244) adolescents followed from grade 10 (M age = 15.5) to grade 11 (M age = 16.5). Peer networks were derived from best friend nominations. Self-reports were used to assess weapon carrying. Aggression and victimization were assessed using both self- and peer-reports. Use of dynamic social network modeling (SIENA) allowed prediction of weapon carrying in grade 11 as a function of weapon carrying of befriended peers, aggression, and victimization in grade 10, while selection processes and structural network effects (reciprocity and transitivity) were controlled for. Peer influence processes accounted for changes in weapon carrying over time. Self-reported victimization decreased weapon carrying 1 year later. Peer-reported victimization increased the likelihood of weapon carrying, particularly for highly aggressive adolescents. Boys were more likely to carry weapons than girls, but the processes associated with weapon carrying did not differ for boys and girls. These findings revealed that, in this population-based sample, weapon carrying of best friends, as well as aggression, contributed to the proliferation of weapons in friendship networks, suggesting processes of peer contagion as well as individual vulnerability to weapon carrying. Copyright © 2012 Society for Adolescent Health and Medicine. Published by Elsevier Inc. All rights reserved.

Guide of good practices for occupational radiological protection in plutonium facilities

DOE Office of Scientific and Technical Information (OSTI.GOV)

NONE

1998-06-01

This Technical Standard (TS) does not contain any new requirements. Its purpose is to provide guides to good practice, update existing reference material, and discuss practical lessons learned relevant to the safe handling of plutonium. the technical rationale is given to allow US Department of Energy (DOE) health physicists to adapt the recommendations to similar situations throughout the DOE complex. Generally, DOE contractor health physicists will be responsible to implement radiation protection activities at DOE facilities and DOE health physicists will be responsible for oversight of those activities. This guidance is meant to be useful for both efforts. This TSmore » replaces PNL-6534, Health Physics Manual of Good Practices for Plutonium Facilities, by providing more complete and current information and by emphasizing the situations that are typical of DOE`s current plutonium operations; safe storage, decontamination, and decommissioning (environmental restoration); and weapons disassembly.« less

Stabilizing stored PuO2 with addition of metal impurities

NASA Astrophysics Data System (ADS)

Moten, Shafaq; Huda, Muhammad

Plutonium oxides is of widespread significance due its application in nuclear fuels, space missions, as well as the long-termed storage of plutonium from spent fuel and nuclear weapons. The processes to refine and store plutonium bring many other elements in contact with the plutonium metal and thereby affect the chemistry of the plutonium. Pure plutonium metal corrodes to an oxide in air with the most stable form of this oxide is stoichiometric plutonium dioxide, PuO2. Defects such as impurities and vacancies can form in the plutonium dioxide before, during and after the refining processes as well as during storage. An impurity defect manifests itself at the bottom of the conduction band and affects the band gap of the unit cell. Studying the interaction between transition metals and plutonium dioxide is critical for better, more efficient storage plans as well as gaining insights to provide a better response to potential threats of exposure to the environment. Our study explores the interaction of a few metals within the plutonium dioxide structure which have a likelihood of being exposed to the plutonium dioxide powder. Using Density Functional Theory, we calculated a substituted metal impurity in PuO2 supercell. We repeated the calculations with an additional oxygen vacancy. Our results reveal interesting volume contraction of PuO2 supercell when one plutonium atom is substituted with a metal atom. The authors acknowledge the Texas Computing Center (TACC) at The University of Texas at Austin and High Performance Computing (HPC) at The University of Texas at Arlington.

Quarterly technical progress report, February 1, 1996--April 30, 1996

DOE Office of Scientific and Technical Information (OSTI.GOV)

NONE

This report from the Amarillo National REsource Center for PLutonium provides research highlights and provides information regarding the public dissemination of information. The center is a a scientific resource for information regarding the issues of the storage, disposition, potential utilization and transport of plutonium, high explosives, and other hazardous materials generated from nuclear weapons dismantlement. The center responds to informational needs and interpretation of technical and scientific data raised by interested parties and advisory groups. Also, research efforts are carried out on remedial action programs and biological/agricultural studies.

Experimental validation of a coupled neutron-photon inverse radiation transport solver

NASA Astrophysics Data System (ADS)

Mattingly, John; Mitchell, Dean J.; Harding, Lee T.

2011-10-01

Sandia National Laboratories has developed an inverse radiation transport solver that applies nonlinear regression to coupled neutron-photon deterministic transport models. The inverse solver uses nonlinear regression to fit a radiation transport model to gamma spectrometry and neutron multiplicity counting measurements. The subject of this paper is the experimental validation of that solver. This paper describes a series of experiments conducted with a 4.5 kg sphere of α-phase, weapons-grade plutonium. The source was measured bare and reflected by high-density polyethylene (HDPE) spherical shells with total thicknesses between 1.27 and 15.24 cm. Neutron and photon emissions from the source were measured using three instruments: a gross neutron counter, a portable neutron multiplicity counter, and a high-resolution gamma spectrometer. These measurements were used as input to the inverse radiation transport solver to evaluate the solver's ability to correctly infer the configuration of the source from its measured radiation signatures.

KSC-2011-7861

NASA Image and Video Library

2011-11-21

CAPE CANAVERAL, Fla. -- Members of the media view the Radiological Control Center (RADCC) at NASA's Kennedy Space Center in Florida during a tour regarding safety equipment and procedures for the upcoming launch of the Mars Science Laboratory (MSL) mission. The MSL spacecraft includes a multi-mission radioisotope thermoelectric generator (MMRTG) that will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. MSL's components include a car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 26 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Frankie Martin

KSC-2011-7856

NASA Image and Video Library

2011-11-21

CAPE CANAVERAL, Fla. -- Randy Scott, director of Kennedy Space Center's Radiological Control Center (RADCC), speaks to media during a tour regarding safety equipment and procedures for the upcoming launch of the Mars Science Laboratory (MSL) mission. Behind him is Steve Homann, senior advisor for the Department of Energy. The MSL spacecraft includes a multi-mission radioisotope thermoelectric generator (MMRTG) that will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. MSL's components include a car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 26 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Frankie Martin

KSC-2011-7860

NASA Image and Video Library

2011-11-21

CAPE CANAVERAL, Fla. -- Members of the media take a tour of the Radiological Control Center (RADCC) at NASA's Kennedy Space Center in Florida. The tour focused on safety equipment and procedures for the upcoming launch of the Mars Science Laboratory (MSL) mission. The MSL spacecraft includes a multi-mission radioisotope thermoelectric generator (MMRTG) that will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. MSL's components include a car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 26 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Frankie Martin

KSC-2011-7859

NASA Image and Video Library

2011-11-21

CAPE CANAVERAL, Fla. -- Surrounded by monitors and consoles, Randy Scott, director of Kennedy Space Center's Radiological Control Center (RADCC), speaks to media during a tour regarding safety equipment and procedures for the upcoming launch of the Mars Science Laboratory (MSL) mission. The MSL spacecraft includes a multi-mission radioisotope thermoelectric generator (MMRTG) that will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. MSL's components include a car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 26 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Frankie Martin

KSC-2011-7858

NASA Image and Video Library

2011-11-21

CAPE CANAVERAL, Fla. -- Steve Homann, senior advisor for the Department of Energy, speaks to media during a tour of the Radiological Control Center (RADCC) at NASA's Kennedy Space Center in Florida. The tour focused on safety equipment and procedures for the upcoming launch of the Mars Science Laboratory (MSL) mission. The MSL spacecraft includes a multi-mission radioisotope thermoelectric generator (MMRTG) that will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. MSL's components include a car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 26 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Frankie Martin

KSC-2011-7855

NASA Image and Video Library

2011-11-21

CAPE CANAVERAL, Fla. -- Several instruments are displayed for the media during a tour of the Radiological Control Center (RADCC) at NASA's Kennedy Space Center in Florida. The tour focused on safety equipment and procedures for the upcoming launch of the Mars Science Laboratory (MSL) mission. The MSL spacecraft includes a multi-mission radioisotope thermoelectric generator (MMRTG) that will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. MSL's components include a car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 26 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Frankie Martin

KSC-2011-7862

NASA Image and Video Library

2011-11-21

CAPE CANAVERAL, Fla. -- During a tour of the Radiological Control Center (RADCC) at NASA's Kennedy Space Center in Florida, members of the media listen as Ryan Bechtel of the U.S. Department of Energy explains safety equipment and procedures for the upcoming launch of the Mars Science Laboratory (MSL) mission. The MSL spacecraft includes a multi-mission radioisotope thermoelectric generator (MMRTG) that will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. MSL's components include a car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 26 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Frankie Martin

KSC-2011-7857

NASA Image and Video Library

2011-11-21

CAPE CANAVERAL, Fla. -- Steve Homann, senior advisor for the Department of Energy, speaks to media during a tour of the Radiological Control Center (RADCC) at NASA's Kennedy Space Center in Florida. The tour focused on safety equipment and procedures for the upcoming launch of the Mars Science Laboratory (MSL) mission. The MSL spacecraft includes a multi-mission radioisotope thermoelectric generator (MMRTG) that will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. MSL's components include a car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 26 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Frankie Martin

Residual radioactivity in the soil of the Semipalatinsk Nuclear Test Site in the former USSR.

PubMed

Yamamoto, M; Tsukatani, T; Katayama, Y

1996-08-01

This paper deals with our efforts to survey residual radioactivity in the soil sampled at the Semipalatinsk Nuclear Test Site and at off-site areas in Kazakhstan. The soil was sampled at the hypocenter where the first Soviet nuclear explosion was carried out on 29 August 1949, and at the bank of the crater called "Bolapan," which was formed by an underground nuclear detonation on 15 January 1965 along the Shagan River. As a comparison, other soil was also sampled in the cities of Kurchatov and Almaty. These data have allowed a preliminary evaluation of the contemporary radioactive contamination of the land in and around the test site. At the first nuclear explosion site and at Bolapan, higher than background levels of 239,240Pu with weapons-grade plutonium were detected together with fission and activation products such as 137Cs, 60Co, 152Eu, and 154Eu.

Complex chromosome aberrations persist in individuals many years after occupational exposure to densely ionizing radiation: an mFISH study.

PubMed

Hande, M Prakash; Azizova, Tamara V; Burak, Ludmilla E; Khokhryakov, Valentin F; Geard, Charles R; Brenner, David J

2005-09-01

Long-lived, sensitive, and specific biomarkers of particular mutagenic agents are much sought after and potentially have broad applications in the fields of cancer biology, epidemiology, and prevention. Many clastogens induce a spectrum of chromosome aberrations, and some of them can be exploited as biomarkers of exposure. Densely ionizing radiation, for example, alpha particle radiation (from radon or plutonium) and neutron radiation, preferentially induces complex chromosome aberrations, which can be detected by the 24-color multifluor fluorescence in situ hybridization (mFISH) technique. We report the detection and quantification of stable complex chromosome aberrations in lymphocytes of healthy former nuclear-weapons workers, who were exposed many years ago to plutonium, gamma rays, or both, at the Mayak weapons complex in Russia. We analyzed peripheral-blood lymphocytes from these individuals for the presence of persistent complex chromosome aberrations. A significantly elevated frequency of complex chromosome translocations was detected in the highly exposed plutonium workers but not in the group exposed only to high doses of gamma radiation. No such differences were found for simple chromosomal aberrations. The results suggest that stable complex chromosomal translocations represent a long-lived, quantitative, low-background biomarker of densely ionizing radiation for human populations exposed many years ago. (c) 2005 Wiley-Liss, Inc.

The Manhattan Project

Science.gov Websites

Short History of Oak Ridge National Laboratory (1943 - 1993) Los Alamos, New Mexico * Selected as Atomic Weapons Laboratory * Site Selection * History @ Los Alamos Hanford, Washington * Selected as Plutonium Production Facility * History of the Hanford Site 1943 - 1990 Chicago, Illinois * Promethean Boldness at

Integrating workplace exposure databases for occupational medicine services and epidemiologic studies at a former nuclear weapons facility.

PubMed

Ruttenber, A J; McCrea, J S; Wade, T D; Schonbeck, M F; LaMontagne, A D; Van Dyke, M V; Martyny, J W

2001-02-01

We outline methods for integrating epidemiologic and industrial hygiene data systems for the purpose of exposure estimation, exposure surveillance, worker notification, and occupational medicine practice. We present examples of these methods from our work at the Rocky Flats Plant--a former nuclear weapons facility that fabricated plutonium triggers for nuclear weapons and is now being decontaminated and decommissioned. The weapons production processes exposed workers to plutonium, gamma photons, neutrons, beryllium, asbestos, and several hazardous chemical agents, including chlorinated hydrocarbons and heavy metals. We developed a job exposure matrix (JEM) for estimating exposures to 10 chemical agents in 20 buildings for 120 different job categories over a production history spanning 34 years. With the JEM, we estimated lifetime chemical exposures for about 12,000 of the 16,000 former production workers. We show how the JEM database is used to estimate cumulative exposures over different time periods for epidemiological studies and to provide notification and determine eligibility for a medical screening program developed for former workers. We designed an industrial hygiene data system for maintaining exposure data for current cleanup workers. We describe how this system can be used for exposure surveillance and linked with the JEM and databases on radiation doses to develop lifetime exposure histories and to determine appropriate medical monitoring tests for current cleanup workers. We also present time-line-based graphical methods for reviewing and correcting exposure estimates and reporting them to individual workers.

Some less conventional options for plutonium disposal

NASA Astrophysics Data System (ADS)

Stoll, Dr. Wolfgang, Prof.

2000-07-01

Disposition of weapons Pu (W-Pu) aims at the replacement of military access restrictions by inherent longlasting technical barriers to make the return into the weapons state difficult and not rewarding anymore. At the time of the NAS-study in 1994, two ways were perceived to be mature and selected: Fissioning of W-Pu as LWR-MOX and the disposal in a vitrified radionuclide-spiked form.1 Both options since have been questioned for equality, met different acceptance at both superpowers and showed slow progress. A criterion to measure disarmament would be the amount of W-Pu in the different proliferation resistant forms, multiplied by the effort needed for each form to return to weapons quality.

Plutonium in the atmosphere: A global perspective.

PubMed

Thakur, P; Khaing, H; Salminen-Paatero, S

2017-09-01

A number of potential source terms have contributed plutonium isotopes to the atmosphere. The atmospheric nuclear weapon tests conducted between 1945 and 1980 and the re-entry of the burned SNAP-9A satellite in 1964, respectively. It is generally believed that current levels of plutonium in the stratosphere are negligible and compared with the levels generally found at surface-level air. In this study, the time trend analysis and long-term behavior of plutonium isotopes ( 239+240 Pu and 238 Pu) in the atmosphere were assessed using historical data collected by various national and international monitoring networks since 1960s. An analysis of historical data indicates that 239+240 Pu concentration post-1984 is still frequently detectable, whereas 238 Pu is detected infrequently. Furthermore, the seasonal and time-trend variation of plutonium concentration in surface air followed the stratospheric trends until the early 1980s. After the last Chinese test of 1980, the plutonium concentrations in surface air dropped to the current levels, suggesting that the observed concentrations post-1984 have not been under stratospheric control, but rather reflect the environmental processes such as resuspension. Recent plutonium atmospheric air concentrations data show that besides resuspension, other environmental processes such as global dust storms and biomass burning/wildfire also play an important role in redistributing plutonium in the atmosphere. Copyright © 2017 Elsevier Ltd. All rights reserved.

Uranium and Thorium

ERIC Educational Resources Information Center

Finch, Warren I.

1978-01-01

The results of President Carter's policy on non-proliferation of nuclear weapons are expected to slow the growth rate in energy consumption, put the development of the breeder reactor in question, halt plans to reprocess and recycle uranium and plutonium, and expand facilities to supply enriched uranium. (Author/MA)

Crystalline matrices for the immobilization of plutonium and actinides

DOE Office of Scientific and Technical Information (OSTI.GOV)

Anderson, E.B.; Burakov, E.E.; Galkin, Ya.B.

1996-05-01

The management of weapon plutonium, disengaged as a result of conversion, is considered together with the problem of the actinide fraction of long-lived high level radioactive wastes. It is proposed to use polymineral ceramics based on crystalline host-phases: zircon ZrSiO{sub 4} and zirconium dioxide ZrO{sub 2}, for various variants of the management of plutonium and actinides (including the purposes of long-term safe storage or final disposal from the human activity sphere). It is shown that plutonium and actinides are able to form with these phases on ZrSiO{sub 4} and ZrO{sub 2} was done on laboratory level by the hot pressingmore » method, using the plasmochemical calcination technology. To incorporate simulators of plutonium into the structure of ZrSiO{sub 4} and ZrO{sub 2} in the course of synthesis, an original method developed by the authors as a result of studying the high-uranium zircon (Zr,U) SiO{sub 4} form Chernobyl {open_quotes}lavas{close_quotes} was used.« less

Proliferation dangers associated with nuclear medicine: getting weapons-grade uranium out of radiopharmaceutical production.

PubMed

Williams, Bill; Ruff, Tilman A

2007-01-01

Abolishing the threat of nuclear war requires the outlawing of nuclear weapons and dismantling current nuclear weapon stockpiles, but also depends on eliminating access to fissile material (nuclear weapon fuel). The near-universal use of weapons-grade, highly enriched uranium (HEU) to produce radiopharmaceuticals is a significant proliferation hazard. Health professionals have a strategic opportunity and obligation to progress the elimination of medically-related commerce in HEU, closing one of the most vulnerable pathways to the much-feared 'terrorist bomb'.

Determination of 240Pu/239Pu isotopic ratios in human tissues collected from areas around the Semipalatinsk Nuclear Test Site by sector-field high resolution ICP-MS.

PubMed

Yamamoto, M; Oikawa, S; Sakaguchi, A; Tomita, J; Hoshi, M; Apsalikov, K N

2008-09-01

Information on the 240Pu/239Pu isotope ratios in human tissues for people living around the Semipalatinsk Nuclear Test Site (SNTS) was deduced from 9 sets of soft tissues and bones, and 23 other bone samples obtained by autopsy. Plutonium was radiochemically separated and purified, and plutonium isotopes (239Pu and 240Pu) were determined by sector-field high resolution inductively coupled plasma-mass spectrometry. For most of the tissue samples from the former nine subjects, low 240Pu/239Pu isotope ratios were determined: bone, 0.125 +/- 0.018 (0.113-0.145, n = 4); lungs, 0.063 +/- 0.010 (0.051-0.078, n = 5); and liver, 0.148 +/- 0.026 (0.104-0.189, n = 9). Only 239Pu was detected in the kidney samples; the amount of 240Pu was too small to be measured, probably due to the small size of samples analyzed. The mean 240Pu/239Pu isotope ratio for bone samples from the latter 23 subjects was 0.152 +/- 0.034, ranging from 0.088 to 0.207. A significant difference (a two-tailed Student's t test; 95% significant level, alpha = 0.05) between mean 240Pu/239Pu isotope ratios for the tissue samples and for the global fallout value (0.178 +/- 0.014) indicated that weapons-grade plutonium from the atomic bombs has been incorporated into the human tissues, especially lungs, in the residents living around the SNTS. The present 239,240Pu concentrations in bone, lung, and liver samples were, however, not much different from ranges found for human tissues from other countries that were due solely to global fallout during the 1970's-1980's.

Nuclear pursuits

DOE Office of Scientific and Technical Information (OSTI.GOV)

Not Available

1993-05-01

This table lists quantities of warheads (in stockpile, peak number per year, total number built, number of known test explosions), weapon development milestones (developers of the atomic bomb and hydrogen bomb, date of first operational ICBM, first nuclear-powered naval SSN in service, first MIRVed missile deployed), and testing milestones (first fission test, type of boosted fission weapon, multistage thermonuclear test, number of months from fission bomb to multistage thermonuclear bomb, etc.), and nuclear infrastructure (assembly plants, plutonium production reactors, uranium enrichment plants, etc.). Countries included in the tally are the United States, Soviet Union, Britain, France, and China.

Policy and Technical Issues Facing a Fissile Material (Cutoff) Treaty

DOE PAGES

von Hippel, Frank; Mian, Zia

2015-05-18

We report the largest obstacle to creating nuclear weapons, starting with the ones that destroyed Hiroshima and Nagasaki, has been to make sufficient quantities of fissile materials – highly enriched uranium (HEU) and plutonium – to sustain an explosive fission chain reaction.1 Recognition of this fact has, for more than fifty years, underpinned both the support for and the opposition to adoption of an international treaty banning at a minimum the production of more fissile materials for nuclear weapons, commonly referred to as a fissile material cutoff treaty (FMCT).

Microdistribution and Long-Term Retention of 239Pu (NO3)4 in the Respiratory Tracts of an Acutely Exposed Plutonium Worker and Experimental Beagle Dogs

DOE Office of Scientific and Technical Information (OSTI.GOV)

Nielsen, Christopher E.; Wilson, Dulaney A.; Brooks, Antone L.

The long-term retention of inhaled soluble forms of plutonium raises concerns as to the potential health effects in persons working in nuclear energy or the nuclear weapons program. The distributions of long-term retained inhaled plutonium-nitrate [239Pu (NO3)4] deposited in the lungs of an accidentally exposed nuclear worker (Human Case 0269) and in the lungs of experimentally exposed beagle dogs with varying initial lung depositions were determined via autoradiographs of selected histological lung, lymph node, trachea, and nasal turbinate tissue sections. These studies showed that both the human and dogs had a non-uniform distribution of plutonium throughout the lung tissue. Fibroticmore » scar tissue effectively encapsulated a portion of the plutonium and prevented its clearance from the body or translocation to other tissues and diminished dose to organ parenchyma. Alpha radiation activity from deposited plutonium in Human Case 0269 was observed primarily along the sub-pleural regions while no alpha activity was seen in the tracheobronchial lymph nodes of this individual. However, relatively high activity levels in the tracheobronchial lymph nodes of the beagles indicated the lymphatic system was effective in clearing deposited plutonium from the lung tissues. In both the human case and beagle dogs, the appearance of retained plutonium within the respiratory tract was inconsistent with current biokinetic models of clearance for soluble forms of plutonium. Bound plutonium can have a marked effect on the dose to the lungs and subsequent radiation exposure has the potential increase in cancer risk.« less

A simple model for the critical mass of a nuclear weapon

NASA Astrophysics Data System (ADS)

Reed, B. Cameron

2018-07-01

A probability-based model for estimating the critical mass of a fissile isotope is developed. The model requires introducing some concepts from nuclear physics and incorporating some approximations, but gives results correct to about a factor of two for uranium-235 and plutonium-239.

Measurements of plutonium, 237Np, and 137Cs in the BCR 482 lichen reference material

DOE Office of Scientific and Technical Information (OSTI.GOV)

Lavelle, Kevin B.; Miller, Jeffrey L.; Hanson, Susan K.

Select anthropogenic radionuclides were measured in lichen reference material, BCR 482. This material was originally collected in Axalp, Switzerland in 1991 and is composed of the epiphytic lichen Pseudevernia furfuracea. Samples from three separate bottles of BCR 482 were analyzed for uranium, neptunium, and plutonium isotopes by inductively coupled plasma mass spectrometry (ICP-MS) and analyzed for cesium-137 by gamma-ray spectrometry. The isotopic composition of the radionuclides measured in BCR 482 suggests contributions from both global fallout resulting from historical nuclear weapons testing and more volatile materials released following the Chernobyl accident.

Measurements of plutonium, 237Np, and 137Cs in the BCR 482 lichen reference material

DOE PAGES

Lavelle, Kevin B.; Miller, Jeffrey L.; Hanson, Susan K.; ...

2015-10-01

Select anthropogenic radionuclides were measured in lichen reference material, BCR 482. This material was originally collected in Axalp, Switzerland in 1991 and is composed of the epiphytic lichen Pseudevernia furfuracea. Samples from three separate bottles of BCR 482 were analyzed for uranium, neptunium, and plutonium isotopes by inductively coupled plasma mass spectrometry (ICP-MS) and analyzed for cesium-137 by gamma-ray spectrometry. The isotopic composition of the radionuclides measured in BCR 482 suggests contributions from both global fallout resulting from historical nuclear weapons testing and more volatile materials released following the Chernobyl accident.

Passive Neutron Non-Destructive Assay for Remediation of Radiological Waste at Hanford Burial Grounds- 13189

DOE Office of Scientific and Technical Information (OSTI.GOV)

Simpson, A.; Pitts, M.; Ludowise, J.D.

The Hanford burial grounds contains a broad spectrum of low activity radioactive wastes, transuranic (TRU) wastes, and hazardous wastes including fission products, byproduct material (thorium and uranium), plutonium and laboratory chemicals. A passive neutron non-destructive assay technique has been developed for characterization of shielded concreted drums exhumed from the burial grounds. This method facilitates the separation of low activity radiological waste containers from TRU waste containers exhumed from the burial grounds. Two identical total neutron counting systems have been deployed, each consisting of He-3 detectors surrounded by a polyethylene moderator. The counts are processed through a statistical filter that removesmore » outliers in order to suppress cosmic spallation events and electronic noise. Upon completion of processing, a 'GO / NO GO' signal is provided to the operator based on a threshold level equivalent to 0.5 grams of weapons grade plutonium in the container being evaluated. This approach allows instantaneous decisions to be made on how to proceed with the waste. The counting systems have been set up using initial on-site measurements (neutron emitting standards loaded into surrogate waste containers) combined with Monte Carlo modeling techniques. The benefit of this approach is to allow the systems to extend their measurement ranges, in terms of applicable matrix types and container sizes, with minimal interruption to the operations at the burial grounds. (authors)« less

Excess plutonium disposition: The deep borehole option

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ferguson, K.L.

1994-08-09

This report reviews the current status of technologies required for the disposition of plutonium in Very Deep Holes (VDH). It is in response to a recent National Academy of Sciences (NAS) report which addressed the management of excess weapons plutonium and recommended three approaches to the ultimate disposition of excess plutonium: (1) fabrication and use as a fuel in existing or modified reactors in a once-through cycle, (2) vitrification with high-level radioactive waste for repository disposition, (3) burial in deep boreholes. As indicated in the NAS report, substantial effort would be required to address the broad range of issues relatedmore » to deep bore-hole emplacement. Subjects reviewed in this report include geology and hydrology, design and engineering, safety and licensing, policy decisions that can impact the viability of the concept, and applicable international programs. Key technical areas that would require attention should decisions be made to further develop the borehole emplacement option are identified.« less

A long view of global plutonium management

DOE Office of Scientific and Technical Information (OSTI.GOV)

Wagner, R.L. Jr.

1995-10-01

Dealing with the large and growing world inventories of fissile materials from all sources is a major part of the long term challenge of limiting the danger from nuclear weapons. Providing clean, safe nuclear power may also be needed to prevent conditions from arising which could lead to large scale nuclear weapon (re)armament. ADTT technologies might reconcile the seeming dilemma of providing nuclear power while maintaining a very low world inventory of nuclear materials which can be used in weapons. This vision for ADTT should be tested in a variety of ways, including comparisons with competing approaches and with othermore » objectives. Such testing is one part of constructing a path for a decades-long, worldwide implementation campaign for ADTT.« less

Plutonium isotopic signatures in soils and their variation (2011-2014) in sediment transiting a coastal river in the Fukushima Prefecture, Japan.

PubMed

Jaegler, Hugo; Pointurier, Fabien; Onda, Yuichi; Hubert, Amélie; Laceby, J Patrick; Cirella, Maëva; Evrard, Olivier

2018-05-04

The Fukushima Daiichi Nuclear Power Plant (FDNPP) accident resulted in a significant release of radionuclides that were deposited on soils in Northeastern Japan. Plutonium was detected at trace levels in soils and sediments collected around the FDNPP. However, little is known regarding the spatial-temporal variation of plutonium in sediment transiting rivers in the region. In this study, plutonium isotopic compositions were first measured in soils (n = 5) in order to investigate the initial plutonium deposition. Then, plutonium isotopic compositions were measured on flood sediment deposits (n = 12) collected after major typhoon events in 2011, 2013 and 2014. After a thorough radiochemical purification, isotopic ratios ( 240 Pu/ 239 Pu, 241 Pu/ 239 Pu and 242 Pu/ 239 Pu) were measured with a Multi-Collector Inductively Coupled Mass Spectrometer (MC ICP-MS), providing discrimination between plutonium derived from global fallout, from atmospheric nuclear weapon tests, and plutonium derived from the FDNPP accident. Results demonstrate that soils with the most Fukushima-derived plutonium were in the main radiocaesium plume and that there was a variable mixture of plutonium sources in the flood sediment samples. Plutonium concentrations and isotopic ratios generally decreased between 2011 and 2014, reflecting the progressive erosion and transport of contaminated sediment in this coastal river during flood events. Exceptions to this general trend were attributed to the occurrence of decontamination works or the remobilisation of contaminated material during typhoons. The different plutonium concentrations and isotopic ratios obtained on three aliquots of a single sample suggest that the Fukushima-derived plutonium was likely borne by discrete plutonium-containing particles. In the future, these particles should be isolated and further characterized in order to better understand the fate of this long-lived radionuclide in the environment. Copyright © 2018 Elsevier Ltd. All rights reserved.

Uncertainties in the North Korean Nuclear Threat

DTIC Science & Technology

2010-01-01

Bermudez, Joseph S., “The Democratic People’s Republic of Korea and Unconventional Weapons,” in Peter R. Lavoy, Scott D. Sagan , and James J. Wirtz, eds...Korea Has ‘Weaponized’ Plutonium,” Associated Press, January 17, 2009. Robbins, Carla Anne, and Gordon Fairclough, “North Korea Sparks Proliferation

The Feed Materials Program of the Manhattan Project: A Foundational Component of the Nuclear Weapons Complex

NASA Astrophysics Data System (ADS)

Reed, B. Cameron

2014-12-01

The feed materials program of the Manhattan Project was responsible for procuring uranium-bearing ores and materials and processing them into forms suitable for use as source materials for the Project's uranium-enrichment factories and plutonium-producing reactors. This aspect of the Manhattan Project has tended to be overlooked in comparison with the Project's more dramatic accomplishments, but was absolutely vital to the success of those endeavors: without appropriate raw materials and the means to process them, nuclear weapons and much of the subsequent cold war would never have come to pass. Drawing from information available in Manhattan Engineer District Documents, this paper examines the sources and processing of uranium-bearing materials used in making the first nuclear weapons and how the feed materials program became a central foundational component of the postwar nuclear weapons complex.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Robertson, Janeen Denise

In a mortality study of white males who had worked at the Rocky Flats Nuclear Weapons Plant between 1952 and 1979, an increased number of deaths from benign and unspecified intracranial neoplasms was found. A case-control study nested within this cohort investigated the hypothesis that an association existed between brain tumor death and exposure to either internally deposited plutonium or external ionizing radiation. There was no statistically significant association found between estimated radiation exposure from internally deposited plutonium and the development of brain tumors. Exposure by job or work area showed no significant difference between the cohort and the controlmore » groups. An update of the study found elevated risk estimates for (1) all lymphopoietic neoplasms, and (2) all causes of death in employees with body burdens greater than or equal to two nanocuries of plutonium. There was an excess of brain tumors for the entire cohort. Similar cohort studies conducted on worker populations from other plutonium handling facilities have not yet shown any elevated risks for brain tumors. Historically, the Rocky Flats Nuclear Weapons Plant used large quantities of chemicals in their production operations. The use of solvents, particularly carbon tetrachloride, was unique to Rocky Flats. No investigation of the possible confounding effects of chemical exposures was done in the initial studies. The objectives of the present study are to (1) investigate the history of chemical use at the Rocky Flats facility; (2) locate and analyze chemical monitoring information in order to assess employee exposure to the chemicals that were used in the highest volume; and (3) determine the feasibility of establishing a chemical exposure assessment model that could be used in future epidemiology studies.« less

Nevada Applied Ecology Group publications. [Bibliography of radioecological studies at NTS with special reference to plutonium

DOE Office of Scientific and Technical Information (OSTI.GOV)

White, M.G.; Pfuderer, H.A.

This bibliography serves as a guide to the environmental studies sponsored by the Nevada Applied Ecology Group (NAEG) at the Department of Energy Nevada Test Site nuclear weapons complex. The NAEG is part of the Nevada Operations Office of the United States Department of Energy. The references included in the bibliography reflect the interests of the NAEG (e.g., hazard evaluation of the nuclear safety-shot sites). The objectives of the NAEG plutonium studies at the Nevada Test Site were defined as follows: (1) delineate locations of contamination; (2) determine concentrations in ecosystem components; (3) quantify rates of movements among ecosystem components;more » (4) evaluate radiological hazards of plutonium; (5) identify areas which need to be cleaned up or treated; and (6) develop techniques for cleanup or treatment.« less

The myth of the ``proliferation-resistant'' closed nuclear fuel cycle

NASA Astrophysics Data System (ADS)

Lyman, Edwin S.

2000-07-01

National nuclear energy programs that engage in reprocessing of spent nuclear fuel (SNF) and the development of "closed" nuclear fuel cycles based on the utilization of plutonium process and store large quantities of weapons-usable nuclear materials in forms vulnerable to diversion or theft by national or subnational groups. Proliferation resistance, an idea dating back at least as far as the International Fuel Cycle Evaluation (INFCE) of the late 1970s, is a loosely defined term referring to processes for chemical separation of SNF that do not extract weapons-usable materials in a purified form.

North Korea’s Nuclear Weapons: Technical Issues

DTIC Science & Technology

2009-05-26

Warren Strobel , “North Korean nuclear documents challenge CIA assertions,” McClatchyNewspapers, May 28, 2008. 23 “N.K. says plutonium ‘weaponized’ and...Chosun Ilbo, January 29, 2008. 78 Lee Chi-dong, “N Korea Complains About Slow Provision of Energy Aid,” Yonhap News, June 5, 2008. 79 “N. Korea

KSC-2011-7900

NASA Image and Video Library

2011-11-17

CAPE CANAVERAL, Fla. -- In the Vertical Integration Facility at Space Launch Complex-41 on Cape Canaveral Air Force Station, spacecraft technicians install the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission on the Curiosity rover. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is scheduled for Nov. 25. For more information, visit http://www.nasa.gov/msl. Photo credit: Department of Energy/Idaho National Laboratory

A Physicist Looks at the Terrorist Threat

NASA Astrophysics Data System (ADS)

Muller, Richard

2009-05-01

Many people fear a terrorist nuclear device, smuggled into the United States, as the one weapon that could surpass the destruction and impact of 9-11. I'll review the design of nuclear weapons, with emphasis on the kinds that can be developed by rogue nations, terrorist groups, and high-school students. Saddam, prior to the first gulf war, was developing a uranium bomb, similar to the one that destroyed Hiroshima. His calutrons (named after my university) were destroyed by the United Nations. The North Korean nuclear weapon was, like the U.S. bomb used on Nagasaki, based on plutonium. Its test released the energy equivalent of about 400 tons of TNT. Although some people have speculated that they were attempting to build a small bomb, it is far more likely that this weapon was a fizzle, with less than 1 percent of the plutonium exploded. In contrast, the energy released from burning jet fuel at the 9-11 World Trade Center attack was the equivalent of 900 tons of TNT for each plane -- over twice that of the North Korean Nuke. The damage came from the fact that gasoline delivers 10 kilocalories per gram, about 15 times the energy of an equal weight of TNT. It is this huge energy per gram that also accounts for our addiction to gasoline; per gram, high performance lithium-ion computer batteries carry only 1 percent as much energy. A dirty bomb (radiological weapon) is also unattractive to terrorists because of the threhold effect: doses less than 100 rem produce no radiation illness and will leave no dead bodies at the scene. That may be why al Qaeda instructed Jose Padilla to abandon his plans for a dirty bomb attack in Chicago, and to try a fossil fuel attack (natural gas) instead. I will argue that the biggest terrorist threat is the conventional low-tech one, such as an airplane attack on a crowded stadium using the explosive fuel that they can legally buy at the corner station.

The scheme for evaluation of isotopic composition of fast reactor core in closed nuclear fuel cycle

NASA Astrophysics Data System (ADS)

Saldikov, I. S.; Ternovykh, M. Yu; Fomichenko, P. A.; Gerasimov, A. S.

2017-01-01

The PRORYV (i.e. «Breakthrough» in Russian) project is currently under development. Within the framework of this project, fast reactors BN-1200 and BREST-OD-300 should be built to, inter alia, demonstrate possibility of the closed nuclear fuel cycle technologies with plutonium as a main source of power. Russia has a large inventory of plutonium which was accumulated in the result of reprocessing of spent fuel of thermal power reactors and conversion of nuclear weapons. This kind of plutonium will be used for development of initial fuel assemblies for fast reactors. To solve the closed nuclear fuel modeling tasks REPRORYV code was developed. It simulates the mass flow for nuclides in the closed fuel cycle. This paper presents the results of modeling of a closed nuclear fuel cycle, nuclide flows considering the influence of the uncertainty on the outcome of neutron-physical characteristics of the reactor.

Nuclear Weapons Council: Enhancing Interagency Collaboration Could Help with Implementation of Expanded Responsibilities

DTIC Science & Technology

2015-05-01

provide a cross section of the types of programs and activities the Council oversees. Specifically, we selected the B61 -12 life-extension program; the... B61 -12 life-extension program; the W76-1 life-extension program; the plutonium strategy; and budget- related activities,7 such as the Council’s

H CANYON PROCESSING IN CORRELATION WITH FH ANALYTICAL LABS

DOE Office of Scientific and Technical Information (OSTI.GOV)

Weinheimer, E.

2012-08-06

Management of radioactive chemical waste can be a complicated business. H Canyon and F/H Analytical Labs are two facilities present at the Savannah River Site in Aiken, SC that are at the forefront. In fact H Canyon is the only large-scale radiochemical processing facility in the United States and this processing is only enhanced by the aid given from F/H Analytical Labs. As H Canyon processes incoming materials, F/H Labs provide support through a variety of chemical analyses. Necessary checks of the chemical makeup, processing, and accountability of the samples taken from H Canyon process tanks are performed at themore » labs along with further checks on waste leaving the canyon after processing. Used nuclear material taken in by the canyon is actually not waste. Only a small portion of the radioactive material itself is actually consumed in nuclear reactors. As a result various radioactive elements such as Uranium, Plutonium and Neptunium are commonly found in waste and may be useful to recover. Specific processing is needed to allow for separation of these products from the waste. This is H Canyon's specialty. Furthermore, H Canyon has the capacity to initiate the process for weapons-grade nuclear material to be converted into nuclear fuel. This is one of the main campaigns being set up for the fall of 2012. Once usable material is separated and purified of impurities such as fission products, it can be converted to an oxide and ultimately turned into commercial fuel. The processing of weapons-grade material for commercial fuel is important in the necessary disposition of plutonium. Another processing campaign to start in the fall in H Canyon involves the reprocessing of used nuclear fuel for disposal in improved containment units. The importance of this campaign involves the proper disposal of nuclear waste in order to ensure the safety and well-being of future generations and the environment. As processing proceeds in the fall, H Canyon will have a substantial number of samples being sent to F/H Labs. All analyses of these samples are imperative to safe and efficient processing. The important campaigns to occur would be impossible without feedback from analyses such as chemical makeup of solutions, concentrations of dissolution acids and nuclear material, as well as nuclear isotopic data. The necessity of analysis for radiochemical processing is evident. Processing devoid of F/H Lab's feedback would go against the ideals of a safety-conscious and highly accomplished processing facility such as H Canyon.« less

Nuclear waste forms for actinides

PubMed Central

Ewing, Rodney C.

1999-01-01

The disposition of actinides, most recently 239Pu from dismantled nuclear weapons, requires effective containment of waste generated by the nuclear fuel cycle. Because actinides (e.g., 239Pu and 237Np) are long-lived, they have a major impact on risk assessments of geologic repositories. Thus, demonstrable, long-term chemical and mechanical durability are essential properties of waste forms for the immobilization of actinides. Mineralogic and geologic studies provide excellent candidate phases for immobilization and a unique database that cannot be duplicated by a purely materials science approach. The “mineralogic approach” is illustrated by a discussion of zircon as a phase for the immobilization of excess weapons plutonium. PMID:10097054

Trends in Bullying, Physical Fighting, and Weapon Carrying Among 6th- Through 10th-Grade Students From 1998 to 2010: Findings From a National Study

PubMed Central

Brooks-Russell, Ashley; Wang, Jing; Iannotti, Ronald J.

2014-01-01

Objectives. We examined trends from 1998 to 2010 in bullying, bullying victimization, physical fighting, and weapon carrying and variations by gender, grade level, and race/ethnicity among US adolescents. Methods. The Health Behavior in School-Aged Children surveys of nationally representative samples of students in grades 6 through 10 were completed in 1998 (n = 15 686), 2002 (n = 14 818), 2006 (n = 9229), and 2010 (n = 10 926). We assessed frequency of bullying behaviors, physical fighting, and weapon carrying as well as weapon type and subtypes of bullying. We conducted logistic regression analyses, accounting for the complex sampling design, to identify trends and variations by demographic factors. Results. Bullying perpetration, bullying victimization, and physical fighting declined from 1998 to 2010. Weapon carrying increased for White students only. Declines in bullying perpetration and victimization were greater for boys than for girls. Declines in bullying perpetration and physical fighting were greater for middle-school students than for high-school students. Conclusions. Declines in most violent behaviors are encouraging; however, lack of decline in weapon carrying merits further attention. PMID:24825213

LIFE Materials: Overview of Fuels and Structural Materials Issues Volume 1

DOE Office of Scientific and Technical Information (OSTI.GOV)

Farmer, J

2008-09-08

The National Ignition Facility (NIF) project, a laser-based Inertial Confinement Fusion (ICF) experiment designed to achieve thermonuclear fusion ignition and burn in the laboratory, is under construction at the Lawrence Livermore National Laboratory (LLNL) and will be completed in April of 2009. Experiments designed to accomplish the NIF's goal will commence in late FY2010 utilizing laser energies of 1 to 1.3 MJ. Fusion yields of the order of 10 to 20 MJ are expected soon thereafter. Laser initiated fusion-fission (LIFE) engines have now been designed to produce nuclear power from natural or depleted uranium without isotopic enrichment, and from spentmore » nuclear fuel from light water reactors without chemical separation into weapons-attractive actinide streams. A point-source of high-energy neutrons produced by laser-generated, thermonuclear fusion within a target is used to achieve ultra-deep burn-up of the fertile or fissile fuel in a sub-critical fission blanket. Fertile fuels including depleted uranium (DU), natural uranium (NatU), spent nuclear fuel (SNF), and thorium (Th) can be used. Fissile fuels such as low-enrichment uranium (LEU), excess weapons plutonium (WG-Pu), and excess highly-enriched uranium (HEU) may be used as well. Based upon preliminary analyses, it is believed that LIFE could help meet worldwide electricity needs in a safe and sustainable manner, while drastically shrinking the nation's and world's stockpile of spent nuclear fuel and excess weapons materials. LIFE takes advantage of the significant advances in laser-based inertial confinement fusion that are taking place at the NIF at LLNL where it is expected that thermonuclear ignition will be achieved in the 2010-2011 timeframe. Starting from as little as 300 to 500 MW of fusion power, a single LIFE engine will be able to generate 2000 to 3000 MWt in steady state for periods of years to decades, depending on the nuclear fuel and engine configuration. Because the fission blanket in a fusion-fission hybrid system is subcritical, a LIFE engine can burn any fertile or fissile nuclear material, including un-enriched natural or depleted U and SNF, and can extract a very high percentage of the energy content of its fuel resulting in greatly enhanced energy generation per metric ton of nuclear fuel, as well as nuclear waste forms with vastly reduced concentrations of long-lived actinides. LIFE engines could thus provide the ability to generate vast amounts of electricity while greatly reducing the actinide content of any existing or future nuclear waste and extending the availability of low cost nuclear fuels for several thousand years. LIFE also provides an attractive pathway for burning excess weapons Pu to over 99% FIMA (fission of initial metal atoms) without the need for fabricating or reprocessing mixed oxide fuels (MOX). Because of all of these advantages, LIFE engines offer a pathway toward sustainable and safe nuclear power that significantly mitigates nuclear proliferation concerns and minimizes nuclear waste. An important aspect of a LIFE engine is the fact that there is no need to extract the fission fuel from the fission blanket before it is burned to the desired final level. Except for fuel inspection and maintenance process times, the nuclear fuel is always within the core of the reactor and no weapons-attractive materials are available outside at any point in time. However, an important consideration when discussing proliferation concerns associated with any nuclear fuel cycle is the ease with which reactor fuel can be converted to weapons usable materials, not just when it is extracted as waste, but at any point in the fuel cycle. Although the nuclear fuel remains in the core of the engine until ultra deep actinide burn up is achieved, soon after start up of the engine, once the system breeds up to full power, several tons of fissile material is present in the fission blanket. However, this fissile material is widely dispersed in millions of fuel pebbles, which can be tagged as individual accountable items, and thus made difficult to divert in large quantities. Several topical reports are being prepared on the materials and processes required for the LIFE engine. Specific materials of interest include: (1) Baseline TRISO Fuel (TRISO); (2) Inert Matrix Fuel (IMF) & Other Alternative Solid Fuels; (3) Beryllium (Be) & Molten Lead Blankets (Pb/PbLi); (4) Molten Salt Coolants (FLIBE/FLiNaBe/FLiNaK); (5) Molten Salt Fuels (UF4 + FLIBE/FLiNaBe); (6) Cladding Materials for Fuel & Beryllium; (7) ODS FM Steel (ODS); (8) Solid First Wall (SFW); and (9) Solid-State Tritium Storage (Hydrides).« less

Preparation of plutonium-bearing ceramics via mechanically activated precursor

NASA Astrophysics Data System (ADS)

Chizhevskaya, S. V.; Stefanovsky, S. V.

2000-07-01

The problem of excess weapons plutonium disposition is suggested to be solved by means of its incorporation in stable ceramics with high chemical durability and radiation resistivity. The most promising host phases for plutonium as well as uranium and neutron poisons (gadolinium, hafnium) are zirconolite, pyrochlore, zircon, zirconia [1,2], and murataite [3]. Their production requires high temperatures and a fine-grained homogeneous precursor to reach final waste form with high quality and low leachability. Currently various routes to homogeneous products preparation such as sol-gel technology, wet-milling, and grinding in a ball or planetary mill are used. The best result demonstrates sol-gel technology but this route is very complicated. An alternative technology for preparation of ceramic precursors is the treatment of the oxide batch with high mechanical energy [4]. Such a treatment produces combination of mechanical (fine milling with formation of various defects, homogenization) and chemical (split bonds with formation of active centers—free radicals, ion-radicals, etc.) effects resulting in higher reactivity of the activated batch.

Deploying Nuclear Detection Systems: A Proposed Strategy for Combating Nuclear Terrorism

DTIC Science & Technology

2007-07-01

lower cost than other gamma radiation detectors (if increased count rate is all one is looking for). Low cost makes plastic scintillation detectors...material, particularly enriched uranium and plutonium, the basic fuel for nuclear bombs. • Measures to strengthen international institutions to... uranium to specifications required for a nuclear weapon.1 This illicit shipment of centrifuges was part of an international nuclear materials

Science and technology review, April 1997

DOE Office of Scientific and Technical Information (OSTI.GOV)

Upadhye, R.

1997-04-01

This month's issue has the following articles: (1) The Laboratory in the News; (2) Commentary by Tom Isaacs--Shaping Nuclear Materials Policy; (3) Dealing with a Dangerous Surplus from the Cold War--Since the end of the Cold War, the Laboratory has been spearheading studies on the disposition of surplus weapons plutonium; (4) Volcanoes: A Peek into Our Planet's Plumbing; and (5) Optical Networks: The Wave of the Future.

Low and Increasing Trajectories of Perpetration of Physical Dating Violence: 7-Year Associations with Suicidal Ideation, Weapons, and Substance Use.

PubMed

Orpinas, Pamela; Nahapetyan, Lusine; Truszczynski, Natalia

2017-05-01

Understanding the interrelation among problem behaviors and their change over time is fundamental for prevention research. The Healthy Teens Longitudinal Study followed a cohort of adolescents from Grades 6-12. Prior research identified two distinct trajectories of perpetration of physical dating violence: Low and Increasing. The purpose of this study was to examine whether adolescents in these two trajectories differed longitudinally on other problem behaviors: (1) suicidal ideation and attempts, (2) weapon-carrying and threats with a weapon, and (3) substance use, particularly alcohol and marijuana. The sample consisted of 588 randomly-selected students (52% males; 49% White, 36% Black, 12% Latino). Students completed a self-reported, computer-based survey each spring from Grades 6-12. To examine significant differences by perpetration of physical dating violence trajectory, we used Chi-square test and generalized estimating equations modeling. Across most grades, significantly more students in Increasing than in the Low trajectory reported suicidal ideation and attempts, carried a weapon, and threatened someone with a weapon. Adolescents in the Increasing trajectory also had higher trajectories of alcohol use, being drunk, and marijuana use than those in the Low trajectory. All differences were already significant in Grade 6. The difference in the rate of change between groups was not significant. This longitudinal study highlights that problem behaviors-physical dating violence, suicidal ideation and attempts, weapon carrying and threats, marijuana and alcohol use-cluster together as early as sixth grade and the clustering persists over time. The combination of these behaviors poses a great public health concern and highlight the need for early interventions.

Supplying the nuclear arsenal: Production reactor technology, management, and policy, 1942--1992

DOE Office of Scientific and Technical Information (OSTI.GOV)

Carlisle, R.P.; Zenzen, J.M.

1994-01-01

This book focuses on the lineage of America`s production reactors, those three at Hanford and their descendants, the reactors behind America`s nuclear weapons. The work will take only occasional sideways glances at the collateral lines of descent, the reactor cousins designed for experimental purposes, ship propulsion, and electric power generation. Over the decades from 1942 through 1992, fourteen American production reactors made enough plutonium to fuel a formidable arsenal of more than twenty thousand weapons. In the last years of that period, planners, nuclear engineers, and managers struggled over designs for the next generation of production reactors. The story ofmore » fourteen individual machines and of the planning effort to replace them might appear relatively narrow. Yet these machines lay at the heart of the nation`s nuclear weapons complex. The story of these machines is the story of arming the winning weapon, supplying the nuclear arms race. This book is intended to capture the history of the first fourteen production reactors, and associated design work, in the face of the end of the Cold War.« less

Fuel Fraction Analysis of 500 MWth Gas Cooled Fast Reactor with Nitride (UN-PuN) Fuel without Refueling

NASA Astrophysics Data System (ADS)

Dewi Syarifah, Ratna; Su'ud, Zaki; Basar, Khairul; Irwanto, Dwi

2017-01-01

Nuclear Power Plant (NPP) is one of candidates which can support electricity demand in the world. The Generation IV NPP has fourth main objective, i.e. sustainability, economics competitiveness, safety and reliability, and proliferation and physical protection. One of Gen-IV reactor type is Gas Cooled Fast Reactor (GFR). In this study, the analysis of fuel fraction in small GFR with nitride fuel has been done. The calculation was performed by SRAC code, both Pij and CITATION calculation. SRAC2002 system is a code system applicable to analyze the neutronics of variety reactor type. And for the data library used JENDL-3.2. The step of SRAC calculation is fuel pin calculated by Pij calculation until the data homogenized, after it homogenized we calculate core reactor. The variation of fuel fraction is 40% up to 65%. The optimum design of 500MWth GFR without refueling with 10 years burn up time reach when radius F1:F2:F3 = 50cm:30cm:30cm and height F1:F2:F3 = 50cm:40cm:30cm, variation percentage Plutonium in F1:F2:F3 = 7%:10%:13%. The optimum fuel fraction is 41% with addition 2% Plutonium weapon grade mix in the fuel. The excess reactivity value in this case 1.848% and the k-eff value is 1.01883. The high burn up reached when the fuel fraction is low. In this study 41% fuel fraction produce faster fissile fuel, so it has highest burn-up level than the other fuel fraction.

U, Pu, and Am nuclear signatures of the Thule hydrogen bomb debris.

PubMed

Eriksson, Mats; Lindahl, Patric; Roos, Per; Dahlgaard, Henning; Holm, Elis

2008-07-01

This study concerns an arctic marine environment that was contaminated by actinide elements after a nuclear accident in 1968, the so-called Thule accident In this study we have analyzed five isolated hot particles as well as sediment samples containing particles from the weapon material for the determination of the nuclear fingerprint of the accident. We report that the fissile material in the hydrogen weapons involved in the Thule accident was a mixture of highly enriched uranium and weapon-grade plutonium and that the main fissile material was 235U (about 4 times more than the mass of 239Pu). In the five hot particles examined, the measured uranium atomic ratio was 235U/238U = 1.02 +/- 0.16 and the Pu-isotopic ratios were as follows: 24Pu/239Pu = 0.0551 +/- 0.0008 (atom ratio), 238Pu/239+240Pu = 0.0161 +/- 0.0005 (activity ratio), 241Pu/239+240Pu = 0.87 +/- 0.12 (activity ratio), and 241Am/ 239+240Pu = 0.169 +/- 0.005 (activity ratio) (reference date 2001-10-01). From the activity ratios of 241Pu/241Am, we estimated the time of production of this weapon material to be from the late 1950s to the early 1960s. The results from reanalyzed bulk sediment samples showed the presence of more than one Pu source involved in the accident, confirming earlier studies. The 238Pu/239+240PU activity ratio and the 240Pu/ 239Pu atomic ratio were divided into at least two Pu-isotopic ratio groups. For both Pu-isotopic ratios, one ratio group had identical ratios as the five hot particles described above and for the other groups the Pu isotopic ratios were lower (238Pu/ 239+240PU activity ratio approximately 0.01 and the 240Pu/P239Pu atomic ratio 0.03). On the studied particles we observed that the U/Pu ratio decreased as a function of the time these particles were present in the sediment. We hypothesis that the decrease in the ratio is due to a preferential leaching of U relative to Pu from the particle matrix.

KSC-2011-7898

NASA Image and Video Library

2011-11-17

CAPE CANAVERAL, Fla. -- In the Vertical Integration Facility at Space Launch Complex-41 on Cape Canaveral Air Force Station, a turning fixture lowers the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission toward the radioisotope power system integration cart (RIC). Once the MMRTG is secured on the cart, it will be installed on the Curiosity rover. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is scheduled for Nov. 25. For more information, visit http://www.nasa.gov/msl. Photo credit: Department of Energy/Idaho National Laboratory

Study on Utilization of Super Grade Plutonium in Molten Salt Reactor FUJI-U3 using CITATION Code

NASA Astrophysics Data System (ADS)

Wulandari, Cici; Waris, Abdul; Pramuditya, Syeilendra; Asril, Pramutadi AM; Novitrian

2017-07-01

FUJI-U3 type of Molten Salt Reactor (MSR) has a unique design since it consists of three core regions in order to avoid the replacement of graphite as moderator. MSR uses floride as a nuclear fuel salt with the most popular chemical composition is LiF-BeF2-ThF4-233UF4. ThF4 and 233UF4 are the fertile and fissile materials, respectively. On the other hand, LiF and BeF2 working as both fuel and heat transfer medium. In this study, the super grade plutonium will be utilized as substitution of 233U since plutonium is easier to be obtained compared to 233U as main fuel. Neutronics calculation was performed by using PIJ and CITATION modules of SRAC 2002 code with JENDL 3.2 as nuclear data library.

Biomedical aspects of natural and manufactured environmental radioactivity

DOE Office of Scientific and Technical Information (OSTI.GOV)

Hodge, V.

1996-12-31

While weapons testing has altered natural radioactivity background, manufactured radioactivity in most parts of the world constitutes but a very small fraction of the total alpha, beta, and gamma radioactivity in soil, air, water, and the biota. For example, in the early 1970s, we found what appeared to be the highest natural concentration of radioactivity ever reported in fish while attempting to measure the manufactured plutonium ({sup 239}Pu and {sup 240}Pu) in organs of oceanic tuna. The natural alpha emitter polonium ({sup 210}Po) was discovered in the same organs at orders of magnitude higher concentrations. In particular, the caecum, whichmore » is a digestive organ composed of many small closed-ended sacs, contained concentrations of polonium as high as 79 pCi/g of wet tissue and lesser amounts of two manufactured isotopes: 0.0001 pCi/g of plutonium and 0.01 pCi/g of radiocesium ({sup 137}Cs). This equates to {approximately}80 rem/yr of radiation dose to this organ, overwhelmingly from the natural polonium, or {approximately}5000 times higher than is found in the human liver, the highest polonium concentration in man. The average background radiation for humans, for comparison, is {approximately}0.2 rem/yr, but the dose for Japanese, whose diet is high in seafood, is {approximately}15 rem/yr. The question arose: {open_quotes}Are these high concentrations of natural polonium limited to oceanic fish?{close_quotes} To answer this question, polonium was determined in the organs of striped bass and catfish from Lake Mead. In a related study, the plutonium and radiocesium ({sup 137}Cs) distributions in soils were determined to ascertain the impact of weapons testing on the natural background radioactivity of soils.« less

``Recycling'' Nuclear Power Plant Waste: Technical Difficulties and Proliferation Concerns

NASA Astrophysics Data System (ADS)

Lyman, Edwin

2007-04-01

One of the most vexing problems associated with nuclear energy is the inability to find a technically and politically viable solution for the disposal of long-lived radioactive waste. The U.S. plan to develop a geologic repository for spent nuclear fuel at Yucca Mountain in Nevada is in jeopardy, as a result of managerial incompetence, political opposition and regulatory standards that may be impossible to meet. As a result, there is growing interest in technologies that are claimed to have the potential to drastically reduce the amount of waste that would require geologic burial and the length of time that the waste would require containment. A scenario for such a vision was presented in the December 2005 Scientific American. While details differ, these technologies share a common approach: they require chemical processing of spent fuel to extract plutonium and other long-lived actinide elements, which would then be ``recycled'' into fresh fuel for advanced reactors and ``transmuted'' into shorter-lived fission products. Such a scheme is the basis for the ``Global Nuclear Energy Partnership,'' a major program unveiled by the Department of Energy (DOE) in early 2006. This concept is not new, but has been studied for decades. Major obstacles include fundamental safety issues, engineering feasibility and cost. Perhaps the most important consideration in the post-9/11 era is that these technologies involve the separation of plutonium and other nuclear weapon-usable materials from highly radioactive fission products, providing opportunities for terrorists seeking to obtain nuclear weapons. While DOE claims that it will only utilize processes that do not produce ``separated plutonium,'' it has offered no evidence that such technologies would effectively deter theft. It is doubtful that DOE's scheme can be implemented without an unacceptable increase in the risk of nuclear terrorism.

THE ATTRACTIVENESS OF MATERIAS ASSOCIATED WITH THORIUM-BASED NUCLEAR FUEL CYCLES FOR PHWRS

DOE Office of Scientific and Technical Information (OSTI.GOV)

Prichard, Andrew W.; Niehus, Mark T.; Collins, Brian A.

2011-07-17

This paper reports the continued evaluation of the attractiveness of materials mixtures containing special nuclear materials (SNM) associated with thorium based nuclear fuel cycles. Specifically, this paper examines a thorium fuel cycle in which a pressurized heavy water reactor (PHWR) is fueled with mixtures of natural uranium/233U/thorium. This paper uses a PHWR fueled with natural uranium as a base fuel cycle, and then compares material attractiveness of fuel cycles that use 233U/thorium salted with natural uranium. The results include the material attractiveness of fuel at beginning of life (BoL), end of life (EoL), and the number of fuel assemblies requiredmore » to collect a bare critical mass of plutonium or uranium. This study indicates what is required to render the uranium as having low utility for use in nuclear weapons; in addition, this study estimates the increased number of assemblies required to accumulate a bare critical mass of plutonium that has a higher utility for use in nuclear weapons. This approach identifies that some fuel cycles may be easier to implement the International Atomic Energy Agency (IAEA) safeguards approach and have a more effective safeguards by design outcome. For this study, approximately one year of fuel is required to be reprocessed to obtain one bare critical mass of plutonium. Nevertheless, the result of this paper suggests that all spent fuel needs to be rigorously safeguarded and provided with high levels of physical protection. This study was performed at the request of the United States Department of Energy /National Nuclear Security Administration (DOE/NNSA). The methodology and key findings will be presented.« less

Using Downhole Probes to Locate and Characterize Buried Transuranic and Mixed Low Level Waste

DOE Office of Scientific and Technical Information (OSTI.GOV)

Steinman, Donald K; Bramblett, Richard L; Hertzog, Russel C

2012-06-25

Borehole logging probes were developed and tested to locate and quantify transuranic elements in subsurface disposal areas and in contaminated sites at USDOE Weapons Complex sites. A new method of measuring very high levels of chlroine in the subsurface was developed using pulsed neutron technology from oilfield applications. The probes were demonstrated at the Hanford site in wells containing plutonium and other contaminants.

International Partnerships to Combat Weapons of Mass Destruction

DTIC Science & Technology

2008-05-01

public, plant , and animal), medicine , economics, law enforcement, and the scientific process itself—and thus engage a range of expert and stakeholder...OCCASIONAL PAPER 6 and replace them with fossil fuel plants ; a multilateral effort to dispose of 34 tons of Russian plutonium; and a number of...nonproliferation benefits: there is no technology ‘silver bullet’ that can be built into an enrichment plant or reprocessing plant that can prevent a

An independent evaluation of plutonium body burdens in populations near Los Alamos Laboratory using human autopsy data.

PubMed

Gaffney, Shannon H; Donovan, Ellen P; Shonka, Joseph J; Le, Matthew H; Widner, Thomas E

2013-06-01

In the mid-1940s, the United States began producing atomic weapon components at the Los Alamos National Laboratory (LANL). In an attempt to better understand historical exposure to nearby residents, this study evaluates plutonium activity in human tissue relative to residential location and length of time at residence. Data on plutonium activity in the lung, vertebrae, and liver of nearby residents were obtained during autopsies as a part of the Los Alamos Tissue Program. Participant residential histories and the distance from each residence to the primary plutonium processing buildings at LANL were evaluated in the analysis. Summary statistics, including Student t-tests and simple regressions, were calculated. Because the biological half-life of plutonium can vary significantly by organ, data were analyzed separately by tissue type (lung, liver, vertebrae). The ratios of plutonium activity (vertebrae:liver; liver:lung) were also analyzed in order to evaluate the importance of timing of exposure. Tissue data were available for 236 participants who lived in a total of 809 locations, of which 677 were verified postal addresses. Residents of Los Alamos were found to have higher plutonium activities in the lung than non-residents. Further, those who moved to Los Alamos before 1955 had higher lung activities than those who moved there later. These trends were not observed with the liver, vertebrae, or vertebrae:liver and liver:lung ratio data, however, and should be interpreted with caution. Although there are many limitations to this study, including the amount of available data and the analytical methods used to analyze the tissue, the overall results indicate that residence (defined as the year that the individual moved to Los Alamos) may have had a strong correlation to plutonium activity in human tissue. This study is the first to present the results of Los Alamos Autopsy Program in relation to residential status and location in Los Alamos. Copyright © 2012 Elsevier GmbH. All rights reserved.

What Lies Beneath Can Be Imaged

DOE Office of Scientific and Technical Information (OSTI.GOV)

Johnson, Tim

The Hanford Site was quickly established to help end World War II, making history for producing the plutonium used in the world’s first nuclear weapons. Throughout the Cold War years, Hanford employees produced plutonium for most of the more than 60,000 weapons in the U.S. nuclear arsenal stockpile. Today, the once highly active nuclear reactors are shut down. And the mission at Hanford turned full-circle as scientists, engineers and specialists work to clean up our nation’s most contaminated nuclear site. PNNL Computational Geophysicist Tim Johnson is helping decision-makers understand the complexity and breadth of the contamination in soils at Hanford.more » Tim and others are applying remote, high-resolution geophysical imaging to determine the extent of contamination in the soil below the surface and understand the processes controlling its movement. They also provide real-time imaging of remediation processes that are working to limit the movement of contaminants below the surface and toward water resources. Geophysical imaging simply means that PNNL scientists are combining the techniques of geology, physics, mathematics and chemistry with supercomputer modeling to create three-dimensional images of the waste and its movement. These real-time, remote images are essential in reducing the uncertainty associated with cleanup costs and remediation technologies.« less

Measurement of 240Pu/239Pu isotopic ratios in soils from the Marshall Islands using ICP-MS.

PubMed

Muramatsu, Y; Hamilton, T; Uchida, S; Tagami, K; Yoshida, S; Robison, W

2001-10-20

Nuclear weapons tests conducted by the United States in the Marshall Islands produced significant quantities of regional or tropospheric fallout contamination. Here we report on some preliminary inductively coupled plasma-mass spectrometry (ICP-MS) measurements of plutonium isolated from seven composite soil samples collected from Bikini, Enewetak and Rongelap Atolls in the northern Marshall Islands. These data show that 240Pu/239Pu isotopic signatures in surface soils from the Marshall Island vary significantly and could potentially be used to help quantify the range and extent of fallout deposition (and associated impacts) from specific weapons tests. 137Cs and 60Co were also determined on the same set of soil samples for comparative purposes.

Preliminary study on weapon grade uranium utilization in molten salt reactor miniFUJI

NASA Astrophysics Data System (ADS)

Aji, Indarta Kuncoro; Waris, A.

2014-09-01

Preliminary study on weapon grade uranium utilization in 25MWth and 50MWth of miniFUJI MSR (molten salt reactor) has been carried out. In this study, a very high enriched uranium that we called weapon grade uranium has been employed in UF4 composition. The 235U enrichment is 90 - 95 %. The results show that the 25MWth miniFUJI MSR can get its criticality condition for 1.56 %, 1.76%, and 1.96% of UF4 with 235U enrichment of at least 93%, 90%, and 90%, respectively. In contrast, the 50 MWth miniFUJI reactor can be critical for 1.96% of UF4 with 235U enrichment of at smallest amount 95%. The neutron spectra are almost similar for each power output.

SLIGHTLY IRRADIATED FUEL (SIF) INTERIM DISPOSITION PROJECT

DOE Office of Scientific and Technical Information (OSTI.GOV)

NORTON SH

2010-02-23

CH2M HILL Plateau Remediation Company (CH2M HILL PRC) is proud to submit the Slightly Irradiated Fuel (SIF) Interim Disposition Project for consideration by the Project Management Institute as Project of the Year for 2010. The SIF Project was a set of six interrelated sub-projects that delivered unique stand-alone outcomes, which, when integrated, provided a comprehensive and compliant system for storing high risk special nuclear materials. The scope of the six sub-projects included the design, construction, testing, and turnover of the facilities and equipment, which would provide safe, secure, and compliant Special Nuclear Material (SNM) storage capabilities for the SIF material.more » The project encompassed a broad range of activities, including the following: Five buildings/structures removed, relocated, or built; Two buildings renovated; Structural barriers, fencing, and heavy gates installed; New roadways and parking lots built; Multiple detection and assessment systems installed; New and expanded communication systems developed; Multimedia recording devices added; and A new control room to monitor all materials and systems built. Project challenges were numerous and included the following: An aggressive 17-month schedule to support the high-profile Plutonium Finishing Plant (PFP) decommissioning; Company/contractor changeovers that affected each and every project team member; Project requirements that continually evolved during design and construction due to the performance- and outcome-based nature ofthe security objectives; and Restrictions imposed on all communications due to the sensitive nature of the projects In spite of the significant challenges, the project was delivered on schedule and $2 million under budget, which became a special source of pride that bonded the team. For years, the SIF had been stored at the central Hanford PFP. Because of the weapons-grade piutonium produced and stored there, the PFP had some of the tightest security on the Hanford nuclear reservation. Workers had to pass through metal detectors when they arrived at the plant and materials leaving the plant had to be scanned for security reasons. Whereas other high-security nuclear materials were shipped from the PFP to Savannah River, S.C. as part ofa Department of Energy (DOE) program to consolidate weapons-grade plutonium, it was determined that the SIF should remain onsite pending disposition to a national repository. Nevertheless, the SIF still requires a high level of security that the PFP complex has always provided. With the 60-year PFP mission of producing and storing plutonium concluded, the environmental cleanup plans for Hanford call for the demolition of the 63-building PFP complex. Consequently, if the SIF remained at PFP it not only would have interfered with the environmental cleanup plans, but would have required $100 million in facility upgrades to meet increased national security requirements imposed after the 9/11 terrorist attacks. A new smaller and more cost-effective area was needed to store this material, which led to the SIF Project. Once the SIF project was successfully completed and the SIF was safely removed from PFP, the existing Protected Area at PFP could be removed, and demolition could proceed more quickly without being encumbered by restrictive security requirements that an active Protected Area requires. The lightened PFP security level brought by safely removing and storing the SIF would also yield lowered costs for deactivation and demolition, as well as reduce overall life-cycle costs.« less

Past Exposure to Densely Ionizing Radiation Leaves a Unique Permanent Signature in the Genome

PubMed Central

Hande, M. Prakash; Azizova, Tamara V.; Geard, Charles R.; Burak, Ludmilla E.; Mitchell, Catherine R.; Khokhryakov, Valentin F.; Vasilenko, Evgeny K.; Brenner, David J.

2003-01-01

Speculation has long surrounded the question of whether past exposure to ionizing radiation leaves a unique permanent signature in the genome. Intrachromosomal rearrangements or deletions are produced much more efficiently by densely ionizing radiation than by chemical mutagens, x-rays, or endogenous aging processes. Until recently, such stable intrachromosomal aberrations have been very hard to detect, but a new chromosome band painting technique has made their detection practical. We report the detection and quantification of stable intrachromosomal aberrations in lymphocytes of healthy former nuclear-weapons workers who were exposed to plutonium many years ago. Even many years after occupational exposure, more than half the blood cells of the healthy plutonium workers contain large (>6 Mb) intrachromosomal rearrangements. The yield of these aberrations was highly correlated with plutonium dose to the bone marrow. The control groups contained very few such intrachromosomal aberrations. Quantification of this large-scale chromosomal damage in human populations exposed many years earlier will lead to new insights into the mechanisms and risks of cytogenetic damage. PMID:12679897

Independent verification of plutonium decontamination on Johnston Atoll (1992--1996)

DOE Office of Scientific and Technical Information (OSTI.GOV)

Wilson-Nichols, M.J.; Wilson, J.E.; McDowell-Boyer, L.M.

1998-05-01

The Field Command, Defense Special Weapons Agency (FCDSWA) (formerly FCDNA) contracted Oak Ridge National Laboratory (ORNL) Environmental Technology Section (ETS) to conduct an independent verification (IV) of the Johnston Atoll (JA) Plutonium Decontamination Project by an interagency agreement with the US Department of Energy in 1992. The main island is contaminated with the transuranic elements plutonium and americium, and soil decontamination activities have been ongoing since 1984. FCDSWA has selected a remedy that employs a system of sorting contaminated particles from the coral/soil matrix, allowing uncontaminated soil to be reused. The objective of IV is to evaluate the effectiveness ofmore » remedial action. The IV contractor`s task is to determine whether the remedial action contractor has effectively reduced contamination to levels within established criteria and whether the supporting documentation describing the remedial action is adequate. ORNL conducted four interrelated tasks from 1992 through 1996 to accomplish the IV mission. This document is a compilation and summary of those activities, in addition to a comprehensive review of the history of the project.« less

Plutonium isotopes in the Hungarian environment.

PubMed

Varga, Beata; Tarján, Sandor; Vajda, Nora

2008-04-01

More than 50 soil samples were analysed from different parts of the country, the activity concentration of 239+240Pu was in the range of 0.01-0.84 Bq/kg dry soil with the average of 0.10 Bq/kg. 238Pu could be detected only in few moss samples and 238Pu/239+240Pu ratio determines the origin of plutonium. 241Pu was determined by liquid scintillation spectrometry. The activity concentration of this isotope in the soil is between 0.04 and 3.74 Bq/kg with the average of 0.82 Bq/kg, while in the moss is also similar 0.01-2.07 Bq/kg fresh mass with the average of 0.43 Bq/kg. Significant difference could not be observed between the different types of soils occurring in the country, but the results could be sorted according to the sampling carried out on undisturbed or cultivated area. The isotope ratios 241Pu/239+240Pu prove that the origin of the plutonium in Hungary is the global fallout determined by the atmospheric nuclear weapon tests.

The Military Significance of Small Uranium Enrichment Facilities Fed with Low-Enrichment Uranium (Redacted)

DTIC Science & Technology

1969-12-01

a five-year supply of enriched uranium for reactor fuel . Nevertheless, it seems clear that some foreign enrichment developments are approaching a...produc- tion of fissile material could powerfully influence the assessment of risks and benefits of a nuclear weapons development program . Since... program is likely to include the production of its own relatively pure fissile plutonium. This would involve more rapid cycling and reprocessing of fuel

Atoms for peace and the nonproliferation treaty: unintended consequences

DOE Office of Scientific and Technical Information (OSTI.GOV)

Streeper, Charles Blamires

2009-01-01

In April 2009, President Obama revived nonproliferation and arms control efforts with a speech calling for the worldwide abolition of nuclear weapons. His speech correctly acknowledged the threat of nuclear terrorism and the vulnerabilities of the related unsecure nuclear materials. Unfortunately, the president did not mention and has not mentioned in any speech the threat posed by at-risk radiological materials. Nonproliferation efforts have a well documented history of focus on special nuclear materials (fissionable weapons usable materials or SNM), and other key materials (chemical and biological) and technologies for a Weapon of Mass Destruction (WMD). Such intense focus on WMDmore » related materials/technologies is essential for international safety and security and merit continued attention and funding. However, the perception that radioactive sealed sources (sources) are of less concern than WMD is unfortunate. These perceptions are based solely on the potentially enormous and tragic consequences associated with their deliberate or accidental misuse and proliferation concerns. However, there is a documented history of overemphasis on the nuclear threat at the expense of ignoring the far more likely and also devastating chemical and biological threats. The radiological threat should not be minimized or excluded from policy discussions and decisions on these far ranging scopes of threat to the international community. Sources have a long history of use; and a wider distribution worldwide than fissile materials. Pair this with their broad ranges in isotopes/activities along with scant national and international attention and mechanisms for their safe and secure management and it is not difficult to envision a deadly threat. Arguments that minimize or divert attention away from sources may have the effect of distracting necessary policy attention on preventing/mitigating a radiological dispersal event. The terrorist attacks on 9/11 should be a clear reminder of the inherent danger of diminishing or dismissing lower-level threats in exchange for enhanced focus on high priority special nuclear materials with the basis for this emphasis being solely on the magnitude of the consequences of a single event. Mitigating all possible or likely terrorist attacks is impossible; however, weaponized sources, in the form of a radiological dispersal device, have been a declared target material of Al-Qaida. Eisenhower's Atoms for Peace initiative promoted the spread of the paradoxical beneficial yet destructive properties of the atom. Typically, the focus of nonproliferation efforts focuses on the fissile materials associated with Weapons of Mass Destruction, with less emphasis on radioactive materials that could be used for a Weapon of Mass Disruption. Most nonproliferation policy discussion involves securing or preventing the diversion of weapons grade fissile materials (uranium (U) with concentration of over 90% of the isotope {sup 235}U (HEU) and plutonium with more than 90% of the isotope {sup 239}Pu), with scant attention given to the threat posed by a prolific quantity of sources spread worldwide. Further acerbating the problem of inattention, it appears that the momentum of the continued evolution in the beneficial applications of sources will only increase in the near future. Several expert studies have demonstrated on the potentially devastating economic, psychological and public health impacts of terrorist use of a radiological dispersal or radiation emitting device (ROD/RED) in a metropolis. The development of such a weapon, from the acquisition of the radioactive material to the technical knowledge needed to fashion it into an ROD, is many orders of magnitude easier than diverting enough fissile material for and fabrication/acquisition of a nuclear weapon. Unlike nuclear weapons, worldwide, there are many well documented accounts of accidental and purposeful diversions of radioactive materials from regulatory control. As of the end of 2008, the International Atomic Energy Agency's (IAEA) Illicit Trafficking Database had logged 1562 incidents, of which only 18 include weapons grade nuclear materials. As much as 66% of the radioactive material involved in these incidents was not recovered. Since 2004, there has been a 75% increase in incidents of unrecoverable material, much of which is labeled dangerous with potential for deterministic health affects if misused. This makes clear that a black market of illicit trade in sources exists. The incidents reported to the IAEA's database rely only on voluntary state reporting; therefore, the number of lost or stolen sources is expected to be much higher.« less

An Iranium bomb?

DOE Office of Scientific and Technical Information (OSTI.GOV)

Albright, D.

1995-07-01

This year, the nuclear proliferation spotlight has swung away from Iraq and North Korea, only to focus on Iran. Western intelligence agencies have assembled a substantial body of evidence suggesting that, although Iran signed the Nuclear Non-Proliferation Treaty (NPT), it is secretly pursuing a broad, organized effort to develop nuclear weapons. US officials say that Iran is attempting to acquire nuclear technologies that are not consistent with a strictly peaceful program. Intelligence agencies have detected procurement patterns that point to a weapons program. Iran has a multifaceted strategy to develop options to make nuclear weapons: Iran has sought, with limitedmore » success, to buy nuclear power and research facilities from many countries, particularly China and Russia; Iran has shopped quietly in many countries, particularly in Western and Eastern Europe, for a wide range of nuclear-related or dual-use nuclear items that might enable it to put together facilities to enrich uranium, separate plutonium, and make nuclear weapons. There is little public information about how effective this clandestine shopping has been or which countries have been contacted; There is no evidence that Iran has bought any fissile material - but not for wont of trying, and the matter continues to be scrutinized very closely.« less

Preliminary study on weapon grade uranium utilization in molten salt reactor miniFUJI

DOE Office of Scientific and Technical Information (OSTI.GOV)

Aji, Indarta Kuncoro; Waris, A., E-mail: awaris@fi.itb.ac.id

Preliminary study on weapon grade uranium utilization in 25MWth and 50MWth of miniFUJI MSR (molten salt reactor) has been carried out. In this study, a very high enriched uranium that we called weapon grade uranium has been employed in UF{sub 4} composition. The {sup 235}U enrichment is 90 - 95 %. The results show that the 25MWth miniFUJI MSR can get its criticality condition for 1.56 %, 1.76%, and 1.96% of UF{sub 4} with {sup 235}U enrichment of at least 93%, 90%, and 90%, respectively. In contrast, the 50 MWth miniFUJI reactor can be critical for 1.96% of UF{sub 4}more » with {sup 235}U enrichment of at smallest amount 95%. The neutron spectra are almost similar for each power output.« less

Characterizing subcritical assemblies with time of flight fixed by energy estimation distributions

NASA Astrophysics Data System (ADS)

Monterial, Mateusz; Marleau, Peter; Pozzi, Sara

2018-04-01

We present the Time of Flight Fixed by Energy Estimation (TOFFEE) as a measure of the fission chain dynamics in subcritical assemblies. TOFFEE is the time between correlated gamma rays and neutrons, subtracted by the estimated travel time of the incident neutron from its proton recoil. The measured subcritical assembly was the BeRP ball, a 4.482 kg sphere of α-phase weapons grade plutonium metal, which came in five configurations: bare, 0.5, 1, and 1.5 in iron, and 1 in nickel closed fitting shell reflectors. We extend the measurement with MCNPX-PoliMi simulations of shells ranging up to 6 inches in thickness, and two new reflector materials: aluminum and tungsten. We also simulated the BeRP ball with different masses ranging from 1 to 8 kg. A two-region and single-region point kinetics models were used to model the behavior of the positive side of the TOFFEE distribution from 0 to 100 ns. The single region model of the bare cases gave positive linear correlations between estimated and expected neutron decay constants and leakage multiplications. The two-region model provided a way to estimate neutron multiplication for the reflected cases, which correlated positively with expected multiplication, but the nature of the correlation (sub or superlinear) changed between material types. Finally, we found that the areal density of the reflector shells had a linear correlation with the integral of the two-region model fit. Therefore, we expect that with knowledge of reflector composition, one could determine the shell thickness, or vice versa. Furthermore, up to a certain amount and thickness of the reflector, the two-region model provides a way of distinguishing bare and reflected plutonium assemblies.

Source-dependent and source-independent controls on plutonium oxidation state and colloid associations in groundwater.

PubMed

Buesseler, Ken O; Kaplan, Daniel I; Dai, Minhan; Pike, Steven

2009-03-01

Plutonium (Pu) was characterized for its isotopic composition, oxidation states, and association with colloids in groundwater samples near disposal basins in F-Area of the Savannah River Site and compared to similar samples collected six years earlier. Two sources of Pu were identified, the disposal basins, which contained a 24Pu/l39Pu isotopic signature consistent with weapons grade Pu, and 244Cm, a cocontaminant that is a progenitor radionuclide of 24Pu. 24Pu that originated primarily from 244Cm tended to be appreciably more oxidized (Pu(V/VI)), less associated with colloids (approximately 1 kDa - 0.2 microm), and more mobile than 239Pu, as suggested by our prior studies at this site. This is not evidence of isotope fractionation but rather "source-dependent" controls on 240Pu speciation which are processes that are not at equilibrium, i.e., processes that appear kinetically hindered. There were also "source-independent" controls on 239Pu speciation, which are those processes that follow thermodynamic equilibrium with their surroundings. For example, a groundwater pH increase in one well from 4.1 in 1998 to 6.1 in 2004 resulted in an order of magnitude decrease in groundwater 239Pu concentrations. Similarly, the fraction of 239Pu in the reduced Pu(III/IV) and colloidal forms increased systematically with decreases in redox condition in 2004 vs 1998. This research demonstrates the importance of source-dependent and source-independent controls on Pu speciation which would impact Pu mobility during changes in hydrological, chemical, or biological conditions on both seasonal and decadal time scales, and over short spatial scales. This implies more dynamic shifts in Pu speciation, colloids association, and transport in groundwater than commonly believed.

Preliminary results of calculations for heavy-water nuclear-power-plant reactors employing 235U, 233U, and 232Th as a fuel and meeting requirements of a nonproliferation of nuclear weapons

NASA Astrophysics Data System (ADS)

Ioffe, B. L.; Kochurov, B. P.

2012-02-01

A physical design is developed for a gas-cooled heavy-water nuclear reactor intended for a project of a nuclear power plant. As a fuel, the reactor would employ thorium with a small admixture of enriched uranium that contains not more than 20% of 235U. It operates in the open-cycle mode involving 233U production from thorium and its subsequent burnup. The reactor meets the conditions of a nonproliferation of nuclear weapons: the content of fissionable isotopes in uranium at all stages of the process, including the final one, is below the threshold for constructing an atomic bomb, the amount of product plutonium being extremely small.

A fast semi-quantitative method for Plutonium determination in an alpine firn/ice core

NASA Astrophysics Data System (ADS)

Gabrieli, J.; Cozzi, G.; Vallelonga, P.; Schwikowski, M.; Sigl, M.; Boutron, C.; Barbante, C.

2009-04-01

Plutonium is present in the environment as a consequence of atmospheric nuclear tests carried out in the 1960s, nuclear weapons production and releases by the nuclear industry over the past 50 years. Plutonium, unlike uranium, is essentially anthropogenic and it was first produced and isolated in 1940 by deuteron bombardment of uranium in the cyclotron of Berkeley University. It exists in five main isotopes, 238Pu, 239Pu, 240Pu, 241Pu, 242Pu, derived from civilian and military sources (weapons production and detonation, nuclear reactors, nuclear accidents). In the environment, 239Pu is the most abundant isotope. Approximately 6 tons of 239Pu have been released into the environment as a result of 541 atmospheric weapon tests Nuclear Pu fallout has been studied in various environmental archives, such as sediments, soil and herbarium grass. Mid-latitude ice cores have been studied as well, on Mont Blanc, the Western Alps and on Belukha Glacier, Siberian Altai. We present a Pu record obtained by analyzing 52 discrete samples of an alpine firn/ice core from Colle Gnifetti (M. Rosa, 4450 m a.s.l.), dating from 1945 to 1991. The239Pu signal was recorded directly, without preliminary cleaning or preconcentration steps, using an ICP-SFMS (Thermo Element2) equipped with a desolvation system (APEX). 238UH+ interferences were negligible for U concentrations lower than 50 ppt as verified both in spiked fresh snow and pre-1940 ice samples. The shape of 239Pu profile reflects the three main periods of atmospheric nuclear weapons testing: the earliest peak starts in 1954/55 to 1958 and includes the first testing period which reached a maximum in 1958. Despite a temporary halt in testing in 1959/60, the Pu concentration decreased only by half with respect to the 1958 peak. In 1961/62 Pu concentrations rapidly increased reaching a maximum in 1963, which was about 40% more intense than the 1958 peak. After the sign of the "Limited Test Ban Treaty" between USA and URSS in 1964, Pu deposition decreased very sharply reaching a minimum in 1967. The third period (1967-1975) is characterized by irregular Pu profiles with smaller peaks (about 20-30% compared to the 1964 peak) which could be due to French and Chinese tests. Comparison with the Pu profiles obtained from the Col du Dome and Belukha ice cores by AMS (Accelerator Mass Spectrometry) shows very good agreement. Considering the semi-quantitative method and the analytical uncertainty, the results are also quantitatively comparable. However, the Pu concentrations at Colle Gnifetti are normally 2-3 times greater than in Col du Dome. This could be explained by different air mass transport or, more likely, different accumulation rates at each site.

2. VIEW LOOKING NORTHEAST AT BUILDING 444 UNDER CONSTRUCTION. BUILDING ...

Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

2. VIEW LOOKING NORTHEAST AT BUILDING 444 UNDER CONSTRUCTION. BUILDING 444 WAS THE PRIMARY NON-PLUTONIUM MANUFACTURING FACILITY AT THE ROCKY FLATS PLANT. MANUFACTURING PROCESSES COMPLETED IN THIS BUILDING WERE USED TO FABRICATE WEAPONS COMPONENTS AND ASSEMBLIES FOR A VARIETY OF MATERIALS, INCLUDING DEPLETED URANIUM, BERYLLIUM, STAINLESS STEEL, ALUMINUM, AND VANADIUM. (4/25/52) - Rocky Flats Plant, Non-Nuclear Production Facility, South of Cottonwood Avenue, west of Seventh Avenue & east of Building 460, Golden, Jefferson County, CO

Characterization of Representative Materials in Support of Safe, Long Term Storage of Surplus Plutonium in DOE-STD-3013 Containers

DOE Office of Scientific and Technical Information (OSTI.GOV)

Narlesky, Joshua E.; Stroud, Mary Ann; Smith, Paul Herrick

2013-02-15

The Surveillance and Monitoring Program is a joint Los Alamos National Laboratory/Savannah River Site effort funded by the Department of Energy-Environmental Management to provide the technical basis for the safe, long-term storage (up to 50 years) of over 6 metric tons of plutonium stored in over 5,000 DOE-STD-3013 containers at various facilities around the DOE complex. The majority of this material is plutonium that is surplus to the nuclear weapons program, and much of it is destined for conversion to mixed oxide fuel for use in US nuclear power plants. The form of the plutonium ranges from relatively pure metalmore » and oxide to very impure oxide. The performance of the 3013 containers has been shown to depend on moisture content and on the levels, types and chemical forms of the impurities. The oxide materials that present the greatest challenge to the storage container are those that contain chloride salts. Other common impurities include oxides and other compounds of calcium, magnesium, iron, and nickel. Over the past 15 years the program has collected a large body of experimental data on 54 samples of plutonium, with 53 chosen to represent the broader population of materials in storage. This paper summarizes the characterization data, moisture analysis, particle size, surface area, density, wattage, actinide composition, trace element impurity analysis, and shelf life surveillance data and includes origin and process history information. Limited characterization data on fourteen nonrepresentative samples is also presented.« less

Characterization of representative materials in support of safe, long term storage of surplus plutonium in DOE-STD-3013 containers

DOE Office of Scientific and Technical Information (OSTI.GOV)

Smith, Paul H; Narlesky, Joshua E; Worl, Laura A

2010-01-01

The Surveillance and Monitoring Program (SMP) is a joint LANL/SRS effort funded by DOE/EM to provide the technical basis for the safe, long-term storage (up to 50 years) of over 6 metric tons of plutonium stored in over 5000 DOE-STD-3013 containers at various facilities around the DOE complex. The majority of this material is plutonium that is surplus to the nuclear weapons program, and much of it is destined for conversion to mixed oxide fuel for use in US nuclear power plants. The form of the plutonium ranges from relatively pure metal and oxide to very impure oxide. The performancemore » of the 3013 containers has been shown to depend on moisture content and on the levels, types and chemical forms of the impurities. The oxide materials that present the greatest challenge to the storage container are those that contain chloride salts. The chlorides (NaCl, KCl, CaCl{sub 2}, and MgCl{sub 2}) range from less than half of the impurities present to nearly all the impurities. Other common impurities include oxides and other compounds of calcium, magnesium, iron, and nickel. Over the past 15 years the program has collected a large body of experimental data on over 60 samples of plutonium chosen to represent the broader population of materials in storage. This paper will summarize the characterization data, including the origin and process history, particle size, surface area, density, calorimetry, chemical analysis, moisture analysis, prompt gamma, gas generation and corrosion behavior.« less

Vertical and horizontal fluxes of plutonium and americium in the western Mediterranean and the Strait of Gibraltar.

PubMed

León Vintró, L; Mitchell, P I; Condren, O M; Downes, A B; Papucci, C; Delfanti, R

1999-09-30

New data on the vertical distributions of plutonium and americium in the waters of the western Mediterranean and the Strait of Gibraltar are examined in terms of the processes governing their delivery to, transport in and removal from the water column within the basin. Residence times for plutonium and americium in surface waters of approximately 15 and approximately 3 years, respectively, are deduced, and it is shown that by the mid 1990s only approximately 35% of the 239,240Pu and approximately 5% of the 241Am deposited as weapons fallout still resided in the water column. Present 239,240Pu inventories in the water column and the underlying sediments are estimated to be approximately 25 TBq and approximately 40 TBq, respectively, which reconcile well with the time-integrated fallout deposition in this zone, taken to be approximately 69 TBq. The data show that there are significant net outward fluxes of plutonium and americium from the basin through the Strait of Gibraltar at the present time. These appear to be compensated by net inward fluxes of similar magnitude through the Strait of Sicily. Thus, the time-integrated fallout deposition in the western basin can be accounted for satisfactorily in terms of present water column and sediment inventories. Enhanced scavenging on the continental shelves, as evidenced by the appreciably higher transuranic concentrations in shelf sediments, supports this contention.

Uncovering Special Nuclear Materials by Low-energy Nuclear Reaction Imaging

NASA Astrophysics Data System (ADS)

Rose, P. B.; Erickson, A. S.; Mayer, M.; Nattress, J.; Jovanovic, I.

2016-04-01

Weapons-grade uranium and plutonium could be used as nuclear explosives with extreme destructive potential. The problem of their detection, especially in standard cargo containers during transit, has been described as “searching for a needle in a haystack” because of the inherently low rate of spontaneous emission of characteristic penetrating radiation and the ease of its shielding. Currently, the only practical approach for uncovering well-shielded special nuclear materials is by use of active interrogation using an external radiation source. However, the similarity of these materials to shielding and the required radiation doses that may exceed regulatory limits prevent this method from being widely used in practice. We introduce a low-dose active detection technique, referred to as low-energy nuclear reaction imaging, which exploits the physics of interactions of multi-MeV monoenergetic photons and neutrons to simultaneously measure the material’s areal density and effective atomic number, while confirming the presence of fissionable materials by observing the beta-delayed neutron emission. For the first time, we demonstrate identification and imaging of uranium with this novel technique using a simple yet robust source, setting the stage for its wide adoption in security applications.

Uncovering Special Nuclear Materials by Low-energy Nuclear Reaction Imaging

DOE Office of Scientific and Technical Information (OSTI.GOV)

Rose, Jr., P. B.; Erickson, A. S.; Mayer, Michael F.

Weapons-grade uranium and plutonium could be used as nuclear explosives with extreme destructive potential. The problem of their detection, especially in standard cargo containers during transit, has been described as “searching for a needle in a haystack” because of the inherently low rate of spontaneous emission of characteristic penetrating radiation and the ease of its shielding. Currently, the only practical approach for uncovering well-shielded special nuclear materials is by use of active interrogation using an external radiation source. However, the similarity of these materials to shielding and the required radiation doses that may exceed regulatory limits prevent this method frommore » being widely used in practice. We introduce a low-dose active detection technique, referred to as low-energy nuclear reaction imaging, which exploits the physics of interactions of multi-MeV monoenergetic photons and neutrons to simultaneously measure the material’s areal density and effective atomic number, while confirming the presence of fissionable materials by observing the beta-delayed neutron emission. For the first time, we demonstrate identification and imaging of uranium with this novel technique using a simple yet robust source, setting the stage for its wide adoption in security applications.« less

Uncovering Special Nuclear Materials by Low-energy Nuclear Reaction Imaging

DOE PAGES

Rose, P. B.; Erickson, A. S.; Mayer, M.; ...

2016-04-18

Weapons-grade uranium and plutonium could be used as nuclear explosives with extreme destructive potential. The problem of their detection, especially in standard cargo containers during transit, has been described as “searching for a needle in a haystack” because of the inherently low rate of spontaneous emission of characteristic penetrating radiation and the ease of its shielding. Currently, the only practical approach for uncovering well-shielded special nuclear materials is by use of active interrogation using an external radiation source. However, the similarity of these materials to shielding and the required radiation doses that may exceed regulatory limits prevent this method frommore » being widely used in practice. We introduce a low-dose active detection technique, referred to as low-energy nuclear reaction imaging, which exploits the physics of interactions of multi-MeV monoenergetic photons and neutrons to simultaneously measure the material’s areal density and effective atomic number, while confirming the presence of fissionable materials by observing the beta-delayed neutron emission. For the first time, we demonstrate identification and imaging of uranium with this novel technique using a simple yet robust source, setting the stage for its wide adoption in security applications.« less

KSC-2011-7835

NASA Image and Video Library

2011-11-17

CAPE CANAVERAL, Fla. -- Enclosed in the protective mesh container known as the "gorilla cage," the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission is lifted up the side of the Vertical Integration Facility at Space Launch Complex 41. The generator will be installed on the MSL spacecraft, encapsulated within the payload fairing. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat produced by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Heat emitted by the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Dimitri Gerondidakis

KSC-2011-7829

NASA Image and Video Library

2011-11-17

CAPE CANAVERAL, Fla. -- The Atlas V rocket set to launch NASA's Mars Science Laboratory (MSL) mission is illuminated inside the Vertical Integration Facility at Space Launch Complex 41, where employees have gathered to hoist the spacecraft's multi-mission radioisotope thermoelectric generator (MMRTG). The generator will be lifted up to the top of the rocket and installed on the MSL spacecraft, encapsulated within the payload fairing. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat produced by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Heat emitted by the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Dimitri Gerondidakis

KSC-2011-6715

NASA Image and Video Library

2011-07-13

CAPE CANAVERAL, Fla. -- In the Payload Hazardous Servicing Facility at NASA's Kennedy Space Center in Florida, spacecraft technicians from NASA's Jet Propulsion Laboratory park the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission on its support base in the airlock following the MMRTG fit check on the Curiosity rover in the high bay. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Kim Shiflett

KSC-2011-6731

NASA Image and Video Library

2011-07-14

CAPE CANAVERAL, Fla. -- At NASA's Kennedy Space Center in Florida, the trailer transporting the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission arrives at the RTG storage facility (RTGF). The MMRTG is returning to the RTGF following a fit check on MSL's Curiosity rover in the Payload Hazardous Servicing Facility (PHSF). The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Troy Cryder

KSC-2011-6710

NASA Image and Video Library

2011-07-13

CAPE CANAVERAL, Fla. -- In the high bay of the Payload Hazardous Servicing Facility at NASA's Kennedy Space Center in Florida, a spacecraft technician from NASA's Jet Propulsion Laboratory conducts a visual inspection of the cooling tubes on the exterior of the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission following the MMRTG fit check on the Curiosity rover. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Kim Shiflett

KSC-2011-7827

NASA Image and Video Library

2011-11-17

CAPE CANAVERAL, Fla. -- Outside the Vertical Integration Facility at Space Launch Complex 41, an area has been cordoned off beside the trailer which has arrived at the pad carrying the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission. The generator will be lifted up to the top of the rocket and installed on the MSL spacecraft, encapsulated within the payload fairing. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat produced by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Heat emitted by the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Dimitri Gerondidakis

KSC-2011-6709

NASA Image and Video Library

2011-07-13

CAPE CANAVERAL, Fla. -- In the high bay of the Payload Hazardous Servicing Facility at NASA's Kennedy Space Center in Florida, the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission is positioned on a support base with the aid of a turning fixture following the MMRTG fit check on the Curiosity rover. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Kim Shiflett

KSC-2011-6713

NASA Image and Video Library

2011-07-13

CAPE CANAVERAL, Fla. -- In the high bay of the Payload Hazardous Servicing Facility at NASA's Kennedy Space Center in Florida, a spacecraft technician from NASA's Jet Propulsion Laboratory conducts a visual inspection of the cooling tubes on the exterior of the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission following the MMRTG fit check on the Curiosity rover. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Kim Shiflett

KSC-2011-6707

NASA Image and Video Library

2011-07-13

CAPE CANAVERAL, Fla. -- In the high bay of the Payload Hazardous Servicing Facility at NASA's Kennedy Space Center in Florida, the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission is lowered onto a support base with the aid of a turning fixture following the MMRTG fit check on the Curiosity rover. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Kim Shiflett

KSC-2011-7836

NASA Image and Video Library

2011-11-17

CAPE CANAVERAL, Fla. -- Enclosed in the protective mesh container known as the "gorilla cage," the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission is hoisted up beside the Atlas V rocket standing in the Vertical Integration Facility at Space Launch Complex 41. The generator will be installed on the MSL spacecraft, encapsulated within the payload fairing. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat produced by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Heat emitted by the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Dimitri Gerondidakis

KSC-2011-6732

NASA Image and Video Library

2011-07-14

CAPE CANAVERAL, Fla. -- At the RTG storage facility (RTGF) at NASA's Kennedy Space Center in Florida, preparations are under way to offload the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission from the MMRTG trailer. The MMRTG is returning to the RTGF following a fit check on MSL's Curiosity rover in the Payload Hazardous Servicing Facility (PHSF). The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Troy Cryder

KSC-2011-6714

NASA Image and Video Library

2011-07-13

CAPE CANAVERAL, Fla. -- In the Payload Hazardous Servicing Facility at NASA's Kennedy Space Center in Florida, spacecraft technicians from NASA's Jet Propulsion Laboratory roll the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission on its support base from the high bay into the airlock following the MMRTG fit check on the Curiosity rover. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Kim Shiflett

KSC-2011-7833

NASA Image and Video Library

2011-11-17

CAPE CANAVERAL, Fla. -- Enclosed in the protective mesh container known as the "gorilla cage," the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission is lifted off the ground at the Vertical Integration Facility at Space Launch Complex 41. The generator will be hoisted up to the top of the rocket and installed on the MSL spacecraft, encapsulated within the payload fairing. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat produced by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Heat emitted by the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Dimitri Gerondidakis

KSC-2011-6744

NASA Image and Video Library

2011-07-14

CAPE CANAVERAL, Fla. -- The multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission is uncovered in the high bay of the RTG storage facility (RTGF) at NASA's Kennedy Space Center in Florida. The MMRTG was returned to the RTGF following a fit check on MSL's Curiosity rover in the Payload Hazardous Servicing Facility (PHSF). The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Troy Cryder

KSC-2011-7894

NASA Image and Video Library

2011-11-17

CAPE CANAVERAL, Fla. -- At Space Launch Complex-41 on Cape Canaveral Air Force Station, spacecraft technicians in the Vertical Integration Facility prepare to install the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission on the Curiosity rover. The MMRTG is enclosed in a protective mesh container, known as the "gorilla cage," which protects it during transport and allows any excess heat generated to dissipate into the air. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is scheduled for Nov. 25. For more information, visit http://www.nasa.gov/msl. Photo credit: Department of Energy/Idaho National Laboratory

KSC-2011-7899

NASA Image and Video Library

2011-11-17

CAPE CANAVERAL, Fla. -- In the Vertical Integration Facility at Space Launch Complex-41 on Cape Canaveral Air Force Station, the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission, secured to a turning fixture, is positioned on the radioisotope power system integration cart (RIC). The MMRTG will be installed on the Curiosity rover with the aid of the RIC. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is scheduled for Nov. 25. For more information, visit http://www.nasa.gov/msl. Photo credit: Department of Energy/Idaho National Laboratory

KSC-2011-6730

NASA Image and Video Library

2011-07-14

CAPE CANAVERAL, Fla. -- At NASA's Kennedy Space Center in Florida, the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission, secured inside the MMRTG trailer, makes its way between the Payload Hazardous Servicing Facility (PHSF) and the RTG storage facility. The MMRTG is being moved following a fit check on MSL's Curiosity rover in the PHSF. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Troy Cryder

Uncovering Special Nuclear Materials by Low-energy Nuclear Reaction Imaging

PubMed Central

Rose, P. B.; Erickson, A. S.; Mayer, M.; Nattress, J.; Jovanovic, I.

2016-01-01

Weapons-grade uranium and plutonium could be used as nuclear explosives with extreme destructive potential. The problem of their detection, especially in standard cargo containers during transit, has been described as “searching for a needle in a haystack” because of the inherently low rate of spontaneous emission of characteristic penetrating radiation and the ease of its shielding. Currently, the only practical approach for uncovering well-shielded special nuclear materials is by use of active interrogation using an external radiation source. However, the similarity of these materials to shielding and the required radiation doses that may exceed regulatory limits prevent this method from being widely used in practice. We introduce a low-dose active detection technique, referred to as low-energy nuclear reaction imaging, which exploits the physics of interactions of multi-MeV monoenergetic photons and neutrons to simultaneously measure the material’s areal density and effective atomic number, while confirming the presence of fissionable materials by observing the beta-delayed neutron emission. For the first time, we demonstrate identification and imaging of uranium with this novel technique using a simple yet robust source, setting the stage for its wide adoption in security applications. PMID:27087555

Uncovering Special Nuclear Materials by Low-energy Nuclear Reaction Imaging.

PubMed

Rose, P B; Erickson, A S; Mayer, M; Nattress, J; Jovanovic, I

2016-04-18

Weapons-grade uranium and plutonium could be used as nuclear explosives with extreme destructive potential. The problem of their detection, especially in standard cargo containers during transit, has been described as "searching for a needle in a haystack" because of the inherently low rate of spontaneous emission of characteristic penetrating radiation and the ease of its shielding. Currently, the only practical approach for uncovering well-shielded special nuclear materials is by use of active interrogation using an external radiation source. However, the similarity of these materials to shielding and the required radiation doses that may exceed regulatory limits prevent this method from being widely used in practice. We introduce a low-dose active detection technique, referred to as low-energy nuclear reaction imaging, which exploits the physics of interactions of multi-MeV monoenergetic photons and neutrons to simultaneously measure the material's areal density and effective atomic number, while confirming the presence of fissionable materials by observing the beta-delayed neutron emission. For the first time, we demonstrate identification and imaging of uranium with this novel technique using a simple yet robust source, setting the stage for its wide adoption in security applications.

Grading Practices--Watching Out for Land Mines.

ERIC Educational Resources Information Center

Nottingham, Marv

1988-01-01

The A to F grading pattern is a highly subjective practice that demands great expertise and assumes a high degree of test validity. This article discusses the merits of extra credit assignments, homework, and "pop" quizzes; outlines defensible grading procedures; and discusses common grading problems, such as using grades as weapons. (MLH)

Nuclear Archeology in a Bottle: Evidence of Pre-Trinity U.S. Weapons Activities from a Waste Burial Site

DOE Office of Scientific and Technical Information (OSTI.GOV)

Schwantes, Jon M.; Douglas, Matthew; Bonde, Steven E.

2009-02-15

During World War II, the Hanford Site in Washington was chosen for plutonium production. In 2004, a bottle containing a sample of plutonium was recovered from a Hanford waste trench. Isotopic age dating indicated the sample was separated from the fuel pellet 64 ±2.8 years earlier. Detectable products of secondary nuclear reactions, such as 22Na, proved useful as 1) a detectable analog for alpha emitting actinides, 2) an indicator of sample splitting, and 3) a measure of the time since sample splitting. The sample origin was identified as the X-10 reactor, Oak Ridge, TN. Corroborated by historical documents, we concludedmore » this sample was part of the first batch of Pu separated at T-Plant, Hanford, the world’s first industrial-scale reprocessing facility, on December 9, 1944.« less

The Manhattan Project

NASA Astrophysics Data System (ADS)

Reed, B. Cameron

2014-10-01

The Manhattan Project was the United States Army’s program to develop and deploy nuclear weapons during World War II. In these devices, which are known popularly as ‘atomic bombs’, energy is released not by a chemical explosion but by the much more violent process of fission of nuclei of heavy elements via a neutron-mediated chain-reaction. Three years after taking on this project in mid-1942, the Army’s Manhattan Engineer District produced three nuclear bombs of two different designs. Two of these devices were fueled with the 239 isotope of the synthetic element plutonium, while the third employed the rare 235 isotope of uranium. One of the plutonium devices, code-named Trinity, was detonated in a test in southern New Mexico on 16 July 1945; this was the world’s first nuclear explosion. Three weeks later, on 6 August, the uranium bomb, Little Boy, was dropped on the Japanese city of Hiroshima. On 9 August the second plutonium device, Fat Man, was dropped on Nagasaki. Together, the two bombings killed over 100 000 people and were at least partially responsible for the Japanese government’s 14 August decision to surrender. This article surveys, at an undergraduate level, the science and history of the Manhattan Project.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Fox, T.; Tietjen, G.L.; McInroy, J.F.

The Autopsy Tissue Program was begun in 1960. To date, tissues on 900 or more persons in 7 geographic regions have been collected and analyzed for plutonium content. The tissues generally consist of lung, liver, kidney, lymph, bone, and gonadal tissues for each individual. The original objective of the program was to determine the level of plutonium in human tissues due solely to fallout from weapons testing. The baseline thus established was to be used to evaluate future changes. From the first, this program was beset with chemical and statistical difficulties. Many factors whose effects were not recognized and notmore » planned for were found later to be important. Privacy and ethical considerations hindered the gathering of adequate data. Since the chemists were looking for amounts of plutonium very close to background, possible contamination was a very real problem. Widely used chemical techniques introduced a host of statistical problems. The difficulties encountered touch on areas common to large data sets, unusual outlier detection methods minimum detection limits, problems with aliquot sizes, and time-trends in the data. The conclusions point out areas to which the biologists will have to devote much more careful attention than was believed.« less

History of 232-F, tritium extraction processing

DOE Office of Scientific and Technical Information (OSTI.GOV)

Blackburn, G.W.

1994-08-01

In 1950 the Atomic Energy Commission authorized the Savannah River Project principally for the production of tritium and plutonium-239 for use in thermonuclear weapons. 232-F was built as an interim facility in 1953--1954, at a cost of $3.9M. Tritium extraction operations began in October, 1955, after the reactor and separations startups. In July, 1957 a larger tritium facility began operation in 232-H. In 1958 the capacity of 232-H was doubled. Also, in 1957 a new task was assigned to Savannah River, the loading of tritium into reservoirs that would be actual components of thermonuclear weapons. This report describes the historymore » of 232-F, the process for tritium extraction, and the lessons learned over the years that were eventually incorporated into the new Replacement Tritium Facility.« less

Characterization of U/Pu Particles Originating From the Nuclear Weapon Accidents at Palomares, Spain, 1966 And Thule, Greenland, 1968

DOE Office of Scientific and Technical Information (OSTI.GOV)

Lind, O.C.; Salbu, B.; Janssens, K.

2007-07-10

Following the USAF B-52 bomber accidents at Palomares, Spain in 1966 and at Thule, Greenland in 1968, radioactive particles containing uranium (U) and plutonium (Pu) were dispersed into the environment. To improve long-term environmental impact assessments for the contaminated ecosystems, particles from the two sites have been isolated and characterized with respect to properties influencing particle weathering rates. Low [239]Pu/[235]U (0.62-0.78) and [240]Pu/[239]Pu (0.055-0.061) atom ratios in individual particles from both sites obtained by Inductively Coupled Plasma Mass Spectrometry (ICP-MS) show that the particles contain highly enriched U and weapon-grade Pu. Furthermore, results from electron microscopy with Energy Dispersive X-raymore » analysis (EDX) and synchrotron radiation (SR) based micrometer-scale X-ray fluorescence ({micro}-XRF) 2D mapping demonstrated that U and Pu coexist throughout the 1-50 {micro}m sized particles, while surface heterogeneities were observed in EDX line scans. SR-based micrometer-scale X-ray Absorption Near Edge Structure Spectroscopy ({micro}-XANES) showed that the particles consisted of an oxide mixture of U (predominately UO[2] with the presence ofU[3][8]) and Pu ((III)/(IV), (V)/(V) or (III), (IV) and (V)). Neither metallic U or Pu nor uranyl or Pu(VI) could be observed. Characteristics such as elemental distributions, morphology and oxidation states are remarkably similar for the Palomares and Thule particles, reflecting that they originate from similar source and release scenarios. Thus, these particle characteristics are more dependent on the original material from which the particles are derived (source) and the formation of particles (release scenario) than the environmental conditions to which the particles have been exposed since the late 1960s.« less

Are Zeros Your Ultimate Weapon?

ERIC Educational Resources Information Center

Guskey, Thomas R.

2004-01-01

Grading is one of a teacher's greatest challenges and most important professional responsibilities. However, few teachers have any formal training in grading methods, and most teachers have limited knowledge about the effectiveness of various grading practices. As a consequence, when teachers develop their grading policies, they typically reflect…

The ``Nuclear Renaissance'' and the Spread of Nuclear Weapons

NASA Astrophysics Data System (ADS)

Lyman, Edwin S.

2007-05-01

As interest grows around the world in nuclear power as an energy source that could help control greenhouse gas emissions, some have proclaimed the arrival of a ``nuclear renaissance.'' But can the increased risks of more nuclear power be managed? The political crisis surrounding Iran's pursuit of uranium enrichment has exposed weaknesses in the nuclear nonproliferation regime. Also, al Qaeda's declared interest in weapons of mass destruction raises the concern that terrorists could acquire nuclear weapons by stealing materials from poorly secured facilities. Growth of nuclear energy would require the construction of many additional uranium enrichment plants. And the generation of more spent nuclear fuel without a credible waste disposal strategy would increase political support for reprocessing, which separates large quantities of weapon-usable plutonium from spent fuel. There is little evidence that the various institutional arrangements and technical schemes proposed to mitigate the security risks of a major nuclear expansion would be effective. This talk will focus on the measures necessary to allow large-scale global growth of nuclear power without resulting in an unacceptably high risk of nuclear proliferation and nuclear terrorism, and will discuss the feasibility of such measures. To cite this abstract, use the following reference: http://meetings.aps.org/link/BAPS.2007.OSS07.E1.2

Weapon Carrying Among Victims of Bullying.

PubMed

Pham, Tammy B; Schapiro, Lana E; John, Majnu; Adesman, Andrew

2017-12-01

To examine, in a large, nationally representative sample of high school students, the association between bullying victimization and carrying weapons to school and to determine to what extent past experience of 1, 2, or 3 additional indicators of peer aggression increases the likelihood of weapon carrying by victims of bullying (VoBs). National data from the 2015 Youth Risk Behavior Survey were analyzed for grades 9 to 12 ( N = 15 624). VoB groups were determined by self-report of being bullied at school and additional adverse experiences: fighting at school, being threatened or injured at school, and skipping school out of fear for one's safety. Weapon carrying was measured by a dichotomized (ie, ≥1 vs 0) report of carrying a gun, knife, or club on school property. VoB groups were compared with nonvictims with respect to weapon carrying by logistic regression adjusting for sex, grade, and race/ethnicity. When surveyed, 20.2% of students reported being a VoB in the past year, and 4.1% reported carrying a weapon to school in the past month. VoBs experiencing 1, 2, or 3 additional risk factors were successively more likely to carry weapons to school. The subset of VoBs who experienced all 3 additional adverse experiences were more likely to carry weapons to school compared with nonvictims (46.4% vs 2.5%, P < .001). Pediatricians should recognize that VoBs, especially those who have experienced 1 or more indicators of peer aggression in conjunction, are at substantially increased risk of weapon carrying. Copyright © 2017 by the American Academy of Pediatrics.

Tritium and plutonium in waters from the Bering and Chukchi Seas

USGS Publications Warehouse

Landa, E.R.; Beals, D.M.; Halverson, J.E.; Michel, R.L.; Cefus, G.R.

1999-01-01

During the summer of 1993, seawater in the Bering and Chukchi Seas was sampled on a joint Russian-American cruise [BERPAC] of the RV Okean to determine concentrations of tritium, 239Pu and 240Pu. Concentrations of tritium were determined by electrolytic enrichment and liquid scintilation counting. Tritium levels ranged up to 420 mBq L-1 showed no evidence of inputs other than those attribute atmospheric nuclear weapons testing. Plutonium was recovered from water samples by ferric hydroxide precipitation, and concentrations were determined by thermal ionization mass spectrometry. 239+240Pu concentrations ranged from <1 to 5.5 [mu]Bq L-1. These concentrations are lower than those measured in water samples from other parts of the ocean during the mid-1960's to the late 1980's. The 240Pu:239Pu ratios, although associated with large uncertainties, suggest that most of the plutonium is derived from world-wide fallout. As points of comparison, the highest concentrations of tritium and plutonium observed here were about five orders of magnitude lower than the maximum permissible concentrations allowed in water released to the off-site environs from licensed nuclear facilities in the United States. This study and others sponsored by the International Atomic Energy Agency and the Office of Naval Research's Arctic Nuclear Waste Assessment Program are providing data for the assessment of potential radiological impacts in the Arctic regions associated with nuclear waste disposal by the former Soviet Union.

Cladding and duct materials for advanced nuclear recycle reactors

NASA Astrophysics Data System (ADS)

Allen, T. R.; Busby, J. T.; Klueh, R. L.; Maloy, S. A.; Toloczko, M. B.

2008-01-01

The expanded use of nuclear energy without risk of nuclear weapons proliferation and with safe nuclear waste disposal is a primary goal of the Global Nuclear Energy Partnership (GNEP). To achieve that goal the GNEP is exploring advanced technologies for recycling spent nuclear fuel that do not separate pure plutonium, and advanced reactors that consume transuranic elements from recycled spent fuel. The GNEP’s objectives will place high demands on reactor clad and structural materials. This article discusses the materials requirements of the GNEP’s advanced nuclear recycle reactors program.

Localization and spectral isolation of special nuclear material using stochastic image reconstruction

NASA Astrophysics Data System (ADS)

Hamel, M. C.; Polack, J. K.; Poitrasson-Rivière, A.; Clarke, S. D.; Pozzi, S. A.

2017-01-01

In this work we present a technique for isolating the gamma-ray and neutron energy spectra from multiple radioactive sources localized in an image. Image reconstruction algorithms for radiation scatter cameras typically focus on improving image quality. However, with scatter cameras being developed for non-proliferation applications, there is a need for not only source localization but also source identification. This work outlines a modified stochastic origin ensembles algorithm that provides localized spectra for all pixels in the image. We demonstrated the technique by performing three experiments with a dual-particle imager that measured various gamma-ray and neutron sources simultaneously. We showed that we could isolate the peaks from 22Na and 137Cs and that the energy resolution is maintained in the isolated spectra. To evaluate the spectral isolation of neutrons, a 252Cf source and a PuBe source were measured simultaneously and the reconstruction showed that the isolated PuBe spectrum had a higher average energy and a greater fraction of neutrons at higher energies than the 252Cf. Finally, spectrum isolation was used for an experiment with weapons grade plutonium, 252Cf, and AmBe. The resulting neutron and gamma-ray spectra showed the expected characteristics that could then be used to identify the sources.

KSC-2011-6745

NASA Image and Video Library

2011-07-14

CAPE CANAVERAL, Fla. -- The multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission is position behind mobile plexiglass radiation shields in the high bay of the RTG storage facility (RTGF) at NASA's Kennedy Space Center in Florida. The MMRTG was returned to the RTGF following a fit check on MSL's Curiosity rover in the Payload Hazardous Servicing Facility (PHSF). The generator will remain in the RTGF until is moved to the pad for integration on the rover. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Troy Cryder

KSC-2011-6708

NASA Image and Video Library

2011-07-13

CAPE CANAVERAL, Fla. -- In the high bay of the Payload Hazardous Servicing Facility at NASA's Kennedy Space Center in Florida, the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission, still connected to the turning fixture, rests on a support base following the MMRTG fit check on the Curiosity rover. A mobile plexiglass radiation shield is in place between the MMRTG and the spacecraft technicians, at right, to help minimize the employees' radiation exposure. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Kim Shiflett

KSC-2011-6700

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- In the high bay of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida, spacecraft technicians from NASA's Jet Propulsion Laboratory prepare to attach the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission onto the aft of the Curiosity rover for a fit check with the aid of the MMRTG integration cart. The MMRTG then will be removed and installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6701

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- In the high bay of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida, spacecraft technicians from NASA's Jet Propulsion Laboratory use extension tools to attach the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission on the MMRTG integration cart onto the aft of the Curiosity rover for a fit check. The MMRTG then will be removed and installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6706

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- In the high bay of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida, the descent stage for NASA's Mars Science Laboratory (MSL) mission awaits installation on the Curiosity rover, in the background at right. MSL's multi-mission radioisotope thermoelectric generator has been installed onto the aft of the rover for a fit check. The descent stage will cradle the rover and its MMRTG during their approach to the surface of Mars. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6698

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- In the high bay of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida, spacecraft technicians from NASA's Jet Propulsion Laboratory transfer the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission onto the aft of the Curiosity rover for a fit check with the aid of the MMRTG integration cart. The MMRTG then will be removed and installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6705

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- In the high bay of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida, the descent stage for NASA's Mars Science Laboratory (MSL) mission awaits installation on the Curiosity rover, in the background at right. MSL's multi-mission radioisotope thermoelectric generator has been installed onto the aft of the rover for a fit check. The descent stage will cradle the rover and its MMRTG during their approach to the surface of Mars. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6699

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- In the high bay of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida, spacecraft technicians from NASA's Jet Propulsion Laboratory transfer the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission onto the aft of the Curiosity rover for a fit check with the aid of the MMRTG integration cart. The MMRTG then will be removed and installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6678

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- The multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission is delivered to the airlock doors of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida inside the MMRTG trailer. In the PHSF, the MMRTG temporarily will be installed on the MSL rover, Curiosity, for a fit check but will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6702

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- In the high bay of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida, the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission is detached from the MMRTG integration cart and installed onto the aft of the Curiosity rover for a fit check. Next, the MMRTG will be removed and later installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6651

NASA Image and Video Library

2011-06-30

CAPE CANAVERAL, Fla. -- The multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory mission, enclosed in a shipping cask, rolls into the high bay of the RTG storage facility at NASA's Kennedy Space Center in Florida. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for evidence on whether Mars has had environments favorable to microbial life, including chemical ingredients for life. The unique rover will use a laser to look inside rocks and release its gasses so that the rover’s spectrometer can analyze and send the data back to Earth. Launch of MSL aboard a United Launch Alliance Atlas V rocket is scheduled for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station in Florida. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Frankie Martin

KSC-2011-6658

NASA Image and Video Library

2011-06-30

CAPE CANAVERAL, Fla. -- In the high bay of the RTG storage facility at NASA's Kennedy Space Center in Florida, a crane lifts the shipping cask enclosing the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory mission from its transportation pallet. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for evidence on whether Mars has had environments favorable to microbial life, including chemical ingredients for life. The unique rover will use a laser to look inside rocks and release its gasses so that the rover’s spectrometer can analyze and send the data back to Earth. Launch of MSL aboard a United Launch Alliance Atlas V rocket is scheduled for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station in Florida. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Frankie Martin

KSC-2011-6677

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- The multi-mission radioisotope thermoelectric generator (MMRTG) trailer backs toward the airlock doors of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida. The MMRTG for NASA's Mars Science Laboratory (MSL) mission is being transferred into the PHSF, where it will be installed on the MSL rover, Curiosity, for a fit check. The MMRTG will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-7896

NASA Image and Video Library

2011-11-17

CAPE CANAVERAL, Fla. -- In the Vertical Integration Facility at Space Launch Complex-41 on Cape Canaveral Air Force Station, the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission is uncovered during preparations to install it on MSL's Curiosity rover. The mesh container, known as the "gorilla cage," is suspended above the generator as it is lifted off the MMRTG's support base. The cage protects the MMRTG during transport and allows any excess heat generated to dissipate into the air. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is scheduled for Nov. 25. For more information, visit http://www.nasa.gov/msl. Photo credit: Department of Energy/Idaho National Laboratory

KSC-2011-7895

NASA Image and Video Library

2011-11-17

CAPE CANAVERAL, Fla. -- In the Vertical Integration Facility at Space Launch Complex-41 on Cape Canaveral Air Force Station, spacecraft technicians guide the mesh container protecting the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission as a crane lifts it from around the generator. The container, known as the "gorilla cage," protects the MMRTG during transport and allows any excess heat generated to dissipate into the air. Next, the MMRTG will be installed on MSL's Curiosity rover. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is scheduled for Nov. 25. For more information, visit http://www.nasa.gov/msl. Photo credit: Department of Energy/Idaho National Laboratory

KSC-2011-6716

NASA Image and Video Library

2011-07-13

CAPE CANAVERAL, Fla. -- The multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission rests on its support base in the airlock of the Payload Hazardous Servicing Facility at NASA's Kennedy Space Center in Florida following the MMRTG fit check on the Curiosity rover in the high bay. In the background, at right, is the mesh container, known as the "gorilla cage," which protects the MMRTG during transport and allows any excess heat generated to dissipate into the air. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Kim Shiflett

KSC-2011-6647

NASA Image and Video Library

2011-06-30

CAPE CANAVERAL, Fla. -- The multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory mission, enclosed in a shipping cask, is seen through the open door of the MMRTG trailer that delivered it to the RTG storage facility at NASA's Kennedy Space Center in Florida. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for evidence on whether Mars has had environments favorable to microbial life, including chemical ingredients for life. The unique rover will use a laser to look inside rocks and release its gasses so that the rover’s spectrometer can analyze and send the data back to Earth. Launch of MSL aboard a United Launch Alliance Atlas V rocket is scheduled for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station in Florida. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Frankie Martin

KSC-2011-6650

NASA Image and Video Library

2011-06-30

CAPE CANAVERAL, Fla. -- Workers use a forklift to transport the shipping cask enclosing the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory mission to the door of the high bay of the RTG storage facility at NASA's Kennedy Space Center in Florida. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for evidence on whether Mars has had environments favorable to microbial life, including chemical ingredients for life. The unique rover will use a laser to look inside rocks and release its gasses so that the rover’s spectrometer can analyze and send the data back to Earth. Launch of MSL aboard a United Launch Alliance Atlas V rocket is scheduled for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station in Florida. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Frankie Martin

KSC-2011-6648

NASA Image and Video Library

2011-06-30

CAPE CANAVERAL, Fla. -- Workers use a forklift to offload the shipping cask enclosing the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory mission from the MMRTG trailer that delivered it to the RTG storage facility at NASA's Kennedy Space Center in Florida. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for evidence on whether Mars has had environments favorable to microbial life, including chemical ingredients for life. The unique rover will use a laser to look inside rocks and release its gasses so that the rover’s spectrometer can analyze and send the data back to Earth. Launch of MSL aboard a United Launch Alliance Atlas V rocket is scheduled for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station in Florida. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Frankie Martin

KSC-2011-6653

NASA Image and Video Library

2011-06-30

CAPE CANAVERAL, Fla. -- In the high bay of the RTG storage facility at NASA's Kennedy Space Center in Florida, measurements are taken to determine the level of radioactivity emitted from the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory mission, enclosed in a shipping cask in the background. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for evidence on whether Mars has had environments favorable to microbial life, including chemical ingredients for life. The unique rover will use a laser to look inside rocks and release its gasses so that the rover’s spectrometer can analyze and send the data back to Earth. Launch of MSL aboard a United Launch Alliance Atlas V rocket is scheduled for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station in Florida. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Frankie Martin

KSC-2011-6662

NASA Image and Video Library

2011-06-30

CAPE CANAVERAL, Fla. -- In the high bay of the RTG storage facility at NASA's Kennedy Space Center in Florida, Department of Energy contractor employees remove the external and internal protective layers of the shipping cask enclosing the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory mission. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for evidence on whether Mars has had environments favorable to microbial life, including chemical ingredients for life. The unique rover will use a laser to look inside rocks and release its gasses so that the rover’s spectrometer can analyze and send the data back to Earth. Launch of MSL aboard a United Launch Alliance Atlas V rocket is scheduled for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station in Florida. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Frankie Martin

KSC-2011-6663

NASA Image and Video Library

2011-06-30

CAPE CANAVERAL, Fla. -- In the high bay of the RTG storage facility at NASA's Kennedy Space Center in Florida, the external and internal protective layers of the shipping cask are lifted from around the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory mission. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for evidence on whether Mars has had environments favorable to microbial life, including chemical ingredients for life. The unique rover will use a laser to look inside rocks and release its gasses so that the rover’s spectrometer can analyze and send the data back to Earth. Launch of MSL aboard a United Launch Alliance Atlas V rocket is scheduled for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station in Florida. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Frankie Martin

KSC-2011-6659

NASA Image and Video Library

2011-06-30

CAPE CANAVERAL, Fla. -- In the RTG storage facility at NASA's Kennedy Space Center in Florida, the shipping cask enclosing the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory mission is lowered to the floor of the high bay in preparation for lifting the cask from around the MMRTG. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for evidence on whether Mars has had environments favorable to microbial life, including chemical ingredients for life. The unique rover will use a laser to look inside rocks and release its gasses so that the rover’s spectrometer can analyze and send the data back to Earth. Launch of MSL aboard a United Launch Alliance Atlas V rocket is scheduled for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station in Florida. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Frankie Martin

KSC-2011-6649

NASA Image and Video Library

2011-06-30

CAPE CANAVERAL, Fla. -- Workers use a forklift to offload the shipping cask enclosing the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory mission from the MMRTG trailer that delivered it to the RTG storage facility at NASA's Kennedy Space Center in Florida. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for evidence on whether Mars has had environments favorable to microbial life, including chemical ingredients for life. The unique rover will use a laser to look inside rocks and release its gasses so that the rover’s spectrometer can analyze and send the data back to Earth. Launch of MSL aboard a United Launch Alliance Atlas V rocket is scheduled for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station in Florida. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Frankie Martin

KSC-2011-6660

NASA Image and Video Library

2011-06-30

CAPE CANAVERAL, Fla. -- In the high bay of the RTG storage facility at NASA's Kennedy Space Center in Florida, the shipping cask enclosing the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory mission is lifted from around the MMRTG using guide rods installed on the support base. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for evidence on whether Mars has had environments favorable to microbial life, including chemical ingredients for life. The unique rover will use a laser to look inside rocks and release its gasses so that the rover’s spectrometer can analyze and send the data back to Earth. Launch of MSL aboard a United Launch Alliance Atlas V rocket is scheduled for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station in Florida. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Frankie Martin

KSC-2011-6697

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- In the high bay of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida, the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission is attached to the MMRTG integration cart. The cart will be used to install the MMRTG on the Curiosity rover for a fit check. The rover is on an elevated work stand, at right. The MMRTG then will be removed and installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6711

NASA Image and Video Library

2011-07-13

CAPE CANAVERAL, Fla. -- In the high bay of the Payload Hazardous Servicing Facility at NASA's Kennedy Space Center in Florida, a spacecraft technician from NASA's Jet Propulsion Laboratory conducts a visual inspection of the cooling tubes on the exterior of the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission following the MMRTG fit check on the Curiosity rover. At right is the Curiosity rover on an elevated work stand. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Kim Shiflett

KSC-2011-6695

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- In the high bay of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida, the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission on the turning fixture is lowered onto the MMRTG integration cart. The cart will be used to install the MMRTG on the Curiosity rover for a fit check. The rover is on an elevated work stand, at right. The MMRTG will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6712

NASA Image and Video Library

2011-07-13

CAPE CANAVERAL, Fla. -- In the high bay of the Payload Hazardous Servicing Facility at NASA's Kennedy Space Center in Florida, a spacecraft technician from NASA's Jet Propulsion Laboratory conducts a visual inspection of the cooling tubes on the exterior of the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission following the MMRTG fit check on the Curiosity rover. At right is the Curiosity rover on an elevated work stand. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Kim Shiflett

KSC-2011-6684

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- Workers dressed in clean room attire, known as bunny suits, transfer the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission on its holding base from the airlock of the Payload Hazardous Servicing Facility (PHSF) into the facility's high bay. In the high bay, the MMRTG temporarily will be installed on the MSL rover, Curiosity, for a fit check but will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

Plutonium Decontamination of Uranium using CO2 Cleaning

DOE Office of Scientific and Technical Information (OSTI.GOV)

Blau, M

A concern of the Department of Energy (DOE) Environmental Management (EM) and Defense Programs (DP), and of the Los Alamos National Laboratory (LANL) and the Lawrence Livermore National Laboratory (LLNL), is the disposition of thousands of legacy and recently generated plutonium (Pu)-contaminated, highly enriched uranium (HEU) parts. These parts take up needed vault space. This presents a serious problem for LLNL, as site limit could result in the stoppage of future weapons work. The Office of Fissile Materials Disposition (NN-60) will also face a similar problem as thousands of HEU parts will be created with the disassembly of site-return pitsmore » for plutonium recovery when the Pit Disassembly and Conversion Facility (PDCF) at the Savannah River Site (SRS) becomes operational. To send HEU to the Oak Ridge National Laboratory and the Y-12 Plant for disposition, the contamination for metal must be less than 20 disintegrations per minute (dpm) of swipable transuranic per 100 cm{sup 2} of surface area or the Pu bulk contamination for oxide must be less than 210 parts per billion (ppb). LANL has used the electrolytic process on Pu-contaminated HEU weapon parts with some success. However, this process requires that a different fixture be used for every configuration; each fixture cost approximately $10K. Moreover, electrolytic decontamination leaches the uranium metal substrate (no uranium or plutonium oxide) from the HEU part. The leaching rate at the uranium metal grain boundaries is higher than that of the grains and depends on the thickness of the uranium oxide layer. As the leaching liquid flows past the HEU part, it carries away plutonium oxide contamination and uranium oxide. The uneven uranium metal surface created by the leaching becomes a trap for plutonium oxide contamination. In addition, other DOE sites have used CO{sub 2} cleaning for Pu decontamination successfully. In the 1990's, the Idaho National Engineering Laboratory investigated this technology and showed that CO{sub 2} pellet blasting (or CO{sub 2} cleaning) reduced both fixed and smearable contamination on tools. In 1997, LLNL proved that even tritium contamination could be removed from a variety of different matrices using CO{sub 2}cleaning. CO{sub 2} cleaning is a non-toxic, nonconductive, nonabrasive decontamination process whose primary cleaning mechanisms are: (1) Impact of the CO{sub 2} pellets loosens the bond between the contaminant and the substrate. (2) CO{sub 2} pellets shatter and sublimate into a gaseous state with large expansion ({approx}800 times). The expanding CO{sub 2} gas forms a layer between the contaminant and the substrate that acts as a spatula and peels off the contaminant. (3) Cooling of the contaminant assists in breaking its bond with the substrate. Thus, LLNL conducted feasibility testing to determine if CO{sub 2} pellet blasting could remove Pu contamination (e.g., uranium oxide) from uranium metal without abrading the metal matrix. This report contains a summary of events and the results of this test.« less

Reconstructed plutonium fallout in the GV7 firn core from Northern Victoria Land, East Antarctica

NASA Astrophysics Data System (ADS)

Hwang, H.; Han, Y.; Kang, J.; Lee, K.; Hong, S.; Hur, S. D.; Narcisi, B.; Frezzotti, M.

2017-12-01

Atmospheric nuclear explosions during the period from the 1940s to the 1980s are the major anthropogenic source of plutonium (Pu) in the environment. In this work, we analyzed fg g-1 levels of artificial Pu, released predominantly by atmospheric nuclear weapons tests. We measured 351 samples which collected a 78 m-depth fire core at the site of GV7 (S 70°41'17.1", E 158°51'48.9", 1950 m a.s.l.), Northern Victoria Land, East Antarctica. To determine the Pu concentration in the samples, we used an inductively coupled plasma sector field mass spectrometry coupled with an Apex high-efficiency sample introduction system, which has the advantages of small sample consumption and simple sample preparation. We reconstructed the firn core Pu fallout record for the period after 1954 CE shows a significant fluctuation in agreement with past atmospheric nuclear testing. These data will contribute to ice core research by providing depth-age information.

Zirconia-magnesia inert matrix fuel and waste form: Synthesis, characterization and chemical performance in an advanced fuel cycle

NASA Astrophysics Data System (ADS)

Holliday, Kiel Steven

There is a significant buildup in plutonium stockpiles throughout the world, because of spent nuclear fuel and the dismantling of weapons. The radiotoxicity of this material and proliferation risk has led to a desire for destroying excess plutonium. To do this effectively, it must be fissioned in a reactor as part of a uranium free fuel to eliminate the generation of more plutonium. This requires an inert matrix to volumetrically dilute the fissile plutonium. Zirconia-magnesia dual phase ceramic has been demonstrated to be a favorable material for this task. It is neutron transparent, zirconia is chemically robust, magnesia has good thermal conductivity and the ceramic has been calculated to conform to current economic and safety standards. This dissertation contributes to the knowledge of zirconia-magnesia as an inert matrix fuel to establish behavior of the material containing a fissile component. First, the zirconia-magnesia inert matrix is synthesized in a dual phase ceramic containing a fissile component and a burnable poison. The chemical constitution of the ceramic is then determined. Next, the material performance is assessed under conditions relevant to an advanced fuel cycle. Reactor conditions were assessed with high temperature, high pressure water. Various acid solutions were used in an effort to dissolve the material for reprocessing. The ceramic was also tested as a waste form under environmental conditions, should it go directly to a repository as a spent fuel. The applicability of zirconia-magnesia as an inert matrix fuel and waste form was tested and found to be a promising material for such applications.

Determination of origin and intended use of plutonium metal using nuclear forensic techniques.

PubMed

Rim, Jung H; Kuhn, Kevin J; Tandon, Lav; Xu, Ning; Porterfield, Donivan R; Worley, Christopher G; Thomas, Mariam R; Spencer, Khalil J; Stanley, Floyd E; Lujan, Elmer J; Garduno, Katherine; Trellue, Holly R

2017-04-01

Nuclear forensics techniques, including micro-XRF, gamma spectrometry, trace elemental analysis and isotopic/chronometric characterization were used to interrogate two, potentially related plutonium metal foils. These samples were submitted for analysis with only limited production information, and a comprehensive suite of forensic analyses were performed. Resulting analytical data was paired with available reactor model and historical information to provide insight into the materials' properties, origins, and likely intended uses. Both were super-grade plutonium, containing less than 3% 240 Pu, and age-dating suggested that most recent chemical purification occurred in 1948 and 1955 for the respective metals. Additional consideration of reactor modeling feedback and trace elemental observables indicate plausible U.S. reactor origin associated with the Hanford site production efforts. Based on this investigation, the most likely intended use for these plutonium foils was 239 Pu fission foil targets for physics experiments, such as cross-section measurements, etc. Copyright © 2017 Elsevier B.V. All rights reserved.

Determination of origin and intended use of plutonium metal using nuclear forensic techniques

DOE PAGES

Rim, Jung H.; Kuhn, Kevin J.; Tandon, Lav; ...

2017-04-01

Nuclear forensics techniques, including micro-XRF, gamma spectrometry, trace elemental analysis and isotopic/chronometric characterization were used to interrogate two, potentially related plutonium metal foils. These samples were submitted for analysis with only limited production information, and a comprehensive suite of forensic analyses were performed. Resulting analytical data was paired with available reactor model and historical information to provide insight into the materials’ properties, origins, and likely intended uses. Both were super-grade plutonium, containing less than 3% 240Pu, and age-dating suggested that most recent chemical purification occurred in 1948 and 1955 for the respective metals. Additional consideration of reactor modelling feedback andmore » trace elemental observables indicate plausible U.S. reactor origin associated with the Hanford site production efforts. In conclusion, based on this investigation, the most likely intended use for these plutonium foils was 239Pu fission foil targets for physics experiments, such as cross-section measurements, etc.« less

Industrial scale-plant for HLW partitioning in Russia

DOE Office of Scientific and Technical Information (OSTI.GOV)

Dzekun, E.G.; Glagolenko, Y.V.; Drojko, E.G.

1996-12-31

Radiochemical plant of PA <> at Ozersk, which was come on line in December 1948 originally for weapon plutonium production and reoriented on the reprocessing of spent fuel, till now keeps on storage HLW of the military program. Application of the vitrification method since 1986 has not essentially reduced HLW volumes. So, as of September 1, 1995 vitrification installations had been processed 9590 m{sup 3} HLW and 235 MCi of radionuclides was included in glass. However only 1100 m{sup 3} and 20.5 MCi is part of waste of the military program. The reason is the fact, that the technology andmore » equipment of vitrification were developed for current waste of Purex-process, for which low contents of corrosion-dangerous impurity to materials of vitrification installation is characteristic of. With reference to HLW, which are growing at PA <> in the course of weapon plutonium production, the program of Science-Research Works includes the following main directions of work. Development of technology and equipment of installations for immobilising HLW with high contents of impurity into a solid form at induction melter. Application of High-temperature Adsorption Method for sorption of radionuclides from HLW on silica gel. Application of Partitioning Method of radionuclides from HLW, based on extraction cesium and strontium into cobalt dicarbollyde or crown-ethers, but also on recovery of cesium radionuclides by sorption on inorganic sorbents. In this paper the results of work on creation of first industrial scale-plant for partitioning HLW by the extraction and sorption methods are reported.« less

Natural radionuclide and plutonium content in Black Sea bottom sediments

DOE Office of Scientific and Technical Information (OSTI.GOV)

Strezov, A.; Stoilova, T.; Yordanova, I.

1996-01-01

The content of uranium, thorium, radium, lead, polonium, and plutonium in bottom sediments and algae from two locations at the Bulgarian Black Sea coast have been determined. Some parent:progeny ratios for evaluation of the geochemical behavior of the nuclides have been estimated as well. The extractable and total uranium and thorium are determined by two separate radiochemical procedures to differentiate the more soluble chemical forms of the elements and to estimate the potential hazard for the biosphere and for humans. No distinct seasonal variation as well as no significant change in total and extractable uranium (also for {sup 226}Ra) contentmore » is observed. The same is valid for extractable thorium while the total thorium content in the first two seasons is slightly higher. Our data show that {sup 210}Po content is accumulated more in the sediments than {sup 210}Pb, and the evaluated disequilibria suggest that the two radionuclides belong to more recent sediment layers deposited in the slime samples compared to the silt ones for the different seasons. The obtained values for plutonium are in the lower limits of the data cited in literature, which is quite clear as there are no plutonium discharge facilities at the Bulgarian Black Sea coast. The obtained values for the activity ratio {sup 238}Pu: {sup 239+240}Pu are higher for Bjala sediments compared to those of Kaliakra. The ratio values are out of the variation range for the global contamination with weapon tests fallout plutonium which is probably due to Chernobyl accident contribution. The dependence of natural radionuclide content on the sediment type as well as the variation of nuclide accumulation for two types of algae in two sampling locations for five consecutive seasons is evaluated. No serious contamination with natural radionuclides in the algae is observed. 38 refs., 6 figs., 7 tabs.« less

Plutonium Finishing Plant (PFP) HVAC System Component Index

DOE Office of Scientific and Technical Information (OSTI.GOV)

DICK, J.D.

2000-02-28

The Plutonium Finishing Plant (PFP) WAC System includes sub-systems 25A through 25K. Specific system boundaries and justifications are contained in HNF-SD-CP-SDD-005, ''Definition and Means of Maintaining the Ventilation System Confinement Portion of the PFP Safety Envelope.'' The procurement requirements associated with the system necessitates procurement of some system equipment as Commercial Grade Items in accordance with HNF-PRO-268, ''Control of Purchased Items and Services.'' This document lists safety class and safety significant components for the Heating Ventilation Air Conditioning and specifies the critical characteristics for Commercial Grade Items, as required by HNF-PRO-268 and HNF-PRO-1819. These are the minimum specifications that themore » equipment must meet in order to properly perform its safety function. There may be several manufacturers or models that meet the critical characteristics for any one item.« less

Towards Production of Additive Manufacturing Grade Metallic Powders on the Battlefield

DTIC Science & Technology

2017-10-01

ARL-RP-0618 ● OCT 2017 US Army Research Laboratory Towards Production of Additive Manufacturing Grade Metallic Powders on the...Research Laboratory Towards Production of Additive Manufacturing Grade Metallic Powders on the Battlefield by Marc Pepi Weapons and...REPORT TYPE Reprint 3. DATES COVERED (From - To) June 2016–June 2017 4. TITLE AND SUBTITLE Towards Production of Additive Manufacturing Grade

Weapon Carrying in Israeli Schools: The Contribution of Individual and School Factors

ERIC Educational Resources Information Center

Khoury-Kassabri, Mona; Astor, Ron Avi; Benbenishty, Rami

2007-01-01

The present study employed an ecological perspective to examine the relative predictive power of individual and school contextual factors on weapon carrying at school. The study is based on a nationally representative sample of 10,400 students in Grades 7 through 11 in 162 schools across Israel. Hierarchical logistic modeling examined the…

Gender Differences in the Relative Impact of Physical and Relational Bullying on Adolescent Injury and Weapon Carrying

ERIC Educational Resources Information Center

Dukes, Richard L.; Stein, Judith A.; Zane, Jazmin I.

2010-01-01

Using structural equation modeling, concurrent associations were assessed among physical bullying, relational bullying, physical victimization, relational victimization, injury and weapon carrying using data from the population of 1300 adolescent girls and 1362 adolescent boys in grades 7-12 in a Colorado school district. For both genders, being a…

Selected Indicators of Adolescent Violence & Safety at School.

ERIC Educational Resources Information Center

Mikow, Victoria A.

Fights, weapons, and stolen or intentionally damaged property are common concerns of most schools in North Carolina. The results of this survey indicate that 27 percent of all 9th-12th grade students reported carrying a weapon (gun, knife, club) within the month prior to this survey. A significant percentage of students do not feel safe at school…

Plutonium weathering on Johnston Atoll

DOE Office of Scientific and Technical Information (OSTI.GOV)

Wolf, S.E.; Bates, J.K.; Buck, E.C.

1995-12-31

Johnston Atoll was contaminated with transuranic elements, particularly plutonium, by atmospheric nuclear weapons tests and aborted nuclear devices. Initial cleanup operations and and an extensive soil remediation program were performed. However, many areas contained a low-level continuum of activity, and subsurface contamination has been detected. Discrete hot particles and contaminated soil were characterized to determine whether the spread of activity was caused by weathering. Analytical techniques included gamma spectrometry, alpha spectrometry, and inductively coupled plasma-mass spectrometry to determine transuranic elemental and isotopic composition. Ultrafiltration and small-particle handling techniques were employed to isolate individual particles. Optical microscopy, scanning electron microscopy, analyticalmore » transmission electron microscopy, energy dispersive X-ray spectroscopy, and electron energy loss spectroscopy were used to characterize individual particles. Analyses of the hot particles showed that they are aborted nuclear warhead fragments that been melted and weathered in the presence of water and CaCO{sub 3}. It was concluded that the formation of aqueous ionic (Pu/Am)-CO{sub 3} coordinated complexes, during environmental exposure to large volumes of rainwater and carbonate-satured seawater, enhanced the solubility of transuranic elements. The (Pu/Am)-CO{sub 3} complexes sorbed onto colloidal CaCO{sub 3} and coral soil surfaces as they were exposed to rain and seawater. This mechanism led to greater dispersal of plutonium and americium than would be expected by physical transport of discrete hot particles alone.« less

Technical approaches to reducing the threat of nuclear terrorism

NASA Astrophysics Data System (ADS)

Priedhorsky, William C.

2005-04-01

The threat of a nuclear attack on the United States by terrorists using a smuggled weapon is now considered more likely than an attack by a nuclear-armed ballistic missle. Consequently it is important to understand what can be done to detect and intercept a nuclear weapon being smuggled into the United States. A significant quantity of smuggled nuclear material has been intercepted already, but science and technology have so far contributed little to its interception. The critical special nuclear materials, plutonium and highly enriched uranium, are only weakly radioactive and detection of their radioactivity is limited both by atmospheric attenuation and by competition with natural backgrounds. Although many schemes for long-range detection of radioactivity have been proposed, none so far appears feasible. Detection of nuclear radiation can be improved using new technologies and sensing systems, but it will still be possible only at relatively small distances. Consequently the best approach to containing dangerous nuclear materials is at their sources; containment within lengthy borders and large areas is extremely difficult.

Evaluation of isotopic composition of fast reactor core in closed nuclear fuel cycle

NASA Astrophysics Data System (ADS)

Tikhomirov, Georgy; Ternovykh, Mikhail; Saldikov, Ivan; Fomichenko, Peter; Gerasimov, Alexander

2017-09-01

The strategy of the development of nuclear power in Russia provides for use of fast power reactors in closed nuclear fuel cycle. The PRORYV (i.e. «Breakthrough» in Russian) project is currently under development. Within the framework of this project, fast reactors BN-1200 and BREST-OD-300 should be built to, inter alia, demonstrate possibility of the closed nuclear fuel cycle technologies with plutonium as a main source of energy. Russia has a large inventory of plutonium which was accumulated in the result of reprocessing of spent fuel of thermal power reactors and conversion of nuclear weapons. This kind of plutonium will be used for development of initial fuel assemblies for fast reactors. The closed nuclear fuel cycle concept of the PRORYV assumes self-supplied mode of operation with fuel regeneration by neutron capture reaction in non-enriched uranium, which is used as a raw material. Operating modes of reactors and its characteristics should be chosen so as to provide the self-sufficient mode by using of fissile isotopes while refueling by depleted uranium and to support this state during the entire period of reactor operation. Thus, the actual issue is modeling fuel handling processes. To solve these problems, the code REPRORYV (Recycle for PRORYV) has been developed. It simulates nuclide streams in non-reactor stages of the closed fuel cycle. At the same time various verified codes can be used to evaluate in-core characteristics of a reactor. By using this approach various options for nuclide streams and assess the impact of different plutonium content in the fuel, fuel processing conditions, losses during fuel processing, as well as the impact of initial uncertainties on neutron-physical characteristics of reactor are considered in this study.

Review of Excess Weapons Plutonium Disposition LLNL Contract Work in Russia-(English)

DOE Office of Scientific and Technical Information (OSTI.GOV)

Jardine, L; Borisov, G B

This third meeting of the recently completed and ongoing Russian plutonium immobilization contract work was held at the State Education Center (SEC) in St. Petersburg on January 14-18, 2002. The meeting agenda is reprinted here as Appendix A and the attendance list as Appendix B. The meeting had 58 Russian participants from 21 Russian organizations, including the industrial sites (Mayak, Krasonayarsk-26, Tomsk), scientific institutes (VNIINM, KRI, VNIPIPT, RIAR), design organizations (VNIPIET and GSPI), universities (Nyzhny Novgorod, Urals Technical), Russian Academy of Sciences (Institute of Physical Chemistry or IPhCh, Institute of Ore-Deposit Geology, Petrography, Mineralogy, and Geochemistry or IGEM), Radon-Moscow, S&TCmore » Podol'osk, Kharkov-Ukraine, GAN-SEC-NRS and SNIIChM, the RF Ministry of Atomic Energy (Minatom) and Gosatomnadzor (GAN). This volume, published by LLNL, documents this third annual meeting. Forty-nine technical papers were presented by the Russian participants, and nearly all of these have been collected in this Proceedings. The two objectives for the meeting were to: (1) Bring together the Russian organizations, experts, and managers performing this contract work into one place for four days to review and discuss their work amongst each other. (2) Publish a meeting summary and proceedings of all the excellent Russian plutonium immobilization and other plutonium disposition contract work in one document so that the wide extent of the Russian immobilization activities are documented, referencable and available for others to use, as were the Proceedings of the two previous meetings. Attendees gave talks describing their LLNL contract work and submitted written papers documenting their contract work (in English and Russian), in both hard copy and on computer disks. Simultaneous translation into Russian and English was used for presentations made at the State Region Educational Center (SEC).« less

Carrying a Weapon to School: The Influence of Youth Assets at Home and School

ERIC Educational Resources Information Center

Marsh, Shawn C.; Evans, William P.

2007-01-01

Eighth and tenth grade students (n= 1,619) reported on exposure to risk and protective assets in their day-to-day lives. The relationship between carrying a weapon to school and risk and protective factors in the home and school ecological domains was explored through logistic regression conducted separately by gender. Environmental control in the…

DOE Office of Scientific and Technical Information (OSTI.GOV)

Rim, Jung H.; Kuhn, Kevin J.; Tandon, Lav

Nuclear forensics techniques, including micro-XRF, gamma spectrometry, trace elemental analysis and isotopic/chronometric characterization were used to interrogate two, potentially related plutonium metal foils. These samples were submitted for analysis with only limited production information, and a comprehensive suite of forensic analyses were performed. Resulting analytical data was paired with available reactor model and historical information to provide insight into the materials’ properties, origins, and likely intended uses. Both were super-grade plutonium, containing less than 3% 240Pu, and age-dating suggested that most recent chemical purification occurred in 1948 and 1955 for the respective metals. Additional consideration of reactor modelling feedback andmore » trace elemental observables indicate plausible U.S. reactor origin associated with the Hanford site production efforts. In conclusion, based on this investigation, the most likely intended use for these plutonium foils was 239Pu fission foil targets for physics experiments, such as cross-section measurements, etc.« less

Critical assembly: A technical history of Los Alamos during the Oppenheimer years, 1943--1945

DOE Office of Scientific and Technical Information (OSTI.GOV)

Hoddeson, L.; Henriksen, P.W.; Meade, R.A.

1993-11-01

This volume treats the technical research that led to the first atomic bombs. The authors explore how the ``critical assembly`` of scientists, engineers, and military Personnel at Los Alamos collaborated during World War II, blending their traditions to create a new approach to large-scale research. The research was characterized by strong mission orientation, multidisciplinary teamwork, expansion of the scientists` traditional methodology with engineering techniques, and a trail-and-error methodology responding to wartime deadlines. The book opens with an introduction laying out major themes. After a synopsis of the prehistory of the bomb project, from the discovery of nuclear fission to themore » start of the Manhattan Engineer District, and an overview of the early materials program, the book examines the establishment of the Los Alamos Laboratory, the implosion and gun assembly programs, nuclear physics research, chemistry and metallurgy, explosives, uranium and plutonium development, confirmation of spontaneous fission in pile-produced plutonium, the thermonuclear bomb, critical assemblies, the Trinity test, and delivery of the combat weapons.« less

Decommissioning, Dismantling and Disarming: a Unique Information Showroom Inside the G2 Reactor at Marcoule Centre (France) - 12068

DOE Office of Scientific and Technical Information (OSTI.GOV)

Volant, Emmanuelle; Garnier, Cedric

2012-07-01

The paper aims at presenting the new information showroom called 'Escom G2' (for 'Espace Communication') inaugurated by the French Atomic Energy and Alternative Energies Commission (CEA) in spring 2011. This showroom is settled directly inside the main building of the G2 nuclear reactor: a facility formerly dedicated to weapon-grade plutonium production since the late 1950's at the Marcoule nuclear centre, in south of France. After its shutdown, and reprocessing of the last spent fuels, a first dismantling step was successfully completed from 1986 to 1996. Unique in France and in Europe, Escom G2 is focused on France dismantling expertise andmore » its action for disarmament. This showroom comprises of a 300-square meters permanent exhibition, organized around four themes: France strategy for disarmament, decommissioning and dismantling technical aspects, uranium and plutonium production cycles. Each of these topics is illustrated with posters, photos, models and technical pieces from the dismantled plants. It is now used to present France's action in disarmament to highly ranked audiences such as: state representatives, diplomats, journalists... The paper explains the background story of this original project. As a matter of fact, in 1996 France was the first nuclear state to decide to shut down and dismantle its fissile material production facilities for nuclear weapons. First, the paper presents the history of the G2 reactor in the early ages of Marcoule site, its operating highlights as well as its main dismantling operations, are presented. In Marcoule, where the three industrial-scale reactors G1, G2 and G3 used to be operated for plutonium production (to be then reprocessed in the nearby UP1 plant), the initial dismantling phase has now been completed (in 1980's for G1 and in 1996 for G2 and G3). The second phase, aimed at completely dismantling these three reactors, will restart in 2020, and is directly linked to the opening of a future national storage facility for irradiated graphite waste. Then, the paper recalls communication events and official visits hosted in Pierrelatte and Marcoule, following a formal invitation from the French President Mr. Nicolas Sarkozy. These visits, which were organized in order to illustrate the irreversibility of these dismantling operations, allowed visitors to discovers places that used to be former highly classified areas. Three official visits were organized in 2008 and 2009 for representatives of the Conference on Disarmament Member States, non-governmental experts and journalists. All participants visited the dismantled uranium enrichment plant in Pierrelatte, the G2 reactor and the UP1 plant in Marcoule. The visits were successful and visitors were especially impressed by the G2 reactor and its massive industrial architecture, symbolic of the early ages of nuclear history. In late 2010, this feedback convinced CEA Military Application Directorate (CEA DAM) that a permanent showroom could be installed inside the reactor, making it possible to preserve the cultural value of this historical landmark, and to continue its ongoing effort of communication and outreach. The paper explains the design of this concept: the museography project with a professional designer, the communication material conception and the features of such an original place. (authors)« less

KSC-2011-6696

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- In the high bay of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida, the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission is attached to the MMRTG integration cart. The cart will be used to install the MMRTG on the Curiosity rover for a fit check. The wheels of the rover appear to stick out on either side of the cart. The MMRTG will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6687

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- In the high bay of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida, spacecraft technicians from NASA's Jet Propulsion Laboratory connect a crane to a turning fixture connected to the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission. The fixture will lift and lower the MMRTG onto the MMRTG integration cart. The cart will be used to install the MMRTG on Curiosity for a fit check. The MMRTG will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6686

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- In the high bay of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida, spacecraft technicians from NASA's Jet Propulsion Laboratory guide a turning fixture onto the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission. The fixture will be used to lift and lower the MMRTG onto the MMRTG integration cart. The cart will be used to install the MMRTG on Curiosity for a fit check. The MMRTG will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6691

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- In the high bay of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida, spacecraft technicians from NASA's Jet Propulsion Laboratory rotate the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission, using the turning fixture to align the MMRTG with the angle of the MMRTG integration cart behind it. The cart will be used to install the MMRTG on the Curiosity rover for a fit check. The rover is on an elevated work stand, at right. The MMRTG will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6689

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- In the high bay of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida, spacecraft technicians from NASA's Jet Propulsion Laboratory attach guide ropes to the turning fixture connected to the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission during preparations to lift it from its support base. The turning fixture will lift and lower the MMRTG onto the MMRTG integration cart. The cart will be used to install the MMRTG on Curiosity for a fit check. The MMRTG will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6690

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- In the high bay of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida, a crane lifts the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission from its support base, at left, toward the MMRTG integration cart behind it. The cart will be used to install the MMRTG on the Curiosity rover for a fit check. The rover appears above the heads of the spacecraft technicians, at right. The MMRTG will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6680

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- At NASA's Kennedy Space Center in Florida, a forklift positions the protective mesh container enclosing the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission onto the floor of the airlock of the Payload Hazardous Servicing Facility (PHSF). The container, known as the "gorilla cage," protects the MMRTG and allows any excess heat generated to dissipate into the air. In the PHSF, the MMRTG temporarily will be installed on the MSL rover, Curiosity, for a fit check but will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6727

NASA Image and Video Library

2011-07-14

CAPE CANAVERAL, Fla. -- At NASA's Kennedy Space Center in Florida, a forklift lifts the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission into the MMRTG trailer. The MMRTG is enclosed in a mesh container, known as the "gorilla cage," which protects it during transport and allows any excess heat generated to dissipate into the air. The MMRTG is being moved to the RTG storage facility following a fit check on MSL's Curiosity rover in the Payload Hazardous Servicing Facility (PHSF). The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Troy Cryder

KSC-2011-6667

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- In the high bay of the RTG storage facility at NASA's Kennedy Space Center in Florida, the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission is enclosed in a protective mesh container, known as the "gorilla cage," for transport to the Payload Hazardous Servicing Facility (PHSF). The cage protects the MMRTG and allows any excess heat generated to dissipate into the air. In the PHSF, the MMRTG temporarily will be installed on the MSL rover, Curiosity, for a fit check but will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6722

NASA Image and Video Library

2011-07-14

CAPE CANAVERAL, Fla. -- In the airlock of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida, t he multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission awaits transport to the RTG storage facility. The MMRTG is enclosed in a mesh container, known as the "gorilla cage," which protects it during transport and allows any excess heat generated to dissipate into the air. The MMRTG was in the PHSF for a fit check on MSL's Curiosity rover. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Troy Cryder

KSC-2011-6726

NASA Image and Video Library

2011-07-14

CAPE CANAVERAL, Fla. -- A forklift transfers the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission from the airlock of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida to the MMRTG trailer. The MMRTG is enclosed in a mesh container, known as the "gorilla cage," which protects it during transport and allows any excess heat generated to dissipate into the air. The MMRTG is being moved to the RTG storage facility following a fit check on MSL's Curiosity rover in the PHSF. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Troy Cryder

KSC-2011-6682

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- In the airlock of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida, the protective mesh container enclosing the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission is lifted from around the MMRTG. The container, known as the "gorilla cage," protects the MMRTG during transport and allows any excess heat generated to dissipate into the air. In the PHSF, the MMRTG temporarily will be installed on the MSL rover, Curiosity, for a fit check but will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6735

NASA Image and Video Library

2011-07-14

CAPE CANAVERAL, Fla. -- A forklift moves the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission into the high bay of the RTG storage facility (RTGF) at NASA's Kennedy Space Center in Florida. The MMRTG is enclosed in a mesh container, known as the "gorilla cage," which protects it during transport and allows any excess heat generated to dissipate into the air. The MMRTG is returning to the RTGF following a fit check on MSL's Curiosity rover in the Payload Hazardous Servicing Facility (PHSF). The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Troy Cryder

KSC-2011-6652

NASA Image and Video Library

2011-06-30

CAPE CANAVERAL, Fla. -- Workers reconnect the coolant hoses to the shipping cask enclosing the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory mission upon its arrival in the high bay of the RTG storage facility at NASA's Kennedy Space Center in Florida. Coolant flows through the hoses to dissipate any excess heat generated by the MMRTG. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for evidence on whether Mars has had environments favorable to microbial life, including chemical ingredients for life. The unique rover will use a laser to look inside rocks and release its gasses so that the rover’s spectrometer can analyze and send the data back to Earth. Launch of MSL aboard a United Launch Alliance Atlas V rocket is scheduled for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station in Florida. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Frankie Martin

KSC-2011-6734

NASA Image and Video Library

2011-07-14

CAPE CANAVERAL, Fla. -- A forklift moves the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission from the MMRTG trailer to the RTG storage facility (RTGF) at NASA's Kennedy Space Center in Florida. The MMRTG is enclosed in a mesh container, known as the "gorilla cage," which protects it during transport and allows any excess heat generated to dissipate into the air. The MMRTG is returning to the RTGF following a fit check on MSL's Curiosity rover in the Payload Hazardous Servicing Facility (PHSF). The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Troy Cryder

KSC-2011-6725

NASA Image and Video Library

2011-07-14

CAPE CANAVERAL, Fla. -- A forklift carrying the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission backs away from the airlock of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida. The MMRTG is enclosed in a mesh container, known as the "gorilla cage," which protects it during transport and allows any excess heat generated to dissipate into the air. The MMRTG is being moved to the RTG storage facility following a fit check on MSL's Curiosity rover in the PHSF. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Troy Cryder

KSC-2011-6736

NASA Image and Video Library

2011-07-14

CAPE CANAVERAL, Fla. -- Department of Energy workers park the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission in the high bay of the RTG storage facility (RTGF) at NASA's Kennedy Space Center in Florida. The MMRTG is enclosed in a mesh container, known as the "gorilla cage," which protects it during transport and allows any excess heat generated to dissipate into the air. The MMRTG is returning to the RTGF following a fit check on MSL's Curiosity rover in the Payload Hazardous Servicing Facility (PHSF). The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Troy Cryder

KSC-2011-6679

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- At NASA's Kennedy Space Center in Florida, a forklift carries the protective mesh container, known as the "gorilla cage," enclosing the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission into the airlock of the Payload Hazardous Servicing Facility (PHSF). The cage protects the MMRTG and allows any excess heat generated to dissipate into the air. In the PHSF, the MMRTG temporarily will be installed on the MSL rover, Curiosity, for a fit check but will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6743

NASA Image and Video Library

2011-07-14

CAPE CANAVERAL, Fla. -- In the high bay of the RTG storage facility (RTGF) at NASA's Kennedy Space Center in Florida, the mesh container enclosing the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission is lifted from around the MMRTG. The container, known as the "gorilla cage," protects the MMRTG during transport and allows any excess heat generated to dissipate into the air. The cage is being removed following the return of the MMRTG to the RTGF from a fit check on MSL's Curiosity rover in the Payload Hazardous Servicing Facility (PHSF). The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Troy Cryder

KSC-2011-6666

NASA Image and Video Library

2011-06-30

CAPE CANAVERAL, Fla. -- In the RTG storage facility at NASA's Kennedy Space Center in Florida, the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory mission, with guide rods still installed on its support base, has been uncovered on the high bay floor. The MMRTG no longer needs supplemental cooling since any excess heat generated can dissipate into the air in the high bay. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for evidence on whether Mars has had environments favorable to microbial life, including chemical ingredients for life. The unique rover will use a laser to look inside rocks and release its gasses so that the rover’s spectrometer can analyze and send the data back to Earth. Launch of MSL aboard a United Launch Alliance Atlas V rocket is scheduled for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station in Florida. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Frankie Martin

KSC-2011-6721

NASA Image and Video Library

2011-07-14

CAPE CANAVERAL, Fla. -- A forklift approaches the airlock of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida where the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission awaits transport to the RTG storage facility. The MMRTG is enclosed in a mesh container, known as the "gorilla cage," which protects it during transport and allows any excess heat generated to dissipate into the air. The MMRTG was in the PHSF for a fit check on MSL's Curiosity rover. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Troy Cryder

KSC-2011-6704

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- In the high bay of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida, the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission is installed onto the aft of the Curiosity rover for a fit check. In view are the MMRTG's cooling fins which function like the radiator on a car and will reflect any excess heat generated by the MMRTG to prevent interference with the rover's electronics. Next, the MMRTG will be removed and later installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6723

NASA Image and Video Library

2011-07-14

CAPE CANAVERAL, Fla. -- A forklift moves into position to lift the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission from the floor of the Payload Hazardous Servicing Facility (PHSF) airlock at NASA's Kennedy Space Center in Florida. The MMRTG is enclosed in a mesh container, known as the "gorilla cage," which protects it during transport and allows any excess heat generated to dissipate into the air. The MMRTG is being transported to the RTG storage facility following a fit check on MSL's Curiosity rover in the PHSF. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Troy Cryder

KSC-2011-6733

NASA Image and Video Library

2011-07-14

CAPE CANAVERAL, Fla. -- The multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission is lifted from the MMRTG trailer at the RTG storage facility (RTGF) at NASA's Kennedy Space Center in Florida. The MMRTG is enclosed in a mesh container, known as the "gorilla cage," which protects it during transport and allows any excess heat generated to dissipate into the air. The MMRTG is returning to the RTGF following a fit check on MSL's Curiosity rover in the Payload Hazardous Servicing Facility (PHSF). The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Troy Cryder

KSC-2011-6703

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- In the high bay of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida, the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission is installed onto the aft of the Curiosity rover for a fit check. In view are the MMRTG's cooling fins which function like the radiator on a car and will reflect any excess heat generated by the MMRTG to prevent interference with the rover's electronics. Next, the MMRTG will be removed and later installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6717

NASA Image and Video Library

2011-07-13

CAPE CANAVERAL, Fla. -- In the airlock of the Payload Hazardous Servicing Facility at NASA's Kennedy Space Center in Florida, Department of Energy employees prepare the support base of the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission for installation of the mesh container, known as the "gorilla cage." The cage, in the background at right, protects the MMRTG during transport and allows any excess heat generated to dissipate into the air. Transport of the MMRTG to the RTG storage facility follows the completion of the MMRTG fit check on the Curiosity rover. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Kim Shiflett

KSC-2011-6665

NASA Image and Video Library

2011-06-30

CAPE CANAVERAL, Fla. -- In the high bay of the RTG storage facility at NASA's Kennedy Space Center in Florida, the external and internal protective layers of the shipping cask are lifted away from the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory mission. The MMRTG no longer needs supplemental cooling since any excess heat generated can dissipate into the air in the high bay. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for evidence on whether Mars has had environments favorable to microbial life, including chemical ingredients for life. The unique rover will use a laser to look inside rocks and release its gasses so that the rover’s spectrometer can analyze and send the data back to Earth. Launch of MSL aboard a United Launch Alliance Atlas V rocket is scheduled for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station in Florida. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Frankie Martin

KSC-2011-6646

NASA Image and Video Library

2011-06-30

CAPE CANAVERAL, Fla. -- The multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission, enclosed in a shipping cask in the MMRTG trailer, arrives at the RTG storage facility at NASA's Kennedy Space Center in Florida. During transport, coolant flows through hoses connected to the cask to dissipate any excess heat generated by the MMRTG. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for evidence on whether Mars has had environments favorable to microbial life, including chemical ingredients for life. The unique rover will use a laser to look inside rocks and release its gasses so that the rover’s spectrometer can analyze and send the data back to Earth. Launch of MSL aboard a United Launch Alliance Atlas V rocket is scheduled for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station in Florida. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Frankie Martin

KSC-2011-6724

NASA Image and Video Library

2011-07-14

CAPE CANAVERAL, Fla. -- A forklift moves into position to lift the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission from the floor of the Payload Hazardous Servicing Facility (PHSF) airlock at NASA's Kennedy Space Center in Florida. The MMRTG is enclosed in a mesh container, known as the "gorilla cage," which protects it during transport and allows any excess heat generated to dissipate into the air. The MMRTG is being moved to the RTG storage facility following a fit check on MSL's Curiosity rover in the PHSF. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Troy Cryder

KSC-2011-6681

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- In the airlock of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida, the protective mesh container enclosing the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission is lifted from around the MMRTG. The container, known as the "gorilla cage," protects the MMRTG during transport and allows any excess heat generated to dissipate into the air. In the PHSF, the MMRTG temporarily will be installed on the MSL rover, Curiosity, for a fit check but will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6728

NASA Image and Video Library

2011-07-14

CAPE CANAVERAL, Fla. -- At NASA's Kennedy Space Center in Florida, a forklift lifts the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission into the MMRTG trailer. The MMRTG is enclosed in a mesh container, known as the "gorilla cage," which protects it during transport and allows any excess heat generated to dissipate into the air. The MMRTG is being moved to the RTG storage facility following a fit check on MSL's Curiosity rover in the Payload Hazardous Servicing Facility (PHSF). The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Troy Cryder

KSC-2011-6675

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- Outside the RTG storage facility at NASA's Kennedy Space Center in Florida, the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission, enclosed in the protective mesh container known as the "gorilla cage," is strapped down inside the MMRTG trailer for transport to the Payload Hazardous Servicing Facility (PHSF). The cage protects the MMRTG and allows any excess heat generated to dissipate into the air. In the PHSF, the MMRTG temporarily will be installed on the MSL rover, Curiosity, for a fit check but will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6654

NASA Image and Video Library

2011-06-30

CAPE CANAVERAL, Fla. -- In the high bay of the RTG storage facility at NASA's Kennedy Space Center in Florida, Innovative Health Applications employee Mike McPherson measures the level of radioactivity emitted from the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory mission, enclosed in a shipping cask at right. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for evidence on whether Mars has had environments favorable to microbial life, including chemical ingredients for life. The unique rover will use a laser to look inside rocks and release its gasses so that the rover’s spectrometer can analyze and send the data back to Earth. Launch of MSL aboard a United Launch Alliance Atlas V rocket is scheduled for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station in Florida. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Frankie Martin

KSC-2011-6661

NASA Image and Video Library

2011-06-30

CAPE CANAVERAL, Fla. -- In the high bay of the RTG storage facility at NASA's Kennedy Space Center in Florida, Innovative Health Applications employee David Lake measures the level of radioactivity emitted from the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory mission as the external protective layer of the shipping cask is removed. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for evidence on whether Mars has had environments favorable to microbial life, including chemical ingredients for life. The unique rover will use a laser to look inside rocks and release its gasses so that the rover’s spectrometer can analyze and send the data back to Earth. Launch of MSL aboard a United Launch Alliance Atlas V rocket is scheduled for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station in Florida. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Frankie Martin

KSC-2011-6656

NASA Image and Video Library

2011-06-30

CAPE CANAVERAL, Fla. -- In the high bay of the RTG storage facility at NASA's Kennedy Space Center in Florida, Department of Energy contractor employees attach cables to the shipping cask enclosing the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory mission during preparations to lift it from its transportation pallet. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for evidence on whether Mars has had environments favorable to microbial life, including chemical ingredients for life. The unique rover will use a laser to look inside rocks and release its gasses so that the rover’s spectrometer can analyze and send the data back to Earth. Launch of MSL aboard a United Launch Alliance Atlas V rocket is scheduled for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station in Florida. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Frankie Martin

KSC-2011-6655

NASA Image and Video Library

2011-06-30

CAPE CANAVERAL, Fla. -- In the high bay of the RTG storage facility at NASA's Kennedy Space Center in Florida, preparations are under way to attach the shipping cask enclosing the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory mission to the cables that will lift it from its transportation pallet. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for evidence on whether Mars has had environments favorable to microbial life, including chemical ingredients for life. The unique rover will use a laser to look inside rocks and release its gasses so that the rover’s spectrometer can analyze and send the data back to Earth. Launch of MSL aboard a United Launch Alliance Atlas V rocket is scheduled for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station in Florida. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Frankie Martin

KSC-2011-6657

NASA Image and Video Library

2011-06-30

CAPE CANAVERAL, Fla. -- In the high bay of the RTG storage facility at NASA's Kennedy Space Center in Florida, a Department of Energy contractor employee attaches a crane to the shipping cask enclosing the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory mission during preparations to lift it from its transportation pallet. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for evidence on whether Mars has had environments favorable to microbial life, including chemical ingredients for life. The unique rover will use a laser to look inside rocks and release its gasses so that the rover’s spectrometer can analyze and send the data back to Earth. Launch of MSL aboard a United Launch Alliance Atlas V rocket is scheduled for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station in Florida. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Frankie Martin

KSC-2011-6729

NASA Image and Video Library

2011-07-14

CAPE CANAVERAL, Fla. -- At NASA's Kennedy Space Center in Florida, preparations are under way to secure the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission in the MMRTG trailer. The MMRTG is enclosed in a mesh container, known as the "gorilla cage," which protects it during transport and allows any excess heat generated to dissipate into the air. The MMRTG is being moved to the RTG storage facility following a fit check on MSL's Curiosity rover in the Payload Hazardous Servicing Facility (PHSF). The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Troy Cryder

KSC-2011-6692

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- In the high bay of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida, spacecraft technicians from NASA's Jet Propulsion Laboratory guide the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission on the turning fixture toward the MMRTG integration cart. The cart will be used to install the MMRTG on the Curiosity rover for a fit check. The rover is on an elevated work stand, at right. The MMRTG will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6693

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- In the high bay of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida, spacecraft technicians from NASA's Jet Propulsion Laboratory guide the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission on the turning fixture toward the MMRTG integration cart. The cart will be used to install the MMRTG on the Curiosity rover for a fit check. The rover is on an elevated work stand, at right. The MMRTG will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6694

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- In the high bay of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida, spacecraft technicians from NASA's Jet Propulsion Laboratory position the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission on the turning fixture above the MMRTG integration cart. The cart will be used to install the MMRTG on the Curiosity rover for a fit check. The rover is on an elevated work stand, at right. The MMRTG will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6685

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- Workers dressed in clean room attire, known as bunny suits, transfer the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission on its holding base through the doors of the airlock of the Payload Hazardous Servicing Facility (PHSF) into the facility's high bay. In the high bay, the MMRTG temporarily will be installed on the MSL rover, Curiosity (in the background, at right), for a fit check using the MMRTG integration cart (in the background, at left). The MMRTG will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

Recent weapon carrying and substance use among United States Virgin Islands youth.

PubMed

Lloyd, J J; Delva, J; Arria, A M

2000-08-01

The objective of the present study was to estimate the strength of the associations between recent weapon carrying and alcohol, cigarette, and illicit drug use among US Virgin Islands (USVI) youth. Data from 1,124 students in Grades 7-12 were analyzed using the conditional form of multiple logistic regression. Compared with youth who did not carry a weapon. youth who carried a weapon were more likely to be male and recent cigarette, alcohol, and illicit drug users. After matching on school and controlling for age, sex, race, neigborhood characteristics, and affiliation with friends who use alcohol and illegal drugs, the associations with cigarette smoking and illicit drug use remained both moderate and statistically significant (odds ratio [OR] = 4.31, p < .001; OR = 2.99, p < .001, respectively). These findings identify a potentially high-risk population that could be targeted for interventions to reduce weapon carrying among youth.

Method for removal of metal atoms from aqueous solution using suspended plant cells

DOEpatents

Jackson, Paul J.; Torres, deceased, Agapito P.; Delhaize, Emmanuel

1992-01-01

The use of plant suspension cultures to remove ionic metallic species and TNT-based explosives and their oxidation products from aqueous solution is described. Several plant strains were investigated including D. innoxia, Citrus citrus, and Black Mexican Sweet Corn. All showed significant ability to remove metal ions. Ions removed to sub-ppm levels include barium, iron, and plutonium. D. innoxia cells growing in media containing weapons effluent contaminated with Ba.sup.2+ also remove TNT, other explosives and oxidation products thereof from solution. The use of dead, dehydrated cells were also found to be of use in treating waste directly.

Method for removal of explosives from aqueous solution using suspended plant cells

DOEpatents

Jackson, Paul J.; Torres, deceased, Agapito P.; Delhaize, Emmanuel

1994-01-01

The use of plant suspension cultures to remove ionic metallic species and TNT-based explosives and their oxidation products from aqueous solution is described. Several plant strains were investigated including D. innoxia, Citrus citrus, and Black Mexican Sweet Corn. All showed significant ability to remove metal ions. Ions removed to sub-ppm levels include barium, iron, and plutonium. D. innoxia cells growing in media containing weapons effluent contaminated with Ba.sup.2+ also remove TNT, other explosives and oxidation products thereof from solution. The use of dead, dehydrated cells was also found to be of use in treating waste directly.

Effects of a youth substance use prevention program on stealing, fighting, and weapon use.

PubMed

Nieri, Tanya; Apkarian, Jacob; Kulis, Stephen; Marsiglia, Flavio Francisco

2015-02-01

Using a sample of sixth graders in 11 public schools in a large Southwestern city, this longitudinal study examined how a model substance use prevention program, keepin' it REAL, that was implemented in 7th grade, influenced three other problem behaviors (fighting, weapon use, stealing), measured in 8th grade. Using a non-equivalent control group design, we compared 259 students in the intervention to 322 students in a treatment-as-usual condition. At baseline, 37% of the sample reported fighting in the last 30 days; 31% reported stealing in the last 30 days, and 16% reported using a weapon in the last 30 days. Regression analyses adjusted for students nested in schools through multi-level modeling and for missing data through multiple imputation. We found that at posttest the rates of all three behaviors were lower in the intervention group than the control group at posttest: 35 versus 37% got into a fight in the last 30 days; 24 versus 31% stole something in the last 30 days; and 16 versus 25% used a weapon in the last 30 days. The program impact for fighting and stealing was not statistically significant and involved minimal effect sizes. The program impact for weapon use was not statistically significant but had an effect size comparable to that for other problem behavior interventions. Promoting positive development via life skills may be a key to broadening program impact.

Effects of a youth substance use prevention program on stealing, fighting, and weapon use

PubMed Central

Nieri, Tanya; Apkarian, Jacob; Kulis, Stephen; Marsiglia, Flavio Francisco

2014-01-01

Using a sample of sixth graders in 11 public schools in a large Southwestern city, this longitudinal study examined how a model substance use prevention program, keepin’ it REAL, that was implemented in 7th grade, influenced three other problem behaviors (fighting, weapon use, stealing), measured in 8th grade. Using a non-equivalent control group design, we compared 259 students in the intervention to 322 students in a treatment-as-usual condition. At baseline, 37% of the sample reported fighting in the last 30 days; 31% reported stealing in the last 30 days, and 16% reported using a weapon in the last 30 days. Regression analyses adjusted for students nested in schools through multi-level modeling and for missing data through multiple imputation. We found that at posttest the rates of all three behaviors were lower in the intervention group than the control group at posttest: 35% versus 37% got into a fight in the last 30 days; 24% versus 31% stole something in the last 30 days; and 16% versus 25% used a weapon in the last 30 days. The program impact for fighting and stealing was not statistically significant and involved minimal effect sizes. The program impact for weapon use was not statistically significant but had an effect size comparable to that for other problem behavior interventions. Promoting positive development via life skills may be a key to broadening program impact. PMID:25352527

On the distribution and inventories of radionuclides in dated sediments around the Swedish coast.

PubMed

Olszewski, Grzegorz; Andersson, Pål; Lindahl, Patric; Eriksson, Mats

2018-06-01

The activity concentrations and distribution of 137 Cs, 238 Pu, 239+240 Pu, 241 Am, and 210 Pb was determined by the analysis of six sediment cores from the Baltic Sea and Kattegat. The chronology of the sediment cores has been used to evaluate the origin and time trend of the radionuclide sources in these sediments. The sediment cores were dated with a 210 Pb model and the results were validated with fallout peaks, assumed to originate from the global nuclear weapons testing and the Chernobyl accident. Source identification, using the isotopic and radionuclide activity ratios, showed that the Chernobyl accident is the main source of 137 Cs in the Baltic Sea; for 239+240 Pu and 241 Am the dominant source was shown to be fallout from nuclear weapons tests. For 238 Pu and 241 Am the Chernobyl accident had a significant impact on the direct fallout into the Baltic Proper, with up to a 65% contribution in the sediment slices dated to 1986. In these sediment slices the maximum activity ratios of 238 Pu/ 239+240 Pu and 241 Am/ 239+240 Pu were 0.314 ± 0.008 and 1.29 ± 0.06, respectively. The ratios clearly deviate from the corresponding ratios for global nuclear weapons fallout (around 0.028 and 0.54, respectively). Calculated inventories were 63-175 Bq·m -2 for 239+240 Pu, 2.8-7.8 for 238 Pu Bq·m -2 and 0.92-44.4 kBq·m -2 for 137 Cs. Different fallout patterns for 137 Cs and plutonium isotopes from the Chernobyl accident were confirmed through depth profiles analyses. The maximum inventory of 137 Cs was observed in the Bothnian Sea, while Chernobyl-derived plutonium was found to be mostly present in Northern Baltic Proper. The radionuclides distribution in the depth profiles shows how contaminated water affects the sediment as it passes sampling stations according to the current circulation pattern in the Baltic Sea. Additionally, the effect of increased activity concentrations from of river discharges in the most contaminated area in the Bothnian Sea was observed. Copyright © 2017 Elsevier Ltd. All rights reserved.

CHEMICAL DIFFERENCES BETWEEN SLUDGE SOLIDS AT THE F AND H AREA TANK FARMS

DOE Office of Scientific and Technical Information (OSTI.GOV)

Reboul, S.

2012-08-29

The primary source of waste solids received into the F Area Tank Farm (FTF) was from PUREX processing performed to recover uranium and plutonium from irradiated depleted uranium targets. In contrast, two primary sources of waste solids were received into the H Area Tank Farm (HTF): a) waste from PUREX processing; and b) waste from H-modified (HM) processing performed to recover uranium and neptunium from burned enriched uranium fuel. Due to the differences between the irradiated depleted uranium targets and the burned enriched uranium fuel, the average compositions of the F and H Area wastes are markedly different from onemore » another. Both F and H Area wastes contain significant amounts of iron and aluminum compounds. However, because the iron content of PUREX waste is higher than that of HM waste, and the aluminum content of PUREX waste is lower than that of HM waste, the iron to aluminum ratios of typical FTF waste solids are appreciably higher than those of typical HTF waste solids. Other constituents present at significantly higher concentrations in the typical FTF waste solids include uranium, nickel, ruthenium, zinc, silver, cobalt and copper. In contrast, constituents present at significantly higher concentrations in the typical HTF waste solids include mercury, thorium, oxalate, and radionuclides U-233, U-234, U-235, U-236, Pu-238, Pu-242, Cm-244, and Cm-245. Because of the higher concentrations of Pu-238 in HTF, the long-term concentrations of Th-230 and Ra-226 (from Pu-238 decay) will also be higher in HTF. The uranium and plutonium distributions of the average FTF waste were found to be consistent with depleted uranium and weapons grade plutonium, respectively (U-235 comprised 0.3 wt% of the FTF uranium, and Pu-240 comprised 6 wt% of the FTF plutonium). In contrast, at HTF, U-235 comprised 5 wt% of the uranium, and Pu-240 comprised 17 wt% of the plutonium, consistent with enriched uranium and high burn-up plutonium. X-ray diffraction analyses of various FTF and HTF samples indicated that the primary crystalline compounds of iron in sludge solids are Fe{sub 2}O{sub 3}, Fe{sub 3}O{sub 4}, and FeO(OH), and the primary crystalline compounds of aluminum are Al(OH){sub 3} and AlO(OH). Also identified were carbonate compounds of calcium, magnesium, and sodium; a nitrated sodium aluminosilicate; and various uranium compounds. Consistent with expectations, oxalate compounds were identified in solids associated with oxalic acid cleaning operations. The most likely oxidation states and chemical forms of technetium are assessed in the context of solubility, since technetium-99 is a key risk driver from an environmental fate and transport perspective. The primary oxidation state of technetium in SRS sludge solids is expected to be Tc(IV). In salt waste, the primary oxidation state is expected to be Tc(VII). The primary form of technetium in sludge is expected to be a hydrated technetium dioxide, TcO{sub 2} {center_dot} xH{sub 2}O, which is relatively insoluble and likely co-precipitated with iron. In salt waste solutions, the primary form of technetium is expected to be the very soluble pertechnetate anion, TcO{sub 4}{sup -}. The relative differences between the F and H Tank Farm waste provide a basis for anticipating differences that will occur as constituents of FTF and HTF waste residue enter the environment over the long-term future. If a constituent is significantly more dominant in one of the Tank Farms, its long-term environmental contribution will likely be commensurately higher, assuming the environmental transport conditions of the two Tank Farms share some commonality. It is in this vein that the information cited in this document is provided - for use during the generation, assessment, and validation of Performance Assessment modeling results.« less

Emitted radiation characteristics of plutonium dioxide radioisotope thermoelectric generators

NASA Technical Reports Server (NTRS)

Gingo, P. J.; Steyn, J. J.

1971-01-01

The nuclear and emitted radiation characteristics of the radioisotope elements and impurities in commercial grade plutonium dioxide are presented in detail. The development of the methods of analysis are presented. Radioisotope thermoelectric generators (RTG) of 1575, 3468 and 5679 thermal watts are characterized with respect to neutron and gamma photon source strength as well as spatial and number flux distribution. The results are presented as a function of detector position and light element contamination concentration for fuel age ranging from 'fresh' to 18 years. The data may be used to obtain results for given O-18 and Pu-236 concentrations. The neutron and gamma photon flux and dose calculations compare favorably with reported experimental values for SNAP-27.

Routine inspection effort required for verification of a nuclear material production cutoff convention

DOE Office of Scientific and Technical Information (OSTI.GOV)

Dougherty, D.; Fainberg, A.; Sanborn, J.

On 27 September 1993, President Clinton proposed {open_quotes}... a multilateral convention prohibiting the production of highly enriched uranium or plutonium for nuclear explosives purposes or outside of international safeguards.{close_quotes} The UN General Assembly subsequently adopted a resolution recommending negotiation of a non-discriminatory, multilateral, and internationally and effectively verifiable treaty (hereinafter referred to as {open_quotes}the Cutoff Convention{close_quotes}) banning the production of fissile material for nuclear weapons. The matter is now on the agenda of the Conference on Disarmament, although not yet under negotiation. This accord would, in effect, place all fissile material (defined as highly enriched uranium and plutonium) produced aftermore » entry into force (EIF) of the accord under international safeguards. {open_quotes}Production{close_quotes} would mean separation of the material in question from radioactive fission products, as in spent fuel reprocessing, or enrichment of uranium above the 20% level, which defines highly enriched uranium (HEU). Facilities where such production could occur would be safeguarded to verify that either such production is not occurring or that all material produced at these facilities is maintained under safeguards.« less

10. AERIAL VIEW LOOKING NORTHWEST AT THE 400AREA COMPLEX. THIS ...

Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

10. AERIAL VIEW LOOKING NORTHWEST AT THE 400-AREA COMPLEX. THIS AREA OF THE PLANT MANUFACTURED NON-PLUTONIUM WEAPONS COMPONENTS FROM BERYLLIUM, DEPLETED URANIUM, AND STAINLESS STEEL. THE 400 - AREA ALSO INCLUDED A FACILITY FOR THE MODIFICATION OF SAFE SECURE TRANSPORT VEHICLES FOR SPECIAL NUCLEAR MATERIALS BEING SHIPPED TO AND FROM THE SITE. BUILDING 444, IN THE UPPER RIGHT EDGE OF THE PHOTOGRAPH, WAS THE ORIGINAL PLANT A. THE LARGE BUILDING IN THE TOP OF THE PHOTOGRAPH IS BUILDING 460, BUILT AS A STATE-OF-THE-ART STAINLESS STEEL MANUFACTURING FACILITY (6/27/95). - Rocky Flats Plant, Bounded by Indiana Street & Routes 93, 128 & 72, Golden, Jefferson County, CO

The physics design of accelerator-driven transmutation systems

DOE Office of Scientific and Technical Information (OSTI.GOV)

Venneri, F.

1995-10-01

Nuclear systems under study in the Los Alamos Accelerator-Driven Transmutation Technology program (ADTT) will allow the destruction of nuclear spent fuel and weapons-return plutonium, as well as the production of nuclear energy from the thorium cycle, without a long-lived radioactive waste stream. The subcritical systems proposed represent a radical departure from traditional nuclear concepts (reactors), yet the actual implementation of ADTT systems is based on modest extrapolations of existing technology. These systems strive to keep the best that the nuclear technology has developed over the years, within a sensible conservative design envelope and eventually manage to offer a safe, lessmore » expensive and more environmentally sound approach to nuclear power.« less

Atomic Bomb: The Story of the Manhattan Project; How nuclear physics became a global geopolitical game-changer

NASA Astrophysics Data System (ADS)

Reed, Bruce Cameron

2015-06-01

This volume, prepared by an acknowledged expert on the Manhattan Project, gives a concise, fast-paced account of all major aspects of the project at a level accessible to an undergraduate college or advanced high-school student familiar with some basic concepts of energy, atomic structure, and isotopes. The text describes the underlying scientific discoveries that made nuclear weapons possible, how the project was organized, the daunting challenges faced and overcome in obtaining fissile uranium and plutonium, and in designing workable bombs, the dramatic Trinity test carried out in the desert of southern New Mexico in July 1945, and the bombings of Hiroshima and Nagasaki.

Sources of the transuranic elements plutonium and neptunium in arctic marine sediments.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Cooper, L. W.; Kelley, J. M.; Bond, L. A.

2000-01-01

We report here thermal ionization mass spectrometry measurements of {sup 239}Pu, {sup 240}Pu, {sup 241}Pu, {sup 242}Pu, and {sup 237}Np isolated from oceanic, estuarine, and riverine sediments from the Arctic Ocean Basin. {sup 238}Pu/{sup 239+240}Pu activity ratios are also reported for alpha spectrometric analyses undertaken on a subset of these samples. Our results indicate that the Pu in sediments on the Alaskan shelf and slope, as well as that in the deep basins (Amerasian and Eurasian) of the Arctic Ocean, has its origin in stratospheric and tropospheric fallout. Sediments from the Ob and Yenisei Rivers show isotopic Pu signatures thatmore » are distinctly different from those of northern-hemisphere stratospheric fallout and indicate the presence of weapons-grade Pu originating from nuclear fuel reprocessing wastes generated at Russian facilities within these river catchments. Consequently, sediments of the Eurasian Arctic Ocean, particularly those in the Barents and Kara Seas, probably contain a mixture of Pu from stratospheric fallout, tropospheric fallout, and fuel-reprocessing wastes of riverine origin. In particular, the {sup 241}Pu/{sup 239}Pu ratios observed in these sediments are inconsistent with significant contributions of Pu to the arctic sediments studied from western European reprocessing facilities, principally Sellafield in the UK. Several other potential sources of Pu to arctic sediments can also be excluded as significant based upon the transuranic isotope ratios presented.« less

KSC-2011-6688

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- In the high bay of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida, preparations are under way for a crane to lift the turning fixture connected to the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission from its support base. Between the MMRTG and the spacecraft technicians at right is a mobile plexiglass radiation shield to help minimize the employees' radiation exposure. The turning fixture will lift and lower the MMRTG onto the MMRTG integration cart. The cart will be used to install the MMRTG on Curiosity for a fit check. The MMRTG will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6674

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- Outside the RTG storage facility at NASA's Kennedy Space Center in Florida, the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission, enclosed in the protective mesh container, known as the "gorilla cage," is positioned inside the MMRTG trailer that will transport it to the Payload Hazardous Servicing Facility (PHSF). The cage protects the MMRTG and allows any excess heat generated to dissipate into the air. In the PHSF, the MMRTG temporarily will be installed on the MSL rover, Curiosity, for a fit check but will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6738

NASA Image and Video Library

2011-07-14

CAPE CANAVERAL, Fla. -- A crane is positioned over the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission in the high bay of the RTG storage facility (RTGF) at NASA's Kennedy Space Center in Florida. Preparations are under way to lift the mesh container, known as the "gorilla cage," from the support base on which the MMRTG is resting. The cage protects the MMRTG during transport and allows any excess heat generated to dissipate into the air. The MMRTG is returning to the RTGF following a fit check on MSL's Curiosity rover in the Payload Hazardous Servicing Facility (PHSF). The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Troy Cryder

KSC-2011-6664

NASA Image and Video Library

2011-06-30

CAPE CANAVERAL, Fla. -- In the high bay of the RTG storage facility at NASA's Kennedy Space Center in Florida, a Department of Energy contractor employee guides the external and internal protective layers of the shipping cask as they are lifted from around the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory mission. The MMRTG no longer needs supplemental cooling since any excess heat generated can dissipate into the air in the high bay. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for evidence on whether Mars has had environments favorable to microbial life, including chemical ingredients for life. The unique rover will use a laser to look inside rocks and release its gasses so that the rover’s spectrometer can analyze and send the data back to Earth. Launch of MSL aboard a United Launch Alliance Atlas V rocket is scheduled for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station in Florida. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Frankie Martin

KSC-2011-6737

NASA Image and Video Library

2011-07-14

CAPE CANAVERAL, Fla. -- Department of Energy workers position mobile plexiglass radiation shields around the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission upon its arrival in the high bay of the RTG storage facility (RTGF) at NASA's Kennedy Space Center in Florida. The shields are designed to minimize the employees' radiation exposure. The MMRTG is enclosed in a mesh container, known as the "gorilla cage," which protects it during transport and allows any excess heat generated to dissipate into the air. The MMRTG is returning to the RTGF following a fit check on MSL's Curiosity rover in the Payload Hazardous Servicing Facility (PHSF). The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Troy Cryder

KSC-2011-6719

NASA Image and Video Library

2011-07-13

CAPE CANAVERAL, Fla. -- In the airlock of the Payload Hazardous Servicing Facility at NASA's Kennedy Space Center in Florida, Department of Energy employees lower the mesh container, known as the "gorilla cage," toward the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission. The mobile plexiglass radiation shields in the foreground help minimize the employees' radiation exposure. The cage protects the MMRTG during transport and allows any excess heat generated to dissipate into the air. Transport of the MMRTG to the RTG storage facility follows the completion of the MMRTG fit check on the Curiosity rover. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Kim Shiflett

KSC-2011-6741

NASA Image and Video Library

2011-07-14

CAPE CANAVERAL, Fla. -- In the high bay of the RTG storage facility (RTGF) at NASA's Kennedy Space Center in Florida, Department of Energy workers guide the mesh container enclosing the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission as it is lifted by a crane. The container, known as the "gorilla cage," protects the MMRTG during transport and allows any excess heat generated to dissipate into the air. The cage is being removed from around the MMRTG following it return to the RTGF from a fit check on MSL's Curiosity rover in the Payload Hazardous Servicing Facility (PHSF). The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Troy Cryder

KSC-2011-6673

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- Outside the RTG storage facility at NASA's Kennedy Space Center in Florida, a forklift positions the protective mesh container, known as the "gorilla cage," enclosing the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission inside the MMRTG trailer that will transport it to the Payload Hazardous Servicing Facility (PHSF). The cage protects the MMRTG and allows any excess heat generated to dissipate into the air. In the PHSF, the MMRTG temporarily will be installed on the MSL rover, Curiosity, for a fit check but will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6739

NASA Image and Video Library

2011-07-14

CAPE CANAVERAL, Fla. -- In the high bay of the RTG storage facility (RTGF) at NASA's Kennedy Space Center in Florida, Department of Energy workers attach a crane to the mesh container enclosing the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission. The container, known as the "gorilla cage," protects it during transport and allows any excess heat generated to dissipate into the air. The cage is being removed from around the MMRTG following it return to the RTGF from a fit check on MSL's Curiosity rover in the Payload Hazardous Servicing Facility (PHSF). The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Troy Cryder

KSC-2011-6720

NASA Image and Video Library

2011-07-13

CAPE CANAVERAL, Fla. -- In the airlock of the Payload Hazardous Servicing Facility at NASA's Kennedy Space Center in Florida, a Department of Energy employee positions the mesh container, known as the "gorilla cage," on the support base of the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission. The mobile plexiglass radiation shields, in the foreground at right, helps minimize the employees' radiation exposure. The cage protects the MMRTG during transport and allows any excess heat generated to dissipate into the air. Transport of the MMRTG to the RTG storage facility follows the completion of the MMRTG fit check on the Curiosity rover. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Kim Shiflett

KSC-2011-6676

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- Outside the RTG storage facility at NASA's Kennedy Space Center in Florida, the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission, enclosed in the protective mesh container known as the "gorilla cage," is strapped down inside the MMRTG trailer and ready for transport to the Payload Hazardous Servicing Facility (PHSF). The cage protects the MMRTG and allows any excess heat generated to dissipate into the air. In the PHSF, the MMRTG temporarily will be installed on the MSL rover, Curiosity, for a fit check but will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6670

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- Outside the high bay of the RTG storage facility at NASA's Kennedy Space Center in Florida, a forklift picks up the protective mesh container, known as the "gorilla cage," enclosing the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission for its move to the Payload Hazardous Servicing Facility (PHSF). The cage protects the MMRTG and allows any excess heat generated to dissipate into the air. In the PHSF, the MMRTG temporarily will be installed on the MSL rover, Curiosity, for a fit check but will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6669

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- Department of Energy contractor employees roll the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission, enclosed in a protective mesh container known as the "gorilla cage," toward a forklift outside the high bay of the RTG storage facility at NASA's Kennedy Space Center in Florida for its move to the Payload Hazardous Servicing Facility (PHSF). The cage protects the MMRTG and allows any excess heat generated to dissipate into the air. In the PHSF, the MMRTG temporarily will be installed on the MSL rover, Curiosity, for a fit check but will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6672

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- Outside the RTG storage facility at NASA's Kennedy Space Center in Florida, a forklift carries the protective mesh container, known as the "gorilla cage," enclosing the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission toward the MMRTG trailer that will transport it to the Payload Hazardous Servicing Facility (PHSF). The cage protects the MMRTG and allows any excess heat generated to dissipate into the air. In the PHSF, the MMRTG temporarily will be installed on the MSL rover, Curiosity, for a fit check but will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6668

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- Department of Energy contractor employees roll the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission, enclosed in a protective mesh container known as the "gorilla cage," out of the high bay of the RTG storage facility at NASA's Kennedy Space Center in Florida for its move to the Payload Hazardous Servicing Facility (PHSF). The cage protects the MMRTG and allows any excess heat generated to dissipate into the air. In the PHSF, the MMRTG temporarily will be installed on the MSL rover, Curiosity, for a fit check but will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6718

NASA Image and Video Library

2011-07-13

CAPE CANAVERAL, Fla. -- In the airlock of the Payload Hazardous Servicing Facility at NASA's Kennedy Space Center in Florida, Department of Energy employees lower the mesh container, known as the "gorilla cage," toward the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission. The employees are standing behind mobile plexiglass radiation shields to help minimize the employees' radiation exposure. The cage protects the MMRTG during transport and allows any excess heat generated to dissipate into the air. Transport of the MMRTG to the RTG storage facility follows the completion of the MMRTG fit check on the Curiosity rover. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Kim Shiflett

Accumulation and release of 241Am by a macrophyte of the Yenisei River (Elodea canadensis).

PubMed

Bolsunovsky, A; Zotina, T; Bondareva, L

2005-01-01

The source of radioactive contamination of the Yenisei River floodplain, including contamination with transuranic elements, is the Mining-and-Chemical Combine of the Russian Ministry of Atomic Energy, which has for many years been producing weapons-grade plutonium. Transuranic elements have been detected not only in the soil and sediment of the river but also in the biomass of aquatic plants. This work is an investigation of accumulation and release of 241Am by a submerged macrophyte of the Yenisei River (Elodea canadensis) in laboratory experiments. In 2000-2003, laboratory experiments were carried out with biomass of E. canadensis Mich. and filtered river water. The samples were collected from the Yenisei River upstream of the discharge of the Combine's radioactive effluent. The experiments showed that 241Am is accumulated by Elodea biomass: the activity concentration of 241Am can reach 3280+/-240 Bq/g, with the concentration factor for 241Am 16 600+/-2200l/kg. Results of chemical fractionation have proved that in the course of 241Am accumulation by Elodea biomass, 241Am tightly bound to biomass increases from 11% to 27% of the total 241Am in the biomass. Release of 241Am from the decaying Elodea biomass has been evaluated experimentally. By the end of the experiment (lasting up to 127 days), the Elodea plants had lost up to 65% of their initial 241Am activity and the rate of 241Am release into the water environment reached 23 Bq/day.

Dangers associated with civil nuclear power programmes: weaponization and nuclear waste.

PubMed

Boulton, Frank

2015-07-24

The number of nuclear power plants in the world rose exponentially to 420 by 1990 and peaked at 438 in 2002; but by 2014, as closed plants were not replaced, there were just 388. In spite of using more renewable energy, the world still relies on fossil fuels, but some countries plan to develop new nuclear programmes. Spent nuclear fuel, one of the most dangerous and toxic materials known, can be reprocessed into fresh fuel or into weapons-grade materials, and generates large amounts of highly active waste. This article reviews available literature on government and industry websites and from independent analysts on world energy production, the aspirations of the 'new nuclear build' programmes in China and the UK, and the difficulties in keeping the environment safe over an immense timescale while minimizing adverse health impacts and production of greenhouse gases, and preventing weaponization by non-nuclear-weapons states acquiring civil nuclear technology.

Gender differences in the relative impact of physical and relational bullying on adolescent injury and weapon carrying.

PubMed

Dukes, Richard L; Stein, Judith A; Zane, Jazmin I

2010-12-01

Using structural equation modeling, concurrent associations were assessed among physical bullying, relational bullying, physical victimization, relational victimization, injury and weapon carrying using data from the population of 1300 adolescent girls and 1362 adolescent boys in grades 7-12 in a Colorado school district. For both genders, being a relational bully was a significantly stronger predictor of weapon carrying than being a physical bully, and both bullying types were significant predictors of more weapon carrying. For both genders, being a victim of physical bullying, a victim of relational bullying, or being a relational bully significantly predicted more injury. In latent means comparisons, adolescent girls reported more relational victimization and adolescent boys reported more physical bullying and victimization, more weapon carrying, and more injury. The relative strength of relational bullying on weapon carrying, and the health-related consequences of bullying on interpersonal violence and injury support concerted efforts in schools to mitigate these behaviors. Attention to differences related to age and gender also is indicated in the design of bullying mitigation programs. Copyright © 2010 Society for the Study of School Psychology. Published by Elsevier Ltd. All rights reserved.

Further evaluations of the toxicity of irradiated advanced heavy water reactor fuels.

PubMed

Edwards, Geoffrey W R; Priest, Nicholas D

2014-11-01

The neutron economy and online refueling capability of heavy water moderated reactors enable them to use many different fuel types, such as low enriched uranium, plutonium mixed with uranium, or plutonium and/or U mixed with thorium, in addition to their traditional natural uranium fuel. However, the toxicity and radiological protection methods for fuels other than natural uranium are not well established. A previous paper by the current authors compared the composition and toxicity of irradiated natural uranium to that of three potential advanced heavy water fuels not containing plutonium, and this work uses the same method to compare irradiated natural uranium to three other fuels that do contain plutonium in their initial composition. All three of the new fuels are assumed to incorporate plutonium isotopes characteristic of those that would be recovered from light water reactor fuel via reprocessing. The first fuel investigated is a homogeneous thorium-plutonium fuel designed for a once-through fuel cycle without reprocessing. The second fuel is a heterogeneous thorium-plutonium-U bundle, with graded enrichments of U in different parts of a single fuel assembly. This fuel is assumed to be part of a recycling scenario in which U from previously irradiated fuel is recovered. The third fuel is one in which plutonium and Am are mixed with natural uranium. Each of these fuels, because of the presence of plutonium in the initial composition, is determined to be considerably more radiotoxic than is standard natural uranium. Canadian nuclear safety regulations require that techniques be available for the measurement of 1 mSv of committed effective dose after exposure to irradiated fuel. For natural uranium fuel, the isotope Pu is a significant contributor to the committed effective dose after exposure, and thermal ionization mass spectrometry is sensitive enough that the amount of Pu excreted in urine is sufficient to estimate internal doses, from all isotopes, as low as 1 mSv. In addition, if this method is extended so that Pu is also measured, then the combined amount of Pu and Pu is sufficiently high in the thorium-plutonium fuel that a committed effective dose of 1 mSv would be measurable. However, the fraction of Pu and Pu in the other two fuels is sufficiently low that a 1 mSv dose would remain below the detection limit using this technique. Thus new methods, such as fecal measurements of Pu (or other alpha emitters), will be required to measure exposure to these new fuels.

A Moratorium in Name Only

ERIC Educational Resources Information Center

Daleus, Lennart

1975-01-01

A nationwide debate occurred in Sweden concerning their nuclear power program. The debate centered on safety, waste management, and use of weapons-grade material. Parliament voted for nuclear power despite negative public opinion. (MR)

Innovations in the Assay of Un-Segregated Multi-Isotopic Grade TRU Waste Boxes with SuperHENC and FRAM Technology

DOE Office of Scientific and Technical Information (OSTI.GOV)

Simpson, A. P.; Barber, S.; Abdurrahman, N. M.

2006-07-01

The Super High Efficiency Neutron Coincidence Counter (SuperHENC) was originally developed by BIL Solutions Inc., Los Alamos National Laboratory (LANL) and Rocky Flats Environmental Technology Site (RFETS) for assay of transuranic (TRU) waste in Standard Waste Boxes (SWB) at Rocky Flats. This mobile system was a key component in the shipment of over 4,000 SWBs to the Waste Isolation Pilot Plant (WIPP) in Carlsbad, New Mexico. The system was WIPP certified in 2001 and operated at the site for four years. The success of this system, a passive neutron coincidence counter combined with high resolution gamma spectroscopy, led to themore » order of two new units, delivered to Hanford in 2004. Several new challenges were faced at Hanford: For example, the original RFETS system was calibrated for segregated waste streams such that metals, plastics, wet combustibles and dry combustibles were separated by 'Item Description Codes' prior to assay. Furthermore, the RFETS mission of handling only weapons grade plutonium, enabled the original SuperHENC to benefit from the use of known Pu isotopics. Operations at Hanford, as with most other DOE sites, generate un-segregated waste streams, with a wide diversity of Pu isotopics. Consequently, the new SuperHENCs are required to deal with new technical challenges. The neutron system's software and calibration methodology have been modified to encompass these new requirements. In addition, PC-FRAM software has been added to the gamma system, providing a robust isotopic measurement capability. Finally a new software package has been developed that integrates the neutron and gamma data to provide a final assay results and analysis report. The new system's performance has been rigorously tested and validated against WIPP quality requirements. These modifications, together with the mobile platform, make the new SuperHENC far more versatile in handling diverse waste streams and allow for rapid redeployment around the DOE complex. (authors)« less

Plutonium activities and 240Pu/ 239Pu atom ratios in sediment cores from the east China sea and Okinawa Trough: Sources and inventories

NASA Astrophysics Data System (ADS)

Wang, Zhong-liang; Yamada, Masatoshi

2005-05-01

Plutonium concentrations and 240Pu/ 239Pu atom ratios in the East China Sea and Okinawa Trough sediment cores were determined by isotope dilution inductively coupled plasma mass spectrometry after separation using ion-exchange chromatography. The results showed that 240Pu/ 239Pu atom ratios in the East China Sea and Okinawa Trough sediments, ranging from 0.21 to 0.33, were much higher than the reported value of global fallout (0.18). The highest 240Pu/ 239Pu ratios (0.32-0.33) were observed in the deepest Okinawa Trough sediment samples. These ratios suggested the US nuclear weapons tests in the early 1950s at the Pacific Proving Grounds in the Marshall Islands were a major source of plutonium in the East China Sea and Okinawa Trough sediments, in addition to the global fallout source. It was proposed that close-in fallout plutonium was delivered from the Pacific Proving Grounds test sites via early direct tropospheric fallout and transportation by the North Pacific Equatorial Circulation system and Kuroshio Current into the Okinawa Trough and East China Sea. The total 239 + 240 Pu inventories in the cores were about 150-200% of that expected from direct global fallout; about 46-67% of the total inventories were delivered from the Pacific Proving Grounds. Much higher 239 + 240 Pu inventories were observed in the East China Sea sediments than in sediments of the Okinawa Trough, because in the open oceans, part of the 239 + 240 Pu was still retained in the water column, and continued Pu scavenging was higher over the margin than the trough. According to the vertical distributions of 239 + 240 Pu activities and 240Pu/ 239Pu atom ratios in these cores, it was concluded that sediment mixing was the dominant process in controlling profiles of plutonium in this area. Faster mixing in the coastal samples has homogenized the entire 240Pu/ 239Pu ratio record today; slightly slower mixing and less scavenging in the Okinawa Trough have left the surface sediment ratios closer to the modern North Pacific water end member and higher ratios (0.30-0.34) at the bottom of the cores.

18. VIEW OF THE NORTH ELEVATION OF BUILDING 71 (771) ...

Library of Congress Historic Buildings Survey, Historic Engineering Record, Historic Landscapes Survey

18. VIEW OF THE NORTH ELEVATION OF BUILDING 71 (771) UNDER CONSTRUCTION IN 1952. BUILDING 71 WAS THE ORIGINAL PLUTONIUM OPERATIONS BUILDING. PRODUCTION BUILDINGS WERE BUILT INTO HILLSIDES AND/OR BELOW GRADE AS A SAFETY MEASURE AGAINST RUSSIAN ATTACK (3/2/52). - Rocky Flats Plant, Bounded by Indiana Street & Routes 93, 128 & 72, Golden, Jefferson County, CO

Congress targets DOE plants

NASA Astrophysics Data System (ADS)

Maggs, William Ward

Calling the Department of Energy's management of the nation's crippled nuclear weapons production complex “a 35-year secret chemical war waged against people living near DOE's sites,” Representative Thomas Luken (D-OH) opened a congressional hearing on February 23 with an appeal to DOE Secretary-designate James Watkins to release secret health records of workers at the plants. In testimony that followed, Comptroller General Charles Bowsher told a subcommittee of the House Energy and Commerce Committee that President Bush's new budget does not go far enough on the long and costly road of cleaning up and modernizing the contaminated and aging facilities. The renovation is expected to cost up to $155 billion.By next month, 11 of the 17 installations that make up the DOE complex will be on the EPA's Superfund list of the nation's most contaminated waste sites. Some o f the DOE facilities, including the Rocky Flats plant in Denver, Colo., the Hanford Reservation in eastern Washington, and the Savannah River plant in South Carolina, are among the most polluted sites ever identified by EPA. The principal function of the facilities, the production of tritium and plutonium for nuclear weapons, has stopped, creating what DOE has characterized as a looming national security crisis.

Applications of Elpasolites as a Multimode Radiation Sensor

NASA Astrophysics Data System (ADS)

Guckes, Amber

This study consists of both computational and experimental investigations. The computational results enabled detector design selections and confirmed experimental results. The experimental results determined that the CLYC scintillation detector can be applied as a functional and field-deployable multimode radiation sensor. The computational study utilized MCNP6 code to investigate the response of CLYC to various incident radiations and to determine the feasibility of its application as a handheld multimode sensor and as a single-scintillator collimated directional detection system. These simulations include: • Characterization of the response of the CLYC scintillator to gamma-rays and neutrons; • Study of the isotopic enrichment of 7Li versus 6Li in the CLYC for optimal detection of both thermal neutrons and fast neutrons; • Analysis of collimator designs to determine the optimal collimator for the single CLYC sensor directional detection system to assay gamma rays and neutrons; Simulations of a handheld CLYC multimode sensor and a single CLYC scintillator collimated directional detection system with the optimized collimator to determine the feasibility of detecting nuclear materials that could be encountered during field operations. These nuclear materials include depleted uranium, natural uranium, low-enriched uranium, highly-enriched uranium, reactor-grade plutonium, and weapons-grade plutonium. The experimental study includes the design, construction, and testing of both a handheld CLYC multimode sensor and a single CLYC scintillator collimated directional detection system. Both were designed in the Inventor CAD software and based on results of the computational study to optimize its performance. The handheld CLYC multimode sensor is modular, scalable, low?power, and optimized for high count rates. Commercial?off?the?shelf components were used where possible in order to optimize size, increase robustness, and minimize cost. The handheld CLYC multimode sensor was successfully tested to confirm its ability for gamma-ray and neutron detection, and gamma?ray and neutron spectroscopy. The sensor utilizes wireless data transfer for possible radiation mapping and network?centric deployment. The handheld multimode sensor was tested by performing laboratory measurements with various gamma-ray sources and neutron sources. The single CLYC scintillator collimated directional detection system is portable, robust, and capable of source localization and identification. The collimator was designed based on the results of the computational study and is constructed with high density polyethylene (HDPE) and lead (Pb). The collimator design and construction allows for the directional detection of gamma rays and fast neutrons utilizing only one scintillator which is interchangeable. For this study, a CLYC-7 scintillator was used. The collimated directional detection system was tested by performing laboratory directional measurements with various gamma-ray sources, 252Cf and a 239PuBe source.

HOW OLD IS IT? - 241PU/241AM NUCLEAR FORENSIC CHRONOLOGY REFERENCE MATERIALS

PubMed Central

Fitzgerald, Ryan; Inn, Kenneth G.W.; Horgan, Christopher

2018-01-01

One material attribute for nuclear forensics is material age. 241Pu is almost always present in uranium- and plutonium-based nuclear weapons, which pose the greatest threat to our security. The in-growth of 241Am due to the decay of 241Pu provides an excellent chronometer of the material. A well-characterized 241Pu/241Am standard is needed to validate measurement capability, as a basis for between-laboratory comparability, and as material for verifying laboratory performance. This effort verifies the certification of a 38 year old 241Pu Standard Reference Material (SRM4340) through alpha-gamma anticoincidence counting, and also establishes the separation date to two weeks of the documented date. PMID:29720779

Reassessing the Effects of Early Adolescent Alcohol Use on Later Antisocial Behavior: A Longitudinal Study of Students in Victoria, Australia and Washington State, United States

PubMed Central

Hemphill, Sheryl A.; Heerde, Jessica A.; Scholes-Balog, Kirsty E.; Smith, Rachel; Herrenkohl, Todd I.; Toumbourou, John W.; Catalano, Richard F.

2013-01-01

The effect of early adolescent alcohol use on antisocial behavior was examined at one- and two-year follow-up in Washington, United States and Victoria, Australia. Each state used the same methods to survey statewide representative samples of students (N = 1,858, 52% female) in 2002 (Grade 7 [G7]), 2003 (Grade 8 [G8]), and 2004 (Grade 9 [G9]). Rates of lifetime, current, frequent, and heavy episodic alcohol use were higher in Victoria than Washington State, whereas rates of five antisocial behaviors were generally comparable across states. After controlling for established risk factors, few associations between alcohol use and antisocial behavior remained, except that G7 current use predicted G8 police arrests and stealing and G9 carrying a weapon and stealing; G7 heavy episodic use predicted G8 and G9 police arrests; and G7 lifetime use predicted G9 carrying a weapon. Hence, risk factors other than alcohol were stronger predictors of antisocial behaviors. PMID:25132702

Sedimentary record of plutonium in the North Yellow Sea and the response to catchment environmental changes of inflow rivers.

PubMed

Xu, Yihong; Pan, Shaoming; Gao, Jianhua; Hou, Xiaolin; Ma, Yongfu; Hao, Yongpei

2018-09-01

Plutonium (Pu) isotopes were first determined in surface and core sediment samples collected from the northern North Yellow Sea (NYS) to elucidate their source terms and deposition process as well as the response to catchment environmental changes of inflow rivers. 240 Pu/ 239 Pu atom ratios in all sediments showed the typical global fallout value of ∼0.18 without any influences from the nuclear weapons tests conducted recently in the North Korea or early in the Pacific Proving Ground. The large variation of 239+240 Pu activities (0.022-0.515 mBq/g) observed in surface sediments should be mainly attributed to the re-suspension and transportation of fine sediments influenced by the Liaonan Costal Current. Based on the two 239+249 Pu depth profiles with easily observed onset fallout levels (1952) and global fallout peaks (1963), 239+240 Pu served as a valid time mark in the coastal sedimentary system. Riverine input Pu contributed only 15-27% to the total global fallout inventory (92.5-108.8 Bq/m 2 ) in the northern NYS, much lower than that in the Yangtze River estuary (77-80%), indicating a better soil conservation in the northeast China due to higher forest coverage compared to the Yangtze River's drainage basin. The increase of riverine input Pu after 1980s reflected the more intense soil erosion degree caused by the land use and cover change due to the increment of human activities in the northeast China at the same period. Our results demonstrated that plutonium is a good indicator for studying sedimentary process and its response to the environment in the coastal area. Copyright © 2018 Elsevier Ltd. All rights reserved.

Migration of conservative and sorbing radionuclides in heterogeneous fractured rock aquifers at the Nevada Test Site

NASA Astrophysics Data System (ADS)

Boryta, J. R.; Wolfsberg, A. V.

2003-12-01

The Nevada Test Site (NTS) is the United States continental nuclear weapons testing site. The larger underground tests, including BENHAM and TYBO, were conducted at Pahute Mesa. The BENHAM test, conducted in 1968, was detonated 1.4 km below the surface and the TYBO test, conducted in 1975, was detonated at a depth of 765 m. Between 1996 and 1998, several radionuclides were discovered in trace concentrations in a monitoring well complex 273 m from TYBO and 1300 m from BENHAM. Previous studies associated with these measurements have focused primarily on a) plutonium discovered in the observation wells, which was identified through isotopic finger printing as originating at BENHAM, b) colloid-facilitated plutonium transport processes, and c) vertical convection in subsurface nuclear test collapse chimneys. In addition to plutonium, several other non-, weakly-, and strongly-sorbing radionuclides were discovered in trace concentrations in the observation wells, including tritium, carbon-14, chlorine-36, iodine-129, technetium-99, neptunium-237, strontium-90, cesium-137, americium-241, and europium-152,154,155. The range in retardation processes affecting these different radionuclides provides additional information for assessing groundwater solute transport model formulations. For all radionuclides, simulation results are most sensitive to the fracture porosity and fracture aperture. Additionally, for weakly sorbing Np, simulation results are highly sensitive to the matrix sorption coefficient. For strongly sorbing species, migration in the absence of colloids can only be simulated if fracture apertures are set very large, reducing the amount of diffusion that can occur. For these species, colloid-facilitated transport appears to be a more likely explanation for the measurements. This is corroborated with colloid-transport model simulations.

Nuclear waste disposal—pyrochlore (A2B2O7): Nuclear waste form for the immobilization of plutonium and "minor" actinides

NASA Astrophysics Data System (ADS)

Ewing, Rodney C.; Weber, William J.; Lian, Jie

2004-06-01

During the past half-century, the nuclear fuel cycle has generated approximately 1400 metric tons of plutonium and substantial quantities of the "minor" actinides, such as Np, Am, and Cm. The successful disposition of these actinides has an important impact on the strategy for developing advanced nuclear fuel cycles, weapons proliferation, and the geologic disposal of high-level radioactive waste. During the last decade, there has been substantial interest in the use of the isometric pyrochlore structure-type, A2B2O7, for the immobilization of actinides. Most of the interest has focused on titanate-pyrochlore because of its chemical durability; however, these compositions experience a radiation-induced transition from the crystalline-to-aperiodic state due to radiation damage from the alpha-decay of actinides. Depending on the actinide concentration, the titanate pyrochlore will become amorphous in less than 1000 years of storage. Recently, systematic ion beam irradiations of a variety of pyrochlore compositions has revealed that many zirconate pyrochlores do not become amorphous, but remain crystalline as a defect fluorite structure-type due to disordering of the A- and B-site cations. The zirconate pyrochlores will remain crystalline even to very high doses, greater than 100 displacements per atom. Systematic experimental studies of actinide-doped and ion beam-irradiated pyrochlore, analyses of natural U- and Th-bearing pyrochlore, and simulations of the energetics of the disordering process now provide a rather detailed understanding of the structural and chemical controls on the response of pyrochlore to radiation. These results provide a solid basis for predicting the behavior and durability of pyrochlore used to immobilize plutonium.

Plutonium in the WIPP environment: its detection, distribution and behavior.

PubMed

Thakur, P; Ballard, S; Nelson, R

2012-05-01

The Waste Isolation Pilot Plant (WIPP) is the only operating deep underground geologic nuclear repository in the United States. It is located in southeastern New Mexico, approximately 655 m (2150 ft) below the surface of the Earth in a bedded Permian evaporite salt formation. This mined geologic repository is designed for the safe disposal of transuranic (TRU) wastes generated from the US defense program. Aerosol and soil samples have been collected near the WIPP site to investigate the sources of plutonium in the WIPP environment since the late 1990s, well before WIPP received its first shipment. Activities of (238)Pu, (239+240)Pu and (241)Am were determined by alpha spectrometry following a series of chemical separations. The concentrations of Al and U were determined in a separate set of samples by inductively coupled plasma mass spectrometry. The annual airborne concentrations of (239+240)Pu during the period from 1998 to 2010 show no systematic interannual variations. However, monthly (239+240)Pu particulate concentrations show a typical seasonal variation with a maximum in spring, the time when strong and gusty winds frequently give rise to blowing dust. Resuspension of soil particles containing weapons fallout is considered to be the predominant source of plutonium in the WIPP area. Further, this work characterizes the source, temporal variation and its distribution with depth in a soil profile to evaluate the importance of transport mechanisms affecting the fate of these radionuclides in the WIPP environment. The mean (137)Cs/(239+240)Pu, (241)Am/(239+240)Pu activity ratio and (240)Pu/(239)Pu atom ratio observed in the WIPP samples are consistent with the source being largely global fallout. There is no evidence of any release from the WIPP contributing to radionuclide concentrations in the environment.

Quantitative NDA measurements of advanced reprocessing product materials containing uranium, neptunium, plutonium, and americium

NASA Astrophysics Data System (ADS)

Goddard, Braden

The ability of inspection agencies and facility operators to measure powders containing several actinides is increasingly necessary as new reprocessing techniques and fuel forms are being developed. These powders are difficult to measure with nondestructive assay (NDA) techniques because neutrons emitted from induced and spontaneous fission of different nuclides are very similar. A neutron multiplicity technique based on first principle methods was developed to measure these powders by exploiting isotope-specific nuclear properties, such as the energy-dependent fission cross sections and the neutron induced fission neutron multiplicity. This technique was tested through extensive simulations using the Monte Carlo N-Particle eXtended (MCNPX) code and by one measurement campaign using the Active Well Coincidence Counter (AWCC) and two measurement campaigns using the Epithermal Neutron Multiplicity Counter (ENMC) with various (alpha,n) sources and actinide materials. Four potential applications of this first principle technique have been identified: (1) quantitative measurement of uranium, neptunium, plutonium, and americium materials; (2) quantitative measurement of mixed oxide (MOX) materials; (3) quantitative measurement of uranium materials; and (4) weapons verification in arms control agreements. This technique still has several challenges which need to be overcome, the largest of these being the challenge of having high-precision active and passive measurements to produce results with acceptably small uncertainties.

Critical Need for Plutonium and Uranium Isotopic Standards with Lower Uncertainties

DOE PAGES

Mathew, Kattathu Joseph; Stanley, Floyd E.; Thomas, Mariam R.; ...

2016-09-23

Certified reference materials (CRMs) traceable to national and international safeguards database are a critical prerequisite for ensuring that nuclear measurement systems are free of systematic biases. CRMs are used to validate measurement processes associated with nuclear analytical laboratories. Diverse areas related to nuclear safeguards are impacted by the quality of the CRM standards available to analytical laboratories. These include: nuclear forensics, radio-chronometry, national and international safeguards, stockpile stewardship, nuclear weapons infrastructure and nonproliferation, fuel fabrication, waste processing, radiation protection, and environmental monitoring. For the past three decades the nuclear community is confronted with the strange situation that improvements in measurementmore » data quality resulting from the improved accuracy and precision achievable with modern multi-collector mass spectrometers could not be fully exploited due to large uncertainties associated with CRMs available from New Brunswick Laboratory (NBL) that are used for instrument calibration and measurement control. Similar conditions prevail for both plutonium and uranium isotopic standards and for impurity element standards in uranium matrices. Herein, the current status of U and Pu isotopic standards available from NBL is reviewed. Critical areas requiring improvement in the quality of the nuclear standards to enable the U. S. and international safeguards community to utilize the full potential of modern multi-collector mass spectrometer instruments are highlighted.« less

Site restoration: Estimation of attributable costs from plutonium-dispersal accidents

DOE Office of Scientific and Technical Information (OSTI.GOV)

Chanin, D.I.; Murfin, W.B.

1996-05-01

A nuclear weapons accident is an extremely unlikely event due to the extensive care taken in operations. However, under some hypothetical accident conditions, plutonium might be dispersed to the environment. This would result in costs being incurred by the government to remediate the site and compensate for losses. This study is a multi-disciplinary evaluation of the potential scope of the post-accident response that includes technical factors, current and proposed legal requirements and constraints, as well as social/political factors that could influence decision making. The study provides parameters that can be used to assess economic costs for accidents postulated to occurmore » in urban areas, Midwest farmland, Western rangeland, and forest. Per-area remediation costs have been estimated, using industry-standard methods, for both expedited and extended remediation. Expedited remediation costs have been evaluated for highways, airports, and urban areas. Extended remediation costs have been evaluated for all land uses except highways and airports. The inclusion of cost estimates in risk assessments, together with the conventional estimation of doses and health effects, allows a fuller understanding of the post-accident environment. The insights obtained can be used to minimize economic risks by evaluation of operational and design alternatives, and through development of improved capabilities for accident response.« less

Critical Need for Plutonium and Uranium Isotopic Standards with Lower Uncertainties

DOE Office of Scientific and Technical Information (OSTI.GOV)

Mathew, Kattathu Joseph; Stanley, Floyd E.; Thomas, Mariam R.

Certified reference materials (CRMs) traceable to national and international safeguards database are a critical prerequisite for ensuring that nuclear measurement systems are free of systematic biases. CRMs are used to validate measurement processes associated with nuclear analytical laboratories. Diverse areas related to nuclear safeguards are impacted by the quality of the CRM standards available to analytical laboratories. These include: nuclear forensics, radio-chronometry, national and international safeguards, stockpile stewardship, nuclear weapons infrastructure and nonproliferation, fuel fabrication, waste processing, radiation protection, and environmental monitoring. For the past three decades the nuclear community is confronted with the strange situation that improvements in measurementmore » data quality resulting from the improved accuracy and precision achievable with modern multi-collector mass spectrometers could not be fully exploited due to large uncertainties associated with CRMs available from New Brunswick Laboratory (NBL) that are used for instrument calibration and measurement control. Similar conditions prevail for both plutonium and uranium isotopic standards and for impurity element standards in uranium matrices. Herein, the current status of U and Pu isotopic standards available from NBL is reviewed. Critical areas requiring improvement in the quality of the nuclear standards to enable the U. S. and international safeguards community to utilize the full potential of modern multi-collector mass spectrometer instruments are highlighted.« less

KSC-04PD-1654

NASA Technical Reports Server (NTRS)

2004-01-01

KENNEDY SPACE CENTER, FLA. At the ribbon cutting for the Enhanced Firing Range on Schwartz Rd. at Kennedy Space Center, Dave Saleeba (left with weapon) and Center Director Jim Kennedy (right, with weapon) practice firing on the new range. Saleeba is assistant administrator with the Office of Security Management and Safeguards at NASA Headquarters and was a guest speaker at the ceremony. NASAs Federal Law Enforcement Training Academys firing range has been upgraded to include a rifle-grade shoot house, a portable, tactical shoot-back trailer for cover and concealment drills, automated running targets and a new classroom facility. They are added to the existing three firearms ranges, pistol-grade shoot house, obstacle course and rappel tower. NASAs Security Management and Safeguards Office funded the enhancements in order to improve ability to train the KSC security force and to support local, state and federal law enforcement agencies in Homeland Security.

The American atom: A documentary history of nuclear policies from the discovery of fission to the present

DOE Office of Scientific and Technical Information (OSTI.GOV)

Williams, R.C.; Cantelon, P.L.

1984-01-01

In selecting these historical documents the authors have applied three general tests: first, does the document help tell the story of the development of American nuclear policy in a nontechnical way; second, is the source primary rather than secondary, written by an actor in the drama rather than by a member of the audience; third, does the document provide coverage of the major chapters in the story. The Manhattan Project was America's $2 billion secret project to build an atomic bomb. Many documents associated with the project have come to light only in recent years. In Section II they usemore » the letters of J. Robert Oppenheimer and the recently declassified minutes of policy committees to tell the story of how the bomb was designed and built and how the decision was made to drop the first uranium and plutonium devices on the Japanese cities of Hiroshima and Nagasaki in 1945. How did a weapon of war become the key to a peacetime industry. In considering atomic energy after World War II, they focus in Section III on the legislative enabling acts that established the Atomic Energy Commission, the short-lived dream of international control of nuclear weapons under the Baruch Plan, and the ''atoms for peace'' program of President Dwight D. Eisenhower. By 1954 the highly classified work on nuclear weapons paralleled a new development of nuclear energy and power reactors. Knowledge was shared with both private industry and other countries. The fruits of this program are considered in the later section on nuclear power.« less

Accelerator-driven Transmutation of Waste

NASA Astrophysics Data System (ADS)

Venneri, Francesco

1998-04-01

Nuclear waste from commercial power plants contains large quantities of plutonium, other fissionable actinides, and long-lived fission products that are potential proliferation concerns and create challenges for the long-term storage. Different strategies for dealing with nuclear waste are being followed by various countries because of their geologic situations and their views on nuclear energy, reprocessing and non-proliferation. The current United States policy is to store unprocessed spent reactor fuel in a geologic repository. Other countries are opting for treatment of nuclear waste, including partial utilization of the fissile material contained in the spent fuel, prior to geologic storage. Long-term uncertainties are hampering the acceptability and eventual licensing of a geologic repository for nuclear spent fuel in the US, and driving up its cost. The greatest concerns are with the potential for radiation release and exposure from the spent fuel for tens of thousands of years and the possible diversion and use of the actinides contained in the waste for weapons construction. Taking advantage of the recent breakthroughs in accelerator technology and of the natural flexibility of subcritical systems, the Accelerator-driven Transmutation of Waste (ATW) concept offers the United States and other countries the possibility to greatly reduce plutonium, higher actinides and environmentally hazardous fission products from the waste stream destined for permanent storage. ATW does not eliminate the need for, but instead enhances the viability of permanent waste repositories. Far from being limited to waste destruction, the ATW concept also brings to the table new technologies that could be relevant for next-generation power producing reactors. In the ATW concept, spent fuel would be shipped to the ATW site where the plutonium, transuranics and selected long-lived fission products would be destroyed by fission or transmutation in their first and only pass through the facility, using an accelerator-driven subcritical burner cooled by liquid lead/bismuth and limited pyrochemical treatment of the spent fuel and residual waste. This approach contrasts with the present-day practices of aqueous reprocessing (Europe and Japan), in which high purity plutonium is produced and used in the fabrication of fresh mixed oxide fuel (MOX) that is shipped off-site for use in light water reactors.

KSC-2011-6683

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- In the airlock of the Payload Hazardous Servicing Facility (PHSF) at NASA's Kennedy Space Center in Florida, the protective mesh container enclosing the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission is lowered to the floor of the airlock beside the MMRTG. The container, known as the "gorilla cage," protects the MMRTG during transport and allows any excess heat generated to dissipate into the air. Next, the airlock will be transitioned into a clean room by purging the air of any particles. In the PHSF, the MMRTG temporarily will be installed on the MSL rover, Curiosity, for a fit check but will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6742

NASA Image and Video Library

2011-07-14

CAPE CANAVERAL, Fla. -- In the high bay of the RTG storage facility (RTGF) at NASA's Kennedy Space Center in Florida, the mesh container enclosing the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission is lifted from around the MMRTG. The container, known as the "gorilla cage," protects the MMRTG during transport and allows any excess heat generated to dissipate into the air. The cage is being removed following the return of the MMRTG to the RTGF from a fit check on MSL's Curiosity rover in the Payload Hazardous Servicing Facility (PHSF). The workers at right are observing the operation from behind a mobile plexiglass radiation shield to minimize their radiation exposure. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Troy Cryder

KSC-2011-6671

NASA Image and Video Library

2011-07-12

CAPE CANAVERAL, Fla. -- Outside the RTG storage facility at NASA's Kennedy Space Center in Florida, a plexiglass shield has been installed on the forklift enlisted to move the protective mesh container, known as the "gorilla cage," enclosing the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission. The shield minimizes the amount of debris dispersed by the wheels of the forklift that can contact the gorilla cage. The cage protects the MMRTG and allows any excess heat generated to dissipate into the air. The MMRTG is being moved to the Payload Hazardous Servicing Facility (PHSF) where it temporarily will be installed on the MSL rover, Curiosity, for a fit check but will be installed on the rover for launch at the pad. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. Curiosity, MSL's car-sized rover, has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is planned for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Cory Huston

KSC-2011-6740

NASA Image and Video Library

2011-07-14

CAPE CANAVERAL, Fla. -- In the high bay of the RTG storage facility (RTGF) at NASA's Kennedy Space Center in Florida, Department of Energy workers guide the mesh container enclosing the multi-mission radioisotope thermoelectric generator (MMRTG) for NASA's Mars Science Laboratory (MSL) mission as it is lifted by a crane. The container, known as the "gorilla cage," protects the MMRTG during transport and allows any excess heat generated to dissipate into the air. The cage is being removed from around the MMRTG following it return to the RTGF from a fit check on MSL's Curiosity rover in the Payload Hazardous Servicing Facility (PHSF). The workers at right are observing the operation from behind a mobile plexiglass radiation shield to minimize their radiation exposure. The MMRTG will generate the power needed for the mission from the natural decay of plutonium-238, a non-weapons-grade form of the radioisotope. Heat given off by this natural decay will provide constant power through the day and night during all seasons. MSL's components include a compact car-sized rover, Curiosity, which has 10 science instruments designed to search for signs of life, including methane, and help determine if the gas is from a biological or geological source. Waste heat from the MMRTG will be circulated throughout the rover system to keep instruments, computers, mechanical devices and communications systems within their operating temperature ranges. Launch of MSL aboard a United Launch Alliance Atlas V rocket is targeted for Nov. 25 from Space Launch Complex 41 on Cape Canaveral Air Force Station. For more information, visit http://www.nasa.gov/msl. Photo credit: NASA/Troy Cryder

Predictors of Weapon-Related Behaviors among African American, Latino, and White Youth.

PubMed

Shetgiri, Rashmi; Boots, Denise Paquette; Lin, Hua; Cheng, Tina L

2016-04-01

To identify risk and protective factors for weapon involvement among African American, Latino, and white adolescents. The National Longitudinal Study of Adolescent to Adult Health is a nationally representative survey of 7th-12th grade students. Predictors at wave 1 and outcome at wave 2 were analyzed. Data were collected in the mid-1990s, when rates of violent crime had been declining. The outcome was a dichotomous measure of weapon-involvement in the past year, created using 3 items (weapon-carrying, pulled gun/knife, shot/stabbed someone). Bivariate and multilevel logistic regression analyses examined associations of individual, peer, family, and community characteristics with weapon involvement; stratified analyses were conducted with African American, Latino, and white subsamples. Emotional distress and substance use were risk factors for all groups. Violence exposure and peer delinquency were risk factors for whites and African Americans. Gun availability in the home was associated with weapon involvement for African Americans only. High educational aspirations were protective for African Americans and Latinos, but higher family connectedness was protective for Latinos only. Interventions to prevent weapon-related behaviors among African American, Latino, and white adolescents may benefit from addressing emotional distress and substance use. Risk and protective factors vary by race/ethnicity after adjusting for individual, peer, family, and community characteristics. Addressing violence exposure, minimizing the influence of delinquent peers, promoting educational aspirations, and enhancing family connectedness could guide tailoring of violence prevention interventions. Copyright © 2016 Elsevier Inc. All rights reserved.

Predictors of Weapon-Related Behaviors Among African-American, Latino, and White Youth

PubMed Central

Shetgiri, Rashmi; Boots, Denise Paquette; Lin, Hua; Cheng, Tina L.

2016-01-01

Objective To identify risk and protective factors for weapon involvement among African-American, Latino, and white adolescents. Study design The National Longitudinal Study of Adolescent to Adult Health is a nationally-representative survey of 7th–12th grade students. Predictors at Wave 1 and outcome at Wave 2 were analyzed. Data were collected in the mid-1990s, when rates of violent crime had been declining. The outcome was a dichotomous measure of weapon-involvement in the past year, created using 3 items (weapon-carrying, pulled gun/knife, shot/stabbed someone). Bivariate and multilevel logistic regression analyses examined associations of individual, peer, family, and community characteristics with weapon involvement; stratified analyses were conducted with African-American, Latino, and white subsamples. Results Emotional distress and substance use were risk factors for all groups. Violence exposure and peer delinquency were risk factors for whites and African Americans. Gun availability in the home was associated with weapon involvement for African Americans only. High educational aspirations were protective for African Americans and Latinos, but higher family connectedness was protective for Latinos only. Conclusions Interventions to prevent weapon-related behaviors among African American, Latino, and white adolescents may benefit from addressing emotional distress and substance use. Risk and protective factors vary by race/ethnicity after adjusting for individual, peer, family, and community characteristics. Addressing violence exposure, minimizing the influence of delinquent peers, promoting educational aspirations, and enhancing family connectedness could guide tailoring of violence prevention interventions. PMID:26778260

Radiochemical Processing Laboratory (RPL) at PNNL

DOE Office of Scientific and Technical Information (OSTI.GOV)

Peurrung, Tony; Clark, Sue; Bryan, Sam

2017-03-23

Nuclear research is one of the core components of PNNL's mission. The centerpiece of PNNL's nuclear research is the Radiochemical Processing Laboratory (RPL), a Category 2 nuclear facility with state-of-the-art instrumentation, scientific expertise, and specialized capabilities that enable research with significant quantities of fissionable materials and other radionuclides—from tritium to plutonium. High impact radiological research has been conducted in the RPL since the 1950's, when nuclear weapons and energy production at Hanford were at the forefront of national defense. Since then, significant investments have been made in the RPL to maintain it as a premier nuclear science research facility supportingmore » multiple programs. Most recently, PNNL is developing a world-class analytical electron microscopy facility dedicated to the characterization of radiological materials.« less

High level radioactive waste vitrification process equipment component testing

NASA Astrophysics Data System (ADS)

Siemens, D. H.; Health, W. C.; Larson, D. E.; Craig, S. N.; Berger, D. N.; Goles, R. W.

1985-04-01

Remote operability and maintainability of vitrification equipment were assessment under shielded cell conditions. The equipment tested will be applied to immobilize high level and transuranic liquid waste slurries that resulted from plutonium production for defense weapons. Equipment tested included: a turntable for handling waste canisters under the melter; a removable discharge cone in the melter overflow section; a thermocouple jumper that extends into a shielded cell; remote instrument and electrical connectors; remote, mechanical, and heat transfer aspects of the melter glass overflow section; a reamer to clean out plugged nozzles in the melter top; a closed circuit camera to view the melter interior; and a device to retrieve samples of the glass product. A test was also conduucted to evaluate liquid metals for use in a liquid metal sealing system.

THE INTEGRATION OF A PROPOSED ZONE CLOSURE APPROACH FOR THE PLUTONIUM FINISHING PLANT (PFP) DECOMMISSIONING & THE PFP ZONE HANFORD SITE WASHINGTON

DOE Office of Scientific and Technical Information (OSTI.GOV)

HOPKINS, A.M.

2005-02-23

The Plutonium Finishing Plant (PFP) and associated processing facilities are located in the 200 area of the Hanford Site in Eastern Washington. This area is part of what is now called the Central Plateau. In order to achieve closure of the contaminated facilities and waste sites at Hanford on the Central Plateau (CP), a geographic re-districting of the area into zones has been proposed in the recently published Plan for Central Plateau Closure. One of the 22 zones proposed in the Central Plateau encompasses the PFP and ancillary facilities. Approximately eighty six buildings are included in the PFP Zone. Thismore » paper addresses the approach for the closure of the PFP Zone within the Central Plateau. The PFP complex of buildings forms the bulk of the structures in the PFP Zone. For closure of the above-grade portion of structures within the PFP complex, the approach is to remove them to a state called ''slab-on-grade'' per the criteria contained in PFP End Point Criteria document and as documented in action memoranda. For below-grade portions of the structures (such as below-grade rooms, pipe trenches and underground ducts), the approach is to remove as much residual contamination as practicable and to fill the void spaces with clean fill material such as sand, grout, or controlled density fill. This approach will be modified as planning for the waste sites progresses to ensure that the actions of the PFP decommissioning projects do not negatively impact future planned actions under the CERCLA. Cribs, settling tanks, septic tanks and other miscellaneous below-grade void spaces will either be cleaned to the extent practicable and filled or will be covered with an environmental barrier as determined by further studies and CERCLA decision documents. Currently, between two and five environmental barriers are proposed to be placed over waste sites and remaining building slabs in the PFP Zone.« less

Medical Effects of a Transuranic "Dirty Bomb".

PubMed

Durakovic, Asaf

2017-03-01

The modern military battlefields are characterized by the use of nonconventional weapons such as encountered in the conflicts of the Gulf War I and Gulf War II. Recent warfare in Iraq, Afghanistan, and the Balkans has introduced radioactive weapons to the modern war zone scenarios. This presents the military medicine with a new area of radioactive warfare with the potential large scale contamination of military and civilian targets with the variety of radioactive isotopes further enhanced by the clandestine use of radioactive materials in the terrorist radioactive warfare. Radioactive dispersal devices (RDDs), including the "dirty bomb," involve the use of organotropic radioisotopes such as iodine 131, cesium 137, strontium 90, and transuranic elements. Some of the current studies of RDDs involve large-scale medical effects, social and economic disruption of the society, logistics of casualty management, cleanup, and transportation preparedness, still insufficiently addressed by the environmental and mass casualty medicine. The consequences of a dirty bomb, particularly in the terrorist use in urban areas, are a subject of international studies of multiple agencies involved in the management of disaster medicine. The long-term somatic and genetic impact of some from among over 400 radioisotopes released in the nuclear fission include somatic and transgenerational genetic effects with the potential challenges of the genomic stability of the biosphere. The global contamination is additionally heightened by the presence of transuranic elements in the modern warzone, including depleted uranium recently found to contain plutonium 239, possibly the most dangerous substance known to man with one pound of plutonium capable of causing 8 billion cancers. The planning for the consequences of radioactive dirty bomb are being currently studied in reference to the alkaline earths, osteotropic, and stem cell hazards of internally deposited radioactive isotopes, in particular uranium and transuranic elements. The spread of radioactive materials in the area of the impact would expose both military and civilian personnel to the blast and dust with both inhalational, somatic, and gastrointestinal exposure, in the aftermath of the deployment of RDDs. The quantities of radioactive materials have proliferated from the original quantity of plutonium first isolated in 1941 from 0.5 mg to the current tens of thousands of kilograms in the strategic nuclear arsenal with the obvious potential consequences to the biosphere and mankind. In an event of RDD employment, the immediate goal of disaster and mass casualty medicine would be a synchronized effort to contain the scope of the event, followed by cleanup and treatment procedures. A pragmatic approach to this problem is not always possible because of unpredictability of the terrorist-use scenarios. Reprint & Copyright © 2017 Association of Military Surgeons of the U.S.

Sorption/Desorption Interactions of Plutonium with Montmorillonite

NASA Astrophysics Data System (ADS)

Begg, J.; Zavarin, M.; Zhao, P.; Kersting, A. B.

2012-12-01

Plutonium (Pu) release to the environment through nuclear weapon development and the nuclear fuel cycle is an unfortunate legacy of the nuclear age. In part due to public health concerns over the risk of Pu contamination of drinking water, predicting the behavior of Pu in both surface and sub-surface water is a topic of continued interest. Typically it was assumed that Pu mobility in groundwater would be severely restricted, as laboratory adsorption studies commonly show that naturally occurring minerals can effectively remove plutonium from solution. However, evidence for the transport of Pu over significant distances at field sites highlights a relative lack of understanding of the fundamental processes controlling plutonium behavior in natural systems. At several field locations, enhanced mobility is due to Pu association with colloidal particles that serve to increase the transport of sorbed contaminants (Kersting et al., 1999; Santschi et al., 2002, Novikov et al., 2006). The ability for mineral colloids to transport Pu is in part controlled by its oxidation state and the rate of plutonium adsorption to, and desorption from, the mineral surface. Previously we have investigated the adsorption affinity of Pu for montmorillonite colloids, finding affinities to be similar over a wide range of Pu concentrations. In the present study we examine the stability of adsorbed Pu on the mineral surface. Pu(IV) at an initial concentration of 10-10 M was pre-equilibrated with montmorillonite in a background electrolyte at pH values of 4, 6 and 8. Following equilibration, aliquots of the suspensions were placed in a flow cell and Pu-free background electrolyte at the relevant pH was passed through the system. Flow rates were varied in order to investigate the kinetics of desorption and hence gain a mechanistic understanding of the desorption process. The flow cell experiments demonstrate that desorption of Pu from the montmorillonite surface cannot be modeled as a simple first order process. Furthermore, a pH dependence was observed, with less desorbed at pH 4 compared to pH 8. We suggest the pH dependence is likely controlled by reoxidation of Pu(IV) to Pu(V) and aqueous speciation. We will present models used to describe desorption behavior and discuss the implications for Pu transport. References: Kersting, A.B.; Efurd, D.W.; Finnegan, D.L.; Rokop, D.J.; Smith, D.K.; Thompson J.L. (1999) Migration of plutonium in groundwater at the Nevada Test Site, Nature, 397, 56-59. Novikov A.P.; Kalmykov, S.N.; Utsunomiya, S.; Ewing, R.C.; Horreard, F.; Merkulov, A.; Clark, S.B.; Tkachev, V.V.; Myasoedov, B.F. (2006) Colloid transport of plutonium in the far-field of the Mayak Production Association, Russia, Science, 314, 638-641. Santschi, P.H.; Roberts, K.; Guo, L. (2002) The organic nature of colloidal actinides transported in surface water environments. Environ. Sci. Technol., 36, 3711-3719. This work was funded by U. S. DOE Office of Biological & Environmental Sciences, Subsurface Biogeochemistry Research Program, and performed under the auspices of the U. S. Department of Energy by Lawrence Livermore National Security, LLC under Contract DE-AC52-07NA27344. LLNL-ABS-570161

OPTIMIZATION OF HETEROGENEOUS UTILIZATION OF THORIUM IN PWRS TO ENHANCE PROLIFERATION RESISTANCE AND REDUCE WASTE.

DOE Office of Scientific and Technical Information (OSTI.GOV)

TODOSOW,M.; KAZIMI,M.

2004-08-01

Issues affecting the implementation, public perception and acceptance of nuclear power include: proliferation, radioactive waste, safety, and economics. The thorium cycle directly addresses the proliferation and waste issues, but optimization studies of core design and fuel management are needed to ensure that it fits within acceptable safety and economic margins. Typical pressurized water reactors, although loaded with uranium fuel, produce 225 to 275 kg of plutonium per gigawatt-year of operation. Although the spent fuel is highly radioactive, it nevertheless offers a potential proliferation pathway because the plutonium is relatively easy to separate, amounts to many critical masses, and does notmore » present any significant intrinsic barrier to weapon assembly. Uranium 233, on the other hand, produced by the irradiation of thorium, although it too can be used in weapons, may be ''denatured'' by the addition of natural, depleted or low enriched uranium. Furthermore, it appears that the chemical behavior of thoria or thoria-urania fuel makes it a more stable medium for the geological disposal of the spent fuel. It is therefore particularly well suited for a once-through fuel cycle. The use of thorium as a fertile material in nuclear fuel has been of interest since the dawn of nuclear power technology due to its abundance and to potential neutronic advantages. Early projects include homogeneous mixtures of thorium and uranium oxides in the BORAX-IV, Indian Point I, and Elk River reactors, as well as heterogeneous mixtures in the Shippingport seed-blanket reactor. However these projects were developed under considerably different circumstances than those which prevail at present. The earlier applications preceded the current proscription, for non-proliferation purposes, of the use of uranium enriched to more than 20 w/o in {sup 235}U, and has in practice generally prohibited the use of uranium highly enriched in {sup 235}U. They were designed when the expected burnup of light water fuel was on the order of 25 MWD/kgU--about half the present day value--and when it was expected that the spent fuel would be recycled to recover its fissile content.« less

Long-range tropospheric transport of uranium and plutonium weapons fallout from Semipalatinsk nuclear test site to Norway.

PubMed

Wendel, Cato Christian; Fifield, L Keith; Oughton, Deborah H; Lind, Ole Christian; Skipperud, Lindis; Bartnicki, Jerzy; Tims, Stephen G; Høibråten, Steinar; Salbu, Brit

2013-09-01

A combination of state-of-the-art isotopic fingerprinting techniques and atmospheric transport modelling using real-time historical meteorological data has been used to demonstrate direct tropospheric transport of radioactive debris from specific nuclear detonations at the Semipalatinsk test site in Kazakhstan to Norway via large areas of Europe. A selection of archived air filters collected at ground level at 9 stations in Norway during the most intensive atmospheric nuclear weapon testing periods (1957-1958 and 1961-1962) has been screened for radioactive particles and analysed with respect to the concentrations and atom ratios of plutonium (Pu) and uranium (U) using accelerator mass spectrometry (AMS). Digital autoradiography screening demonstrated the presence of radioactive particles in the filters. Concentrations of (236)U (0.17-23nBqm(-3)) and (239+240)Pu (1.3-782μBqm(-3)) as well as the atom ratios (240)Pu/(239)Pu (0.0517-0.237) and (236)U/(239)Pu (0.0188-0.7) varied widely indicating several different sources. Filter samples from autumn and winter tended to have lower atom ratios than those sampled in spring and summer, and this likely reflects a tropospheric influence in months with little stratospheric fallout. Very high (236)U, (239+240)Pu and gross beta activity concentrations as well as low (240)Pu/(239)Pu (0.0517-0.077), (241)Pu/(239)Pu (0.00025-0.00062) and (236)U/(239)Pu (0.0188-0.046) atom ratios, characteristic of close-in and tropospheric fallout, were observed in filters collected at all stations in Nov 1962, 7-12days after three low-yield detonations at Semipalatinsk (Kazakhstan). Atmospheric transport modelling (NOAA HYSPLIT_4) using real-time meteorological data confirmed that long range transport of radionuclides, and possibly radioactive particles, from Semipalatinsk to Norway during this period was plausible. The present work shows that direct tropospheric transport of fallout from atmospheric nuclear detonations periodically may have had much larger influence on radionuclide air concentrations and deposition than previously anticipated. Copyright © 2013 Elsevier Ltd. All rights reserved.

Future Remains: Industrial Heritage at the Hanford Plutonium Works

NASA Astrophysics Data System (ADS)

Freer, Brian

This dissertation argues that U.S. environmental and historic preservation regulations, industrial heritage projects, history, and art only provide partial frameworks for successfully transmitting an informed story into the long range future about nuclear technology and its related environmental legacy. This argument is important because plutonium from nuclear weapons production is toxic to humans in very small amounts, threatens environmental health, has a half-life of 24, 110 years and because the industrial heritage project at Hanford is the first time an entire U.S. Department of Energy weapons production site has been designated a U.S. Historic District. This research is situated within anthropological interest in industrial heritage studies, environmental anthropology, applied visual anthropology, as well as wider discourses on nuclear studies. However, none of these disciplines is really designed or intended to be a completely satisfactory frame of reference for addressing this perplexing challenge of documenting and conveying an informed story about nuclear technology and its related environmental legacy into the long range future. Others have thought about this question and have made important contributions toward a potential solution. Examples here include: future generations movements concerning intergenerational equity as evidenced in scholarship, law, and amongst Native American groups; Nez Perce and Confederated Tribes of the Umatilla Indian Reservation responses to the Hanford End State Vision and Hanford's Canyon Disposition Initiative; as well as the findings of organizational scholars on the advantages realized by organizations that have a long term future perspective. While these ideas inform the main line inquiry of this dissertation, the principal approach put forth by the researcher of how to convey an informed story about nuclear technology and waste into the long range future is implementation of the proposed Future Remains clause, as originated by the author, by amendment to two U.S. federal laws: National Historic Preservation Act and Comprehensive Environmental Response, Compensation, and Liability Act. The dissertation provides a case study in public anthropology. The findings of the dissertation include recommendations whereby the Future Remains clause gives historic preservation and cultural resources a leading and ongoing role in facilitating real-time forward looking historical documentation at environmental restoration projects at United States National Priorities List (i.e., "Superfund") sites.

Electrokinetic remediation of plutonium-contaminated nuclear site wastes: results from a pilot-scale on-site trial.

PubMed

Agnew, Kieran; Cundy, Andrew B; Hopkinson, Laurence; Croudace, Ian W; Warwick, Phillip E; Purdie, Philip

2011-02-28

This paper examines the field-scale application of a novel low-energy electrokinetic technique for the remediation of plutonium-contaminated nuclear site soils, using soil wastes from the Atomic Weapons Establishment (AWE) Aldermaston site, Berkshire, UK as a test medium. Soils and sediments with varying composition, contaminated with Pu through historical site operations, were electrokinetically treated at laboratory-scale with and without various soil pre-conditioning agents. Results from these bench-scale trials were used to inform a larger on-site remediation trial, using an adapted containment pack with battery power supply. 2.4 m(3) (ca. 4t onnes) of Pu-contaminated soil was treated for 60 days at a power consumption of 33 kWh/m(3), and then destructively sampled. Radiochemical data indicate mobilisation of Pu in the treated soil, and migration (probably as a negatively charged Pu-citrate complex) towards the anodic compartment of the treatment cell. Soil in the cathodic zone of the treatment unit was remediated to a level below free-release disposal thresholds (1.7 Bq/g, or <0.4 Bq/g above background activities). The data show the potential of this method as a low-cost, on-site tool for remediation of radioactively contaminated soils and wastes which can be operated remotely on working sites, with minimal disruption to site infrastructure or operations. Copyright © 2010 Elsevier B.V. All rights reserved.

Technical solutions to nonproliferation challenges

NASA Astrophysics Data System (ADS)

Satkowiak, Lawrence

2014-05-01

The threat of nuclear terrorism is real and poses a significant challenge to both U.S. and global security. For terrorists, the challenge is not so much the actual design of an improvised nuclear device (IND) but more the acquisition of the special nuclear material (SNM), either highly enriched uranium (HEU) or plutonium, to make the fission weapon. This paper provides two examples of technical solutions that were developed in support of the nonproliferation objective of reducing the opportunity for acquisition of HEU. The first example reviews technologies used to monitor centrifuge enrichment plants to determine if there is any diversion of uranium materials or misuse of facilities to produce undeclared product. The discussion begins with a brief overview of the basics of uranium processing and enrichment. The role of the International Atomic Energy Agency (IAEA), its safeguard objectives and how the technology evolved to meet those objectives will be described. The second example focuses on technologies developed and deployed to monitor the blend down of 500 metric tons of HEU from Russia's dismantled nuclear weapons to reactor fuel or low enriched uranium (LEU) under the U.S.-Russia HEU Purchase Agreement. This reactor fuel was then purchased by U.S. fuel fabricators and provided about half the fuel for the domestic power reactors. The Department of Energy established the HEU Transparency Program to provide confidence that weapons usable HEU was being blended down and thus removed from any potential theft scenario. Two measurement technologies, an enrichment meter and a flow monitor, were combined into an automated blend down monitoring system (BDMS) and were deployed to four sites in Russia to provide 24/7 monitoring of the blend down. Data was downloaded and analyzed periodically by inspectors to provide the assurances required.

Technical solutions to nonproliferation challenges

DOE Office of Scientific and Technical Information (OSTI.GOV)

Satkowiak, Lawrence

2014-05-09

The threat of nuclear terrorism is real and poses a significant challenge to both U.S. and global security. For terrorists, the challenge is not so much the actual design of an improvised nuclear device (IND) but more the acquisition of the special nuclear material (SNM), either highly enriched uranium (HEU) or plutonium, to make the fission weapon. This paper provides two examples of technical solutions that were developed in support of the nonproliferation objective of reducing the opportunity for acquisition of HEU. The first example reviews technologies used to monitor centrifuge enrichment plants to determine if there is any diversionmore » of uranium materials or misuse of facilities to produce undeclared product. The discussion begins with a brief overview of the basics of uranium processing and enrichment. The role of the International Atomic Energy Agency (IAEA), its safeguard objectives and how the technology evolved to meet those objectives will be described. The second example focuses on technologies developed and deployed to monitor the blend down of 500 metric tons of HEU from Russia's dismantled nuclear weapons to reactor fuel or low enriched uranium (LEU) under the U.S.-Russia HEU Purchase Agreement. This reactor fuel was then purchased by U.S. fuel fabricators and provided about half the fuel for the domestic power reactors. The Department of Energy established the HEU Transparency Program to provide confidence that weapons usable HEU was being blended down and thus removed from any potential theft scenario. Two measurement technologies, an enrichment meter and a flow monitor, were combined into an automated blend down monitoring system (BDMS) and were deployed to four sites in Russia to provide 24/7 monitoring of the blend down. Data was downloaded and analyzed periodically by inspectors to provide the assurances required.« less

Moscow meltdown: Can Russia survive

DOE Office of Scientific and Technical Information (OSTI.GOV)

Stern, J.E.

Western intelligence analysts and policy makers should pay closer attention to the centrifugal forces in Russia for two primary reasons: nuclear weapons are located in some of the most volatile regions, and central control of the armed forces is eroding. If Russia were to fragment, thousands of weapons and tons of fissile materials would be dispersed to new states with little safeguards infrastructure and little experience in controlling borders, a situation potentially far more dangerous than the breakup of the Soviet Union. Nuclear research, production, maintenance, and dismantlement facilities, plus uranium enrichment and plutonium separation facilities, could be inherited bymore » new, unstable states. Further devolution of political authority could loosen control over sensitive exports and increase the risk of terrorist acquisition of fissile materials. This article discusses the confusion over the legitimacy of the physical and political boundaries of the Russian Federation; then, the economic incentives for regionalism in Russia; next, the main ethnic groups in Russia and the roots of ethnic nationalism in the Russian Federation. It then discusses political disarray in the center and in the regions, and the lack of unity among order-enforcing entities; focuses in somewhat more detail on the Volga-Ural region, where there is a concentration of nuclear weapons and facilities, and which is especially volatile politically. These factors taken together call into question Russia's viability as a state. In post-communist Russia, chaos has replaced order; license has replaced terror. Order-enforcing entities are eviscerated or in conflict. Neither economic shock therapy nor Group of Seven funds can help with these problems; Russia will not be a state until new unifying institutions are created, whether they are democratic or authoritarian.« less

Self-harm and suicide attempts among high-risk, urban youth in the U.S.: shared and unique risk and protective factors.

PubMed

Swahn, Monica H; Ali, Bina; Bossarte, Robert M; Van Dulmen, Manfred; Crosby, Alex; Jones, Angela C; Schinka, Katherine C

2012-01-01

The extent to which self-harm and suicidal behavior overlap in community samples of vulnerable youth is not well known. Secondary analyses were conducted of the "linkages study" (N = 4,131), a cross-sectional survey of students enrolled in grades 7, 9, 11/12 in a high-risk community in the U.S. in 2004. Analyses were conducted to determine the risk and protective factors (i.e., academic grades, binge drinking, illicit drug use, weapon carrying, child maltreatment, social support, depression, impulsivity, self-efficacy, parental support, and parental monitoring) associated with both self-harm and suicide attempt. Findings show that 7.5% of participants reported both self-harm and suicide attempt, 2.2% of participants reported suicide attempt only, and 12.4% of participants reported self-harm only. Shared risk factors for co-occurring self-harm and suicide attempt include depression, binge drinking, weapon carrying, child maltreatment, and impulsivity. There were also important differences by sex, grade level, and race/ethnicity that should be considered for future research. The findings show that there is significant overlap in the modifiable risk factors associated with self-harm and suicide attempt that can be targeted for future research and prevention strategies.

APPROACHING CRYOGENIC GE PERFORMANCE WITH PELTIER COOLED CDTE

DOE Office of Scientific and Technical Information (OSTI.GOV)

Khusainov, A. K.; Iwanczyk, J. S.; Patt, B. E.

A new class of hand-held, portable spectrometers based on large area (lcm2) CdTe detectors of thickness up to 3mm has been demonstrated to produce energy resolution of between 0.3 and 0.5% FWHM at 662 keV. The system uses a charge loss correction circuit for improved efficiency, and detector temperature stabilization to ensure consistent operation of the detector during field measurements over a wide range of ambient temperature. The system can operate continuously for up to 8hrs on rechargeable batteries. The signal output from the charge loss corrector is compatible with most analog and digital spectroscopy amplifiers and multi channel analyzers.more » Using a detector measuring 11.2 by 9.1 by 2.13 mm3, we have recently been able to obtain the first wide-range plutonium gamma-ray isotopic analysis with other than a cryogenically cooled germanium spectrometer. The CdTe spectrometer is capable of measuring small plutonium reference samples in about one hour, covering the range from low to high burnup. The isotopic analysis software used to obtain these results was FRAM, Version 4 from LANL. The new spectrometer is expected to be useful for low-grade assay, as well as for some in-situ plutonium gamma-ray isotopics in lieu of cryogenically cooled Ge.« less

Preliminary fabrication and characterisation of inert matrix and thoria fuels for plutonium disposition in light water reactors

NASA Astrophysics Data System (ADS)

Vettraino, F.; Magnani, G.; La Torretta, T.; Marmo, E.; Coelli, S.; Luzzi, L.; Ossi, P.; Zappa, G.

1999-08-01

The plutonium disposition is presently acknowledged as a most urgent issue at the world level. Inert matrix and thoria fuel concepts for Pu burning in LWRs show good potential in providing effective and ultimate solutions to this issue. In non-fertile (U-free) inert matrix fuel, plutonium oxide is diluted within inert oxides such as stabilised ZrO 2, Al 2O 3, MgO or MgAl 2O 4. Thoria addition, which helps improve neutronic characteristics of inert fuels, appears as a promising variant of U-free fuel. In the context of an R&D activity aimed at assessing the feasibility of the fuel concept above, simulated fuel pellets have been produced both from dry-powder metallurgy and the sol-gel route. Results show that they can be fabricated by matching basic nuclear grade specifications such as the required geometry, density and microstructure. Some characterisation testing dealing with thermo-physical properties, ion irradiation damage and solubility also have been started. Results from thermo-physical measurements at room temperature have been achieved. A main feature stemming from solubility testing outcomes is a very high chemical stability which should render the fuel strongly diversion resistant and suitable for direct final disposal in deep geological repository (once-through solution).

DETERMINING THE INFECTIOUS DOSE-50 FOR WEAPONS-GRADE ANTHRAX IN RHESUS MONKEYS USING A BIOLOGICALLY-BASED MODEL

EPA Science Inventory

One of the significant discoveries following the bioterrorist episodes beginning in October 2001 was that a modified form of Bacillus anthracis (Ames strain) was the causative agent. Physical alteration of the inoculum had occurred; the electrostatic charge had been removed and t...

Collaborative Russian-US work in nuclear material protection, control and accounting at the Institute of Physics and Power Engineering. 2: Extension to additional facilities

DOE Office of Scientific and Technical Information (OSTI.GOV)

Kuzin, V.V.; Pshakin, G.M.; Belov, A.P.

1996-12-31

During 1995, collaborative Russian-US nuclear material protection, control, and accounting (MPC and A) tasks at the Institute of Physics and Power Engineering (IPPE) in Obninsk, Russia focused on improving the protection of nuclear materials at the BFS Fast Critical Facility. BFS has tens of thousands of fuel disks containing highly enriched uranium and weapons-grade plutonium that are used to simulate the core configurations of experimental reactors in two critical assemblies. Completed tasks culminated in demonstrations of newly implemented equipment (Russian and US) and methods that enhanced the MPC and A at BFS through computerized accounting, nondestructive inventory verification measurements, personnelmore » identification and access control, physical inventory taking, physical protection, and video surveillance. The collaborative work with US Department of Energy national laboratories is now being extended. In 1996 additional tasks to improve MPC and A have been implemented at BFS, the Technological Laboratory for Fuel Fabrication (TLFF) the Central Storage Facility (CSF), and for the entire site. The TLFF reclads BFS uranium metal fuel disks (process operations and transfers of fissile material). The CSF contains many different types of nuclear material. MPC and A at these additional facilities will be integrated with that at BFS as a prototype site-wide approach. Additional site-wide tasks encompass communications and tamper-indicating devices. Finally, new storage alternatives are being implemented that will consolidate the more attractive nuclear materials in a better-protected nuclear island. The work this year represents not just the addition of new facilities and the site-wide approach, but the systematization of the MPC and A elements that are being implemented as a first step and the more comprehensive ones planned.« less

PRELIMINARY DATA CALL REPORT ADVANCED BURNER REACTOR START UP FUEL FABRICATION FACILITY

DOE Office of Scientific and Technical Information (OSTI.GOV)

S. T. Khericha

2007-04-01

The purpose of this report is to provide data for preparation of a NEPA Environmental Impact Statement in support the U. S. Department of Energy (DOE) Global Nuclear Energy Partnership (GNEP). One of the GNEP objectives is to reduce the inventory of long lived actinide from the light water reactor (LWR) spent fuel. The LWR spent fuel contains Plutonium (Pu) -239 and other transuranics (TRU) such as Americium-241. One of the options is to transmute or burn these actinides in fast neutron spectra as well as generate the electricity. A sodium-cooled Advanced Recycling Reactor (ARR) concept has been proposed tomore » achieve this goal. However, fuel with relatively high TRU content has not been used in the fast reactor. To demonstrate the utilization of TRU fuel in a fast reactor, an Advanced Burner Reactor (ABR) prototype of ARR is proposed, which would necessarily be started up using weapons grade (WG) Pu fuel. The WG Pu is distinguished by relatively highest proportions of Pu-239 and lesser amount of other actinides. The WG Pu will be used as the startup fuel along with TRU fuel in lead test assemblies. Because such fuel is not currently being produced in the US, a new facility (or new capability in an existing facility) is being considered for fabrication of WG Pu fuel for the ABR. This report is provided in response to ‘Data Call’ for the construction of startup fuel fabrication facility. It is anticipated that the facility will provide the startup fuel for 10-15 years and will take to 3 to 5 years to construct.« less

A Blueprint for GNEP Advanced Burner Reactor Startup Fuel Fabrication Facility

DOE Office of Scientific and Technical Information (OSTI.GOV)

S. Khericha

2010-12-01

The purpose of this article is to identify the requirements and issues associated with design of GNEP Advanced Burner Reactor Fuel Facility. The report was prepared in support of providing data for preparation of a NEPA Environmental Impact Statement in support the U. S. Department of Energy (DOE) Global Nuclear Energy Partnership (GNEP). One of the GNEP objectives was to reduce the inventory of long lived actinide from the light water reactor (LWR) spent fuel. The LWR spent fuel contains Plutonium (Pu) -239 and other transuranics (TRU) such as Americium-241. One of the options is to transmute or burn thesemore » actinides in fast neutron spectra as well as generate the electricity. A sodium-cooled Advanced Recycling Reactor (ARR) concept was proposed to achieve this goal. However, fuel with relatively high TRU content has not been used in the fast reactor. To demonstrate the utilization of TRU fuel in a fast reactor, an Advanced Burner Reactor (ABR) prototype of ARR was proposed, which would necessarily be started up using weapons grade (WG) Pu fuel. The WG Pu is distinguished by relatively highest proportions of Pu-239 and lesser amount of other actinides. The WG Pu was assumed to be used as the startup fuel along with TRU fuel in lead test assemblies. Because such fuel is not currently being produced in the US, a new facility (or new capability in an existing facility) was being considered for fabrication of WG Pu fuel for the ABR. It was estimated that the facility will provide the startup fuel for 10-15 years and would take 3 to 5 years to construct.« less

Characterization of biocenoses in the storage reservoirs of liquid radioactive wastes of Mayak PA. Initial descriptive report.

PubMed

Pryakhin, E A; Mokrov, Yu G; Tryapitsina, G A; Ivanov, I A; Osipov, D I; Atamanyuk, N I; Deryabina, L V; Shaposhnikova, I A; Shishkina, E A; Obvintseva, N A; Egoreichenkov, E A; Styazhkina, E V; Osipova, O F; Mogilnikova, N I; Andreev, S S; Tarasov, O V; Geras'kin, S A; Trapeznikov, A V; Akleyev, A V

2016-01-01

As a result of operation of the Mayak Production Association (Mayak PA), Chelyabinsk Oblast, Russia, an enterprise for production and separation of weapon-grade plutonium in the Soviet Union, ecosystems of a number of water bodies have been radioactively contaminated. The article presents information about the current state of ecosystems of 6 special industrial storage reservoirs of liquid radioactive waste from Mayak PA: reservoirs R-3, R-4, R-9, R-10, R-11 and R-17. At present the excess of the radionuclide content in the water of the studied reservoirs and comparison reservoirs (Shershnyovskoye and Beloyarskoye reservoirs) is 9 orders of magnitude for (90)Sr and (137)Cs, and 6 orders of magnitude for alpha-emitting radionuclides. According to the level of radioactive contamination, the reservoirs of the Mayak PA could be arranged in the ascending order as follows: R-11, R-10, R-4, R-3, R-17 and R-9. In 2007-2012 research of the status of the biocenoses of these reservoirs in terms of phytoplankton, zooplankton, bacterioplankton, zoobenthos, aquatic plants, ichthyofauna, avifauna parameters was performed. The conducted studies revealed decrease in species diversity in reservoirs with the highest levels of radioactive and chemical contamination. This article is an initial descriptive report on the status of the biocenoses of radioactively contaminated reservoirs of the Mayak PA, and is the first article in a series of publications devoted to the studies of the reaction of biocenoses of the fresh-water reservoirs of the Mayak PA to a combination of natural and man-made factors, including chronic radiation exposure. Copyright © 2015 Elsevier Ltd. All rights reserved.

Was Nazi Germany on the Road to an Atomic Bomb after all?

NASA Astrophysics Data System (ADS)

Lustig, Harry

2006-04-01

The story of Germany's efforts to develop a nuclear weapon during World War II is a much written about and contentious subject. However there has been agreement on one thing: by the end of the War the Germans had not achieved and were nowhere near to building a bomb. The dispute therefore has been about why Germany did not succeed. Now, from Germany, comes a challenge to this truth, in the provocative book Hitlers Bombe by Rainer Karlsch. The bombshell in Hitler's Bombe is the assertion that German scientists developed and tested a primitive fission and fusion nuclear weapon in March 1945. Karlsch bases this claim on testimony of witnesses in 1962, previously secret Russian documents, and the results of soil tests carried out in 2004 and 2005. However the physics is very murky and it seems out of the question that Germany had enough Uranium 235 or produced any Plutonium for a bomb. Hitlers Bombe also makes other, better documented and more credible revisionist assertions. These include the claim that the Nazis did continue to try to build a bomb after 1942 and that not Werner Heisenberg, but Kurt Diebner and Walther Gerlach were then the leaders of the German Uranium project. Karlsch's book therefore deserves more attention from physicists and historians than it has received in the United States.

Historic Manhattan Project Sites at Los Alamos

DOE Office of Scientific and Technical Information (OSTI.GOV)

McGehee, Ellen

The Manhattan Project laboratory constructed at Los Alamos, New Mexico, beginning in 1943, was intended from the start to be temporary and to go up with amazing speed. Because most of those WWII-era facilities were built with minimal materials and so quickly, much of the original infrastructure was torn down in the late '40s and early '50s and replaced by more permanent facilities. However, a few key facilities remained, and are being preserved and maintained for historic significance. Four such sites are visited briefly in this video, taking viewers to V-Site, the buildings where the first nuclear explosive device wasmore » pre-assembled in preparation for the Trinity Test in Southern New Mexico. Included is another WWII area, Gun Site. So named because it was the area where scientists and engineers tested the so-called "gun method" of assembling nuclear materials -- the fundamental design of the Little Boy weapon that was eventually dropped on Hiroshima. The video also goes to Pajarito Site, home of the "Slotin Building" and "Pond Cabin." The Slotin Building is the place where scientist Louis Slotin conducted a criticality experiment that went awry in early 1946, leading to his unfortunate death, and the Pond Cabin served the team of eminent scientist Emilio Segre who did early chemistry work on plutonium that ultimately led to the Fat Man weapon.« less

Historic Manhattan Project Sites at Los Alamos

ScienceCinema

McGehee, Ellen

2018-05-11

The Manhattan Project laboratory constructed at Los Alamos, New Mexico, beginning in 1943, was intended from the start to be temporary and to go up with amazing speed. Because most of those WWII-era facilities were built with minimal materials and so quickly, much of the original infrastructure was torn down in the late '40s and early '50s and replaced by more permanent facilities. However, a few key facilities remained, and are being preserved and maintained for historic significance. Four such sites are visited briefly in this video, taking viewers to V-Site, the buildings where the first nuclear explosive device was pre-assembled in preparation for the Trinity Test in Southern New Mexico. Included is another WWII area, Gun Site. So named because it was the area where scientists and engineers tested the so-called "gun method" of assembling nuclear materials -- the fundamental design of the Little Boy weapon that was eventually dropped on Hiroshima. The video also goes to Pajarito Site, home of the "Slotin Building" and "Pond Cabin." The Slotin Building is the place where scientist Louis Slotin conducted a criticality experiment that went awry in early 1946, leading to his unfortunate death, and the Pond Cabin served the team of eminent scientist Emilio Segre who did early chemistry work on plutonium that ultimately led to the Fat Man weapon.

Radiostrontium accumulation in animal bones: development of a radiochemical method by ultra low-level liquid scintillation counting for its quantification.

PubMed

Iammarino, Marco; Dell'Oro, Daniela; Bortone, Nicola; Mangiacotti, Michele; Chiaravalle, Antonio Eugenio

2018-03-31

Strontium-90 (90Sr) is a fission product, resulting from the use of uranium and plutonium in nuclear reactors and weapons. Consequently, it may be found in the environment as a consequence of nuclear fallouts, nuclear weapon testing, and not correct waste management. When present in the environment, strontium-90 may be taken into animal body by drinking water, eating food, or breathing air. The primary health effects are bone tumors and tumors of the blood-cell forming organs, due to beta particles emitted by both 90Sr and yttrium-90 (90Y). Moreover, another health concern is represented by inhibition of calcification and bone deformities in animals. Actually, radiometric methods for the determination of 90Sr in animal bones are lacking. This article describers a radiochemical method for the determination of 90Sr in animal bones, by ultra low-level liquid scintillation counting. The method precision and trueness have been demonstrated through validation tests (CV% = 12.4%; mean recovery = 98.4%). Detection limit and decision threshold corresponding to 8 and 3 mBecquerel (Bq) kg-1, respectively, represent another strong point of this analytical procedure. This new radiochemical method permits the selective extraction of 90Sr, without interferences, and it is suitable for radiocontamination surveillance programs, and it is also an improvement with respect to food safety controls.

Investigation into the Feasibility of Highly Enriched Uranium Detection by External Neutron Stimulation (Expanded Study)

DTIC Science & Technology

2006-05-01

26 1.10.1 Radiation Isotope Detector Operation ...... 27 1.10.2 HEU Counts in Radioisotope with 1 kg HEU.. 27 1.10.3 Radiation Isotope ...REACTOR GRADE PLUTONIUM ........... 173 10.2 GAMMA EMITTING ISOTOPES IN CARGO MATERIAL ............. 177 10.3 MCNP ANALYSIS OF GAMMA TRANSPORT FROM A...experiment at USNA using a germanium detector .......................... 31 1-13 Counts in the radiation isotope detector versus counting time for 1

DOE Office of Scientific and Technical Information (OSTI.GOV)

NONE

This article is a review of the agreement between the United States and two of the former Soviet republics to buy and convert weapons-grade uranium into reactor fuel. Under this 20 year agreement, the US Enrichment Corporation will buy 500 metric tons for a price of $11.9B. This will convert into 15,260 tons of low-enriched uranium.

Optical and Electronic Transport Properties of Luminescent Semiconductors, Amorphous Materials and Metastable Solids.

DTIC Science & Technology

1979-02-26

Williams, Electronic States of Semiconductors with Graded Periodic Inhomogeneities, Phys. Rev. Eli, 2200 (1975) . 7. P. DiBona and R. Ewing, ESR of...Fellow) - K. Daghir, Ph.D. (1974) (IBM) P. DiBona , M.S. (1967), Ph.D. (1974) (U.S. Navy, Surface Weapons Research Laboratory) D. Hoover (current

Toxicity of inhaled plutonium dioxide in beagle dogs

DOE Office of Scientific and Technical Information (OSTI.GOV)

Muggenburg, M.A.; Guilmette, R.A.; Mewhinney, J.A.

This study was conducted to determine the biological effects of inhaled {sup 238}PuO{sub 2} over the life spans of 144 beagle dogs. The dogs inhaled one of two sizes of monodisperse aerosols of {sup 238}PuO{sub 2} to achieve graded levels of initial lung burden (ILB). The aerosols also contained {sup 169}Yb to provide a {gamma}-ray-emitting label for the {sup 238}Pu inhaled by each dog. Excreta were collected periodically over each dog`s life span to estimate plutonium excretion; at death, the tissues were analyzed radiochemically for plutonium activity. The tissue content and the amount of plutonium excreted were used to estimatemore » the ILB. These data for each dog were used in a dosimetry model to estimate the ILB. These data for each dog were used in a dosimetry model to estimate tissue doses. The lung, skeleton and liver received the highest {alpha}-particle doses, ranging from 0.16-68 Gy for the liver. At death, all dogs were necropsied, and all organs and lesions were sampled and examined by histopathology. Findings of non-neoplastic changes included neutropenia and lymphopenia that developed in a dose-related fashion soon after inhalation exposure. These effects persisted for up to 5 years in some animals, but no other health effects could be related to the blood changes observed. Radiation pneumonitis was observed among the dogs with the highest ILBs. Deaths from radiation pneumonitis occurred from 1.5 to 5.4 years after exposure. Tumors of the lung, skeleton and liver occurred beginning at about 3 years after exposure. These findings in dogs suggest that similar dose-related biological effects could be expected in humans accidentally exposed to {sup 238}PuO{sub 2}. 89 refs., 10 figs., 11 tab.« less

Isotopic signatures: An important tool in today`s world

DOE Office of Scientific and Technical Information (OSTI.GOV)

Rokop, D.J.; Efurd, D.W.; Benjamin, T.M.

1995-12-01

High-sensitivity/high-accuracy actinide measurement techniques developed to support weapons diagnostic capabilities at the Los Alamos National Laboratory are now being used for environmental monitoring. The measurement techniques used are Thermal Ionization Mass Spectrometry (TIMS), Alpha Spectrometry(AS), and High Resolution Gamma Spectrometry(HRGS). These techniques are used to address a wide variety of actinide inventory issues: Environmental surveillance, site characterizations, food chain member determination, sedimentary records of activities, and treaty compliance concerns. As little as 10 femtograms of plutonium can be detected in samples and isotopic signatures determined on samples containing sub-100 femtogram amounts. Uranium, present in all environmental samples, can generally yieldmore » isotopic signatures of anthropogenic origin when present at the 40 picogam/gram level. Solid samples (soils, sediments, fauna, and tissue) can range from a few particles to several kilograms in size. Water samples can range from a few milliliters to as much as 200 liters.« less

Enrico Fermi - And the Revolutions of Modern Physics

NASA Astrophysics Data System (ADS)

Cooper, Dan

1999-02-01

In 1938, at the age of 37, Enrico Fermi was awarded the Nobel Prize in Physics. That same year he emigrated from Italy to the United States and, in the course of his experiments, discovered nuclear fission--a process which forms the basis of nuclear power and atomic bombs. Soon the brilliant physicist was involved in the top secret race to produce the deadliest weapon on Earth. He created the first self-sustaining chain reaction, devised new methods for purifying plutonium, and eventually participated in the first atomic test. This compelling biography traces Fermis education in Italy, his meteoric career in the scientific world, his escape from fascism to America, and the ingenious experiments he devised and conducted at the University of Rome, Columbia University, and the Los Alamos laboratory. The book also presents a mini-course in quantum and nuclear physics in an accessible, fast-paced narrative that invokes all the dizzying passion of Fermis brilliant discoveries.

Presence of plutonium contamination in soils from Palomares (Spain).

PubMed

Jiménez-Ramos, M C; García-Tenorio, R; Vioque, I; Manjón, G; García-León, M

2006-08-01

More than 30 years after the occurrence of an aircraft accident which involved the detonation of two nuclear weapons in the surrounding area of the village of Palomares (Spain), the affected terrestrial area has been investigated for remaining transuranic contamination. Evidence from the presence of this contamination was initially found through the analysis of the 241Am inventories in superficial soil samples collected in the region, and was confirmed through the analysis of the (239+240)Pu inventories and their associated 238Pu/(239+240)Pu activity ratios in the same samples. However, it was also observed that a considerable fraction of the remaining contamination in the area was present in particulate form, i.e. as "hot particles". The work performed in our laboratory for identification, isolation and characterisation of these "hot particles" as well as some conclusions obtained from these analyses are outlined in this paper.

A Report to Congress on Long-Term Stewardship. Volume II, Site Summaries

DOE Office of Scientific and Technical Information (OSTI.GOV)

None, None

2001-01-01

During World War II and the Cold War, the Federal government developed and operated a vast network of industrial facilities for the research, production, and testing of nuclear weapons, as well as for other scientific and engineering research. These processes left a legacy of radioactive and chemical waste, environmental contamination, and hazardous facilities and materials at well over a 100 sites in 30 States and one U.S. Territory. Hundreds of thousand of acres of residually contaminated soils, contaminated groundwater, surface water and sediment contamination, and contaminated buildings are present at many sites across the country. These sites range in sizemore » from less than one acre, containing only a single facility, to large sites spanning over 100,000 acres with huge uranium enrichment plants and plutonium processing canyons. Since 1989, the U.S. Department of Energy’s (DOE) Environmental Management (EM) program has made significant progress in addressing this environmental legacy. Millions of cubic meters of waste have been removed, stabilized, or disposed of, resulting in significant risk and cost reduction. In addition, DOE began disposing of transuranic (i.e., plutonium-contaminated) waste in the nation’s first deep geologic repository – the Waste Isolation Pilot Plant in New Mexico. DOE is now carrying out its long-term stewardship obligations at dozens of sites, including smaller sites where DOE has completed cleanup work for the entire site and many larger sites where DOE has remediated portions of the site.« less

Using the Theory of Planned Behavior to Predict Aggression and Weapons Carrying In Urban African American Early Adolescent Youth

PubMed Central

Finigan-Carr, Nadine M.; Cheng, Tina L.; Gielen, Andrea; Haynie, Denise L.; Simons-Morton, Bruce

2015-01-01

Aggressive and weapons carrying behaviors are indicative of youth violence. The Theory of Planned Behavior (Ajzen, 1991) is used in the current analysis to improve our understanding of violence-related behaviors. We examine the influence of perceived behavioral control (self-control and decision making) as a part of the overall framework for understanding the risk and protective factors for aggressive behaviors and weapons carrying. As the baseline assessment of an intervention trial, survey data were collected on 452 sixth grade students (50% girls; 96.6% African American; mean age 12.0) from urban middle schools. 18.4% carried a weapon in the prior 12 months with boys more likely to carry a weapon than girls (22.5% vs. 14.2%, p=0.02). 78.4% of youth reported aggressive behaviors with no significant differences found between girls (81.3%) and boys (75.5%). In logistic regression models, having peers who engage in problem behaviors was found to be a significant risk factor. Youth with peers who engaged in numerous problem behaviors were 5 times more likely to be aggressive than those who reported little or no peer problem behaviors. Teens who reported that their parents opposed aggression (OR: 0.76; CI: 0.66, 0.88) and who used self-control strategies (OR: 0.59; CI: 0.39, 0.87) were found to report less aggressive behaviors. For weapons carrying, being a girl (OR: 0.56; CI: 0.32, 0.97) and self-control (OR: 0.52; CI: 0.29, 0.92) were protective factors. This study demonstrated that the TPB may provide a useful framework for the development of violence prevention programs. PMID:25228369

Involvement of school students in fights with weapons: prevalence and associated factors in Brazil.

PubMed

Melo, Alice Cristina Medeiros; Garcia, Leila Posenato

2016-09-22

Violence, as well as other behaviors, is often intensified during adolescence and early adulthood. The objective of this study is estimate the prevalence of Brazilian school students involvement in fights with weapons and to analyze the associated factors. This is a cross-sectional study using data from the National School Student Health Survey conducted in 2012 with 9 th grade elementary school students attending 2842 schools in all 27 Brazilian Federative Units. The outcome studied was involvement in fights with firearms and/or cold weapons in the 30 days prior to the interview. Poisson regression was used to estimate the prevalence ratios and 95 % confidence intervals (95 % CI). The analyses were stratified by sex. Fifty seven thousand and eighty nine female students and 52,015 male students were included; the prevalence of their involvement in fights with weapons was 7.2 (95 % CI 6.9-7.5) and 13.8 (95 % CI 13.4-14.3), respectively. In the adjusted analysis the factors associated with male student involvement in fights with weapons were: being older, working, having smoked a cigarette, consumed alcoholic beverages and illicit drugs recently, insomnia, not having any close friends, skipping classes without parental supervision, having suffered aggression from a family member, reporting feeling unsafe on the way to or from school and/or at school. The same associated factors were found among female students in addition to not living with their father and/or mother and having suffered bullying. There was no association with type of school in either sex. Involvement in fights with weapons was greater among older male students. Health-risk behaviors, mental health characteristics, parental supervision and context of violence also showed association with the outcomes.

Studying How Plants Defend Themselves: A Chemical Weapon Produced by Chilli Fruit

ERIC Educational Resources Information Center

Nantawanit, Nantawan; Panijpan, Bhinyo; Ruenwongsa, Pintip

2011-01-01

Students often prefer to study animals rather than plants, because they see plants as passive, less interesting organisms. This paper proposes a simple hands-on laboratory exercise for high-school students (grade 12) to arouse their interest in learning about plants and to demonstrate to them that plants are active organisms capable of defending…

WEAPONS-GRADE ANTHRAX: DETERMINING THE ID-50 (INHALATION) IN RHESUS MONKEYS USING A BIOLOGICALLY-BASED MODEL FOR USE IN HUMAN RISK ASSESSMENT

EPA Science Inventory

One of the significant discoveries following the bioterrorist attacks of October 2001 was that a modified form of Bacillus anthracis (Ames strain) was the causative agent. Physical alteration of the inoculum had occurred; the electrostatic charge had been altered and the resultin...

Laser and gas centrifuge enrichment

NASA Astrophysics Data System (ADS)

Heinonen, Olli

2014-05-01

Principles of uranium isotope enrichment using various laser and gas centrifuge techniques are briefly discussed. Examples on production of high enriched uranium are given. Concerns regarding the possibility of using low end technologies to produce weapons grade uranium are explained. Based on current assessments commercial enrichment services are able to cover the global needs of enriched uranium in the foreseeable future.

Optimizing the Sustainment of U.S. Army Weapon Systems

DTIC Science & Technology

2016-03-17

Current Military Rank/Civilian Grade ................................................................................ 33 Figure 9: Education Level...across the military services from lows experienced in the wake of fiscal year 2013 sequestration when only 2 Army non-missioned brigade combat teams...committee notes that recovery from these ebbs in readiness has taken time, with most military services reporting a return to pre-sequester levels of

The National School Safety Center's Report on School Associated Violent Deaths

ERIC Educational Resources Information Center

National School Safety Center (NJ1), 2010

2010-01-01

A school-associated violent death is any homicide, suicide, or weapons-related violent death in the United States in which the fatal injury occurred: (1) on the property of a functioning public, private or parochial elementary or secondary school, Kindergarten through grade 12, (including alternative schools); (2) on the way to or from regular…

CONVERSION OF PLUTONIUM TRIFLUORIDE TO PLUTONIUM TETRAFLUORIDE

DOEpatents

Fried, S.; Davidson, N.R.

1957-09-10

A large proportion of the trifluoride of plutonium can be converted, in the absence of hydrogen fluoride, to the tetrafiuoride of plutonium. This is done by heating plutonium trifluoride with oxygen at temperatures between 250 and 900 deg C. The trifiuoride of plutonium reacts with oxygen to form plutonium tetrafluoride and plutonium oxide, in a ratio of about 3 to 1. In the presence of moisture, plutonium tetrafluoride tends to hydrolyze at elevated temperatures and therefore it is desirable to have the process take place under anhydrous conditions.

Pyrochemical process for extracting plutonium from an electrolyte salt

DOEpatents

Mullins, L.J.; Christensen, D.C.

1982-09-20

A pyrochemical process for extracting plutonium from a plutonium-bearing salt is disclosed. The process is particularly useful in the recovery of plutonium for electrolyte salts which are left over from the electrorefining of plutonium. In accordance with the process, the plutonium-bearing salt is melted and mixed with metallic calcium. The calcium reduces ionized plutonium in the salt to plutonium metal, and also causes metallic plutonium in the salt, which is typically present as finely dispersed metallic shot, to coalesce. The reduced and coalesced plutonium separates out on the bottom of the reaction vessel as a separate metallic phase which is readily separable from the overlying salt upon cooling of the mixture. Yields of plutonium are typically on the order of 95%. The stripped salt is virtually free of plutonium and may be discarded to low-level waste storage.

Pyrochemical process for extracting plutonium from an electrolyte salt

DOEpatents

Mullins, Lawrence J.; Christensen, Dana C.

1984-01-01

A pyrochemical process for extracting plutonium from a plutonium-bearing salt is disclosed. The process is particularly useful in the recovery of plutonium from electrolyte salts which are left over from the electrorefining of plutonium. In accordance with the process, the plutonium-bearing salt is melted and mixed with metallic calcium. The calcium reduces ionized plutonium in the salt to plutonium metal, and also causes metallic plutonium in the salt, which is typically present as finely dispersed metallic shot, to coalesce. The reduced and coalesced plutonium separates out on the bottom of the reaction vessel as a separate metallic phase which is readily separable from the overlying salt upon cooling of the mixture. Yields of plutonium are typically on the order of 95%. The stripped salt is virtually free of plutonium and may be discarded to low-level waste storage.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Volpe, Tristan A.

Why do states wait for prolonged periods of time with the technical capacity to produce nuclear weapons? Only a handful of countries have ever acquired the sensitive nuclear fuel cycle technology needed to produce fissile material for nuclear weapons. Yet the enduring trend over the last five decades is for these states to delay or forgo exercising the nuclear weapons option provided by uranium enrichment or plutonium reprocessing capabilities. I show that states pause at this threshold stage because they use nuclear technology to bargain for concessions from both allies and adversaries. But when does nuclear latency offer bargaining benefits?more » My central argument is that challengers must surmount a dilemma to make coercive diplomacy work: the more they threaten to proliferate, the harder it becomes to reassure others that compliance will be rewarded with nuclear restraint. I identify a range of mechanisms able to solve this credibility problem, from arms control over breakout capacity to third party mediation and confidence building measures. Since each step towards the bomb raises the costs of implementing these policies, a state hits a sweet spot when it first acquires enrichment and/or reprocessing (ENR) technology. Subsequent increases in proliferation capability generate diminishing returns at the bargaining table for two reasons: the state must go to greater lengths to make a credible nonproliferation promise, and nuclear programs exhibit considerable path dependency as they mature over time. Contrary to the conventional wisdom about power in world politics, less nuclear latency thereby yields more coercive threat advantages. I marshal new primary source evidence from archives and interviews to identify episodes in the historical record when states made clear decisions to use ENR technology as a bargaining chip, and employ this theory of proliferation persuasion to explain how Japan, North Korea, and Iran succeeded and failed to barter concessions from the United States. By clarifying when countries are able to leverage steps towards the bomb for international political gain, my work advances our understanding of proliferation and coercive diplomacy.« less

Challenges associated with the behaviour of radioactive particles in the environment.

PubMed

Salbu, Brit; Kashparov, Valery; Lind, Ole Christian; Garcia-Tenorio, Rafael; Johansen, Mathew P; Child, David P; Roos, Per; Sancho, Carlos

2018-06-01

A series of different nuclear sources associated with the nuclear weapon and fuel cycles have contributed to the release of radioactive particles to the environment. Following nuclear weapon tests, safety tests, conventional destruction of weapons, reactor explosions and fires, a major fraction of released refractory radionuclides such as uranium (U) and plutonium (Pu) were present as entities ranging from sub microns to fragments. Furthermore, radioactive particles and colloids have been released from reprocessing facilities and civil reactors, from radioactive waste dumped at sea, and from NORM sites. Thus, whenever refractory radionuclides are released to the environment following nuclear events, radioactive particles should be expected. Results from many years of research have shown that particle characteristics such as elemental composition depend on the source, while characteristics such as particle size distribution, structure, and oxidation state influencing ecosystem transfer depend also on the release scenarios. When radioactive particles are deposited in the environment, weathering processes occur and associated radionuclides are subsequently mobilized, changing the apparent K d . Thus, particles retained in soils or sediments are unevenly distributed, and dissolution of radionuclides from particles may be partial. For areas affected by particle contamination, the inventories can therefore be underestimated, and impact and risk assessments may suffer from unacceptable large uncertainties if radioactive particles are ignored. To integrate radioactive particles into environmental impact assessments, key challenges include the linking of particle characteristics to specific sources, to ecosystem transfer, and to uptake and retention in biological systems. To elucidate these issues, the EC-funded COMET and RATE projects and the IAEA Coordinated Research Program on particles have revisited selected contaminated sites and archive samples. This COMET position paper summarizes new knowledge on key sources that have contributed to particle releases, including particle characteristics based on advanced techniques, with emphasis on particle weathering processes as well as on heterogeneities in biological samples to evaluate potential uptake and retention of radioactive particles. Copyright © 2017 Elsevier Ltd. All rights reserved.

The Role of Sociability Self-Concept in the Relationship between Exposure to and Concern about Aggression in Middle School

ERIC Educational Resources Information Center

Miller, Janice Williams

2013-01-01

This study examined middle grades students' sociability self-concept and their perceptions about feeling safe at school. Participants' (N = 420) exposure to school aggression and concern about the potential for violence at school were measured across four critical areas: fighting, bullying, stealing, and seeing weapons. Results indicated a limited…

Exposure to Violence and Sexual Risk among Early Adolescents in Urban Middle Schools

ERIC Educational Resources Information Center

Coyle, Karin K.; Guinosso, Stephanie A.; Glassman, Jill R.; Anderson, Pamela M.; Wilson, Helen W.

2017-01-01

This article examines the relationship between exposure to violence, fear of exposure to violence, and sexual risk among a sample of urban middle school youth. The sample included 911 seventh-grade students who completed self-report surveys. Approximately 20% of the sample reported at least one direct threat or injury with a weapon in the past 3…

With Speech as My Weapon: Emma Goldman and the First Amendment. A Unit of Study for Grades 8-12.

ERIC Educational Resources Information Center

Falk, Candace; Cole, Stephen; Thomas, Sally

This supplementary teaching unit provides students with the opportunity to explore freedom of expression by focusing on Emma Goldman (1869-1940), a major figure in the history of American radicalism and feminism. In a period when the expression of controversial ideas was dangerous, Goldman insisted on her right to challenge conventions. She…

The Authoritative Parenting Index: predicting health risk behaviors among children and adolescents.

PubMed

Jackson, C; Henriksen, L; Foshee, V A

1998-06-01

Public health research demonstrates increasing interest in mobilizing parental influence to prevent health risk behaviors among children and adolescents. This research focuses on authoritative parenting, which previous studies suggest can prevent health risk behaviors among youth. To evaluate the reliability and validity of a new survey measure of authoritative parenting, data from studies of (1) substance use in a sample of 1,236 fourth- and sixth-grade students; (2) weapon carrying and interpersonal violence in a sample of 1,490 ninth- and tenth-grade students, and (3) anger, alienation, and conflict resolution in a sample of 224 seventh- and eighth-grade students were analyzed. The Authoritative Parenting Index had a factor structure consistent with a theoretical model of the construct; had acceptable reliability; showed grade, sex, and ethnic differences consistent with other studies; and identified parenting types that varied as hypothesized with multiple indicators of social competence and health risk behaviors among children and adolescents.

Applications of Digitized 3-D Position-Sensitive CdZnTe Spectrometers for National Security and Nuclear Nonproliferation

NASA Astrophysics Data System (ADS)

Streicher, Michael W.

A nuclear weapon detonation remains one of the gravest threats to the global community. Although the likelihood of a nuclear event remains small, the economic and political ramifications of an event are vast. The surest way to reduce the probability of an incident is to account for the special nuclear materials (SNM) which can be used to produce a nuclear weapon. Materials which can be used to manufacture a radiological dispersion device ("dirty bomb") must also be monitored. Rapidly-deployable, commercially-available, room-temperature imaging gamma-ray spectrometers are improving the ability of authorities to intelligently and quickly respond to threats. New electronics which digitally-sample the radiation-induced signals in CdZnTe detectors have expanded the capabilities of these sensors. This thesis explores national security applications where digital readout of CdZnTe detectors significantly enhances capabilities. Radioactive sources can be detected more quickly using digitally-sampled CdZnTe detector due to the improved energy resolution. The excellent energy resolution also improves the accuracy of measurements of uranium enrichment and allows users to measure plutonium grade. Small differences in the recorded gamma-ray energy spectrum can be used to estimate the effective atomic number and mass thickness of materials shielding SNM sources. Improved position resolution of gamma-ray interactions through digital readout allows high resolution gamma-ray images of SNM revealing information about the source configuration. CdZnTe sensors can detect the presence of neutrons, indirectly, through measurement of gamma rays released during capture of thermal neutrons by Cd-113 or inelastic scattering with any constituent nuclei. Fast neutrons, such as those released following fission, can be directly detected through elastic scattering interactions in the detector. Neutrons are a strong indicator of fissile material, and the background neutron rate is much lower than the gamma-ray background rate. Neutrons can more easily penetrate shielding materials as well which can greatly aid in the detection of shielded SNM. Digital CdZnTe readout enables the sensors to maintain excellent energy resolution at high count rates. Pulse pile-up and preamplifier decay can be monitored and corrected for on an event-by-event basis limiting energy resolution degradation in dose rates higher than 100 mR/hr. Finally, new iterations of the digital electronics have enhanced gamma-ray detection capabilities at high photon energies. Currently, gamma rays with energy up to 4.4 MeV have been detected. High-energy photon detection is critical for many proposed active interrogation systems.

PLUTONIUM-CERIUM-COBALT AND PLUTONIUM-CERIUM-NICKEL ALLOYS

DOEpatents

Coffinberry, A.S.

1959-08-25

>New plutonium-base teroary alloys useful as liquid reactor fuels are described. The alloys consist of 10 to 20 atomic percent cobalt with the remainder plutonium and cerium in any desired proportion, with the plutonium not in excess of 88 atomic percent; or, of from 10 to 25 atomic percent nickel (or mixture of nickel and cobalt) with the remainder plutonium and cerium in any desired proportion, with the plutonium not in excess of 86 atomic percent. The stated advantages of these alloys over unalloyed plutonium for reactor fuel use are a lower melting point and a wide range of permissible plutonium dilution.

Possession of weapon and school violence among adolescents and their association with history of traumatic brain injury, substance use and mental health issues.

PubMed

Ilie, Gabriela; Mann, Robert E; Boak, Angela; Hamilton, Hayley A; Rehm, Jürgen; Cusimano, Michael D

2017-02-01

Assessment of the association between illegal possession of weapon and assault on school property among adolescents with and without a history of traumatic brain injury (TBI) while assessing risk factors for these outcomes. Data were derived from the Centre for Addiction and Mental Health's 2013 Ontario Student Drug Use and Health Survey completed by students in grades 7-12 (ages 11-20). In this sample of 5478 adolescents, 6.1% (95% CI: 5.0, 7.4) reported carrying a weapon (e.g., gun or knife) on school property, 10.8% (95% CI: 9.5, 12.3) were engaged in a physical fight and 6.4% (95% CI: 5.4, 7.6) reported having beat up or hurt someone on purpose at school, during last year. Youth who reported carrying a weapon, who were engaged in a physical fight and those who assaulted peers on school property during last year had statistically significantly higher odds of reporting a history of TBIs, being male, in first years of high-school, scored positive for elevated psychological distress, and were current regular alcohol (weapon possession only) and cannabis users. Previously it was thought that alcohol and drugs were the main contributors to school violence. Here we show that history of TBIs is yet another significant predictor of violence at school among adolescents. The results suggest that school vigilance and combined violence and TBI prevention, treatment and rehabilitation programs in this population are warranted. Copyright © 2016 Elsevier Ltd. All rights reserved.

On the future of civilian plutonium: An assessment of technological impediments to nuclear terrorism and proliferation

NASA Astrophysics Data System (ADS)

Avedon, Roger Edmond

This dissertation addresses the value of developing diversion- and theft-resistant nuclear power technology, given uncertain future demand for nuclear power, and uncertain risks of nuclear terrorism and of proliferation from the reprocessing of civilian plutonium. The methodology comprises four elements: Economics. An economic growth model coupled with market penetration effects for plutonium and for the hypothetical new technology provides a range of estimates for future nuclear demand. A flow model accounts for the longevity of capital assets (nuclear plants) over time. Terrorism. The commercial nuclear fuel cycle may provide a source of fissile material for terrorists seeking to construct a crude nuclear device. An option value model is used to estimate the effects of the hypothetical new technology on reducing the probability of theft. A game theoretic model is used to explore the deterrence value of physical security and then to draw conclusions about how learning on the part of terrorists or security forces might affect the theft estimate. The principal uncertainties in the theft model can be updated using Bayesian techniques as new data emerge. Proliferation. Access to fissile material is the principal technical impediment to a state's acquisition of nuclear weapons. A game theoretic model is used to determine the circumstances under which a state may proliferate via diversion. The model shows that the hypothetical new technology will have little value for counter-proliferation if diversion is not a preferred proliferation method. A technology policy analysis of the choice of proliferation method establishes that diversion is unlikely to be used because it has no constituency among the important parties to the decision, namely the political leadership, the scientific establishment, and the military. Value. The decision whether to develop a diversion- and theft-resistant fuel cycle depends on the perceived value of avoiding nuclear terrorism and proliferation. The opportunity cost of such events is prohibitively difficult to assess. Instead, recent nonproliferation efforts and long term funding of organizations with nonproliferation objectives suggest a willingness-to-pay to avoid breaches in nuclear security. The cancellation of the Integral Fast Reactor in 1994 is analyzed using the methodology developed in the dissertation.

Background Radioactivity in River and Reservoir Sediments near Los Alamos, New Mexico

DOE Office of Scientific and Technical Information (OSTI.GOV)

S.G.McLin; D.W. Lyons

2002-05-05

As part of its continuing Environmental Surveillance Program, regional river and lake-bottom sediments have been collected annually by Los Alamos National Laboratory (the Laboratory) since 1974 and 1979, respectively. These background samples are collected from three drainage basins at ten different river stations and five reservoirs located throughout northern New Mexico and southern Colorado. Radiochemical analyses for these sediments include tritium, strontium-90, cesium-137, total uranium, plutonium-238, plutonium-239,-240, americium-241, gross alpha, gross beta, and gross gamma radioactivity. Detection-limit radioactivity originates as worldwide fallout from aboveground nuclear weapons testing and satellite reentry into Earth's atmosphere. Spatial and temporal variations in individual analytemore » levels originate from atmospheric point-source introductions and natural rate differences in airborne deposition and soil erosion. Background radioactivity values on sediments reflect this variability, and grouped river and reservoir sediment samples show a range of statistical distributions that appear to be analyte dependent. Traditionally, both river and reservoir analyte data were blended together to establish background levels. In this report, however, we group background sediment data according to two criteria. These include sediment source (either river or reservoir sediments) and station location relative to the Laboratory (either upstream or downstream). These grouped data are statistically evaluated through 1997, and background radioactivity values are established for individual analytes in upstream river and reservoir sediments. This information may be used to establish the existence and areal extent of trace-level environmental contamination resulting from historical Laboratory research activities since the early 1940s.« less

Les perspectives de l'énergie nucléaire dans le cadre des changements climatiquesThe future of nuclear energy in relation with climate change

NASA Astrophysics Data System (ADS)

Dautray, Robert

2001-12-01

Electronuclear energy associated with hydrogen production can replace fossil fuels while emitting as few greenhouse gases as renewable energies. Besides waste management for which a solution has to be rapidly demonstrated, other key issues are to be examined to complete the demonstration of the viability of electronuclear energy. First, waste management and evolution of plutonium and its daughters must be considered together. A basic study has already been performed but what else to be done is huge and cannot be achieved in France (because of its geological and geographic features, because of the rural distribution of its population, etc.), except if a substantial and quite focused endeavour could bring concerned populations and workers, protection and confidence - which requires from the latter, represented by their elected representatives and thus by a public authority, that they work out "a general protection and confidence criterion for concerned populations and workers". The unique solution in order to protect public health from a potential major danger is to bury as soon as possible all of the ultimate waste products, keeping in mind all of the unfavourable factors such as residual power of these products, their mobility in the confining geological beds and then through aquifers. There are so many categories of waste products whose treatment requires different durations, that storing is necessary in order to make them compatible after sorting by means of chemical separation (called reprocessing). Among all of these potential risks, the present-day most serious one, by far, is that of plutonium and its daughters, which are the most potentially radiotoxic. The unique solution consists in a separation of plutonium (and its daughters), followed by its fissions until a rather complete reduction in a product able to be buried after dilution in a matrix (for example, vitrification). But that solution faces serious handicaps. The examination of waste products and especially of the potentially most dangerous and difficult to treat, that is plutonium (and its daughters), leads thus necessarily to a 'plutonium (and its daughters) plan'. Nuclear safety is a major preoccupation. The French electronuclear stock is a recognized success and when it will be necessary to replace the latter, it will be possible to use the European Pressurized Reactor French-German project; the latter includes protections against very unlikely events and its implementation would be a factor of substantial progress for nuclear safety. Radioprotection, as well as its scientific bases, epidemiology and radiobiology, have funding that is not at the level of the funding devoted to the technical and industrial realizations. As for proliferation, it can be noticed that the countries that have recently at their disposal nuclear weapons have done it independently of their eventual electronuclear stock and furthermore each of the latter used a different scientific and technical process. As for the eventual relations between reprocessing and proliferation, the problem should be solved if the total produced plutonium could be denatured in the reactors of the electronuclear stock. It must be noticed that the major potential danger would rather be the dispersion of radiotoxic products about which the department of ONU in charge of all of these questions is aware of increasing contraband from eastern Europe since some years.

Mineral Deposits and Mineral Potential of the China Lake Complex of the Naval Weapons Center, China Lake, California

DTIC Science & Technology

1983-12-01

Tucker and R. J. Sampson. 16 A field check of the area confirmed many of the physical aspects of the property as reported, but the tungsten grades...iron, mercury, perlite, pumice, aggregate, evaporites, travertine, and diatomite . Geothermal and water-producing strata were also investigated. The...Prospect ( Diatomite ) (N-1602) ..... ... 436 Evaporites .......... ....................... .436 Bonanza Group (N-1502) ..... ............... ... 436

Who Should Control Nuclear Technology? A Curriculum Unit for Contemporary U.S. and World History, Grades 9-12.

ERIC Educational Resources Information Center

Zimney, Michelle; Boston, Jane

Since the end of World War II and the onset of the "new age," nuclear technology has remained high on the world's agenda as questions regarding sovereignty and the balance of power, control of the development and spread of nuclear weapons, non-military uses for nuclear technology, and nuclear safety are debated among and within nations.…

"Our Issues, Our People--Math as Our Weapon": Critical Mathematics in a Chicago Neighborhood High School

ERIC Educational Resources Information Center

Gutstein, Eric

2016-01-01

This article provides an example of, and lessons from, teaching and learning critical mathematics in a Chicago public neighborhood high school with a social justice focus. It is based on a qualitative study of my untracked, 12th-grade mathematics class, a full-year enactment of mathematics for social and racial justice. Students were Black and…

DOE Office of Scientific and Technical Information (OSTI.GOV)

Johnson, Bradley R.

The Hidden Cost of Nuclear Weapons The Cold War arms race drove an intense plutonium production program in the U.S. This campaign produced approximately 100 tons of plutonium over 40 years. The epicenter of plutonium production in the United States was the Hanford site, a 586 square mile reservation owned by the Department of Energy and located on the Colombia River in Southeastern Washington. Plutonium synthesis relied on nuclear reactors to convert uranium to plutonium within the reactor fuel rods. After a sufficient amount of conversion occurred, the rods were removed from the reactor and allowed to cool. They weremore » then dissolved in an acid bath and chemically processed to separate and purify plutonium from the rest of the constituents in the used reactor fuel. The acidic waste was then neutralized using sodium hydroxide and the resulting mixture of liquids and precipitates (small insoluble particles) was stored in huge underground waste tanks. The byproducts of the U.S. plutonium production campaign include over 53 million gallons of high-level radioactive waste stored in 177 large underground tanks at Hanford and another 34 million gallons stored at the Savannah River Site in South Carolina. This legacy nuclear waste represents one of the largest environmental clean-up challenges facing the world today. The nuclear waste in the Hanford tanks is a mixture of liquids and precipitates that have settled into sludge. Some of these tanks are now over 60 years old and a small number of them are leaking radioactive waste into the ground and contaminating the environment. The solution to this nuclear waste challenge is to convert the mixture of solids and liquids into a durable material that won't disperse into the environment and create hazards to the biosphere. What makes this difficult is the fact that the radioactive half-lives of some of the radionuclides in the waste are thousands to millions of years long. (The half-life of a radioactive substance is the amount of time it takes for one-half of the material to undergo radioactive decay.) In general, the ideal material would need to be durable for approximately 10 half-lives to allow the activity to decay to negligible levels. However, the potential health effects of each radionuclide vary depending on what type of radiation is emitted, the energy of that emission, and the susceptibility for the human body to accumulate and concentrate that particular element. Consequently, actual standards tend to be based on limiting the dose (energy deposited per unit mass) that is introduced into the environment. The Environmental Protection Agency (EPA) has the responsibility to establish standards for nuclear waste disposal to protect the health and safety of the public. For example, the Energy Policy Act of 1992 directed the EPA to establish radiation protection standards for the Yucca Mountain geologic repository for nuclear wastes. The standards for Yucca Mountain were promulgated in 2008, and limit the dose to 15 millirem per year for the first 10,000 years, and 100 milirem per year between 10,000 years and 1 million years (40 CFR Part 197; http://www.epa.gov/radiation/yucca/2008factsheet.html). So, the challenge is two-fold: (1) develop a material (a waste form) that is capable of immobilizing the waste over geologic time scales, and (2) develop a process to convert the radioactive sludge in the tanks into this durable waste form material. Glass: Hard, durable, inert, and with infinite chemical versatility Molten glass is a powerful solvent liquid, which can be designed to dissolve almost anything. When solidified, it can be one of the most chemically inert substances known to man. Nature's most famous analogue to glass is obsidian, a vitreous product of volcanic activity; formations over 17 million years old have been found. Archaeologists have found man-made glass specimens that are five thousand years old.« less

Solvent extraction system for plutonium colloids and other oxide nano-particles

DOEpatents

Soderholm, Lynda; Wilson, Richard E; Chiarizia, Renato; Skanthakumar, Suntharalingam

2014-06-03

The invention provides a method for extracting plutonium from spent nuclear fuel, the method comprising supplying plutonium in a first aqueous phase; contacting the plutonium aqueous phase with a mixture of a dielectric and a moiety having a first acidity so as to allow the plutonium to substantially extract into the mixture; and contacting the extracted plutonium with second a aqueous phase, wherein the second aqueous phase has a second acidity higher than the first acidity, so as to allow the extracted plutonium to extract into the second aqueous phase. The invented method facilitates isolation of plutonium polymer without the formation of crud or unwanted emulsions.

SEPARATION OF PLUTONIUM

DOEpatents

Maddock, A.G.; Smith, F.

1959-08-25

A method is described for separating plutonium from uranium and fission products by treating a nitrate solution of fission products, uranium, and hexavalent plutonium with a relatively water-insoluble fluoride to adsorb fission products on the fluoride, treating the residual solution with a reducing agent for plutonium to reduce its valence to four and less, treating the reduced plutonium solution with a relatively insoluble fluoride to adsorb the plutonium on the fluoride, removing the solution, and subsequently treating the fluoride with its adsorbed plutonium with a concentrated aqueous solution of at least one of a group consisting of aluminum nitrate, ferric nitrate, and manganous nitrate to remove the plutonium from the fluoride.

Effect of Americium-241 Content on Plutonium Radiation Source Terms

DOE Office of Scientific and Technical Information (OSTI.GOV)

Rainisch, R.

1998-12-28

The management of excess plutonium by the US Department of Energy includes a number of storage and disposition alternatives. Savannah River Site (SRS) is supporting DOE with plutonium disposition efforts, including the immobilization of certain plutonium materials in a borosilicate glass matrix. Surplus plutonium inventories slated for vitrification include materials with elevated levels of Americium-241. The Am-241 content of plutonium materials generally reflects in-growth of the isotope due to decay of plutonium and is age-dependent. However, select plutonium inventories have Am-241 levels considerably above the age-based levels. Elevated levels of americium significantly impact radiation source terms of plutonium materials andmore » will make handling of the materials more difficult. Plutonium materials are normally handled in shielded glove boxes, and the work entails both extremity and whole body exposures. This paper reports results of an SRS analysis of plutonium materials source terms vs. the Americium-241 content of the materials. Data with respect to dependence and magnitude of source terms on/vs. Am-241 levels are presented and discussed. The investigation encompasses both vitrified and un-vitrified plutonium oxide (PuO2) batches.« less

Integrating the stabilization of nuclear materials

DOE Office of Scientific and Technical Information (OSTI.GOV)

Dalton, H.F.

1996-05-01

In response to Recommendation 94-1 of the Defense Nuclear Facilities Safety Board, the Department of Energy committed to stabilizing specific nuclear materials within 3 and 8 years. These efforts are underway. The Department has already repackaged the plutonium at Rocky Flats and metal turnings at Savannah River that had been in contact with plastic. As this effort proceeds, we begin to look at activities beyond stabilization and prepare for the final disposition of these materials. To describe the plutonium materials being stabilize, Figure 1 illustrates the quantities of plutonium in various forms that will be stabilized. Plutonium as metal comprisesmore » 8.5 metric tons. Plutonium oxide contains 5.5 metric tons of plutonium. Plutonium residues and solutions, together, contain 7 metric tons of plutonium. Figure 2 shows the quantity of plutonium-bearing material in these four categories. In this depiction, 200 metric tons of plutonium residues and 400 metric tons of solutions containing plutonium constitute most of the material in the stabilization program. So, it is not surprising that much of the work in stabilization is directed toward the residues and solutions, even though they contain less of the plutonium.« less

DOE Office of Scientific and Technical Information (OSTI.GOV)

Dunn, Darrell; Poinssot, Christophe; Begg, Bruce

Management of nuclear waste remains an important international topic that includes reprocessing of commercial nuclear fuel, waste-form design and development, storage and disposal packaging, the process of repository site selection, system design, and performance assessment. Requirements to manage and dispose of materials from the production of nuclear weapons, and the renewed interest in nuclear power, in particular through the Generation IV Forum and the Advanced Fuel Cycle Initiative, can be expected to increase the need for scientific advances in waste management. A broad range of scientific and engineering disciplines is necessary to provide safe and effective solutions and address complexmore » issues. This volume offers an interdisciplinary perspective on materials-related issues associated with nuclear waste management programs. Invited and contributed papers cover a wide range of topics including studies on: spent fuel; performance assessment and models; waste forms for low- and intermediate-level waste; ceramic and glass waste forms for plutonium and high-level waste; radionuclides; containers and engineered barriers; disposal environments and site characteristics; and partitioning and transmutation.« less

Potential Signatures of Semi-volatile Compounds Associated With Nuclear Processing

DOE Office of Scientific and Technical Information (OSTI.GOV)

Probasco, Kathleen M.; Birnbaum, Jerome C.; Maughan, A. D.

2002-06-01

Semi-volatile chemicals associated with nuclear processes (e.g., the reprocessing of uranium to produce plutonium for nuclear weapons, or the separation of actinides from processing waste streams), can provide sticky residues or signatures that will attach to piping, ducting, soil, water, or other surface media. Volatile compounds, that are more suitable for electro-optical sensing, have been well studied. However, the semi-volatile compounds have not been well documented or studied. A majority of these semi-volatile chemicals are more robust than typical gaseous or liquid chemicals and can have lifetimes of several weeks, months, or years in the environment. However, large data gapsmore » exist concerning these potential signature compounds and more research is needed to fill these data gaps so that important signature information is not overlooked or discarded. This report investigates key semi-volatile compounds associated with nuclear separations, identifies available chemical and physical properties, and discusses the degradation products that would result from hydrolysis, radiolysis and oxidation reactions on these compounds.« less

Applications of a Fast Neutron Detector System to Verification of Special Nuclear Materials

NASA Astrophysics Data System (ADS)

Mayo, Douglas R.; Byrd, Roger C.; Ensslin, Norbert; Krick, Merlyn S.; Mercer, David J.; Miller, Michael C.; Prettyman, Thomas H.; Russo, Phyllis A.

1998-04-01

An array of boron-loaded plastic optically coupled to bismuth germanate scintillators has been developed to detect neutrons for measurement of special nuclear materials. The phoswiched detection system has the advantage of a high neutron detection efficiency and short die-away time. This is achieved by mixing the moderator (plastic) and the detector (^10B) at the molecular level. Simulations indicate that the neutron capture probabilities equal or exceed those of the current thermal neutron multiplicity techniques which have the moderator (polyethylene) and detectors (^3He gas proportional tubes) macroscopically separate. Experiments have been performed to characterize the response of these detectors and validate computer simulations. The fast neutron detection system may be applied to the quantitative assay of plutonium in high (α,n) backgrounds, with emphasis on safeguards and enviromental scenarios. Additional applications of the insturment, in a non-quantative mode, has been tested for possible verification activities involving dismantlement of nuclear weapons. A description of the detector system, simulations and preliminary data will be presented.

Non-proliferation, safeguards, and security for the fissile materials disposition program immobilization alternatives

DOE Office of Scientific and Technical Information (OSTI.GOV)

Duggan, R.A.; Jaeger, C.D.; Tolk, K.M.

1996-05-01

The Department of Energy is analyzing long-term storage and disposition alternatives for surplus weapons-usable fissile materials. A number of different disposition alternatives are being considered. These include facilities for storage, conversion and stabilization of fissile materials, immobilization in glass or ceramic material, fabrication of fissile material into mixed oxide (MOX) fuel for reactors, use of reactor based technologies to convert material into spent fuel, and disposal of fissile material using geologic alternatives. This paper will focus on how the objectives of reducing security and proliferation risks are being considered, and the possible facility impacts. Some of the areas discussed inmore » this paper include: (1) domestic and international safeguards requirements, (2) non-proliferation criteria and measures, (3) the threats, and (4) potential proliferation, safeguards, and security issues and impacts on the facilities. Issues applicable to all of the possible disposition alternatives will be discussed in this paper. However, particular attention is given to the plutonium immobilization alternatives.« less

A prototype experiment for cooperative monitoring of nuclear reactors with cubic meter scale antineutrino detectors

NASA Astrophysics Data System (ADS)

Bernstein, A.; Allen, M.; Bowden, N.; Brennan, J.; Carr, D. J.; Estrada, J.; Hagmann, C.; Lund, J. C.; Madden, N. W.; Winant, C. D.

2005-09-01

Our Lawrence Livermore National Laboratory/Sandia National Laboratories collaboration has deployed a cubic-meter-scale antineutrino detector to demonstrate non-intrusive and automatic monitoring of the power levels and plutonium content of a nuclear reactor. Reactor monitoring of this kind is required for all non-nuclear weapons states under the Nuclear Nonproliferation Treaty (NPT), and is implemented by the International Atomic Energy Agency (IAEA). Since the antineutrino count rate and energy spectrum depend on the relative yields of fissioning isotopes in the reactor core, changes in isotopic composition can be observed without ever directly accessing the core. Data from a cubic meter scale antineutrino detector, coupled with the well-understood principles that govern the core's evolution in time, can be used to determine whether the reactor is being operated in an illegitimate way. Our group has deployed a detector at the San Onofre reactor site in California to demonstrate this concept. This paper describes the concept and shows preliminary results from 8 months of operation.

Location analysis and strontium-90 concentrations in deer antlers on the Hanford Site

DOE Office of Scientific and Technical Information (OSTI.GOV)

Tiller, B L; Eberhardt, L E; Poston, T M

1995-05-01

The primary objective of this study was to examine the levels of strontium-90 ({sup 90}Sr) in deer antlers collected from near previously active reactor sites and distant from the reactor sites along that portion of the Columbia River which borders the Hanford Site. A second objective was to analyze the movements and home-ranges of mule deer residing within these areas and determine to what extent this information contributes to the observed {sup 90}Sr concentrations. {sup 90}Sr is a long-lived radionuclide (29.1 year half life) produced by fission in irradiated fuel in plutonium production reactors on the Hanford Site. It ismore » also a major component of atmospheric fallout from weapons testing. Concentrations of radionuclides found in the developed environment onsite do not pose a health concern to humans or various wildlife routinely monitored. However, elevated levels of radionuclides in found biota may indicate routes of exposure requiring attention.« less

Using the theory of planned behavior to predict aggression and weapons carrying in urban African American early adolescent youth.

PubMed

Finigan-Carr, Nadine M; Cheng, Tina L; Gielen, Andrea; Haynie, Denise L; Simons-Morton, Bruce

2015-04-01

Aggressive and weapons carrying behaviors are indicative of youth violence. The theory of planned behavior is used in the current analysis to improve our understanding of violence-related behaviors. We examine the influence of perceived behavioral control (self-control and decision making) as a part of the overall framework for understanding the risk and protective factors for aggressive behaviors and weapons carrying. As the baseline assessment of an intervention trial, survey data were collected on 452 sixth-grade students (50% girls; 96.6% African American; mean age 12.0 years) from urban middle schools. A total of 18.4% carried a weapon in the prior 12 months, with boys more likely to carry a weapon than girls (22.5% vs. 14.2%, p = .02). Of the youth, 78.4% reported aggressive behaviors with no significant differences found between girls (81.3%) and boys (75.5%). In logistic regression models, having peers who engage in problem behaviors was found to be a significant risk factor. Youth with peers who engaged in numerous problem behaviors were five times more likely to be aggressive than those who reported little or no peer problem behaviors. Teens who reported that their parents opposed aggression (odds ratio [OR] = 0.76; confidence interval [CI] = 0.66, 0.88) and who used self-control strategies (OR = 0.59; CI = 0.39, 0.87) were found to report less aggressive behaviors. For weapons carrying, being a girl (OR = 0.56; CI = 0.32, 0.97) and self-control (OR = 0.52; CI = 0.29, 0.92) were protective factors. This study demonstrated that the theory of planned behavior may provide a useful framework for the development of violence prevention programs. Practitioners should consider integrating strategies for developing healthy relationships and improving self-control. © 2014 Society for Public Health Education.

Method for dissolving plutonium dioxide

DOEpatents

Tallent, Othar K.

1978-01-01

The fluoride-catalyzed, non-oxidative dissolution of plutonium dioxide in HNO.sub.3 is significantly enhanced in rate by oxidizing dissolved plutonium ions. It is believed that the oxidation of dissolved plutonium releases fluoride ions from a soluble plutonium-fluoride complex for further catalytic action.

METHOD FOR OBTAINING PLUTONIUM METAL AND ALLOYS OF PLUTONIUM FROM PLUTONIUM TRICHLORIDE

DOEpatents

Reavis, J.G.; Leary, J.A.; Maraman, W.J.

1962-11-13

A process is given for both reducing plutonium trichloride to plutonium metal using cerium as the reductant and simultaneously alloying such plutonium metal with an excess of cerium or cerium and cobalt sufficient to yield the desired nuclear reactor fuel composition. The process is conducted at a temperature from about 550 to 775 deg C, at atmospheric pressure, without the use of booster reactants, and a substantial decontamination is effected in the product alloy of any rare earths which may be associated with the source of the plutonium. (AEC)

THE INTEGRATION OF THE 241-Z BUILDING DECONTAMINATION & DECOMMISSIONING (D&D) UNDER COMPREHENSIVE ENVIRONMENTAL RESPONSE COMPENSATION & LIABILITY ACT (CERCLA) WITH RESOURCE CONSERVATION & RECOVERY ACT (RCRA) CLOSURE AT THE PLUTONIUM FINISHING PLANT (PFP)

DOE Office of Scientific and Technical Information (OSTI.GOV)

HOPKINS, A.M.

2007-02-20

The 241-Z treatment and storage tanks, a hazardous waste Treatment, Storage and Disposal (TSD) unit permitted pursuant to the ''Resource Conservation and Recovery Act of 1976'' (RCRA) and Washington State ''Hazardous Waste Management Act, RCW 70.105'', have been deactivated and are being actively decommissioned. The 241-Z TSD unit managed non-listed radioactive contaminated waste water, containing trace RCRA characteristic constituents. The 241-Z TSD unit consists of below grade tanks (D-4, D-5, D-7, D-8, and an overflow tank) located in a concrete containment vault, sample glovebox GB-2-241-ZA, and associated ancillary piping and equipment. The tank system is located beneath the 241-Z building.more » The 241-Z building is not a portion of the TSD unit. The sample glovebox is housed in the above-grade building. Waste managed at the TSD unit was received via underground mining from Plutonium Finishing Plant (PFP) sources. Tank D-6, located in the D-6 vault cell, is a past-practice tank that was taken out of service in 1972 and has never operated as a portion of the RCRA TSD unit. CERCLA actions address Tank D-6, its containment vault cell, and soil beneath the cell that was potentially contaminated during past-practice operations and any other potential past-practice contamination identified during 241-Z closure, while outside the scope of the ''Hanford Facility Dangerous Waste Closure Plant, 241-Z Treatment and Storage Tanks''.« less

Identifying children at risk for being bullies in the United States.

PubMed

Shetgiri, Rashmi; Lin, Hua; Flores, Glenn

2012-01-01

To identify risk factors associated with the greatest and lowest prevalence of bullying perpetration among U.S. children. Using the 2001-2002 Health Behavior in School-Aged Children, a nationally representative survey of U.S. children in 6th-10th grades, bivariate analyses were conducted to identify factors associated with any (once or twice or more), moderate (two to three times/month or more), and frequent (weekly or more) bullying. Stepwise multivariable analyses identified risk factors associated with bullying. Recursive partitioning analysis (RPA) identified risk factors which, in combination, identify students with the highest and lowest bullying prevalence. The prevalence of any bullying in the 13,710 students was 37.3%, moderate bullying was 12.6%, and frequent bullying was 6.6%. Characteristics associated with bullying were similar in the multivariable analyses and RPA clusters. In RPA, the highest prevalence of any bullying (67%) accrued in children with a combination of fighting and weapon-carrying. Students who carry weapons, smoke, and drink alcohol more than 5 to 6 days/week were at greatest risk for moderate bullying (61%). Those who carry weapons, smoke, have more than one alcoholic drink per day, have above-average academic performance, moderate/high family affluence, and feel irritable or bad-tempered daily were at greatest risk for frequent bullying (68%). Risk clusters for any, moderate, and frequent bullying differ. Children who fight and carry weapons are at greatest risk of any bullying. Weapon-carrying, smoking, and alcohol use are included in the greatest risk clusters for moderate and frequent bullying. Risk-group categories may be useful to providers in identifying children at the greatest risk for bullying and in targeting interventions. Copyright © 2012 Academic Pediatric Association. Published by Elsevier Inc. All rights reserved.

Identifying Children At Risk for Being Bullies in the US

PubMed Central

Shetgiri, Rashmi; Lin, Hua; Flores, Glenn

2012-01-01

Objective To identify risk factors associated with the highest and lowest prevalence of bullying perpetration among US children. Methods Using the 2001–2002 Health Behavior in School-Aged Children, a nationally-representative survey of US children in 6th–10th grades, bivariate analyses were conducted to identify factors associated with any (≥ once or twice), moderate (≥ two-three times/month), and frequent (≥ weekly) bullying. Stepwise multivariable analyses identified risk factors associated with bullying. Recursive partitioning analysis (RPA) identified risk factors which, in combination, identify students with the highest and lowest bullying prevalence. Results The prevalence of any bullying in the 13,710 students was 37.3%, moderate bullying was 12.6%, and frequent bullying was 6.6%. Characteristics associated with bullying were similar in the multivariable analyses and RPA clusters. In RPA, the highest prevalence of any bullying (67%) accrued in children with a combination of fighting and weapon-carrying. Students who carry weapons, smoke, and drink alcohol more than 5–6 days weekly were at highest risk for moderate bullying (61%). Those who carry weapons, smoke, drink > once daily, have above-average academic performance, moderate/high family affluence, and feel irritable or bad-tempered daily were at highest risk for frequent bullying (68%). Conclusions Risk clusters for any, moderate, and frequent bullying differ. Children who fight and carry weapons are at highest risk of any bullying. Weapon-carrying, smoking, and alcohol use are included in the highest risk clusters for moderate and frequent bullying. Risk-group categories may be useful to providers in identifying children at highest risks for bullying and in targeting interventions. PMID:22989731

METHOD OF SEPARATING PLUTONIUM

DOEpatents

Brown, H.S.; Hill, O.F.

1958-02-01

Plutonium hexafluoride is a satisfactory fluorinating agent and may be reacted with various materials capable of forming fluorides, such as copper, iron, zinc, etc., with consequent formation of the metal fluoride and reduction of the plutonium to the form of a lower fluoride. In accordance with the present invention, it has been found that the reactivity of plutonium hexafluoride with other fluoridizable materials is so great that the process may be used as a method of separating plutonium from mixures containing plutonium hexafluoride and other vaporized fluorides even though the plutonium is present in but minute quantities. This process may be carried out by treating a mixture of fluoride vapors comprising plutonium hexafluoride and fluoride of uranium to selectively reduce the plutonium hexafluoride and convert it to a less volatile fluoride, and then recovering said less volatile fluoride from the vapor by condensation.

ADSORPTION-BISMUTH PHOSPHATE METHOD FOR SEPARATING PLUTONIUM

DOEpatents

Russell, E.R.; Adamson, A.W.; Boyd, G.E.

1960-06-28

A process is given for separating plutonium from uranium and fission products. Plutonium and uranium are adsorbed by a cation exchange resin, plutonium is eluted from the adsorbent, and then, after oxidation to the hexavalent state, the plutonium is contacted with a bismuth phosphate carrier precipitate.

PLUTONIUM-HYDROGEN REACTION PRODUCT, METHOD OF PREPARING SAME AND PLUTONIUM POWDER THEREFROM

DOEpatents

Fried, S.; Baumbach, H.L.

1959-12-01

A process is described for forming plutonlum hydride powder by reacting hydrogen with massive plutonium metal at room temperature and the product obtained. The plutonium hydride powder can be converted to plutonium powder by heating to above 200 deg C.

Chemical Disposition of Plutonium in Hanford Site Tank Wastes

DOE Office of Scientific and Technical Information (OSTI.GOV)

Delegard, Calvin H.; Jones, Susan A.

2015-05-07

This report examines the chemical disposition of plutonium (Pu) in Hanford Site tank wastes, by itself and in its observed and potential interactions with the neutron absorbers aluminum (Al), cadmium (Cd), chromium (Cr), iron (Fe), manganese (Mn), nickel (Ni), and sodium (Na). Consideration also is given to the interactions of plutonium with uranium (U). No consideration of the disposition of uranium itself as an element with fissile isotopes is considered except tangentially with respect to its interaction as an absorber for plutonium. The report begins with a brief review of Hanford Site plutonium processes, examining the various means used tomore » recover plutonium from irradiated fuel and from scrap, and also examines the intermediate processing of plutonium to prepare useful chemical forms. The paper provides an overview of Hanford tank defined-waste–type compositions and some calculations of the ratios of plutonium to absorber elements in these waste types and in individual waste analyses. These assessments are based on Hanford tank waste inventory data derived from separately published, expert assessments of tank disposal records, process flowsheets, and chemical/radiochemical analyses. This work also investigates the distribution and expected speciation of plutonium in tank waste solution and solid phases. For the solid phases, both pure plutonium compounds and plutonium interactions with absorber elements are considered. These assessments of plutonium chemistry are based largely on analyses of idealized or simulated tank waste or strongly alkaline systems. The very limited information available on plutonium behavior, disposition, and speciation in genuine tank waste also is discussed. The assessments show that plutonium coprecipitates strongly with chromium, iron, manganese and uranium absorbers. Plutonium’s chemical interactions with aluminum, nickel, and sodium are minimal to non-existent. Credit for neutronic interaction of plutonium with these absorbers occurs only if they are physically proximal in solution or the plutonium present in the solid phase is intimately mixed with compounds or solutions of these absorbers. No information on the potential chemical interaction of plutonium with cadmium was found in the technical literature. Definitive evidence of sorption or adsorption of plutonium onto various solid phases from strongly alkaline media is less clear-cut, perhaps owing to fewer studies and to some well-attributed tests run under conditions exceeding the very low solubility of plutonium. The several studies that are well-founded show that only about half of the plutonium is adsorbed from waste solutions onto sludge solid phases. The organic complexants found in many Hanford tank waste solutions seem to decrease plutonium uptake onto solids. A number of studies show plutonium sorbs effectively onto sodium titanate. Finally, this report presents findings describing the behavior of plutonium vis-à-vis other elements during sludge dissolution in nitric acid based on Hanford tank waste experience gained by lab-scale tests, chemical and radiochemical sample characterization, and full-scale processing in preparation for strontium-90 recovery from PUREX sludges.« less

Plutonium-related work and cause-specific mortality at the United States Department of Energy Hanford Site.

PubMed

Wing, Steve; Richardson, David; Wolf, Susanne; Mihlan, Gary

2004-02-01

Health effects of working with plutonium remain unclear. Plutonium workers at the United States Department of Energy (US-DOE) Hanford Site in Washington State, USA were evaluated for increased risks of cancer and non-cancer mortality. Periods of employment in jobs with routine or non-routine potential for plutonium exposure were identified for 26,389 workers hired between 1944 and 1978. Life table regression was used to examine associations of length of employment in plutonium jobs with confirmed plutonium deposition and with cause specific mortality through 1994. Incidence of confirmed internal plutonium deposition in all plutonium workers was 15.4 times greater than in other Hanford jobs. Plutonium workers had low death rates compared to other workers, particularly for cancer causes. Mortality for several causes was positively associated with length of employment in routine plutonium jobs, especially for employment at older ages. At ages 50 and above, death rates for non-external causes of death, all cancers, cancers of tissues where plutonium deposits, and lung cancer, increased 2.0 +/- 1.1%, 2.6 +/- 2.0%, 4.9 +/- 3.3%, and 7.1 +/- 3.4% (+/-SE) per year of employment in routine plutonium jobs, respectively. Workers employed in jobs with routine potential for plutonium exposure have low mortality rates compared to other Hanford workers even with adjustment for demographic, socioeconomic, and employment factors. This may be due, in part, to medical screening. Associations between duration of employment in jobs with routine potential for plutonium exposure and mortality may indicate occupational exposure effects. Copyright 2004 Wiley-Liss, Inc.

Isotopic Details of the Spent Catawba-1 MOX Fuel Rods at ORNL

DOE Office of Scientific and Technical Information (OSTI.GOV)

Ellis, Ronald James

The United States Department of Energy funded Shaw/AREVA MOX Services LLC to fabricate four MOX Lead Test Assemblies (LTA) from weapons-grade plutonium. A total of four MOX LTAs (including MX03) were irradiated in the Catawba Nuclear Station (Unit 1) Catawba-1 PWR which operated at a total thermal power of 3411 MWt and had a core with 193 total fuel assemblies. The MOX LTAs were irradiated along with Duke Energy s irradiation of eight Westinghouse Next Generation Fuel (NGF) LEU LTAs (ref.1) and the remaining 181 LEU fuel assemblies. The MX03 LTA was irradiated in the Catawba-1 PWR core (refs.2,3) duringmore » cycles C-16 and C-17. C-16 began on June 5, 2005, and ended on November 11, 2006, after 499 effective full power days (EFPDs). C-17 started on December 29, 2006, (after a shutdown of 48 days) and continued for 485 EFPDs. The MX03 and three other MOX LTAs (and other fuel assemblies) were discharged at the end of C-17 on May 3, 2008. The design of the MOX LTAs was based on the (Framatome ANP, Inc.) Mark-BW/MOX1 17 17 fuel assembly design (refs. 4,5,6) for use in Westinghouse PWRs, but with MOX fuel rods with three Pu loading ranges: the nominal Pu loadings are 4.94 wt%, 3.30 wt%, and 2.40 wt%, respectively, for high, medium, and low Pu content. The Mark-BW/MOX1 (MOX LTA) fuel assembly design is the same as the Advanced Mark-BW fuel assembly design but with the LEU fuel rods replaced by MOX fuel rods (ref. 5). The fabrication of the fuel pellets and fuel rods for the MOX LTAs was performed at the Cadarache facility in France, with the fabrication of the LTAs performed at the MELOX facility, also in France.« less

Delayed Gamma-ray Spectroscopy for Safeguards Applications

DOE Office of Scientific and Technical Information (OSTI.GOV)

Mozin, Vladimir

The delayed gamma-ray assay technique utilizes an external neutron source (D-D, D-T, or electron accelerator-driven), and high-resolution gamma-ray spectrometers to perform characterization of SNM materials behind shielding and in complex configurations such as a nuclear fuel assembly. High-energy delayed gamma-rays (2.5 MeV and above) observed following the active interrogation, provide a signature for identification of specific fissionable isotopes in a mixed sample, and determine their relative content. Potential safeguards applications of this method are: 1) characterization of fresh and spent nuclear fuel assemblies in wet or dry storage; 2) analysis of uranium enrichment in shielded or non-characterized containers or inmore » the presence of a strong radioactive background and plutonium contamination; 3) characterization of bulk and waste and product streams at SNM processing plants. Extended applications can include warhead confirmation and warhead dismantlement confirmation in the arms control area, as well as SNM diagnostics for the emergency response needs. In FY16 and prior years, the project has demonstrated the delayed gamma-ray measurement technique as a robust SNM assay concept. A series of empirical and modeling studies were conducted to characterize its response sensitivity, develop analysis methodologies, and analyze applications. Extensive experimental tests involving weapons-grade Pu, HEU and depleted uranium samples were completed at the Idaho Accelerator Center and LLNL Dome facilities for various interrogation time regimes and effects of the neutron source parameters. A dedicated delayed gamma-ray response modeling technique was developed and its elements were benchmarked in representative experimental studies, including highresolution gamma-ray measurements of spent fuel at the CLAB facility in Sweden. The objective of the R&D effort in FY17 is to experimentally demonstrate the feasibility of the delayed gamma-ray interrogation of shielded SNM samples with portable neutron sources suitable for field applications.« less

PRODUCTION OF PLUTONIUM METAL

DOEpatents

Lyon, W.L.; Moore, R.H.

1961-01-17

A process is given for producing plutonium metal by the reduction of plutonium chloride, dissolved in alkali metal chloride plus or minus aluminum chloride, with magnesium or a magnesium-aluminum alloy at between 700 and 800 deg C and separating the plutonium or plutonium-aluminum alloy formed from the salt.

Program manager: The Journal of the Defense Systems Management College. Volume 14, Number 2, March-April 1985,

DTIC Science & Technology

1985-04-01

author and ProgramRationale, approach and results of Manager, and forward two copies of the reprinted - 10 to reduce spiraling weapon material to the...Technologies ADVAL STRUCTURAL 5 DESIGN/ MATERIALS P’rogram Nlam.4er 4 .’ . I...reading grade sciecnce and mathematics achieved on vanced technological societies, yet it is els It iwver tor somei rninorit\\’ groups,. national tests

PROCESS OF FORMING PLUOTONIUM SALTS FROM PLUTONIUM EXALATES

DOEpatents

Garner, C.S.

1959-02-24

A process is presented for converting plutonium oxalate to other plutonium compounds by a dry conversion method. According to the process, lower valence plutonium oxalate is heated in the presence of a vapor of a volatile non- oxygenated monobasic acid, such as HCl or HF. For example, in order to produce plutonium chloride, the pure plutonium oxalate is heated to about 700 deg C in a slow stream of hydrogen plus HCl. By the proper selection of an oxidizing or reducing atmosphere, the plutonium halide product can be obtained in either the plus 3 or plus 4 valence state.

EXAFS/XANES studies of plutonium-loaded sodalite/glass waste forms

NASA Astrophysics Data System (ADS)

Richmann, Michael K.; Reed, Donald T.; Kropf, A. Jeremy; Aase, Scott B.; Lewis, Michele A.

2001-09-01

A sodalite/glass ceramic waste form is being developed to immobilize highly radioactive nuclear wastes in chloride form, as part of an electrochemical cleanup process. Two types of simulated waste forms were studied: where the plutonium was alone in an LiCl/KCl matrix and where simulated fission-product elements were added representative of the electrometallurgical treatment process used to recover uranium from spent nuclear fuel also containing plutonium and a variety of fission products. Extended X-ray absorption fine structure spectroscopy (EXAFS) and X-ray absorption near-edge spectroscopy (XANES) studies were performed to determine the location, oxidation state, and particle size of the plutonium within these waste form samples. Plutonium was found to segregate as plutonium(IV) oxide with a crystallite size of at least 4.8 nm in the non-fission-element case and 1.3 nm with fission elements present. No plutonium was observed within the sodalite in the waste form made from the plutonium-loaded LiCl/KCl eutectic salt. Up to 35% of the plutonium in the waste form made from the plutonium-loaded simulated fission-product salt may be segregated with a heavy-element nearest neighbor other than plutonium or occluded internally within the sodalite lattice.

DOE Office of Scientific and Technical Information (OSTI.GOV)

Chrzanowski, P; Walter, K

For the Laboratory and staff, 2006 was a year of outstanding achievements. As our many accomplishments in this annual report illustrate, the Laboratory's focus on important problems that affect our nation's security and our researchers breakthroughs in science and technology have led to major successes. As a national laboratory that is part of the Department of Energy's National Nuclear Security Administration (DOE/NNSA), Livermore is a key contributor to the Stockpile Stewardship Program for maintaining the safety, security, and reliability of the nation's nuclear weapons stockpile. The program has been highly successful, and our annual report features some of the Laboratory'smore » significant stockpile stewardship accomplishments in 2006. A notable example is a long-term study with Los Alamos National Laboratory, which found that weapon pit performance will not sharply degrade from the aging effects on plutonium. The conclusion was based on a wide range of nonnuclear experiments, detailed simulations, theoretical advances, and thorough analyses of the results of past nuclear tests. The study was a superb scientific effort. The continuing success of stockpile stewardship enabled NNSA in 2006 to lay out Complex 2030, a vision for a transformed nuclear weapons complex that is more responsive, cost efficient, and highly secure. One of the ways our Laboratory will help lead this transformation is through the design and development of reliable replacement warheads (RRWs). Compared to current designs, these warheads would have enhanced performance margins and security features and would be less costly to manufacture and maintain in a smaller, modernized production complex. In early 2007, NNSA selected Lawrence Livermore and Sandia National Laboratories-California to develop ''RRW-1'' for the U.S. Navy. Design efforts for the RRW, the plutonium aging work, and many other stockpile stewardship accomplishments rely on computer simulations performed on NNSA's Advanced Simulation and Computing (ASC) Program supercomputers at Livermore. ASC Purple and BlueGene/L, the world's fastest computer, together provide nearly a half petaflop (500 trillion operations per second) of computer power for use by the three NNSA national laboratories. Livermore-led teams were awarded the Gordon Bell Prize for Peak Performance in both 2005 and 2006. The winning simulations, run on BlueGene/L, investigated the properties of materials at the length and time scales of atomic interactions. The computing power that makes possible such detailed simulations provides unprecedented opportunities for scientific discovery. Laboratory scientists are meeting the extraordinary challenge of creating experimental capabilities to match the resolution of supercomputer simulations. Working with a wide range of collaborators, we are developing experimental tools that gather better data at the nanometer and subnanosecond scales. Applications range from imaging biomolecules to studying matter at extreme conditions of pressure and temperature. The premier high-energy-density experimental physics facility in the world will be the National Ignition Facility (NIF) when construction is completed in 2009. We are leading the national effort to perform the first fusion ignition experiments using NIF's 192-beam laser and prepare to explore some of the remaining important issues in weapons physics. With scientific colleagues from throughout the nation, we are also designing revolutionary experiments on NIF to advance the fields of astrophysics, planetary physics, and materials science. Mission-directed, multidisciplinary science and technology at Livermore is also focused on reducing the threat posed by the proliferation of weapons of mass destruction as well as their acquisition and use by terrorists. The Laboratory helps this important national effort by providing its unique expertise, integration analyses, and operational support to the Department of Homeland Security. For this vital facet of the Laboratory's national security mission, we are developing advanced technologies, such as a pocket-size explosives detector and an airborne persistent surveillance system, both of which earned R&D 100 Awards. Altogether, Livermore won seven R&D 100 Awards in 2006, the most for any organization. Emerging threats to national and global security go beyond defense and homeland security. Livermore pursues major scientific and technical advances to meet the need for a clean environment; clean, abundant energy; better water management; and improved human health. Our annual report highlights the link between human activities and the warming of tropical oceans, as well as techniques for imaging biological molecules and detecting bone cancer in its earliest stages. In addition, we showcase many scientific discoveries: distant planets, the composition of comets, a new superheavy element.« less

STRIPPING PROCESS FOR PLUTONIUM

DOEpatents

Kolodney, M.

1959-10-01

A method for removing silver, nickel, cadmium, zinc, and indium coatings from plutonium objects while simultaneously rendering the plutonium object passive is described. The coated plutonium object is immersed as the anode in an electrolyte in which the plutonium is passive and the coating metal is not passive, using as a cathode a metal which does not dissolve rapidly in the electrolyte. and passing an electrical current through the electrolyte until the coating metal is removed from the plutonium body.

PLUTONIUM-CUPFERRON COMPLEX AND METHOD OF REMOVING PLUTONIUM FROM SOLUTION

DOEpatents

Potratz, H.A.

1959-01-13

A method is presented for separating plutonium from fission products present in solutions of neutronirradiated uranium. The process consists in treating such acidic solutions with cupferron so that the cupferron reacts with the plutonium present to form an insoluble complex. This plutonium cupferride precipitates and may then be separated from the solution.

Lithium metal reduction of plutonium oxide to produce plutonium metal

DOEpatents

Coops, Melvin S.

1992-01-01

A method is described for the chemical reduction of plutonium oxides to plutonium metal by the use of pure lithium metal. Lithium metal is used to reduce plutonium oxide to alpha plutonium metal (alpha-Pu). The lithium oxide by-product is reclaimed by sublimation and converted to the chloride salt, and after electrolysis, is removed as lithium metal. Zinc may be used as a solvent metal to improve thermodynamics of the reduction reaction at lower temperatures. Lithium metal reduction enables plutonium oxide reduction without the production of huge quantities of CaO--CaCl.sub.2 residues normally produced in conventional direct oxide reduction processes.